Articles | Volume 20, issue 4
https://doi.org/10.5194/acp-20-2177-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-2177-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
The day-to-day co-variability between mineral dust and cloud glaciation: a proxy for heterogeneous freezing
Diego Villanueva
CORRESPONDING AUTHOR
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Bernd Heinold
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Patric Seifert
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Hartwig Deneke
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Martin Radenz
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Ina Tegen
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Related authors
No articles found.
Sofía Gómez Maqueo Anaya, Sudharaj Aryasree, Konrad Kandler, Eduardo José dos Santos Souza, Khanneh Wadinga Fomba, Dietrich Althausen, Maria Kezoudi, Matthias Faust, Bernd Heinold, Ina Tegen, Moritz Haarig, Holger Baars, and Kerstin Schepanski
EGUsphere, https://doi.org/10.5194/egusphere-2026-23, https://doi.org/10.5194/egusphere-2026-23, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
During the JATAC 2022 campaign in Cape Verde, Saharan dust aerosols were collected and analyzed for mineral composition. Mineralogy is crucial for dust–radiation and dust–cloud interactions. We improve dust representation in an atmospheric model by refining the translation of soil into aerosol particle size distributions. Validation with mineral and elemental measurements shows improved representation of some minerals and reveals biases missed by mineral-only comparisons.
Hannes Jascha Griesche, Ronny Engelmann, Martin Radenz, Julian Hofer, Dietrich Althausen, Albert Ansmann, Kevin Barry, Jessie Creamean, Cristofer Jimenez, and Patric Seifert
EGUsphere, https://doi.org/10.5194/egusphere-2025-5708, https://doi.org/10.5194/egusphere-2025-5708, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
A full annual cycle of mixed-phase ice-formation temperatures in the high Arctic is presented. Ship-based remote sensing with lidar and cloud radar from the Arctic expedition MOSAiC was used to investigate the impact of surface processes on mixed-phase cloud properties. Surface mixed-layer cloud coupling was derived base on radiosonde profiles. Combined with INP filter samples, sea ice concentration and back-trajectory analysis an influence of surface processes on the cloud properties was found.
Jonas Witthuhn, Hartwig Deneke, Andreas Macke, Oscar Ritter, Jens Redemann, Connor J. Flynn, Abdulamid A. Fakoya, Bradley F. Lamkin, Emily D. Lenhardt, Logan T. Mitchell, Emily K. West, David M. Romps, Rusen Öktem, and Heike Kalesse-Los
EGUsphere, https://doi.org/10.5194/egusphere-2025-5808, https://doi.org/10.5194/egusphere-2025-5808, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
This study examines how solar irradiance changes when sunlight passes from clear sky into cloud shadows, focusing on 3‑D radiative effects of shallow cumulus clouds. Using data from a dense pyranometer network and cloud masks from cameras we found that irradiance can rise up to 20 % above clear‑sky levels near cloud edges. Key drivers include sun‑cloud geometry and microphysical cloud properties. The results highlight the need to incorporate such 3‑D effects in atmospheric models.
Kevin Ohneiser, Patric Seifert, Willi Schimmel, Fabian Senf, Tom Gaudek, Martin Radenz, Audrey Teisseire, Veronika Ettrichrätz, Teresa Vogl, Nina Maherndl, Nils Pfeifer, Jan Henneberger, Anna J. Miller, Nadja Omanovic, Christopher Fuchs, Huiying Zhang, Fabiola Ramelli, Robert Spirig, Anton Kötsche, Heike Kalesse-Los, Maximilian Maahn, Heather Corden, Alexis Berne, Majid Hajipour, Hannes Griesche, Julian Hofer, Ronny Engelmann, Annett Skupin, Albert Ansmann, and Holger Baars
Atmos. Chem. Phys., 25, 17363–17386, https://doi.org/10.5194/acp-25-17363-2025, https://doi.org/10.5194/acp-25-17363-2025, 2025
Short summary
Short summary
This study focuses on a seeder-feeder cloud system on 8 Jan 2024 in Eriswil, Switzerland. It is shown how the interaction of these cloud systems changes the cloud microphysical properties and the precipitation patterns. A big set of advanced remote-sensing techniques and retrieval algorithms are applied, so that a detailed view on the seeder-feeder cloud system is available. The gained knowledge can be used to improve weather models and weather forecasts.
Cristofer Jimenez, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Ronny Engelmann, Martin Radenz, Julian Hofer, Dietrich Althausen, Daniel A. Knopf, Sandro Dahlke, Johannes Bühl, Holger Baars, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 25, 12955–12981, https://doi.org/10.5194/acp-25-12955-2025, https://doi.org/10.5194/acp-25-12955-2025, 2025
Short summary
Short summary
We studied the water and ice phases of Arctic mixed-phase clouds (MPCs) using dual FOV polarization lidar and Doppler radar on board Polarstern during the MOSAiC expedition. Two long-lasting Arctic MPCs and year-round statistics show persistent droplet activation and dominant immersion freezing, indicating well-filled cloud condensation nuclei and ice-nucleating particle reservoirs. These findings help explain MPC longevity and may improve cloud life cycle representation in weather and climate models.
Hanna Wiedenhaus, Roland Schrödner, Ralf Wolke, Marie L. Luttkus, Shubhi Arora, Laurent Poulain, Radek Lhotka, Petr Vodička, Jaroslav Schwarz, Petra Pokorna, Jakub Ondráček, Vladimir Ždímal, Hartmut Herrmann, and Ina Tegen
Atmos. Chem. Phys., 25, 12893–12922, https://doi.org/10.5194/acp-25-12893-2025, https://doi.org/10.5194/acp-25-12893-2025, 2025
Short summary
Short summary
This study examines winter air quality in central Europe, focusing on the impact of domestic heating. Using a chemical transport model and measurements, it was found that the model underestimated organic particle concentrations. This was due to an underestimation of gases from domestic heating that form secondary organic particles. Improving the model by increasing these emissions and the particle formation led to better results, demonstrating the important role of heating emissions in winter.
Friederike Keil, Markus Quante, Bernd Heinold, and Volker Matthias
EGUsphere, https://doi.org/10.5194/egusphere-2025-4374, https://doi.org/10.5194/egusphere-2025-4374, 2025
Short summary
Short summary
Using model simulations, we studied convective weather events to see how urban aerosol emissions influence cloud microphysics and precipitation. By tracing urban air masses from convective clouds back to their emission sources, we could isolate the effects of emissions. The results show a significant influence of urban emissions. Depending on the weather, urban emissions can either delay, enhance, or suppress precipitation, highlighting cities' complex role in shaping local rainfall.
Majid Hajipour, Patric Seifert, Hannes Griesche, Kevin Ohneiser, and Martin Radenz
Atmos. Meas. Tech., 18, 5199–5222, https://doi.org/10.5194/amt-18-5199-2025, https://doi.org/10.5194/amt-18-5199-2025, 2025
Short summary
Short summary
This study presents an approach that enables the detection of the shape and orientation of multiple types of co-located hydrometeors in mixed-phase cloud systems. This information is key for improving the understanding of these clouds, as they do contain ice and liquid water simultaneously, making them relevant for the precipitation budget and radiative balance of the Earth's atmosphere. The retrieval is based on elevation scans of polarimetric cloud radars and can therefore be flexibly applied.
Christopher Fuchs, Fabiola Ramelli, Anna J. Miller, Nadja Omanovic, Robert Spirig, Huiying Zhang, Patric Seifert, Kevin Ohneiser, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 25, 12177–12196, https://doi.org/10.5194/acp-25-12177-2025, https://doi.org/10.5194/acp-25-12177-2025, 2025
Short summary
Short summary
We quantify diffusional ice crystal growth in natural clouds using cloud seeding experiments. We report growth rates for 14 experiments between −5.1 °C and −8.3 °C and observe strong variations depending on the cloud characteristics. Comparing our growth rates to laboratory data, we found similar temperature-dependent trends, but the laboratory rates are higher. These data fill the gap in quantitative in situ observation of ice crystal growth, helping to validate models and laboratory experiments.
Moritz Zeising, Laurent Oziel, Silke Thoms, Özgür Gürses, Judith Hauck, Bernd Heinold, Svetlana N. Losa, Manuela van Pinxteren, Christoph Völker, Sebastian Zeppenfeld, and Astrid Bracher
EGUsphere, https://doi.org/10.5194/egusphere-2025-4190, https://doi.org/10.5194/egusphere-2025-4190, 2025
Short summary
Short summary
We assess the implementation of additional organic carbon pathways into a global setup of a numerical model, which simulates the ocean circulation, sea ice, and biogeochemical processes. With a focus on the Arctic Ocean, this model tracks the temporal and spatial dynamics of phytoplankton, exudation of organic carbon, and its aggregation to so-called transparent exopolymer particles. We evaluate the simulation using measurements from ship-based and remote-sensing campaigns in the Arctic Ocean.
Tom Gaudek, Cristofer Jimenez, Kevin Ohneiser, Christopher Fuchs, Jan Henneberger, Johannes Bühl, Andi Klamt, Albert Ansmann, Ronny Engelmann, and Patric Seifert
EGUsphere, https://doi.org/10.5194/egusphere-2025-4105, https://doi.org/10.5194/egusphere-2025-4105, 2025
Short summary
Short summary
This study introduces the maximum diameter (Dmax) of precipitation particles measured by a two-dimensional video disdrometer (2DVD) as a novel parameter. Dmax is applied in a cloud seeding study during the Cloudlab campaign and, for the first time, in a MOSAiC case to evaluate the LIRAS-ice remote-sensing retrieval of in-cloud ice crystal size and number. Both quantities agreed well with the 2DVD measurements under ideal conditions, highlighting the potential of Dmax for precipitation studies.
