Articles | Volume 23, issue 1
https://doi.org/10.5194/acp-23-663-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-663-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 Jan 2023
Research article |
| 16 Jan 2023
| 16 Jan 2023
Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
Sibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USA
Ewa M. Bednarz
Sibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USA
Walker R. Lee
Sibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USA
Ben Kravitz
Department of Earth and Atmospheric Science, Indiana University, Bloomington, IN, USA
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Andy Jones
Met Office Hadley Centre, Exeter, UK
Jim M. Haywood
Met Office Hadley Centre, Exeter, UK
College of Engineering, Mathematics and Physical Sciences, University of Exeter, Exeter, UK
Douglas G. MacMartin
Sibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USA
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Earth Syst. Dynam., 16, 1325–1341, https://doi.org/10.5194/esd-16-1325-2025, https://doi.org/10.5194/esd-16-1325-2025, 2025
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Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer
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Martin Juckes, Karl E. Taylor, Fabrizio Antonio, David Brayshaw, Carlo Buontempo, Jian Cao, Paul J. Durack, Michio Kawamiya, Hyungjun Kim, Tomas Lovato, Chloe Mackallah, Matthew Mizielinski, Alessandra Nuzzo, Martina Stockhause, Daniele Visioni, Jeremy Walton, Briony Turner, Eleanor O'Rourke, and Beth Dingley
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Christina V. Brodowsky, Timofei Sukhodolov, Gabriel Chiodo, Valentina Aquila, Slimane Bekki, Sandip S. Dhomse, Michael Höpfner, Anton Laakso, Graham W. Mann, Ulrike Niemeier, Giovanni Pitari, Ilaria Quaglia, Eugene Rozanov, Anja Schmidt, Takashi Sekiya, Simone Tilmes, Claudia Timmreck, Sandro Vattioni, Daniele Visioni, Pengfei Yu, Yunqian Zhu, and Thomas Peter
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Anton Laakso, Daniele Visioni, Ulrike Niemeier, Simone Tilmes, and Harri Kokkola
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This study is the second in a two-part series in which we explore the dependency of the impacts of stratospheric sulfur injections on both the model employed and the strategy of injection utilized. The study uncovers uncertainties associated with these techniques to cool climate, highlighting how the simulated climate impacts are dependent on both the selected model and the magnitude of the injections. We also show that estimating precipitation impacts of aerosol injection is a complex task.
Daniele Visioni, Alan Robock, Jim Haywood, Matthew Henry, Simone Tilmes, Douglas G. MacMartin, Ben Kravitz, Sarah J. Doherty, John Moore, Chris Lennard, Shingo Watanabe, Helene Muri, Ulrike Niemeier, Olivier Boucher, Abu Syed, Temitope S. Egbebiyi, Roland Séférian, and Ilaria Quaglia
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Yan Zhang, Douglas G. MacMartin, Daniele Visioni, Ewa M. Bednarz, and Ben Kravitz
Earth Syst. Dynam., 15, 191–213, https://doi.org/10.5194/esd-15-191-2024, https://doi.org/10.5194/esd-15-191-2024, 2024
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Injecting SO2 into the lower stratosphere can temporarily reduce global mean temperature and mitigate some risks associated with climate change, but injecting it at different latitudes and seasons would have different impacts. This study introduces new stratospheric aerosol injection (SAI) strategies and explores the importance of the choice of SAI strategy, demonstrating that it notably affects the distribution of aerosol cloud, injection efficiency, and various surface climate impacts.
Ewa M. Bednarz, Amy H. Butler, Daniele Visioni, Yan Zhang, Ben Kravitz, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 13665–13684, https://doi.org/10.5194/acp-23-13665-2023, https://doi.org/10.5194/acp-23-13665-2023, 2023
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We use a state-of-the-art Earth system model and a set of stratospheric aerosol injection (SAI) strategies to achieve the same level of global mean surface cooling through different combinations of location and/or timing of the injection. We demonstrate that the choice of SAI strategy can lead to contrasting impacts on stratospheric and tropospheric temperatures, circulation, and chemistry (including stratospheric ozone), thereby leading to different impacts on regional surface climate.
Matthew Henry, Jim Haywood, Andy Jones, Mohit Dalvi, Alice Wells, Daniele Visioni, Ewa M. Bednarz, Douglas G. MacMartin, Walker Lee, and Mari R. Tye
Atmos. Chem. Phys., 23, 13369–13385, https://doi.org/10.5194/acp-23-13369-2023, https://doi.org/10.5194/acp-23-13369-2023, 2023
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Solar climate interventions, such as injecting sulfur in the stratosphere, may be used to offset some of the adverse impacts of global warming. We use two independently developed Earth system models to assess the uncertainties around stratospheric sulfur injections. The injection locations and amounts are optimized to maintain the same pattern of surface temperature. While both models show reduced warming, the change in rainfall patterns (even without sulfur injections) is uncertain.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Ilaria Quaglia, Claudia Timmreck, Ulrike Niemeier, Daniele Visioni, Giovanni Pitari, Christina Brodowsky, Christoph Brühl, Sandip S. Dhomse, Henning Franke, Anton Laakso, Graham W. Mann, Eugene Rozanov, and Timofei Sukhodolov
Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, https://doi.org/10.5194/acp-23-921-2023, 2023
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The last very large explosive volcanic eruption we have measurements for is the eruption of Mt. Pinatubo in 1991. It is therefore often used as a benchmark for climate models' ability to reproduce these kinds of events. Here, we compare available measurements with the results from multiple experiments conducted with climate models interactively simulating the aerosol cloud formation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
Atmos. Chem. Phys., 23, 687–709, https://doi.org/10.5194/acp-23-687-2023, https://doi.org/10.5194/acp-23-687-2023, 2023
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Jadwiga H. Richter, Daniele Visioni, Douglas G. MacMartin, David A. Bailey, Nan Rosenbloom, Brian Dobbins, Walker R. Lee, Mari Tye, and Jean-Francois Lamarque
Geosci. Model Dev., 15, 8221–8243, https://doi.org/10.5194/gmd-15-8221-2022, https://doi.org/10.5194/gmd-15-8221-2022, 2022
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Solar climate intervention using stratospheric aerosol injection is a proposed method of reducing global mean temperatures to reduce the worst consequences of climate change. We present a new modeling protocol aimed at simulating a plausible deployment of stratospheric aerosol injection and reproducibility of simulations using other Earth system models: Assessing Responses and Impacts of Solar climate intervention on the Earth system with stratospheric aerosol injection (ARISE-SAI).
Mari R. Tye, Katherine Dagon, Maria J. Molina, Jadwiga H. Richter, Daniele Visioni, Ben Kravitz, and Simone Tilmes
Earth Syst. Dynam., 13, 1233–1257, https://doi.org/10.5194/esd-13-1233-2022, https://doi.org/10.5194/esd-13-1233-2022, 2022
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We examined the potential effect of stratospheric aerosol injection (SAI) on extreme temperature and precipitation. SAI may cause daytime temperatures to cool but nighttime to warm. Daytime cooling may occur in all seasons across the globe, with the largest decreases in summer. In contrast, nighttime warming may be greatest at high latitudes in winter. SAI may reduce the frequency and intensity of extreme rainfall. The combined changes may exacerbate drying over parts of the global south.
