Articles | Volume 13, issue 5
https://doi.org/10.5194/acp-13-2445-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-2445-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
04 Mar 2013
Research article |
| 04 Mar 2013
Anthropogenic carbon dioxide source areas observed from space: assessment of regional enhancements and trends
O. Schneising
Institute of Environmental Physics (IUP), University of Bremen FB1, Bremen, Germany
J. Heymann
Institute of Environmental Physics (IUP), University of Bremen FB1, Bremen, Germany
M. Buchwitz
Institute of Environmental Physics (IUP), University of Bremen FB1, Bremen, Germany
M. Reuter
Institute of Environmental Physics (IUP), University of Bremen FB1, Bremen, Germany
H. Bovensmann
Institute of Environmental Physics (IUP), University of Bremen FB1, Bremen, Germany
J. P. Burrows
Institute of Environmental Physics (IUP), University of Bremen FB1, Bremen, Germany
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We quantified changes in atmospheric methane concentrations using satellite data and a dynamic linear model approach. We calculated global annual methane increases for the years 2019–2022, which are in good agreement with other sources. For zonal methane growth rates, we identified strong inter-hemispheric differences in 2019 and 2022. For 2022, we could attribute decreases in the global growth rate to the Northern Hemisphere, possibly related to a reduction in anthropogenic emissions.
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Atmos. Meas. Tech., 16, 669–694, https://doi.org/10.5194/amt-16-669-2023, https://doi.org/10.5194/amt-16-669-2023, 2023
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Atmos. Meas. Tech., 15, 3401–3437, https://doi.org/10.5194/amt-15-3401-2022, https://doi.org/10.5194/amt-15-3401-2022, 2022
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Michael Buchwitz, Maximilian Reuter, Oliver Schneising, Stefan Noël, Bettina Gier, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Akihiko Kuze, Hiroshi Suto, Yukio Yoshida, David Crisp, and Christopher O'Dell
Atmos. Chem. Phys., 18, 17355–17370, https://doi.org/10.5194/acp-18-17355-2018, https://doi.org/10.5194/acp-18-17355-2018, 2018
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We present a new satellite data set of column-averaged mixing ratios of carbon dioxide (CO2), which covers the time period 2003 to 2016. We used this data set to compute annual mean atmospheric CO2 growth rates. We show that the growth rate is highest during 2015 and 2016 despite nearly constant CO2 emissions from fossil fuel burning in recent years. The high growth rates are attributed to year 2015-2016 El Nino episodes. We present correlations with fossil fuel emissions and ENSO indices.
Michael Buchwitz, Oliver Schneising, Maximilian Reuter, Jens Heymann, Sven Krautwurst, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Christian Frankenberg, and Alexander J. Turner
Atmos. Chem. Phys., 17, 5751–5774, https://doi.org/10.5194/acp-17-5751-2017, https://doi.org/10.5194/acp-17-5751-2017, 2017
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J. Heymann, M. Reuter, M. Hilker, M. Buchwitz, O. Schneising, H. Bovensmann, J. P. Burrows, A. Kuze, H. Suto, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, S. Kawakami, R. Kivi, I. Morino, C. Petri, C. Roehl, M. Schneider, V. Sherlock, R. Sussmann, V. A. Velazco, T. Warneke, and D. Wunch
Atmos. Meas. Tech., 8, 2961–2980, https://doi.org/10.5194/amt-8-2961-2015, https://doi.org/10.5194/amt-8-2961-2015, 2015
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M. Reuter, M. Buchwitz, M. Hilker, J. Heymann, O. Schneising, D. Pillai, H. Bovensmann, J. P. Burrows, H. Bösch, R. Parker, A. Butz, O. Hasekamp, C. W. O'Dell, Y. Yoshida, C. Gerbig, T. Nehrkorn, N. M. Deutscher, T. Warneke, J. Notholt, F. Hase, R. Kivi, R. Sussmann, T. Machida, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 13739–13753, https://doi.org/10.5194/acp-14-13739-2014, https://doi.org/10.5194/acp-14-13739-2014, 2014
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G. D. Hayman, F. M. O'Connor, M. Dalvi, D. B. Clark, N. Gedney, C. Huntingford, C. Prigent, M. Buchwitz, O. Schneising, J. P. Burrows, C. Wilson, N. Richards, and M. Chipperfield