Audrey Teisseire, Patric Seifert, Kevin Ohneiser, Maximilian Maahn, Robert Spirig, and Jan Henneberger
EGUsphere, https://doi.org/10.5194/egusphere-2025-3923, https://doi.org/10.5194/egusphere-2025-3923, 2025
Short summary
Short summary
This study evaluates the vertical distribution of particle shape (VDPS) method for identifying particle shapes and riming/aggregation using in-situ and multi-frequency radar data from the CLOUDLAB campaign. Despite non-Rayleigh scattering effects, results show that the VDPS method using a Ka-band scanning cloud radar in slanted depolarization ratio (SLDR) mode is effective for hydrometeor classification.
Marcus Klingebiel, André Ehrlich, Micha Gryschka, Nils Risse, Nina Maherndl, Imke Schirmacher, Sophie Rosenburg, Sabine Hörnig, Manuel Moser, Evelyn Jäkel, Michael Schäfer, Hartwig Deneke, Mario Mech, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 25, 9787–9801, https://doi.org/10.5194/acp-25-9787-2025, https://doi.org/10.5194/acp-25-9787-2025, 2025
Short summary
Short summary
Our study is using aircraft measurements from the HALO-(𝒜𝒞)³ campaign to investigate the transition from organized Arctic cloud street structures to more scattered clouds, which we call isotropic cloud patterns. We show that lower wind speeds cause this transition. In addition, we look at the changes in the cloud coverage, the height of the clouds, the cloud particles, and the radiative properties.
Simone Pulimeno, Angelo Lupi, Vito Vitale, Claudia Frangipani, Carlos Toledano, Stelios Kazadzis, Natalia Kouremeti, Christoph Ritter, Sandra Graßl, Kerstin Stebel, Vitali Fioletov, Ihab Abboud, Sandra Blindheim, Lynn Ma, Norm O’Neill, Piotr Sobolewski, Pawan Gupta, Elena Lind, Thomas F. Eck, Antti Hyvärinen, Veijo Aaltonen, Rigel Kivi, Janae Csavina, Dmitry Kabanov, Sergey M. Sakerin, Olga R. Sidorova, Robert S. Stone, Hagen Telg, Laura Riihimaki, Raul R. Cordero, Martin Radenz, Ronny Engelmann, Michel Van Roozendal, Anatoli Chaikovsky, Philippe Goloub, Junji Hisamitsu, and Mauro Mazzola
EGUsphere, https://doi.org/10.5194/egusphere-2025-2527, https://doi.org/10.5194/egusphere-2025-2527, 2025
Short summary
Short summary
This study analyzed aerosols optical properties over the Arctic and Antarctic to measure them even during long periods of darkness. It found that pollution in the Arctic is decreasing, likely due to European emission regulations, while wildfires are becoming a more important source of particles. In Antarctica, particle levels are higher near the coast than inland, and vary by season. These results help us better understand how air pollution and climate are changing at the Earth’s poles.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Julian Hofer, Moritz Haarig, Ulla Wandinger, Bernd Heinold, Ina Tegen, Matthias Faust, Holger Baars, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
Atmos. Chem. Phys., 25, 9737–9764, https://doi.org/10.5194/acp-25-9737-2025, https://doi.org/10.5194/acp-25-9737-2025, 2025
Short summary
Short summary
This study investigates how hematite in Sahara dust affects how dust particles interact with radiation. Using lidar data from Cabo Verde (2021–2022) and hematite content from atmospheric model simulations, the results show that a higher hematite fraction leads to a decrease in the particle backscattering coefficients in a spectrally different way. These findings can improve the representation of mineral dust in climate models, particularly regarding their radiative effect.
Job I. Wiltink, Hartwig Deneke, Chiel C. van Heerwaarden, and Jan Fokke Meirink
Atmos. Meas. Tech., 18, 3917–3936, https://doi.org/10.5194/amt-18-3917-2025, https://doi.org/10.5194/amt-18-3917-2025, 2025
Short summary
Short summary
Global horizontal irradiance retrievals from satellite observations are affected by spatial displacements due to parallax and cloud shadows. We assess different approaches to correct for these displacements and quantify their added value by comparison with a network of ground-based pyranometer observations. The corrections are found to become increasingly important at higher spatial resolutions and are most relevant for variable cloud types.
Kevin Ohneiser, Markus Hartmann, Heike Wex, Patric Seifert, Anja Hardt, Anna Miller, Katharina Baudrexl, Werner Thomas, Veronika Ettrichrätz, Maximilian Maahn, Tom Gaudek, Willi Schimmel, Fabian Senf, Hannes Griesche, Martin Radenz, and Jan Henneberger
EGUsphere, https://doi.org/10.5194/egusphere-2025-3675, https://doi.org/10.5194/egusphere-2025-3675, 2025
Short summary
Short summary
This study highlights the efficiency of supercooled stratus clouds to remove ice-nucleating particles (INPs). In our measurement scenarios within the planetary boundary layer lower concentrations of INP under supercooled stratus conditions were found than with temperatures above freezing. Within the free troposphere a lot more INPs were found to be available which means that the free troposphere must be taken into account as an important source of INPs.
Zhaolong Wu, Patric Seifert, Yun He, Holger Baars, Haoran Li, Cristofer Jimenez, Chengcai Li, and Albert Ansmann
Atmos. Meas. Tech., 18, 3611–3634, https://doi.org/10.5194/amt-18-3611-2025, https://doi.org/10.5194/amt-18-3611-2025, 2025
Short summary
Short summary
This study introduces a novel method to detect horizontally oriented ice crystals (HOICs) using two ground-based polarization lidars at different zenith angles, based on a yearlong dataset collected in Beijing. Combined with cloud radar and reanalysis data, the fine categorization results reveal HOICs occur in calm winds and moderately cold temperatures and are influenced by turbulence near cloud bases. The results enhance our understanding of cloud processes and improve atmospheric models.
Hossein Panahifar, Maria Poutli, George Kotsias, Argyro Nisantzi, Silas Michaelides, Diofantos Hadjimitsis, Patric Seifert, Albert Ansmann, and Rodanthi-Elisavet Mamouri
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLVIII-G-2025, 1153–1158, https://doi.org/10.5194/isprs-archives-XLVIII-G-2025-1153-2025, https://doi.org/10.5194/isprs-archives-XLVIII-G-2025-1153-2025, 2025
Anisbel Leon-Marcos, Moritz Zeising, Manuela van Pinxteren, Sebastian Zeppenfeld, Astrid Bracher, Elena Barbaro, Anja Engel, Matteo Feltracco, Ina Tegen, and Bernd Heinold
Geosci. Model Dev., 18, 4183–4213, https://doi.org/10.5194/gmd-18-4183-2025, https://doi.org/10.5194/gmd-18-4183-2025, 2025
Short summary
Short summary
This study represents the primary marine organic aerosol (PMOA) emissions, focusing on their sea–atmosphere transfer. Using the FESOM2.1–REcoM3 model, concentrations of key organic biomolecules were estimated and integrated into the ECHAM6.3–HAM2.3 aerosol–climate model. Results highlight the influence of marine biological activity and surface winds on PMOA emissions, with reasonably good agreement with observations improving aerosol representation in the southern oceans.
Anisbel Leon-Marcos, Manuela van Pinxteren, Sebastian Zeppenfeld, Moritz Zeising, Astrid Bracher, Laurent Oziel, Ina Tegen, and Bernd Heinold
EGUsphere, https://doi.org/10.5194/egusphere-2025-2829, https://doi.org/10.5194/egusphere-2025-2829, 2025
Short summary
Short summary
This study links modelled ocean surface concentrations of key marine organic groups with the aerosol-climate model ECHAM-HAM to quantify species-resolved primary marine organic aerosol emissions from 1990 to 2019. Results show strong seasonality, driven by productivity and summer sea ice loss. Emissions and burdens increased over time with more frequent positive anomalies in the last decade, revealing an overall upward trend with regional differences across the Arctic and aerosol species.
Albert Ansmann, Cristofer Jimenez, Johanna Roschke, Johannes Bühl, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Daniel A. Knopf, Sandro Dahlke, Tom Gaudek, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 25, 4847–4866, https://doi.org/10.5194/acp-25-4847-2025, https://doi.org/10.5194/acp-25-4847-2025, 2025
Short summary
Short summary
In this study, we focus on the potential impact of wildfire smoke on cirrus formation. For the first time, state-of-the-art aerosol and cirrus observations with lidar and radar, presented in this paper (Part 1 of a series of two articles), are closely linked to the comprehensive modeling of gravity-wave-induced ice nucleation in cirrus evolution processes, presented in a companion paper (Part 2). We found a clear impact of wildfire smoke on cirrus evolution.
Benedikt Gast, Cristofer Jimenez, Albert Ansmann, Moritz Haarig, Ronny Engelmann, Felix Fritzsch, Athena A. Floutsi, Hannes Griesche, Kevin Ohneiser, Julian Hofer, Martin Radenz, Holger Baars, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 25, 3995–4011, https://doi.org/10.5194/acp-25-3995-2025, https://doi.org/10.5194/acp-25-3995-2025, 2025
Short summary
Short summary
In this study, we discuss the enhanced detection capabilities of a fluorescence lidar in the case of optically thin aerosol layers in the upper troposphere and lower stratosphere (UTLS) region. Our results suggest that such thin aerosol layers are not so rare in the UTLS and can potentially trigger and impact cirrus cloud formation through heterogeneous ice nucleation. By altering the microphysical cloud properties, this could affect clouds' evolution and lifetime and thus their climate effect.
Carola Barrientos-Velasco, Christopher J. Cox, Hartwig Deneke, J. Brant Dodson, Anja Hünerbein, Matthew D. Shupe, Patrick C. Taylor, and Andreas Macke
Atmos. Chem. Phys., 25, 3929–3960, https://doi.org/10.5194/acp-25-3929-2025, https://doi.org/10.5194/acp-25-3929-2025, 2025
Short summary
Short summary
Understanding how clouds affect the climate, especially in the Arctic, is crucial. This study used data from the largest polar expedition in history, MOSAiC, and the CERES satellite to analyse the impact of clouds on radiation. Simulations showed accurate results, aligning with observations. Over the year, clouds caused the atmospheric surface system to lose 5.2 W m−² of radiative energy to space, while the surface gained 25 W m−² and the atmosphere cooled by 30.2 W m−².
