Articles | Volume 23, issue 20
https://doi.org/10.5194/acp-23-13523-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-13523-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Evaluation of liquid cloud albedo susceptibility in E3SM using coupled eastern North Atlantic surface and satellite retrievals
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA
Po-Lun Ma
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA
Matthew W. Christensen
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA
Johannes Mülmenstädt
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA
Shuaiqi Tang
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA
Jerome Fast
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA
Related authors
Matthew W. Christensen, Andrew Geiss, Adam C. Varble, and Po-Lun Ma
EGUsphere, https://doi.org/10.5194/egusphere-2025-3850, https://doi.org/10.5194/egusphere-2025-3850, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We used satellite data and machine learning to better understand how tiny particles in the atmosphere affect clouds and their brightness. At higher spatial resolution, we discovered a new “M”-shaped pattern in the relationship between cloud water and droplet concentration unlike the inverted-V shape observed at coarsely gridded scales. Cloud water increases more with droplet concentration when rain is present. These findings support the development of next-generation atmospheric models.
Naser Mahfouz, Hassan Beydoun, Johannes Mülmenstädt, Noel Keen, Adam C. Varble, Luca Bertagna, Peter Bogenschutz, Andrew Bradley, Matthew W. Christensen, T. Conrad Clevenger, Aaron Donahue, Jerome Fast, James Foucar, Jean-Christophe Golaz, Oksana Guba, Walter Hannah, Benjamin Hillman, Robert Jacob, Wuyin Lin, Po-Lun Ma, Yun Qian, Balwinder Singh, Christopher Terai, Hailong Wang, Mingxuan Wu, Kai Zhang, Andrew Gettelman, Mark Taylor, L. Ruby Leung, Peter Caldwell, and Susannah Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2025-1868, https://doi.org/10.5194/egusphere-2025-1868, 2025
Short summary
Short summary
Our study assesses the aerosol effective radiative forcing in a global cloud-resolving atmosphere model at ultra-high resolution. We demonstrate that global ERFaer signal can be robustly reproduced across resolutions when aerosol activation processes are carefully parameterized. Further, we argue that simplified prescribed aerosol schemes will open the door for further process/mechanism studies under controlled conditions.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
Atmos. Chem. Phys., 24, 13633–13652, https://doi.org/10.5194/acp-24-13633-2024, https://doi.org/10.5194/acp-24-13633-2024, 2024
Short summary
Short summary
Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in dry, warm air, which can lead to cloud dissipation. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence have led us to conclude.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa Emmons
Atmos. Chem. Phys., 24, 13477–13502, https://doi.org/10.5194/acp-24-13477-2024, https://doi.org/10.5194/acp-24-13477-2024, 2024
Short summary
Short summary
Aerosol property measurements recently collected on the ground and by a research aircraft in central Argentina during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable data set needed to evaluate and improve model predictions of aerosols in a traditionally data-sparse region of South America.
Fan Mei, Jennifer M. Comstock, Mikhail S. Pekour, Jerome D. Fast, Krista L. Gaustad, Beat Schmid, Shuaiqi Tang, Damao Zhang, John E. Shilling, Jason M. Tomlinson, Adam C. Varble, Jian Wang, L. Ruby Leung, Lawrence Kleinman, Scot Martin, Sebastien C. Biraud, Brian D. Ermold, and Kenneth W. Burk
Earth Syst. Sci. Data, 16, 5429–5448, https://doi.org/10.5194/essd-16-5429-2024, https://doi.org/10.5194/essd-16-5429-2024, 2024
Short summary
Short summary
Our study explores a comprehensive dataset from airborne field studies (2013–2018) conducted using the US Department of Energy's Gulfstream 1 (G-1). The 236 flights span diverse regions, including the Arctic, US Southern Great Plains, US West Coast, eastern North Atlantic, Amazon Basin in Brazil, and Sierras de Córdoba range in Argentina. This dataset provides unique insights into atmospheric dynamics, aerosols, and clouds and makes data available in a more accessible format.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
Short summary
Short summary
Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Matthew W. Christensen, Peng Wu, Adam C. Varble, Heng Xiao, and Jerome D. Fast
Atmos. Chem. Phys., 24, 6455–6476, https://doi.org/10.5194/acp-24-6455-2024, https://doi.org/10.5194/acp-24-6455-2024, 2024
Short summary
Short summary
Clouds are essential to keep Earth cooler by reflecting sunlight back to space. We show that an increase in aerosol concentration suppresses precipitation in clouds, causing them to accumulate water and expand in a polluted environment with stronger turbulence and radiative cooling. This process enhances their reflectance by 51 %. It is therefore prudent to account for cloud fraction changes in assessments of aerosol–cloud interactions to improve predictions of climate change.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
Short summary
Short summary
Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Shuaiqi Tang, Adam C. Varble, Jerome D. Fast, Kai Zhang, Peng Wu, Xiquan Dong, Fan Mei, Mikhail Pekour, Joseph C. Hardin, and Po-Lun Ma
Geosci. Model Dev., 16, 6355–6376, https://doi.org/10.5194/gmd-16-6355-2023, https://doi.org/10.5194/gmd-16-6355-2023, 2023
Short summary
Short summary
To assess the ability of Earth system model (ESM) predictions, we developed a tool called ESMAC Diags to understand how aerosols, clouds, and aerosol–cloud interactions are represented in ESMs. This paper describes its version 2 functionality. We compared the model predictions with measurements taken by planes, ships, satellites, and ground instruments over four regions across the world. Results show that this new tool can help identify model problems and guide future development of ESMs.
Adam C. Varble, Adele L. Igel, Hugh Morrison, Wojciech W. Grabowski, and Zachary J. Lebo
Atmos. Chem. Phys., 23, 13791–13808, https://doi.org/10.5194/acp-23-13791-2023, https://doi.org/10.5194/acp-23-13791-2023, 2023
Short summary
Short summary
As atmospheric particles called aerosols increase in number, the number of droplets in clouds tends to increase, which has been theorized to increase storm intensity. We critically evaluate the evidence for this theory, showing that flaws and limitations of previous studies coupled with unaddressed cloud process complexities draw it into question. We provide recommendations for future observations and modeling to overcome current uncertainties.
Zhe Feng, Joseph Hardin, Hannah C. Barnes, Jianfeng Li, L. Ruby Leung, Adam Varble, and Zhixiao Zhang
Geosci. Model Dev., 16, 2753–2776, https://doi.org/10.5194/gmd-16-2753-2023, https://doi.org/10.5194/gmd-16-2753-2023, 2023
Short summary
Short summary
PyFLEXTRKR is a flexible atmospheric feature tracking framework with specific capabilities to track convective clouds from a variety of observations and model simulations. The package has a collection of multi-object identification algorithms and has been optimized for large datasets. This paper describes the algorithms and demonstrates applications for tracking deep convective cells and mesoscale convective systems from observations and model simulations at a wide range of scales.
Matthew W. Christensen, Po-Lun Ma, Peng Wu, Adam C. Varble, Johannes Mülmenstädt, and Jerome D. Fast
Atmos. Chem. Phys., 23, 2789–2812, https://doi.org/10.5194/acp-23-2789-2023, https://doi.org/10.5194/acp-23-2789-2023, 2023
Short summary
Short summary
An increase in aerosol concentration (tiny airborne particles) is shown to suppress rainfall and increase the abundance of droplets in clouds passing over Graciosa Island in the Azores. Cloud drops remain affected by aerosol for several days across thousands of kilometers in satellite data. Simulations from an Earth system model show good agreement, but differences in the amount of cloud water and its extent remain despite modifications to model parameters that control the warm-rain process.
Shuaiqi Tang, Jerome D. Fast, Kai Zhang, Joseph C. Hardin, Adam C. Varble, John E. Shilling, Fan Mei, Maria A. Zawadowicz, and Po-Lun Ma
Geosci. Model Dev., 15, 4055–4076, https://doi.org/10.5194/gmd-15-4055-2022, https://doi.org/10.5194/gmd-15-4055-2022, 2022
Short summary
Short summary
We developed an Earth system model (ESM) diagnostics package to compare various types of aerosol properties simulated in ESMs with aircraft, ship, and surface measurements from six field campaigns across spatial scales. The diagnostics package is coded and organized to be flexible and modular for future extension to other field campaign datasets and adapted to higher-resolution model simulations. Future releases will include comprehensive cloud and aerosol–cloud interaction diagnostics.
Matthew W. Christensen, Andrew Geiss, Adam C. Varble, and Po-Lun Ma
EGUsphere, https://doi.org/10.5194/egusphere-2025-3850, https://doi.org/10.5194/egusphere-2025-3850, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We used satellite data and machine learning to better understand how tiny particles in the atmosphere affect clouds and their brightness. At higher spatial resolution, we discovered a new “M”-shaped pattern in the relationship between cloud water and droplet concentration unlike the inverted-V shape observed at coarsely gridded scales. Cloud water increases more with droplet concentration when rain is present. These findings support the development of next-generation atmospheric models.
Dan Lubin, Xun Zou, Johannes Mülmenstädt, Andrew Vogelmann, Maria Cadeddu, and Damao Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2025-2768, https://doi.org/10.5194/egusphere-2025-2768, 2025
Short summary
Short summary
The US Department of Energy Atmospheric Radiation Measurement (ARM) North Slope of Alaska Facility has measured solar and atmospheric infrared radiation, and cloud properties, for the past 25 years. Statistically significant trends are emerging, including increasing infrared radiation due to a warming atmosphere, and decreasing solar radiation due to increasing liquid water content in clouds. These trends are influenced by large-scale atmospheric circulation patterns and by atmospheric rivers.
Robert S. Arthur, Alex Rybchuk, Timothy W. Juliano, Gabriel Rios, Sonia Wharton, Julie K. Lundquist, and Jerome D. Fast
Wind Energ. Sci., 10, 1187–1209, https://doi.org/10.5194/wes-10-1187-2025, https://doi.org/10.5194/wes-10-1187-2025, 2025
Short summary
Short summary
This paper evaluates a new model configuration for wind energy forecasting in complex terrain. We compare model results to observations in the Altamont Pass (California, USA), where wind channeling through a mountain gap leads to increased energy production. We demonstrate that the new model configuration performs similarly to a more established approach, with some evidence of improved wind speed predictions, and provide guidance for future model testing.
Naser Mahfouz, Hassan Beydoun, Johannes Mülmenstädt, Noel Keen, Adam C. Varble, Luca Bertagna, Peter Bogenschutz, Andrew Bradley, Matthew W. Christensen, T. Conrad Clevenger, Aaron Donahue, Jerome Fast, James Foucar, Jean-Christophe Golaz, Oksana Guba, Walter Hannah, Benjamin Hillman, Robert Jacob, Wuyin Lin, Po-Lun Ma, Yun Qian, Balwinder Singh, Christopher Terai, Hailong Wang, Mingxuan Wu, Kai Zhang, Andrew Gettelman, Mark Taylor, L. Ruby Leung, Peter Caldwell, and Susannah Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2025-1868, https://doi.org/10.5194/egusphere-2025-1868, 2025
Short summary
Short summary
Our study assesses the aerosol effective radiative forcing in a global cloud-resolving atmosphere model at ultra-high resolution. We demonstrate that global ERFaer signal can be robustly reproduced across resolutions when aerosol activation processes are carefully parameterized. Further, we argue that simplified prescribed aerosol schemes will open the door for further process/mechanism studies under controlled conditions.
Fan Mei, Qi Zhang, Damao Zhang, Jerome D. Fast, Gourihar Kulkarni, Mikhail S. Pekour, Christopher R. Niedek, Susanne Glienke, Israel Silber, Beat Schmid, Jason M. Tomlinson, Hardeep S. Mehta, Xena Mansoura, Zezhen Cheng, Gregory W. Vandergrift, Nurun Nahar Lata, Swarup China, and Zihua Zhu
Atmos. Chem. Phys., 25, 3425–3444, https://doi.org/10.5194/acp-25-3425-2025, https://doi.org/10.5194/acp-25-3425-2025, 2025
Short summary
Short summary
This study highlights the unique capability of the ArcticShark, an uncrewed aerial system, in measuring vertically resolved atmospheric properties. Data from 32 research flights in 2023 reveal seasonal patterns and correlations with conventional measurements. The consistency and complementarity of in situ and remote sensing methods are highlighted. The study demonstrates the ArcticShark’s versatility in bridging data gaps and improving the understanding of vertical atmospheric structures.