Atmos. Chem. Phys., 14, 13257–13280, https://doi.org/10.5194/acp-14-13257-2014, https://doi.org/10.5194/acp-14-13257-2014, 2014
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B. Dils, M. Buchwitz, M. Reuter, O. Schneising, H. Boesch, R. Parker, S. Guerlet, I. Aben, T. Blumenstock, J. P. Burrows, A. Butz, N. M. Deutscher, C. Frankenberg, F. Hase, O. P. Hasekamp, J. Heymann, M. De Mazière, J. Notholt, R. Sussmann, T. Warneke, D. Griffith, V. Sherlock, and D. Wunch
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Atmos. Chem. Phys., 14, 133–141, https://doi.org/10.5194/acp-14-133-2014, https://doi.org/10.5194/acp-14-133-2014, 2014
Rolf Müller, Lennart Bengtsson, John Birks, John Burrows, Ruprecht Jaenicke, and Richard S. Stolarski
Hist. Geo Space. Sci. Discuss., https://doi.org/10.5194/hgss-2025-2, https://doi.org/10.5194/hgss-2025-2, 2025
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This paper reports a few anecdotes from the life of Paul Crutzen, which were contributed by friends and colleagues. Taken together these anecdotes should shed some light on the person Paul Crutzen, which is perhaps less visible, when focusing only on his scientific achievements.
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EGUsphere, https://doi.org/10.5194/egusphere-2025-1977, https://doi.org/10.5194/egusphere-2025-1977, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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India poses a significant methane emission burden, but limited observations challenge accurate national estimations. This study combines satellite retrievals, ground measurements, and models to improve India’s 2018–2019 methane budget. Derived emissions are higher than national reports but lower than global inventories. The findings highlight the potential of satellite instruments to report emissions accurately. Expanded methane monitoring is vital for meeting climate change mitigation targets.
Johann Rasmus Nüß, Nikos Daskalakis, Fabian Günther Piwowarczyk, Angelos Gkouvousis, Oliver Schneising, Michael Buchwitz, Maria Kanakidou, Maarten C. Krol, and Mihalis Vrekoussis
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We estimate carbon monoxide emissions through inverse modeling, an approach where measurements of tracers in the atmosphere are fed to a model to calculate backwards in time (inverse) where the tracers came from. We introduce measurements from a new satellite instrument and show that, in most places globally, these on their own sufficiently constrain the emissions. This alleviates the need for additional datasets, which could shorten the delay for future carbon monoxide source estimates.
Miriam Latsch, Andreas Richter, John P. Burrows, and Hartmut Bösch
EGUsphere, https://doi.org/10.5194/egusphere-2025-107, https://doi.org/10.5194/egusphere-2025-107, 2025
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This study presents our advanced methods to better detect ship-related nitrogen dioxide (NO2) emissions in TROPOMI satellite data. By applying filtering techniques, we identify numerous global shipping routes, including previously undetectable ones, and emissions from offshore platforms. Additionally, we compare the filtered satellite data with CAMS global model data to estimate the differences between observed and modelled NO2 emissions.
Ella Kivimäki, Tuula Aalto, Michael Buchwitz, Kari Luojus, Jouni Pulliainen, Kimmo Rautiainen, Oliver Schneising, Anu-Maija Sundström, Johanna Tamminen, Aki Tsuruta, and Hannakaisa Lindqvist
EGUsphere, https://doi.org/10.5194/egusphere-2025-249, https://doi.org/10.5194/egusphere-2025-249, 2025
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We investigate how environmental variables influencing natural methane fluxes explain the large-scale seasonal variability of satellite-observed methane at Northern high latitudes. Our findings show that soil moisture, snow cover, and soil temperature have the strongest influence, with snowmelt playing a surprisingly significant role, likely through soil isolation and wetting. This study highlights the value of multi-satellite observations for understanding large-scale wetland emissions.
