Articles | Volume 14, issue 20
https://doi.org/10.5194/acp-14-11475-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-11475-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
30 Oct 2014
Research article |
| 30 Oct 2014
Simulating black carbon and dust and their radiative forcing in seasonal snow: a case study over North China with field campaign measurements
C. Zhao
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Z. Hu
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, Lanzhou University, Gansu, China
Y. Qian
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
L. Ruby Leung
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, Lanzhou University, Gansu, China
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
J. Jin
Departments of Watershed Sciences and Plants, Soils, and Climate, Utah State University, Logan, UT, USA
M. G. Flanner
University of Michigan, Ann Arbor, MI, USA
R. Zhang
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, Lanzhou University, Gansu, China
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
H. Yan
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, Lanzhou University, Gansu, China
Z. Lu
Argonne National Laboratory Argonne, IL, USA
D. G. Streets
Argonne National Laboratory Argonne, IL, USA
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In this study, we improved the calculation of how aerosols in the air interact with radiation in WRF-Chem. The original model used a simplified method, but we developed a more accurate approach. We found that the new method significantly changes the estimated aerosols' properties and their effects on radiation, especially for dust aerosols. It also impacts the simulated weather conditions. Our work highlights the importance of correctly representing aerosol-radiation interactions in models.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1487, https://doi.org/10.5194/egusphere-2024-1487, 2024
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke-amount observations, aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss-rate assumptions vary enormously among models, causing uncertainties that require systematic in-situ measurements to resolve.
Xia Wang, Tao Che, Xueyin Ruan, Shanna Yue, Jing Wang, Chun Zhao, and Lei Geng
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-37, https://doi.org/10.5194/gmd-2024-37, 2024
Preprint under review for GMD
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We employed the WRF-Chem model to parameterize atmospheric nitrate deposition in snow and evaluated its performance in simulating snow cover, snow depth, and concentrations of black carbon (BC), dust, and nitrate using new observations from Northern China. The results generally exhibit reasonable agreement with field observations in northern China, demonstrating the model's capability to simulate snow properties, including concentrations of reservoir species.
Fang Li, Xiang Song, Sandy P. Harrison, Jennifer R. Marlon, Zhongda Lin, L. Ruby Leung, Jörg Schwinger, Virginie Marécal, Shiyu Wang, Daniel S. Ward, Xiao Dong, Hanna Lee, Lars Nieradzik, Sam S. Rabin, and Roland Séférian
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-85, https://doi.org/10.5194/gmd-2024-85, 2024
Preprint under review for GMD
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This study provides the first comprehensive assessment of historical fire simulations from 19 CMIP6 ESMs. Most models reproduce global total, spatial pattern, seasonality, and regional historical changes well, but fail to simulate the recent decline in global burned area and underestimate the fire sensitivity to wet-dry conditions. They addressed three critical issues in CMIP5. We present targeted guidance for fire scheme development and methodologies to generate reliable fire projections.
Taufiq Hassan, Kai Zhang, Jianfeng Li, Balwinder Singh, Shixuan Zhang, Hailong Wang, and Po-Lun Ma
Geosci. Model Dev., 17, 3507–3532, https://doi.org/10.5194/gmd-17-3507-2024, https://doi.org/10.5194/gmd-17-3507-2024, 2024
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Anthropogenic aerosol emissions are an essential part of global aerosol models. Significant errors can exist from the loss of emission heterogeneity. We introduced an emission treatment that significantly improved aerosol emission heterogeneity in high-resolution model simulations, with improvements in simulated aerosol surface concentrations. The emission treatment will provide a more accurate representation of aerosol emissions and their effects on climate.
Lingcheng Li, Gautam Bisht, Dalei Hao, and L. Ruby Leung
Earth Syst. Sci. Data, 16, 2007–2032, https://doi.org/10.5194/essd-16-2007-2024, https://doi.org/10.5194/essd-16-2007-2024, 2024
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This study fills a gap to meet the emerging needs of kilometer-scale Earth system modeling by developing global 1 km land surface parameters for land use, vegetation, soil, and topography. Our demonstration simulations highlight the substantial impacts of these parameters on spatial variability and information loss in water and energy simulations. Using advanced explainable machine learning methods, we identified influential factors driving spatial variability and information loss.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
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We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Bryce E. Harrop, Jian Lu, L. Ruby Leung, William K. M. Lau, Kyu-Myong Kim, Brian Medeiros, Brian J. Soden, Gabriel A. Vecchi, Bosong Zhang, and Balwinder Singh
Geosci. Model Dev., 17, 3111–3135, https://doi.org/10.5194/gmd-17-3111-2024, https://doi.org/10.5194/gmd-17-3111-2024, 2024
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Seven new experimental setups designed to interfere with cloud radiative heating have been added to the Energy Exascale Earth System Model (E3SM). These experiments include both those that test the mean impact of cloud radiative heating and those examining its covariance with circulations. This paper documents the code changes and steps needed to run these experiments. Results corroborate prior findings for how cloud radiative heating impacts circulations and rainfall patterns.
Weiming Ma, Hailong Wang, Gang Chen, Yun Qian, Ian Baxter, Yiling Huo, and Mark W. Seefeldt
Atmos. Chem. Phys., 24, 4451–4472, https://doi.org/10.5194/acp-24-4451-2024, https://doi.org/10.5194/acp-24-4451-2024, 2024
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Extreme warming events with surface temperature going above 0°C can occur in the high-Arctic winter. Although reanalysis data show that these events were short-lived and occurred rarely during 1980–2021, they have become more frequent, stronger, and longer lasting latterly. A dipole pattern, comprising high- and low-pressure systems, is found to be the key in driving them. These findings have implications for the recent changes in sea ice, hydrological cycle, and ecosystem over the Arctic.
Pengfei Shi, L. Ruby Leung, Bin Wang, Kai Zhang, Samson M. Hagos, and Shixuan Zhang
Geosci. Model Dev., 17, 3025–3040, https://doi.org/10.5194/gmd-17-3025-2024, https://doi.org/10.5194/gmd-17-3025-2024, 2024
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Improving climate predictions have profound socio-economic impacts. This study introduces a new weakly coupled land data assimilation (WCLDA) system for a coupled climate model. We demonstrate improved simulation of soil moisture and temperature in many global regions and throughout the soil layers. Furthermore, significant improvements are also found in reproducing the time evolution of the 2012 US Midwest drought. The WCLDA system provides the groundwork for future predictability studies.
Philip Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1031, https://doi.org/10.5194/egusphere-2024-1031, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming & climate impacts from greenhouse gas increases. The strategy slightly changes clouds in 6 ocean regions to reflect more sunlight & cool Earth. Example changes in clouds & climate are shown for 3 climate models. Clouds change differently between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
John T. Fasullo, Jean-Christophe Golaz, Julie M. Caron, Nan Rosenbloom, Gerald A. Meehl, Warren Strand, Sasha Glanville, Samantha Stevenson, Maria Molina, Christine A. Shields, Chengzhu Zhang, James Benedict, Hailong Wang, and Tony Bartoletti
Earth Syst. Dynam., 15, 367–386, https://doi.org/10.5194/esd-15-367-2024, https://doi.org/10.5194/esd-15-367-2024, 2024
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Climate model large ensembles provide a unique and invaluable means for estimating the climate response to external forcing agents and quantify contrasts in model structure. Here, an overview of the Energy Exascale Earth System Model (E3SM) version 2 large ensemble is given along with comparisons to large ensembles from E3SM version 1 and versions 1 and 2 of the Community Earth System Model. The paper provides broad and important context for users of these ensembles.
Meng Li, Junichi Kurokawa, Qiang Zhang, Jung-Hun Woo, Tazuko Morikawa, Satoru Chatani, Zifeng Lu, Yu Song, Guannan Geng, Hanwen Hu, Jinseok Kim, Owen R. Cooper, and Brian C. McDonald
Atmos. Chem. Phys., 24, 3925–3952, https://doi.org/10.5194/acp-24-3925-2024, https://doi.org/10.5194/acp-24-3925-2024, 2024
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In this work, we developed MIXv2, a mosaic Asian emission inventory for 2010–2017. With high spatial (0.1°) and monthly temporal resolution, MIXv2 integrates anthropogenic and open biomass burning emissions across seven sectors following a mosaic methodology. It provides CO2 emissions data alongside nine key pollutants and three chemical mechanisms. Our publicly accessible gridded monthly emissions data can facilitate long-term atmospheric and climate model analyses.
Lingbo Li, Hong-Yi Li, Guta Abeshu, Jinyun Tang, L. Ruby Leung, Chang Liao, Zeli Tan, Hanqin Tian, Peter Thornton, and Xiaojuan Yang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-43, https://doi.org/10.5194/essd-2024-43, 2024
Preprint under review for ESSD
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We have developed a new map that reveals how organic carbon from soil leaches into headwater streams over the contiguous United States. We use advanced artificial intelligence techniques and a massive amount of data, including observations at over 2,500 gauges and a wealth of climate and environmental information. The map is a critical step in understanding and predicting how carbon moves through our environment, hence a useful tool for tackling climate challenges.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-778, https://doi.org/10.5194/egusphere-2024-778, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in drier, warmer air, which can lead to a reduction in cloud. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence had led us to conclude.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Honglin Pan, Jianping Huang, Jiming Li, Zhongwei Huang, Minzhong Wang, Ali Mamtimin, Wen Huo, Fan Yang, Tian Zhou, and Kanike Raghavendra Kumar
Earth Syst. Sci. Data, 16, 1185–1207, https://doi.org/10.5194/essd-16-1185-2024, https://doi.org/10.5194/essd-16-1185-2024, 2024
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We applied several correction procedures and rigorously checked for data quality constraints during the long observation period spanning almost 14 years (2007–2020). Nevertheless, some uncertainties remain, mainly due to technical constraints and limited documentation of the measurements. Even though not completely accurate, this strategy is expected to at least reduce the inaccuracy of the computed characteristic value of aerosol optical parameters.
Yuxin Zhao, Jiming Li, Deyu Wen, Yarong Li, Yuan Wang, and Jianping Huang
EGUsphere, https://doi.org/10.5194/egusphere-2024-480, https://doi.org/10.5194/egusphere-2024-480, 2024
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This study identifies deep convection systems (DCSs), including deep convection core and anvils over Tibetan Plateau and Tropical Oceans. The results show that the DCSs over TP are less frequent, exhibiting narrower and thinner cores and anvils compared to those over TO. The TP DCSs show stronger longwave cloud radiative effect on the surface and low-level atmosphere. Unique aerosol-cloud-precipitation interaction is found in TP DCSs, due to the cold cloud bases.
Chen Zhang, John J. Cassano, Mark Seefeldt, Hailong Wang, Weiming Ma, and Wen-wen Tung
EGUsphere, https://doi.org/10.5194/egusphere-2024-320, https://doi.org/10.5194/egusphere-2024-320, 2024
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An atmospheric river (AR) is a long, narrow corridor of moisture transport in the atmosphere. ARs are crucial for moisture and heat transport into the polar regions. Our study examines the role of ARs on the surface energy budget (SEB) in the Arctic. The results reveal distinct seasonality and land-sea-sea ice contrasts due to the impacts of ARs on the SEB. The conclusions provide greater insights into the current and future role of ARs on the Arctic climate system.
Hui Wan, Kai Zhang, Christopher J. Vogl, Carol S. Woodward, Richard C. Easter, Philip J. Rasch, Yan Feng, and Hailong Wang
Geosci. Model Dev., 17, 1387–1407, https://doi.org/10.5194/gmd-17-1387-2024, https://doi.org/10.5194/gmd-17-1387-2024, 2024
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Sophisticated numerical models of the Earth's atmosphere include representations of many physical and chemical processes. In numerical simulations, these processes need to be calculated in a certain sequence. This study reveals the weaknesses of the sequence of calculations used for aerosol processes in a global atmosphere model. A revision of the sequence is proposed and its impacts on the simulated global aerosol climatology are evaluated.
Donghui Xu, Gautam Bisht, Zeli Tan, Chang Liao, Tian Zhou, Hong-Yi Li, and L. Ruby Leung
Geosci. Model Dev., 17, 1197–1215, https://doi.org/10.5194/gmd-17-1197-2024, https://doi.org/10.5194/gmd-17-1197-2024, 2024
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We aim to disentangle the hydrological and hydraulic controls on streamflow variability in a fully coupled earth system model. We found that calibrating only one process (i.e., traditional calibration procedure) will result in unrealistic parameter values and poor performance of the water cycle, while the simulated streamflow is improved. To address this issue, we further proposed a two-step calibration procedure to reconcile the impacts from hydrological and hydraulic processes on streamflow.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
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This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Yang Yang, Yang Zhou, Hailong Wang, Mengyun Li, Huimin Li, Pinya Wang, Xu Yue, Ke Li, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 24, 1177–1191, https://doi.org/10.5194/acp-24-1177-2024, https://doi.org/10.5194/acp-24-1177-2024, 2024
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This study reveals that extreme ozone pollution over the North China Plain and Yangtze River Delta is due to the chemical production related to hot and dry conditions, and the regional transport explains the ozone pollution over the Sichuan Basin and Pearl River Delta. The frequency of meteorological conditions of the extreme ozone pollution increases from the past to the future. The sustainable scenario is the optimal path to retaining clean air in China in the future.
Ye Liu, Yun Qian, Larry K. Berg, Zhe Feng, Jianfeng Li, Jingyi Chen, and Zhao Yang
EGUsphere, https://doi.org/10.5194/egusphere-2024-112, https://doi.org/10.5194/egusphere-2024-112, 2024
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Various weather conditions influence different intense rains in southeastern Texas. MCSs contribute to both average and extreme rainfall year-round, while IDC play a role in heavy rain during summer and fall. In spring, fall, and winter, frontal weather triggers convection, while in summer, IDC is linked to both fronts and high-pressure systems, and MCSs are more associated with fronts. Front-associated convection starts around 1100 UTC, while high-pressure-related convection starts a bit later.
Yuying Zhang, Shaocheng Xie, Yi Qin, Wuyin Lin, Jean-Christophe Golaz, Xue Zheng, Po-Lun Ma, Yun Qian, Qi Tang, Christopher R. Terai, and Meng Zhang
Geosci. Model Dev., 17, 169–189, https://doi.org/10.5194/gmd-17-169-2024, https://doi.org/10.5194/gmd-17-169-2024, 2024
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We performed systematic evaluation of clouds simulated in the Energy
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Exascale Earth System Model (E3SMv2) to document model performance and understand what updates in E3SMv2 have caused changes in clouds from E3SMv1 to E3SMv2. We find that stratocumulus clouds along the subtropical west coast of continents are dramatically improved, primarily due to the retuning done in CLUBB. This study offers additional insights into clouds simulated in E3SMv2 and will benefit future E3SM developments.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
EGUsphere, https://doi.org/10.5194/egusphere-2023-3149, https://doi.org/10.5194/egusphere-2023-3149, 2024
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We examined marine boundary-layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement in simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration are different, which warrants further investigation.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Dongyu Feng, Zeli Tan, Donghui Xu, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 27, 3911–3934, https://doi.org/10.5194/hess-27-3911-2023, https://doi.org/10.5194/hess-27-3911-2023, 2023
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This study assesses the flood risks concurrently induced by river flooding and coastal storm surge along the coast of the contiguous United States using statistical and numerical models. We reveal a few hotspots of such risks, the critical spatial variabilities within a river basin and over the whole US coast, and the uncertainties of the risk assessment. We highlight the importance of weighing different risk measures to avoid underestimating or exaggerating the compound flood impacts.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Lingcheng Li, Yilin Fang, Zhonghua Zheng, Mingjie Shi, Marcos Longo, Charles D. Koven, Jennifer A. Holm, Rosie A. Fisher, Nate G. McDowell, Jeffrey Chambers, and L. Ruby Leung
Geosci. Model Dev., 16, 4017–4040, https://doi.org/10.5194/gmd-16-4017-2023, https://doi.org/10.5194/gmd-16-4017-2023, 2023
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Accurately modeling plant coexistence in vegetation demographic models like ELM-FATES is challenging. This study proposes a repeatable method that uses machine-learning-based surrogate models to optimize plant trait parameters in ELM-FATES. Our approach significantly improves plant coexistence modeling, thus reducing errors. It has important implications for modeling ecosystem dynamics in response to climate change.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
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High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Koichi Sakaguchi, L. Ruby Leung, Colin M. Zarzycki, Jihyeon Jang, Seth McGinnis, Bryce E. Harrop, William C. Skamarock, Andrew Gettelman, Chun Zhao, William J. Gutowski, Stephen Leak, and Linda Mearns
Geosci. Model Dev., 16, 3029–3081, https://doi.org/10.5194/gmd-16-3029-2023, https://doi.org/10.5194/gmd-16-3029-2023, 2023
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We document details of the regional climate downscaling dataset produced by a global variable-resolution model. The experiment is unique in that it follows a standard protocol designed for coordinated experiments of regional models. We found negligible influence of post-processing on statistical analysis, importance of simulation quality outside of the target region, and computational challenges that our model code faced due to rapidly changing super computer systems.
Aishwarya Raman, Thomas Hill, Paul J. DeMott, Balwinder Singh, Kai Zhang, Po-Lun Ma, Mingxuan Wu, Hailong Wang, Simon P. Alexander, and Susannah M. Burrows
Atmos. Chem. Phys., 23, 5735–5762, https://doi.org/10.5194/acp-23-5735-2023, https://doi.org/10.5194/acp-23-5735-2023, 2023
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Ice-nucleating particles (INPs) play an important role in cloud processes and associated precipitation. Yet, INPs are not accurately represented in climate models. This study attempts to uncover these gaps by comparing model-simulated INP concentrations against field campaign measurements in the SO for an entire year, 2017–2018. Differences in INP concentrations and variability between the model and observations have major implications for modeling cloud properties in high latitudes.
Zhe Feng, Joseph Hardin, Hannah C. Barnes, Jianfeng Li, L. Ruby Leung, Adam Varble, and Zhixiao Zhang
Geosci. Model Dev., 16, 2753–2776, https://doi.org/10.5194/gmd-16-2753-2023, https://doi.org/10.5194/gmd-16-2753-2023, 2023
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PyFLEXTRKR is a flexible atmospheric feature tracking framework with specific capabilities to track convective clouds from a variety of observations and model simulations. The package has a collection of multi-object identification algorithms and has been optimized for large datasets. This paper describes the algorithms and demonstrates applications for tracking deep convective cells and mesoscale convective systems from observations and model simulations at a wide range of scales.
Zeyu Xue, Paul Ullrich, and Lai-Yung Ruby Leung
Hydrol. Earth Syst. Sci., 27, 1909–1927, https://doi.org/10.5194/hess-27-1909-2023, https://doi.org/10.5194/hess-27-1909-2023, 2023
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We examine the sensitivity and robustness of conclusions drawn from the PGW method over the NEUS by conducting multiple PGW experiments and varying the perturbation spatial scales and choice of perturbed meteorological variables to provide a guideline for this increasingly popular regional modeling method. Overall, we recommend PGW experiments be performed with perturbations to temperature or the combination of temperature and wind at the gridpoint scale, depending on the research question.
Pengwei Li, Yang Yang, Hailong Wang, Su Li, Ke Li, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 23, 5403–5417, https://doi.org/10.5194/acp-23-5403-2023, https://doi.org/10.5194/acp-23-5403-2023, 2023
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We use a novel technique that can attribute O3 to precursors to investigate O3 changes in the United States during 1995–2019. We found that the US domestic energy and surface transportation emission reductions are primarily responsible for the O3 decrease in summer. In winter, factors such as nitrogen oxide emission reduction in the context of its inhibition of ozone production, increased aviation and shipping activities, and large-scale circulation changes contribute to the O3 increases.
Hongxia Zhu, Rui Li, Shuping Yang, Chun Zhao, Zhe Jiang, and Chen Huang
Atmos. Chem. Phys., 23, 2421–2437, https://doi.org/10.5194/acp-23-2421-2023, https://doi.org/10.5194/acp-23-2421-2023, 2023
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The impacts of atmospheric dust aerosols and cloud dynamic conditions on precipitation vertical development in southeastern China were studied using multiple satellite observations. It was found that the precipitating drops under dusty conditions grow faster in the middle layer but slower in the upper and lower layers compared with their pristine counterparts. Quantitative estimation of the sensitivity of the precipitation top temperature to the dust aerosol optical depth is also provided.
Dalei Hao, Gautam Bisht, Karl Rittger, Timbo Stillinger, Edward Bair, Yu Gu, and L. Ruby Leung
The Cryosphere, 17, 673–697, https://doi.org/10.5194/tc-17-673-2023, https://doi.org/10.5194/tc-17-673-2023, 2023
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We comprehensively evaluated the snow simulations in E3SM land model over the western United States in terms of spatial patterns, temporal correlations, interannual variabilities, elevation gradients, and change with forest cover of snow properties and snow phenology. Our study underscores the need for diagnosing model biases and improving the model representations of snow properties and snow phenology in mountainous areas for more credible simulation and future projection of mountain snowpack.
Chandan Sarangi, Yun Qian, L. Ruby Leung, Yang Zhang, Yufei Zou, and Yuhang Wang
Atmos. Chem. Phys., 23, 1769–1783, https://doi.org/10.5194/acp-23-1769-2023, https://doi.org/10.5194/acp-23-1769-2023, 2023
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We show that for air quality, the densely populated eastern US may see even larger impacts of wildfires due to long-distance smoke transport and associated positive climatic impacts, partially compensating the improvements from regulations on anthropogenic emissions. This study highlights the tension between natural and anthropogenic contributions and the non-local nature of air pollution that complicate regulatory strategies for improving future regional air quality for human health.
Mengyun Li, Yang Yang, Hailong Wang, Huimin Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1533–1544, https://doi.org/10.5194/acp-23-1533-2023, https://doi.org/10.5194/acp-23-1533-2023, 2023
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Using the GEOS-Chem model, the impact of the quasi-biennial oscillation (QBO) on summertime tropospheric O3 in China is investigated. In the warm phases of sea surface temperature anomalies over the eastern tropical Pacific, the QBO has a significant positive correlation with near-surface O3 concentrations over central China. The QBO impacts on O3 pollution in China are mainly a result of changing vertical transport of O3.