Audrey Teisseire, Anne-Claire Billault-Roux, Teresa Vogl, and Patric Seifert
Atmos. Meas. Tech., 18, 1499–1517, https://doi.org/10.5194/amt-18-1499-2025, https://doi.org/10.5194/amt-18-1499-2025, 2025
Short summary
Short summary
This study demonstrates the ability of a new method delivering the vertical distribution of particle shape to highlight riming and aggregation processes, identifying graupel and aggregates, respectively, as isometric particles. The distinction between these processes can be achieved using lidar or spectral techniques, as demonstrated in the case studies. The capability of the new method to identify rimed particles and aggregates without differentiating them can simplify statistical work.
Teresa Vogl, Martin Radenz, Fabiola Ramelli, Rosa Gierens, and Heike Kalesse-Los
Atmos. Meas. Tech., 17, 6547–6568, https://doi.org/10.5194/amt-17-6547-2024, https://doi.org/10.5194/amt-17-6547-2024, 2024
Short summary
Short summary
In this study, we present a toolkit of two Python algorithms to extract information from Doppler spectra measured by ground-based cloud radars. In these Doppler spectra, several peaks can be formed due to populations of droplets/ice particles with different fall velocities coexisting in the same measurement time and height. The two algorithms can detect peaks and assign them to certain particle types, such as small cloud droplets or fast-falling ice particles like graupel.
Job I. Wiltink, Hartwig Deneke, Yves-Marie Saint-Drenan, Chiel C. van Heerwaarden, and Jan Fokke Meirink
Atmos. Meas. Tech., 17, 6003–6024, https://doi.org/10.5194/amt-17-6003-2024, https://doi.org/10.5194/amt-17-6003-2024, 2024
Short summary
Short summary
Meteosat Spinning Enhanced Visible and Infrared Imager (SEVIRI) global horizontal irradiance (GHI) retrievals are validated at standard and increased spatial resolution against a network of 99 pyranometers. GHI accuracy is strongly dependent on the cloud regime. Days with variable cloud conditions show significant accuracy improvements when retrieved at higher resolution. We highlight the benefits of dense network observations and a cloud-regime-resolved approach in validating GHI retrievals.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
Short summary
Short summary
The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Zili He, Quentin Libois, Najda Villefranque, Hartwig Deneke, Jonas Witthuhn, and Fleur Couvreux
Atmos. Chem. Phys., 24, 11391–11408, https://doi.org/10.5194/acp-24-11391-2024, https://doi.org/10.5194/acp-24-11391-2024, 2024
Short summary
Short summary
This study uses observations and simulations to analyze how cumulus clouds affect spacial solar radiation variability on the ground. Results show that the simulations reproduce the observations well and improve understanding of cloud impacts on radiation. The research also indicates that a few strategically placed sensors, capitalizing on measurement timing, can effectively measure these variations, aiding in the development of detailed weather prediction models.
Andreas Walbröl, Janosch Michaelis, Sebastian Becker, Henning Dorff, Kerstin Ebell, Irina Gorodetskaya, Bernd Heinold, Benjamin Kirbus, Melanie Lauer, Nina Maherndl, Marion Maturilli, Johanna Mayer, Hanno Müller, Roel A. J. Neggers, Fiona M. Paulus, Johannes Röttenbacher, Janna E. Rückert, Imke Schirmacher, Nils Slättberg, André Ehrlich, Manfred Wendisch, and Susanne Crewell
Atmos. Chem. Phys., 24, 8007–8029, https://doi.org/10.5194/acp-24-8007-2024, https://doi.org/10.5194/acp-24-8007-2024, 2024
Short summary
Short summary
To support the interpretation of the data collected during the HALO-(AC)3 campaign, which took place in the North Atlantic sector of the Arctic from 7 March to 12 April 2022, we analyze how unusual the weather and sea ice conditions were with respect to the long-term climatology. From observations and ERA5 reanalysis, we found record-breaking warm air intrusions and a large variety of marine cold air outbreaks. Sea ice concentration was mostly within the climatological interquartile range.
Nadja Omanovic, Sylvaine Ferrachat, Christopher Fuchs, Jan Henneberger, Anna J. Miller, Kevin Ohneiser, Fabiola Ramelli, Patric Seifert, Robert Spirig, Huiying Zhang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 6825–6844, https://doi.org/10.5194/acp-24-6825-2024, https://doi.org/10.5194/acp-24-6825-2024, 2024
Short summary
Short summary
We present simulations with a high-resolution numerical weather prediction model to study the growth of ice crystals in low clouds following glaciogenic seeding. We show that the simulated ice crystals grow slower than observed and do not consume as many cloud droplets as measured in the field. This may have implications for forecasting precipitation, as the ice phase is crucial for precipitation at middle and high latitudes.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
Short summary
Short summary
Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Henriette Gebauer, Athena Augusta Floutsi, Moritz Haarig, Martin Radenz, Ronny Engelmann, Dietrich Althausen, Annett Skupin, Albert Ansmann, Cordula Zenk, and Holger Baars
Atmos. Chem. Phys., 24, 5047–5067, https://doi.org/10.5194/acp-24-5047-2024, https://doi.org/10.5194/acp-24-5047-2024, 2024
Short summary
Short summary
Sulfate aerosol from the volcanic eruption at La Palma in 2021 was observed over Cabo Verde. We characterized the aerosol burden based on a case study of lidar and sun photometer observations. We compared the volcanic case to the typical background conditions (reference case) to quantify the volcanic pollution. We show the first ever measurements of the extinction coefficient, lidar ratio and depolarization ratio at 1064 nm for volcanic sulfate.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Matthias Faust, Holger Baars, Bernd Heinold, Julian Hofer, Ina Tegen, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
Geosci. Model Dev., 17, 1271–1295, https://doi.org/10.5194/gmd-17-1271-2024, https://doi.org/10.5194/gmd-17-1271-2024, 2024
Short summary
Short summary
Mineral dust aerosol particles vary greatly in their composition depending on source region, which leads to different physicochemical properties. Most atmosphere–aerosol models consider mineral dust aerosols to be compositionally homogeneous, which ultimately increases model uncertainty. Here, we present an approach to explicitly consider the heterogeneity of the mineralogical composition for simulations of the Saharan atmospheric dust cycle with regard to dust transport towards the Atlantic.
Audrey Teisseire, Patric Seifert, Alexander Myagkov, Johannes Bühl, and Martin Radenz
Atmos. Meas. Tech., 17, 999–1016, https://doi.org/10.5194/amt-17-999-2024, https://doi.org/10.5194/amt-17-999-2024, 2024
Short summary
Short summary
The vertical distribution of particle shape (VDPS) method, introduced in this study, aids in characterizing the density-weighted shape of cloud particles from scanning slanted linear depolarization ratio (SLDR)-mode cloud radar observations. The VDPS approach represents a new, versatile way to study microphysical processes by combining a spheroidal scattering model with real measurements of SLDR.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
Short summary
Short summary
An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Anja Hünerbein, Sebastian Bley, Hartwig Deneke, Jan Fokke Meirink, Gerd-Jan van Zadelhoff, and Andi Walther
Atmos. Meas. Tech., 17, 261–276, https://doi.org/10.5194/amt-17-261-2024, https://doi.org/10.5194/amt-17-261-2024, 2024
Short summary
Short summary
The ESA cloud, aerosol and radiation mission EarthCARE will provide active profiling and passive imaging measurements from a single satellite platform. The passive multi-spectral imager (MSI) will add information in the across-track direction. We present the cloud optical and physical properties algorithm, which combines the visible to infrared MSI channels to determine the cloud top pressure, optical thickness, particle size and water path.
Hannes Jascha Griesche, Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 24, 597–612, https://doi.org/10.5194/acp-24-597-2024, https://doi.org/10.5194/acp-24-597-2024, 2024
Short summary
Short summary
The Arctic is strongly affected by climate change and the role of clouds therein is not yet completely understood. Measurements from the Arctic expedition PS106 were used to simulate radiative fluxes with and without clouds at very low altitudes (below 165 m), and their radiative effect was calculated to be 54 Wm-2. The low heights of these clouds make them hard to observe. This study shows the importance of accurate measurements and simulations of clouds and gives suggestions for improvements.
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
Short summary
Short summary
For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Michael Weger and Bernd Heinold
Atmos. Chem. Phys., 23, 13769–13790, https://doi.org/10.5194/acp-23-13769-2023, https://doi.org/10.5194/acp-23-13769-2023, 2023
Short summary
Short summary
This study investigates the effects of complex terrain on air pollution trapping using a numerical model which simulates the dispersion of emissions under real meteorological conditions. The additionally simulated aerosol age allows us to distinguish areas that accumulate aerosol over time from areas that are more influenced by fresh emissions. The Dresden Basin, a widened section of the Elbe Valley in eastern Germany, is selected as the target area in a case study to demonstrate the concept.