Michael Weimer, Michael Hilker, Stefan Noël, Max Reuter, Michael Buchwitz, Blanca Fuentes Andrade, Rüdiger Lang, Bernd Sierk, Yasjka Meijer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
EGUsphere, https://doi.org/10.5194/egusphere-2024-3857, https://doi.org/10.5194/egusphere-2024-3857, 2025
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Optical detectors have a maximum signal (saturation). Exceedance means that the measurement has to be discarded. We investigate where saturation will occur for the future European satellite mission dedicated to CO2 Monitoring (CO2M) and strategies to avoid saturation. It impacts coverage and precision, both important for estimation of local CO2 emissions. We find that taking two pictures per sampling should be sufficient to avoid saturation for CO2M with some impact on the CO2 precision.
Maximilian Reuter, Michael Hilker, Stefan Noël, Antonio Di Noia, Michael Weimer, Oliver Schneising, Michael Buchwitz, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
Atmos. Meas. Tech., 18, 241–264, https://doi.org/10.5194/amt-18-241-2025, https://doi.org/10.5194/amt-18-241-2025, 2025
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Carbon dioxide (CO2) and methane (CH4) are the main anthropogenic greenhouse gases. The European Copernicus CO2 monitoring satellite mission CO2M will provide measurements of their atmospheric concentrations, but the accuracy requirements are demanding and conventional retrieval methods computationally expensive. We present a new retrieval algorithm based on artificial neural networks that has the potential to meet the stringent requirements of the CO2M mission with minimal computational effort.
Seunghwan Seo, Si-Wan Kim, Kyoung-Min Kim, Andreas Richter, Kezia Lange, John P. Burrows, Junsung Park, Hyunkee Hong, Hanlim Lee, Ukkyo Jeong, Jung-Hun Woo, and Jhoon Kim
Atmos. Meas. Tech., 18, 115–128, https://doi.org/10.5194/amt-18-115-2025, https://doi.org/10.5194/amt-18-115-2025, 2025
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Over the Seoul metropolitan area, tropospheric NO2 vertical column densities from the Geostationary Environment Monitoring Spectrometer show distinct seasonal features. Also, varying a priori data have substantial impacts on the observed NO2 columns. The a priori data from different chemical transport models resulted in differences of up to −18.3 %. Notably, diurnal patterns of observed NO2 columns are similar for all datasets, although their a priori data exhibit contrasting diurnal patterns.
Phuc Thi Minh Ha, Yugo Kanaya, Kazuyo Yamaji, Syuichi Itahashi, Satoru Chatani, Takashi Sekiya, Maria Dolores Andrés Hernández, John Philip Burrows, Hans Schlager, Michael Lichtenstern, Mira Poehlker, and Bruna Holanda
EGUsphere, https://doi.org/10.5194/egusphere-2024-2064, https://doi.org/10.5194/egusphere-2024-2064, 2024
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Black carbon and CO are important to climate change. EMeRGe airborne observation can identify the suitability of emission inventories used in CMAQv5.0.2 model for Asian polluted regions. GFEDv4.1s is suitable for fire emissions. Anthropogenic BC and CO emissions from Philippines (REASv2.1) are insufficient. The estimated Chinese emissions in 2018 are 0.65±0.25 TgBC, 166±65 TgCO and 12.4±4.8 PgCO2, suggesting a reduction and increment for China's BC and CO emissions in the HTAPv2.2z inventory.
Alexei Rozanov, Christine Pohl, Carlo Arosio, Adam Bourassa, Klaus Bramstedt, Elizaveta Malinina, Landon Rieger, and John P. Burrows
Atmos. Meas. Tech., 17, 6677–6695, https://doi.org/10.5194/amt-17-6677-2024, https://doi.org/10.5194/amt-17-6677-2024, 2024
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We developed a new algorithm to retrieve vertical distributions of aerosol extinction coefficients in the stratosphere. The algorithm is applied to measurements of scattered solar light from the spaceborne OMPS-LP (Ozone Mapper and Profiler Suite Limb Profiler) instrument. The retrieval results are compared to data from other spaceborne instruments and used to investigate the evolution of the aerosol plume following the eruption of the Hunga Tonga–Hunga Ha'apai volcano in January 2022.