Andrew Geiss and Po-Lun Ma
Geosci. Model Dev., 18, 1809–1827, https://doi.org/10.5194/gmd-18-1809-2025, https://doi.org/10.5194/gmd-18-1809-2025, 2025
Short summary
Short summary
Particles in the Earth's atmosphere strongly impact the planet's energy budget, and atmosphere simulations require accurate representation of their interaction with light. This work introduces two approaches to represent light scattering by small particles. The first is a scattering simulator based on Mie theory implemented in Python. The second is a neural network emulator that is more accurate than existing methods and is fast enough to be used in climate and weather simulations.
Katherine M. Smith, Alice M. Barthel, LeAnn M. Conlon, Luke P. Van Roekel, Anthony Bartoletti, Jean-Christophe Golaz, Chengzhu Zhang, Carolyn Branecky Begeman, James J. Benedict, Gautam Bisht, Yan Feng, Walter Hannah, Bryce E. Harrop, Nicole Jeffery, Wuyin Lin, Po-Lun Ma, Mathew E. Maltrud, Mark R. Petersen, Balwinder Singh, Qi Tang, Teklu Tesfa, Jonathan D. Wolfe, Shaocheng Xie, Xue Zheng, Karthik Balaguru, Oluwayemi Garuba, Peter Gleckler, Aixue Hu, Jiwoo Lee, Ben Moore-Maley, and Ana C. Ordoñez
Geosci. Model Dev., 18, 1613–1633, https://doi.org/10.5194/gmd-18-1613-2025, https://doi.org/10.5194/gmd-18-1613-2025, 2025
Short summary
Short summary
Version 2.1 of the U.S. Department of Energy's Energy Exascale Earth System Model (E3SM) adds the Fox-Kemper et al. (2011) mixed-layer eddy parameterization, which restratifies the ocean surface layer through an overturning streamfunction. Results include surface layer bias reduction in temperature, salinity, and sea ice extent in the North Atlantic; a small strengthening of the Atlantic meridional overturning circulation; and improvements to many atmospheric climatological variables.
Brandon M. Duran, Casey J. Wall, Nicholas J. Lutsko, Takuro Michibata, Po-Lun Ma, Yi Qin, Margaret L. Duffy, Brian Medeiros, and Matvey Debolskiy
Atmos. Chem. Phys., 25, 2123–2146, https://doi.org/10.5194/acp-25-2123-2025, https://doi.org/10.5194/acp-25-2123-2025, 2025
Short summary
Short summary
We use satellite simulator data generated by global climate models to investigate how aerosol particles impact the radiative properties of liquid clouds. Specifically, we quantify the radiative perturbations arising from aerosol-driven changes in the number density of cloud droplets, the vertically integrated cloud water mass, and the cloud amount. Our results show that, in models, aerosol effects on the number density of cloud droplets contribute the most to anthropogenic climate forcing.
Sheng-Lun Tai, Zhao Yang, Brian Gaudet, Koichi Sakaguchi, Larry Berg, Colleen Kaul, Yun Qian, Ye Liu, and Jerome Fast
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-599, https://doi.org/10.5194/essd-2024-599, 2025
Revised manuscript accepted for ESSD
Short summary
Short summary
Our study created a high-resolution soil moisture dataset for the eastern U.S. by integrating satellite data with a land surface model and advanced algorithms, achieving 1-km scale analyses. Validated against multiple networks and datasets, it demonstrated superior accuracy. This dataset is vital for understanding soil moisture dynamics, especially during droughts, and highlights the need for improved modeling of clay soils to refine future predictions.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
Atmos. Chem. Phys., 24, 13633–13652, https://doi.org/10.5194/acp-24-13633-2024, https://doi.org/10.5194/acp-24-13633-2024, 2024
Short summary
Short summary
Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in dry, warm air, which can lead to cloud dissipation. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence have led us to conclude.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa Emmons
Atmos. Chem. Phys., 24, 13477–13502, https://doi.org/10.5194/acp-24-13477-2024, https://doi.org/10.5194/acp-24-13477-2024, 2024
Short summary
Short summary
Aerosol property measurements recently collected on the ground and by a research aircraft in central Argentina during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable data set needed to evaluate and improve model predictions of aerosols in a traditionally data-sparse region of South America.
Fan Mei, Jennifer M. Comstock, Mikhail S. Pekour, Jerome D. Fast, Krista L. Gaustad, Beat Schmid, Shuaiqi Tang, Damao Zhang, John E. Shilling, Jason M. Tomlinson, Adam C. Varble, Jian Wang, L. Ruby Leung, Lawrence Kleinman, Scot Martin, Sebastien C. Biraud, Brian D. Ermold, and Kenneth W. Burk
Earth Syst. Sci. Data, 16, 5429–5448, https://doi.org/10.5194/essd-16-5429-2024, https://doi.org/10.5194/essd-16-5429-2024, 2024
Short summary
Short summary
Our study explores a comprehensive dataset from airborne field studies (2013–2018) conducted using the US Department of Energy's Gulfstream 1 (G-1). The 236 flights span diverse regions, including the Arctic, US Southern Great Plains, US West Coast, eastern North Atlantic, Amazon Basin in Brazil, and Sierras de Córdoba range in Argentina. This dataset provides unique insights into atmospheric dynamics, aerosols, and clouds and makes data available in a more accessible format.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
Short summary
Short summary
We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
Short summary
Short summary
Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Naser Mahfouz, Johannes Mülmenstädt, and Susannah Burrows
Atmos. Chem. Phys., 24, 7253–7260, https://doi.org/10.5194/acp-24-7253-2024, https://doi.org/10.5194/acp-24-7253-2024, 2024
Short summary
Short summary
Climate models are our primary tool to probe past, present, and future climate states unlike the more recent observation record. By constructing a hypothetical model configuration, we show that present-day correlations are insufficient to predict a persistent uncertainty in climate projection (how much sun because clouds will reflect in a changing climate). We hope our result will contribute to the scholarly conversation on better utilizing observations to constrain climate uncertainties.
Matthew W. Christensen, Peng Wu, Adam C. Varble, Heng Xiao, and Jerome D. Fast
Atmos. Chem. Phys., 24, 6455–6476, https://doi.org/10.5194/acp-24-6455-2024, https://doi.org/10.5194/acp-24-6455-2024, 2024
Short summary
Short summary
Clouds are essential to keep Earth cooler by reflecting sunlight back to space. We show that an increase in aerosol concentration suppresses precipitation in clouds, causing them to accumulate water and expand in a polluted environment with stronger turbulence and radiative cooling. This process enhances their reflectance by 51 %. It is therefore prudent to account for cloud fraction changes in assessments of aerosol–cloud interactions to improve predictions of climate change.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
Short summary
Short summary
Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Taufiq Hassan, Kai Zhang, Jianfeng Li, Balwinder Singh, Shixuan Zhang, Hailong Wang, and Po-Lun Ma
Geosci. Model Dev., 17, 3507–3532, https://doi.org/10.5194/gmd-17-3507-2024, https://doi.org/10.5194/gmd-17-3507-2024, 2024
Short summary
Short summary
Anthropogenic aerosol emissions are an essential part of global aerosol models. Significant errors can exist from the loss of emission heterogeneity. We introduced an emission treatment that significantly improved aerosol emission heterogeneity in high-resolution model simulations, with improvements in simulated aerosol surface concentrations. The emission treatment will provide a more accurate representation of aerosol emissions and their effects on climate.
Yu Yao, Po-Lun Ma, Yi Qin, Matthew W. Christensen, Hui Wan, Kai Zhang, Balwinder Singh, Meng Huang, and Mikhail Ovchinnikov
EGUsphere, https://doi.org/10.5194/egusphere-2024-523, https://doi.org/10.5194/egusphere-2024-523, 2024
Preprint withdrawn
Short summary
Short summary
Giant aerosols have substantial effects on warm rain formation. However, it remains challenging to quantify the impact of giant particles at global scale. In this work, we applied earth system model to investigate its impacts by implementing new giant aerosol treatments to consider its physical process. We found this approach substantially affect liquid cloud and improved model's precipitation response to aerosols. Our findings demonstrate the significant impact of giant aerosols on climate.
Kirsten L. Findell, Zun Yin, Eunkyo Seo, Paul A. Dirmeyer, Nathan P. Arnold, Nathaniel Chaney, Megan D. Fowler, Meng Huang, David M. Lawrence, Po-Lun Ma, and Joseph A. Santanello Jr.
Geosci. Model Dev., 17, 1869–1883, https://doi.org/10.5194/gmd-17-1869-2024, https://doi.org/10.5194/gmd-17-1869-2024, 2024
Short summary
Short summary
We outline a request for sub-daily data to accurately capture the process-level connections between land states, surface fluxes, and the boundary layer response. This high-frequency model output will allow for more direct comparison with observational field campaigns on process-relevant timescales, enable demonstration of inter-model spread in land–atmosphere coupling processes, and aid in targeted identification of sources of deficiencies and opportunities for improvement of the models.
Jianfeng Li, Kai Zhang, Taufiq Hassan, Shixuan Zhang, Po-Lun Ma, Balwinder Singh, Qiyang Yan, and Huilin Huang
Geosci. Model Dev., 17, 1327–1347, https://doi.org/10.5194/gmd-17-1327-2024, https://doi.org/10.5194/gmd-17-1327-2024, 2024
Short summary
Short summary
By comparing E3SM simulations with and without regional refinement, we find that model horizontal grid spacing considerably affects the simulated aerosol mass budget, aerosol–cloud interactions, and the effective radiative forcing of anthropogenic aerosols. The study identifies the critical physical processes strongly influenced by model resolution. It also highlights the benefit of applying regional refinement in future modeling studies at higher or even convection-permitting resolutions.
Yuying Zhang, Shaocheng Xie, Yi Qin, Wuyin Lin, Jean-Christophe Golaz, Xue Zheng, Po-Lun Ma, Yun Qian, Qi Tang, Christopher R. Terai, and Meng Zhang
Geosci. Model Dev., 17, 169–189, https://doi.org/10.5194/gmd-17-169-2024, https://doi.org/10.5194/gmd-17-169-2024, 2024
Short summary
Short summary
We performed systematic evaluation of clouds simulated in the Energy
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Yang Wang, Chanakya Bagya Ramesh, Scott E. Giangrande, Jerome Fast, Xianda Gong, Jiaoshi Zhang, Ahmet Tolga Odabasi, Marcus Vinicius Batista Oliveira, Alyssa Matthews, Fan Mei, John E. Shilling, Jason Tomlinson, Die Wang, and Jian Wang
Atmos. Chem. Phys., 23, 15671–15691, https://doi.org/10.5194/acp-23-15671-2023, https://doi.org/10.5194/acp-23-15671-2023, 2023
Short summary
Short summary
We report the vertical profiles of aerosol properties over the Southern Great Plains (SGP), a region influenced by shallow convective clouds, land–atmosphere interactions, boundary layer turbulence, and the aerosol life cycle. We examined the processes that drive the aerosol population and distribution in the lower troposphere over the SGP. This study helps improve our understanding of aerosol–cloud interactions and the model representation of aerosol processes.
Shuaiqi Tang, Adam C. Varble, Jerome D. Fast, Kai Zhang, Peng Wu, Xiquan Dong, Fan Mei, Mikhail Pekour, Joseph C. Hardin, and Po-Lun Ma
Geosci. Model Dev., 16, 6355–6376, https://doi.org/10.5194/gmd-16-6355-2023, https://doi.org/10.5194/gmd-16-6355-2023, 2023
Short summary
Short summary
To assess the ability of Earth system model (ESM) predictions, we developed a tool called ESMAC Diags to understand how aerosols, clouds, and aerosol–cloud interactions are represented in ESMs. This paper describes its version 2 functionality. We compared the model predictions with measurements taken by planes, ships, satellites, and ground instruments over four regions across the world. Results show that this new tool can help identify model problems and guide future development of ESMs.
Adam C. Varble, Adele L. Igel, Hugh Morrison, Wojciech W. Grabowski, and Zachary J. Lebo
Atmos. Chem. Phys., 23, 13791–13808, https://doi.org/10.5194/acp-23-13791-2023, https://doi.org/10.5194/acp-23-13791-2023, 2023
Short summary
Short summary
As atmospheric particles called aerosols increase in number, the number of droplets in clouds tends to increase, which has been theorized to increase storm intensity. We critically evaluate the evidence for this theory, showing that flaws and limitations of previous studies coupled with unaddressed cloud process complexities draw it into question. We provide recommendations for future observations and modeling to overcome current uncertainties.