James Barry, Stefanie Meilinger, Klaus Pfeilsticker, Anna Herman-Czezuch, Nicola Kimiaie, Christopher Schirrmeister, Rone Yousif, Tina Buchmann, Johannes Grabenstein, Hartwig Deneke, Jonas Witthuhn, Claudia Emde, Felix Gödde, Bernhard Mayer, Leonhard Scheck, Marion Schroedter-Homscheidt, Philipp Hofbauer, and Matthias Struck
Atmos. Meas. Tech., 16, 4975–5007, https://doi.org/10.5194/amt-16-4975-2023, https://doi.org/10.5194/amt-16-4975-2023, 2023
Short summary
Short summary
Measured power data from solar photovoltaic (PV) systems contain information about the state of the atmosphere. In this work, power data from PV systems in the Allgäu region in Germany were used to determine the solar irradiance at each location, using state-of-the-art simulation and modelling. The results were validated using concurrent measurements of the incoming solar radiation in each case. If applied on a wider scale, this algorithm could help improve weather and climate models.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
Short summary
Short summary
The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Suvarna Fadnavis, Bernd Heinold, T. P. Sabin, Anne Kubin, Katty Huang, Alexandru Rap, and Rolf Müller
Atmos. Chem. Phys., 23, 10439–10449, https://doi.org/10.5194/acp-23-10439-2023, https://doi.org/10.5194/acp-23-10439-2023, 2023
Short summary
Short summary
The influence of the COVID-19 lockdown on the Himalayas caused increases in snow cover and a decrease in runoff, ultimately leading to an enhanced snow water equivalent. Our findings highlight that, out of the two processes causing a retreat of Himalayan glaciers – (1) slow response to global climate change and (2) fast response to local air pollution – a policy action on the latter is more likely to be within the reach of possible policy action to help billions of people in southern Asia.
Holger Baars, Joshua Walchester, Elizaveta Basharova, Henriette Gebauer, Martin Radenz, Johannes Bühl, Boris Barja, Ulla Wandinger, and Patric Seifert
Atmos. Meas. Tech., 16, 3809–3834, https://doi.org/10.5194/amt-16-3809-2023, https://doi.org/10.5194/amt-16-3809-2023, 2023
Short summary
Short summary
In 2018, the Aeolus satellite of the European Space Agency (ESA) was launched to improve weather forecasts through global measurements of wind profiles. Given the novel lidar technique onboard, extensive validation efforts have been needed to verify the observations. For this reason, we performed long-term validation measurements in Germany and Chile. We found significant improvement in the data products due to a new algorithm version and can confirm the general validity of Aeolus observations.
Fabian Senf, Bernd Heinold, Anne Kubin, Jason Müller, Roland Schrödner, and Ina Tegen
Atmos. Chem. Phys., 23, 8939–8958, https://doi.org/10.5194/acp-23-8939-2023, https://doi.org/10.5194/acp-23-8939-2023, 2023
Short summary
Short summary
Wildfire smoke is a significant source of airborne atmospheric particles that can absorb sunlight. Extreme fires in particular, such as those during the 2019–2020 Australian wildfire season (Black Summer fires), can considerably affect our climate system. In the present study, we investigate the various effects of Australian smoke using a global climate model to clarify how the Earth's atmosphere, including its circulation systems, adjusted to the extraordinary amount of Australian smoke.
Anja Hünerbein, Sebastian Bley, Stefan Horn, Hartwig Deneke, and Andi Walther
Atmos. Meas. Tech., 16, 2821–2836, https://doi.org/10.5194/amt-16-2821-2023, https://doi.org/10.5194/amt-16-2821-2023, 2023
Short summary
Short summary
The Multi-Spectral Imager (MSI) on board the EarthCARE satellite will provide the information needed for describing the cloud and aerosol properties in the cross-track direction, complementing the measurements from the Cloud Profiling Radar, Atmospheric Lidar and Broad-Band Radiometer. The accurate discrimination between clear and cloudy pixels is an essential first step. Therefore, the cloud mask algorithm provides a cloud flag, cloud phase and cloud type product for the MSI observations.
Athena Augusta Floutsi, Holger Baars, Ronny Engelmann, Dietrich Althausen, Albert Ansmann, Stephanie Bohlmann, Birgit Heese, Julian Hofer, Thomas Kanitz, Moritz Haarig, Kevin Ohneiser, Martin Radenz, Patric Seifert, Annett Skupin, Zhenping Yin, Sabur F. Abdullaev, Mika Komppula, Maria Filioglou, Elina Giannakaki, Iwona S. Stachlewska, Lucja Janicka, Daniele Bortoli, Eleni Marinou, Vassilis Amiridis, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Boris Barja, and Ulla Wandinger
Atmos. Meas. Tech., 16, 2353–2379, https://doi.org/10.5194/amt-16-2353-2023, https://doi.org/10.5194/amt-16-2353-2023, 2023
Short summary
Short summary
DeLiAn is a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio) and the Ångström exponent. The data collection is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarization lidar measurements and currently covers two wavelengths, 355 and 532 nm, for 13 aerosol categories ranging from basic aerosol types to mixtures.
Samuel Kwakye, Heike Kalesse-Los, Maximilian Maahn, Patric Seifert, Roel van Klink, Christian Wirth, and Johannes Quaas
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-69, https://doi.org/10.5194/amt-2023-69, 2023
Publication in AMT not foreseen
Short summary
Short summary
Insect numbers in the atmosphere can be calculated using polarimetric weather radar but they have to be identified and separated from other echoes, especially weather phenomena. Here, the separation is demonstrated using three machine-learning algorithms and insect count data from suction traps and the nature of radar measurements of different radar echoes is revealed. Random forest is the best separating algorithm and insect echoes radar measurements are distinct.
Kevin Ohneiser, Albert Ansmann, Jonas Witthuhn, Hartwig Deneke, Alexandra Chudnovsky, Gregor Walter, and Fabian Senf
Atmos. Chem. Phys., 23, 2901–2925, https://doi.org/10.5194/acp-23-2901-2023, https://doi.org/10.5194/acp-23-2901-2023, 2023
Short summary
Short summary
This study shows that smoke layers can reach the tropopause via the self-lofting effect within 3–7 d in the absence of pyrocumulonimbus convection if the
aerosol optical thickness is larger than approximately 2 for a longer time period. When reaching the stratosphere, wildfire smoke can sensitively influence the stratospheric composition on a hemispheric scale and thus can affect the Earth’s climate and the ozone layer.
Willi Schimmel, Heike Kalesse-Los, Maximilian Maahn, Teresa Vogl, Andreas Foth, Pablo Saavedra Garfias, and Patric Seifert
Atmos. Meas. Tech., 15, 5343–5366, https://doi.org/10.5194/amt-15-5343-2022, https://doi.org/10.5194/amt-15-5343-2022, 2022
Short summary
Short summary
This study introduces the novel Doppler radar spectra-based machine learning approach VOODOO (reVealing supercOOled liquiD beyOnd lidar attenuatiOn). VOODOO is a powerful probability-based extension to the existing Cloudnet hydrometeor target classification, enabling the detection of liquid-bearing cloud layers beyond complete lidar attenuation via user-defined p* threshold. VOODOO performs best for (multi-layer) stratiform and deep mixed-phase clouds with liquid water path > 100 g m−2.
Albert Ansmann, Kevin Ohneiser, Alexandra Chudnovsky, Daniel A. Knopf, Edwin W. Eloranta, Diego Villanueva, Patric Seifert, Martin Radenz, Boris Barja, Félix Zamorano, Cristofer Jimenez, Ronny Engelmann, Holger Baars, Hannes Griesche, Julian Hofer, Dietrich Althausen, and Ulla Wandinger
Atmos. Chem. Phys., 22, 11701–11726, https://doi.org/10.5194/acp-22-11701-2022, https://doi.org/10.5194/acp-22-11701-2022, 2022
Short summary
Short summary
For the first time we present a systematic study on the impact of wildfire smoke on ozone depletion in the Arctic (2020) and Antarctic stratosphere (2020, 2021). Two major fire events in Siberia and Australia were responsible for the observed record-breaking stratospheric smoke pollution. Our analyses were based on lidar observations of smoke parameters (Polarstern, Punta Arenas) and NDACC Arctic and Antarctic ozone profiles as well as on Antarctic OMI satellite observations of column ozone.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
Short summary
Short summary
The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Bernd Heinold, Holger Baars, Boris Barja, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Nick Schutgens, Fabian Senf, Roland Schrödner, Diego Villanueva, and Ina Tegen
Atmos. Chem. Phys., 22, 9969–9985, https://doi.org/10.5194/acp-22-9969-2022, https://doi.org/10.5194/acp-22-9969-2022, 2022
Short summary
Short summary
The extreme 2019–2020 Australian wildfires produced massive smoke plumes lofted into the lower stratosphere by pyrocumulonimbus convection. Most climate models do not adequately simulate the injection height of such intense fires. By combining aerosol-climate modeling with prescribed pyroconvective smoke injection and lidar observations, this study shows the importance of the representation of the most extreme wildfire events for estimating the atmospheric energy budget.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
Short summary
Short summary
Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Hannes J. Griesche, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 22, 9313–9348, https://doi.org/10.5194/acp-22-9313-2022, https://doi.org/10.5194/acp-22-9313-2022, 2022
Short summary
Short summary
This article describes an intercomparison of radiative fluxes and cloud properties from satellite, shipborne observations, and 1D radiative transfer simulations. The analysis focuses on research for PS106 expedition aboard the German research vessel, Polarstern. The results are presented in detailed case studies, time series for the PS106 cruise and extended to the central Arctic region. The findings illustrate the main periods of agreement and discrepancies of both points of view.
Kevin Ohneiser, Albert Ansmann, Bernd Kaifler, Alexandra Chudnovsky, Boris Barja, Daniel A. Knopf, Natalie Kaifler, Holger Baars, Patric Seifert, Diego Villanueva, Cristofer Jimenez, Martin Radenz, Ronny Engelmann, Igor Veselovskii, and Félix Zamorano
Atmos. Chem. Phys., 22, 7417–7442, https://doi.org/10.5194/acp-22-7417-2022, https://doi.org/10.5194/acp-22-7417-2022, 2022
Short summary
Short summary
We present and discuss 2 years of long-term lidar observations of the largest stratospheric perturbation by wildfire smoke ever observed. The smoke originated from the record-breaking Australian fires in 2019–2020 and affects climate conditions and even the ozone layer in the Southern Hemisphere. The obvious link between dense smoke occurrence in the stratosphere and strong ozone depletion found in the Arctic and in the Antarctic in 2020 can be regarded as a new aspect of climate change.