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, https://doi.org/10.5194/essd-16-5227-2024, 2024
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Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Swathi Maratt Satheesan, Kai-Uwe Eichmann, John P. Burrows, Mark Weber, Ryan Stauffer, Anne M. Thompson, and Debra Kollonige
Atmos. Meas. Tech., 17, 6459–6484, https://doi.org/10.5194/amt-17-6459-2024, https://doi.org/10.5194/amt-17-6459-2024, 2024
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CHORA, an advanced cloud convective differential technique, enhances the accuracy of tropospheric-ozone retrievals. Unlike the traditional Pacific cloud reference sector scheme, CHORA introduces a local-cloud reference sector and an alternative approach (CLCT) for precision. Analysing monthly averaged TROPOMI data from 2018 to 2022 and validating with SHADOZ ozonesonde data, CLCT outperforms other methods and so is the preferred choice, especially in future geostationary satellite missions.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, Jong-Uk Park, and Hanlim Lee
Atmos. Meas. Tech., 17, 6315–6344, https://doi.org/10.5194/amt-17-6315-2024, https://doi.org/10.5194/amt-17-6315-2024, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Sven Krautwurst, Christian Fruck, Sebastian Wolff, Jakob Borchardt, Oke Huhs, Konstantin Gerilowski, Michał Gałkowski, Christoph Kiemle, Mathieu Quatrevalet, Martin Wirth, Christian Mallaun, John P. Burrows, Christoph Gerbig, Andreas Fix, Hartmut Bösch, and Heinrich Bovensmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-3182, https://doi.org/10.5194/egusphere-2024-3182, 2024
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Anomalously high CH4 emissions from landfills in Madrid, Spain, have been observed by satellite measurements in recent years. Our investigations of these waste facilities using passive and active airborne remote sensing measurements confirm these high emission rates with values of up to 13 th-1 during the overflight and show excellent agreement between the two techniques. A large fraction of the emissions is attributed to active landfill sites.
Steffen Vanselow, Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Hartmut Boesch, and John P. Burrows
Atmos. Chem. Phys., 24, 10441–10473, https://doi.org/10.5194/acp-24-10441-2024, https://doi.org/10.5194/acp-24-10441-2024, 2024
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We developed an algorithm to automatically detect persistent methane source regions, to quantify their emissions and to determine their source types, by analyzing TROPOMI data from 2018–2021. The over 200 globally detected natural and anthropogenic source regions include small-scale point sources such as individual coal mines and larger-scale source regions such as wetlands and large oil and gas fields.
Falco Monsees, Alexei Rozanov, John P. Burrows, Mark Weber, Annette Rinke, Ralf Jaiser, and Peter von der Gathen
Atmos. Chem. Phys., 24, 9085–9099, https://doi.org/10.5194/acp-24-9085-2024, https://doi.org/10.5194/acp-24-9085-2024, 2024
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Cyclones strongly influence weather predictability but still cannot be fully characterised in the Arctic because of the sparse coverage of meteorological measurements. A potential approach to compensate for this is the use of satellite measurements of ozone, because cyclones impact the tropopause and therefore also ozone. In this study we used this connection to investigate the correlation between ozone and the tropopause in the Arctic and to identify cyclones with satellite ozone observations.