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
Short summary
Short summary
Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
Chupeng Zhang, Shangfei Hai, Yang Gao, Yuhang Wang, Shaoqing Zhang, Lifang Sheng, Bin Zhao, Shuxiao Wang, Jingkun Jiang, Xin Huang, Xiaojing Shen, Junying Sun, Aura Lupascu, Manish Shrivastava, Jerome D. Fast, Wenxuan Cheng, Xiuwen Guo, Ming Chu, Nan Ma, Juan Hong, Qiaoqiao Wang, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 23, 10713–10730, https://doi.org/10.5194/acp-23-10713-2023, https://doi.org/10.5194/acp-23-10713-2023, 2023
Short summary
Short summary
New particle formation is an important source of atmospheric particles, exerting critical influences on global climate. Numerical models are vital tools to understanding atmospheric particle evolution, which, however, suffer from large biases in simulating particle numbers. Here we improve the model chemical processes governing particle sizes and compositions. The improved model reveals substantial contributions of newly formed particles to climate through effects on cloud condensation nuclei.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
Short summary
Short summary
Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Aishwarya Raman, Thomas Hill, Paul J. DeMott, Balwinder Singh, Kai Zhang, Po-Lun Ma, Mingxuan Wu, Hailong Wang, Simon P. Alexander, and Susannah M. Burrows
Atmos. Chem. Phys., 23, 5735–5762, https://doi.org/10.5194/acp-23-5735-2023, https://doi.org/10.5194/acp-23-5735-2023, 2023
Short summary
Short summary
Ice-nucleating particles (INPs) play an important role in cloud processes and associated precipitation. Yet, INPs are not accurately represented in climate models. This study attempts to uncover these gaps by comparing model-simulated INP concentrations against field campaign measurements in the SO for an entire year, 2017–2018. Differences in INP concentrations and variability between the model and observations have major implications for modeling cloud properties in high latitudes.
Zhe Feng, Joseph Hardin, Hannah C. Barnes, Jianfeng Li, L. Ruby Leung, Adam Varble, and Zhixiao Zhang
Geosci. Model Dev., 16, 2753–2776, https://doi.org/10.5194/gmd-16-2753-2023, https://doi.org/10.5194/gmd-16-2753-2023, 2023
Short summary
Short summary
PyFLEXTRKR is a flexible atmospheric feature tracking framework with specific capabilities to track convective clouds from a variety of observations and model simulations. The package has a collection of multi-object identification algorithms and has been optimized for large datasets. This paper describes the algorithms and demonstrates applications for tracking deep convective cells and mesoscale convective systems from observations and model simulations at a wide range of scales.
Andrew Geiss, Po-Lun Ma, Balwinder Singh, and Joseph C. Hardin
Geosci. Model Dev., 16, 2355–2370, https://doi.org/10.5194/gmd-16-2355-2023, https://doi.org/10.5194/gmd-16-2355-2023, 2023
Short summary
Short summary
Atmospheric aerosols play a critical role in Earth's climate, but it is too computationally expensive to directly model their interaction with radiation in climate simulations. This work develops a new neural-network-based parameterization of aerosol optical properties for use in the Energy Exascale Earth System Model that is much more accurate than the current one; it also introduces a unique model optimization method that involves randomly generating neural network architectures.
William K. Jones, Matthew W. Christensen, and Philip Stier
Atmos. Meas. Tech., 16, 1043–1059, https://doi.org/10.5194/amt-16-1043-2023, https://doi.org/10.5194/amt-16-1043-2023, 2023
Short summary
Short summary
Geostationary weather satellites have been used to detect storm clouds since their earliest applications. However, this task remains difficult as imaging satellites cannot observe the strong vertical winds that are characteristic of storm clouds. Here we introduce a new method that allows us to detect the early development of storms and continue to track them throughout their lifetime, allowing us to study how their early behaviour affects subsequent weather.
Matthew W. Christensen, Po-Lun Ma, Peng Wu, Adam C. Varble, Johannes Mülmenstädt, and Jerome D. Fast
Atmos. Chem. Phys., 23, 2789–2812, https://doi.org/10.5194/acp-23-2789-2023, https://doi.org/10.5194/acp-23-2789-2023, 2023
Short summary
Short summary
An increase in aerosol concentration (tiny airborne particles) is shown to suppress rainfall and increase the abundance of droplets in clouds passing over Graciosa Island in the Azores. Cloud drops remain affected by aerosol for several days across thousands of kilometers in satellite data. Simulations from an Earth system model show good agreement, but differences in the amount of cloud water and its extent remain despite modifications to model parameters that control the warm-rain process.
Marine Bonazzola, Hélène Chepfer, Po-Lun Ma, Johannes Quaas, David M. Winker, Artem Feofilov, and Nick Schutgens
Geosci. Model Dev., 16, 1359–1377, https://doi.org/10.5194/gmd-16-1359-2023, https://doi.org/10.5194/gmd-16-1359-2023, 2023
Short summary
Short summary
Aerosol has a large impact on climate. Using a lidar aerosol simulator ensures consistent comparisons between modeled and observed aerosol. We present a lidar aerosol simulator that applies a cloud masking and an aerosol detection threshold. We estimate the lidar signals that would be observed at 532 nm by the Cloud-Aerosol Lidar with Orthogonal Polarization overflying the atmosphere predicted by a climate model. Our comparison at the seasonal timescale shows a discrepancy in the Southern Ocean.
Siegfried Schobesberger, Emma L. D'Ambro, Lejish Vettikkat, Ben H. Lee, Qiaoyun Peng, David M. Bell, John E. Shilling, Manish Shrivastava, Mikhail Pekour, Jerome Fast, and Joel A. Thornton
Atmos. Meas. Tech., 16, 247–271, https://doi.org/10.5194/amt-16-247-2023, https://doi.org/10.5194/amt-16-247-2023, 2023
Short summary
Short summary
We present a new, highly sensitive technique for measuring atmospheric ammonia, an important trace gas that is emitted mainly by agriculture. We deployed the instrument on an aircraft during research flights over rural Oklahoma. Due to its fast response, we could analyze correlations with turbulent winds and calculate ammonia emissions from nearby areas at 1 to 2 km resolution. We observed high spatial variability and point sources that are not resolved in the US National Emissions Inventory.
Jerome D. Fast, David M. Bell, Gourihar Kulkarni, Jiumeng Liu, Fan Mei, Georges Saliba, John E. Shilling, Kaitlyn Suski, Jason Tomlinson, Jian Wang, Rahul Zaveri, and Alla Zelenyuk
Atmos. Chem. Phys., 22, 11217–11238, https://doi.org/10.5194/acp-22-11217-2022, https://doi.org/10.5194/acp-22-11217-2022, 2022
Short summary
Short summary
Recent aircraft measurements from the HI-SCALE campaign conducted over the Southern Great Plains (SGP) site in Oklahoma are used to quantify spatial variability of aerosol properties in terms of grid spacings typically used by weather and climate models. Surprisingly large horizontal gradients in aerosol properties were frequently observed in this rural area. This spatial variability can be used as an uncertainty range when comparing surface point measurements with model predictions.
Meng Huang, Po-Lun Ma, Nathaniel W. Chaney, Dalei Hao, Gautam Bisht, Megan D. Fowler, Vincent E. Larson, and L. Ruby Leung
Geosci. Model Dev., 15, 6371–6384, https://doi.org/10.5194/gmd-15-6371-2022, https://doi.org/10.5194/gmd-15-6371-2022, 2022
Short summary
Short summary
The land surface in one grid cell may be diverse in character. This study uses an explicit way to account for that subgrid diversity in a state-of-the-art Earth system model (ESM) and explores its implications for the overlying atmosphere. We find that the shallow clouds are increased significantly with the land surface diversity. Our work highlights the importance of accurately representing the land surface and its interaction with the atmosphere in next-generation ESMs.
Bernd Heinold, Holger Baars, Boris Barja, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Nick Schutgens, Fabian Senf, Roland Schrödner, Diego Villanueva, and Ina Tegen
Atmos. Chem. Phys., 22, 9969–9985, https://doi.org/10.5194/acp-22-9969-2022, https://doi.org/10.5194/acp-22-9969-2022, 2022
Short summary
Short summary
The extreme 2019–2020 Australian wildfires produced massive smoke plumes lofted into the lower stratosphere by pyrocumulonimbus convection. Most climate models do not adequately simulate the injection height of such intense fires. By combining aerosol-climate modeling with prescribed pyroconvective smoke injection and lidar observations, this study shows the importance of the representation of the most extreme wildfire events for estimating the atmospheric energy budget.
Fan Mei, Mikhail S. Pekour, Darielle Dexheimer, Gijs de Boer, RaeAnn Cook, Jason Tomlinson, Beat Schmid, Lexie A. Goldberger, Rob Newsom, and Jerome D. Fast
Earth Syst. Sci. Data, 14, 3423–3438, https://doi.org/10.5194/essd-14-3423-2022, https://doi.org/10.5194/essd-14-3423-2022, 2022
Short summary
Short summary
This work focuses on an expanding number of data sets observed using ARM TBS (133 flights) and UAS (seven flights) platforms by the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility. These data streams provide new perspectives on spatial variability of atmospheric and surface parameters, helping to address critical science questions in Earth system science research, such as the aerosol–cloud interaction in the boundary layer.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
Short summary
Short summary
Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Shuaiqi Tang, Jerome D. Fast, Kai Zhang, Joseph C. Hardin, Adam C. Varble, John E. Shilling, Fan Mei, Maria A. Zawadowicz, and Po-Lun Ma
Geosci. Model Dev., 15, 4055–4076, https://doi.org/10.5194/gmd-15-4055-2022, https://doi.org/10.5194/gmd-15-4055-2022, 2022
Short summary
Short summary
We developed an Earth system model (ESM) diagnostics package to compare various types of aerosol properties simulated in ESMs with aircraft, ship, and surface measurements from six field campaigns across spatial scales. The diagnostics package is coded and organized to be flexible and modular for future extension to other field campaign datasets and adapted to higher-resolution model simulations. Future releases will include comprehensive cloud and aerosol–cloud interaction diagnostics.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
Short summary
Short summary
Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
Short summary
Short summary
An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Artem G. Feofilov, Hélène Chepfer, Vincent Noël, Rodrigo Guzman, Cyprien Gindre, Po-Lun Ma, and Marjolaine Chiriaco
Atmos. Meas. Tech., 15, 1055–1074, https://doi.org/10.5194/amt-15-1055-2022, https://doi.org/10.5194/amt-15-1055-2022, 2022
Short summary
Short summary
Space-borne lidars have been providing invaluable information of atmospheric optical properties since 2006, and new lidar missions are on the way to ensure continuous observations. In this work, we compare the clouds estimated from space-borne ALADIN and CALIOP lidar observations. The analysis of collocated data shows that the agreement between the retrieved clouds is good up to 3 km height. Above that, ALADIN detects 40 % less clouds than CALIOP, except for polar stratospheric clouds (PSCs).
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
Short summary
Short summary
Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Zhonghua Zheng, Matthew West, Lei Zhao, Po-Lun Ma, Xiaohong Liu, and Nicole Riemer
Atmos. Chem. Phys., 21, 17727–17741, https://doi.org/10.5194/acp-21-17727-2021, https://doi.org/10.5194/acp-21-17727-2021, 2021
Short summary
Short summary
Aerosol mixing state is an important emergent property that affects aerosol radiative forcing and aerosol–cloud interactions, but it has not been easy to constrain this property globally. We present a framework for evaluating the error in aerosol mixing state induced by aerosol representation assumptions, which is one of the important contributors to structural uncertainty in aerosol models. Our study provides insights into potential improvements to model process representation for aerosols.
Raghavendra Krishnamurthy, Rob K. Newsom, Larry K. Berg, Heng Xiao, Po-Lun Ma, and David D. Turner
Atmos. Meas. Tech., 14, 4403–4424, https://doi.org/10.5194/amt-14-4403-2021, https://doi.org/10.5194/amt-14-4403-2021, 2021
Short summary
Short summary
Planetary boundary layer (PBL) height is a critical parameter in atmospheric models. Continuous PBL height measurements from remote sensing measurements are important to understand various boundary layer mechanisms, especially during daytime and evening transition periods. Due to several limitations in existing methodologies to detect PBL height from a Doppler lidar, in this study, a machine learning (ML) approach is tested. The ML model is observed to improve the accuracy by over 50 %.