Huimin Li, Yang Yang, Jianbing Jin, Hailong Wang, Ke Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1131–1145, https://doi.org/10.5194/acp-23-1131-2023, https://doi.org/10.5194/acp-23-1131-2023, 2023
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Future climate change will aggravate ozone pollution in Asia, especially in high-forcing scenarios. Ozone pollution in China will expand from North China to South China and extend into the cold season in a warmer future. The emphasis of this work is to quantify the impacts of future climate change on O3 pollution in Asia, which is of great significance for future O3 pollution mitigation strategies.
Younjoo J. Lee, Wieslaw Maslowski, John J. Cassano, Jaclyn Clement Kinney, Anthony P. Craig, Samy Kamal, Robert Osinski, Mark W. Seefeldt, Julienne Stroeve, and Hailong Wang
The Cryosphere, 17, 233–253, https://doi.org/10.5194/tc-17-233-2023, https://doi.org/10.5194/tc-17-233-2023, 2023
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During 1979–2020, four winter polynyas occurred in December 1986 and February 2011, 2017, and 2018 north of Greenland. Instead of ice melting due to the anomalous warm air intrusion, the extreme wind forcing resulted in greater ice transport offshore. Based on the two ensemble runs, representing a 1980s thicker ice vs. a 2010s thinner ice, a dominant cause of these winter polynyas stems from internal variability of atmospheric forcing rather than from the forced response to a warming climate.
Yuxin Zhao, Jiming Li, Lijie Zhang, Cong Deng, Yarong Li, Bida Jian, and Jianping Huang
Atmos. Chem. Phys., 23, 743–769, https://doi.org/10.5194/acp-23-743-2023, https://doi.org/10.5194/acp-23-743-2023, 2023
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Diurnal variations of clouds play an important role in the radiative budget and precipitation. Based on satellite observations, reanalysis, and CMIP6 outputs, the diurnal variations in total cloud cover and cloud vertical distribution over the Tibetan Plateau are explored. The diurnal cycle of cirrus is a key focus and found to have different characteristics from those found in the tropics. The relationship between the diurnal cycle of cirrus and meteorological factors is also discussed.
Cynthia H. Whaley, Kathy S. Law, Jens Liengaard Hjorth, Henrik Skov, Stephen R. Arnold, Joakim Langner, Jakob Boyd Pernov, Garance Bergeron, Ilann Bourgeois, Jesper H. Christensen, Rong-You Chien, Makoto Deushi, Xinyi Dong, Peter Effertz, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Greg Huey, Ulas Im, Rigel Kivi, Louis Marelle, Tatsuo Onishi, Naga Oshima, Irina Petropavlovskikh, Jeff Peischl, David A. Plummer, Luca Pozzoli, Jean-Christophe Raut, Tom Ryerson, Ragnhild Skeie, Sverre Solberg, Manu A. Thomas, Chelsea Thompson, Kostas Tsigaridis, Svetlana Tsyro, Steven T. Turnock, Knut von Salzen, and David W. Tarasick
Atmos. Chem. Phys., 23, 637–661, https://doi.org/10.5194/acp-23-637-2023, https://doi.org/10.5194/acp-23-637-2023, 2023
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This study summarizes recent research on ozone in the Arctic, a sensitive and rapidly warming region. We find that the seasonal cycles of near-surface atmospheric ozone are variable depending on whether they are near the coast, inland, or at high altitude. Several global model simulations were evaluated, and we found that because models lack some of the ozone chemistry that is important for the coastal Arctic locations, they do not accurately simulate ozone there.
Dalei Hao, Gautam Bisht, Karl Rittger, Edward Bair, Cenlin He, Huilin Huang, Cheng Dang, Timbo Stillinger, Yu Gu, Hailong Wang, Yun Qian, and L. Ruby Leung
Geosci. Model Dev., 16, 75–94, https://doi.org/10.5194/gmd-16-75-2023, https://doi.org/10.5194/gmd-16-75-2023, 2023
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Snow with the highest albedo of land surface plays a vital role in Earth’s surface energy budget and water cycle. This study accounts for the impacts of snow grain shape and mixing state of light-absorbing particles with snow on snow albedo in the E3SM land model. The findings advance our understanding of the role of snow grain shape and mixing state of LAP–snow in land surface processes and offer guidance for improving snow simulations and radiative forcing estimates in Earth system models.
Huilin Huang, Yun Qian, Ye Liu, Cenlin He, Jianyu Zheng, Zhibo Zhang, and Antonis Gkikas
Atmos. Chem. Phys., 22, 15469–15488, https://doi.org/10.5194/acp-22-15469-2022, https://doi.org/10.5194/acp-22-15469-2022, 2022
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Using a clustering method developed in the field of artificial neural networks, we identify four typical dust transport patterns across the Sierra Nevada, associated with the mesoscale and regional-scale wind circulations. Our results highlight the connection between dust transport and dominant weather patterns, which can be used to understand dust transport in a changing climate.
Yang Yang, Liangying Zeng, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 22, 14489–14502, https://doi.org/10.5194/acp-22-14489-2022, https://doi.org/10.5194/acp-22-14489-2022, 2022
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Using an aerosol–climate model, dust pollution in China affected by different spatial and temporal types of El Niño are examined. Both eastern and central Pacific El Niño and short-duration El Niño increase winter dust concentrations over northern China, while long-duration El Niño decreases concentrations. Only long-duration El Niño events can significantly affect dust over China in the following spring. This study has profound implications for air pollution control and dust storm prediction.
Dongyu Feng, Zeli Tan, Darren Engwirda, Chang Liao, Donghui Xu, Gautam Bisht, Tian Zhou, Hong-Yi Li, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 26, 5473–5491, https://doi.org/10.5194/hess-26-5473-2022, https://doi.org/10.5194/hess-26-5473-2022, 2022
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Sea level rise, storm surge and river discharge can cause coastal backwater effects in downstream sections of rivers, creating critical flood risks. This study simulates the backwater effects using a large-scale river model on a coastal-refined computational mesh. By decomposing the backwater drivers, we revealed their relative importance and long-term variations. Our analysis highlights the increasing strength of backwater effects due to sea level rise and more frequent storm surge.
Yilin Fang, L. Ruby Leung, Charles D. Koven, Gautam Bisht, Matteo Detto, Yanyan Cheng, Nate McDowell, Helene Muller-Landau, S. Joseph Wright, and Jeffrey Q. Chambers
Geosci. Model Dev., 15, 7879–7901, https://doi.org/10.5194/gmd-15-7879-2022, https://doi.org/10.5194/gmd-15-7879-2022, 2022
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We develop a model that integrates an Earth system model with a three-dimensional hydrology model to explicitly resolve hillslope topography and water flow underneath the land surface to understand how local-scale hydrologic processes modulate vegetation along water availability gradients. Our coupled model can be used to improve the understanding of the diverse impact of local heterogeneity and water flux on nutrient availability and plant communities.
Zachary Fair, Mark Flanner, Adam Schneider, and S. McKenzie Skiles
The Cryosphere, 16, 3801–3814, https://doi.org/10.5194/tc-16-3801-2022, https://doi.org/10.5194/tc-16-3801-2022, 2022
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Snow grain size is important to determine the age and structure of snow, but it is difficult to measure. Snow grain size can be found from airborne and spaceborne observations by measuring near-infrared energy reflected from snow. In this study, we use the SNICAR radiative transfer model and a Monte Carlo model to examine how snow grain size measurements change with snow structure and solar zenith angle. We show that improved understanding of these variables improves snow grain size precision.
Meng Huang, Po-Lun Ma, Nathaniel W. Chaney, Dalei Hao, Gautam Bisht, Megan D. Fowler, Vincent E. Larson, and L. Ruby Leung
Geosci. Model Dev., 15, 6371–6384, https://doi.org/10.5194/gmd-15-6371-2022, https://doi.org/10.5194/gmd-15-6371-2022, 2022
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The land surface in one grid cell may be diverse in character. This study uses an explicit way to account for that subgrid diversity in a state-of-the-art Earth system model (ESM) and explores its implications for the overlying atmosphere. We find that the shallow clouds are increased significantly with the land surface diversity. Our work highlights the importance of accurately representing the land surface and its interaction with the atmosphere in next-generation ESMs.
Yilin Fang, L. Ruby Leung, Ryan Knox, Charlie Koven, and Ben Bond-Lamberty
Geosci. Model Dev., 15, 6385–6398, https://doi.org/10.5194/gmd-15-6385-2022, https://doi.org/10.5194/gmd-15-6385-2022, 2022
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Accounting for water movement in the soil and water transport within the plant is important for plant growth in Earth system modeling. We implemented different numerical approaches for a plant hydrodynamic model and compared their impacts on the simulated aboveground biomass (AGB) at single points and globally. We found care should be taken when discretizing the number of soil layers for numerical simulations as it can significantly affect AGB if accuracy and computational costs are of concern.
Xueyin Ruan, Chun Zhao, Rahul A. Zaveri, Pengzhen He, Xinming Wang, Jingyuan Shao, and Lei Geng
Geosci. Model Dev., 15, 6143–6164, https://doi.org/10.5194/gmd-15-6143-2022, https://doi.org/10.5194/gmd-15-6143-2022, 2022
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Accurate prediction of aerosol pH in chemical transport models is essential to aerosol modeling. This study examines the performance of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) on aerosol pH predictions and the sensitivities to emissions of nonvolatile cations and NH3, aerosol-phase state assumption, and heterogeneous sulfate production. Temporal evolution of aerosol pH during haze cycles in Beijing and the driving factors are also presented and discussed.
Sol Kim, L. Ruby Leung, Bin Guan, and John C. H. Chiang
Geosci. Model Dev., 15, 5461–5480, https://doi.org/10.5194/gmd-15-5461-2022, https://doi.org/10.5194/gmd-15-5461-2022, 2022
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The Energy Exascale Earth System Model (E3SM) project is a state-of-the-science Earth system model developed by the US Department of Energy (DOE). Understanding how the water cycle behaves in this model is of particular importance to the DOE’s mission. Atmospheric rivers (ARs) – which are crucial to the global water cycle – move vast amounts of water vapor through the sky and produce rain and snow. We find that this model reliably represents atmospheric rivers around the world.
Lingcheng Li, Gautam Bisht, and L. Ruby Leung
Geosci. Model Dev., 15, 5489–5510, https://doi.org/10.5194/gmd-15-5489-2022, https://doi.org/10.5194/gmd-15-5489-2022, 2022
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Land surface heterogeneity plays a critical role in the terrestrial water, energy, and biogeochemical cycles. Our study systematically quantified the effects of four dominant heterogeneity sources on water and energy partitioning via Sobol' indices. We found that atmospheric forcing and land use land cover are the most dominant heterogeneity sources in determining spatial variability of water and energy partitioning. Our findings can help prioritize the future development of land surface models.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
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Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Donghui Xu, Gautam Bisht, Khachik Sargsyan, Chang Liao, and L. Ruby Leung
Geosci. Model Dev., 15, 5021–5043, https://doi.org/10.5194/gmd-15-5021-2022, https://doi.org/10.5194/gmd-15-5021-2022, 2022
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The runoff outputs in Earth system model simulations involve high uncertainty, which needs to be constrained by parameter calibration. In this work, we used a surrogate-assisted Bayesian framework to efficiently calibrate the runoff-generation processes in the Energy Exascale Earth System Model v1 at a global scale. The model performance was improved compared to the default parameter after calibration, and the associated parametric uncertainty was significantly constrained.
Jiyuan Gao, Yang Yang, Hailong Wang, Pinya Wang, Huimin Li, Mengyun Li, Lili Ren, Xu Yue, and Hong Liao
Atmos. Chem. Phys., 22, 7131–7142, https://doi.org/10.5194/acp-22-7131-2022, https://doi.org/10.5194/acp-22-7131-2022, 2022
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China has been implementing a sequence of policies for clean air since the year 2013. The aerosol decline produced a 0.09 ± 0.10°C warming during 2013–2017 estimated in this study, and the increase in ozone in the lower troposphere during this time period accelerated the warming, leading to a total 0.16 ± 0.15°C temperature increase in eastern China. Residential emission reductions led to a cooling effect because of a substantial decrease in light-absorbing aerosols.
Yun Lin, Jiwen Fan, Pengfei Li, Lai-yung Ruby Leung, Paul J. DeMott, Lexie Goldberger, Jennifer Comstock, Ying Liu, Jong-Hoon Jeong, and Jason Tomlinson
Atmos. Chem. Phys., 22, 6749–6771, https://doi.org/10.5194/acp-22-6749-2022, https://doi.org/10.5194/acp-22-6749-2022, 2022
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How sea spray aerosols may affect cloud and precipitation over the region by acting as ice-nucleating particles (INPs) is unknown. We explored the effects of INPs from marine aerosols on orographic cloud and precipitation for an atmospheric river event observed during the 2015 ACAPEX field campaign. The marine INPs enhance the formation of ice and snow, leading to less shallow warm clouds but more mixed-phase and deep clouds. This work suggests models need to consider the impacts of marine INPs.
Xue Zheng, Qing Li, Tian Zhou, Qi Tang, Luke P. Van Roekel, Jean-Christophe Golaz, Hailong Wang, and Philip Cameron-Smith
Geosci. Model Dev., 15, 3941–3967, https://doi.org/10.5194/gmd-15-3941-2022, https://doi.org/10.5194/gmd-15-3941-2022, 2022
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We document the model experiments for the future climate projection by E3SMv1.0. At the highest future emission scenario, E3SMv1.0 projects a strong surface warming with rapid changes in the atmosphere, ocean, sea ice, and land runoff. Specifically, we detect a significant polar amplification and accelerated warming linked to the unmasking of the aerosol effects. The impact of greenhouse gas forcing is examined in different climate components.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
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Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Pinya Wang, Yang Yang, Huimin Li, Lei Chen, Ruijun Dang, Daokai Xue, Baojie Li, Jianping Tang, L. Ruby Leung, and Hong Liao
Atmos. Chem. Phys., 22, 4705–4719, https://doi.org/10.5194/acp-22-4705-2022, https://doi.org/10.5194/acp-22-4705-2022, 2022
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China is now suffering from both severe ozone (O3) pollution and heat events. We highlight that North China Plain is the hot spot of the co-occurrences of extremes in O3 and high temperatures in China. Such coupled extremes exhibit an increasing trend during 2014–2019 and will continue to increase until the middle of this century. And the coupled extremes impose more severe health impacts to human than O3 pollution occurring alone because of elevated O3 levels and temperatures.
Chloe A. Whicker, Mark G. Flanner, Cheng Dang, Charles S. Zender, Joseph M. Cook, and Alex S. Gardner
The Cryosphere, 16, 1197–1220, https://doi.org/10.5194/tc-16-1197-2022, https://doi.org/10.5194/tc-16-1197-2022, 2022
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Snow and ice surfaces are important to the global climate. Current climate models use measurements to determine the reflectivity of ice. This model uses physical properties to determine the reflectivity of snow, ice, and darkly pigmented impurities that reside within the snow and ice. Therefore, the modeled reflectivity is more accurate for snow/ice columns under varying climate conditions. This model paves the way for improvements in the portrayal of snow and ice within global climate models.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Sally S.-C. Wang, Yun Qian, L. Ruby Leung, and Yang Zhang
Atmos. Chem. Phys., 22, 3445–3468, https://doi.org/10.5194/acp-22-3445-2022, https://doi.org/10.5194/acp-22-3445-2022, 2022
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This study develops an interpretable machine learning (ML) model predicting monthly PM2.5 fire emission over the contiguous US at 0.25° resolution and compares the prediction skills of the ML and process-based models. The comparison facilitates attributions of model biases and better understanding of the strengths and uncertainties in the two types of models at regional scales, for informing future model development and their applications in fire emission projection.
Guta Wakbulcho Abeshu, Hong-Yi Li, Zhenduo Zhu, Zeli Tan, and L. Ruby Leung
Earth Syst. Sci. Data, 14, 929–942, https://doi.org/10.5194/essd-14-929-2022, https://doi.org/10.5194/essd-14-929-2022, 2022
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Existing riverbed sediment particle size data are sparsely available at individual sites. We develop a continuous map of median riverbed sediment particle size over the contiguous US corresponding to millions of river segments based on the existing observations and machine learning methods. This map is useful for research in large-scale river sediment using model- and data-driven approaches, teaching environmental and earth system sciences, planning and managing floodplain zones, etc.
Hong-Yi Li, Zeli Tan, Hongbo Ma, Zhenduo Zhu, Guta Wakbulcho Abeshu, Senlin Zhu, Sagy Cohen, Tian Zhou, Donghui Xu, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 26, 665–688, https://doi.org/10.5194/hess-26-665-2022, https://doi.org/10.5194/hess-26-665-2022, 2022
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We introduce a new multi-process river sediment module for Earth system models. Application and validation over the contiguous US indicate a satisfactory model performance over large river systems, including those heavily regulated by reservoirs. This new sediment module enables future modeling of the transportation and transformation of carbon and nutrients carried by the fine sediment along the river–ocean continuum to close the global carbon and nutrient cycles.
Ye Liu, Yun Qian, and Larry K. Berg
Wind Energ. Sci., 7, 37–51, https://doi.org/10.5194/wes-7-37-2022, https://doi.org/10.5194/wes-7-37-2022, 2022
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Uncertainties in initial conditions (ICs) decrease the accuracy of wind speed forecasts. We find that IC uncertainties can alter wind speed by modulating the weather system. IC uncertainties in local thermal gradient and large-scale circulation jointly contribute to wind speed forecast uncertainties. Wind forecast accuracy in the Columbia River Basin is confined by initial uncertainties in a few specific regions, providing useful information for more intense measurement and modeling studies.
Xiaodong Wang, Chun Zhao, Mingyue Xu, Qiuyan Du, Jianqiu Zheng, Yun Bi, Shengfu Lin, and Yali Luo
Geosci. Model Dev., 15, 199–218, https://doi.org/10.5194/gmd-15-199-2022, https://doi.org/10.5194/gmd-15-199-2022, 2022
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Regional models are widely used to investigate aerosol climatic impacts. However, there are few studies examining the sensitivities of modeling results to regional domain size. In this study, the regional model is used to study the aerosol impacts on the East Asian summer monsoon system and focus on the modeling sensitivities to domain size. This study highlights the important impacts of domain size on regional modeling results of aerosol climatic impacts, which may not be limited to East Asia.
Mark G. Flanner, Julian B. Arnheim, Joseph M. Cook, Cheng Dang, Cenlin He, Xianglei Huang, Deepak Singh, S. McKenzie Skiles, Chloe A. Whicker, and Charles S. Zender
Geosci. Model Dev., 14, 7673–7704, https://doi.org/10.5194/gmd-14-7673-2021, https://doi.org/10.5194/gmd-14-7673-2021, 2021
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We present the technical formulation and evaluation of a publicly available code and web-based model to simulate the spectral albedo of snow. Our model accounts for numerous features of the snow state and ambient conditions, including the the presence of light-absorbing matter like black and brown carbon, mineral dust, volcanic ash, and snow algae. Carbon dioxide snow, found on Mars, is also represented. The model accurately reproduces spectral measurements of clean and contaminated snow.
Claudia Tebaldi, Kalyn Dorheim, Michael Wehner, and Ruby Leung
Earth Syst. Dynam., 12, 1427–1501, https://doi.org/10.5194/esd-12-1427-2021, https://doi.org/10.5194/esd-12-1427-2021, 2021
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We address the question of how large an initial condition ensemble of climate model simulations should be if we are concerned with accurately projecting future changes in temperature and precipitation extremes. We find that for most cases (and both models considered), an ensemble of 20–25 members is sufficient for many extreme metrics, spatial scales and time horizons. This may leave computational resources to tackle other uncertainties in climate model simulations with our ensembles.
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021, https://doi.org/10.5194/acp-21-16121-2021, 2021
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This study investigates precipitation impacts on long-range transport of North American outflow over the western North Atlantic Ocean (WNAO). Results demonstrate that precipitation scavenging plays a significant role in modifying surface aerosol concentrations over the WNAO, especially in winter and spring due to large-scale scavenging processes. This study highlights how precipitation impacts surface aerosol properties with relevance for other marine regions vulnerable to continental outflow.
Dalei Hao, Gautam Bisht, Yu Gu, Wei-Liang Lee, Kuo-Nan Liou, and L. Ruby Leung
Geosci. Model Dev., 14, 6273–6289, https://doi.org/10.5194/gmd-14-6273-2021, https://doi.org/10.5194/gmd-14-6273-2021, 2021
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Topography exerts significant influence on the incoming solar radiation at the land surface. This study incorporated a well-validated sub-grid topographic parameterization in E3SM land model (ELM) version 1.0. The results demonstrate that sub-grid topography has non-negligible effects on surface energy budget, snow cover, and surface temperature over the Tibetan Plateau and that the ELM simulations are sensitive to season, elevation, and spatial scale.
Jingyu Yao, Zhongming Gao, Jianping Huang, Heping Liu, and Guoyin Wang
Atmos. Chem. Phys., 21, 15589–15603, https://doi.org/10.5194/acp-21-15589-2021, https://doi.org/10.5194/acp-21-15589-2021, 2021
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Gap-filling usually accounts for a large source of uncertainties in the annual CO2 fluxes, though gap-filling CO2 fluxes is challenging at dryland sites due to small fluxes. Using data collected from a semiarid site, four machine learning methods are evaluated with different lengths of artificial gaps. The artificial neural network and random forest methods outperform the other methods. With these methods, uncertainties in the annual CO2 flux at this site are estimated to be within 16 g C m−2.
Lili Ren, Yang Yang, Hailong Wang, Pinya Wang, Lei Chen, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 21, 15431–15445, https://doi.org/10.5194/acp-21-15431-2021, https://doi.org/10.5194/acp-21-15431-2021, 2021
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Due to the COVID-19 pandemic, human activities were strictly restricted in China. Even though anthropogenic aerosol emissions largely decreased, haze events still occurred. Our results shows that PM2.5 over the North China Plain is largely contributed by local sources. For other regions in China, PM2.5 is largely contributed from nonlocal sources. As emission reduction is a future goal, aerosol long-range transport and unfavorable meteorology are increasingly important to air quality.