Michael Weger, Holger Baars, Henriette Gebauer, Maik Merkel, Alfred Wiedensohler, and Bernd Heinold
Geosci. Model Dev., 15, 3315–3345, https://doi.org/10.5194/gmd-15-3315-2022, https://doi.org/10.5194/gmd-15-3315-2022, 2022
Short summary
Short summary
Numerical models are an important tool to assess the air quality in cities,
as they can provide near-continouos data in time and space. In this paper,
air pollution for an entire city is simulated at a high spatial resolution of 40 m.
At this spatial scale, the effects of buildings on the atmosphere,
like channeling or blocking of the air flow, are directly represented by diffuse obstacles in the used model CAIRDIO. For model validation, measurements from air-monitoring sites are used.
Birgit Heese, Athena Augusta Floutsi, Holger Baars, Dietrich Althausen, Julian Hofer, Alina Herzog, Silke Mewes, Martin Radenz, and Yoav Y. Schechner
Atmos. Chem. Phys., 22, 1633–1648, https://doi.org/10.5194/acp-22-1633-2022, https://doi.org/10.5194/acp-22-1633-2022, 2022
Short summary
Short summary
The aerosol distribution over Haifa, Israel, was measured for 2 years by a laser-based vertically resolved measurement technique called lidar. From these data, the aerosol types and their percentages of the observed aerosol mixtures were identified in terms of their size and shape. We found mostly desert dust from the surrounding deserts and sea salt from the close-by Mediterranean Sea. But aerosols from anthropogenic and industrial pollution from local and far away sources were also detected.
Heike Kalesse-Los, Willi Schimmel, Edward Luke, and Patric Seifert
Atmos. Meas. Tech., 15, 279–295, https://doi.org/10.5194/amt-15-279-2022, https://doi.org/10.5194/amt-15-279-2022, 2022
Short summary
Short summary
It is important to detect the vertical distribution of cloud droplets and ice in mixed-phase clouds. Here, an artificial neural network (ANN) previously developed for Arctic clouds is applied to a mid-latitudinal cloud radar data set. The performance of this technique is contrasted to the Cloudnet target classification. For thick/multi-layer clouds, the machine learning technique is better at detecting liquid than Cloudnet, but if lidar data are available Cloudnet is at least as good as the ANN.
Moritz Haarig, Albert Ansmann, Ronny Engelmann, Holger Baars, Carlos Toledano, Benjamin Torres, Dietrich Althausen, Martin Radenz, and Ulla Wandinger
Atmos. Chem. Phys., 22, 355–369, https://doi.org/10.5194/acp-22-355-2022, https://doi.org/10.5194/acp-22-355-2022, 2022
Short summary
Short summary
The irregular shape of dust particles makes it difficult to treat them correctly in optical models. Atmospheric measurements of dust optical properties are therefore of great importance. The present study increases the space of observed parameters from 355 and 532 nm towards 1064 nm, which is of special importance for large dust particles. The lidar ratio influenced by mineralogy and the depolarization ratio influenced by shape are measured for the first time at all three wavelengths.
Martin Radenz, Johannes Bühl, Patric Seifert, Holger Baars, Ronny Engelmann, Boris Barja González, Rodanthi-Elisabeth Mamouri, Félix Zamorano, and Albert Ansmann
Atmos. Chem. Phys., 21, 17969–17994, https://doi.org/10.5194/acp-21-17969-2021, https://doi.org/10.5194/acp-21-17969-2021, 2021
Short summary
Short summary
This study brings together long-term ground-based remote-sensing observations of mixed-phase clouds at three key locations of aerosol–cloud interactions in the Northern and Southern Hemisphere midlatitudes. The findings contribute several new aspects on the nature of the excess of supercooled liquid clouds in the Southern Hemisphere, such as a long-term lidar-based estimate of ice-nucleating particle profiles as well as the effects of boundary layer coupling and gravity waves on ice formation.
Silke Trömel, Clemens Simmer, Ulrich Blahak, Armin Blanke, Sabine Doktorowski, Florian Ewald, Michael Frech, Mathias Gergely, Martin Hagen, Tijana Janjic, Heike Kalesse-Los, Stefan Kneifel, Christoph Knote, Jana Mendrok, Manuel Moser, Gregor Köcher, Kai Mühlbauer, Alexander Myagkov, Velibor Pejcic, Patric Seifert, Prabhakar Shrestha, Audrey Teisseire, Leonie von Terzi, Eleni Tetoni, Teresa Vogl, Christiane Voigt, Yuefei Zeng, Tobias Zinner, and Johannes Quaas
Atmos. Chem. Phys., 21, 17291–17314, https://doi.org/10.5194/acp-21-17291-2021, https://doi.org/10.5194/acp-21-17291-2021, 2021
Short summary
Short summary
The article introduces the ACP readership to ongoing research in Germany on cloud- and precipitation-related process information inherent in polarimetric radar measurements, outlines pathways to inform atmospheric models with radar-based information, and points to remaining challenges towards an improved fusion of radar polarimetry and atmospheric modelling.
Kevin Ohneiser, Albert Ansmann, Alexandra Chudnovsky, Ronny Engelmann, Christoph Ritter, Igor Veselovskii, Holger Baars, Henriette Gebauer, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, and Marion Maturilli
Atmos. Chem. Phys., 21, 15783–15808, https://doi.org/10.5194/acp-21-15783-2021, https://doi.org/10.5194/acp-21-15783-2021, 2021
Short summary
Short summary
The highlight of the lidar measurements during the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition of the German icebreaker Polarstern (October 2019–October 2020) was the detection of a persistent, 10 km deep Siberian wildfire smoke layer in the upper troposphere and lower stratosphere (UTLS) from about 7–8 km to 17–18 km height that could potentially have impacted the record-breaking ozone depletion over the Arctic in the spring of 2020.
Jonas Witthuhn, Anja Hünerbein, Florian Filipitsch, Stefan Wacker, Stefanie Meilinger, and Hartwig Deneke
Atmos. Chem. Phys., 21, 14591–14630, https://doi.org/10.5194/acp-21-14591-2021, https://doi.org/10.5194/acp-21-14591-2021, 2021
Short summary
Short summary
Knowledge of aerosol–radiation interactions is important for understanding the climate system and for the renewable energy sector. Here, two complementary approaches are used to assess the consistency of the underlying aerosol properties and the resulting radiative effect in clear-sky conditions over Germany in 2015. An approach based on clear-sky models and broadband irradiance observations is contrasted to the use of explicit radiative transfer simulations using CAMS reanalysis data.
Ronny Engelmann, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, Marion Maturilli, Igor Veselovskii, Cristofer Jimenez, Robert Wiesen, Holger Baars, Johannes Bühl, Henriette Gebauer, Moritz Haarig, Patric Seifert, Ulla Wandinger, and Andreas Macke
Atmos. Chem. Phys., 21, 13397–13423, https://doi.org/10.5194/acp-21-13397-2021, https://doi.org/10.5194/acp-21-13397-2021, 2021
Short summary
Short summary
A Raman lidar was operated aboard the icebreaker Polarstern during MOSAiC and monitored aerosol and cloud layers in the central Arctic up to 30 km height. The article provides an overview of the spectrum of aerosol profiling observations and shows aerosol–cloud interaction studies for liquid-water and ice clouds. A highlight was the detection of a 10 km deep wildfire smoke layer over the North Pole up to 17 km height from the fire season of 2019, which persisted over the whole winter period.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
Short summary
Short summary
The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Tobias Peter Bauer, Peter Holtermann, Bernd Heinold, Hagen Radtke, Oswald Knoth, and Knut Klingbeil
Geosci. Model Dev., 14, 4843–4863, https://doi.org/10.5194/gmd-14-4843-2021, https://doi.org/10.5194/gmd-14-4843-2021, 2021
Short summary
Short summary
We present the coupled atmosphere–ocean model system ICONGETM. The added value and potential of using the latest coupling technologies are discussed in detail. An exchange grid handles the different coastlines from the unstructured atmosphere and the structured ocean grids. Due to a high level of automated processing, ICONGETM requires only minimal user input. The application to a coastal upwelling scenario demonstrates significantly improved model results compared to uncoupled simulations.
Hartwig Deneke, Carola Barrientos-Velasco, Sebastian Bley, Anja Hünerbein, Stephan Lenk, Andreas Macke, Jan Fokke Meirink, Marion Schroedter-Homscheidt, Fabian Senf, Ping Wang, Frank Werner, and Jonas Witthuhn
Atmos. Meas. Tech., 14, 5107–5126, https://doi.org/10.5194/amt-14-5107-2021, https://doi.org/10.5194/amt-14-5107-2021, 2021
Short summary
Short summary
The SEVIRI instrument flown on the European geostationary Meteosat satellites acquires multi-spectral images at a relatively coarse pixel resolution of 3 × 3 km2, but it also has a broadband high-resolution visible channel with 1 × 1 km2 spatial resolution. In this study, the modification of an existing cloud property and solar irradiance retrieval to use this channel to improve the spatial resolution of its output products as well as the resulting benefits for applications are described.
Hannes J. Griesche, Kevin Ohneiser, Patric Seifert, Martin Radenz, Ronny Engelmann, and Albert Ansmann
Atmos. Chem. Phys., 21, 10357–10374, https://doi.org/10.5194/acp-21-10357-2021, https://doi.org/10.5194/acp-21-10357-2021, 2021
Short summary
Short summary
Heterogeneous ice formation in Arctic mixed-phase clouds under consideration of their surface-coupling state is investigated. Cloud phase and macrophysical properties were determined by means of lidar and cloud radar measurements, the coupling state, and cloud minimum temperature by radiosonde profiles. Above −15 °C cloud minimum temperature, surface-coupled clouds are more likely to contain ice by a factor of 2–6. By means of a literature survey, causes of the observed effects are discussed.