Sam J. Silva, Po-Lun Ma, Joseph C. Hardin, and Daniel Rothenberg
Geosci. Model Dev., 14, 3067–3077, https://doi.org/10.5194/gmd-14-3067-2021, https://doi.org/10.5194/gmd-14-3067-2021, 2021
Short summary
Short summary
The activation of aerosol into cloud droplets is an important but uncertain process in the Earth system. The physical and chemical interactions that govern this process are too computationally expensive to explicitly resolve in modern Earth system models. Here, we demonstrate how hybrid machine learning approaches can provide a potential path forward, enabling the representation of the more detailed physics and chemistry at a reduced computational cost while still retaining physical information.
Maria A. Zawadowicz, Kaitlyn Suski, Jiumeng Liu, Mikhail Pekour, Jerome Fast, Fan Mei, Arthur J. Sedlacek, Stephen Springston, Yang Wang, Rahul A. Zaveri, Robert Wood, Jian Wang, and John E. Shilling
Atmos. Chem. Phys., 21, 7983–8002, https://doi.org/10.5194/acp-21-7983-2021, https://doi.org/10.5194/acp-21-7983-2021, 2021
Short summary
Short summary
This paper describes the results of a recent field campaign in the eastern North Atlantic, where two mass spectrometers were deployed aboard a research aircraft to measure the chemistry of aerosols and trace gases. Very clean conditions were found, dominated by local sulfate-rich acidic aerosol and very aged organics. Evidence of
long-range transport of aerosols from the continents was also identified.
Jiumeng Liu, Liz Alexander, Jerome D. Fast, Rodica Lindenmaier, and John E. Shilling
Atmos. Chem. Phys., 21, 5101–5116, https://doi.org/10.5194/acp-21-5101-2021, https://doi.org/10.5194/acp-21-5101-2021, 2021
Short summary
Short summary
To bridge the gaps in modeling and observational results due to insufficient understanding of aerosol properties, co-located measurements of aerosols and trace gases were conducted at SGP during the HI-SCALE campaign. Organic aerosols at the SGP site exhibited to be highly oxidized, and biogenic emissions appear to largely control the formation of organic aerosols. Seasonal variations of sources and meteorological impacts likely resulted in the highly oxygenated feature of aerosols.
Jingyu Wang, Jiwen Fan, Robert A. Houze Jr., Stella R. Brodzik, Kai Zhang, Guang J. Zhang, and Po-Lun Ma
Geosci. Model Dev., 14, 719–734, https://doi.org/10.5194/gmd-14-719-2021, https://doi.org/10.5194/gmd-14-719-2021, 2021
Short summary
Short summary
This paper presents an evaluation of the E3SM model against NEXRAD radar observations for the warm seasons during 2014–2016. The COSP forward simulator package is implemented in the model to generate radar reflectivity, and the NEXRAD observations are coarsened to the model resolution for comparison. The model severely underestimates the reflectivity above 4 km. Sensitivity tests on the parameters from cumulus parameterization and cloud microphysics do not improve this model bias.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
Short summary
Short summary
Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Laura Palacios-Peña, Jerome D. Fast, Enrique Pravia-Sarabia, and Pedro Jiménez-Guerrero
Geosci. Model Dev., 13, 5897–5915, https://doi.org/10.5194/gmd-13-5897-2020, https://doi.org/10.5194/gmd-13-5897-2020, 2020
Short summary
Short summary
The main objective of this work is to study the impact of the representation of aerosol size distribution on aerosol optical properties over central Europe and the Mediterranean Basin during a summertime aerosol episode using the WRF-Chem online model. Results reveal that the reduction in the standard deviation of the accumulation mode leads to the largest impacts on aerosol optical depth (AOD) representation due to a transfer of particles from the accumulation mode to the coarse mode.
Peter A. Bogenschutz, Shuaiqi Tang, Peter M. Caldwell, Shaocheng Xie, Wuyin Lin, and Yao-Sheng Chen
Geosci. Model Dev., 13, 4443–4458, https://doi.org/10.5194/gmd-13-4443-2020, https://doi.org/10.5194/gmd-13-4443-2020, 2020
Short summary
Short summary
This paper documents a tool that has been developed that can be used to accelerate the development and understanding of climate models. This version of the model, known as a the single-column model, is much faster to run than the full climate model, and we demonstrate that this tool can be used to quickly exploit model biases that arise due to physical processes. We show examples of how this single-column model can directly benefit the field.
Caroline A. Poulsen, Gregory R. McGarragh, Gareth E. Thomas, Martin Stengel, Matthew W. Christensen, Adam C. Povey, Simon R. Proud, Elisa Carboni, Rainer Hollmann, and Roy G. Grainger
Earth Syst. Sci. Data, 12, 2121–2135, https://doi.org/10.5194/essd-12-2121-2020, https://doi.org/10.5194/essd-12-2121-2020, 2020
Short summary
Short summary
We have created a satellite cloud and radiation climatology from the ATSR-2 and AATSR on board ERS-2 and Envisat, respectively, which spans the period 1995–2012. The data set was created using a combination of optimal estimation and neural net techniques. The data set was created as part of the ESA Climate Change Initiative program. The data set has been compared with active CALIOP lidar measurements and compared with MAC-LWP AND CERES-EBAF measurements and is shown to have good performance.
Cited articles
Abdul-Razzak, H. and Ghan, S. J.: A parameterization of aerosol activation: 2. Multiple aerosol types, J. Geophys. Res., 105, 6837–6844, https://doi.org/10.1029/1999JD901161, 2000.
Ackerman, A. S., Kirkpatrick, M. P., Stevens, D. E., and Toon, O. B.: The impact of humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432, 1014–1017, https://doi.org/10.1038/nature03174, 2004.
Albrecht, B. A.: Aerosols, Cloud Microphysics, and Fractional Cloudiness, Science, 245, 1227–1230, https://doi.org/10.1126/science.245.4923.1227, 1989.
ARM – Atmospheric Radiation Measurement user facility: Interpolated Sonde (INTERPOLATEDSONDE), 2016-01-01 to 2020-12-31, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Jensen, M., Giangrande, S., Fairless, T., and Zhou, A., ARM Data Center [data set], https://doi.org/10.5439/1095316, 2013a.
ARM – Atmospheric Radiation Measurement user facility: Minnis Cloud Products Using Visst Algorithm (VISSTGRIDM10MINNIS), 2016-01-01 to 2018-02-20, Eastern North Atlantic (ENA) External Data (satellites and others) (X1), ARM Data Center [data set], https://adc.arm.gov/discovery/#/results/datastream::enavisstgridm10minnisX1.c1 (last access: 12 August 2021), 2013b.
ARM – Atmospheric Radiation Measurement user facility: Surface Meteorological Instrumentation (MET), 2016-01-01 to 2020-12-31, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Kyrouac J., and Shi, Y., ARM Data Center [data set], https://doi.org/10.5439/1786358, 2013c.
ARM – Atmospheric Radiation Measurement user facility: Cloud Optical Properties from MFRSR Using Min Algorithm (MFRSRCLDOD1MIN), 2016-01-01 to 2020-12-31, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Zhang, D., ARM Data Center [data set], https://doi.org/10.5439/1027296, 2014a.
ARM – Atmospheric Radiation Measurement user facility: Laser Disdrometer Quantities (LDQUANTS), 2016-01-01 to 2020-12-31, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Hardin, J., Giangrande, S., and Zhou, A., ARM Data Center [data set], https://doi.org/10.5439/1432694, 2014b.
ARM – Atmospheric Radiation Measurement user facility: Minnis Cloud Products Using Visst Algorithm (VISSTPXM10MINNIS), 2016-01-01 to 2018-02-20, Eastern North Atlantic (EN) External Data (satellites and others) (X1), ARM Data Center [data set], https://adc.arm.gov/discovery/#/results/datastream::enavisstpx2dm10minnisX1.c1 (last access: 12 August 2021), 2014c.
ARM – Atmospheric Radiation Measurement user facility: MWR Retrievals with MWRRET Version 2 (MWRRET2TURN), 2016-01-01 to 2020-12-31, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Gaustad, K., ARM Data Center [data set], https://doi.org/10.5439/1566156, 2014d.
ARM – Atmospheric Radiation Measurement user facility: Active Remote Sensing of CLouds (ARSCL) product using Ka-band ARM Zenith Radars (ARSCLKAZRBND1KOLLIAS), 2016-01-01 to 2020-12-31, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Johnson, K., Giangrande, S., and Toto, T., ARM Data Center [data set], https://doi.org/10.5439/1393438, 2015.
ARM – Atmospheric Radiation Measurement user facility: Cloud Condensation Nuclei Particle Counter (AOSCCN1COLAVG), 2016-06-22 to 2020-10-28, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Koontz, A. and Flynn, C., ARM Data Center [data set], https://doi.org/10.5439/1255094, 2016a.
ARM – Atmospheric Radiation Measurement user facility: Cloud Condensation Nuclei Particle Counter (AOSCCN1COLSPECTRA), 2016-06-22 to 2020-10-28, Eastern North Atlantic (ENA) Graciosa Island, Azores, Portugal (C1), compiled by: Uin, J., ARM Data Center [data set], https://doi.org/10.5439/1342134, 2016b.
ARM – Atmospheric Radiation Measurement user facility: Minnis Cloud Products Using Visst Algorithm (VISSTGRIDM11MINNIS), 2018-02-20 to 2020-12-31, Eastern North Atlantic (EN) External Data (satellites and others) (X1), ARM Data Center [data set], https://adc.arm.gov/discovery/#/results/datastream::enavisstgridm11minnisX1.c1 (last access: 12 August 2021), 2018a.
ARM – Atmospheric Radiation Measurement user facility: Minnis Cloud Products Using Visst Algorithm (VISSTPX2DM11MINNIS), 2018-02-20 to 2020-12-31, Eastern North Atlantic (ENA) External Data (satellites and others) (X1), ARM Data Center [data set], https://adc.arm.gov/discovery/#/results/datastream::enavisstpx2dm11minnisX1.c1 (last access: 12 August 2021), 2018b.
Bellouin, N., Quaas, J., Gryspeerdt, E., Kinne, D., Stier, P., Watson-Parris, D., Boucher, O., Carslaw, K. S., Christensen, M., Daniau, A.-L., Dufresne, J.-L., Feingold, G., Fiedler, S., Forster, P., Gettelman, A., Haywood, J. M., Lohmann, U., Malavelle, F., Mauritsen, T., McCoy, D. T., Myhre, G., Mülmenstädt, J., Neubauer, D., Possner, A., Rugenstein, M., Sato, Y., Schulz, M., Schwartz, S. E., Sourdeval, O., Storelvmo, T., Toll, V., Winker, D., and Stevens, B.: Bounding global aerosol radiative forcing of climate change, Rev. Geophys., 58, e2019RG000660, https://doi.org/10.1029/2019RG000660, 2020.
Bennartz, R.: Global assessment of marine boundary layer cloud droplet number concentration from satellite, J. Geophys. Res.-Atmos., 112, D02201, https://doi.org/10.1029/2006JD007547, 2007.
Bodas-Salcedo, A., Webb, M. J., Bony, S., Chepfer, H., Dufresne, J.-L., Klein, S. A., Zhang, Y., Marchand, R., Haynes, J. M., Pincus, R., and John, V. O.: COSP: Satellite simulation software for model assessment, B. Am. Meteorol. Soc., 92, 1023–1043, https://doi.org/10.1175/2011BAMS2856.1, 2011.
Boers, R. and Mitchell, R. M.: Absorption feedback in stratocumulus clouds influence on cloud top albedo, Tellus A, 46, 229–241, https://doi.org/10.1034/j.1600-0870.1994.00001.x, 1994.
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster, P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S., Sherwood, S., Stevens, B., and Zhang, X.: Clouds and aerosols, in: Climate change 2013: The physical science basis, Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, Chap. 7, edited by: Stocker, T., Qin, D., Plattner, G.-K., Tignor, M., Allen, S., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P., Cambridge University Press, Cambridge, UK and New York, NY, USA, 571–658, https://doi.org/10.1017/CBO9781107415324.016, 2013.
Brenguier, J.-L., Burnet, F., and Geoffroy, O.: Cloud optical thickness and liquid water path – does the k coefficient vary with droplet concentration?, Atmos. Chem. Phys., 11, 9771–9786, https://doi.org/10.5194/acp-11-9771-2011, 2011.
Bretherton, C. S., Blossey, P. N., and Uchida, J.: Cloud droplet sedimentation, entrainment efficiency, and subtropical stratocumulus albedo, Geophys. Res. Lett., 34, L03813, https://doi.org/10.1029/2006GL027648, 2007.