Mingshuai Zhang, Chun Zhao, Yuhan Yang, Qiuyan Du, Yonglin Shen, Shengfu Lin, Dasa Gu, Wenjing Su, and Cheng Liu
Geosci. Model Dev., 14, 6155–6175, https://doi.org/10.5194/gmd-14-6155-2021, https://doi.org/10.5194/gmd-14-6155-2021, 2021
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Biogenic volatile organic compounds (BVOCs) can influence atmospheric chemistry and secondary pollutant formation. This study examines the performance of different versions of the Model of Emissions of Gases and Aerosols from Nature (MEGAN) in modeling BVOCs and ozone and their sensitivities to vegetation distributions over eastern China. The results suggest more accurate vegetation distribution and measurements of BVOC emission fluxes are needed to reduce the uncertainties.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
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The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
Liangying Zeng, Yang Yang, Hailong Wang, Jing Wang, Jing Li, Lili Ren, Huimin Li, Yang Zhou, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 21, 10745–10761, https://doi.org/10.5194/acp-21-10745-2021, https://doi.org/10.5194/acp-21-10745-2021, 2021
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Using an aerosol–climate model, the impacts of El Niño with different durations on aerosols in China are examined. The modulation on aerosol concentrations and haze days by short-duration El Niño events is 2–3 times more than that by long-duration El Niño events in China. The frequency of short-duration El Niño has been increasing significantly in recent decades, suggesting that El Niño events have exerted increasingly intense modulation on aerosol pollution in China over the past few decades.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Bida Jian, Jiming Li, Guoyin Wang, Yuxin Zhao, Yarong Li, Jing Wang, Min Zhang, and Jianping Huang
Atmos. Chem. Phys., 21, 9809–9828, https://doi.org/10.5194/acp-21-9809-2021, https://doi.org/10.5194/acp-21-9809-2021, 2021
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We evaluate the performance of the AMIP6 model in simulating cloud albedo over marine subtropical regions and the impacts of different aerosol types and meteorological factors on the cloud albedo based on multiple satellite datasets and reanalysis data. The results show that AMIP6 demonstrates moderate improvement over AMIP5 in simulating the monthly variation in cloud albedo, and changes in different aerosol types and meteorological factors can explain ~65 % of the changes in the cloud albedo.
Jianfeng Li, Zhe Feng, Yun Qian, and L. Ruby Leung
Earth Syst. Sci. Data, 13, 827–856, https://doi.org/10.5194/essd-13-827-2021, https://doi.org/10.5194/essd-13-827-2021, 2021
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Deep convection has different properties at different scales. We develop a 4 km h−1 observational data product of mesoscale convective systems and isolated deep convection in the United States from 2004–2017. We find that both types of convective systems contribute significantly to precipitation east of the Rocky Mountains but with distinct spatiotemporal characteristics. The data product will be useful for observational analyses and model evaluations of convection events at different scales.
Xiaoyu Hu, Jinming Ge, Jiajing Du, Qinghao Li, Jianping Huang, and Qiang Fu
Atmos. Meas. Tech., 14, 1743–1759, https://doi.org/10.5194/amt-14-1743-2021, https://doi.org/10.5194/amt-14-1743-2021, 2021
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Cloud radars are powerful instruments that can probe detailed cloud structures. However, radar echoes in the lower atmosphere are always contaminated by clutter. We proposed a multi-dimensional probability distribution function that can effectively discriminate low-level clouds from clutter by considering their different features in several variables. We applied this method to the radar observations at the SACOL site and found the results have good agreement with lidar detection.
Zhuang Wang, Cheng Liu, Zhouqing Xie, Qihou Hu, Meinrat O. Andreae, Yunsheng Dong, Chun Zhao, Ting Liu, Yizhi Zhu, Haoran Liu, Chengzhi Xing, Wei Tan, Xiangguang Ji, Jinan Lin, and Jianguo Liu
Atmos. Chem. Phys., 20, 14917–14932, https://doi.org/10.5194/acp-20-14917-2020, https://doi.org/10.5194/acp-20-14917-2020, 2020
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Significant stratification of aerosols was observed in North China. Polluted dust dominated above the PBL, and anthropogenic aerosols prevailed within the PBL, which is mainly driven by meteorological conditions. The key role of the elevated dust is to alter atmospheric thermodynamics and stability, causing the suppression of turbulence exchange and a decrease in PBL height, especially during the dissipation stage, thereby inhibiting dissipation of persistent heavy surface haze pollution.
Zachary Fair, Mark Flanner, Kelly M. Brunt, Helen Amanda Fricker, and Alex Gardner
The Cryosphere, 14, 4253–4263, https://doi.org/10.5194/tc-14-4253-2020, https://doi.org/10.5194/tc-14-4253-2020, 2020
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Ice on glaciers and ice sheets may melt and pond on ice surfaces in summer months. Detection and observation of these meltwater ponds is important for understanding glaciers and ice sheets, and satellite imagery has been used in previous work. However, image-based methods struggle with deep water, so we used data from the Ice, Clouds, and land Elevation Satellite-2 (ICESat-2) and the Airborne Topographic Mapper (ATM) to demonstrate the potential for lidar depth monitoring.
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
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The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Maoyi Huang, Yi Xu, Marcos Longo, Michael Keller, Ryan G. Knox, Charles D. Koven, and Rosie A. Fisher
Biogeosciences, 17, 4999–5023, https://doi.org/10.5194/bg-17-4999-2020, https://doi.org/10.5194/bg-17-4999-2020, 2020
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The Functionally Assembled Terrestrial Ecosystem Simulator (FATES) is enhanced to mimic the ecological, biophysical, and biogeochemical processes following a logging event. The model can specify the timing and aerial extent of logging events; determine the survivorship of cohorts in the disturbed forest; and modifying the biomass, coarse woody debris, and litter pools. This study lays the foundation to simulate land use change and forest degradation in FATES as part of an Earth system model.
Stefan Rahimi, Xiaohong Liu, Chun Zhao, Zheng Lu, and Zachary J. Lebo
Atmos. Chem. Phys., 20, 10911–10935, https://doi.org/10.5194/acp-20-10911-2020, https://doi.org/10.5194/acp-20-10911-2020, 2020
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Dark particles emitted to the atmosphere can absorb sunlight and heat the air. As these particles settle, they may darken the surface, especially over snow-covered regions like the Rocky Mountains. This darkening of the surface may lead to changes in snowpack, affecting the local meteorology and hydrology. We seek to evaluate whether these light-absorbing particles more prominently affect this region through their atmospheric presence or their on-snow presence.
Bethany Sutherland, Ben Kravitz, Philip J. Rasch, and Hailong Wang
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-228, https://doi.org/10.5194/gmd-2020-228, 2020
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Through a cascade of physical mechanisms, a change in one location can trigger a response in a different location. These responses and the mechanisms that cause them are difficult to detect. Here we propose a method, using global climate models, to detect possible relationships between changes in one region and responses throughout the globe caused by that change. A change in the Pacific ocean is used as a test case to determine the effectiveness of the method.
Lili Ren, Yang Yang, Hailong Wang, Rudong Zhang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 9067–9085, https://doi.org/10.5194/acp-20-9067-2020, https://doi.org/10.5194/acp-20-9067-2020, 2020
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Observations show that the concentrations of Arctic aerosols have declined since the early 1980s, which potentially contributed to the recent, rapid Arctic warming. We found that changes in sulfate and black carbon aerosols over the midlatitudes of the Northern Hemisphere had a larger impact on Arctic temperature than other regions and that the aerosol-induced temperature change explained approximately 20 % of the observed Arctic warming during 1980–2018.
Charles D. Koven, Ryan G. Knox, Rosie A. Fisher, Jeffrey Q. Chambers, Bradley O. Christoffersen, Stuart J. Davies, Matteo Detto, Michael C. Dietze, Boris Faybishenko, Jennifer Holm, Maoyi Huang, Marlies Kovenock, Lara M. Kueppers, Gregory Lemieux, Elias Massoud, Nathan G. McDowell, Helene C. Muller-Landau, Jessica F. Needham, Richard J. Norby, Thomas Powell, Alistair Rogers, Shawn P. Serbin, Jacquelyn K. Shuman, Abigail L. S. Swann, Charuleka Varadharajan, Anthony P. Walker, S. Joseph Wright, and Chonggang Xu
Biogeosciences, 17, 3017–3044, https://doi.org/10.5194/bg-17-3017-2020, https://doi.org/10.5194/bg-17-3017-2020, 2020
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Tropical forests play a crucial role in governing climate feedbacks, and are incredibly diverse ecosystems, yet most Earth system models do not take into account the diversity of plant traits in these forests and how this diversity may govern feedbacks. We present an approach to represent diverse competing plant types within Earth system models, test this approach at a tropical forest site, and explore how the representation of disturbance and competition governs traits of the forest community.
Pablo E. Saide, Meng Gao, Zifeng Lu, Daniel L. Goldberg, David G. Streets, Jung-Hun Woo, Andreas Beyersdorf, Chelsea A. Corr, Kenneth L. Thornhill, Bruce Anderson, Johnathan W. Hair, Amin R. Nehrir, Glenn S. Diskin, Jose L. Jimenez, Benjamin A. Nault, Pedro Campuzano-Jost, Jack Dibb, Eric Heim, Kara D. Lamb, Joshua P. Schwarz, Anne E. Perring, Jhoon Kim, Myungje Choi, Brent Holben, Gabriele Pfister, Alma Hodzic, Gregory R. Carmichael, Louisa Emmons, and James H. Crawford
Atmos. Chem. Phys., 20, 6455–6478, https://doi.org/10.5194/acp-20-6455-2020, https://doi.org/10.5194/acp-20-6455-2020, 2020
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Air quality forecasts over the Korean Peninsula captured aerosol optical depth but largely overpredicted surface PM during a Chinese haze transport event. Model deficiency was related to the calculation of optical properties. In order to improve it, aerosol size representation needs to be refined in the calculations, and the representation of aerosol properties, such as size distribution, chemical composition, refractive index, hygroscopicity parameter, and density, needs to be improved.
Meixin Zhang, Chun Zhao, Zhiyuan Cong, Qiuyan Du, Mingyue Xu, Yu Chen, Ming Chen, Rui Li, Yunfei Fu, Lei Zhong, Shichang Kang, Delong Zhao, and Yan Yang
Atmos. Chem. Phys., 20, 5923–5943, https://doi.org/10.5194/acp-20-5923-2020, https://doi.org/10.5194/acp-20-5923-2020, 2020
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Analysis of multiple numerical experiments over the Himalayas and Tibetan Plateau (TP) shows that the complex topography results in 50 % stronger overall cross-Himalayan transport during the pre-monsoon season primarily due to the strengthened efficiency of near-surface meridional transport towards the TP, enhanced wind speed in some valleys and deeper valley channels associated with larger transported BC mass volume, which leads to 30–50 % stronger BC radiative heating over the TP.
Kurt C. Solander, Brent D. Newman, Alessandro Carioca de Araujo, Holly R. Barnard, Z. Carter Berry, Damien Bonal, Mario Bretfeld, Benoit Burban, Luiz Antonio Candido, Rolando Célleri, Jeffery Q. Chambers, Bradley O. Christoffersen, Matteo Detto, Wouter A. Dorigo, Brent E. Ewers, Savio José Filgueiras Ferreira, Alexander Knohl, L. Ruby Leung, Nate G. McDowell, Gretchen R. Miller, Maria Terezinha Ferreira Monteiro, Georgianne W. Moore, Robinson Negron-Juarez, Scott R. Saleska, Christian Stiegler, Javier Tomasella, and Chonggang Xu
Hydrol. Earth Syst. Sci., 24, 2303–2322, https://doi.org/10.5194/hess-24-2303-2020, https://doi.org/10.5194/hess-24-2303-2020, 2020
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We evaluate the soil moisture response in the humid tropics to El Niño during the three most recent super El Niño events. Our estimates are compared to in situ soil moisture estimates that span five continents. We find the strongest and most consistent soil moisture decreases in the Amazon and maritime southeastern Asia, while the most consistent increases occur over eastern Africa. Our results can be used to improve estimates of soil moisture in tropical ecohydrology models at multiple scales.
Yi Zeng, Minghuai Wang, Chun Zhao, Siyu Chen, Zhoukun Liu, Xin Huang, and Yang Gao
Geosci. Model Dev., 13, 2125–2147, https://doi.org/10.5194/gmd-13-2125-2020, https://doi.org/10.5194/gmd-13-2125-2020, 2020
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Dust aerosol can impact many processes of the Earth system, but large uncertainties still remain in dust simulations. In this study, we investigated dust simulation sensitivity to two dust emission schemes and three dry deposition schemes using WRF-Chem. An optimal combination of dry deposition scheme and dust emission scheme has been identified to best simulate the dust storm in comparison with observation. Our results highlight the importance of dry deposition schemes for dust simulation.
Yufei Zou, Yuhang Wang, Zuowei Xie, Hailong Wang, and Philip J. Rasch
Atmos. Chem. Phys., 20, 4999–5017, https://doi.org/10.5194/acp-20-4999-2020, https://doi.org/10.5194/acp-20-4999-2020, 2020
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We analyze the relationship between winter air stagnation and pollution extremes over eastern China and preceding Arctic sea ice loss based on climate modeling and dynamic diagnoses. We find significant increases in both the probability and intensity of air stagnation extremes in the modeling result driven by regional sea ice and sea surface temperature changes over the Pacific sector of the Arctic. We reveal the considerable impact of the Arctic climate change on mid-latitude weather extremes.
Qiuyan Du, Chun Zhao, Mingshuai Zhang, Xue Dong, Yu Chen, Zhen Liu, Zhiyuan Hu, Qiang Zhang, Yubin Li, Renmin Yuan, and Shiguang Miao
Atmos. Chem. Phys., 20, 2839–2863, https://doi.org/10.5194/acp-20-2839-2020, https://doi.org/10.5194/acp-20-2839-2020, 2020
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Simulated diurnal PM2.5 with WRF-Chem is primarily controlled by planetary boundary layer (PBL) mixing and emission variations. Modeling bias is likely primarily due to inefficient PBL mixing of primary PM2.5 during the night. The increase in PBL mixing strength during the night can significantly reduce biases. This study underscores that more effort is needed to improve the boundary mixing processes of pollutants in models with observations of PBL structure and mixing fluxes besides PBL height.
Yang Yang, Sijia Lou, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 20, 2579–2590, https://doi.org/10.5194/acp-20-2579-2020, https://doi.org/10.5194/acp-20-2579-2020, 2020
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Aerosol concentration decreased in Europe during 1980–2018, of which 7 % was induced by the changes in non-European emissions. Aerosols transported from other source regions are increasingly important to air quality in Europe. Contributions to the sulfate radiative forcing over Europe from both European and non-European emissions should decrease at a comparable rate in the next three decades. Future changes in non-European emissions are important in causing regional climate change in Europe.
Zhiyuan Hu, Jianping Huang, Chun Zhao, Qinjian Jin, Yuanyuan Ma, and Ben Yang
Atmos. Chem. Phys., 20, 1507–1529, https://doi.org/10.5194/acp-20-1507-2020, https://doi.org/10.5194/acp-20-1507-2020, 2020
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This study investigates intercontinental transport of dust plums and distribution characteristics of dust at different altitudes over the Tibetan Plateau (TP). The results show that dust particles are emitted into atmosphere and then transport to the TP. The East Asian dust trasnports southward and is lifted up to the TP in northern slop, while the North Afican dust and Middle East dust transport eastward and concentrate in both northern and southern slops, then is lifted up to the TP.
Hailong Wang, Jeremy G. Fyke, Jan T. M. Lenaerts, Jesse M. Nusbaumer, Hansi Singh, David Noone, Philip J. Rasch, and Rudong Zhang
The Cryosphere, 14, 429–444, https://doi.org/10.5194/tc-14-429-2020, https://doi.org/10.5194/tc-14-429-2020, 2020
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Using a climate model with unique water source tagging, we found that sea-ice anomalies in the Southern Ocean and accompanying SST changes have a significant influence on Antarctic precipitation and its source attribution through their direct impact on moisture sources and indirect impact on moisture transport. This study also highlights the importance of atmospheric dynamics in affecting the thermodynamic impact of sea-ice anomalies on regional Antarctic precipitation.
Joseph M. Cook, Andrew J. Tedstone, Christopher Williamson, Jenine McCutcheon, Andrew J. Hodson, Archana Dayal, McKenzie Skiles, Stefan Hofer, Robert Bryant, Owen McAree, Andrew McGonigle, Jonathan Ryan, Alexandre M. Anesio, Tristram D. L. Irvine-Fynn, Alun Hubbard, Edward Hanna, Mark Flanner, Sathish Mayanna, Liane G. Benning, Dirk van As, Marian Yallop, James B. McQuaid, Thomas Gribbin, and Martyn Tranter
The Cryosphere, 14, 309–330, https://doi.org/10.5194/tc-14-309-2020, https://doi.org/10.5194/tc-14-309-2020, 2020
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Melting of the Greenland Ice Sheet (GrIS) is a major source of uncertainty for sea level rise projections. Ice-darkening due to the growth of algae has been recognized as a potential accelerator of melting. This paper measures and models the algae-driven ice melting and maps the algae over the ice sheet for the first time. We estimate that as much as 13 % total runoff from the south-western GrIS can be attributed to these algae, showing that they must be included in future mass balance models.
Yufei Zou, Yuhang Wang, Yun Qian, Hanqin Tian, Jia Yang, and Ernesto Alvarado
Atmos. Chem. Phys., 20, 995–1020, https://doi.org/10.5194/acp-20-995-2020, https://doi.org/10.5194/acp-20-995-2020, 2020
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Fire is a natural phenomenon that has a long history of interactions with the environment and human activity. The complex interactions were less represented in previous fire and climate models. Here we use a new global fire model with improved modeling capability to study how fire responds and contributes to climate change. The modeling results show increased global fire activity in the future driven by climate change, which in turn modulates local and remote climate and ecosystems.
Adeyemi A. Adebiyi, Jasper F. Kok, Yang Wang, Akinori Ito, David A. Ridley, Pierre Nabat, and Chun Zhao
Atmos. Chem. Phys., 20, 829–863, https://doi.org/10.5194/acp-20-829-2020, https://doi.org/10.5194/acp-20-829-2020, 2020
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Although atmospheric dust particles produce significant impacts on the Earth system, most climate models still have difficulty representing the basic processes that affect these particles. In this study, we present new constraints on dust properties that consistently outperform the conventional climate models, when compared to independent measurements. As a result, our constraints can be used to improve climate models or serve as an alternative in constraining dust impacts on the Earth system.
Edward Gryspeerdt, Johannes Mülmenstädt, Andrew Gettelman, Florent F. Malavelle, Hugh Morrison, David Neubauer, Daniel G. Partridge, Philip Stier, Toshihiko Takemura, Hailong Wang, Minghuai Wang, and Kai Zhang
Atmos. Chem. Phys., 20, 613–623, https://doi.org/10.5194/acp-20-613-2020, https://doi.org/10.5194/acp-20-613-2020, 2020
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Aerosol radiative forcing is a key uncertainty in our understanding of the human forcing of the climate, with much of this uncertainty coming from aerosol impacts on clouds. Observation-based estimates of the radiative forcing are typically smaller than those from global models, but it is not clear if they are more reliable. This work shows how the forcing components in global climate models can be identified, highlighting similarities between the two methods and areas for future investigation.
Zhen Liu, Yi Ming, Chun Zhao, Ngar Cheung Lau, Jianping Guo, Massimo Bollasina, and Steve Hung Lam Yim
Atmos. Chem. Phys., 20, 223–241, https://doi.org/10.5194/acp-20-223-2020, https://doi.org/10.5194/acp-20-223-2020, 2020
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OH and HO2 radicals are important trace constituents of the atmosphere that are closely coupled via several types of reaction. This paper describes a new laboratory method to simultaneously determine OH kinetics and HO2 yields from chemical processes. The instrument also provides some time resolution on HO2 detection allowing one to separate HO2 produced from the target reaction from HO2 arising from secondary chemistry. Examples of applications are presented.
Fei Liu, Bryan N. Duncan, Nickolay A. Krotkov, Lok N. Lamsal, Steffen Beirle, Debora Griffin, Chris A. McLinden, Daniel L. Goldberg, and Zifeng Lu
Atmos. Chem. Phys., 20, 99–116, https://doi.org/10.5194/acp-20-99-2020, https://doi.org/10.5194/acp-20-99-2020, 2020
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We present a novel method to infer CO2 emissions from individual power plants, based on satellite observations of co-emitted NO2. We find that the CO2 emissions estimated by our satellite-based method during 2005–2017 are in reasonable agreement with the CEMS measurements for US power plants. The broader implication of our methodology is that it has the potential to provide an additional constraint on CO2 emissions from power plants in regions of the world without reliable emissions accounting.
Hongbin Yu, Yang Yang, Hailong Wang, Qian Tan, Mian Chin, Robert C. Levy, Lorraine A. Remer, Steven J. Smith, Tianle Yuan, and Yingxi Shi
Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, https://doi.org/10.5194/acp-20-139-2020, 2020
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Emissions and long-range transport of mineral dust and
combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on interannual variability and possible trends in combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017).
Zhiyuan Hu, Jianping Huang, Chun Zhao, Yuanyuan Ma, Qinjian Jin, Yun Qian, L. Ruby Leung, Jianrong Bi, and Jianmin Ma
Atmos. Chem. Phys., 19, 12709–12730, https://doi.org/10.5194/acp-19-12709-2019, https://doi.org/10.5194/acp-19-12709-2019, 2019
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This study investigates aerosol chemical compositions and relative contributions to total aerosols in the western US. The results show that trans-Pacific aerosols have a maximum concentration in the boreal spring, with the greatest contribution from dust. Over western North America, the trans-Pacific aerosols dominate the column-integrated aerosol mass and number concentration. However, near the surface, aerosols mainly originated from local emissions.
Mingchen Ma, Yang Gao, Yuhang Wang, Shaoqing Zhang, L. Ruby Leung, Cheng Liu, Shuxiao Wang, Bin Zhao, Xing Chang, Hang Su, Tianqi Zhang, Lifang Sheng, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 19, 12195–12207, https://doi.org/10.5194/acp-19-12195-2019, https://doi.org/10.5194/acp-19-12195-2019, 2019
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Ozone pollution has become severe in China, and extremely high ozone episodes occurred in summer 2017 over the North China Plain. While meteorology impacts are clear, we find that enhanced biogenic emissions, previously ignored by the community, driven by high vapor pressure deficit, land cover change and urban landscape contribute substantially to ozone formation. This study has significant implications for ozone pollution control with more frequent heat waves and urbanization growth in future.