Ilaria Quaglia, Daniele Visioni, Giovanni Pitari, and Ben Kravitz
Atmos. Chem. Phys., 22, 5757–5773, https://doi.org/10.5194/acp-22-5757-2022, https://doi.org/10.5194/acp-22-5757-2022, 2022
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Carbonyl sulfide is a gas that mixes very well in the atmosphere and can reach the stratosphere, where it reacts with sunlight and produces aerosol. Here we propose that, by increasing surface fluxes by an order of magnitude, the number of stratospheric aerosols produced may be enough to partially offset the warming produced by greenhouse gases. We explore what effect this would have on the atmospheric composition.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Debra K. Weisenstein, Daniele Visioni, Henning Franke, Ulrike Niemeier, Sandro Vattioni, Gabriel Chiodo, Thomas Peter, and David W. Keith
Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, https://doi.org/10.5194/acp-22-2955-2022, 2022
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This paper explores a potential method of geoengineering that could be used to slow the rate of change of climate over decadal scales. We use three climate models to explore how injections of accumulation-mode sulfuric acid aerosol change the large-scale stratospheric particle size distribution and radiative forcing response for the chosen scenarios. Radiative forcing per unit sulfur injected and relative to the change in aerosol burden is larger with particulate than with SO2 injections.
Daniele Visioni, Simone Tilmes, Charles Bardeen, Michael Mills, Douglas G. MacMartin, Ben Kravitz, and Jadwiga H. Richter
Atmos. Chem. Phys., 22, 1739–1756, https://doi.org/10.5194/acp-22-1739-2022, https://doi.org/10.5194/acp-22-1739-2022, 2022
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Aerosols are simulated in a simplified way in climate models: in the model analyzed here, they are represented in every grid as described by three simple logarithmic distributions, mixing all different species together. The size can evolve when new particles are formed, particles merge together to create a larger one or particles are deposited to the surface. This approximation normally works fairly well. Here we show however that when large amounts of sulfate are simulated, there are problems.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, and Ben Kravitz
Earth Syst. Dynam., 13, 201–217, https://doi.org/10.5194/esd-13-201-2022, https://doi.org/10.5194/esd-13-201-2022, 2022
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Adding SO2 to the stratosphere could temporarily cool the planet by reflecting more sunlight back to space. However, adding SO2 at different latitude(s) and season(s) leads to significant differences in regional surface climate. This study shows that, to cool the planet by 1–1.5 °C, there are likely six to eight choices of injection latitude(s) and season(s) that lead to meaningfully different distributions of climate impacts.
Anton Laakso, Ulrike Niemeier, Daniele Visioni, Simone Tilmes, and Harri Kokkola
Atmos. Chem. Phys., 22, 93–118, https://doi.org/10.5194/acp-22-93-2022, https://doi.org/10.5194/acp-22-93-2022, 2022
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The use of different spatio-temporal sulfur injection strategies with different magnitudes to create an artificial reflective aerosol layer to cool the climate is studied using sectional and modal aerosol schemes in a climate model. There are significant differences in the results depending on the aerosol microphysical module used. Different spatio-temporal injection strategies have a significant impact on the magnitude and zonal distribution of radiative forcing and atmospheric dynamics.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Henning Franke, Ulrike Niemeier, and Daniele Visioni
Atmos. Chem. Phys., 21, 8615–8635, https://doi.org/10.5194/acp-21-8615-2021, https://doi.org/10.5194/acp-21-8615-2021, 2021
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Stratospheric aerosol modification (SAM) can alter the quasi-biennial oscillation (QBO). Our simulations with two different models show that the characteristics of the QBO response are primarily determined by the meridional structure of the aerosol-induced heating. Therefore, the QBO response to SAM depends primarily on the location of injection, while injection type and rate act to scale the specific response. Our results have important implications for evaluating adverse side effects of SAM.
Eliza K. Duncan, George Jordan, Paul Kim, James M. Haywood, Duncan Watson-Parris, Ben Johnson, Alistair Sellar, Zak Kipling, João Teixeira, Florent Malavelle, and Daniel G. Partridge
EGUsphere, https://doi.org/10.5194/egusphere-2026-1043, https://doi.org/10.5194/egusphere-2026-1043, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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The 2014–15 Holuhraun eruption offers a natural experiment to assess how well climate models can capture the changes in aerosol associated with the plume. We investigate the aerosol lifecycle during transport to identify key differences in climate models' representation of aerosol processes, which could affect the models’ ability to capture changes in cloud properties. Our study highlights the importance of the representation of boundary layer nucleation processes in climate models.
Daniele Visioni, Alan Robock, Alistair Duffey, Matthew Henry, Haruki Hirasawa, Walker R. Lee, Cindy Wang, Kelsey Roberts, Shingo Watanabe, Michelle S. Reboita, Masahiro Sugiyama, Ben Kravitz, Jim Haywood, Simone Tilmes, Frederic Bonou, Jack Chen, Timofei Sukodolov, Sandro Vattioni, Andrin Jörimann, Diego Villanueva, Ryan Vella, Paul Farron, Ewa M. Bednarz, Ulrike Niemeier, Colleen Golja, and Juan A. Anel
EGUsphere, https://doi.org/10.5194/egusphere-2026-2417, https://doi.org/10.5194/egusphere-2026-2417, 2026
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
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The Geoengineering Model Intercomparison Project is a coordinated international model intercomparison effort aiming to provide robust experimental protocols for simulations of various Solar Radiation Modification (SRM) methods. In this manuscript, we describe a list of novel experiments decided by the community, to be run by climate models to better understand sources of uncertainty in SRM. We also show and discuss some preliminary results from a few climate models.
Haruki Hirasawa, Matthew Henry, Philip J. Rasch, Robert Wood, Sarah J. Doherty, James Haywood, Alex Wong, Jean-Francois Lamarque, Ezra Brody, and Hailong Wang
Geosci. Model Dev., 19, 3257–3283, https://doi.org/10.5194/gmd-19-3257-2026, https://doi.org/10.5194/gmd-19-3257-2026, 2026
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Marine cloud brightening (MCB) is a proposal to emit sea salt aerosols to make clouds more reflective and cool the climate. Here, we use three climate models to study a hypothetical future where MCB is used to maintain temperatures near 2020–2039 conditions. The simulation results indicate that using MCB in midlatitude ocean regions can keep the climate close to present day conditions. This reduces many of the negative impacts shown in previous studies, informing future modeling efforts.
Isobel M. Parry, Paul D. L. Ritchie, Olivier Boucher, Peter M. Cox, James M. Haywood, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Earth Syst. Dynam., 17, 387–414, https://doi.org/10.5194/esd-17-387-2026, https://doi.org/10.5194/esd-17-387-2026, 2026
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Contrary to some expectations, results from the latest Earth System Models suggest that Solar Radiation Geoengineering could protect the Amazon rainforest from climate-driven dieback. Under Stratospheric Aerosol Injection, carbon storage in Amazonia was projected to increase by a mean of 10.8 % relative to a high CO2 emissions scenario, and even by 8.6% compared to a more conventional medium CO2 emissions scenario.
Alistair Duffey, Walker Lee, Lauren Wheeler, Peter Irvine, Benjamin Wagman, Matthew Henry, Daniele Visioni, Michel Tsamados, and Douglas MacMartin
Earth Syst. Dynam., 17, 353–385, https://doi.org/10.5194/esd-17-353-2026, https://doi.org/10.5194/esd-17-353-2026, 2026
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Adding a layer of reflective particles high in the atmosphere is one suggested way of cooling the planet and reducing the impacts of climate change. This technique might be less logistically difficult in the high latitudes, because the material could be released at lower altitude there. Here, we use new simulations in three earth system models to assess how this form of intervention, High-Latitude Low-Altitude Stratospheric Aerosol Injection (HiLLA-SAI), would impact the global climate.