Christine Pohl, Felix Wrana, Alexei Rozanov, Terry Deshler, Elizaveta Malinina, Christian von Savigny, Landon A. Rieger, Adam E. Bourassa, and John P. Burrows
Atmos. Meas. Tech., 17, 4153–4181, https://doi.org/10.5194/amt-17-4153-2024, https://doi.org/10.5194/amt-17-4153-2024, 2024
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Knowledge of stratospheric aerosol characteristics is important for understanding chemical and climate aerosol feedbacks. Two particle size distribution parameters, the aerosol extinction coefficient and the effective radius, are obtained from SCIAMACHY limb observations. The aerosol characteristics show good agreement with independent data sets from balloon-borne and satellite observations. This data set expands the limited knowledge of stratospheric aerosol characteristics.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Chem. Phys., 24, 7609–7621, https://doi.org/10.5194/acp-24-7609-2024, https://doi.org/10.5194/acp-24-7609-2024, 2024
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Large quantities of CO and CO2 are emitted during conventional steel production. As satellite-based estimates of CO2 emissions at the facility level are challenging, co-emitted CO can indicate the carbon footprint of steel plants. We estimate CO emissions for German steelworks and use CO2 emissions from emissions trading data to derive a sector-specific CO/CO2 emission ratio for the steel industry; it is a prerequisite to use CO as a proxy for CO2 emissions from similar steel production sites.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Stefan Noël, Michael Buchwitz, Michael Hilker, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
Atmos. Meas. Tech., 17, 2317–2334, https://doi.org/10.5194/amt-17-2317-2024, https://doi.org/10.5194/amt-17-2317-2024, 2024
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FOCAL-CO2M is one of the three operational retrieval algorithms which will be used to derive XCO2 and XCH4 from measurements of the forthcoming European CO2M mission. We present results of applications of FOCAL-CO2M to simulated spectra, from which confidence is gained that the algorithm is able to fulfil the challenging requirements on systematic errors for the CO2M mission (spatio-temporal bias ≤ 0.5 ppm for XCO2 and ≤ 5 ppb for XCH4).
Andrea Orfanoz-Cheuquelaf, Carlo Arosio, Alexei Rozanov, Mark Weber, Annette Ladstätter-Weißenmayer, John P. Burrows, Anne M. Thompson, Ryan M. Stauffer, and Debra E. Kollonige
Atmos. Meas. Tech., 17, 1791–1809, https://doi.org/10.5194/amt-17-1791-2024, https://doi.org/10.5194/amt-17-1791-2024, 2024
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Valuable information on the tropospheric ozone column (TrOC) can be obtained globally by combining space-borne limb and nadir measurements (limb–nadir matching, LNM). This study describes the retrieval of TrOC from the OMPS instrument (since 2012) using the LNM technique. The OMPS-LNM TrOC was compared with ozonesondes and other satellite measurements, showing a good agreement with a negative bias within 1 to 4 DU. This new dataset is suitable for pollution studies.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-516, https://doi.org/10.5194/egusphere-2024-516, 2024
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This study assesses atmospheric composition using air quality models during aircraft campaigns in Europe and Asia, focusing on carbonaceous aerosols and trace gases. While carbon monoxide is well modeled, other pollutants have moderate to weak agreement with observations. Wind speed modeling is reliable for identifying pollution plumes, where models tend to overestimate concentrations. This highlights challenges in accurately modeling aerosol and trace gas composition, particularly in cities.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-521, https://doi.org/10.5194/egusphere-2024-521, 2024
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This study explores the proportional relationships between carbonaceous aerosols (black and organic carbon) and trace gases using airborne measurements from two campaigns in Europe and East Asia. Differences between regions were found, but air quality models struggled to reproduce them accurately. We show that these proportional relationships can help to constrain models and can be used to infer aerosol concentrations from satellite observations of trace gases, especially in urban areas.