Cadeddu, M. P., Liljegren, J. C., and Turner, D. D.: The Atmospheric radiation measurement (ARM) program network of microwave radiometers: instrumentation, data, and retrievals, Atmos. Meas. Tech., 6, 2359–2372, https://doi.org/10.5194/amt-6-2359-2013, 2013.
Cadeddu, M. P., Ghate, V. P., and Mech, M.: Ground-based observations of cloud and drizzle liquid water path in stratocumulus clouds, Atmos. Meas. Tech., 13, 1485–1499, https://doi.org/10.5194/amt-13-1485-2020, 2020.
Cadeddu, M. P., Ghate, V. P., Turner, D. D., and Surleta, T. E.: Boundary layer moisture variability at the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic observatory during marine conditions, Atmos. Chem. Phys., 23, 3453–3470, https://doi.org/10.5194/acp-23-3453-2023, 2023.
Carslaw, K., Lee, L., Reddington, C., Pringle, K. J., Rap, A., Forster, P. M., Mann, G. W., Spracklen, D. V., Woodhouse, M. T., Regayre, L. A., and Pierce, J. R.: Large contribution of natural aerosols to uncertainty in indirect forcing, Nature, 503, 67–71, https://doi.org/10.1038/nature12674, 2013.
Chen, YC., Christensen, M., Stephens, G., and Seinfeld, J. H.: Satellite-based estimate of global aerosol–cloud radiative forcing by marine warm clouds, Nat. Geosci., 7, 643–646, https://doi.org/10.1038/ngeo2214, 2014.
Christensen, M. W., Neubauer, D., Poulsen, C. A., Thomas, G. E., McGarragh, G. R., Povey, A. C., Proud, S. R., and Grainger, R. G.: Unveiling aerosol–cloud interactions – Part 1: Cloud contamination in satellite products enhances the aerosol indirect forcing estimate, Atmos. Chem. Phys., 17, 13151–13164, https://doi.org/10.5194/acp-17-13151-2017, 2017.
Christensen, M. W., Jones, W. K., and Stier, P.: Aerosols Enhance Cloud Lifetime and Brightness along the Stratus-to-Cumulus Transition, P. Natl. Acad. Sci. USA, 117, 17591–17598, https://doi.org/10.1073/pnas.1921231117, 2020.
Christensen, M. W., Gettelman, A., Cermak, J., Dagan, G., Diamond, M., Douglas, A., Feingold, G., Glassmeier, F., Goren, T., Grosvenor, D. P., Gryspeerdt, E., Kahn, R., Li, Z., Ma, P.-L., Malavelle, F., McCoy, I. L., McCoy, D. T., McFarquhar, G., Mülmenstädt, J., Pal, S., Possner, A., Povey, A., Quaas, J., Rosenfeld, D., Schmidt, A., Schrödner, R., Sorooshian, A., Stier, P., Toll, V., Watson-Parris, D., Wood, R., Yang, M., and Yuan, T.: Opportunistic experiments to constrain aerosol effective radiative forcing, Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, 2022.
Christensen, M. W., Ma, P.-L., Wu, P., Varble, A. C., Mülmenstädt, J., and Fast, J.: Evaluation of aerosol-cloud interactions in E3SSM using a Lagrangian framework, Atmos. Chem. Phys., 23, 2789–2812, https://doi.org/10.5194/acp-23-2789-2023, 2023.
Clothiaux, E. E., Ackerman, T. P., Mace, G. G., Moran, K. P., Marchand, R. T., Miller, M. A., and Martner, B. E.: Objective determination of cloud heights and radar reflectivities using a combination of active remote sensors at the ARM CART sites, J. Appl. Meteorol., 39, 645–665, https://doi.org/10.1175/1520-0450(2000)039<0645:ODOCHA>2.0.CO;2, 2000.
Coakley, J. A., Bernstein, R. L., and Durkee, P. A.: Effect of Ship-Stack Effluents on Cloud Reflectivity, Science, 237, 1020–1022, https://doi.org/10.1126/science.237.4818.1020, 1987.
Danabasoglu, G., Lamarque, J.-F., Bacmeister, J., Bailey, D. A., DuVivier, A. K., Edwards, J., Emmons, L. K., Fasullo, J., Garcia, R., Gettelman, A., Hannay, C., Holland, M. M., Large, W. G., Lauritzen, P. H., Lawrence, D. M., Lenaerts, J. T. M., Lindsay, K., Lipscomb, W. H., Mills, M. J., Neale, R., Oleson, K. W., Otto-Bliesner, B., Phillips, A. S., Sacks, W., Tilmes, S., van Kampenhout, L., Vertenstein, M., Bertini, A., Dennis, J., Deser, C., Fischer, C., Fox-Kemper, B., Kay, J. E., Kinnison, D., Kushner, P. J., Larson, V. E., Long, M. C., Mickelson, S., Moore, J. K., Nienhouse, E., Polvani, L., Rasch, P. J., and Strand, W. G.: The Community Earth System Model Version 2 (CESM2), J. Adv. Model. Earth Syst., 12, e2019MS001916, https://doi.org/10.1029/2019MS001916, 2020.
Dong, X., Xi, B., Kennedy, A., Minnis, P., and Wood, R.: A 19-month record of marine aerosol-cloud-radiation properties derived from DOE ARM Mobile Facility deployment at the Azores. Part I: cloud fraction and single-layered MBL cloud properties, J. Climate, 27, 3665–3682, https://doi.org/10.1175/JCLI-D-13-00553.1, 2014.
Dong, X., Schwantes, A. C., Xi, B., and Wu, P.: Investigation of the marine boundary layer cloud and CCN properties under coupled and decoupled conditions over the Azores, J. Geophys. Res.-Atmos., 120, 6179–6191, https://doi.org/10.1002/2014JD022939, 2015.
Douglas, A. and L'Ecuyer, T.: Quantifying variations in shortwave aerosol–cloud–radiation interactions using local meteorology and cloud state constraints, Atmos. Chem. Phys., 19, 6251–6268, https://doi.org/10.5194/acp-19-6251-2019, 2019.
Douglas, A. and L'Ecuyer, T.: Quantifying cloud adjustments and the radiative forcing due to aerosol–cloud interactions in satellite observations of warm marine clouds, Atmos. Chem. Phys., 20, 6225–6241, https://doi.org/10.5194/acp-20-6225-2020, 2020.
Eastman, R., Wood, R., and Bretherton, C. S.: Time Scales of Clouds and Cloud-Controlling Variables in Subtropical Stratocumulus from a Lagrangian Perspective, J. Atmos. Sci., 73, 3079–3091, https://doi.org/10.1175/JAS-D-16-0050.1, 2016.
Eastman, R., Terai, C. R., Grosvenor, D. P., and Wood, R.: Evaluating the Lagrangian Evolution of Subtropical Low Clouds in GCMs Using Observations: Mean Evolution, Time Scales, and Responses to Predictors, J. Atmos. Sci., 78, 353–372, https://doi.org/10.1175/JAS-D-20-0178.1, 2021.
Eyring, V., Bony, S., Meehl, G. A., Senior, C. A., Stevens, B., Stouffer, R. J., and Taylor, K. E.: Overview of the Coupled Model Intercomparison Project Phase 6 (CMIP6) experimental design and organization, Geosci. Model Dev., 9, 1937–1958, https://doi.org/10.5194/gmd-9-1937-2016, 2016.
Fairless, T., Jensen, M., Zhou, A., and Giangrande, S. E.: Interpolated sonde and gridded sonde value-added products, US Department of Energy, Atmospheric Radiation Measurement user facility, Richland, Washington, DOE/SC-ARM-TR-183, https://doi.org/10.2172/1248938, 2021.
Feingold, G., Goren, T., and Yamaguchi, T.: Quantifying albedo susceptibility biases in shallow clouds, Atmos. Chem. Phys., 22, 3303–3319, https://doi.org/10.5194/acp-22-3303-2022, 2022.
Gallo, F., Uin, J., Springston, S., Wang, J., Zheng, G., Kuang, C., Wood, R., Azevedo, E. B., McComiskey, A., Mei, F., Theisen, A., Kyrouac, J., and Aiken, A. C.: Identifying a regional aerosol baseline in the eastern North Atlantic using collocated measurements and a mathematical algorithm to mask high-submicron-number-concentration aerosol events, Atmos. Chem. Phys., 20, 7553–7573, https://doi.org/10.5194/acp-20-7553-2020, 2020.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs, L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan, K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A., da Silva, A. M., Gu, W., Kim, G.-K., Koster, R., Lucchesi, R., Merkova, D., Nielsen, J. E., Partyka, G., Pawson, S., Putman, W., Rienecker, M., Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2), J. Climate, 30, 5419–5454, https://doi.org/10.1175/JCLI-D-16-0758.1, 2017.
Gettelman, A. and Morrison, H.: Advanced two-moment bulk microphysics for global models. Part I: Off-line tests and comparison with other schemes, J. Climate, 28, 1268–1287, https://doi.org/10.1175/JCLI-D-14-00102.1, 2015.
Gettelman, A., Morrison, H., Santos, S., Bogenschutz, P., and Caldwell, P. M.: Advanced two-moment bulk microphysics for global models. Part II: Global model solutions and aerosol–cloud interactions, J. Climate, 28, 1288–1307, https://doi.org/10.1175/JCLI-D-14-00103.1, 2015.
Ghan, S., Wang, M., Zhang, S., Ferrachat, S., Gettelman, A., Griesfeller, J., Kipling, Z., Lohmann, U., Morrison, H., Neubauer, D., Partridge, D. G., Stier, P., Takemura, T., Wang, H., and Zhang, K.: Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability, P. Natl. Acad. Sci. USA, 113, 5804–5811, https://doi.org/10.1073/pnas.1514036113, 2016.
Ghan, S. J., Abdul-Razzak, H., Nenes, A., Ming, Y., Liu, X., Ovchinnikov, M., Shipway, B., Meskhidze, N., Xu, J., and Shi, X.: Droplet nucleation: Physically-based parameterizations and comparative evaluation, J. Adv. Model. Earth Syst., 3, M10001, https://doi.org/10.1029/2011MS000074, 2011.
Ghate, V. P. and Cadeddu, M. P.: Drizzle and turbulence below closed cellular marine stratocumulus clouds, J. Geophys. Res.-Atmos., 124, 5724–5737, https://doi.org/10.1029/2018JD030141, 2019.
Ghate, V. P., Cadeddu, M. P., Zheng, X., and O'Connor, E.: Turbulence in the marine boundary layer and air motions below stratocumulus clouds at the ARM Eastern North Atlantic site, J. Appl. Meteorol. Clim., 60, 1495–1510, https://doi.org/10.1175/JAMC-D-21-0087.1, 2021.
Giangrande, S. E., Wang, D., Bartholomew, M. J., Jensen, M. P., Mechem, D. B., Hardin, J. C., and Wood, R.: Midlatitude oceanic cloud and precipitation properties as sampled by the ARM Eastern North Atlantic Observatory, J. Geophys. Res.-Atmos., 124, 4741–4760, https://doi.org/10.1029/2018JD029667, 2019.
Glassmeier, F., Hoffmann, F., Johnson, J. S., Yamaguchi, T., Carslaw, K. S., and Feingold, G.: An emulator approach to stratocumulus susceptibility, Atmos. Chem. Phys., 19, 10191–10203, https://doi.org/10.5194/acp-19-10191-2019, 2019.
Golaz, J.-C., Larson, V. E., and Cotton, W. R.: A PDF-Based Model for Boundary Layer Clouds. Part I: Method and Model Description, J. Atmos. Sci., 59, 3540–3551, https://doi.org/10.1175/1520-0469(2002)059<3540:APBMFB>2.0.CO;2, 2002.