Albert Ansmann, Kevin Ohneiser, Rodanthi-Elisavet Mamouri, Daniel A. Knopf, Igor Veselovskii, Holger Baars, Ronny Engelmann, Andreas Foth, Cristofer Jimenez, Patric Seifert, and Boris Barja
Atmos. Chem. Phys., 21, 9779–9807, https://doi.org/10.5194/acp-21-9779-2021, https://doi.org/10.5194/acp-21-9779-2021, 2021
Short summary
Short summary
We present retrievals of tropospheric and stratospheric height profiles of particle mass, volume, surface area concentration of wildfire smoke layers, and related cloud condensation nuclei (CCN) and ice-nucleating particle (INP) concentrations. The new analysis scheme is applied to ground-based lidar observations of stratospheric Australian smoke over southern South America and to spaceborne lidar observations of tropospheric North American smoke.
Fabiola Ramelli, Jan Henneberger, Robert O. David, Johannes Bühl, Martin Radenz, Patric Seifert, Jörg Wieder, Annika Lauber, Julie T. Pasquier, Ronny Engelmann, Claudia Mignani, Maxime Hervo, and Ulrike Lohmann
Atmos. Chem. Phys., 21, 6681–6706, https://doi.org/10.5194/acp-21-6681-2021, https://doi.org/10.5194/acp-21-6681-2021, 2021
Short summary
Short summary
Orographic mixed-phase clouds are an important source of precipitation, but the ice formation processes within them remain uncertain. Here we investigate the origin of ice crystals in a mixed-phase cloud in the Swiss Alps using aerosol and cloud data from in situ and remote sensing observations. We found that ice formation primarily occurs in cloud top generating cells. Our results indicate that secondary ice processes are active in the feeder region, which can enhance orographic precipitation.
Fabiola Ramelli, Jan Henneberger, Robert O. David, Annika Lauber, Julie T. Pasquier, Jörg Wieder, Johannes Bühl, Patric Seifert, Ronny Engelmann, Maxime Hervo, and Ulrike Lohmann
Atmos. Chem. Phys., 21, 5151–5172, https://doi.org/10.5194/acp-21-5151-2021, https://doi.org/10.5194/acp-21-5151-2021, 2021
Short summary
Short summary
Interactions between dynamics, microphysics and orography can enhance precipitation. Yet the exact role of these interactions is still uncertain. Here we investigate the role of low-level blocking and turbulence for precipitation by combining remote sensing and in situ observations. The observations show that blocked flow can induce the formation of feeder clouds and that turbulence can enhance hydrometeor growth, demonstrating the importance of local flow effects for orographic precipitation.
Michael Weger, Oswald Knoth, and Bernd Heinold
Geosci. Model Dev., 14, 1469–1492, https://doi.org/10.5194/gmd-14-1469-2021, https://doi.org/10.5194/gmd-14-1469-2021, 2021
Short summary
Short summary
A new numerical air-quality transport model for cities is presented, in which buildings are described diffusively. The used diffusive-obstacles approach helps to reduce the computational costs for high-resolution simulations as the grid spacing can be more coarse than in traditional approaches. The research which led to this model development was primarily motivated by the need for a computationally feasible downscaling tool for urban wind and pollution fields from meteorological model output.
Martin Radenz, Patric Seifert, Holger Baars, Athena Augusta Floutsi, Zhenping Yin, and Johannes Bühl
Atmos. Chem. Phys., 21, 3015–3033, https://doi.org/10.5194/acp-21-3015-2021, https://doi.org/10.5194/acp-21-3015-2021, 2021
Cited articles
Albani, S., Mahowald, N. M., Delmonte, B., Maggi, V., and Winckler, G.:
Comparing modeled and observed changes in mineral dust transport and
deposition to Antarctica between the Last Glacial Maximum and current
climates, Clim. Dynam., 38, 1731–1755, https://doi.org/10.1007/s00382-011-1139-5,
2012. a
Ansmann, A., Tesche, M., Althausen, D., Müller, D., Seifert, P.,
Freudenthaler, V., Heese, B., Wiegner, M., Pisani, G., Knippertz, P., and
Dubovik, O.: Influence of Saharan dust on cloud glaciation in southern
Morocco during the Saharan Mineral Dust Experiment,
J. Geophys. Res.-Atmos., 113, https://doi.org/10.1029/2007JD008785, 2008. a, b
Ansmann, A., Rittmeister, F., Engelmann, R., Basart, S., Jorba, O., Spyrou, C., Remy, S., Skupin, A., Baars, H., Seifert, P., Senf, F., and Kanitz, T.: Profiling of Saharan dust from the Caribbean to western Africa – Part 2: Shipborne lidar measurements versus forecasts, Atmos. Chem. Phys., 17, 14987–15006, https://doi.org/10.5194/acp-17-14987-2017, 2017. a, b
Atkinson, J. D., Murray, B. J., Woodhouse, M. T., Whale, T. F., Baustian,
K. J., Carslaw, K. S., Dobbie, S., O'Sullivan, D., and Malkin, T. L.: The
importance of feldspar for ice nucleation by mineral dust in mixed-phase
clouds, Nature, 498, 355–358, https://doi.org/10.1038/nature12278, 2013. a, b, c
Augustin-Bauditz, S., Wex, H., Denjean, C., Hartmann, S., Schneider, J., Schmidt, S., Ebert, M., and Stratmann, F.: Laboratory-generated mixtures of mineral dust particles with biological substances: characterization of the particle mixing state and immersion freezing behavior, Atmos. Chem. Phys., 16, 5531–5543, https://doi.org/10.5194/acp-16-5531-2016, 2016. a
Barahona, D., Molod, A., and Kalesse, H.: Direct estimation of the global
distribution of vertical velocity within cirrus clouds, Sci. Rep.,
7, https://doi.org/10.1038/s41598-017-07038-6, 2017. a
Boose, Y., Welti, A., Atkinson, J., Ramelli, F., Danielczok, A., Bingemer, H. G., Plötze, M., Sierau, B., Kanji, Z. A., and Lohmann, U.: Heterogeneous ice nucleation on dust particles sourced from nine deserts worldwide – Part 1: Immersion freezing, Atmos. Chem. Phys., 16, 15075–15095, https://doi.org/10.5194/acp-16-15075-2016, 2016. a, b, c
Bosilovich, M. G., Robertson, F. R., and Chen, J.: Global energy and water
budgets in MERRA, J. Climate, 24, https://doi.org/10.1175/2011JCLI4175.1, 2011. a
Broadley, S. L., Murray, B. J., Herbert, R. J., Atkinson, J. D., Dobbie, S., Malkin, T. L., Condliffe, E., and Neve, L.: Immersion mode heterogeneous ice nucleation by an illite rich powder representative of atmospheric mineral dust, Atmos. Chem. Phys., 12, 287–307, https://doi.org/10.5194/acp-12-287-2012, 2012. a
Bühl, J., Seifert, P., Myagkov, A., and Ansmann, A.: Measuring ice- and liquid-water properties in mixed-phase cloud layers at the Leipzig Cloudnet station, Atmos. Chem. Phys., 16, 10609–10620, https://doi.org/10.5194/acp-16-10609-2016, 2016. a
Burrows, S. M., Hoose, C., Pöschl, U., and Lawrence, M. G.: Ice nuclei in marine air: biogenic particles or dust?, Atmos. Chem. Phys., 13, 245–267, https://doi.org/10.5194/acp-13-245-2013, 2013. a, b
Cesana, G. and Chepfer, H.: Evaluation of the cloud thermodynamic phase in a
climate model using CALIPSO-GOCCP, J. Geophys. Res.-Atmos., 118, 7922–7937, https://doi.org/10.1002/jgrd.50376, 2013. a, b, c
Cesana, G., Waliser, D. E., Jiang, X., and Li, J. L.: Multimodel evaluation of
cloud phase transition using satellite and reanalysis data,
J. Geophys. Res., 120, 7871–7892, https://doi.org/10.1002/2014JD022932, 2015. a, b
Chepfer, H.: GCM-Oriented CALIPSO Cloud Product, available at: https://climserv.ipsl.polytechnique.fr/cfmip-obs/Calipso_goccp_new.html, last access: 13 February 2019.
Claquin, T., Schulz, M., and Balkanski, Y. J.: Modeling the mineralogy of
atmospheric dust sources, J. Geophys. Res.-Atmos.,
104, https://doi.org/10.1029/1999JD900416, 1999. a, b
Copernicus Atmosphere Monitoring Service (CAMS): MACC-II Consortium, 2011: MACC Reanalysis of Global Atmospheric Composition (2003–2012), available at: http://apps.ecmwf.int/datasets/data/macc-reanalysis/levtype=ml, last access: 13 February 2019.
Cuevas, E., Camino, C., Benedetti, A., Basart, S., Terradellas, E., Baldasano, J. M., Morcrette, J. J., Marticorena, B., Goloub, P., Mortier, A., Berjón, A., Hernández, Y., Gil-Ojeda, M., and Schulz, M.: The MACC-II 2007–2008 reanalysis: atmospheric dust evaluation and characterization over northern Africa and the Middle East, Atmos. Chem. Phys., 15, 3991–4024, https://doi.org/10.5194/acp-15-3991-2015, 2015. a, b
De Boer, G., Morrison, H., Shupe, M. D., and Hildner, R.: Evidence of liquid
dependent ice nucleation in high-latitude stratiform clouds from surface
remote sensors, Geophys. Res. Lett., 38, https://doi.org/10.1029/2010GL046016,
2011. a, b
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi,
S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P.,
Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C.,
Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B.,
Hersbach, H., Hólm, E. V., Isaksen, L., Kållberg, P., Köhler,
M., Matricardi, M., McNally, A. P., Monge-Sanz, B. M., Morcrette, J.-J.,
Park, B.-K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J.-N.,
and Vitart, F.: The ERA-Interim reanalysis: configuration and performance of
the data assimilation system,
Q. J. Roy. Meteor. Soc., 137, 553–597, https://doi.org/10.1002/qj.828, 2011. a
Delanoë, J. and Hogan, R. J.: Combined CloudSat-CALIPSO-MODIS retrievals of the properties of ice clouds, J. Geophys. Res.-Atmos., 115, https://doi.org/10.1029/2009JD012346, 2010.
