Articles | Volume 17, issue 21
https://doi.org/10.5194/acp-17-13283-2017
https://doi.org/10.5194/acp-17-13283-2017
Research article
 | 
09 Nov 2017
Research article |  | 09 Nov 2017

Contributions of the troposphere and stratosphere to CH4 model biases

Zhiting Wang, Thorsten Warneke, Nicholas M. Deutscher, Justus Notholt, Ute Karstens, Marielle Saunois, Matthias Schneider, Ralf Sussmann, Harjinder Sembhi, David W. T. Griffith, Dave F. Pollard, Rigel Kivi, Christof Petri, Voltaire A. Velazco, Michel Ramonet, and Huilin Chen

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Cited articles

Alexe, M., Bergamaschi, P., Segers, A., Detmers, R., Butz, A., Hasekamp, O., Guerlet, S., Parker, R., Boesch, H., Frankenberg, C., Scheepmaker, R. A., Dlugokencky, E., Sweeney, C., Wofsy, S. C., and Kort, E. A.: Inverse modelling of CH4 emissions for 2010–2011 using different satellite retrieval products from GOSAT and SCIAMACHY, Atmos. Chem. Phys., 15, 113–133, https://doi.org/10.5194/acp-15-113-2015, 2015.
Bergamaschi, P., Houweling, S., Segers, A., Krol, M., Frankenberg, C., Scheepmaker, R. A., Dlugokencky, E., Wofsy, S. C., Kort, E. A., Sweeney, C., Schuck, T., Brenninkmeijer, C., Chen, H., Beck, V., and Gerbig, C.: Atmospheric CH4 in the first decade of the 21st century: Inverse modeling analysis using SCIAMACHY satellite retrievals and NOAA surface measurements, J. Geophys. Res., 118, 7350–7369, https://doi.org/10.1002/jgrd.50480, 2013.
Blumenstock, T., Hase, F., Schneider, M., García, O. E., and Sepúlveda, E.: TCCON data from Izana, Tenerife, Spain, Release GGG2014R0. TCCON data archive, hosted by the Carbon Dioxide Information Analysis Center, Oak Ridge Naional Laboratory, Oak Ridge, Tennessee, USA, https://doi.org/10.14291/tccon.ggg2014.izana01.R0/1149295, 2014.
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In this paper we separate the biases of atmospheric methane models into stratospheric and tropospheric parts. It is observed in other studies that simulated total columns of atmospheric methane present a latitudinal bias compared to measurements. The latitudinal gradients are considered to be from the stratosphere. However, our results show that the latitudinal biases could come from the troposphere in two of three models evaluated in this study.
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