Golaz, J. C., Caldwell, P. M., Van Roekel, L. P., Petersen, M. R., Tang, Q., Wolfe, J. D., Abeshu, G., Anantharaj, V., Asay-Davis, X. S., Bader, D. C., Baldwin, S. A., Bisht, G., Bogenschutz, P. A., Branstetter, M., Brunke, M. A., Brus, S. R., Burrows, S. M., Cameron-Smith, P. J., Donahue, A. S., Deakin, M., Easter, R. C., Evans, K. J., Feng, Y., Flanner, M., Foucar, J. G., Fyke, J. G., Griffin, B. M., Hannay, C., Harrop, B. E., Hoffman, M. J., Hunke, E. C., Jacob, R. L., Jacobsen, D.W., Jeffery, N., Jones, P.W., Keen, N. D., Klein, S. A., Larson, V. E., Leung, L. R., Li, H. Y., Lin, W. Y., Lipscomb, W. H., Ma, P. L., Mahajan, S., Maltrud, M. E., Mametjanov, A., McClean, J. L., McCoy, R. B., Neale, R. B., Price, S. F., Qian, Y., Rasch, P. J., Eyre, J. E. J. R., Riley, W. J., Ringler, T. D., Roberts, A. F., Roesler, E. L., Salinger, A. G., Shaheen, Z., Shi, X. Y., Singh, B., Tang, J. Y., Taylor, M. A., Thornton, P. E., Turner, A. K., Veneziani, M., Wan, H., Wang, H. L., Wang, S. L., Williams, D. N., Wolfram, P. J., Worley, P. H., Xie, S. C., Yang, Y., Yoon, J. H., Zelinka, M. D., Zender, C. S., Zeng, X. B., Zhang, C. Z., Zhang, K., Zhang, Y., Zheng, X., Zhou, T., and Zhu, Q.: The DOE E3SM Coupled Model Version 1: Overview and Evaluation at Standard Resolution, J. Adv. Model. Earth Syst., 11, 2089–2129, https://doi.org/10.1029/2018ms001603, 2019.
Golaz, J. C., Van Roekel, L. P., Zheng, X., Roberts, A. F., Wolfe, J. D., Lin, W., Bradley, A. M., Tang, Q., Maltrud, M. E., Forsyth, R. M., Tang, Q., Zhang, C., Zhou, T., Zhang, K., Zender, C. S., Wu, M., Wang, H. L., Turner, A. K., Singh, B., Richter, J. H., Qin, Y., Petersen, M. R., Mametjanov, A., Ma, P. L., Larson, V. E., Krishna, J., Keen, N. D., Jeffery, N., Hunke, E. C., Hannah, W. M., Guba, O., Griffin, B. M., Feng, Y., Engwirda, D., Di Vittorio, A. V., Dang, C., Conlon, L. M., Chen, C.-C.-J., Brunke, M. A., Bisht, G., Benedict, J. J., Asay-Davis, X. S., Zhang, Y., Zhang, M., Zeng, X., Xie, S., Wolfram, P. J., Vo, T., Veneziani, M., Tesfa, T. K., Sreepathi, S., Salinger, A. G., Eyre, J. E. J. R., Prather, M. J., Mahajan, S., Li, Q., Jones, P. W., Jacob, R. L., Huebler, G. W., Huang, X., Hillman, B. R., Harrop, B. E., Foucar, J. G., Fang, Y., Comeau, D. S., Caldwell, P. M., Bartoletti, T., Balaguru, K., Taylor, M. A., McCoy, R. B., Leung, L. R., and Bader, D. C.: The DOE E3SM Model Version 2: Overview of the Physical Model and Initial Model Evaluation, J. Adv. Model. Earth Syst., 14, e2022MD003156, https://doi.org/10.1029/2022MS003156, 2022.
Gong, X., Wang, Y., Xie, H., Zhang, J., Lu, Z., Stratmann, F., Wex, H., Liu, X., and Wang, J.: Maximum supersaturation in marine boundary layer clouds over the North Atlantic, in: 15th Symposium on Aerosol-Cloud-Climate Interactions, 103rd American Meteorological Society Annual Meeting, 8–12 January 2023, Denver, CO, USA, 8B.2, https://ams.confex.com/ams/103ANNUAL/meetingapp.cgi/Paper/417366 (last access: 14 September 2023), 2023.
Goren, T., Kazil, J., Hoffmann, F., Yamaguchi, T., and Feingold, G.: Anthropogenic air pollution delays marine stratocumulus break-up to open-cells, Geophys. Res. Lett., 46, 14135– 14144, https://doi.org/10.1029/2019GL085412, 2019.
Grosvenor, D. P., Sourdeval, O., Zuidema, P., Ackerman, A., Alexandrov, M. D., Bennartz, R., Boers, R., Cairns, B., Chiu, J. C., Christensen, M., Deneke, H., Diamond, M., Feingold, G., Fridlind, A., Hunerbein, A., Knist, C., Kollias, P., Marshak, A., McCoy, D., Merk, D., Painemal, D., Rausch, J., Rosenfeld, D., Russchenberg, H., Seifert, P., Sinclair, K., Stier, P., van Diedenhoven, B., Wendisch, M., Werner, F., Wood, R., Zhang, Z., and Quaas, J.: Remote sensing of droplet number concentration in warm clouds: A review of the current state of knowledge and perspectives, Rev. Geophys., 56, 409–453, https://doi.org/10.1029/2017RG000593, 2018.
Gryspeerdt, E., Quaas, J., and Bellouin, N.: Constraining the aerosol influence on cloud fraction, J. Geophys. Res.-Atmos., 121, 3566–3583, https://doi.org/10.1002/2015JD023744, 2016.
Gryspeerdt, E., Quaas, J., Ferrachat, S., Gettelman, A., Ghan, S., Lohmann, U., Morrison, H., Neubauer, D., Partridge, D. G., Stier, P., Takemura, T., Wang, H., Wang, M., and Zhang, K.: Constraining the instantaneous aerosol influence on cloud albedo, P. Natl. Acad. Sci. USA, 114, 4899–4904, https://doi.org/10.1073/pnas.1617765114, 2017.
Gryspeerdt, E., Goren, T., Sourdeval, O., Quaas, J., Mülmenstädt, J., Dipu, S., Unglaub, C., Gettelman, A., and Christensen, M.: Constraining the aerosol influence on cloud liquid water path, Atmos. Chem. Phys., 19, 5331–5347, https://doi.org/10.5194/acp-19-5331-2019, 2019.
Gryspeerdt, E., Mülmenstädt, J., Gettelman, A., Malavelle, F. F., Morrison, H., Neubauer, D., Partridge, D. G., Stier, P., Takemura, T., Wang, H., Wang, M., and Zhang, K.: Surprising similarities in model and observational aerosol radiative forcing estimates, Atmos. Chem. Phys., 20, 613–623, https://doi.org/10.5194/acp-20-613-2020, 2020.
Gryspeerdt, E., McCoy, D. T., Crosbie, E., Moore, R. H., Nott, G. J., Painemal, D., Small-Griswold, J., Sorooshian, A., and Ziemba, L.: The impact of sampling strategy on the cloud droplet number concentration estimated from satellite data, Atmos. Meas. Tech., 15, 3875–3892, https://doi.org/10.5194/amt-15-3875-2022, 2022.
Hoffmann, F., Glassmeier, F., Yamaguchi, T., and Feingold, G.: Liquid Water Path Steady States in Stratocumulus: Insights from Process-Level Emulation and Mixed-Layer Theory, J. Atmos.Sci., 77, 2203–2215, https://doi.org/10.1175/JAS-D-19-0241.1, 2020.
Ilotoviz, E., Ghate, V. P., and Raveh-Rubin, S.: The impact of slantwise descending dry intrusions on the marine boundary layer and air-sea interface over the ARM Eastern North Atlantic site, J. Geophys. Res.-Atmos., 126, e2020JD033879, https://doi.org/10.1029/2020JD03389, 2021.
Jensen, M. P., V. P. Ghate, D. Wang, D. K. Apoznanski, M. J. Bartholomew, S. E. Giangrande, K. L. Johnson, and Thieman, M. M.: Contrasting characteristics of open- and closed-cellular stratocumulus cloud in the eastern North Atlantic, Atmos. Chem. Phys., 21, 14557–14571, https://doi.org/10.5194/acp-21-14557-2021, 2021.
Jeong, J.-H., Witte, M. K., Glenn, I. B., Smalley, M., Lebsock, M. D., Lamer, K., and Zhu, Z.: Distinct dynamical and structural properties of marine stratocumulus and shallow cumulus clouds in the Eastern North Atlantic, J. Geophys. Res.-Atmos., 127, e2022JD037021, https://doi.org/10.1029/2022JD037021, 2022.
Jiang, H., Xue, H., Teller, A., Feingold, G., and Levin, Z.: Aerosol effects on the lifetime of shallow cumulus, Geophys. Res. Lett., 33, L14806, https://doi.org/10.1029/2006GL026024, 2006.
Jing, X. and Suzuki, K.: The impact of process-based warm rain constraints on the aerosol indirect effect, Geophys. Res. Lett., 45, 10729–10737, https://doi.org/10.1029/2018GL079956, 2018.
Johnson, D. W., Osborne, S., Wood, R., Suhre, K., Johnson, R., Businger, S., Quinn, P. K., Wiedensohler, A., Durkee, P. A., Russell, L. M., Andreae, M. O., O'Dowd, C., Noone, K. J., Bandy, B., Rudolph, J., and Rapsomanikis, S.: An overview of the Lagrangian experiments undertaken during the North Atlantic regional Aerosol Characterisation Experiment (ACE-2), Tellus B, 52, 290–320, https://doi.org/10.3402/tellusb.v52i2.16110, 2000.
Jones, C. R., Bretherton, C. S., and Leon, D.: Coupled vs. decoupled boundary layers in VOCALS-REx, Atmos. Chem. Phys., 11, 7143–7153, https://doi.org/10.5194/acp-11-7143-2011, 2011.
Kang, L., Marchand, R. T., and Smith, W. L.: Evaluation of MODIS and Himawari-8 low clouds retrievals over the Southern Ocean with in situ measurements from the SOCRATES campaign, Earth Space Sci., 8, e2020EA001397, https://doi.org/10.1029/2020EA001397, 2021.
Kazemirad, M. and Miller, M. A.: Summertime post-cold-frontal marine stratocumulus transition processes over the Easter North Atlantic, J. Atmos. Sci., 77, 2011–2037, https://doi.org/10.1175/JAS-D-19-0167.1, 2020.
Kogan, Y. L. and Martin, W. J.: Parameterization of Bulk Condensation in Numerical Cloud Models, J. Atmos. Sci., 51, 1728–1739, https://doi.org/10.1175/1520-0469(1994)051<1728:POBCIN>2.0.CO;2, 1994.
Koren, I., Dagan, G., and Altaratz, O.: From aerosol-limited to invigoration of warm convective clouds, Science, 344, 1143–1146, https://doi.org/10.1126/science.1252595, 2014.
Lamer, K., Naud, C. M., and Booth, J. F.: Relationships between precipitation properties and large-scale conditions during subsidence at the Eastern North Atlantic observatory, J. Geophys. Res.-Atmos., 125, e2019JD031848, https://doi.org/10.1029/2019JD031848, 2020.
Larson, V. E. and Golaz, J.-C.: Using Probability Density Functions to Derive Consistent Closure Relationships among Higher-Order Moments, Mon. Weather Rev., 133, 1023–1042, https://doi.org/10.1175/MWR2902.1, 2005.
Lebsock, M. D., Stephens, G. L., and Kummerow, C.: Multisensor satellite observations of aerosol effects on warm clouds, J. Geophys. Res., 113, D15205, https://doi.org/10.1029/2008JD009876, 2008.
Liu, X., Ma, P.-L., Wang, H., Tilmes, S., Singh, B., Easter, R. C., Ghan, S. J., and Rasch, P. J.: Description and evaluation of a new four-mode version of the Modal Aerosol Module (MAM4) within version 5.3 of the Community Atmosphere Model, Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, 2016.
Long, C. N. and Ackerman, T. P.: Identification of clear skies from broadband pyranometer measurements and calculation of downwelling shortwave cloud effects, J. Geophys. Res.-Atmos., 105, 15609–15626, https://doi.org/10.1029/2000JD900077, 2000.
Ma, P.-L., Harrop, B. E., Larson, V. E., Neale, R. B., Gettelman, A., Morrison, H., Wang, H., Zhang, K., Klein, S. A., Zelinka, M. D., Zhang, Y., Qian, Y., Yoon, J.-H., Jones, C. R., Huang, M., Tai, S.-L., Singh, B., Bogenschutz, P. A., Zheng, X., Lin, W., Quaas, J., Chepfer, H., Brunke, M. A., Zeng, X., Mülmenstädt, J., Hagos, S., Zhang, Z., Song, H., Liu, X., Pritchard, M. S., Wan, H., Wang, J., Tang, Q., Caldwell, P. M., Fan, J., Berg, L. K., Fast, J. D., Taylor, M. A., Golaz, J.-C., Xie, S., Rasch, P. J., and Leung, L. R.: Better calibration of cloud parameterizations and subgrid effects increases the fidelity of the E3SM Atmosphere Model version 1, Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, 2022.