Stefan Rahimi, Xiaohong Liu, Chenglai Wu, William K. Lau, Hunter Brown, Mingxuan Wu, and Yun Qian
Atmos. Chem. Phys., 19, 12025–12049, https://doi.org/10.5194/acp-19-12025-2019, https://doi.org/10.5194/acp-19-12025-2019, 2019
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Light-absorbing particles impact the Earth system in a variety of ways. They can warm the atmosphere by their very presence, or they can warm the atmosphere after they deposit on snow, warm it, and warm the overlying atmosphere. This paper focuses on these two processes as they pertain to black carbon and dust's impacts on the South Asian monsoon. It will be shown that these two aerosols have a significant effect on the monsoon.
Cheng Dang, Charles S. Zender, and Mark G. Flanner
The Cryosphere, 13, 2325–2343, https://doi.org/10.5194/tc-13-2325-2019, https://doi.org/10.5194/tc-13-2325-2019, 2019
George S. Fanourgakis, Maria Kanakidou, Athanasios Nenes, Susanne E. Bauer, Tommi Bergman, Ken S. Carslaw, Alf Grini, Douglas S. Hamilton, Jill S. Johnson, Vlassis A. Karydis, Alf Kirkevåg, John K. Kodros, Ulrike Lohmann, Gan Luo, Risto Makkonen, Hitoshi Matsui, David Neubauer, Jeffrey R. Pierce, Julia Schmale, Philip Stier, Kostas Tsigaridis, Twan van Noije, Hailong Wang, Duncan Watson-Parris, Daniel M. Westervelt, Yang Yang, Masaru Yoshioka, Nikos Daskalakis, Stefano Decesari, Martin Gysel-Beer, Nikos Kalivitis, Xiaohong Liu, Natalie M. Mahowald, Stelios Myriokefalitakis, Roland Schrödner, Maria Sfakianaki, Alexandra P. Tsimpidi, Mingxuan Wu, and Fangqun Yu
Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
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Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).
Chun Zhao, Mingyue Xu, Yu Wang, Meixin Zhang, Jianping Guo, Zhiyuan Hu, L. Ruby Leung, Michael Duda, and William Skamarock
Geosci. Model Dev., 12, 2707–2726, https://doi.org/10.5194/gmd-12-2707-2019, https://doi.org/10.5194/gmd-12-2707-2019, 2019
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Simulations at global uniform and variable resolutions share similar characteristics of precipitation and wind in the refined region. The experiments reveal the significant impacts of resolution on simulating the distribution and intensity of precipitation and updrafts. This study provides evidence supporting the use of convection-permitting global variable-resolution simulations to study extreme precipitation.
Adam Schneider, Mark Flanner, Roger De Roo, and Alden Adolph
The Cryosphere, 13, 1753–1766, https://doi.org/10.5194/tc-13-1753-2019, https://doi.org/10.5194/tc-13-1753-2019, 2019
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To study the process of snow aging, we engineered a prototype instrument called the Near-Infrared Emitting and Reflectance-Monitoring Dome (NERD). Using the NERD, we observed rapid snow aging in experiments with added light absorbing particles (LAPs). Particulate matter deposited on the snow increased absorption of solar energy and enhanced snow melt. These results indicate the role of LAPs' indirect effect on snow aging through a positive feedback mechanism related to the snow grain size.
Chandan Sarangi, Yun Qian, Karl Rittger, Kathryn J. Bormann, Ying Liu, Hailong Wang, Hui Wan, Guangxing Lin, and Thomas H. Painter
Atmos. Chem. Phys., 19, 7105–7128, https://doi.org/10.5194/acp-19-7105-2019, https://doi.org/10.5194/acp-19-7105-2019, 2019
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Radiative forcing induced by deposition of light-absorbing particles (LAPs) on snow is an important surface forcing. Here, we have used high-resolution WRF-Chem (coupled with online snow–LAP–radiation model) simulations for 2013–2014 to estimate the spatial variation in LAP-induced snow albedo darkening effect in high-mountain Asia. Significant improvement in simulated LAP–snow properties with use of a higher spatial resolution for the same model configuration is illustrated over this region.
Min Chen, Chris R. Vernon, Maoyi Huang, Katherine V. Calvin, and Ian P. Kraucunas
Geosci. Model Dev., 12, 1753–1764, https://doi.org/10.5194/gmd-12-1753-2019, https://doi.org/10.5194/gmd-12-1753-2019, 2019
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Demeter is a community spatial downscaling model that disaggregates land use and land cover changes projected by integrated human–Earth system models. However, Demeter has not been intensively calibrated, and we still lack good knowledge about its sensitivity to key parameters and parameter uncertainties. This paper aims to solve this problem.
Xiaoyue Liu, Jianping Huang, Jiping Huang, Changyu Li, and Lei Ding
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2019-36, https://doi.org/10.5194/essd-2019-36, 2019
Revised manuscript not accepted
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Atmospheric oxygen is crucial to life on earth. In this paper, we quantify oxygen consumption and production processes under the impact of human activities to build a dynamic global oxygen budget on a grid scale. Our result shows that the oxygen consumption related to human activities has risen significantly in recent decades while the oxygen production only displays a faint increase. Regionally, boreal forest and Tibetan plateau become the most important sources of atmospheric oxygen.
Yang Yang, Steven J. Smith, Hailong Wang, Catrin M. Mills, and Philip J. Rasch
Atmos. Chem. Phys., 19, 2405–2420, https://doi.org/10.5194/acp-19-2405-2019, https://doi.org/10.5194/acp-19-2405-2019, 2019
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Black carbon (BC) particles exert a potentially large warming influence on the
Earth system. We evaluate regional climate responses, non-linearity, and short-term transient responses to BC emission perturbations. We found that climate responses do not scale linearity with emissions and BC impacts temperature much faster than greenhouse gas forcing. Removing present-day BC emissions results in discernible surface temperature changes for only limited regions of the globe.
Daniel L. Goldberg, Pablo E. Saide, Lok N. Lamsal, Benjamin de Foy, Zifeng Lu, Jung-Hun Woo, Younha Kim, Jinseok Kim, Meng Gao, Gregory Carmichael, and David G. Streets
Atmos. Chem. Phys., 19, 1801–1818, https://doi.org/10.5194/acp-19-1801-2019, https://doi.org/10.5194/acp-19-1801-2019, 2019
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Using satellite data, we are able to estimate the emissions of NOx (NOx=NO+NO2), a toxic group of air pollutants, in the Seoul metropolitan area. We first develop an enhanced satellite product that better observes NO2 in urban regions. Using this new product, we derive NOx emissions to be twice as large as the emissions reported by the South Korean government. The implication is that the measures taken to reduce NOx emissions in South Korea have not been as effective as regulators have thought.
Junxi Zhang, Yang Gao, L. Ruby Leung, Kun Luo, Huan Liu, Jean-Francois Lamarque, Jianren Fan, Xiaohong Yao, Huiwang Gao, and Tatsuya Nagashima
Atmos. Chem. Phys., 19, 887–900, https://doi.org/10.5194/acp-19-887-2019, https://doi.org/10.5194/acp-19-887-2019, 2019
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ACCMIP simulations were used to study NOy deposition over East Asia in the future. Both dry and wet NOy deposition show significant decreases in the 2100s under RCP4.5 and RCP8.5 due to large anthropogenic emission reduction. The changes in climate only significantly affect the wet deposition primarily linked to changes in precipitation. Over the coastal seas of China, weaker transport of NOy from land due to emission reduction infers a larger impact from shipping and lightning emissions.
Ge Zhang, Yang Gao, Wenju Cai, L. Ruby Leung, Shuxiao Wang, Bin Zhao, Minghuai Wang, Huayao Shan, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 19, 565–576, https://doi.org/10.5194/acp-19-565-2019, https://doi.org/10.5194/acp-19-565-2019, 2019
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Based on observed data, this study reveals a distinct seesaw feature of abnormally high and low PM2.5 concentrations in December 2015 and January 2016 over North China. The mechanism of the seesaw pattern was found to be linked to a super El Niño and the Arctic Oscillation (AO). During the mature phase of El Niño in December 2015, the weakened East Asian winter monsoon favors strong haze formation; however, the circulation pattern was reversed in the next month due to the phase change of the AO.
Jiali Qiu, Qichun Yang, Xuesong Zhang, Maoyi Huang, Jennifer C. Adam, and Keyvan Malek
Hydrol. Earth Syst. Sci., 23, 35–49, https://doi.org/10.5194/hess-23-35-2019, https://doi.org/10.5194/hess-23-35-2019, 2019
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Complex water management activities challenge hydrologic modeling. We evaluated how different representations of reservoir operation and agricultural irrigation affect streamflow simulations in the Yakima River basin. Results highlight the importance of the inclusion of reliable reservoir and irrigation information in watershed models for improving watershed hydrology modeling. Models used here are public and hold the promise to benefit water assessment and management in other basins.
Anna Possner, Hailong Wang, Robert Wood, Ken Caldeira, and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 17475–17488, https://doi.org/10.5194/acp-18-17475-2018, https://doi.org/10.5194/acp-18-17475-2018, 2018
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We quantify aerosol–cloud radiative interactions in a regime of deep open-cell stratocumuli (boundary layer depth 1.5 km), a regime which remains largely unexplored within this context and yet is more dominant than cases of shallow stratocumuli previously studied. We simulate substantial increases in albedo in a regime where ship tracks are not found and argue that such changes may escape detection and attribution through remote sensing due to the large natural variability in the system.
Gerhard Krinner, Chris Derksen, Richard Essery, Mark Flanner, Stefan Hagemann, Martyn Clark, Alex Hall, Helmut Rott, Claire Brutel-Vuilmet, Hyungjun Kim, Cécile B. Ménard, Lawrence Mudryk, Chad Thackeray, Libo Wang, Gabriele Arduini, Gianpaolo Balsamo, Paul Bartlett, Julia Boike, Aaron Boone, Frédérique Chéruy, Jeanne Colin, Matthias Cuntz, Yongjiu Dai, Bertrand Decharme, Jeff Derry, Agnès Ducharne, Emanuel Dutra, Xing Fang, Charles Fierz, Josephine Ghattas, Yeugeniy Gusev, Vanessa Haverd, Anna Kontu, Matthieu Lafaysse, Rachel Law, Dave Lawrence, Weiping Li, Thomas Marke, Danny Marks, Martin Ménégoz, Olga Nasonova, Tomoko Nitta, Masashi Niwano, John Pomeroy, Mark S. Raleigh, Gerd Schaedler, Vladimir Semenov, Tanya G. Smirnova, Tobias Stacke, Ulrich Strasser, Sean Svenson, Dmitry Turkov, Tao Wang, Nander Wever, Hua Yuan, Wenyan Zhou, and Dan Zhu
Geosci. Model Dev., 11, 5027–5049, https://doi.org/10.5194/gmd-11-5027-2018, https://doi.org/10.5194/gmd-11-5027-2018, 2018
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This paper provides an overview of a coordinated international experiment to determine the strengths and weaknesses in how climate models treat snow. The models will be assessed at point locations using high-quality reference measurements and globally using satellite-derived datasets. How well climate models simulate snow-related processes is important because changing snow cover is an important part of the global climate system and provides an important freshwater resource for human use.
Jiahui Zhang, Dao-Yi Gong, Rui Mao, Jing Yang, Ziyin Zhang, and Yun Qian
Atmos. Chem. Phys., 18, 16775–16791, https://doi.org/10.5194/acp-18-16775-2018, https://doi.org/10.5194/acp-18-16775-2018, 2018
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The Chinese Spring Festival (also known as the Chinese New Year or Lunar New Year) is the most important festival in China. This paper reports that during the Chinese Spring Festival, the precipitation over southern China has been significantly reduced. The precipitation reduction is due to anomalous northerly winds. We suppose that anomalous atmospheric circulation is likely related to the human activity during holidays. It is an interesting phenomenon.
Yang Li and Mark G. Flanner
Atmos. Chem. Phys., 18, 16005–16018, https://doi.org/10.5194/acp-18-16005-2018, https://doi.org/10.5194/acp-18-16005-2018, 2018
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Light-absorbing impurities enhance snowmelt by boosting the absorption of solar energy. It is therefore important for coupled aerosol–climate and ice sheet models to include this effect, and yet most do not. We conduct several thousand simulations and develop a kernel and linear equations relating melt runoff on the Greenland Ice Sheet to the timing and amount of black carbon within precipitation and dry deposition, which can be used to extend the utility of state-of-the-art aerosol models.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Cenlin He, Mark G. Flanner, Fei Chen, Michael Barlage, Kuo-Nan Liou, Shichang Kang, Jing Ming, and Yun Qian
Atmos. Chem. Phys., 18, 11507–11527, https://doi.org/10.5194/acp-18-11507-2018, https://doi.org/10.5194/acp-18-11507-2018, 2018
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Snow albedo plays a key role in the Earth and climate system. It can be affected by impurities and snow properties. This study implements new parameterizations into a widely used snow model to account for effects of snow shape and black carbon–snow mixing state on snow albedo reduction in the Tibetan Plateau. This study points toward an imperative need for extensive measurements and improved model characterization of snow grain shape and aerosol–snow mixing state in Tibet and elsewhere.
Junxi Zhang, Yang Gao, Kun Luo, L. Ruby Leung, Yang Zhang, Kai Wang, and Jianren Fan
Atmos. Chem. Phys., 18, 9861–9877, https://doi.org/10.5194/acp-18-9861-2018, https://doi.org/10.5194/acp-18-9861-2018, 2018
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We used a regional model to investigate the impact of atmosphere with high temperature and low wind speed on ozone concentration. When these compound events (heat waves and stagnant weather) occur simultaneously, a striking ozone enhancement is revealed. This type of compound event is projected to increase more dominantly compared to single events in the future over the US, Europe, and China, implying the importance of reducing emissions in order to alleviate the impact from the compound events.
Christine A. Shields, Jonathan J. Rutz, Lai-Yung Leung, F. Martin Ralph, Michael Wehner, Brian Kawzenuk, Juan M. Lora, Elizabeth McClenny, Tashiana Osborne, Ashley E. Payne, Paul Ullrich, Alexander Gershunov, Naomi Goldenson, Bin Guan, Yun Qian, Alexandre M. Ramos, Chandan Sarangi, Scott Sellars, Irina Gorodetskaya, Karthik Kashinath, Vitaliy Kurlin, Kelly Mahoney, Grzegorz Muszynski, Roger Pierce, Aneesh C. Subramanian, Ricardo Tome, Duane Waliser, Daniel Walton, Gary Wick, Anna Wilson, David Lavers, Prabhat, Allison Collow, Harinarayan Krishnan, Gudrun Magnusdottir, and Phu Nguyen
Geosci. Model Dev., 11, 2455–2474, https://doi.org/10.5194/gmd-11-2455-2018, https://doi.org/10.5194/gmd-11-2455-2018, 2018
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ARTMIP (Atmospheric River Tracking Method Intercomparison Project) is a community effort with the explicit goal of understanding the uncertainties, and the implications of those uncertainties, in atmospheric river science solely due to detection algorithm. ARTMIP strives to quantify these differences and provide guidance on appropriate algorithmic choices for the science question posed. Project goals, experimental design, and preliminary results are provided.
Kai Zhang, Philip J. Rasch, Mark A. Taylor, Hui Wan, Ruby Leung, Po-Lun Ma, Jean-Christophe Golaz, Jon Wolfe, Wuyin Lin, Balwinder Singh, Susannah Burrows, Jin-Ho Yoon, Hailong Wang, Yun Qian, Qi Tang, Peter Caldwell, and Shaocheng Xie
Geosci. Model Dev., 11, 1971–1988, https://doi.org/10.5194/gmd-11-1971-2018, https://doi.org/10.5194/gmd-11-1971-2018, 2018
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The conservation of total water is an important numerical feature for global Earth system models. Even small conservation problems in the water budget can lead to systematic errors in century-long simulations for sea level rise projection. This study quantifies and reduces various sources of water conservation error in the atmosphere component of the Energy Exascale Earth System Model.
Kai Tang, Zhongwei Huang, Jianping Huang, Teruya Maki, Shuang Zhang, Atsushi Shimizu, Xiaojun Ma, Jinsen Shi, Jianrong Bi, Tian Zhou, Guoyin Wang, and Lei Zhang
Atmos. Chem. Phys., 18, 7131–7148, https://doi.org/10.5194/acp-18-7131-2018, https://doi.org/10.5194/acp-18-7131-2018, 2018
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To our knowledge, this is the first simultaneous field measurement of bioaerosols in dust events at four sites along the transport pathway of Asian dust. The samples were analyzed by means of fluorescence microscopy, scanning electron microscopy, and MiSeq sequencing analysis. The results indicate that dust clouds can carry many bacteria of various types into downwind regions, the alpha and beta diversity of which were investigated.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
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Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
Pieternel F. Levelt, Joanna Joiner, Johanna Tamminen, J. Pepijn Veefkind, Pawan K. Bhartia, Deborah C. Stein Zweers, Bryan N. Duncan, David G. Streets, Henk Eskes, Ronald van der A, Chris McLinden, Vitali Fioletov, Simon Carn, Jos de Laat, Matthew DeLand, Sergey Marchenko, Richard McPeters, Jerald Ziemke, Dejian Fu, Xiong Liu, Kenneth Pickering, Arnoud Apituley, Gonzalo González Abad, Antti Arola, Folkert Boersma, Christopher Chan Miller, Kelly Chance, Martin de Graaf, Janne Hakkarainen, Seppo Hassinen, Iolanda Ialongo, Quintus Kleipool, Nickolay Krotkov, Can Li, Lok Lamsal, Paul Newman, Caroline Nowlan, Raid Suleiman, Lieuwe Gijsbert Tilstra, Omar Torres, Huiqun Wang, and Krzysztof Wargan
Atmos. Chem. Phys., 18, 5699–5745, https://doi.org/10.5194/acp-18-5699-2018, https://doi.org/10.5194/acp-18-5699-2018, 2018
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The aim of this paper is to highlight the many successes of the Ozone Monitoring Instrument (OMI) spanning more than 13 years. Data from OMI have been used in a wide range of applications. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. OMI data continue to be used for new research and applications.
Longtao Wu, Yu Gu, Jonathan H. Jiang, Hui Su, Nanpeng Yu, Chun Zhao, Yun Qian, Bin Zhao, Kuo-Nan Liou, and Yong-Sang Choi
Atmos. Chem. Phys., 18, 5529–5547, https://doi.org/10.5194/acp-18-5529-2018, https://doi.org/10.5194/acp-18-5529-2018, 2018
Rachel M. Hoesly, Steven J. Smith, Leyang Feng, Zbigniew Klimont, Greet Janssens-Maenhout, Tyler Pitkanen, Jonathan J. Seibert, Linh Vu, Robert J. Andres, Ryan M. Bolt, Tami C. Bond, Laura Dawidowski, Nazar Kholod, June-ichi Kurokawa, Meng Li, Liang Liu, Zifeng Lu, Maria Cecilia P. Moura, Patrick R. O'Rourke, and Qiang Zhang
Geosci. Model Dev., 11, 369–408, https://doi.org/10.5194/gmd-11-369-2018, https://doi.org/10.5194/gmd-11-369-2018, 2018
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Historical emission trends are key inputs to Earth systems and atmospheric chemistry models. We present a new data set of historical (1750–2014) anthropogenic gases (CO, CH4, NH3, NOx, SO2, NMVOCs, BC, OC, and CO2) developed with the Community Emissions Data System (CEDS). This improves on existing inventories as it uses consistent methods and data across emissions species, has annual resolution for a longer and more recent time series, and is designed to be transparent and reproducible.
Qianqian Zhou, Guoyong Leng, and Maoyi Huang
Hydrol. Earth Syst. Sci., 22, 305–316, https://doi.org/10.5194/hess-22-305-2018, https://doi.org/10.5194/hess-22-305-2018, 2018
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Our results showed that adaptations through designing and updating urban drainage systems are effective in coping with urban flood risk under climate change. In the case study region, the magnitude of urban flood risk reduction through adaptations is more than double that by climate mitigations. We emphasize the importance of accounting for both global-scale climate mitigation and local-scale adaptations in assessing future urban flood risks in a consistent frame.
Yawen Liu, Kai Zhang, Yun Qian, Yuhang Wang, Yufei Zou, Yongjia Song, Hui Wan, Xiaohong Liu, and Xiu-Qun Yang
Atmos. Chem. Phys., 18, 31–47, https://doi.org/10.5194/acp-18-31-2018, https://doi.org/10.5194/acp-18-31-2018, 2018
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Fire aerosols have large impact on weather and climate through their effect on clouds and radiation, but it is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the nudged hindcast ensemble simulations from global aerosol-climate model. Results show large effects of fire aerosols on both liquid and ice cloud and large ensemble spread of regional mean shortwave cloud radiative forcing over southern Mexico and the central US.
Zhijuan Zhang, Bin Chen, Jianping Huang, Jingjing Liu, Jianrong Bi, Tian Zhou, and Zhongwei Huang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-1000, https://doi.org/10.5194/acp-2017-1000, 2017
Revised manuscript not accepted
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Environmental problems caused by aerosols such as dust aerosols are influencing people's lives and work. Due to different radiative effects of different types of aerosols, detection of the aerosol type is vital for improving our air quality. In this study, the optical properties of pure dust and transported anthropogenic dust are compared by using ground-based Lidar data. Based on our conclusion, detection of different dust aerosols will be more accurate using satellite-based Lidar.
Gautam Bisht, Maoyi Huang, Tian Zhou, Xingyuan Chen, Heng Dai, Glenn E. Hammond, William J. Riley, Janelle L. Downs, Ying Liu, and John M. Zachara
Geosci. Model Dev., 10, 4539–4562, https://doi.org/10.5194/gmd-10-4539-2017, https://doi.org/10.5194/gmd-10-4539-2017, 2017
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A fully coupled three-dimensional surface and subsurface land model, CP v1.0, was developed to simulate three-way interactions among river water, groundwater, and land surface processes. The coupled model can be used for improving mechanistic understanding of ecosystem functioning and biogeochemical cycling along river corridors under historical and future hydroclimatic changes. The dataset presented in this study can also serve as a good benchmarking case for testing other integrated models.