Masaru Yoshioka, Daniel P. Grosvenor, Amy H. Peace, Jim M. Haywood, Ying Chen, and Paul R. Field
Atmos. Chem. Phys., 26, 4341–4358, https://doi.org/10.5194/acp-26-4341-2026, https://doi.org/10.5194/acp-26-4341-2026, 2026
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We used advanced computer simulations to study how aerosol particles from a volcanic eruption in Iceland affected clouds. The eruption plume increased small droplets, but changes in cloud water and horizontal extent were not clear. Satellite comparisons between plume and non-plume regions can miss volcanic effects due to spatial variability in weather and aerosol, but simulations can isolate the impact by comparing cases with and without the eruption.
Lantao Sun, James W. Hurrell, Kristen L. Rasmussen, Bali Summers, Erin A. Sherman, and Ben Kravitz
Geosci. Model Dev., 19, 2239–2256, https://doi.org/10.5194/gmd-19-2239-2026, https://doi.org/10.5194/gmd-19-2239-2026, 2026
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We develop a novel framework using the convection-permitting Weather Research and Forecasting (WRF) model to assess how stratospheric aerosol injection, a solar climate intervention strategy, affects future convective weather over the contiguous U.S. Results demonstrate the feasibility and scientific potential of this approach for evaluating weather-scale impacts and suggest that such intervention may mitigate changes in temperature, precipitation, and convective activity due to warming.
Walker Raymond Lee, Simone Tilmes, and Ewa M. Bednarz
EGUsphere, https://doi.org/10.5194/egusphere-2026-1004, https://doi.org/10.5194/egusphere-2026-1004, 2026
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We present climate model simulation of stratospheric aerosol injection, a proposed method of climate intervention where reflective particles are placed in the stratosphere to cool the planet. We design our simulated interventions to maintain certain surface temperature patterns, and show that the same temperatures can be maintained in different ways because of how the ocean transports heat. This has implications for how climate intervention model experiments are designed in the future.
Jared Farley, Douglas G. MacMartin, Daniele Visioni, Ben Kravitz, Ewa M. Bednarz, Alistair Duffey, Matthew Henry, and Ali Akherati
Geosci. Model Dev., 19, 1809–1831, https://doi.org/10.5194/gmd-19-1809-2026, https://doi.org/10.5194/gmd-19-1809-2026, 2026
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As the climate changes, many are studying sunlight reflection as a potential method of cooling. Such climate intervention could be deployed in many possible ways, including in scenarios where not every actor agrees on the strategy of cooling. These scenarios are so diverse that to explore all of them using earth system models proves to be too costly. In this paper, we develop a simplified climate model that allows users to easily explore climate intervention scenarios of their choice.
Sean Davis, William Ball, Yue Jia, Gabriel Chiodo, Justin Alsing, James Keeble, Hideharu Akiyoshi, Carlo Arosio, Ewa Bednarz, Andreas Chrysanthou, Melanie Coldewey-Egbers, Robert Damadeo, Sandip Dhomse, Mohamadou Diallo, Simone Dietmuller, Roland Eichinger, Stacey Frith, Birgit Hassler, Michaela Hegglin, Daan Hubert, Patrick Jöckel, Béatrice Josse, Natalya Kramarova, Diego Loyola, Eliane Maillard Barras, Marion Marchand, Olaf Morgenstern, David Plummer, Robert Portmann, Karen Rosenlof, Alexei Rozanov, Viktoria Sofieva, Johannes Staehelin, Timofei Sukhodolov, Kleareti Tourpali, Ronald Van der A, H. J. Ray Wang, Krzysztof Wargan, Shingo Watanabe, Mark Weber, Jeannette Wild, Yousuke Yamashita, and Jerry Ziemke
EGUsphere, https://doi.org/10.5194/egusphere-2026-532, https://doi.org/10.5194/egusphere-2026-532, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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This study investigates how tropical ozone levels have changed since 2000 in chemistry climate models and satellite observations to determine how well they agree with one another, and to see if current trends can help predict future levels. At some, satellite records disagree significantly on the magnitude of ozone changes. The study shows a connection between recent ozone trends and future ozone levels, suggesting that satellite measurements could help constrain future ozone changes.
Simone Tilmes, Daniele Visioni, Ilaria Quaglia, Yunqian Zhu, Charles G. Bardeen, Francis Vitt, and Pengfei Yu
Atmos. Chem. Phys., 26, 2649–2666, https://doi.org/10.5194/acp-26-2649-2026, https://doi.org/10.5194/acp-26-2649-2026, 2026
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This study compares two sets of stratospheric aerosol injection (SAI) experiments using the same modeling framework, differing only in their aerosol microphysical schemes. Results show that these two schemes can yield substantially different aerosol burdens, radiative changes, and impacts when simulating the same injection scenarios. These findings suggest that more sophisticated aerosol models may be necessary to accurately assess the efficacy, side effects, and climate impacts of SAI.
Martin B. Andrews, Neal Butchart, James A. Anstey, Ewa Bednarz, Dillon Elsbury, Jorge L. García-Franco, Vinay Kumar, Froila M. Palmeiro, Natasha E. Trencham, Kohei Yoshida, Zhaoyang Chai, Dong-Chan Hong, Kai Huang, Aleena M. Jaison, Yoshio Kawatani, Jeff R. Knight, Pu Lin, François Lott, Yixiong Lu, Hiroaki Naoe, Scott M. Osprey, Jadwiga H. Richter, Federico Serva, Seok-Woo Son, Qi Tang, Shingo Watanabe, and Jinbo Xie
EGUsphere, https://doi.org/10.5194/egusphere-2026-737, https://doi.org/10.5194/egusphere-2026-737, 2026
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The observed winds in the upper atmosphere over the equator have alternating easterly and westerly regions that descend towards the lower atmosphere before dissipating, with a period of approximately 28 months. This is known as the Quasi-Biennial Oscillation (QBO). The QBO is known to influence remote regions of the atmosphere. This paper details the results of multi-model experiments where the QBO is nudged towards the observed QBO allowing the assessment of these remote connections.
Andrin Jörimann, Timofei Sukhodolov, Simone Tilmes, David Plummer, Shingo Watanabe, Hideharu Akiyoshi, Gabriel Chiodo, Daniele Visioni, Sandro Vattioni, Eugene Rozanov, Ewa M. Bednarz, Béatrice Jossé, Yousuke Yamashita, and Thomas Peter
EGUsphere, https://doi.org/10.5194/egusphere-2026-444, https://doi.org/10.5194/egusphere-2026-444, 2026
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We study a future scenario where artificial stratospheric aerosol injections counter medium climate change, to understand possible negative side effects like ozone depletion. The injected aerosol layer is implemented uniformly in five climate models, which eliminates some uncertainty from model-specific aerosol evolution. The models agree well on where and how key thermodynamical (heating, circulation) and chemical processes change, however, the strength of the change varies considerably.
Ewa M. Bednarz, Amy H. Butler, James M. Haywood, Matthew Henry, Andy Jones, Ben Kravitz, Walker R. Lee, Douglas G. MacMartin, Amanda C. Maycock, Takashi Sekiya, Shingo Watanabe, and Daniele Visioni
EGUsphere, https://doi.org/10.5194/egusphere-2026-310, https://doi.org/10.5194/egusphere-2026-310, 2026
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An assessment of the potential impacts of Stratospheric Aerosol Injection, a proposed method to offset global warming, on stratospheric ozone projections over the 21st century using the new multi-model GeoMIP G6-1.5K-SAI experiment. We discuss drivers of the responses, identify areas of model agreement and disagreement and sources of uncertainty. Our results highlight the need to assess any projected SAI impacts in wider strategy and scenario dimension using a multi-model framework.