Mather, J. H. and Voyles, J. W.: The ARM Climate Research Facility: A Review of Structure and Capabilities, B. Am. Meteorol. Soc., 94, 377–392, https://doi.org/10.1175/bams-d-11-00218.1, 2013.
McComiskey, A. and Feingold, G.: The Scale Problem in Quantifying Aerosol Indirect Effects, Atmos. Chem. Phys., 12, 1031–1049, https://doi.org/10.5194/acp-12-1031-2012, 2012.
McComiskey, A., Feingold, G., Frisch, A. S., Turner, D. D., Miller, M. A., Chiu, J. C., Min, Q., and Ogren, J. A.: An assessment of aerosol-cloud interactions in marine stratus clouds based on surface remote sensing, J. Geophys. Res.–Atmos., 114, D09203, https://doi.org/10.1029/2008JD011006, 2009.
Mechem, D. B., Wittman, C. S., Miller, M. A., Yuter, S. E., and de Szoeke, S. P.: Joint synoptic and cloud variability over the Northeast Atlantic near the Azores, J. Appl. Meteorol. Clim., 57, 1273–1290, https://doi.org/10.1175/JAMC-D-17-0211.1, 2018.
Merk, D., Deneke, H., Pospichal, B., and Seifert, P.: Investigation of the adiabatic assumption for estimating cloud micro- and macrophysical properties from satellite and ground observations, Atmos. Chem. Phys., 16, 933–952, https://doi.org/10.5194/acp-16-933-2016, 2016.
Michibata, T., Suzuki, K., Sato, Y., and Takemura, T.: The source of discrepancies in aerosol–cloud–precipitation interactions between GCM and A-Train retrievals, Atmos. Chemi. Phys., 16, 15413–15424, https://doi.org/10.5194/acp-16-15413-2016, 2016.
Min, Q. and Harrison, L. C.: Cloud properties derived from surface MFRSR measurements and comparison with GOES results at the ARM SGP site, Geophys. Res. Lett., 23, 1641–1644, https://doi.org/10.1029/96GL01488, 1996.
Min, Q.-L., Duan, M., and Marchand, R.: Validation of surface retrieved cloud optical properties with in situ measurements at the Atmospheric Radiation Measurement program (ARM) South Great Plains site, J. Geophys. Res., 108, 4547, https://doi.org/10.1029/2003JD003385, 2003.
Minnis, P., Nguyen, L., Palikonda, R., Heck, P. W., Spangenberg, D. A., Doelling, D. R., Ayers, J. K., Smith, J. W. L., Khaiyer, M. M., Trepte, Q. Z., Avey, L. A., Chang, F.-L., Yost, C. R., Chee, T. L., and Szedung, S.-M.: Near-real time cloud retrievals from operational and research meteorological satellites, Proc. SPIE, 7107, 710703, https://doi.org/10.1117/12.800344, 2008.
Minnis, P., Sun-Mack, S., Young, D. F., Heck, P. W., Garber, D. P., Chen, Y., Spangenberg, D. A., Arduini, R. F., Trepte, Q. Z., Smith, W. L., Ayers, J. K., Gibson, S. C., Miller, W. F., Hong, G., Chakrapani, V., Takano, Y., Liou, K. N., Xie, Y., and Yang, P.: CERES Edition-2 Cloud Property Retrievals Using TRMM VIRS and Terra and Aqua MODIS Data – Part I: Algorithms, IEEE T. Geosci. Remote, 49, 4374–4400, https://doi.org/10.1109/tgrs.2011.2144601, 2011.
Mohrmann, J., Bretherton, C. S., McCoy, I. L., McGibbon, J., Wood, R., Ghate, V., Albrecht, B., Sarkar, M., Zuidema, P., and Palikonda, R.: Lagrangian Evolution of the Northeast Pacific Marine Boundary Layer Structure and Cloud during CSET, Mon. Weather Rev., 147, 4681–4700, https://doi.org/10.1175/MWR-D-19-0053.1, 2019.
Morrison, H. and Gettelman, A.: A new two-moment bulk stratiform cloud microphysics scheme in the Community Atmosphere Model, version 3 (CAM3). Part I: Description and numerical tests, J. Climate, 21, 3642–3659, https://doi.org/10.1175/2008JCLI2105.1, 2008.
Mülmenstädt, J. and Feingold, G.: The radiative forcing of aerosol–cloud interactions in liquid clouds: Wrestling and embracing uncertainty, Curr. Clim. Change Rep., 4, 23–40, https://doi.org/10.1007/s40641-018-0089-y, 2018.
Mülmenstädt, J., Gryspeerdt, E., Salzmann, M., Ma, P.-L., Dipu, S., and Quaas, J.: Separating radiative forcing by aerosol–cloud interactions and rapid cloud adjustments in the ECHAM–HAMMOZ aerosol–climate model using the method of partial radiative perturbations, Atmos. Chem. Phys., 19, 15415–15429, https://doi.org/10.5194/acp-19-15415-2019, 2019.
Naud, C. M., Booth, J. F., and Lamraoui, F.: Post cold frontal clouds at the ARM Eastern North Atlantic site: An examination of the relationship between large-scale environment and cloud properties, J. Geophys. Res.-Atmos., 123, 12117–12132, https://doi.org/10.1029/2018JD029015, 2018.
Penner, J. E., Xu, L., and Wang, M.: Satellite methods underestimate indirect climate forcing by aerosols, P. Natl. Acad. Sci. USA, 108, 13404–13408, https://doi.org/10.1073/pnas.1018526108, 2011.
Pincus, R. and Baker, M.: Effects of precipitation on the albedo susceptibility of clouds in the marine boundary layer, Nature, 372, 250–252, https://doi.org/10.1038/372250a0, 1994.
Pincus, R., Baker, M. B., and Bretherton, C. S.: What Controls Stratocumulus Radiative Properties? Lagrangian Observations of Cloud Evolution, J. Atmos. Sci., 54, 2215–2236, https://doi.org/10.1175/1520-0469(1997)054<2215:WCSRPL>2.0.CO;2, 1997.
Pincus, R., Platnick, S., Ackerman, S. A., Hemler, R. S., and Hofmann, R. J. P.: Reconciling simulated and observed views of clouds: MODIS, ISCCP, and the limits of instrument simulators, J. Climate, 25, 4699–4720, https://doi.org/10.1175/JCLI-D-11-00267.1, 2012.
Platnick, S. and Twomey, S.: Determining the Susceptibility of Cloud Albedo to Changes in Droplet Concentration with the Advanced Very High Resolution Radiometer, J. Appl. Meteorol. Clim., 33, 334–347, https://doi.org/10.1175/1520-0450(1994)033<0334:DTSOCA>2.0.CO;2, 1994.
Possner, A., Eastman, R., Bender, F., and Glassmeier, F.: Deconvolution of boundary layer depth and aerosol constraints on cloud water path in subtropical stratocumulus decks, Atmos. Chem. Phys., 20, 3609–3621, https://doi.org/10.5194/acp-20-3609-2020, 2020.
Qiu, S., Zheng, X., Painemal, D., Terai, C., and Zhou, X.: Diurnal variation of aerosol indirect effect for warm marine boundary layer clouds in the eastern north Atlantic, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2023-1676, 2023.
Quaas, J., Boucher, O., Bellouin, N., and Kinne, S.: Satellite-based estimate of the direct and indirect aerosol climate forcing, J. Geophys. Res., 113, D05204, https://doi.org/10.1029/2007JD008962, 2008.
Quaas, J., Ming, Y., Menon, S., Takemura, T., Wang, M., Penner, J., Gettelman, A., Lohmann, U., Bellouin, N., Boucher, O., Sayer, A., Thomas, G., McComiskey, A., Feingold, G., Hoose, C., Kristjánsson, J., Liu, X., Balkanski, Y., Donner, L., Ginoux, P., Stier, P., Grandey, B., Feichter, J., Sednev, I., Bauer, S., Koch, D., Grainger, R., Kirkevåg, A., Iversen, T., Seland, Ø., Easter, R., Ghan, S., Rasch, P., Morrison, H., Lamarque, J.-F., Iacono, M., Kinne, S., and Schulz, M.: Aerosol indirect effects – General circulation model intercomparison and evaluation with satellite data, Atmos. Chem. Phys., 9, 8697–8717, https://doi.org/10.5194/acp-9-8697-2009, 2009.
Quaas, J., Arola, A., Cairns, B., Christensen, M., Deneke, H., Ekman, A. M. L., Feingold, G., Fridlind, A., Gryspeerdt, E., Hasekamp, O., Li, Z., Lipponen, A., Ma, P.-L., Mülmenstädt, J., Nenes, A., Penner, J. E., Rosenfeld, D., Schrödner, R., Sinclair, K., Sourdeval, O., Stier, P., Tesche, M., van Diedenhoven, B., and Wendisch, M.: Constraining the Twomey effect from satellite observations: issues and perspectives, Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, 2020.
Radke, L. F., Coakley, J. A., and King, M. D.: Direct and Remote Sensing Observations of the Effects of Ships on Clouds, Science, 246, 1146–1149, https://doi.org/10.1126/science.246.4934.1146, 1989.
Rasch, P. J., Xie, S., Ma, P.-L., Lin, W., Wang, H., Tang, Q., Burrows, S. M., Caldwell, P., Zhang, K., Easter, R. C., Cameron-Smith, P., Singh, B., Wan, H., Golaz, J.-C., Harrop, B. E., Roesler, E., Bacmeister, J., Larson, V. E., Evans, K. J., Qian, Y., Taylor, M., Leung, L. R., Zhang, Y., Brent, L., Branstetter, M., Hannay, C., Mahajan, S., Mametjanov, A., Neale, R., Richter, J. H., Yoon, J.-H., Zender, C. S., Bader, D., Flanner, M., Foucar, J. G., Jacob, R., Keen, N., Klein, S. A., Liu, X., Salinger, A., Shrivastava, M., and Yang, Y.: An Overview of the Atmospheric Component of the Energy Exascale Earth System Model, J. Adv. Model. Earth Syst., 11, 2377–2411, https://doi.org/10.1029/2019MS001629, 2019.
Rémillard, J. and Tselioudis, G.: Cloud regime variability over the Azores and its application to climate model evaluation, J. Climate, 28, 9707–9720, https://doi.org/10.1175/JCLI-D-15-0066.1, 2015.
Rémillard, J., Kollias, P., Luke, E., and Wood, R.: Marine Boundary Layer Cloud Observations in the Azores, J. Climate, 25, 7381–7398, https://doi.org/10.1175/JCLI-D-11-00610.1, 2012.
Saponaro, G., Sporre, M. K., Neubauer, D., Kokkola, H., Kolmonen, P., Sogacheva, L., Arola, A., de Leeuw, G., Karset, I. H. H., Laaksonen, A., and Lohmann, U.: Evaluation of aerosol and cloud properties in three climate models using MODIS observations and its corresponding COSP simulator, as well as their application in aerosol–cloud interactions, Atmos. Chem. Phys., 20, 1607–1626, https://doi.org/10.5194/acp-20-1607-2020, 2020.
Sato, Y., Goto, D., Michibata, T., Suzuki, K., Takemura, T., Tomita, H., and Nakajima, T.: Aerosol effects on cloud water amounts were successfully simulated by a global cloud-system resolving model, Nat. Commun., 9, 985, https://doi.org/10.1038/s41467-018-03379-6, 2018.
Shinozuka, Y., Clarke, A. D., Nenes, A., Jefferson, A., Wood, R., McNaughton, C. S., Strom, J., Tunved, P., Redemann, J., Thornhill, K. L., Moore, R. H., Lathem, T. L., Lin, J. J., and Yoon, Y. J.: The relationship between cloud condensation nuclei (CCN) concentration and light extinction of dried particles: indications of underlying aerosol processes and implications for satellite-based CCN estimates, Atmos. Chem. Phys., 15, 7585–7604, https://doi.org/10.5194/acp-15-7585-2015, 2015.
Silva, S. J., Ma, P.-L., Hardin, J. C., and Rothenberg, D.: Physically regularized machine learning emulators of aerosol activation, Geosci. Model Dev., 14, 3067–3077, https://doi.org/10.5194/gmd-14-3067-2021, 2021.
Small, J. D., Chuang, P. Y., Feingold, G., and Jiang, H.: Can aerosol decrease cloud lifetime?, Geophys. Res. Lett., 36, L16806, https://doi.org/10.1029/2009GL038888, 2009.