Siyu Chen, Jianping Huang, Nanxuan Jiang, Zhou Zang, Xiaodan Guan, Xiaojun Ma, Zhuo Jia, Xiaorui Zhang, Yanting Zhang, Kangning Huang, Xiaocong Xu, Guolong Zhang, Jiming Li, Ran Yang, and Shujie Liao
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-890, https://doi.org/10.5194/acp-2017-890, 2017
Revised manuscript not accepted
Joseph M. Cook, Andrew J. Hodson, Alex S. Gardner, Mark Flanner, Andrew J. Tedstone, Christopher Williamson, Tristram D. L. Irvine-Fynn, Johan Nilsson, Robert Bryant, and Martyn Tranter
The Cryosphere, 11, 2611–2632, https://doi.org/10.5194/tc-11-2611-2017, https://doi.org/10.5194/tc-11-2611-2017, 2017
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Biological growth darkens snow and ice, causing it to melt faster. This is often referred to as
bioalbedo. Quantifying bioalbedo has not been achieved because of difficulties in isolating the biological contribution from the optical properties of ice and snow, and from inorganic impurities in field studies. In this paper, we provide a physical model that enables bioalbedo to be quantified from first principles and we use it to guide future field studies.
Jeremy Fyke, Jan T. M. Lenaerts, and Hailong Wang
The Cryosphere, 11, 2595–2609, https://doi.org/10.5194/tc-11-2595-2017, https://doi.org/10.5194/tc-11-2595-2017, 2017
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In this CESM modeling study, we uncover regional relationships in snowfall across Antarctica that are corroborated by regional modeling and ice core records. These relationships are driven by variability in large-scale atmospheric moisture transport and dampen overall Antarctic snowfall variability, with implications for Antarctic-sourced sea level variability and detection of an emergent anthropogenic signal in Antarctic mass trends.
Daniel L. Goldberg, Lok N. Lamsal, Christopher P. Loughner, William H. Swartz, Zifeng Lu, and David G. Streets
Atmos. Chem. Phys., 17, 11403–11421, https://doi.org/10.5194/acp-17-11403-2017, https://doi.org/10.5194/acp-17-11403-2017, 2017
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We developed a new satellite NO2 product using a high spatial resolution (1.33 × 1.33 km) model simulation constrained by aircraft observations. The high-resolution satellite product is now able to observe the spatial heterogeneities of NO2 pollution over a large area with more clarity. The satellite is now in better agreement with monitors at ground level observing the same pollution.
Jinming Ge, Zeen Zhu, Chuang Zheng, Hailing Xie, Tian Zhou, Jianping Huang, and Qiang Fu
Atmos. Chem. Phys., 17, 9035–9047, https://doi.org/10.5194/acp-17-9035-2017, https://doi.org/10.5194/acp-17-9035-2017, 2017
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A modified method with a new noise reduction scheme that can reduce the noise distribution to a narrow range is proposed to distinguish clouds and other hydrometeors from noise and recognize more features with weak signal in cloud radar observations. It was found that our method has significant advantages in reducing the rates of both failed negative and false positive hydrometeor identifications in simulated clouds and recognizing clouds with weak signal from our cloud radar observations.
Randal D. Koster, Alan K. Betts, Paul A. Dirmeyer, Marc Bierkens, Katrina E. Bennett, Stephen J. Déry, Jason P. Evans, Rong Fu, Felipe Hernandez, L. Ruby Leung, Xu Liang, Muhammad Masood, Hubert Savenije, Guiling Wang, and Xing Yuan
Hydrol. Earth Syst. Sci., 21, 3777–3798, https://doi.org/10.5194/hess-21-3777-2017, https://doi.org/10.5194/hess-21-3777-2017, 2017
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Large-scale hydrological variability can affect society in profound ways; floods and droughts, for example, often cause major damage and hardship. A recent gathering of hydrologists at a symposium to honor the career of Professor Eric Wood motivates the present survey of recent research on this variability. The surveyed literature and the illustrative examples provided in the paper show that research into hydrological variability continues to be strong, vibrant, and multifaceted.
Yang Yang, Hailong Wang, Steven J. Smith, Richard Easter, Po-Lun Ma, Yun Qian, Hongbin Yu, Can Li, and Philip J. Rasch
Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, https://doi.org/10.5194/acp-17-8903-2017, 2017
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Sulfate has significant impacts on air quality and climate. Local sulfate pollution could result from remote influences, making domestic mitigation efforts inefficient. Using CESM with a sulfur source-tagging technique, we found that, over regions with relatively low emissions, sulfate concentrations are primarily attributed to non-local sources and sulfate indirect radiative forcing over the Southern Hemisphere is more sensitive to emission perturbation than the polluted Northern Hemisphere.
Jianrong Bi, Jianping Huang, Jinsen Shi, Zhiyuan Hu, Tian Zhou, Guolong Zhang, Zhongwei Huang, Xin Wang, and Hongchun Jin
Atmos. Chem. Phys., 17, 7775–7792, https://doi.org/10.5194/acp-17-7775-2017, https://doi.org/10.5194/acp-17-7775-2017, 2017
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We conducted a field campaign on exploring dust aerosol in Dunhuang farmland nearby Gobi deserts. The anthropogenic dust produced by agricultural cultivations exerted a significant superimposed effect on elevated dust loadings. Strong south wind in daytime scavenged the pollution and weak northeast wind at night favorably accumulated air pollutants near the surface. The local emissions remarkably modified the absorptive and optical characteristics of mineral dust in desert source region.
Ling Qi, Qinbin Li, Cenlin He, Xin Wang, and Jianping Huang
Atmos. Chem. Phys., 17, 7459–7479, https://doi.org/10.5194/acp-17-7459-2017, https://doi.org/10.5194/acp-17-7459-2017, 2017
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Black carbon (BC) is the second only to CO2 in heating the planet, but the simulation of BC is associated with large uncertainties. BC burden is largely underestimated over land and overestimated over ocean. Our study finds that a missing process in current Wegener–Bergeron–Findeisen models largely explains the discrepancy in BC simulation over land. We call for more observations of BC in mixed-phase clouds to understand this process and improve the simulation of global BC.
Longtao Wu, Hui Su, Olga V. Kalashnikova, Jonathan H. Jiang, Chun Zhao, Michael J. Garay, James R. Campbell, and Nanpeng Yu
Atmos. Chem. Phys., 17, 7291–7309, https://doi.org/10.5194/acp-17-7291-2017, https://doi.org/10.5194/acp-17-7291-2017, 2017
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The WRF-Chem simulation successfully captures aerosol variations in the cold season in the San Joaquin Valley (SJV) but has poor performance in the warm season. High-resolution model simulation can better resolve nonhomogeneous distribution of anthropogenic emissions in urban areas, resulting in better simulation of aerosols in the cold season in the SJV. Poor performance of the WRF-Chem model in the warm season in the SJV is mainly due to misrepresentation of dust emission and vertical mixing.
Shi Zhong, Yun Qian, Chun Zhao, Ruby Leung, Hailong Wang, Ben Yang, Jiwen Fan, Huiping Yan, Xiu-Qun Yang, and Dongqing Liu
Atmos. Chem. Phys., 17, 5439–5457, https://doi.org/10.5194/acp-17-5439-2017, https://doi.org/10.5194/acp-17-5439-2017, 2017
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An online climate–chemistry coupled model (WRF-Chem) is integrated for 5 years at cloud-permitting scale to quantify the impacts of urbanization-induced changes in land cover and pollutants emission on regional climate in the Yangtze River Delta region in eastern China. Urbanization over this region increases the frequency of extreme precipitation and heat wave in summer. The results could help China government in making policies in mitigating the environmental impact of urbanization.
Huan Yao, Yu Song, Mingxu Liu, Scott Archer-Nicholls, Douglas Lowe, Gordon McFiggans, Tingting Xu, Pin Du, Jianfeng Li, Yusheng Wu, Min Hu, Chun Zhao, and Tong Zhu
Atmos. Chem. Phys., 17, 5205–5219, https://doi.org/10.5194/acp-17-5205-2017, https://doi.org/10.5194/acp-17-5205-2017, 2017
Yang Yang, Hailong Wang, Steven J. Smith, Po-Lun Ma, and Philip J. Rasch
Atmos. Chem. Phys., 17, 4319–4336, https://doi.org/10.5194/acp-17-4319-2017, https://doi.org/10.5194/acp-17-4319-2017, 2017
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The source attributions of black carbon (BC) in China are quantified using the Community Earth System Model by source tagging. BC impacts neighboring regions greatly. Transport is important in increasing BC during regional polluted days. Emissions outside China contribute 35 % of BC direct radiative forcing in China. Efficiency analysis shows that reduction in BC emissions over eastern China could have a greater benefit for regional air quality in China, especially in the winter haze season.
Xiangyu Luo, Hong-Yi Li, L. Ruby Leung, Teklu K. Tesfa, Augusto Getirana, Fabrice Papa, and Laura L. Hess
Geosci. Model Dev., 10, 1233–1259, https://doi.org/10.5194/gmd-10-1233-2017, https://doi.org/10.5194/gmd-10-1233-2017, 2017
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This study shows that alleviating vegetation-caused biases in DEM data, refining channel cross-sectional geometry and Manning roughness coefficients, as well as accounting for backwater effects can effectively improve the modeling of streamflow, river stages and flood extent in the Amazon Basin. The obtained understanding could be helpful to hydrological modeling in basins with evident inundation, which has important implications for improving land–atmosphere interactions in Earth system models.
Teklu K. Tesfa and Lai-Yung Ruby Leung
Geosci. Model Dev., 10, 873–888, https://doi.org/10.5194/gmd-10-873-2017, https://doi.org/10.5194/gmd-10-873-2017, 2017
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Motivated by the significant topographic influence on land surface processes, this study explored two methods to discretize watersheds into two types of subgrid structures to capture spatial heterogeneity for land surface models. Adopting geomorphologic concepts in watershed discretization yields improved capability in capturing subgrid topographic heterogeneity, which also allowed climatic and land cover variability to be better represented with a nominal increase in computational requirements.
Gunnar Myhre, Wenche Aas, Ribu Cherian, William Collins, Greg Faluvegi, Mark Flanner, Piers Forster, Øivind Hodnebrog, Zbigniew Klimont, Marianne T. Lund, Johannes Mülmenstädt, Cathrine Lund Myhre, Dirk Olivié, Michael Prather, Johannes Quaas, Bjørn H. Samset, Jordan L. Schnell, Michael Schulz, Drew Shindell, Ragnhild B. Skeie, Toshihiko Takemura, and Svetlana Tsyro
Atmos. Chem. Phys., 17, 2709–2720, https://doi.org/10.5194/acp-17-2709-2017, https://doi.org/10.5194/acp-17-2709-2017, 2017
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Over the past decades, the geographical distribution of emissions of substances that alter the atmospheric energy balance has changed due to economic growth and pollution regulations. Here, we show the resulting changes to aerosol and ozone abundances and their radiative forcing using recently updated emission data for the period 1990–2015, as simulated by seven global atmospheric composition models. The global mean radiative forcing is more strongly positive than reported in IPCC AR5.
Ben Kravitz, Douglas G. MacMartin, Philip J. Rasch, and Hailong Wang
Atmos. Chem. Phys., 17, 2525–2541, https://doi.org/10.5194/acp-17-2525-2017, https://doi.org/10.5194/acp-17-2525-2017, 2017
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We introduce system identification techniques to climate science wherein multiple dynamic input–output relationships can be simultaneously characterized in a single simulation. This method, involving multiple small perturbations (in space and time) of an input field while monitoring output fields to quantify responses, allows for identification of different timescales of climate response to forcing without substantially pushing the climate far away from a steady state.
Siyu Chen, Jianping Huang, Litai Kang, Hao Wang, Xiaojun Ma, Yongli He, Tiangang Yuan, Ben Yang, Zhongwei Huang, and Guolong Zhang
Atmos. Chem. Phys., 17, 2401–2421, https://doi.org/10.5194/acp-17-2401-2017, https://doi.org/10.5194/acp-17-2401-2017, 2017
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Compared with the TD dust, the importance of the GD dust in eastern China, Japan, and Korea is always neglected. We focused primarily on the dynamic and thermodynamics mechanisms of dust emission and transport over TD and GD and further elucidate the influence of TD and GD dust on the entire East Asia based on a case study using WRF-Chem model in the study.
Jiwen Fan, L. Ruby Leung, Daniel Rosenfeld, and Paul J. DeMott
Atmos. Chem. Phys., 17, 1017–1035, https://doi.org/10.5194/acp-17-1017-2017, https://doi.org/10.5194/acp-17-1017-2017, 2017
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How orographic mixed-phase clouds respond to changes in cloud condensation nuclei (CCN) and ice nucleating particles (INPs) is highly uncertain. We conducted this study to improve understanding of these processes. We found a new mechanism through which CCN can invigorate orographic mixed-phase clouds and drastically intensify snow precipitation when CCN concentrations are high. Our findings have very important implications for orographic precipitation in polluted regions.
Meng Li, Qiang Zhang, Jun-ichi Kurokawa, Jung-Hun Woo, Kebin He, Zifeng Lu, Toshimasa Ohara, Yu Song, David G. Streets, Gregory R. Carmichael, Yafang Cheng, Chaopeng Hong, Hong Huo, Xujia Jiang, Sicong Kang, Fei Liu, Hang Su, and Bo Zheng
Atmos. Chem. Phys., 17, 935–963, https://doi.org/10.5194/acp-17-935-2017, https://doi.org/10.5194/acp-17-935-2017, 2017
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An anthropogenic emission inventory for Asia is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) projects by a mosaic of up-to-date regional emission inventories. The total Asian emissions in 2010 are estimated as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.5 Tg CO, 67.0 Tg NMVOC, 28.7 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2.
Jianrong Bi, Jianping Huang, Brent Holben, and Guolong Zhang
Atmos. Chem. Phys., 16, 15501–15516, https://doi.org/10.5194/acp-16-15501-2016, https://doi.org/10.5194/acp-16-15501-2016, 2016
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Dating absorptive capacity of Asian dust is still an outstanding issue. In this study, we identify two types of Asian dust: Pure Dust (PDU) and Transported Anthropogenic Dust (TDU). Overall average SSA, ASY, Re, and Ri at 550 nm for PDU are 0.935, 0.742, 1.526, and 0.00226, respectively, with 0.921, 0.723, 1.521, and 0.00364 for TDU. Our results promise to update and improve accuracy of Asian dust characteristics in present-day remote sensing applications and regional climate models.
David A. Ridley, Colette L. Heald, Jasper F. Kok, and Chun Zhao
Atmos. Chem. Phys., 16, 15097–15117, https://doi.org/10.5194/acp-16-15097-2016, https://doi.org/10.5194/acp-16-15097-2016, 2016
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Mineral dust aerosol affects climate through interaction with radiation and clouds, human health through contribution to particulate matter, and ecosystem health through nutrient transport and deposition. In this study, we use satellite and in situ retrievals to derive an observational estimate of the global dust AOD with which evaluate modeled dust AOD. Differences in the seasonality and regional distribution of dust AOD between observations and models are highlighted.
Yiquan Jiang, Zheng Lu, Xiaohong Liu, Yun Qian, Kai Zhang, Yuhang Wang, and Xiu-Qun Yang
Atmos. Chem. Phys., 16, 14805–14824, https://doi.org/10.5194/acp-16-14805-2016, https://doi.org/10.5194/acp-16-14805-2016, 2016
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Aerosols from open fires could significantly perturb the global radiation balance and induce climate change. In this study, the CAM5 global climate model is used to investigate the spatial and seasonal characteristics of radiative effects due to fire aerosol–radiation interactions, fire aerosol-cloud interactions and fire aerosol-surface albedo interactions, including radiative effects from all fire aerosols, fire black carbon and fire particulate organic matter.
Reindert J. Haarsma, Malcolm J. Roberts, Pier Luigi Vidale, Catherine A. Senior, Alessio Bellucci, Qing Bao, Ping Chang, Susanna Corti, Neven S. Fučkar, Virginie Guemas, Jost von Hardenberg, Wilco Hazeleger, Chihiro Kodama, Torben Koenigk, L. Ruby Leung, Jian Lu, Jing-Jia Luo, Jiafu Mao, Matthew S. Mizielinski, Ryo Mizuta, Paulo Nobre, Masaki Satoh, Enrico Scoccimarro, Tido Semmler, Justin Small, and Jin-Song von Storch
Geosci. Model Dev., 9, 4185–4208, https://doi.org/10.5194/gmd-9-4185-2016, https://doi.org/10.5194/gmd-9-4185-2016, 2016
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Recent progress in computing power has enabled climate models to simulate more processes in detail and on a smaller scale. Here we present a common protocol for these high-resolution runs that will foster the analysis and understanding of the impact of model resolution on the simulated climate. These runs will also serve as a more reliable source for assessing climate risks that are associated with small-scale weather phenomena such as tropical cyclones.
Tianjun Zhou, Andrew G. Turner, James L. Kinter, Bin Wang, Yun Qian, Xiaolong Chen, Bo Wu, Bin Wang, Bo Liu, Liwei Zou, and Bian He
Geosci. Model Dev., 9, 3589–3604, https://doi.org/10.5194/gmd-9-3589-2016, https://doi.org/10.5194/gmd-9-3589-2016, 2016
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This paper tells why to launch the Global Monsoons Model Inter-comparison Project (GMMIP) and how to achieve its scientific goals on monsoon variability. It addresses the scientific questions to be answered, describes three tiered experiments comprehensively and proposes a basic analysis framework to guide future research. It will help the monsoon research communities to understand the objectives of the GMMIP and the modelling groups involved in the GMMIP conduct the experiments successfully.
Meng Gao, Gregory R. Carmichael, Pablo E. Saide, Zifeng Lu, Man Yu, David G. Streets, and Zifa Wang
Atmos. Chem. Phys., 16, 11837–11851, https://doi.org/10.5194/acp-16-11837-2016, https://doi.org/10.5194/acp-16-11837-2016, 2016
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The WRF-Chem model was used to examine how the winter PM2.5 concentrations change in response to changes in emissions and meteorology in North China from 1960 to 2010. The discussions in this study indicate that dramatic changes in emissions are the main cause of increasing haze events in North China, and long-term trends in atmospheric circulations maybe another important cause. We also found aerosol feedbacks have been significantly enhanced from 1960 to 2010, due to higher aerosol loadings.
Bart van den Hurk, Hyungjun Kim, Gerhard Krinner, Sonia I. Seneviratne, Chris Derksen, Taikan Oki, Hervé Douville, Jeanne Colin, Agnès Ducharne, Frederique Cheruy, Nicholas Viovy, Michael J. Puma, Yoshihide Wada, Weiping Li, Binghao Jia, Andrea Alessandri, Dave M. Lawrence, Graham P. Weedon, Richard Ellis, Stefan Hagemann, Jiafu Mao, Mark G. Flanner, Matteo Zampieri, Stefano Materia, Rachel M. Law, and Justin Sheffield
Geosci. Model Dev., 9, 2809–2832, https://doi.org/10.5194/gmd-9-2809-2016, https://doi.org/10.5194/gmd-9-2809-2016, 2016
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This manuscript describes the setup of the CMIP6 project Land Surface, Snow and Soil Moisture Model Intercomparison Project (LS3MIP).
Jin Ming Ge, Huayue Liu, Jianping Huang, and Qiang Fu
Atmos. Chem. Phys., 16, 7773–7783, https://doi.org/10.5194/acp-16-7773-2016, https://doi.org/10.5194/acp-16-7773-2016, 2016
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Nocturnal low-level jet (NLLJ), which refers to a narrow zone of strong winds, occurs frequently over the Taklimakan Desert. It is found that the NLLJ contains more momentum than without NLLJ, and the downward momentum transfer process is more intense and rapid in the warm season. The coincidence of the larger surface winds during NLLJ days with an enhancement of aerosol optical depth indicates that the NLLJ is an important mechanism for dust emission and transport over this region.
Chun Zhao, Maoyi Huang, Jerome D. Fast, Larry K. Berg, Yun Qian, Alex Guenther, Dasa Gu, Manish Shrivastava, Ying Liu, Stacy Walters, Gabriele Pfister, Jiming Jin, John E. Shilling, and Carsten Warneke
Geosci. Model Dev., 9, 1959–1976, https://doi.org/10.5194/gmd-9-1959-2016, https://doi.org/10.5194/gmd-9-1959-2016, 2016
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In this study, the latest version of MEGAN is coupled within CLM4 in WRF-Chem. In this implementation, MEGAN shares a consistent vegetation map with CLM4. This improved modeling framework is used to investigate the impact of two land surface schemes on BVOCs and examine the sensitivity of BVOCs to vegetation distributions in California. This study indicates that more effort is needed to obtain the most appropriate and accurate land cover data sets for climate and air quality models.
Ben Kravitz, Douglas G. MacMartin, Hailong Wang, and Philip J. Rasch
Earth Syst. Dynam., 7, 469–497, https://doi.org/10.5194/esd-7-469-2016, https://doi.org/10.5194/esd-7-469-2016, 2016
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Most simulations of solar geoengineering prescribe a particular strategy and evaluate its modeled effects. Here we first choose example climate objectives and then design a strategy to meet those objectives in climate models. We show that certain objectives can be met simultaneously even in the presence of uncertainty, and the strategy for meeting those objectives can be ported to other models. This is part of a broader illustration of how uncertainties in solar geoengineering can be managed.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Cenlin He, Wee-Liang Lee, Xing Chang, Qinbin Li, Shuxiao Wang, Hsien-Liang R. Tseng, Lai-Yung R. Leung, and Jiming Hao
Atmos. Chem. Phys., 16, 5841–5852, https://doi.org/10.5194/acp-16-5841-2016, https://doi.org/10.5194/acp-16-5841-2016, 2016
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We examine the impact of buildings on surface solar fluxes in Beijing by accounting for their 3-D structures. We find that inclusion of buildings changes surface solar fluxes by within ±1 W m−2, ±1–10 W m−2, and up to ±100 W m−2 at grid resolutions of 4 km, 800 m, and 90 m, respectively. We can resolve pairs of positive-negative flux deviations on different sides of buildings at ≤ 800 m resolutions. We should treat building-effect on solar fluxes differently in models with different resolutions.