Blanca Fuentes Andrade, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Andreas Richter, Hartmut Boesch, and John P. Burrows
Atmos. Meas. Tech., 17, 1145–1173, https://doi.org/10.5194/amt-17-1145-2024, https://doi.org/10.5194/amt-17-1145-2024, 2024
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We developed a method to estimate CO2 emissions from localized sources, such as power plants, using satellite data and applied it to estimate CO2 emissions from the Bełchatów Power Station (Poland). As the detection of CO2 emission plumes from satellite data is difficult, we used observations of co-emitted NO2 to constrain the emission plume region. Our results agree with CO2 emission estimations based on the power-plant-generated power and emission factors.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Soheila Jafariserajehlou, Sachin S. Gunthe, Andreas Herber, Christoph Ritter, Hartmut Bösch, and John P. Burrows
Atmos. Meas. Tech., 17, 359–375, https://doi.org/10.5194/amt-17-359-2024, https://doi.org/10.5194/amt-17-359-2024, 2024
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Aerosols are suspensions of particles dispersed in the air. In this study, we use a novel retrieval of satellite data to investigate an optical property of aerosols, the aerosol optical depth, in the high Arctic to assess their direct and indirect roles in climate change. This study demonstrates that the presented approach shows good quality and very promising potential.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Chem. Phys., 24, 577–595, https://doi.org/10.5194/acp-24-577-2024, https://doi.org/10.5194/acp-24-577-2024, 2024
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We quantified changes in atmospheric methane concentrations using satellite data and a dynamic linear model approach. We calculated global annual methane increases for the years 2019–2022, which are in good agreement with other sources. For zonal methane growth rates, we identified strong inter-hemispheric differences in 2019 and 2022. For 2022, we could attribute decreases in the global growth rate to the Northern Hemisphere, possibly related to a reduction in anthropogenic emissions.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
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During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, John Philip Burrows, Birger Bohn, Eric Förster, Florian Obersteiner, Andreas Zahn, Theresa Harlaß, Helmut Ziereis, Hans Schlager, Benjamin Schreiner, Flora Kluge, Katja Bigge, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 7799–7822, https://doi.org/10.5194/acp-23-7799-2023, https://doi.org/10.5194/acp-23-7799-2023, 2023
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The applicability of photostationary steady-state (PSS) assumptions to estimate the amount of the sum of peroxy radicals (RO2*) during the EMeRGe airborne observations from the known radical chemistry and onboard measurements of RO2* precursors, photolysis frequencies, and other trace gases such as NOx and O3 was investigated. The comparison of the calculated RO2* with the actual measurements provides an insight into the main processes controlling their concentration in the air masses measured.
Kameswara S. Vinjamuri, Marco Vountas, Luca Lelli, Martin Stengel, Matthew D. Shupe, Kerstin Ebell, and John P. Burrows
Atmos. Meas. Tech., 16, 2903–2918, https://doi.org/10.5194/amt-16-2903-2023, https://doi.org/10.5194/amt-16-2903-2023, 2023
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Clouds play an important role in Arctic amplification. Cloud data from ground-based sites are valuable but cannot represent the whole Arctic. Therefore the use of satellite products is a measure to cover the entire Arctic. However, the quality of such cloud measurements from space is not well known. The paper discusses the differences and commonalities between satellite and ground-based measurements. We conclude that the satellite dataset, with a few exceptions, can be used in the Arctic.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Aishwarya Singh, Yanick Ziegler, Sachin S. Gunthe, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2023-730, https://doi.org/10.5194/egusphere-2023-730, 2023
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Aerosols are suspensions of particles distributed in the air. Depending on their chemical composition, they scatter and/or absorb sunlight and thus cool or warm the earth's atmosphere and its surface. They also provide as a surface in the atmosphere upon which ice or liquid clouds droplets nucleate and grow. In this study, we use satellite observations and model simulations to investigate the properties of aerosols with the goal of assessing their direct and indirect role in climate change.
Kai Krause, Folkard Wittrock, Andreas Richter, Dieter Busch, Anton Bergen, John P. Burrows, Steffen Freitag, and Olesia Halbherr
Atmos. Meas. Tech., 16, 1767–1787, https://doi.org/10.5194/amt-16-1767-2023, https://doi.org/10.5194/amt-16-1767-2023, 2023
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Inland shipping is an important source of nitrogen oxides (NOx). The amount of emitted NOx depends on the characteristics of the individual vessels and the traffic density. Ship emissions are often characterised by the amount of emitted NOx per unit of burnt fuel, and further knowledge about fuel consumption is needed to quantify the total emissions caused by ship traffic. In this study, a new approach to derive absolute emission rates (in g s−1) from onshore measurements is presented.