Delanoë, J. M. E. and Hogan, R. J.: A variational scheme for retrieving ice cloud properties from combined radar, lidar, and infrared radiometer, J. Geophys. Res.-Atmos., 113, https://doi.org/10.1029/2007JD009000, 2008.
Diehl, K. and Wurzler, S.: Heterogeneous Drop Freezing in the Immersion Mode:
Model Calculations Considering Soluble and Insoluble Particles in the Drops,
J. Atmos. Sci.,
61, https://doi.org/10.1175/1520-0469(2004)061<2063:hdfiti>2.0.co;2, 2004. a
Diehl, K., Simmel, M., and Wurzler, S.: Numerical sensitivity studies on the
impact of aerosol properties and drop freezing modes on the glaciation,
microphysics and dynamics of clouds, J. Geophys. Res.-Atmos., 111, https://doi.org/10.1029/2005JD005884, 2006. a
Dietlicher, R., Neubauer, D., and Lohmann, U.: Elucidating ice formation pathways in the aerosol–climate model ECHAM6-HAM2, Atmos. Chem. Phys., 19, 9061–9080, https://doi.org/10.5194/acp-19-9061-2019, 2019. a
Dubovik, O., Smirnov, A., Holben, B. N., King, M. D., Kaufman, Y. J., Eck,
T. F., and Slutsker, I.: Accuracy assessments of aerosol optical properties
retrieved from Aerosol Robotic Network (AERONET) Sun and sky radiance
measurements, J. Geophys. Res.-Atmos., 105, 9791–9806,
https://doi.org/10.1029/2000JD900040, 2000. a
ECMWF: ERA-Interim, available at: https://apps.ecmwf.int/datasets/data/interim-full-daily/levtype=pl/, last access: 13 February 2019.
Eskes, H., Huijnen, V., Arola, A., Benedictow, A., Blechschmidt, A.-M., Botek, E., Boucher, O., Bouarar, I., Chabrillat, S., Cuevas, E., Engelen, R., Flentje, H., Gaudel, A., Griesfeller, J., Jones, L., Kapsomenakis, J., Katragkou, E., Kinne, S., Langerock, B., Razinger, M., Richter, A., Schultz, M., Schulz, M., Sudarchikova, N., Thouret, V., Vrekoussis, M., Wagner, A., and Zerefos, C.: Validation of reactive gases and aerosols in the MACC global analysis and forecast system, Geosci. Model Dev., 8, 3523–3543, https://doi.org/10.5194/gmd-8-3523-2015, 2015. a
Fröhlich-Nowoisky, J., Hill, T. C. J., Pummer, B. G., Yordanova, P., Franc, G. D., and Pöschl, U.: Ice nucleation activity in the widespread soil fungus Mortierella alpina, Biogeosciences, 12, 1057–1071, https://doi.org/10.5194/bg-12-1057-2015, 2015. a
Georgoulias, A. K., Tsikerdekis, A., Amiridis, V., Marinou, E., Benedetti, A., Zanis, P., Alexandri, G., Mona, L., Kourtidis, K. A., and Lelieveld, J.: A 3-D evaluation of the MACC reanalysis dust product over Europe, northern Africa and Middle East using CALIOP/CALIPSO dust satellite observations, Atmos. Chem. Phys., 18, 8601–8620, https://doi.org/10.5194/acp-18-8601-2018, 2018. a
Gryspeerdt, E., Quaas, J., and Bellouin, N.: Constraining the aerosol
influence on cloud fraction, J. Geophys. Res.,
121, https://doi.org/10.1002/2015JD023744, 2016. a, b
Hartmann, S., Wex, H., Clauss, T., Augustin-Bauditz, S., Niedermeier, D.,
Rösch, M., and Stratmann, F.: Immersion Freezing of Kaolinite: Scaling
with Particle Surface Area, J. Atmos. Sci.,
73, https://doi.org/10.1175/JAS-D-15-0057.1, 2016. a
Hauke, J. and Kossowski, T.: Comparison of values of pearson's and spearman's
correlation coefficients on the same sets of data,
Quaestiones Geographicae,
30, https://doi.org/10.2478/v10117-011-0021-1, 2011. a
Hoose, C. and Möhler, O.: Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments, Atmos. Chem. Phys., 12, 9817–9854, https://doi.org/10.5194/acp-12-9817-2012, 2012. a, b
Hoose, C., Lohmann, U., Erdin, R., and Tegen, I.: The global influence of dust
mineralogical composition on heterogeneous ice nucleation in mixed-phase
clouds, Environ. Res. Lett., 3, https://doi.org/10.1088/1748-9326/3/2/025003,
2008. a, b
Hu, Y., Rodier, S., Xu, K. M., Sun, W., Huang, J., Lin, B., Zhai, P., and
Josset, D.: Occurrence, liquid water content, and fraction of supercooled
water clouds from combined CALIOP/IIR/MODIS measurements, J. Geophys. Res.-Atmos., 115, https://doi.org/10.1029/2009JD012384, 2010. a
Huang, L., Jiang, J. H., Wang, Z., Su, H., Deng, M., and Massie, S.:
Climatology of cloud water content associated with different cloud types
observed by A-Train satellites, J. Geophys. Res.,
120, https://doi.org/10.1002/2014JD022779, 2015. a, b
Huang, Y., Siems, S. T., Manton, M. J., Protat, A., and Delanoë, J.: A
study on the low-altitude clouds over the Southern Ocean using the
DARDAR-MASK, J. Geophys. Res.-Atmos., 117,
117, https://doi.org/10.1029/2012JD017800, 2012. a
Johnson, M. S., Meskhidze, N., Kiliyanpilakkil, V. P., and Gassó, S.: Understanding the transport of Patagonian dust and its influence on marine biological activity in the South Atlantic Ocean, Atmos. Chem. Phys., 11, 2487–2502, https://doi.org/10.5194/acp-11-2487-2011, 2011. a
Kanitz, T., Seifert, P., Ansmann, A., Engelmann, R., Althausen, D., Casiccia,
C., and Rohwer, E. G.: Contrasting the impact of aerosols at northern and
southern midlatitudes on heterogeneous ice formation, Geophys. Res. Lett., 38, https://doi.org/10.1029/2011GL048532, 2011. a, b, c, d
Klein, S. A. and Hartmann, D. L.: The seasonal cycle of low stratiform
clouds, J. Climate,
6, https://doi.org/10.1175/1520-0442(1993)006<1587:TSCOLS>2.0.CO;2, 1993. a, b
Kok, J. F.: A scaling theory for the size distribution of emitted dust
aerosols suggests climate models underestimate the size of the global dust
cycle, P. Natl. Acad. Sci. USA, 108, 1016–1021,
https://doi.org/10.1073/pnas.1014798108, 2011. a
Korolev, A., McFarquhar, G., Field, P. R., Franklin, C., Lawson, P., Wang, Z.,
Williams, E., Abel, S. J., Axisa, D., Borrmann, S., Crosier, J., Fugal, J.,
Krämer, M., Lohmann, U., Schlenczek, O., Schnaiter, M., Wendisch, M.,
Korolev, A., McFarquhar, G., Field, P. R., Franklin, C., Lawson, P., Wang,
Z., Williams, E., Abel, S. J., Axisa, D., Borrmann, S., Crosier, J., Fugal,
J., Krämer, M., Lohmann, U., Schlenczek, O., Schnaiter, M., and
Wendisch, M.: Mixed-Phase Clouds: Progress and Challenges, Meteorological Monographs, 58, 5.1–5.50, https://doi.org/10.1175/AMSMONOGRAPHS-D-17-0001.1, 2017. a, b
Lacher, L., DeMott, P. J., Levin, E. J. T., Suski, K. J., Boose, Y., Zipori,
A., Herrmann, E., Bukowiecki, N., Steinbacher, M., Gute, E., Abbatt, J.
P. D., Lohmann, U., and Kanji, Z. A.: Background Free Tropospheric Ice
Nucleating Particle Concentrations at Mixed phase Cloud Conditions, J. Geophys. Res.-Atmos., 123, https://doi.org/10.1029/2018JD028338, 2018. a
Li, F., Ginoux, P., and Ramaswamy, V.: Distribution, transport, and deposition
of mineral dust in the Southern Ocean and Antarctica: Contribution of major
sources, J. Geophys. Res.-Atmos., 113,
https://doi.org/10.1029/2007JD009190, 2008. a
Li, R., Dong, X., Guo, J., Fu, Y., Zhao, C., Wang, Y., and Min, Q.: The
implications of dust ice nuclei effect on cloud top temperature in a complex
mesoscale convective system, Sci. Rep.,
7, https://doi.org/10.1038/s41598-017-12681-0, 2017b. a
Mahowald, N., Albani, S., Kok, J. F., Engelstaeder, S., Scanza, R., Ward,
D. S., and Flanner, M. G.: The size distribution of desert dust aerosols and
its impact on the Earth system, Aeolian Res., 15, 53–71,
https://doi.org/10.1016/j.aeolia.2013.09.002, 2014. a, b
McCoy, D. T., Tan, I., Hartmann, D. L., Zelinka, M. D., and Storelvmo, T.: On
the relationships among cloud cover, mixed-phase partitioning, and planetary
albedo in GCMs, J. Adv. Model. Earth Sy.,
8, https://doi.org/10.1002/2015MS000589, 2016. a
Morrison, A. E., Siems, S. T., and Manton, M. J.: A three-year climatology of
cloud-top phase over the Southern Ocean and North Pacific, J.