Zhiyuan Hu, Chun Zhao, Jianping Huang, L. Ruby Leung, Yun Qian, Hongbin Yu, Lei Huang, and Olga V. Kalashnikova
Geosci. Model Dev., 9, 1725–1746, https://doi.org/10.5194/gmd-9-1725-2016, https://doi.org/10.5194/gmd-9-1725-2016, 2016
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This study conducts the simulation of WRF-Chem with the quasi-global configuration for 2010–2014, and evaluates the simulation with multiple observation datasets for the first time. This study demonstrates that the WRF-Chem quasi-global simulation can be used for investigating trans-Pacific transport of aerosols and providing reasonable inflow chemical boundaries for the western USA to further understand the impact of transported pollutants on the regional air quality and climate.
Xiaodan Guan, Jianping Huang, Yanting Zhang, Yongkun Xie, and Jingjing Liu
Atmos. Chem. Phys., 16, 5159–5169, https://doi.org/10.5194/acp-16-5159-2016, https://doi.org/10.5194/acp-16-5159-2016, 2016
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An obvious peak in the total anthropogenic dust column, with much higher magnitude than those of wet regions, was observed in semi-arid regions. The anthropogenic dust column burden of semi-arid takes a positively correlated with the population and population change, indicating the production of anthropogenic dust in semi-arid regions is partly induced by human activities.
Nickolay A. Krotkov, Chris A. McLinden, Can Li, Lok N. Lamsal, Edward A. Celarier, Sergey V. Marchenko, William H. Swartz, Eric J. Bucsela, Joanna Joiner, Bryan N. Duncan, K. Folkert Boersma, J. Pepijn Veefkind, Pieternel F. Levelt, Vitali E. Fioletov, Russell R. Dickerson, Hao He, Zifeng Lu, and David G. Streets
Atmos. Chem. Phys., 16, 4605–4629, https://doi.org/10.5194/acp-16-4605-2016, https://doi.org/10.5194/acp-16-4605-2016, 2016
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We examine changes in SO2 and NO2 over the world's most polluted regions during the first decade of Aura OMI observations. Over the eastern US, both NO2 and SO2 levels decreased by 40 % and 80 %, respectively. OMI confirmed large reductions in SO2 over eastern Europe's largest coal power plants. The North China Plain has the world's most severe SO2 pollution, but a decreasing trend been observed since 2011, with a 50 % reduction in 2012–2014. India's SO2 and NO2 levels are growing at a fast pace.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Shipeng Zhang, Minghuai Wang, Steven J. Ghan, Aijun Ding, Hailong Wang, Kai Zhang, David Neubauer, Ulrike Lohmann, Sylvaine Ferrachat, Toshihiko Takeamura, Andrew Gettelman, Hugh Morrison, Yunha Lee, Drew T. Shindell, Daniel G. Partridge, Philip Stier, Zak Kipling, and Congbin Fu
Atmos. Chem. Phys., 16, 2765–2783, https://doi.org/10.5194/acp-16-2765-2016, https://doi.org/10.5194/acp-16-2765-2016, 2016
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The variation of aerosol indirect effects (AIE) in several climate models is investigated across different dynamical regimes. Regimes with strong large-scale ascent are shown to be as important as stratocumulus regimes in studying AIE. AIE over regions with high monthly large-scale surface precipitation rate contributes the most to the total aerosol indirect forcing. These results point to the need to reduce the uncertainty in AIE in different dynamical regimes.
Kai Zhang, Chun Zhao, Hui Wan, Yun Qian, Richard C. Easter, Steven J. Ghan, Koichi Sakaguchi, and Xiaohong Liu
Geosci. Model Dev., 9, 607–632, https://doi.org/10.5194/gmd-9-607-2016, https://doi.org/10.5194/gmd-9-607-2016, 2016
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A sub-grid treatment based on Weibull distribution is introduced to CAM5 to take into account the impact of unresolved variability of surface wind speed on sea salt and dust emissions. Simulations show that sub-grid wind variability has relatively small impacts on the global mean sea salt emissions, but considerable influence on dust emissions. Dry convective eddies and mesoscale flows associated with complex topography are the major causes of dust emission enhancement.
X. Liu, P.-L. Ma, H. Wang, S. Tilmes, B. Singh, R. C. Easter, S. J. Ghan, and P. J. Rasch
Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, https://doi.org/10.5194/gmd-9-505-2016, 2016
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In this study, we describe and evaluate a new four-mode version of the Modal Aerosol Module (MAM4) in the Community Atmosphere Model version 5 (CAM5). Compared to the current three-mode version of MAM in CAM5, MAM4 significantly improves the simulation of seasonal variation of BC concentrations in the polar regions, by increasing the BC concentrations in all seasons and particularly in cold seasons.
Y. Feng, V. R. Kotamarthi, R. Coulter, C. Zhao, and M. Cadeddu
Atmos. Chem. Phys., 16, 247–264, https://doi.org/10.5194/acp-16-247-2016, https://doi.org/10.5194/acp-16-247-2016, 2016
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Aerosol radiative effects are of great importance for climate studies over South Asia, such as the weakening of the South Asian monsoon in the 20th century. This study reveals the altitude dependence of commonly underestimated aerosol radiative properties over this region. It further demonstrates the importance of constraining aerosol vertical distributions and partitioning of scattering vs absorbing aerosols in simulating the subsequent regional dynamical and hydrological responses to aerosols.
X. Guan, J. Huang, R. Guo, H. Yu, P. Lin, and Y. Zhang
Atmos. Chem. Phys., 15, 13777–13786, https://doi.org/10.5194/acp-15-13777-2015, https://doi.org/10.5194/acp-15-13777-2015, 2015
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Dynamical adjustment methodology has been applied to the raw surface air temperature and has successfully identified and separated the contribution of dynamically induced temperature (DIT) and radiatively forced temperature (RFT). It found that regional anthropogenic radiative forcing caused the enhanced warming in the semi-arid region, which may be closely associated with local human activities.
R. Zhang, H. Wang, D. A. Hegg, Y. Qian, S. J. Doherty, C. Dang, P.-L. Ma, P. J. Rasch, and Q. Fu
Atmos. Chem. Phys., 15, 12805–12822, https://doi.org/10.5194/acp-15-12805-2015, https://doi.org/10.5194/acp-15-12805-2015, 2015
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We use a global climate model with an explicit source tagging technique to quantify contributions of emissions from various geographical regions and sectors to BC in North America. Model results are evaluated against measurements of near-surface and in-snow BC. We found strong spatial variations of BC and its radiative forcing that can be quantitatively attributed to the various source origins, and also identified a significant source of BC in snow that is likely missing in most climate models.
R. Gonzalez-Abraham, S. H. Chung, J. Avise, B. Lamb, E. P. Salathé Jr., C. G. Nolte, D. Loughlin, A. Guenther, C. Wiedinmyer, T. Duhl, Y. Zhang, and D. G. Streets
Atmos. Chem. Phys., 15, 12645–12665, https://doi.org/10.5194/acp-15-12645-2015, https://doi.org/10.5194/acp-15-12645-2015, 2015
Y. Liu, Y. Sato, R. Jia, Y. Xie, J. Huang, and T. Nakajima
Atmos. Chem. Phys., 15, 12581–12594, https://doi.org/10.5194/acp-15-12581-2015, https://doi.org/10.5194/acp-15-12581-2015, 2015
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We firstly evaluated the Spectral Radiation-Transport Model for Aerosol Species combined with a non-hydrostatic regional model through comparing the simulation results and satellite observations, both in horizontal and vertical. The dust and anthropogenic aerosols in summer over the Tibetan Plateau are evaluated, and their distributions over the TP are presented. The transport of these aerosols over the Tibetan Plateau is also explored via combining the simulation results and reanalysis data.
D. Singh, M. G. Flanner, and J. Perket
The Cryosphere, 9, 2057–2070, https://doi.org/10.5194/tc-9-2057-2015, https://doi.org/10.5194/tc-9-2057-2015, 2015
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Our work quantifies the effect of snow/ice cover on Earth's top-of-atmosphere solar energy budget. We used higher resolution MODIS data, combined with microwave retrievals of snow presence and radiative kernels produced from 4 different models for Cryosphere Radiative Effect (CrRE) estimation. We have estimated a global land-based CrRE of about -2.6Wm-2 during 2001-2013, with about 59% of the effect originating from Antarctica. We were also be able to resolve contribution from mountain glaciers.
C. He, K.-N. Liou, Y. Takano, R. Zhang, M. Levy Zamora, P. Yang, Q. Li, and L. R. Leung
Atmos. Chem. Phys., 15, 11967–11980, https://doi.org/10.5194/acp-15-11967-2015, https://doi.org/10.5194/acp-15-11967-2015, 2015
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
J. P. Huang, J. J. Liu, B. Chen, and S. L. Nasiri
Atmos. Chem. Phys., 15, 11653–11665, https://doi.org/10.5194/acp-15-11653-2015, https://doi.org/10.5194/acp-15-11653-2015, 2015
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To understand the contribution of anthropogenic dust to the total global dust load, a new technique for distinguishing anthropogenic dust from natural dust is proposed by using CALIPSO dust measurements and PBL height retrievals along with a land use data set. Results reveal that local anthropogenic dust aerosol accounts for about 25% of the global continental dust load.
Z. Lu, D. G. Streets, B. de Foy, L. N. Lamsal, B. N. Duncan, and J. Xing
Atmos. Chem. Phys., 15, 10367–10383, https://doi.org/10.5194/acp-15-10367-2015, https://doi.org/10.5194/acp-15-10367-2015, 2015
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Using an exponentially modified Gaussian method and taking into account the effect of wind on NO2 distributions, we estimate 3-year moving-average emissions of summertime NOx from 35 US urban areas directly from NO2 retrievals of the OMI during 2005−2014. Total OMI-derived NOx emissions over US urban areas decreased by 49%, consistent with reductions of 43, 49, and 44% in the bottom-up NOx emissions, the weak-wind OMI NO2 burdens, and the averaged NO2 concentrations, respectively.
Q. Jin, J. Wei, Z.-L. Yang, B. Pu, and J. Huang
Atmos. Chem. Phys., 15, 9897–9915, https://doi.org/10.5194/acp-15-9897-2015, https://doi.org/10.5194/acp-15-9897-2015, 2015
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Satellite data show that Indian summer monsoon (ISM) rainfall is closely associated with Middle East dust aerosols. Numerical modeling shows that the increased ISM rainfall is related to the enhanced southwesterly flow and moisture transport from the Arabian Sea to the Indian subcontinent, associated with the development of an anomalous low-pressure system over the Iranian Plateau and the Arabian Sea due to dust-induced atmospheric heating.
S. Eckhardt, B. Quennehen, D. J. L. Olivié, T. K. Berntsen, R. Cherian, J. H. Christensen, W. Collins, S. Crepinsek, N. Daskalakis, M. Flanner, A. Herber, C. Heyes, Ø. Hodnebrog, L. Huang, M. Kanakidou, Z. Klimont, J. Langner, K. S. Law, M. T. Lund, R. Mahmood, A. Massling, S. Myriokefalitakis, I. E. Nielsen, J. K. Nøjgaard, J. Quaas, P. K. Quinn, J.-C. Raut, S. T. Rumbold, M. Schulz, S. Sharma, R. B. Skeie, H. Skov, T. Uttal, K. von Salzen, and A. Stohl
Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, https://doi.org/10.5194/acp-15-9413-2015, 2015
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The concentrations of sulfate, black carbon and other aerosols in the Arctic are characterized by high values in late winter and spring (so-called Arctic Haze) and low values in summer. Models have long been struggling to capture this seasonality. In this study, we evaluate sulfate and BC concentrations from different updated models and emissions against a comprehensive pan-Arctic measurement data set. We find that the models improved but still struggle to get the maximum concentrations.
R. Zhang, H. Wang, Y. Qian, P. J. Rasch, R. C. Easter, P.-L. Ma, B. Singh, J. Huang, and Q. Fu
Atmos. Chem. Phys., 15, 6205–6223, https://doi.org/10.5194/acp-15-6205-2015, https://doi.org/10.5194/acp-15-6205-2015, 2015
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We use the CAM5 model with a novel source-tagging technique to characterize the fate of BC particles emitted from various geographical regions and sectors and their transport pathways to the Himalayas and Tibetan Plateau (HTP). We show a comprehensive picture of the seasonal and regional dependence of BC source attributions, and find strong seasonal and spatial variations in BC-in-snow radiative forcing in the HTP that can be quantitatively attributed to the various regional/sectoral sources.
R. Kumar, M. C. Barth, V. S. Nair, G. G. Pfister, S. Suresh Babu, S. K. Satheesh, K. Krishna Moorthy, G. R. Carmichael, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 15, 5415–5428, https://doi.org/10.5194/acp-15-5415-2015, https://doi.org/10.5194/acp-15-5415-2015, 2015
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We examine differences in the surface BC between the Bay of Bengal (BoB) and the Arabian Sea (AS) and identify dominant sources of BC in South Asia during ICARB. Anthropogenic emissions were the main source of BC during ICARB and had about 5 times stronger influence on the BoB compared to the AS. Regional-scale transport contributes up to 25% of BC mass concentrations in western and eastern India, suggesting that surface BC mass concentrations cannot be linked directly to the local emissions.
W.-L. Lee, Y. Gu, K. N. Liou, L. R. Leung, and H.-H. Hsu
Atmos. Chem. Phys., 15, 5405–5413, https://doi.org/10.5194/acp-15-5405-2015, https://doi.org/10.5194/acp-15-5405-2015, 2015
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This paper investigates 3-D mountain effects on solar flux distributions and their impact on surface hydrology over the western United States, specifically the Rocky Mountains and the Sierra Nevada, using the global CCSM4 (CAM4/CLM4) with a 0.23°×0.31° resolution for simulations over 6 years. We show that deviations in the net surface fluxes are not only affected by 3-D mountains but also influenced by feedbacks of cloud and snow in association with the long-term simulations.
Y. Fang, C. Liu, and L. R. Leung
Geosci. Model Dev., 8, 781–789, https://doi.org/10.5194/gmd-8-781-2015, https://doi.org/10.5194/gmd-8-781-2015, 2015
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1. A gradient projection method was used to reduce the computation time of carbon-nitrogen spin-up processes in CLM4.
2. Point-scale simulations showed that the cyclic stability of total carbon for some cases differs from that of the periodic atmospheric forcing, and some cases even showed instability.
3. The instability issue is resolved after the hydrology scheme in CLM4 is replaced with a flow model for variably saturated porous media.
S. Kulkarni, N. Sobhani, J. P. Miller-Schulze, M. M. Shafer, J. J. Schauer, P. A. Solomon, P. E. Saide, S. N. Spak, Y. F. Cheng, H. A. C. Denier van der Gon, Z. Lu, D. G. Streets, G. Janssens-Maenhout, C. Wiedinmyer, J. Lantz, M. Artamonova, B. Chen, S. Imashev, L. Sverdlik, J. T. Deminter, B. Adhikary, A. D'Allura, C. Wei, and G. R. Carmichael
Atmos. Chem. Phys., 15, 1683–1705, https://doi.org/10.5194/acp-15-1683-2015, https://doi.org/10.5194/acp-15-1683-2015, 2015
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This study presents a regional-scale modeling analysis of aerosols in the Central Asia region including detailed characterization of seasonal source region and sector contributions along with the predicted changes in distribution of aerosols using 2030 future emission scenarios. The influence of long transport and impact of varied emission sources including dust, biomass burning, and anthropogenic sources on the regional aerosol distributions and the associated transport pathways are discussed.
M. Wang, B. Xu, J. Cao, X. Tie, H. Wang, R. Zhang, Y. Qian, P. J. Rasch, S. Zhao, G. Wu, H. Zhao, D. R. Joswiak, J. Li, and Y. Xie
Atmos. Chem. Phys., 15, 1191–1204, https://doi.org/10.5194/acp-15-1191-2015, https://doi.org/10.5194/acp-15-1191-2015, 2015
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Carbonaceous aerosols recorded in a Tibetan glacier present a distinct seasonal dependence and an increasing trend after 1980, which has important implications for the accelerated glacier melting. We use a global aerosol--climate model to quantify the aerosol source--receptor relationships, showing that emissions in South Asia had the largest contribution. The emission inventories and historical fuel consumption in South Asia are consistent with our ice-core analysis and model results.
J. Li, J. Huang, K. Stamnes, T. Wang, Q. Lv, and H. Jin
Atmos. Chem. Phys., 15, 519–536, https://doi.org/10.5194/acp-15-519-2015, https://doi.org/10.5194/acp-15-519-2015, 2015
S. J. Doherty, C. M. Bitz, and M. G. Flanner
Atmos. Chem. Phys., 14, 11697–11709, https://doi.org/10.5194/acp-14-11697-2014, https://doi.org/10.5194/acp-14-11697-2014, 2014
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Black carbon in snow lowers its albedo, increasing the absorption of sunlight, leading to positive radiative forcing, climate warming and earlier snow-melt. A series of recent studies have used prescribed rates of black carbon deposition to snow to assess the climate effects of black carbon in snow. Here we show that the use of prescribed deposition fluxes in these model studies leads to high biases in snow BC concentrations, caused by the decoupling of BC and snow deposition to the surface.