Cindy Wang, Daniele Visioni, Glen Chua, and Ewa M. Bednarz
Atmos. Chem. Phys., 26, 1339–1357, https://doi.org/10.5194/acp-26-1339-2026, https://doi.org/10.5194/acp-26-1339-2026, 2026
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Stratospheric aerosol injection is a proposed method to slow global warming by adding tiny reflective particles high up in the atmosphere to cool the planet. We study how this proposed method might affect air quality and human health using climate models. We find that the health impacts would likely be small and are mainly driven by changes in climate, not by the particles themselves.
Clara Orbe, Alison Ming, Gabriel Chiodo, Michael Prather, Mohamadou Diallo, Qi Tang, Andreas Chrysanthou, Hiroaki Naoe, Xin Zhou, Irina Thaler, Dillon Elsbury, Ewa Bednarz, Jonathon S. Wright, Aaron Match, Shingo Watanabe, James Anstey, Tobias Kerzenmacher, Stefan Versick, Marion Marchand, Feng Li, and James Keeble
Geosci. Model Dev., 19, 773–794, https://doi.org/10.5194/gmd-19-773-2026, https://doi.org/10.5194/gmd-19-773-2026, 2026
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The quasi-biennial oscillation (QBO) is the main source of wind fluctuations in the tropical stratosphere, which can couple to surface climate. However, models do a poor job of simulating the QBO in the lower stratosphere, for reasons that remain unclear. One possibility is that models do not completely represent how ozone influences the QBO-associated wind variations. Here we propose a multi-model framework for assessing how ozone influences the QBO in recent past and future climates.
Ewa M. Bednarz, Amy H. Butler, Xinyue Wang, Zhihong Zhuo, Wandi Yu, Georgiy Stenchikov, Matthew Toohey, and Yunqian Zhu
Atmos. Chem. Phys., 26, 197–215, https://doi.org/10.5194/acp-26-197-2026, https://doi.org/10.5194/acp-26-197-2026, 2026
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We investigate whether the 2022 Hunga eruption could affect surface climate via indirect pathways using large ensembles of Earth System Model simulations. These suggest that the eruption could have a non-negligible influence on regional surface climate, and we discuss the mechanisms via which such an influence could occur but also highlight that the forcing is relatively weak compared to natural climate variability which significantly hinders the detection of such impacts in the real world.
Anthony C. Jones, James M. Haywood, Matthew Henry, and Alistair Duffey
EGUsphere, https://doi.org/10.5194/egusphere-2025-6332, https://doi.org/10.5194/egusphere-2025-6332, 2026
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Injecting aerosol into the stratosphere has been suggested to rapidly cool the planet and counter climate change. Rival actors who oppose deployment may seek to counter stratospheric aerosol injection. Using a climate model, we investigate whether stratospheric aerosol removal could be hastened by injecting coarse aerosol which promote aerosol growth and gravitational settling. We find that this could be effective, reducing aerosol impacts by 30 % in simulations, and warrants further research.
Katharina Perny, Timofei Sukhodolov, Ales Kuchar, Pavle Arsenovic, Bernadette Rosati, Christoph Brühl, Sandip S. Dhomse, Andrin Jörimann, Anton Laakso, Graham Mann, Ulrike Niemeier, Giovanni Pitari, Ilaria Quaglia, Takashi Sekiya, Kengo Sudo, Claudia Timmreck, Simone Tilmes, Daniele Visioni, and Harald E. Rieder
EGUsphere, https://doi.org/10.5194/egusphere-2025-5915, https://doi.org/10.5194/egusphere-2025-5915, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Major volcanic eruptions, such as the one of Mt. Pinatubo in 1991, can inject large amounts of sulfur dioxide into the stratosphere. The resulting aerosol cloud affects stratospheric temperature and thereby middle atmospheric dynamics and chemistry. Here we investigate similarities and differences across an ensemble of climate models in reproducing the stratospheric temperature signal following the Mt. Pinatubo eruption.
Alex M. Mason, Matthew Henry, Haruki Hirasawa, Fiona M. O'Connor, and James Haywood
EGUsphere, https://doi.org/10.5194/egusphere-2025-5591, https://doi.org/10.5194/egusphere-2025-5591, 2025
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Marine Cloud Brightening (MCB) proposes the spraying of sea salt particles into marine clouds to cool the planet. MCB in midlatitude regions in models gave a relatively even climate response. We use 42 simulations of MCB to target several climate responses. Two optimised combinations are compared to a midlatitude MCB simulation, which improved sea ice restoration and the temperature response pattern, highlighting the importance of high latitude MCB for MCB optimisation in this model.
Huihui Wu, Fanny Peers, Jonathan W. Taylor, Chenjie Yu, Steven J. Abel, Paul A. Barrett, Jamie Trembath, Keith Bower, Jim M. Haywood, and Hugh Coe
Atmos. Chem. Phys., 25, 16589–16609, https://doi.org/10.5194/acp-25-16589-2025, https://doi.org/10.5194/acp-25-16589-2025, 2025
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This study investigates the transport history of African Biomass-Burning aerosols (BBAs) over the Southeast Atlantic (SEA) and their impacts on cloud properties. Using in situ airborne measurements around Ascension Island, this work provides critical parameterizations of aerosol–cloud interactions to improve the assessment of radiative forcing in the SEA region. It also identifies key entrainment regions for understanding the vertical transport process of African BBAs.
Walker Raymond Lee, Daniele Visioni, Benjamin Moore Wagman, Christopher Robert Wentland, Ben Kravitz, Shingo Watanabe, Takashi Sekiya, Andy Jones, Jim Haywood, Matthew Henry, and Ewa Monika Bednarz
EGUsphere, https://doi.org/10.5194/egusphere-2025-5742, https://doi.org/10.5194/egusphere-2025-5742, 2025
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Stratospheric aerosol injection (SAI) is a proposed method of cooling the planet by introducing reflective particles called aerosols into the middle atmosphere to reflect sunlight back into space. We consider recent simulations of SAI from four different climate models. SAI cools the planet effectively in all four models; we examine the impacts on temperature and precipitation in each model and compare to previous experiments. Our simulations will help inform future research and policy.
Ewa M. Bednarz, Valentina Aquila, Amy H. Butler, Peter Colarco, Eric Fleming, Freja F. Østerstrøm, David Plummer, Ilaria Quaglia, William Randel, Michelle L. Santee, Takashi Sekiya, Simone Tilmes, Xinyue Wang, Shingo Watanabe, Wandi Yu, Jun Zhang, Yunqian Zhu, and Zhihong Zhuo
EGUsphere, https://doi.org/10.5194/egusphere-2025-4609, https://doi.org/10.5194/egusphere-2025-4609, 2025
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The 2022 Hunga eruption injected unprecedented quantities of water vapor into the stratosphere, alongside modest amounts of aerosol precursors. We assess its impacts on stratospheric ozone layer using a multi-model ensemble of chemistry-climate simulations. The results confirm the eruption's role in modulating SH mid and high latitudes ozone abundances in the short term, and discuss the different chemical and dynamical processes driving those changes as well as the role of natural variability.
Eliza K. Duncan, Jonathan E. Fieldsend, Alistair Sellar, Emanuele Tovazzi, Paul Kim, James M. Haywood, and Daniel G. Partridge
EGUsphere, https://doi.org/10.5194/egusphere-2025-4298, https://doi.org/10.5194/egusphere-2025-4298, 2025
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Atmospheric aerosol particles are a major confounding factor in accurately representing climate change. We build a novel generic framework to untangle the role of complex processes focusing on a remote site in Antarctica as a case study in near-pristine conditions. Our machine-learning model predicts aerosol concentrations from an airmass history, considering the meteorology and potential sources and removal processes, enabling improved representation in climate models.
