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Volume 17, issue 19
Atmos. Chem. Phys., 17, 12031–12050, 2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: Regional transport and transformation of air pollution in...

Atmos. Chem. Phys., 17, 12031–12050, 2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 10 Oct 2017

Research article | 10 Oct 2017

A modeling study of the nonlinear response of fine particles to air pollutant emissions in the Beijing–Tianjin–Hebei region

Bin Zhao et al.

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Burnett, R. T., Pope, C. A., Ezzati, M., Olives, C., Lim, S. S., Mehta, S., Shin, H. H., Singh, G., Hubbell, B., Brauer, M., Anderson, H. R., Smith, K. R., Balmes, J. R., Bruce, N. G., Kan, H. D., Laden, F., Pruss-Ustun, A., Michelle, C. T., Gapstur, S. M., Diver, W. R., and Cohen, A.: An Integrated Risk Function for Estimating the Global Burden of Disease Attributable to Ambient Fine Particulate Matter Exposure, Environ. Health Persp., 122, 397–403,, 2014.
Cai, S. Y., Wang, Y. J., Zhao, B., Wang, S. X., Chang, X., and Hao, J. M.: The impact of the “Air Pollution Prevention and Control Action Plan” on PM2. 5 concentrations in Jing-Jin-Ji region during 2012–2020, Sci. Total Environ., 580, 197–209,, 2017.
Cheng, I., Zhang, L., Blanchard, P., Dalziel, J., and Tordon, R.: Concentration-weighted trajectory approach to identifying potential sources of speciated atmospheric mercury at an urban coastal site in Nova Scotia, Canada, Atmos. Chem. Phys., 13, 6031–6048,, 2013.
Cheng, Y. F., Zheng, G. J., Wei, C., Mu, Q., Zheng, B., Wang, Z. B., Gao, M., Zhang, Q., He, K. B., Carmichael, G., Pöschl, U., and Su, H.: Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China, Sci. Adv., 2, e1601530,, 2016.
Dong, X. Y., Li, J., Fu, J. S., Gao, Y., Huang, K., and Zhuang, G. S.: Inorganic aerosols responses to emission changes in Yangtze River Delta, China, Sci. Total Environ., 481, 522–532,, 2014.
Publications Copernicus
Short summary
Using over 1000 chemical transport model simulations in the Beijing–Tianjin–Hebei region, we find that the emissions of primary inorganic PM2.5 make the largest contribution to PM2.5 concentrations and thus should be prioritized in PM2.5 control strategies. Among the precursors, PM2.5 concentrations are primarily sensitive to the emissions of NH3, NMVOC+IVOC, and POA, and the sensitivities increase substantially for NH3 and NHx with the increase in emission reduction ratio.
Using over 1000 chemical transport model simulations in the Beijing–Tianjin–Hebei region, we...
Final-revised paper