S. Yu, R. Mathur, J. Pleim, D. Wong, R. Gilliam, K. Alapaty, C. Zhao, and X. Liu
Atmos. Chem. Phys., 14, 11247–11285, https://doi.org/10.5194/acp-14-11247-2014, https://doi.org/10.5194/acp-14-11247-2014, 2014
T. Glotfelty, Y. Zhang, P. Karamchandani, and D. G. Streets
Atmos. Chem. Phys., 14, 9379–9402, https://doi.org/10.5194/acp-14-9379-2014, https://doi.org/10.5194/acp-14-9379-2014, 2014
H. Wan, P. J. Rasch, K. Zhang, Y. Qian, H. Yan, and C. Zhao
Geosci. Model Dev., 7, 1961–1977, https://doi.org/10.5194/gmd-7-1961-2014, https://doi.org/10.5194/gmd-7-1961-2014, 2014
Hongru Yan, Zhanqing Li, Jianping Huang, Maureen Cribb, and Jianjun Liu
Atmos. Chem. Phys., 14, 7113–7124, https://doi.org/10.5194/acp-14-7113-2014, https://doi.org/10.5194/acp-14-7113-2014, 2014
C. He, Q. B. Li, K. N. Liou, J. Zhang, L. Qi, Y. Mao, M. Gao, Z. Lu, D. G. Streets, Q. Zhang, M. M. Sarin, and K. Ram
Atmos. Chem. Phys., 14, 7091–7112, https://doi.org/10.5194/acp-14-7091-2014, https://doi.org/10.5194/acp-14-7091-2014, 2014
F. Yan, E. Winijkul, D. G. Streets, Z. Lu, T. C. Bond, and Y. Zhang
Atmos. Chem. Phys., 14, 5709–5733, https://doi.org/10.5194/acp-14-5709-2014, https://doi.org/10.5194/acp-14-5709-2014, 2014
M. Li, Q. Zhang, D. G. Streets, K. B. He, Y. F. Cheng, L. K. Emmons, H. Huo, S. C. Kang, Z. Lu, M. Shao, H. Su, X. Yu, and Y. Zhang
Atmos. Chem. Phys., 14, 5617–5638, https://doi.org/10.5194/acp-14-5617-2014, https://doi.org/10.5194/acp-14-5617-2014, 2014
T. K. Tesfa, H.-Y. Li, L. R. Leung, M. Huang, Y. Ke, Y. Sun, and Y. Liu
Geosci. Model Dev., 7, 947–963, https://doi.org/10.5194/gmd-7-947-2014, https://doi.org/10.5194/gmd-7-947-2014, 2014
M. Chin, T. Diehl, Q. Tan, J. M. Prospero, R. A. Kahn, L. A. Remer, H. Yu, A. M. Sayer, H. Bian, I. V. Geogdzhayev, B. N. Holben, S. G. Howell, B. J. Huebert, N. C. Hsu, D. Kim, T. L. Kucsera, R. C. Levy, M. I. Mishchenko, X. Pan, P. K. Quinn, G. L. Schuster, D. G. Streets, S. A. Strode, O. Torres, and X.-P. Zhao
Atmos. Chem. Phys., 14, 3657–3690, https://doi.org/10.5194/acp-14-3657-2014, https://doi.org/10.5194/acp-14-3657-2014, 2014
C. Jiao, M. G. Flanner, Y. Balkanski, S. E. Bauer, N. Bellouin, T. K. Berntsen, H. Bian, K. S. Carslaw, M. Chin, N. De Luca, T. Diehl, S. J. Ghan, T. Iversen, A. Kirkevåg, D. Koch, X. Liu, G. W. Mann, J. E. Penner, G. Pitari, M. Schulz, Ø. Seland, R. B. Skeie, S. D. Steenrod, P. Stier, T. Takemura, K. Tsigaridis, T. van Noije, Y. Yun, and K. Zhang
Atmos. Chem. Phys., 14, 2399–2417, https://doi.org/10.5194/acp-14-2399-2014, https://doi.org/10.5194/acp-14-2399-2014, 2014
J. Fan, L. R. Leung, P. J. DeMott, J. M. Comstock, B. Singh, D. Rosenfeld, J. M. Tomlinson, A. White, K. A. Prather, P. Minnis, J. K. Ayers, and Q. Min
Atmos. Chem. Phys., 14, 81–101, https://doi.org/10.5194/acp-14-81-2014, https://doi.org/10.5194/acp-14-81-2014, 2014
D. N. Huntzinger, C. Schwalm, A. M. Michalak, K. Schaefer, A. W. King, Y. Wei, A. Jacobson, S. Liu, R. B. Cook, W. M. Post, G. Berthier, D. Hayes, M. Huang, A. Ito, H. Lei, C. Lu, J. Mao, C. H. Peng, S. Peng, B. Poulter, D. Riccuito, X. Shi, H. Tian, W. Wang, N. Zeng, F. Zhao, and Q. Zhu
Geosci. Model Dev., 6, 2121–2133, https://doi.org/10.5194/gmd-6-2121-2013, https://doi.org/10.5194/gmd-6-2121-2013, 2013
Y. Sun, Z. Hou, M. Huang, F. Tian, and L. Ruby Leung
Hydrol. Earth Syst. Sci., 17, 4995–5011, https://doi.org/10.5194/hess-17-4995-2013, https://doi.org/10.5194/hess-17-4995-2013, 2013
K. N. Liou, Y. Gu, L. R. Leung, W. L. Lee, and R. G. Fovell
Atmos. Chem. Phys., 13, 11709–11721, https://doi.org/10.5194/acp-13-11709-2013, https://doi.org/10.5194/acp-13-11709-2013, 2013
N. Voisin, L. Liu, M. Hejazi, T. Tesfa, H. Li, M. Huang, Y. Liu, and L. R. Leung
Hydrol. Earth Syst. Sci., 17, 4555–4575, https://doi.org/10.5194/hess-17-4555-2013, https://doi.org/10.5194/hess-17-4555-2013, 2013
Y. Fang, M. Huang, C. Liu, H. Li, and L. R. Leung
Geosci. Model Dev., 6, 1977–1988, https://doi.org/10.5194/gmd-6-1977-2013, https://doi.org/10.5194/gmd-6-1977-2013, 2013
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
N. Voisin, H. Li, D. Ward, M. Huang, M. Wigmosta, and L. R. Leung
Hydrol. Earth Syst. Sci., 17, 3605–3622, https://doi.org/10.5194/hess-17-3605-2013, https://doi.org/10.5194/hess-17-3605-2013, 2013
Y. Ke, L. R. Leung, M. Huang, and H. Li
Geosci. Model Dev., 6, 1609–1622, https://doi.org/10.5194/gmd-6-1609-2013, https://doi.org/10.5194/gmd-6-1609-2013, 2013
R. Zhang, D. A. Hegg, J. Huang, and Q. Fu
Atmos. Chem. Phys., 13, 6091–6099, https://doi.org/10.5194/acp-13-6091-2013, https://doi.org/10.5194/acp-13-6091-2013, 2013
H. Wan, P. J. Rasch, K. Zhang, J. Kazil, and L. R. Leung
Geosci. Model Dev., 6, 861–874, https://doi.org/10.5194/gmd-6-861-2013, https://doi.org/10.5194/gmd-6-861-2013, 2013
H. Wang, R. C. Easter, P. J. Rasch, M. Wang, X. Liu, S. J. Ghan, Y. Qian, J.-H. Yoon, P.-L. Ma, and V. Vinoj
Geosci. Model Dev., 6, 765–782, https://doi.org/10.5194/gmd-6-765-2013, https://doi.org/10.5194/gmd-6-765-2013, 2013
D. T. Shindell, J.-F. Lamarque, M. Schulz, M. Flanner, C. Jiao, M. Chin, P. J. Young, Y. H. Lee, L. Rotstayn, N. Mahowald, G. Milly, G. Faluvegi, Y. Balkanski, W. J. Collins, A. J. Conley, S. Dalsoren, R. Easter, S. Ghan, L. Horowitz, X. Liu, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. Skeie, K. Sudo, S. Szopa, T. Takemura, A. Voulgarakis, J.-H. Yoon, and F. Lo
Atmos. Chem. Phys., 13, 2939–2974, https://doi.org/10.5194/acp-13-2939-2013, https://doi.org/10.5194/acp-13-2939-2013, 2013
Y. H. Lee, J.-F. Lamarque, M. G. Flanner, C. Jiao, D. T. Shindell, T. Berntsen, M. M. Bisiaux, J. Cao, W. J. Collins, M. Curran, R. Edwards, G. Faluvegi, S. Ghan, L. W. Horowitz, J. R. McConnell, J. Ming, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. B. Skeie, K. Sudo, T. Takemura, F. Thevenon, B. Xu, and J.-H. Yoon
Atmos. Chem. Phys., 13, 2607–2634, https://doi.org/10.5194/acp-13-2607-2013, https://doi.org/10.5194/acp-13-2607-2013, 2013
K. M. Sterle, J. R. McConnell, J. Dozier, R. Edwards, and M. G. Flanner
The Cryosphere, 7, 365–374, https://doi.org/10.5194/tc-7-365-2013, https://doi.org/10.5194/tc-7-365-2013, 2013
S. Kalenderski, G. Stenchikov, and C. Zhao
Atmos. Chem. Phys., 13, 1999–2014, https://doi.org/10.5194/acp-13-1999-2013, https://doi.org/10.5194/acp-13-1999-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Analysis of secondary inorganic aerosols over the greater Athens area using the EPISODE–CityChem source dispersion and photochemistry model
Global estimates of ambient reactive nitrogen components during 2000–2100 based on the multi-stage model
The role of naphthalene and its derivatives in the formation of secondary organic aerosol in the Yangtze River Delta region, China
Unveiling the optimal regression model for source apportionment of the oxidative potential of PM10
Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 2: Modeling chemical drivers and 3-D new particle formation occurrence
Technical note: Influence of different averaging metrics and temporal resolutions on the aerosol pH calculated by thermodynamic modeling
Dual roles of the inorganic aqueous phase on secondary organic aerosol growth from benzene and phenol
Global source apportionment of aerosols into major emission regions and sectors over 1850–2017
Modeling atmospheric brown carbon in the GISS ModelE Earth system model
Observation-constrained kinetic modeling of isoprene SOA formation in the atmosphere
Significant impact of urban tree biogenic emissions on air quality estimated by a bottom-up inventory and chemistry transport modeling
Secondary organic aerosols derived from intermediate-volatility n-alkanes adopt low-viscous phase state
Cooling radiative forcing effect enhancement of atmospheric amines-mineral particle caused by heterogeneous uptake and oxidation
Modeling the drivers of fine PM pollution over Central Europe: impacts and contributions of emissions from different sources
Reaction of SO3 with H2SO4 and its implications for aerosol particle formation in the gas phase and at the air–water interface
Weakened aerosol–radiation interaction exacerbating ozone pollution in eastern China since China's clean air actions
Uncertainties from biomass burning aerosols in air quality models obscure public health impacts in Southeast Asia
Oxidative potential apportionment of atmospheric PM1: a new approach combining high-sensitive online analysers for chemical composition and offline OP measurement technique
Observed and CMIP6 model simulated organic aerosol response to drought in the contiguous United States during summertime
Aqueous-phase chemistry of glyoxal with multifunctional reduced nitrogen compounds: a potential missing route for secondary brown carbon
An updated modeling framework to simulate Los Angeles air quality – Part 1: Model development, evaluation, and source apportionment
Frequent haze events associated with transport and stagnation over the corridor between the North China Plain and Yangtze River Delta
Evaluation of WRF-Chem-simulated meteorology and aerosols over northern India during the severe pollution episode of 2016
How well are aerosol–cloud interactions represented in climate models? – Part 1: Understanding the sulfate aerosol production from the 2014–15 Holuhraun eruption
pH regulates the formation of organosulfates and inorganic sulfate from organic peroxide reaction with dissolved SO2 in aquatic media
Technical note: Accurate, reliable, and high-resolution air quality predictions by improving the Copernicus Atmosphere Monitoring Service using a novel statistical post-processing method
Contribution of intermediate-volatility organic compounds from on-road transport to secondary organic aerosol levels in Europe
Source-resolved atmospheric metal emissions, concentrations, and their deposition fluxes into the East Asian Seas
Development of an integrated model framework for multi-air-pollutant exposure assessments in high-density cities
CAMx–UNIPAR simulation of secondary organic aerosol mass formed from multiphase reactions of hydrocarbons under the Central Valley urban atmospheres of California
Impact of urbanization on fine particulate matter concentrations over central Europe
Measurement report: Assessing the impacts of emission uncertainty on aerosol optical properties and radiative forcing from biomass burning in peninsular Southeast Asia
The Emissions Model Intercomparison Project (Emissions-MIP): quantifying model sensitivity to emission characteristics
Dynamics-based estimates of decline trend with fine temporal variations in China's PM2.5 emissions
Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US
Reactive organic carbon air emissions from mobile sources in the United States
Development and evaluation of processes affecting simulation of diel fine particulate matter variation in the GEOS-Chem model
Substantially positive contributions of new particle formation to cloud condensation nuclei under low supersaturation in China based on numerical model improvements
Evolution of atmospheric age of particles and its implications for the formation of a severe haze event in eastern China
A multimodel evaluation of the potential impact of shipping on particle species in the Mediterranean Sea
How does tropospheric VOC chemistry affect climate? An investigation of preindustrial control simulations using the Community Earth System Model version 2
Anthropogenic amplification of biogenic secondary organic aerosol production
A dynamic parameterization of sulfuric acid–dimethylamine nucleation and its application in three-dimensional modeling
Modeling dust mineralogical composition: sensitivity to soil mineralogy atlases and their expected climate impacts
Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China
Impact of Landes forest fires on air quality in France during the 2022 summer
Global nitrogen and sulfur deposition mapping using a measurement–model fusion approach
Comprehensive simulations of new particle formation events in Beijing with a cluster dynamics–multicomponent sectional model
Implications of differences between recent anthropogenic aerosol emission inventories for diagnosed AOD and radiative forcing from 1990 to 2019
Unbalanced emission reductions of different species and sectors in China during COVID-19 lockdown derived by multi-species surface observation assimilation
Stelios Myriokefalitakis, Matthias Karl, Kim A. Weiss, Dimitris Karagiannis, Eleni Athanasopoulou, Anastasia Kakouri, Aikaterini Bougiatioti, Eleni Liakakou, Iasonas Stavroulas, Georgios Papangelis, Georgios Grivas, Despina Paraskevopoulou, Orestis Speyer, Nikolaos Mihalopoulos, and Evangelos Gerasopoulos
Atmos. Chem. Phys., 24, 7815–7835, https://doi.org/10.5194/acp-24-7815-2024, https://doi.org/10.5194/acp-24-7815-2024, 2024
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A state-of-the-art thermodynamic model has been coupled with the city-scale chemistry transport model EPISODE–CityChem to investigate the equilibrium between the inorganic gas and aerosol phases over the greater Athens area, Greece. The simulations indicate that the formation of nitrates in an urban environment is significantly affected by local nitrogen oxide emissions, as well as ambient temperature, relative humidity, photochemical activity, and the presence of non-volatile cations.
Rui Li, Yining Gao, Lijia Zhang, Yubing Shen, Tianzhao Xu, Wenwen Sun, and Gehui Wang
Atmos. Chem. Phys., 24, 7623–7636, https://doi.org/10.5194/acp-24-7623-2024, https://doi.org/10.5194/acp-24-7623-2024, 2024
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A three-stage model was developed to obtain the global maps of reactive nitrogen components during 2000–2100. The results implied that cross-validation R2 values of four species showed satisfactory performance (R2 > 0.55). Most reactive nitrogen components, except NH3, in China showed increases during 2000–2013. In the future scenarios, SSP3-7.0 (traditional-energy scenario) and SSP1-2.6 (carbon neutrality scenario) showed the highest and lowest reactive nitrogen component concentrations.
Fei Ye, Jingyi Li, Yaqin Gao, Hongli Wang, Jingyu An, Cheng Huang, Song Guo, Keding Lu, Kangjia Gong, Haowen Zhang, Momei Qin, and Jianlin Hu
Atmos. Chem. Phys., 24, 7467–7479, https://doi.org/10.5194/acp-24-7467-2024, https://doi.org/10.5194/acp-24-7467-2024, 2024
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Naphthalene (Nap) and methylnaphthalene (MN) are key precursors of secondary organic aerosol (SOA), yet their sources and sinks are often inadequately represented in air quality models. In this study, we incorporated detailed emissions, gas-phase chemistry, and SOA parameterization of Nap and MN into CMAQ to address this issue. The findings revealed remarkably high SOA formation potentials for these compounds despite their low emissions in the Yangtze River Delta region during summer.
Vy Dinh Ngoc Thuy, Jean-Luc Jaffrezo, Ian Hough, Pamela A. Dominutti, Guillaume Salque Moreton, Grégory Gille, Florie Francony, Arabelle Patron-Anquez, Olivier Favez, and Gaëlle Uzu
Atmos. Chem. Phys., 24, 7261–7282, https://doi.org/10.5194/acp-24-7261-2024, https://doi.org/10.5194/acp-24-7261-2024, 2024
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The capacity of particulate matter (PM) to generate reactive oxygen species in vivo is represented by oxidative potential (OP). This study focuses on finding the appropriate model to evaluate the oxidative character of PM sources in six sites using the PM sources and OP. Eight regression techniques are introduced to assess the OP of PM. The study highlights the importance of selecting a model according to the input data characteristics and establishes some recommendations for the procedure.
Ming Chu, Xing Wei, Shangfei Hai, Yang Gao, Huiwang Gao, Yujiao Zhu, Biwu Chu, Nan Ma, Juan Hong, Yele Sun, and Xiaohong Yao
Atmos. Chem. Phys., 24, 6769–6786, https://doi.org/10.5194/acp-24-6769-2024, https://doi.org/10.5194/acp-24-6769-2024, 2024
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We used a 20-bin WRF-Chem model to simulate NPF events in the NCP during a three-week observational period in the summer of 2019. The model was able to reproduce the observations during June 29–July 6, which was characterized by a high frequency of NPF occurrence.
Haoqi Wang, Xiao Tian, Wanting Zhao, Jiacheng Li, Haoyu Yu, Yinchang Feng, and Shaojie Song
Atmos. Chem. Phys., 24, 6583–6592, https://doi.org/10.5194/acp-24-6583-2024, https://doi.org/10.5194/acp-24-6583-2024, 2024
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pH is a key property of ambient aerosols, which affect many atmospheric processes. As aerosol pH is a non-conservative parameter, diverse averaging metrics and temporal resolutions may influence the pH values calculated by thermodynamic models. This technical note seeks to quantitatively evaluate the average pH using varied metrics and resolutions. The ultimate goal is to establish standardized reporting practices in future research endeavors.
Jiwon Choi, Myoseon Jang, and Spencer Blau
Atmos. Chem. Phys., 24, 6567–6582, https://doi.org/10.5194/acp-24-6567-2024, https://doi.org/10.5194/acp-24-6567-2024, 2024
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Persistent phenoxy radical (PPR), formed by phenol gas oxidation and its aqueous reaction, catalytically destroys O3 and retards secondary organic aerosol (SOA) growth. Explicit gas mechanisms including the formation of PPR and low-volatility products from the oxidation of phenol or benzene are applied to the UNIPAR model to predict SOA mass via multiphase reactions of precursors. Aqueous reactions of reactive organics increase SOA mass but retard SOA growth via heterogeneously formed PPR.
Yang Yang, Shaoxuan Mou, Hailong Wang, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 24, 6509–6523, https://doi.org/10.5194/acp-24-6509-2024, https://doi.org/10.5194/acp-24-6509-2024, 2024
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The variations in anthropogenic aerosol concentrations and source contributions and their subsequent radiative impact in major emission regions during historical periods are quantified based on an aerosol-tagging system in E3SMv1. Due to the industrial development and implementation of economic policies, sources of anthropogenic aerosols show different variations, which has important implications for pollution prevention and control measures and decision-making for global collaboration.
Maegan A. DeLessio, Kostas Tsigaridis, Susanne E. Bauer, Jacek Chowdhary, and Gregory L. Schuster
Atmos. Chem. Phys., 24, 6275–6304, https://doi.org/10.5194/acp-24-6275-2024, https://doi.org/10.5194/acp-24-6275-2024, 2024
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This study presents the first explicit representation of brown carbon aerosols in the GISS ModelE Earth system model (ESM). Model sensitivity to a range of brown carbon parameters and model performance compared to AERONET and MODIS retrievals of total aerosol properties were assessed. A summary of best practices for incorporating brown carbon into ModelE is also included.
Chuanyang Shen, Xiaoyan Yang, Joel Thornton, John Shilling, Chenyang Bi, Gabriel Isaacman-VanWertz, and Haofei Zhang
Atmos. Chem. Phys., 24, 6153–6175, https://doi.org/10.5194/acp-24-6153-2024, https://doi.org/10.5194/acp-24-6153-2024, 2024
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In this work, a condensed multiphase isoprene oxidation mechanism was developed to simulate isoprene SOA formation from chamber and field studies. Our results show that the measured isoprene SOA mass concentrations can be reasonably reproduced. The simulation results indicate that multifunctional low-volatility products contribute significantly to total isoprene SOA. Our findings emphasize that the pathways to produce these low-volatility species should be considered in models.
Alice Maison, Lya Lugon, Soo-Jin Park, Alexia Baudic, Christopher Cantrell, Florian Couvidat, Barbara D'Anna, Claudia Di Biagio, Aline Gratien, Valérie Gros, Carmen Kalalian, Julien Kammer, Vincent Michoud, Jean-Eudes Petit, Marwa Shahin, Leila Simon, Myrto Valari, Jérémy Vigneron, Andrée Tuzet, and Karine Sartelet
Atmos. Chem. Phys., 24, 6011–6046, https://doi.org/10.5194/acp-24-6011-2024, https://doi.org/10.5194/acp-24-6011-2024, 2024
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This study presents the development of a bottom-up inventory of urban tree biogenic emissions. Emissions are computed for each tree based on their location and characteristics and are integrated in the regional air quality model WRF-CHIMERE. The impact of these biogenic emissions on air quality is quantified for June–July 2022. Over Paris city, urban trees increase the concentrations of particulate organic matter by 4.6 %, of PM2.5 by 0.6 %, and of ozone by 1.0 % on average over 2 months.
Tommaso Galeazzo, Bernard Aumont, Marie Camredon, Richard Valorso, Yong B. Lim, Paul J. Ziemann, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 5549–5565, https://doi.org/10.5194/acp-24-5549-2024, https://doi.org/10.5194/acp-24-5549-2024, 2024
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Secondary organic aerosol (SOA) derived from n-alkanes is a major component of anthropogenic particulate matter. We provide an analysis of n-alkane SOA by chemistry modeling, machine learning, and laboratory experiments, showing that n-alkane SOA adopts low-viscous semi-solid or liquid states. Our results indicate few kinetic limitations of mass accommodation in SOA formation, supporting the application of equilibrium partitioning for simulating n-alkane SOA in large-scale atmospheric models.
Weina Zhang, Jianhua Mai, Zhichao Fan, Yongpeng Ji, Yuemeng Ji, Guiying Li, Yanpeng Gao, and Taicheng An
EGUsphere, https://doi.org/10.5194/egusphere-2024-1048, https://doi.org/10.5194/egusphere-2024-1048, 2024
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Previous studies show distinctive RFE of AOP-mineral mixed particles from individual mineral or AOP particles. This study reveals heterogeneous oxidation causes further RFE enhancement of amine-mineral mixed particle. Note that RFE increment is higher under clean condition than that under polluted condition, which is contributed to high-oxygen-content product. The enhanced RFE of amine-mineral particle caused by heterogenous oxidation is expected to alleviate warming effect.
Lukáš Bartík, Peter Huszár, Jan Karlický, Ondřej Vlček, and Kryštof Eben
Atmos. Chem. Phys., 24, 4347–4387, https://doi.org/10.5194/acp-24-4347-2024, https://doi.org/10.5194/acp-24-4347-2024, 2024
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The presented study deals with the attribution of fine particulate matter (PM2.5) concentrations to anthropogenic emissions over Central Europe using regional-scale models. It calculates the present-day contributions of different emissions sectors to concentrations of PM2.5 and its secondary components. Moreover, the study investigates the effect of chemical nonlinearities by using multiple source attribution methods and secondary organic aerosol calculation methods.
Rui Wang, Yang Cheng, Shasha Chen, Rongrong Li, Yue Hu, Xiaokai Guo, Tianlei Zhang, Fengmin Song, and Hao Li
Atmos. Chem. Phys., 24, 4029–4046, https://doi.org/10.5194/acp-24-4029-2024, https://doi.org/10.5194/acp-24-4029-2024, 2024
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We used quantum chemical calculations, Born–Oppenheimer molecular dynamics simulations, and the ACDC kinetic model to characterize SO3–H2SO4 interaction in the gas phase and at the air–water interface and to study the effect of H2S2O7 on H2SO4–NH3-based clusters. The work expands our understanding of new pathways for the loss of SO3 in acidic polluted areas and helps reveal some missing sources of NPF in metropolitan industrial regions and understand the atmospheric organic–sulfur cycle better.
Hao Yang, Lei Chen, Hong Liao, Jia Zhu, Wenjie Wang, and Xin Li
Atmos. Chem. Phys., 24, 4001–4015, https://doi.org/10.5194/acp-24-4001-2024, https://doi.org/10.5194/acp-24-4001-2024, 2024
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The present study quantifies the response of aerosol–radiation interaction (ARI) to anthropogenic emission reduction from 2013 to 2017, with the main focus on the contribution to changed O3 concentrations over eastern China both in summer and winter using the WRF-Chem model. The weakened ARI due to decreased anthropogenic emission aggravates the summer (winter) O3 pollution by +0.81 ppb (+0.63 ppb), averaged over eastern China.
Margaret R. Marvin, Paul I. Palmer, Fei Yao, Mohd Talib Latif, and Md Firoz Khan
Atmos. Chem. Phys., 24, 3699–3715, https://doi.org/10.5194/acp-24-3699-2024, https://doi.org/10.5194/acp-24-3699-2024, 2024
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We use an atmospheric chemistry model to investigate aerosols emitted from fire activity across Southeast Asia. We find that the limited nature of measurements in this region leads to large uncertainties that significantly hinder the model representation of these aerosols and their impacts on air quality. As a result, the number of monthly attributable deaths is underestimated by as many as 4500, particularly in March at the peak of the mainland burning season.
Julie Camman, Benjamin Chazeau, Nicolas Marchand, Amandine Durand, Grégory Gille, Ludovic Lanzi, Jean-Luc Jaffrezo, Henri Wortham, and Gaëlle Uzu
Atmos. Chem. Phys., 24, 3257–3278, https://doi.org/10.5194/acp-24-3257-2024, https://doi.org/10.5194/acp-24-3257-2024, 2024
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Fine particle (PM1) pollution is a major health issue in the city of Marseille, which is subject to numerous pollution sources. Sampling carried out during the summer enabled a fine characterization of the PM1 sources and their oxidative potential, a promising new metric as a proxy for health impact. PM1 came mainly from combustion sources, secondary ammonium sulfate, and organic nitrate, while the oxidative potential of PM1 came from these sources and from resuspended dust in the atmosphere.
Wei Li and Yuxuan Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-430, https://doi.org/10.5194/egusphere-2024-430, 2024
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This study finds that droughts immensely increased organic aerosol (OA) in the contiguous U.S. during summertime 1998–2019, notably in the Pacific Northwest (PNW) and Southeast (SEUS). The rise of OA in the SEUS is mainly driven by the enhanced formation of isoprene epoxydiols derived secondary organic aerosol due to the increase of isoprene and sulfate, while in the PNW, it is caused by wildfires. Ten climate models captured the OA increase in the PNW, yet greatly underestimated it in the SEUS.