George Jordan, Florent Malavelle, Jim Haywood, Ying Chen, Ben Johnson, Daniel Partridge, Amy Peace, Eliza Duncan, Duncan Watson-Parris, David Neubauer, Anton Laakso, Martine Michou, and Pierre Nabat
Atmos. Chem. Phys., 25, 13393–13428, https://doi.org/10.5194/acp-25-13393-2025, https://doi.org/10.5194/acp-25-13393-2025, 2025
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The 2014–15 Holuhraun eruption created a vast aerosol plume that acted as a natural experiment to assess how well climate models capture changes in cloud properties due to increased aerosol. We find that climate models represent the observed shift to smaller, more numerous cloud droplets well. However, climate models diverge in their aerosol-induced changes to large-scale cloud properties, particularly cloud liquid water content. Our study shows that Holuhraun had a cooling effect on the Earth.
Zhihong Zhuo, Xinyue Wang, Yunqian Zhu, Wandi Yu, Ewa M. Bednarz, Eric Fleming, Peter R. Colarco, Shingo Watanabe, David Plummer, Georgiy Stenchikov, William Randel, Adam Bourassa, Valentina Aquila, Takashi Sekiya, Mark R. Schoeberl, Simone Tilmes, Jun Zhang, Paul J. Kushner, and Francesco S. R. Pausata
Atmos. Chem. Phys., 25, 13161–13176, https://doi.org/10.5194/acp-25-13161-2025, https://doi.org/10.5194/acp-25-13161-2025, 2025
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The 2022 Hunga eruption caused unprecedented stratospheric water injection, triggering unique atmospheric impacts. This study combines observations and model simulations, projecting a stratospheric water vapor anomaly lasting 4–7 years, with significant temperature variations and ozone depletion in the upper atmosphere lasting 7–10 years. These findings offer critical insights into the role of stratospheric water vapor in shaping climate and atmospheric chemistry.
Ilaria Quaglia, Daniele Visioni, Ewa M. Bednarz, Yunqian Zhu, Georgiy Stenchikov, Valentina Aquila, Cheng-Cheng Liu, Graham W. Mann, Yifeng Peng, Takashi Sekiya, Simone Tilmes, Xinyue Wang, Shingo Watanabe, Pengfei Yu, Jun Zhang, and Wandi Yu
EGUsphere, https://doi.org/10.5194/egusphere-2025-3769, https://doi.org/10.5194/egusphere-2025-3769, 2025
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On January 15, 2022, the Hunga volcano eruption released unprecedented amounts of water vapor into the atmosphere alongside a modest amount of SO2. In this work we analyse results from multiple Earth system models. The models agree that the eruption led to small negative radiative forcing from sulfate aerosols and that the contribution from water vapor was minimal. Therefore, the Hunga eruption cannot explain the exceptional surface warming observed in 2023.
Yunqian Zhu, Hideharu Akiyoshi, Valentina Aquila, Elizabeth Asher, Ewa M. Bednarz, Slimane Bekki, Christoph Brühl, Amy H. Butler, Parker Case, Simon Chabrillat, Gabriel Chiodo, Margot Clyne, Peter R. Colarco, Sandip Dhomse, Lola Falletti, Eric Fleming, Ben Johnson, Andrin Jörimann, Mahesh Kovilakam, Gerbrand Koren, Ales Kuchar, Nicolas Lebas, Qing Liang, Cheng-Cheng Liu, Graham Mann, Michael Manyin, Marion Marchand, Olaf Morgenstern, Paul Newman, Luke D. Oman, Freja F. Østerstrøm, Yifeng Peng, David Plummer, Ilaria Quaglia, William Randel, Samuel Rémy, Takashi Sekiya, Stephen Steenrod, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, Rei Ueyama, Daniele Visioni, Xinyue Wang, Shingo Watanabe, Yousuke Yamashita, Pengfei Yu, Wandi Yu, Jun Zhang, and Zhihong Zhuo
Geosci. Model Dev., 18, 5487–5512, https://doi.org/10.5194/gmd-18-5487-2025, https://doi.org/10.5194/gmd-18-5487-2025, 2025
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To understand the climate impact of the 2022 Hunga volcanic eruption, we developed a climate model–observation comparison project. The paper describes the protocols and models that participate in the experiments. We designed several experiments to achieve our goals of this activity: (1) to evaluate the climate model performance and (2) to understand the Earth system responses to this eruption.
Elizabeth Quaye, Ben T. Johnson, James M. Haywood, Guido R. van der Werf, Roland Vernooij, Stephen A. Sitch, and Tom Eames
EGUsphere, https://doi.org/10.5194/egusphere-2025-3936, https://doi.org/10.5194/egusphere-2025-3936, 2025
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We find aerosol optical depths in a global climate model are overestimated during extreme wildfire events if emissions are scaled up by a factor of two, typically applied to improve simulated aerosol on seasonal–annual timescales. We propose a technique where a variable scaling factor is determined by fuel consumption, improving correlation in five fire-affected areas. We explore the impact of this change on aerosol radiative effects, during extreme events and on broader space and time scales.
Ezra Brody, Yan Zhang, Douglas G. MacMartin, Daniele Visioni, Ben Kravitz, and Ewa M. Bednarz
Earth Syst. Dynam., 16, 1325–1341, https://doi.org/10.5194/esd-16-1325-2025, https://doi.org/10.5194/esd-16-1325-2025, 2025
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Stratospheric aerosol injection (SAI) is being studied as a possible supplement to emission reduction to temporarily mitigate some of the risks associated with climate change. The latitudes at which SAI is done determine the effect on the climate. We try to find if there are combinations of latitudes that do a better job of counteracting climate change than existing strategies. We found that there are, but just how significant these improvements are depends on the amount of cooling.
Simone Tilmes, Ewa M. Bednarz, Andrin Jörimann, Daniele Visioni, Douglas E. Kinnison, Gabriel Chiodo, and David Plummer
Atmos. Chem. Phys., 25, 6001–6023, https://doi.org/10.5194/acp-25-6001-2025, https://doi.org/10.5194/acp-25-6001-2025, 2025
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In this paper, we describe the details of a new multi-model intercomparison experiment to assess the effects of Stratospheric Aerosol Intervention (SAI) on stratospheric chemistry and dynamics and, therefore, ozone. Second, we discuss the advantages and differences of the more constrained experiment compared to fully interactive model experiments. This way, we advance the process-level understanding of the drivers of SAI-induced atmospheric responses.
Martin Juckes, Karl E. Taylor, Fabrizio Antonio, David Brayshaw, Carlo Buontempo, Jian Cao, Paul J. Durack, Michio Kawamiya, Hyungjun Kim, Tomas Lovato, Chloe Mackallah, Matthew Mizielinski, Alessandra Nuzzo, Martina Stockhause, Daniele Visioni, Jeremy Walton, Briony Turner, Eleanor O'Rourke, and Beth Dingley
Geosci. Model Dev., 18, 2639–2663, https://doi.org/10.5194/gmd-18-2639-2025, https://doi.org/10.5194/gmd-18-2639-2025, 2025
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The Baseline Climate Variables for Earth System Modelling (ESM-BCVs) are defined as a list of 135 variables which have high utility for the evaluation and exploitation of climate simulations. The list reflects the most frequently used variables from Earth system models based on an assessment of data publication and download records from the largest archive of global climate projects.
