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Volume 17, issue 23
Atmos. Chem. Phys., 17, 14631–14643, 2017
https://doi.org/10.5194/acp-17-14631-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: Quadrennial Ozone Symposium 2016 – Status and trends...

Atmos. Chem. Phys., 17, 14631–14643, 2017
https://doi.org/10.5194/acp-17-14631-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 07 Dec 2017

Research article | 07 Dec 2017

Diurnal variations of BrONO2 observed by MIPAS-B at midlatitudes and in the Arctic

Gerald Wetzel et al.

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Atkinson, R., Baulch, D. L., Cox, R. A., Crowley, J. N., Hampson, R. F., Hynes, R. G., Jenkin, M. E., Rossi, M. J., and Troe, J.: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume III – gas phase reactions of inorganic halogens, Atmos. Chem. Phys., 7, 981–1191, https://doi.org/10.5194/acp-7-981-2007, 2007.
Brasseur, G. and Solomon, S.: Aeronomy of the middle atmosphere, in: Atmos. Oceanograph. Sci. Lib., 3rd Edn., Springer, Dordrecht, the Netherlands, 369 pp., 2005.
Carpenter, L. J., Reimann, S., Burkholder, J. B., Clerbaux, C., Hall, B. D., Hossaini, R., Laube, J. C., and Yvon-Lewis, S. A.: Ozone-Depleting Substances (ODSs) and other gases of interest to the Montreal Protocol, in: Chapter 1 in Scientific Assessment of Ozone Depletion: 2014, Global Ozone Research and Monitoring Project, Report No. 55, World Meteorological Organization, Geneva, Switzerland, 416 pp., 2014.
Dorf, M., Butler, J. H., Butz, A., Camy-Peyret, C., Chipperfield, M. P., Kritten, L., Montzka, S. A., Simmes, B., Weidner, F., and Pfeilsticker, K.: Long-term observations of stratospheric bromine reveal slow down in growth, Geophys. Res. Lett., 33, L24803, https://doi.org/10.1029/2006GL027714, 2006.
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We report the first stratospheric measurements of the diurnal variation in the inorganic bromine (Bry) reservoir species BrONO2 around sunrise and sunset. The main goal of these observations was to check the current understanding of stratospheric bromine chemistry and to estimate the amount of lower-stratospheric Bry. The calculated temporal variation in BrONO2 largely reproduces the balloon-borne observations. The amount of Bry was estimated to be about 21–25 pptv in the lower stratosphere.
We report the first stratospheric measurements of the diurnal variation in the inorganic bromine...
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