Yuemeng Ji, Zhang Shi, Wenjian Li, Jiaxin Wang, Qiuju Shi, Yixin Li, Lei Gao, Ruize Ma, Weijun Lu, Lulu Xu, Yanpeng Gao, Guiying Li, and Taicheng An
Atmos. Chem. Phys., 24, 3079–3091, https://doi.org/10.5194/acp-24-3079-2024, https://doi.org/10.5194/acp-24-3079-2024, 2024
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The formation mechanisms for secondary brown carbon (SBrC) contributed by multifunctional reduced nitrogen compounds (RNCs) remain unclear. Hence, from combined laboratory experiments and quantum chemical calculations, we investigated the heterogeneous reactions of glyoxal (GL) with multifunctional RNCs, which are driven by four-step indirect nucleophilic addition reactions. Our results show a possible missing source for SBrC formation on urban, regional, and global scales.
Elyse A. Pennington, Yuan Wang, Benjamin C. Schulze, Karl M. Seltzer, Jiani Yang, Bin Zhao, Zhe Jiang, Hongru Shi, Melissa Venecek, Daniel Chau, Benjamin N. Murphy, Christopher M. Kenseth, Ryan X. Ward, Havala O. T. Pye, and John H. Seinfeld
Atmos. Chem. Phys., 24, 2345–2363, https://doi.org/10.5194/acp-24-2345-2024, https://doi.org/10.5194/acp-24-2345-2024, 2024
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To assess the air quality in Los Angeles (LA), we improved the CMAQ model by using dynamic traffic emissions and new secondary organic aerosol schemes to represent volatile chemical products. Source apportionment demonstrates that the urban areas of the LA Basin and vicinity are NOx-saturated, with the largest sensitivity of O3 to changes in volatile organic compounds in the urban core. The improvement and remaining issues shed light on the future direction of the model development.
Feifan Yan, Hang Su, Yafang Cheng, Rujin Huang, Hong Liao, Ting Yang, Yuanyuan Zhu, Shaoqing Zhang, Lifang Sheng, Wenbin Kou, Xinran Zeng, Shengnan Xiang, Xiaohong Yao, Huiwang Gao, and Yang Gao
Atmos. Chem. Phys., 24, 2365–2376, https://doi.org/10.5194/acp-24-2365-2024, https://doi.org/10.5194/acp-24-2365-2024, 2024
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PM2.5 pollution is a major air quality issue deteriorating human health, and previous studies mostly focus on regions like the North China Plain and Yangtze River Delta. However, the characteristics of PM2.5 concentrations between these two regions are studied less often. Focusing on the transport corridor region, we identify an interesting seesaw transport phenomenon with stagnant weather conditions, conducive to PM2.5 accumulation over this region, resulting in large health effects.
Prerita Agarwal, David S. Stevenson, and Mathew R. Heal
Atmos. Chem. Phys., 24, 2239–2266, https://doi.org/10.5194/acp-24-2239-2024, https://doi.org/10.5194/acp-24-2239-2024, 2024
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Air pollution levels across northern India are amongst some of the worst in the world, with episodic and hazardous haze events. Here, the ability of the WRF-Chem model to predict air quality over northern India is assessed against several datasets. Whilst surface wind speed and particle pollution peaks are over- and underestimated, respectively, meteorology and aerosol trends are adequately captured, and we conclude it is suitable for investigating severe particle pollution events.
George Jordan, Florent Malavelle, Ying Chen, Amy Peace, Eliza Duncan, Daniel G. Partridge, Paul Kim, Duncan Watson-Parris, Toshihiko Takemura, David Neubauer, Gunnar Myhre, Ragnhild Skeie, Anton Laakso, and James Haywood
Atmos. Chem. Phys., 24, 1939–1960, https://doi.org/10.5194/acp-24-1939-2024, https://doi.org/10.5194/acp-24-1939-2024, 2024
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The 2014–15 Holuhraun eruption caused a huge aerosol plume in an otherwise unpolluted region, providing a chance to study how aerosol alters cloud properties. This two-part study uses observations and models to quantify this relationship’s impact on the Earth’s energy budget. Part 1 suggests the models capture the observed spatial and chemical evolution of the plume, yet no model plume is exact. Understanding these differences is key for Part 2, where changes to cloud properties are explored.
Lin Du, Xiaofan Lv, Makroni Lily, Kun Li, and Narcisse Tsona Tchinda
Atmos. Chem. Phys., 24, 1841–1853, https://doi.org/10.5194/acp-24-1841-2024, https://doi.org/10.5194/acp-24-1841-2024, 2024
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This study explores the pH effect on the reaction of dissolved SO2 with selected organic peroxides. Results show that the formation of organic and/or inorganic sulfate from these peroxides strongly depends on their electronic structures, and these processes are likely to alter the chemical composition of dissolved organic matter in different ways. The rate constants of these reactions exhibit positive pH and temperature dependencies within pH 1–10 and 240–340 K ranges.
Angelo Riccio and Elena Chianese
Atmos. Chem. Phys., 24, 1673–1689, https://doi.org/10.5194/acp-24-1673-2024, https://doi.org/10.5194/acp-24-1673-2024, 2024
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Starting from the Copernicus Atmosphere Monitoring Service (CAMS), we provided a novel ensemble statistical post-processing approach to improve their air quality predictions. Our approach is able to provide reliable short-term forecasts of pollutant concentrations, which is a key challenge in supporting national authorities in their tasks related to EU Air Quality Directives, such as planning and reporting the state of air quality to the citizens.
Stella E. I. Manavi and Spyros N. Pandis
Atmos. Chem. Phys., 24, 891–909, https://doi.org/10.5194/acp-24-891-2024, https://doi.org/10.5194/acp-24-891-2024, 2024
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Organic vapors of intermediate volatility have often been neglected as sources of atmospheric organic aerosol. In this work we use a new approach for their simulation and quantify the contribution of these compounds emitted by transportation sources (gasoline and diesel vehicles) to particulate matter over Europe. The estimated secondary organic aerosol levels are on average 60 % higher than predicted by previous approaches. However, these estimates are probably lower limits.
Shenglan Jiang, Yan Zhang, Guangyuan Yu, Zimin Han, Junri Zhao, Tianle Zhang, and Mei Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-155, https://doi.org/10.5194/egusphere-2024-155, 2024
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This study aims to provide gridded data on sea-wide concentrations, deposition fluxes, and soluble deposition fluxes with detailed source categories of metals by the modified CMAQ model. We developed a monthly emission inventory of six metals – Fe, Al, V, Ni, Zn, and Cu – from land anthropogenic, ship, and dust sources in East Asia in 2017. Our results revealed the contribution of each source to the emissions, concentrations, and deposition fluxes of metals in the East Asian seas.
Zhiyuan Li, Kin-Fai Ho, Harry Fung Lee, and Steve Hung Lam Yim
Atmos. Chem. Phys., 24, 649–661, https://doi.org/10.5194/acp-24-649-2024, https://doi.org/10.5194/acp-24-649-2024, 2024
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This study developed an integrated model framework for accurate multi-air-pollutant exposure assessments in high-density and high-rise cities. Following the proposed integrated model framework, we established multi-air-pollutant exposure models for four major PM10 chemical species as well as four criteria air pollutants with R2 values ranging from 0.73 to 0.93. The proposed framework serves as an important tool for combined exposure assessment in epidemiological studies.
Yujin Jo, Myoseon Jang, Sanghee Han, Azad Madhu, Bonyoung Koo, Yiqin Jia, Zechen Yu, Soontae Kim, and Jinsoo Park
Atmos. Chem. Phys., 24, 487–508, https://doi.org/10.5194/acp-24-487-2024, https://doi.org/10.5194/acp-24-487-2024, 2024
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The CAMx–UNIPAR model simulated the SOA budget formed via multiphase reactions of hydrocarbons and the impact of emissions and climate on SOA characteristics under California’s urban environments during winter 2018. SOA growth was dominated by daytime oxidation of long-chain alkanes and nighttime terpene oxidation with O3 and NO−3 radicals. The spatial distributions of anthropogenic SOA were affected by the northwesterly wind, whereas those of biogenic SOA were insensitive to wind directions.
Peter Huszar, Alvaro Patricio Prieto Perez, Lukáš Bartík, Jan Karlický, and Anahi Villalba-Pradas
Atmos. Chem. Phys., 24, 397–425, https://doi.org/10.5194/acp-24-397-2024, https://doi.org/10.5194/acp-24-397-2024, 2024
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Urbanization transforms rural land into artificial land, while due to human activities, it also introduces a great quantity of emissions. We quantify the impact of urbanization on the final particulate matter pollutant levels by looking not only at these emissions, but also at the way urban land cover influences meteorological conditions, how the removal of pollutants changes due to urban land cover, and how biogenic emissions from vegetation change due to less vegetation in urban areas.
Yinbao Jin, Yiming Liu, Xiao Lu, Xiaoyang Chen, Ao Shen, Haofan Wang, Yinping Cui, Yifei Xu, Siting Li, Jian Liu, Ming Zhang, Yingying Ma, and Qi Fan
Atmos. Chem. Phys., 24, 367–395, https://doi.org/10.5194/acp-24-367-2024, https://doi.org/10.5194/acp-24-367-2024, 2024
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This study aims to address these issues by evaluating eight independent biomass burning (BB) emission inventories (GFED, FINN1.5, FINN2.5 MOS, FINN2.5 MOSVIS, GFAS, FEER, QFED, and IS4FIRES) using the WRF-Chem model and analyzing their impact on aerosol optical properties (AOPs) and direct radiative forcing (DRF) during wildfire events in peninsular Southeast Asia (PSEA) that occurred in March 2019.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Zhen Peng, Lili Lei, Zhe-Min Tan, Meigen Zhang, Aijun Ding, and Xingxia Kou
Atmos. Chem. Phys., 23, 14505–14520, https://doi.org/10.5194/acp-23-14505-2023, https://doi.org/10.5194/acp-23-14505-2023, 2023
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Annual PM2.5 emissions in China consistently decreased by about 3% to 5% from 2017 to 2020 with spatial variations and seasonal dependencies. High-temporal-resolution and dynamics-based PM2.5 emission estimates provide quantitative diurnal variations for each season. Significant reductions in PM2.5 emissions in the North China Plain and northeast of China in 2020 were caused by COVID-19.
Stylianos Kakavas, Spyros N. Pandis, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13555–13564, https://doi.org/10.5194/acp-23-13555-2023, https://doi.org/10.5194/acp-23-13555-2023, 2023
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Water uptake from organic species in aerosol can affect the partitioning of semi-volatile inorganic compounds but are not considered in global and chemical transport models. We address this with a version of the PM-CAMx model that considers such organic water effects and use it to carry out 1-year aerosol simulations over the continental US. We show that such organic water impacts can increase dry PM1 levels by up to 2 μg m-3 when RH levels and PM1 concentrations are high.
Benjamin N. Murphy, Darrell Sonntag, Karl M. Seltzer, Havala O. T. Pye, Christine Allen, Evan Murray, Claudia Toro, Drew R. Gentner, Cheng Huang, Shantanu Jathar, Li Li, Andrew A. May, and Allen L. Robinson
Atmos. Chem. Phys., 23, 13469–13483, https://doi.org/10.5194/acp-23-13469-2023, https://doi.org/10.5194/acp-23-13469-2023, 2023
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We update methods for calculating organic particle and vapor emissions from mobile sources in the USA. Conventionally, particulate matter (PM) and volatile organic carbon (VOC) are speciated without consideration of primary semivolatile emissions. Our methods integrate state-of-the-science speciation profiles and correct for common artifacts when sampling emissions in a laboratory. We quantify impacts of the emission updates on ambient pollution with the Community Multiscale Air Quality model.
Yanshun Li, Randall V. Martin, Chi Li, Brian L. Boys, Aaron van Donkelaar, Jun Meng, and Jeffrey R. Pierce
Atmos. Chem. Phys., 23, 12525–12543, https://doi.org/10.5194/acp-23-12525-2023, https://doi.org/10.5194/acp-23-12525-2023, 2023
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We developed and evaluated processes affecting within-day (diel) variability in PM2.5 concentrations in a chemical transport model over the contiguous US. Diel variability in PM2.5 for the contiguous US is driven by early-morning accumulation into a shallow mixed layer, decreases from mid-morning through afternoon with mixed-layer growth, increases from mid-afternoon through evening as the mixed-layer collapses, and decreases overnight as emissions decrease.
Chupeng Zhang, Shangfei Hai, Yang Gao, Yuhang Wang, Shaoqing Zhang, Lifang Sheng, Bin Zhao, Shuxiao Wang, Jingkun Jiang, Xin Huang, Xiaojing Shen, Junying Sun, Aura Lupascu, Manish Shrivastava, Jerome D. Fast, Wenxuan Cheng, Xiuwen Guo, Ming Chu, Nan Ma, Juan Hong, Qiaoqiao Wang, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 23, 10713–10730, https://doi.org/10.5194/acp-23-10713-2023, https://doi.org/10.5194/acp-23-10713-2023, 2023
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New particle formation is an important source of atmospheric particles, exerting critical influences on global climate. Numerical models are vital tools to understanding atmospheric particle evolution, which, however, suffer from large biases in simulating particle numbers. Here we improve the model chemical processes governing particle sizes and compositions. The improved model reveals substantial contributions of newly formed particles to climate through effects on cloud condensation nuclei.
Xiaodong Xie, Jianlin Hu, Momei Qin, Song Guo, Min Hu, Dongsheng Ji, Hongli Wang, Shengrong Lou, Cheng Huang, Chong Liu, Hongliang Zhang, Qi Ying, Hong Liao, and Yuanhang Zhang
Atmos. Chem. Phys., 23, 10563–10578, https://doi.org/10.5194/acp-23-10563-2023, https://doi.org/10.5194/acp-23-10563-2023, 2023
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The atmospheric age of particles reflects how long particles have been formed and suspended in the atmosphere, which is closely associated with the evolution processes of particles. An analysis of the atmospheric age of PM2.5 provides a unique perspective on the evolution processes of different PM2.5 components. The results also shed lights on how to design effective emission control actions under unfavorable meteorological conditions.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Sara Jutterström, Jana Moldanova, Elisa Majamäki, and Jukka-Pekka Jalkanen
Atmos. Chem. Phys., 23, 10163–10189, https://doi.org/10.5194/acp-23-10163-2023, https://doi.org/10.5194/acp-23-10163-2023, 2023
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The Mediterranean Sea is a heavily trafficked shipping area, and air quality monitoring stations in numerous cities along the Mediterranean coast have detected high levels of air pollutants originating from shipping emissions. The current study investigates how existing restrictions on shipping-related emissions to the atmosphere ensure compliance with legislation. Focus was laid on fine particles and particle species, which were simulated with five different chemical transport models.
Noah A. Stanton and Neil F. Tandon
Atmos. Chem. Phys., 23, 9191–9216, https://doi.org/10.5194/acp-23-9191-2023, https://doi.org/10.5194/acp-23-9191-2023, 2023
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Chemistry in Earth’s atmosphere has a potentially strong but very uncertain impact on climate. Past attempts to fully model chemistry in Earth’s troposphere (the lowest layer of the atmosphere) typically simplified the representation of Earth’s surface, which in turn limited the ability to simulate changes in climate. The cutting-edge model that we use in this study does not require such simplification, and we use it to examine the climate effects of chemical interactions in the troposphere.
Yiqi Zheng, Larry W. Horowitz, Raymond Menzel, David J. Paynter, Vaishali Naik, Jingyi Li, and Jingqiu Mao
Atmos. Chem. Phys., 23, 8993–9007, https://doi.org/10.5194/acp-23-8993-2023, https://doi.org/10.5194/acp-23-8993-2023, 2023
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Biogenic secondary organic aerosols (SOAs) account for a large fraction of fine aerosol at the global scale. Using long-term measurements and a climate model, we investigate anthropogenic impacts on biogenic SOA at both decadal and centennial timescales. Results show that despite reductions in biogenic precursor emissions, SOA has been strongly amplified by anthropogenic emissions since the preindustrial era and exerts a cooling radiative forcing.
Yuyang Li, Jiewen Shen, Bin Zhao, Runlong Cai, Shuxiao Wang, Yang Gao, Manish Shrivastava, Da Gao, Jun Zheng, Markku Kulmala, and Jingkun Jiang
Atmos. Chem. Phys., 23, 8789–8804, https://doi.org/10.5194/acp-23-8789-2023, https://doi.org/10.5194/acp-23-8789-2023, 2023
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We set up a new parameterization for 1.4 nm particle formation rates from sulfuric acid–dimethylamine (SA–DMA) nucleation, fully including the effects of coagulation scavenging and cluster stability. Incorporating the new parameterization into 3-D chemical transport models, we achieved better consistencies between simulation results and observation data. This new parameterization provides new insights into atmospheric nucleation simulations and its effects on atmospheric pollution or health.
María Gonçalves Ageitos, Vincenzo Obiso, Ron L. Miller, Oriol Jorba, Martina Klose, Matt Dawson, Yves Balkanski, Jan Perlwitz, Sara Basart, Enza Di Tomaso, Jerónimo Escribano, Francesca Macchia, Gilbert Montané, Natalie M. Mahowald, Robert O. Green, David R. Thompson, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 8623–8657, https://doi.org/10.5194/acp-23-8623-2023, https://doi.org/10.5194/acp-23-8623-2023, 2023
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Dust aerosols affect our climate differently depending on their mineral composition. We include dust mineralogy in an atmospheric model considering two existing soil maps, which still have large associated uncertainties. The soil data and the distribution of the minerals in different aerosol sizes are key to our model performance. We find significant regional variations in climate-relevant variables, which supports including mineralogy in our current models and the need for improved soil maps.
Jianyan Lu, Sunling Gong, Jian Zhang, Jianmin Chen, Lei Zhang, and Chunhong Zhou
Atmos. Chem. Phys., 23, 8021–8037, https://doi.org/10.5194/acp-23-8021-2023, https://doi.org/10.5194/acp-23-8021-2023, 2023
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WRF/CUACE was used to assess the cloud chemistry contribution in China. Firstly, the CUACE cloud chemistry scheme was found to reproduce well the cloud processing and consumption of H2O2, O3, and SO2, as well as the increase of sulfate. Secondly, during cloud availability in December under a heavy pollution episode, sulfate production increased 60–95 % and SO2 was reduced by over 80 %. This study provides a way to analyze the phenomenon of overestimation of SO2 in many chemical transport models.
Laurent Menut, Arineh Cholakian, Guillaume Siour, Rémy Lapere, Romain Pennel, Sylvain Mailler, and Bertrand Bessagnet
Atmos. Chem. Phys., 23, 7281–7296, https://doi.org/10.5194/acp-23-7281-2023, https://doi.org/10.5194/acp-23-7281-2023, 2023
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This study is about the wildfires occurring in France during the summer 2022. We study the forest fires that took place in the Landes during the summer of 2022. We show the direct impact of these fires on the air quality, especially downstream of the smoke plume towards the Paris region. We quantify the impact of these fires on the pollutants peak concentrations and the possible exceedance of thresholds.
Hannah J. Rubin, Joshua S. Fu, Frank Dentener, Rui Li, Kan Huang, and Hongbo Fu
Atmos. Chem. Phys., 23, 7091–7102, https://doi.org/10.5194/acp-23-7091-2023, https://doi.org/10.5194/acp-23-7091-2023, 2023
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We update the 2010 global deposition budget for nitrogen (N) and sulfur (S) with new regional wet deposition measurements, improving the ensemble results of 11 global chemistry transport models from HTAP II. Our study demonstrates that a global measurement–model fusion approach can substantially improve N and S deposition model estimates at a regional scale and represents a step forward toward the WMO goal of global fusion products for accurately mapping harmful air pollution.
Chenxi Li, Yuyang Li, Xiaoxiao Li, Runlong Cai, Yaxin Fan, Xiaohui Qiao, Rujing Yin, Chao Yan, Yishuo Guo, Yongchun Liu, Jun Zheng, Veli-Matti Kerminen, Markku Kulmala, Huayun Xiao, and Jingkun Jiang
Atmos. Chem. Phys., 23, 6879–6896, https://doi.org/10.5194/acp-23-6879-2023, https://doi.org/10.5194/acp-23-6879-2023, 2023
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New particle formation and growth in polluted environments are not fully understood despite intensive research. We applied a cluster dynamics–multicomponent sectional model to simulate the new particle formation events observed in Beijing, China. The simulation approximately captures how the events evolve. Further diagnosis shows that the oxygenated organic molecules may have been under-detected, and modulating their abundance leads to significantly improved simulation–observation agreement.
Marianne Tronstad Lund, Gunnar Myhre, Ragnhild Bieltvedt Skeie, Bjørn Hallvard Samset, and Zbigniew Klimont
Atmos. Chem. Phys., 23, 6647–6662, https://doi.org/10.5194/acp-23-6647-2023, https://doi.org/10.5194/acp-23-6647-2023, 2023
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Here we show that differences, in magnitude and trend, between recent global anthropogenic emission inventories have a notable influence on simulated regional abundances of anthropogenic aerosol over the 1990–2019 period. This, in turn, affects estimates of radiative forcing. Our findings form a basis for comparing existing and upcoming studies on anthropogenic aerosols using different emission inventories.
Lei Kong, Xiao Tang, Jiang Zhu, Zifa Wang, Yele Sun, Pingqing Fu, Meng Gao, Huangjian Wu, Miaomiao Lu, Qian Wu, Shuyuan Huang, Wenxuan Sui, Jie Li, Xiaole Pan, Lin Wu, Hajime Akimoto, and Gregory R. Carmichael
Atmos. Chem. Phys., 23, 6217–6240, https://doi.org/10.5194/acp-23-6217-2023, https://doi.org/10.5194/acp-23-6217-2023, 2023
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A multi-air-pollutant inversion system has been developed in this study to estimate emission changes in China during COVID-19 lockdown. The results demonstrate that the lockdown is largely a nationwide road traffic control measure with NOx emissions decreasing by ~40 %. Emissions of other species only decreased by ~10 % due to smaller effects of lockdown on other sectors. Assessment results further indicate that the lockdown only had limited effects on the control of PM2.5 and O3 in China.
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