Matthew Henry, Ewa M. Bednarz, and Jim Haywood
Atmos. Chem. Phys., 24, 13253–13268, https://doi.org/10.5194/acp-24-13253-2024, https://doi.org/10.5194/acp-24-13253-2024, 2024
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Stratospheric aerosol injection (SAI) refers to a climate intervention by which aerosols are intentionally added to the high atmosphere to increase the amount of reflected sunlight and reduce Earth's temperature. The climate outcomes of SAI depend on the latitude of injection. While injecting aerosols at the Equator has undesirable side effects, injecting away from the Equator has different effects on temperature, rainfall, ozone, and atmospheric circulation, which are analysed in this work.
Ilaria Quaglia and Daniele Visioni
Earth Syst. Dynam., 15, 1527–1541, https://doi.org/10.5194/esd-15-1527-2024, https://doi.org/10.5194/esd-15-1527-2024, 2024
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On 1 January 2020, international shipping vessels were required to substantially reduce the amount of particulate they emit to improve air quality. In this work we demonstrate how this regulatory change contributed to the anomalous warming observed in recent months using climate model simulations that include such a change. Future policies should also perhaps consider their impact on climate, and climate modelers should promptly include those changes in future modeling efforts.
Ou Wang, Ju Liang, Yuchen Gu, Jim M. Haywood, Ying Chen, Chenwei Fang, and Qin'geng Wang
Atmos. Chem. Phys., 24, 12355–12373, https://doi.org/10.5194/acp-24-12355-2024, https://doi.org/10.5194/acp-24-12355-2024, 2024
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As extreme precipitation events increase in China, this study explores the potential of stratospheric aerosol injection (SAI) to mitigate these effects by the end of the 21st century using the UKESM1 model. Results show that SAI reduces extreme precipitation in eastern China. However, caution is advised due to potential side effects in high-latitude regions, and further optimization is required for future SAI deployment.
Philip J. Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah J. Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
Geosci. Model Dev., 17, 7963–7994, https://doi.org/10.5194/gmd-17-7963-2024, https://doi.org/10.5194/gmd-17-7963-2024, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming and climate impacts from greenhouse gas increases. This slightly changes clouds in six ocean regions to reflect more sunlight and cool the Earth. Example changes in clouds and climate are shown for three climate models. Cloud changes differ between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Christina V. Brodowsky, Timofei Sukhodolov, Gabriel Chiodo, Valentina Aquila, Slimane Bekki, Sandip S. Dhomse, Michael Höpfner, Anton Laakso, Graham W. Mann, Ulrike Niemeier, Giovanni Pitari, Ilaria Quaglia, Eugene Rozanov, Anja Schmidt, Takashi Sekiya, Simone Tilmes, Claudia Timmreck, Sandro Vattioni, Daniele Visioni, Pengfei Yu, Yunqian Zhu, and Thomas Peter
Atmos. Chem. Phys., 24, 5513–5548, https://doi.org/10.5194/acp-24-5513-2024, https://doi.org/10.5194/acp-24-5513-2024, 2024
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The aerosol layer is an essential part of the climate system. We characterize the sulfur budget in a volcanically quiescent (background) setting, with a special focus on the sulfate aerosol layer using, for the first time, a multi-model approach. The aim is to identify weak points in the representation of the atmospheric sulfur budget in an intercomparison of nine state-of-the-art coupled global circulation models.
Anton Laakso, Daniele Visioni, Ulrike Niemeier, Simone Tilmes, and Harri Kokkola
Earth Syst. Dynam., 15, 405–427, https://doi.org/10.5194/esd-15-405-2024, https://doi.org/10.5194/esd-15-405-2024, 2024
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This study is the second in a two-part series in which we explore the dependency of the impacts of stratospheric sulfur injections on both the model employed and the strategy of injection utilized. The study uncovers uncertainties associated with these techniques to cool climate, highlighting how the simulated climate impacts are dependent on both the selected model and the magnitude of the injections. We also show that estimating precipitation impacts of aerosol injection is a complex task.
Daniele Visioni, Alan Robock, Jim Haywood, Matthew Henry, Simone Tilmes, Douglas G. MacMartin, Ben Kravitz, Sarah J. Doherty, John Moore, Chris Lennard, Shingo Watanabe, Helene Muri, Ulrike Niemeier, Olivier Boucher, Abu Syed, Temitope S. Egbebiyi, Roland Séférian, and Ilaria Quaglia
Geosci. Model Dev., 17, 2583–2596, https://doi.org/10.5194/gmd-17-2583-2024, https://doi.org/10.5194/gmd-17-2583-2024, 2024
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This paper describes a new experimental protocol for the Geoengineering Model Intercomparison Project (GeoMIP). In it, we describe the details of a new simulation of sunlight reflection using the stratospheric aerosols that climate models are supposed to run, and we explain the reasons behind each choice we made when defining the protocol.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, Ewa M. Bednarz, and Ben Kravitz
Earth Syst. Dynam., 15, 191–213, https://doi.org/10.5194/esd-15-191-2024, https://doi.org/10.5194/esd-15-191-2024, 2024
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Injecting SO2 into the lower stratosphere can temporarily reduce global mean temperature and mitigate some risks associated with climate change, but injecting it at different latitudes and seasons would have different impacts. This study introduces new stratospheric aerosol injection (SAI) strategies and explores the importance of the choice of SAI strategy, demonstrating that it notably affects the distribution of aerosol cloud, injection efficiency, and various surface climate impacts.
George Jordan, Florent Malavelle, Ying Chen, Amy Peace, Eliza Duncan, Daniel G. Partridge, Paul Kim, Duncan Watson-Parris, Toshihiko Takemura, David Neubauer, Gunnar Myhre, Ragnhild Skeie, Anton Laakso, and James Haywood
Atmos. Chem. Phys., 24, 1939–1960, https://doi.org/10.5194/acp-24-1939-2024, https://doi.org/10.5194/acp-24-1939-2024, 2024
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The 2014–15 Holuhraun eruption caused a huge aerosol plume in an otherwise unpolluted region, providing a chance to study how aerosol alters cloud properties. This two-part study uses observations and models to quantify this relationship’s impact on the Earth’s energy budget. Part 1 suggests the models capture the observed spatial and chemical evolution of the plume, yet no model plume is exact. Understanding these differences is key for Part 2, where changes to cloud properties are explored.
Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
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The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Ewa M. Bednarz, Ryan Hossaini, and Martyn P. Chipperfield
Atmos. Chem. Phys., 23, 13701–13711, https://doi.org/10.5194/acp-23-13701-2023, https://doi.org/10.5194/acp-23-13701-2023, 2023
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We quantify, for the first time, the time-varying impact of uncontrolled emissions of chlorinated very short-lived substances (Cl-VSLSs) on stratospheric ozone using a state-of-the-art chemistry-climate model. We demonstrate that Cl-VSLSs already have a non-negligible impact on stratospheric ozone, including a local reduction of up to ~7 DU in Arctic ozone in the cold winter of 2019/20, and any so future growth in emissions will continue to offset some of the benefits of the Montreal Protocol.
Ewa M. Bednarz, Amy H. Butler, Daniele Visioni, Yan Zhang, Ben Kravitz, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 13665–13684, https://doi.org/10.5194/acp-23-13665-2023, https://doi.org/10.5194/acp-23-13665-2023, 2023
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We use a state-of-the-art Earth system model and a set of stratospheric aerosol injection (SAI) strategies to achieve the same level of global mean surface cooling through different combinations of location and/or timing of the injection. We demonstrate that the choice of SAI strategy can lead to contrasting impacts on stratospheric and tropospheric temperatures, circulation, and chemistry (including stratospheric ozone), thereby leading to different impacts on regional surface climate.
