Articles | Volume 23, issue 10
https://doi.org/10.5194/acp-23-5905-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-5905-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
30 May 2023
Research article |
| 30 May 2023
| 30 May 2023
Coupled mesoscale–microscale modeling of air quality in a polluted city using WRF-LES-Chem
Department of Civil and Environmental Engineering, the Hong Kong
Polytechnic University, Hung Hom, Kowloon, Hong Kong SAR, China
Department of Mechanics & Aerospace Engineering, Southern
University of Science and Technology, Shenzhen, 518055, China
Domingo Muñoz-Esparza
Research Applications Laboratory, National Center for Atmospheric
Research, Boulder, CO 80301, USA
Jianing Dai
Max Planck Institute for Meteorology, 20146 Hamburg, Germany
Cathy Wing Yi Li
Max Planck Institute for Meteorology, 20146 Hamburg, Germany
Pablo Lichtig
Max Planck Institute for Meteorology, 20146 Hamburg, Germany
Roy Chun-Wang Tsang
Environmental Protection Department, Wan Chai, Hong Kong SAR, China
Chun-Ho Liu
Department of Mechanical Engineering, The University of Hong Kong,
Pokfulam, Hong Kong SAR, China
Department of Civil and Environmental Engineering, the Hong Kong
Polytechnic University, Hung Hom, Kowloon, Hong Kong SAR, China
Guy Pierre Brasseur
Department of Civil and Environmental Engineering, the Hong Kong
Polytechnic University, Hung Hom, Kowloon, Hong Kong SAR, China
Max Planck Institute for Meteorology, 20146 Hamburg, Germany
Atmospheric Chemistry Observation & Modeling Laboratory, National
Center for Atmospheric Research, Boulder, CO 80301, USA
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Sinan Gao, Chunsong Lu, Yangang Liu, Seong Soo Yum, Jiashan Zhu, Lei Zhu, Neel Desai, Yongfeng Ma, and Shang Wu
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Revised manuscript not accepted
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Jianing Dai and Tao Wang
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Yuting Wang, Yong-Feng Ma, Domingo Muñoz-Esparza, Cathy W. Y. Li, Mary Barth, Tao Wang, and Guy P. Brasseur
Atmos. Chem. Phys., 21, 3531–3553, https://doi.org/10.5194/acp-21-3531-2021, https://doi.org/10.5194/acp-21-3531-2021, 2021
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James O. Pinto, Anders A. Jensen, Pedro A. Jiménez, Tracy Hertneky, Domingo Muñoz-Esparza, Arnaud Dumont, and Matthias Steiner
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Yujiao Zhu, Likun Xue, Jian Gao, Jianmin Chen, Hongyong Li, Yong Zhao, Zhaoxin Guo, Tianshu Chen, Liang Wen, Penggang Zheng, Ye Shan, Xinfeng Wang, Tao Wang, Xiaohong Yao, and Wenxing Wang
Atmos. Chem. Phys., 21, 1305–1323, https://doi.org/10.5194/acp-21-1305-2021, https://doi.org/10.5194/acp-21-1305-2021, 2021
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This work investigates the long-term changes in new particle formation (NPF) events under reduced SO2 emissions at the summit of Mt. Tai during seven campaigns from 2007 to 2018. We found the NPF intensity increased 2- to 3-fold in 2018 compared to 2007. In contrast, the probability of new particles growing to CCN size largely decreased. Changes to biogenic VOCs and anthropogenic emissions are proposed to explain the distinct NPF characteristics.
Cathy W. Y. Li, Guy P. Brasseur, Hauke Schmidt, and Juan Pedro Mellado
Atmos. Chem. Phys., 21, 483–503, https://doi.org/10.5194/acp-21-483-2021, https://doi.org/10.5194/acp-21-483-2021, 2021
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Intense and localised emissions of pollutants are common in urban environments, in which turbulence cannot mix these segregated pollutants efficiently in the atmosphere. Despite their relatively high resolution, regional models cannot resolve such segregation and assume instantaneous mixing of these pollutants in their model grids, which potentially induces significant error in the subsequent chemical calculation, based on our calculation with a model that explicitly resolves turbulent motions.
Zhenhao Ling, Qianqian Xie, Min Shao, Zhe Wang, Tao Wang, Hai Guo, and Xuemei Wang
Atmos. Chem. Phys., 20, 11451–11467, https://doi.org/10.5194/acp-20-11451-2020, https://doi.org/10.5194/acp-20-11451-2020, 2020
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The observation data from a receptor site in the Pearl River Delta region were analyzed by a photochemical box model with near-explicit chemical mechanisms (i.e., the Master Chemical Mechanism, MCM), improvements with reversible and irreversible heterogeneous processes of glyoxal and methylglyoxal, and the gas-particle partitioning of oxidation products in the present study.
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Short summary
Air quality in urban areas is difficult to simulate in coarse-resolution models. This work exploits the WRF (Weather Research and Forecasting) model coupled with a large-eddy simulation (LES) component and online chemistry to perform high-resolution (33.3 m) simulations of air quality in a large city. The evaluation of the simulations with observations shows that increased model resolution improves the representation of the chemical species near the pollution sources.
Air quality in urban areas is difficult to simulate in coarse-resolution models. This work...
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