Smith, C. J., Kramer, R. J., Myhre, G., Alterskjær, K., Collins, W., Sima, A., Boucher, O., Dufresne, J.-L., Nabat, P., Michou, M., Yukimoto, S., Cole, J., Paynter, D., Shiogama, H., O'Connor, F. M., Robertson, E., Wiltshire, A., Andrews, T., Hannay, C., Miller, R., Nazarenko, L., Kirkevåg, A., Olivié, D., Fiedler, S., Lewinschal, A., Mackallah, C., Dix, M., Pincus, R., and Forster, P. M.: Effective radiative forcing and adjustments in CMIP6 models, Atmos. Chem. Phys., 20, 9591–9618, https://doi.org/10.5194/acp-20-9591-2020, 2020.
Song, H., Zhang, Z., Ma, P., Ghan, S. J., and Wang, M.: An Evaluation of Marine Boundary Layer Cloud Property Simulations in the Community Atmosphere Model Using Satellite Observations: Conventional Subgrid Parameterization versus CLUBB, J. Climate, 31, 2299–2320, https://doi.org/10.1175/JCLI-D-17-0277.1, 2018.
Stephens, G. L., L'Ecuyer, T., Forbes, R., Gettelmen, A., Golaz, J.-C., Bodas-Salcedo, A., Suzuki, K., Gabriel, P., and Haynes, J.: Dreary state of precipitation in global models, J. Geophys. Res., 115, D24211, https://doi.org/10.1029/2010JD014532, 2010.
Stevens, B. and Feingold, G.: Untangling aerosol effects on clouds and precipitation in a buffered system, Nature, 461, 607–613, https://doi.org/10.1038/nature08281, 2009.
Stier, P.: Limitations of passive remote sensing to constrain global cloud condensation nuclei, Atmos. Chem. Phys., 16, 6595–6607, https://doi.org/10.5194/acp-16-6595-2016, 2016.
Suzuki, K., Nakajima, T. Y., and Stephens, G. L.: Particle growth and drop collection efficiency of warm clouds as inferred from joint CloudSat and MODIS observations, J. Atmos. Sci., 67, 3019–3032, https://doi.org/10.1175/2010JAS3463.1, 2010.
Suzuki, K., Stephens, G. L., and Lebsock, M. D.: Aerosol effect on the warm rain formation process: Satellite observations and modeling, J. Geophys. Res.-Atmos., 118, 170–184, https://doi.org/10.1002/jgrd.50043, 2013.
Suzuki, K., Stephens, G. L., Bodas-Salcedo, A., Wang, M., Golaz, J.-C., Yokohata, T., and Tsuyoshi, K.: Evaluation of the warm rain formation process in global models with satellite observations, J. Atmos. Sci., 72, 3996–4014, https://doi.org/10.1175/JAS-D-14-0265.1, 2015.
Swales, D. J., Pincus, R., and Bodas-Salcedo, A.: The Cloud Feedback Model Intercomparison Project Observational Simulator Package: Version 2, Geosci. Model Dev., 11, 77–81, https://doi.org/10.5194/gmd-11-77-2018, 2018.
Tang, S., Fast, J. D., Zhang, K., Hardin, J. C., Varble, A. C., Shilling, J. E., Mei, F., Zawadowicz, M. A., and Ma, P.-L.: Earth System Model Aerosol-Cloud Diagnostics (ESMAC Diags) package version 1: assessing E3SM aerosol predictions using aircraft, ship, and surface measurements, Geosci. Model Dev., 15, 4055–4076, https://doi.org/10.5194/gmd-15-4055-2022, 2022.
Tang, S., Varble, A. C., Fast, J. D., Zhang, K., Wu, P., Dong, X., Mei, F., Pekour, M., Hardin, J. C., and Ma, P.-L.: Earth System Model Aerosol-Cloud Diagnostics Package (ESMAC Diags) Version 2: Assessments of Aerosols, Clouds and Aerosol-Cloud Interactions Through Field Campaign and Long-Term Observations, Geosci. Model Dev. Discuss. [preprint], https://doi.org/10.5194/gmd-2023-51, in review, 2023.
Terai, C. R., Pritchard, M. S., Blossey, P., and Bretherton, C. S.: The impact of resolving subkilometer processes on aerosol-cloud interactions of low-level clouds in global model simulations, J. Adv. Model. Earth Syst., 12, e2020MS002274, https://doi.org/10.1029/2020MS002274, 2020.
Toll, V., Christensen, M., Gassó, S., and Bellouin, N.: Volcano and ship tracks indicate excessive aerosol-induced cloud water increases in a climate model, Geophys. Res. Lett., 44, 12492–12500, https://doi.org/10.1002/2017GL075280, 2017.
Turner, D. D., Clough, S. A., Liljegren, J. C., Clothiaux, E. E., Cady-Pereira, K. E., and Gaustad, K. L.: Retrieving liquid water path and precipitable water vapor from Atmospheric Radiation Measurement (ARM) microwave radiometers, IEEE T. Geosci. Remote, 45, 3680–3690, https://doi.org/10.1109/TGRS.2007.903703, 2007.
Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251–1256, https://doi.org/10.1016/0004-6981(74)90004-3, 1974.
Twomey, S.: The influence of pollution on the shortwave albedo of clouds, J. Atmos. Sci., 34, 1149–1152, https://doi.org/10.1175/1520-0469(1977)034<1149:TIOPOT>2.0.CO;2, 1977.
Varble, A., Ma, P.-L., Christensen, M., Mülmenstädt, J., Tang, S., and Fast, J.: EGUsphere-2023-998 Data and Code [Data set]. In Atmospheric Chemistry and Physics (Version 1), Zenodo [code and data set], https://doi.org/10.5281/zenodo.8436534, 2023.
Wang, H., Easter, R. C., Zhang, R., Ma, P.-L., Singh, B., Zhang, K., Ganguly, D., Rasch, P. J., Burrows, S. M., Ghan, S. J., Lou, S., Qian, Y., Yang, Y., Feng, Y., Flanner, M., Leung, L. R., Liu, X., Shrivastava, M., Sun, J., Tang, Q., Xie, S., and Yoon, J.-H.: Aerosols in the E3SM Version 1: New developments and their impacts on radiative forcing, J. Adv. Model. Earth Syst., 12, e2019MS001851, https://doi.org/10.1029/2019MS001851, 2020.
Wang, J., Wood, R., Jensen, M. P., Chiu, J. C., Liu, Y., Lamer, K., Desai, N., Giangrande, S. E., Knopf, D. A., Kollias, P., Laskin, A., Liu, X., Lu, C., Mechem, D., Mei, F., Starzec, M., Tomlinson, J., Wang, Y., Yum, S. S., Zheng, G., Aiken, A. C., Azevedo, E. B., Blanchard, Y., China, S., Dong, X., Gallo, F., Gao, S., Ghate, V. P., Glienke, S., Goldberger, L., Hardin, J. C., Kuang, C., Luke, E. P., Matthews, A. A., Miller, M. A., Moffet, R., Pekour, M., Schmid, B., Sedlacek, A. J., Shaw, R. A., Shilling, J. E., Sullivan, A., Suski, K., Veghte, D. P., Weber, R., Wyant, M., Yeom, J., Zawadowicz, M., and Zhang, Z.: Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA), B. Am. Meteorol. Soc., 103, E619–E641, https://doi.org/10.1175/BAMS-D-19-0220.1, 2022.
Witte, M. K., Yuan, T., Chuang, P. Y., Platnick, S., Meyer, K. G., Wind, G., and Jonsson, H. H.: MODIS retrievals of cloud effective radius in marine stratocumulus exhibit no significant bias, Geophys. Res. Lett., 45, 10656–10664, https://doi.org/10.1029/2018GL079325, 2018.
Wood, R., Wyant, M., Bretherton, C. S., Rémillard, J., Kollias, P., Fletcher, J., Stemmler, J., Szoeke, S. D., Yuter, S., Miller, M., Mechem, D., Tselioudis, G., Chiu, J. C., Mann, J. A. L., O'Connor, E. J., Hogan, R. J., Dong, X., Miller, M., Ghate, V., Jefferson, A., Min, Q., Minnis, P., Palikonda, R., Albrecht, B., Luke, E., Hannay, C., and Lin, Y.: Clouds, aerosol, and precipitation in the marine boundary layer: An ARM mobile facility deployment, B. Am. Meteorol. Soc., 96, 419–440, https://doi.org/10.1175/BAMS-D-13-00180.1, 2015.
Wu, P., Dong, X., Xi, B., Tian, J., and Ward, D. M.: Profiles of MBL cloud and drizzle microphysical properties retrieved from ground-based observations and validated by aircraft in situ measurements over the Azores, J. Geophys. Res.-Atmos., 125, e2019JD032205, https://doi.org/10.1029/2019JD032205, 2020a.
Wu, P., Dong, X., and Xi, B.: A Climatology of Marine Boundary Layer Cloud and Drizzle Properties Derived from Ground-Based Observations over the Azores, J. Climate, 33, 10133–10148, https://doi.org/10.1175/JCLI-D-20-0272.1, 2020b.
Xue, H. and Feingold, G.: Large-Eddy Simulations of Trade Wind Cumuli: Investigation of Aerosol Indirect Effects, J. Atmos. Sci., 63, 1605–1622, https://doi.org/10.1175/JAS3706.1, 2006.
Zhang, G. J. and McFarlane, N. A.: Sensitivity of climate simulations to the parameterization of cumulus convection in the Canadian climate center general-circulation model, Atmos.-Ocean, 33, 407–446, https://doi.org/10.1080/07055900.1995.9649539, 1995.
Zhang, J., Zhou, X., Goren, T., and Feingold, G.: Albedo susceptibility of northeastern Pacific stratocumulus: the role of covarying meteorological conditions, Atmos. Chem. Phys., 22, 861–880, https://doi.org/10.5194/acp-22-861-2022, 2022.
Zhang, K., Zhang, W., Wan, H., Rasch, P. J., Ghan, S. J., Easter, R. C., Shi, X., Wang, Y., Wang, H., Ma, P.-L., Zhang, S., Sun, J., Burrows, S. M., Shrivastava, M., Singh, B., Qian, Y., Liu, X., Golaz, J.-C., Tang, Q., Zheng, X., Xie, S., Lin, W., Feng, Y., Wang, M., Yoon, J.-H., and Leung, L. R.: Effective radiative forcing of anthropogenic aerosols in E3SM version 1: historical changes, causality, decomposition, and parameterization sensitivities, Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, 2022.
Zhang, Z., Oreopoulos, L., Lebsock, M. D., Mechem, D. B., and Covert, J.: Understanding the microphysical control and spatial-temporal variability of warm rain probability using CloudSat and MODIS observations, Geophys. Res. Lett., 49, e2022GL098863, https://doi.org/10.1029/2022GL098863, 2022.
Zheng, G., Wang, Y., Aiken, A. C., Gallo, F., Jensen, M. P., Kollias, P., Kuang, C., Luke, E., Springston, S., Uin, J., Wood, R., and Wang, J.: Marine boundary layer aerosol in the eastern North Atlantic: seasonal variations and key controlling processes, Atmos. Chem. Phys., 18, 17615–17635, https://doi.org/10.5194/acp-18-17615-2018, 2018.
Zheng, X., Klein, S. A., Ghate, V. P., Santos, S., McGibbon, J., Caldwell, P., Bogenschutz, P., Lin, W., and Cadeddu, M. P.: Assessment of precipitating marine stratocumulus clouds in the E3SMv1 Atmosphere Model: A case study from the ARM MAGIC field campaign, Mon. Weather Rev., 148, 3341–3359, https://doi.org/10.1175/MWR-D-19-0349.1, 2020.
Zheng, X., Xi, B., Dong, X., Wu, P., Logan, T., and Wang, Y.: Environmental effects on aerosol–cloud interaction in non-precipitating marine boundary layer (MBL) clouds over the eastern North Atlantic, Atmos. Chem. Phys., 22, 335–354, https://doi.org/10.5194/acp-22-335-2022, 2022.
Short summary
We evaluate how clouds change in response to changing atmospheric particle (aerosol) concentrations in a climate model and find that the model-predicted cloud brightness increases too much as aerosols increase because the cloud drop number increases too much. Excessive drizzle in the model mutes this difference. Many differences between observational and model estimates are explained by varying assumptions of how much liquid has been lost in clouds, which impacts the estimated cloud drop number.
We evaluate how clouds change in response to changing atmospheric particle (aerosol)...
Altmetrics
Final-revised paper
Preprint