Ewa M. Bednarz, Ryan Hossaini, N. Luke Abraham, and Martyn P. Chipperfield
Geosci. Model Dev., 16, 6187–6209, https://doi.org/10.5194/gmd-16-6187-2023, https://doi.org/10.5194/gmd-16-6187-2023, 2023
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Development and performance of the new DEST chemistry scheme of UM–UKCA is described. The scheme extends the standard StratTrop scheme by including important updates to the halogen chemistry, thus allowing process-oriented studies of stratospheric ozone depletion and recovery, including impacts from both controlled long-lived ozone-depleting substances and emerging issues around uncontrolled, very short-lived substances. It will thus aid studies in support of future ozone assessment reports.
Matthew Henry, Jim Haywood, Andy Jones, Mohit Dalvi, Alice Wells, Daniele Visioni, Ewa M. Bednarz, Douglas G. MacMartin, Walker Lee, and Mari R. Tye
Atmos. Chem. Phys., 23, 13369–13385, https://doi.org/10.5194/acp-23-13369-2023, https://doi.org/10.5194/acp-23-13369-2023, 2023
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Solar climate interventions, such as injecting sulfur in the stratosphere, may be used to offset some of the adverse impacts of global warming. We use two independently developed Earth system models to assess the uncertainties around stratospheric sulfur injections. The injection locations and amounts are optimized to maintain the same pattern of surface temperature. While both models show reduced warming, the change in rainfall patterns (even without sulfur injections) is uncertain.
Chenwei Fang, Jim M. Haywood, Ju Liang, Ben T. Johnson, Ying Chen, and Bin Zhu
Atmos. Chem. Phys., 23, 8341–8368, https://doi.org/10.5194/acp-23-8341-2023, https://doi.org/10.5194/acp-23-8341-2023, 2023
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The responses of Asian summer monsoon duration and intensity to air pollution mitigation are identified given the net-zero future. We show that reducing scattering aerosols makes the rainy season longer and stronger across South Asia and East Asia but that absorbing aerosol reduction has the opposite effect. Our results hint at distinct monsoon responses to emission controls that target different aerosols.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Alice F. Wells, Andy Jones, Martin Osborne, Lilly Damany-Pearce, Daniel G. Partridge, and James M. Haywood
Atmos. Chem. Phys., 23, 3985–4007, https://doi.org/10.5194/acp-23-3985-2023, https://doi.org/10.5194/acp-23-3985-2023, 2023
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In 2019 the Raikoke volcano erupted explosively, emitting the largest injection of SO2 into the stratosphere since 2011. Observations indicated that a large amount of volcanic ash was also injected. Previous studies have identified that volcanic ash can prolong the lifetime of stratospheric aerosol optical depth, which we explore in UKESM1. Comparisons to observations suggest that including ash in model emission schemes can improve the representation of volcanic plumes in global climate models.
Ju Liang and Jim Haywood
Atmos. Chem. Phys., 23, 1687–1703, https://doi.org/10.5194/acp-23-1687-2023, https://doi.org/10.5194/acp-23-1687-2023, 2023
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The recent record-breaking flood events in China during the summer of 2021 highlight the importance of mitigating the risks from future changes in high-impact weather systems under global warming. Based on a state-of-the-art Earth system model, we demonstrate a pilot study on the responses of atmospheric rivers and extreme precipitation over East Asia to anthropogenically induced climate warming and an unconventional mitigation strategy – stratospheric aerosol injection.
Yangxin Chen, Duoying Ji, Qian Zhang, John C. Moore, Olivier Boucher, Andy Jones, Thibaut Lurton, Michael J. Mills, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Earth Syst. Dynam., 14, 55–79, https://doi.org/10.5194/esd-14-55-2023, https://doi.org/10.5194/esd-14-55-2023, 2023
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Solar geoengineering has been proposed as a way of counteracting the warming effects of increasing greenhouse gases by reflecting solar radiation. This work shows that solar geoengineering can slow down the northern-high-latitude permafrost degradation but cannot preserve the permafrost ecosystem as that under a climate of the same warming level without solar geoengineering.
Ilaria Quaglia, Claudia Timmreck, Ulrike Niemeier, Daniele Visioni, Giovanni Pitari, Christina Brodowsky, Christoph Brühl, Sandip S. Dhomse, Henning Franke, Anton Laakso, Graham W. Mann, Eugene Rozanov, and Timofei Sukhodolov
Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, https://doi.org/10.5194/acp-23-921-2023, 2023
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The last very large explosive volcanic eruption we have measurements for is the eruption of Mt. Pinatubo in 1991. It is therefore often used as a benchmark for climate models' ability to reproduce these kinds of events. Here, we compare available measurements with the results from multiple experiments conducted with climate models interactively simulating the aerosol cloud formation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
Atmos. Chem. Phys., 23, 687–709, https://doi.org/10.5194/acp-23-687-2023, https://doi.org/10.5194/acp-23-687-2023, 2023
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Jadwiga H. Richter, Daniele Visioni, Douglas G. MacMartin, David A. Bailey, Nan Rosenbloom, Brian Dobbins, Walker R. Lee, Mari Tye, and Jean-Francois Lamarque
Geosci. Model Dev., 15, 8221–8243, https://doi.org/10.5194/gmd-15-8221-2022, https://doi.org/10.5194/gmd-15-8221-2022, 2022
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Solar climate intervention using stratospheric aerosol injection is a proposed method of reducing global mean temperatures to reduce the worst consequences of climate change. We present a new modeling protocol aimed at simulating a plausible deployment of stratospheric aerosol injection and reproducibility of simulations using other Earth system models: Assessing Responses and Impacts of Solar climate intervention on the Earth system with stratospheric aerosol injection (ARISE-SAI).
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Flossie Brown, Gerd A. Folberth, Stephen Sitch, Susanne Bauer, Marijn Bauters, Pascal Boeckx, Alexander W. Cheesman, Makoto Deushi, Inês Dos Santos Vieira, Corinne Galy-Lacaux, James Haywood, James Keeble, Lina M. Mercado, Fiona M. O'Connor, Naga Oshima, Kostas Tsigaridis, and Hans Verbeeck
Atmos. Chem. Phys., 22, 12331–12352, https://doi.org/10.5194/acp-22-12331-2022, https://doi.org/10.5194/acp-22-12331-2022, 2022
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Surface ozone can decrease plant productivity and impair human health. In this study, we evaluate the change in surface ozone due to climate change over South America and Africa using Earth system models. We find that if the climate were to change according to the worst-case scenario used here, models predict that forested areas in biomass burning locations and urban populations will be at increasing risk of ozone exposure, but other areas will experience a climate benefit.
Mari R. Tye, Katherine Dagon, Maria J. Molina, Jadwiga H. Richter, Daniele Visioni, Ben Kravitz, and Simone Tilmes
Earth Syst. Dynam., 13, 1233–1257, https://doi.org/10.5194/esd-13-1233-2022, https://doi.org/10.5194/esd-13-1233-2022, 2022
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We examined the potential effect of stratospheric aerosol injection (SAI) on extreme temperature and precipitation. SAI may cause daytime temperatures to cool but nighttime to warm. Daytime cooling may occur in all seasons across the globe, with the largest decreases in summer. In contrast, nighttime warming may be greatest at high latitudes in winter. SAI may reduce the frequency and intensity of extreme rainfall. The combined changes may exacerbate drying over parts of the global south.