Climate, 24, 2405–2418, https://doi.org/10.1175/2010JCLI3842.1, 2011. a
Murray, B. J., Broadley, S. L., Wilson, T. W., Atkinson, J. D., and Wills, R. H.: Heterogeneous freezing of water droplets containing kaolinite particles, Atmos. Chem. Phys., 11, 4191–4207, https://doi.org/10.5194/acp-11-4191-2011, 2011. a, b
Niedermeier, D., Shaw, R. A., Hartmann, S., Wex, H., Clauss, T., Voigtländer, J., and Stratmann, F.: Heterogeneous ice nucleation: exploring the transition from stochastic to singular freezing behavior, Atmos. Chem. Phys., 11, 8767–8775, https://doi.org/10.5194/acp-11-8767-2011, 2011. a
Niedermeier, D., Augustin-Bauditz, S., Hartmann, S., Wex, H., Ignatius, K., and
Stratmann, F.: Can we define an asymptotic value for the ice active surface
site density for heterogeneous ice nucleation?, J. Geophys. Res., 210, https://doi.org/10.1002/2014JD022814, 2015. a
Niemand, M., Möhler, O., Vogel, B., Vogel, H., Hoose, C., Connolly, P.,
Klein, H., Bingemer, H., DeMott, P., Skrotzki, J., and Leisner, T.: A
Particle-Surface-Area-Based Parameterization of Immersion Freezing on Desert
Dust Particles, J. Atmos. Sci.,
69, https://doi.org/10.1175/JAS-D-11-0249.1, 2012. a
O'Sullivan, D., Adams, M. P., Tarn, M. D., Harrison, A. D., Vergara-Temprado,
J., Porter, G. C. E., Holden, M. A., Sanchez-Marroquin, A., Carotenuto, F.,
Whale, T. F., McQuaid, J. B., Walshaw, R., Hedges, D. H. P., Burke, I. T.,
Cui, Z., and Murray, B. J.: Contributions of biogenic material to the
atmospheric ice-nucleating particle population in North Western Europe,
Sci. Rep., 8, 13821, https://doi.org/10.1038/s41598-018-31981-7, 2018. a
Petters, M. D. and Wright, T. P.: Revisiting ice nucleation from precipitation
samples, Geophys. Res. Lett., 42, https://doi.org/10.1002/2015GL065733, 2015. a
Price, H. C., Baustian, K. J., McQuaid, J. B., Blyth, A., Bower, K. N.,
Choularton, T., Cotton, R. J., Cui, Z., Field, P. R., Gallagher, M., Hawker,
R., Merrington, A., Miltenberger, A., Neely, R. R., Parker, S. T., Rosenberg,
P. D., Taylor, J. W., Trembath, J., Vergara-Temprado, J., Whale, T. F.,
Wilson, T. W., Young, G., and Murray, B. J.: Atmospheric Ice-Nucleating
Particles in the Dusty Tropical Atlantic, J. Geophys. Res.- Atmos., 123, https://doi.org/10.1002/2017JD027560, 2018. a
Randall, D. A., Wood, R. A., Bony, S., Colman, R., Fichefet, T., Fyve, J.,
Kattsov, V., Pitman, A., Shukla, J., Srinivasan, J., Stouffer, R. J., Sumi,
A., and Taylor, K. E.: Climate Models and Their Evaluation, Climate Change
2007: The Physical Science Basis. Contribution of Working Group I to the
Fourth Assessment Report of the Intergovernmental Panel on Climate Change,
https://doi.org/10.1016/j.cub.2007.06.045, 2007. a
Ridley, D. A., Heald, C. L., Kok, J. F., and Zhao, C.: An observationally constrained estimate of global dust aerosol optical depth, Atmos. Chem. Phys., 16, 15097–15117, https://doi.org/10.5194/acp-16-15097-2016, 2016. a
Sassen, K. and Wang, Z.: Classifying clouds around the globe with the CloudSat
radar: 1-year of results, Geophys. Res. Lett., 35, https://doi.org/10.1029/2007GL032591, 2008. a
Scott, R. C. and Lubin, D.: Unique manifestations of mixed-phase cloud
microphysics over Ross Island and the Ross Ice Shelf, Antarctica,
Geophys. Res. Lett., 43, https://doi.org/10.1002/2015GL067246, 2016. a
Seifert, P., Ansmann, A., Mattis, I., Wandinger, U., Tesche, M., Engelmann, R.,
Müller, D., Pérez, C., and Haustein, K.: Saharan dust and
heterogeneous ice formation: Eleven years of cloud observations at a central
European EARLINET site, J. Geophys. Res.-Atmos., 115, https://doi.org/10.1029/2009JD013222, 2010. a, b, c, d
Seinfeld, J. H. and Pandis, S. N.: Atmospheric Chemistry and Physics: From Air
Pollution to Climate Change, Atmospheric chemistry and physics from air
pollution to climate change, New York, NY, Wiley 1998, Physical
description, xxvii, 1326 p., A WileyInterscience Publication, ISBN 0471178152, 51,
1–4, https://doi.org/10.1080/00139157.1999.10544295, 1998. a
Sullivan, S. C., Lee, D., Oreopoulos, L., and Nenes, A.: Role of updraft
velocity in temporal variability of global cloud hydrometeor number,
P. Natl. Acad. Sci. USA, 113, 5791–5796,
https://doi.org/10.1073/pnas.1514039113, 2016. a
Toth, T. D., Campbell, J. R., Reid, J. S., Tackett, J. L., Vaughan, M. A., Zhang, J., and Marquis, J. W.: Minimum aerosol layer detection sensitivities and their subsequent impacts on aerosol optical thickness retrievals in CALIPSO level 2 data products, Atmos. Meas. Tech., 11, 499–514, https://doi.org/10.5194/amt-11-499-2018, 2018. a
Université de Lille: ICARE Data and Services Center, available at: http://www.icare.univ-lille1.fr/contacts, last access: 13 February 2019.
Vergara-Temprado, J., Murray, B. J., Wilson, T. W., O'Sullivan, D., Browse, J., Pringle, K. J., Ardon-Dryer, K., Bertram, A. K., Burrows, S. M., Ceburnis, D., DeMott, P. J., Mason, R. H., O'Dowd, C. D., Rinaldi, M., and Carslaw, K. S.: Contribution of feldspar and marine organic aerosols to global ice nucleating particle concentrations, Atmos. Chem. Phys., 17, 3637–3658, https://doi.org/10.5194/acp-17-3637-2017, 2017. a, b, c, d
Vergara-Temprado, J., Miltenberger, A. K., Furtado, K., Grosvenor, D. P.,
Shipway, B. J., Hill, A. A., Wilkinson, J. M., Field, P. R., Murray, B. J.,
and Carslaw, K. S.: Strong control of Southern Ocean cloud reflectivity by
ice-nucleating particles, P. Natl. Acad. Sci. USA,
115, 201721627, https://doi.org/10.1073/pnas.1721627115, 2018. a
Welti, A., Lüönd, F., Stetzer, O., and Lohmann, U.: Influence of particle size on the ice nucleating ability of mineral dusts, Atmos. Chem. Phys., 9, 6705–6715, https://doi.org/10.5194/acp-9-6705-2009, 2009.
a
Westbrook, C. D. and Illingworth, A. J.: Evidence that ice forms primarily in
supercooled liquid clouds at temperatures > 27∘C,
Geophys. Res. Lett., 38, https://doi.org/10.1029/2011GL048021, 2011. a, b, c
Wu, Y., Cordero, L., Gross, B., Moshary, F., and Ahmed, S.: Assessment of
CALIPSO attenuated backscatter and aerosol retrievals with a combined
ground-based multi-wavelength lidar and sunphotometer measurement,
Atmos. Environ., 84, 44–53, https://doi.org/10.1016/j.atmosenv.2013.11.016,
2014. a
Zamora, L. M., Kahn, R. A., Huebert, K. B., Stohl, A., and Eckhardt, S.: A satellite-based estimate of combustion aerosol cloud microphysical effects over the Arctic Ocean, Atmos. Chem. Phys., 18, 14949–14964, https://doi.org/10.5194/acp-18-14949-2018, 2018. a
Zhang, D., Wang, Z., and Liu, D.: A global view of midlevel liquid-layer
topped stratiform cloud distribution and phase partition from CALIPSO and
CloudSat measurements, J. Geophys. Res.-Atmos.,
115, https://doi.org/10.1029/2009JD012143, 2010. a, b
Zhang, D., Wang, Z., Heymsfield, A., Fan, J., Liu, D., and Zhao, M.:
Quantifying the impact of dust on heterogeneous ice generation in midlevel
supercooled stratiform clouds, Geophys. Res. Lett.,
39, https://doi.org/10.1029/2012GL052831, 2012. a, b, c
Zhang, D., Liu, D., Luo, T., Wang, Z., and Yin, Y.: Aerosol impacts on cloud
thermodynamic phase change over East Asia observed with CALIPSO and CloudSat
measurements, J. Geophys. Res., 120, 1490–1501,
https://doi.org/10.1002/2014JD022630, 2015. a
Zhang, D., Wang, Z., Kollias, P., Vogelmann, A. M., Yang, K., and Luo, T.: Ice particle production in mid-level stratiform mixed-phase clouds observed with collocated A-Train measurements, Atmos. Chem. Phys., 18, 4317–4327, https://doi.org/10.5194/acp-18-4317-2018, 2018. a, b, c
Short summary
Spaceborne retrievals of cloud phase were analysed together with an atmospheric composition model to assess the global frequency of ice and liquid clouds. This analysis showed that at equal temperature the average occurrence of ice clouds increases for higher dust mixing ratios on a day-to-day basis in the middle and high latitudes. This indicates that mineral dust may have a strong impact on the occurrence of ice clouds even in remote areas.
Spaceborne retrievals of cloud phase were analysed together with an atmospheric composition...
Altmetrics
Final-revised paper
Preprint