Ewa M. Bednarz, Ryan Hossaini, Martyn P. Chipperfield, N. Luke Abraham, and Peter Braesicke
Atmos. Chem. Phys., 22, 10657–10676, https://doi.org/10.5194/acp-22-10657-2022, https://doi.org/10.5194/acp-22-10657-2022, 2022
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Atmospheric impacts of chlorinated very short-lived substances (Cl-VSLS) over the first two decades of the 21st century are assessed using the UM-UKCA chemistry–climate model. Stratospheric input of Cl from Cl-VSLS is estimated at ~130 ppt in 2019. The use of model set-up with constrained meteorology significantly increases the abundance of Cl-VSLS in the lower stratosphere relative to the free-running set-up. The growth in Cl-VSLS emissions significantly impacted recent HCl and COCl2 trends.
Jim M. Haywood, Andy Jones, Ben T. Johnson, and William McFarlane Smith
Atmos. Chem. Phys., 22, 6135–6150, https://doi.org/10.5194/acp-22-6135-2022, https://doi.org/10.5194/acp-22-6135-2022, 2022
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Simulations are presented investigating the influence of moderately absorbing aerosol in the stratosphere to combat the impacts of climate change. A number of detrimental impacts are noted compared to sulfate aerosol, including (i) reduced cooling efficiency, (ii) increased deficits in global precipitation, (iii) delays in the recovery of the stratospheric ozone hole, and (iv) disruption of the stratospheric circulation and the wintertime storm tracks that impact European precipitation.
Ilaria Quaglia, Daniele Visioni, Giovanni Pitari, and Ben Kravitz
Atmos. Chem. Phys., 22, 5757–5773, https://doi.org/10.5194/acp-22-5757-2022, https://doi.org/10.5194/acp-22-5757-2022, 2022
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Carbonyl sulfide is a gas that mixes very well in the atmosphere and can reach the stratosphere, where it reacts with sunlight and produces aerosol. Here we propose that, by increasing surface fluxes by an order of magnitude, the number of stratospheric aerosols produced may be enough to partially offset the warming produced by greenhouse gases. We explore what effect this would have on the atmospheric composition.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Huiying Ren, Erol Cromwell, Ben Kravitz, and Xingyuan Chen
Hydrol. Earth Syst. Sci., 26, 1727–1743, https://doi.org/10.5194/hess-26-1727-2022, https://doi.org/10.5194/hess-26-1727-2022, 2022
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We used a deep learning method called long short-term memory (LSTM) to fill gaps in data collected by hydrologic monitoring networks. LSTM accounted for correlations in space and time and nonlinear trends in data. Compared to a traditional regression-based time-series method, LSTM performed comparably when filling gaps in data with smooth patterns, while it better captured highly dynamic patterns in data. Capturing such dynamics is critical for understanding dynamic complex system behaviors.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Debra K. Weisenstein, Daniele Visioni, Henning Franke, Ulrike Niemeier, Sandro Vattioni, Gabriel Chiodo, Thomas Peter, and David W. Keith
Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, https://doi.org/10.5194/acp-22-2955-2022, 2022
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This paper explores a potential method of geoengineering that could be used to slow the rate of change of climate over decadal scales. We use three climate models to explore how injections of accumulation-mode sulfuric acid aerosol change the large-scale stratospheric particle size distribution and radiative forcing response for the chosen scenarios. Radiative forcing per unit sulfur injected and relative to the change in aerosol burden is larger with particulate than with SO2 injections.
Daniele Visioni, Simone Tilmes, Charles Bardeen, Michael Mills, Douglas G. MacMartin, Ben Kravitz, and Jadwiga H. Richter
Atmos. Chem. Phys., 22, 1739–1756, https://doi.org/10.5194/acp-22-1739-2022, https://doi.org/10.5194/acp-22-1739-2022, 2022
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Aerosols are simulated in a simplified way in climate models: in the model analyzed here, they are represented in every grid as described by three simple logarithmic distributions, mixing all different species together. The size can evolve when new particles are formed, particles merge together to create a larger one or particles are deposited to the surface. This approximation normally works fairly well. Here we show however that when large amounts of sulfate are simulated, there are problems.
Yan Zhang, Douglas G. MacMartin, Daniele Visioni, and Ben Kravitz
Earth Syst. Dynam., 13, 201–217, https://doi.org/10.5194/esd-13-201-2022, https://doi.org/10.5194/esd-13-201-2022, 2022
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Adding SO2 to the stratosphere could temporarily cool the planet by reflecting more sunlight back to space. However, adding SO2 at different latitude(s) and season(s) leads to significant differences in regional surface climate. This study shows that, to cool the planet by 1–1.5 °C, there are likely six to eight choices of injection latitude(s) and season(s) that lead to meaningfully different distributions of climate impacts.
Anton Laakso, Ulrike Niemeier, Daniele Visioni, Simone Tilmes, and Harri Kokkola
Atmos. Chem. Phys., 22, 93–118, https://doi.org/10.5194/acp-22-93-2022, https://doi.org/10.5194/acp-22-93-2022, 2022
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The use of different spatio-temporal sulfur injection strategies with different magnitudes to create an artificial reflective aerosol layer to cool the climate is studied using sectional and modal aerosol schemes in a climate model. There are significant differences in the results depending on the aerosol microphysical module used. Different spatio-temporal injection strategies have a significant impact on the magnitude and zonal distribution of radiative forcing and atmospheric dynamics.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Dawn L. Woodard, Alexey N. Shiklomanov, Ben Kravitz, Corinne Hartin, and Ben Bond-Lamberty
Geosci. Model Dev., 14, 4751–4767, https://doi.org/10.5194/gmd-14-4751-2021, https://doi.org/10.5194/gmd-14-4751-2021, 2021
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We have added a representation of the permafrost carbon feedback to the simple, open-source global carbon–climate model Hector and calibrated the results to be consistent with historical data and Earth system model projections. Our results closely match previous work, estimating around 0.2 °C of warming from permafrost this century. This capability will be useful to explore uncertainties in this feedback and for coupling with integrated assessment models for policy and economic analysis.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Nikolas O. Aksamit, Ben Kravitz, Douglas G. MacMartin, and George Haller
Atmos. Chem. Phys., 21, 8845–8861, https://doi.org/10.5194/acp-21-8845-2021, https://doi.org/10.5194/acp-21-8845-2021, 2021
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There exist robust and influential material features evolving within turbulent fluids that behave as the skeleton for fluid transport pathways. Recent developments in applied mathematics have made the identification of these time-varying structures more rigorous and insightful than ever. Using short-range wind forecasts, we detail how and why these material features can be exploited in an effort to optimize the spread of aerosols in the stratosphere for climate geoengineering.
Henning Franke, Ulrike Niemeier, and Daniele Visioni
Atmos. Chem. Phys., 21, 8615–8635, https://doi.org/10.5194/acp-21-8615-2021, https://doi.org/10.5194/acp-21-8615-2021, 2021
Short summary
Short summary
Stratospheric aerosol modification (SAM) can alter the quasi-biennial oscillation (QBO). Our simulations with two different models show that the characteristics of the QBO response are primarily determined by the meridional structure of the aerosol-induced heating. Therefore, the QBO response to SAM depends primarily on the location of injection, while injection type and rate act to scale the specific response. Our results have important implications for evaluating adverse side effects of SAM.
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Short summary
The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of the atmospheric responses to stratospheric sulfate aerosol injections (SAIs) at various latitudes as simulated by three state-of-the-art Earth system models. We identify similarities and differences in the modeled aerosol burden, investigate the differences in the aerosol approaches between the models, and ultimately show the differences produced in surface climate, temperature and precipitation.
The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of...
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