Anna Agustí-Panareda, Jérôme Barré, Sébastien Massart, Antje Inness, Ilse Aben, Melanie Ades, Bianca C. Baier, Gianpaolo Balsamo, Tobias Borsdorff, Nicolas Bousserez, Souhail Boussetta, Michael Buchwitz, Luca Cantarello, Cyril Crevoisier, Richard Engelen, Henk Eskes, Johannes Flemming, Sébastien Garrigues, Otto Hasekamp, Vincent Huijnen, Luke Jones, Zak Kipling, Bavo Langerock, Joe McNorton, Nicolas Meilhac, Stefan Noël, Mark Parrington, Vincent-Henri Peuch, Michel Ramonet, Miha Razinger, Maximilian Reuter, Roberto Ribas, Martin Suttie, Colm Sweeney, Jérôme Tarniewicz, and Lianghai Wu
Atmos. Chem. Phys., 23, 3829–3859, https://doi.org/10.5194/acp-23-3829-2023, https://doi.org/10.5194/acp-23-3829-2023, 2023
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We present a global dataset of atmospheric CO2 and CH4, the two most important human-made greenhouse gases, which covers almost 2 decades (2003–2020). It is produced by combining satellite data of CO2 and CH4 with a weather and air composition prediction model, and it has been carefully evaluated against independent observations to ensure validity and point out deficiencies to the user. This dataset can be used for scientific studies in the field of climate change and the global carbon cycle.
Linlu Mei, Vladimir Rozanov, Alexei Rozanov, and John P. Burrows
Geosci. Model Dev., 16, 1511–1536, https://doi.org/10.5194/gmd-16-1511-2023, https://doi.org/10.5194/gmd-16-1511-2023, 2023
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This paper summarizes recent developments of aerosol, cloud and surface reflectance databases and models in the framework of the software package SCIATRAN. These updates and developments extend the capabilities of the radiative transfer modeling, especially by accounting for different kinds of vertical inhomogeneties. Vertically inhomogeneous clouds and different aerosol types can be easily accounted for within SCIATRAN (V4.6). The widely used surface models and databases are now available.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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We present airborne imaging DOAS and ground-based stationary and car DOAS measurements conducted during the S5P-VAL-DE-Ruhr campaign in the Rhine-Ruhr region. The measurements are used to validate spaceborne NO2 data products from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Auxiliary data of the TROPOMI NO2 retrieval, such as spatially higher resolved a priori NO2 vertical profiles, surface reflectivity, and cloud treatment are investigated to evaluate their impact.
Dominik Brunner, Gerrit Kuhlmann, Stephan Henne, Erik Koene, Bastian Kern, Sebastian Wolff, Christiane Voigt, Patrick Jöckel, Christoph Kiemle, Anke Roiger, Alina Fiehn, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Jakob Borchardt, Michal Galkowski, Christoph Gerbig, Julia Marshall, Andrzej Klonecki, Pascal Prunet, Robert Hanfland, Margit Pattantyús-Ábrahám, Andrzej Wyszogrodzki, and Andreas Fix
Atmos. Chem. Phys., 23, 2699–2728, https://doi.org/10.5194/acp-23-2699-2023, https://doi.org/10.5194/acp-23-2699-2023, 2023
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We evaluated six atmospheric transport models for their capability to simulate the CO2 plumes from two of the largest power plants in Europe by comparing the models against aircraft observations collected during the CoMet (Carbon Dioxide and Methane Mission) campaign in 2018. The study analyzed how realistically such plumes can be simulated at different model resolutions and how well the planned European satellite mission CO2M will be able to quantify emissions from power plants.
Chuan-Yao Lin, Wan-Chin Chen, Yi-Yun Chien, Charles C. K. Chou, Chian-Yi Liu, Helmut Ziereis, Hans Schlager, Eric Förster, Florian Obersteiner, Ovid O. Krüger, Bruna A. Holanda, Mira L. Pöhlker, Katharina Kaiser, Johannes Schneider, Birger Bohn, Klaus Pfeilsticker, Benjamin Weyland, Maria Dolores Andrés Hernández, and John P. Burrows
Atmos. Chem. Phys., 23, 2627–2647, https://doi.org/10.5194/acp-23-2627-2023, https://doi.org/10.5194/acp-23-2627-2023, 2023
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During the EMeRGe campaign in Asia, atmospheric pollutants were measured on board the HALO aircraft. The WRF-Chem model was employed to evaluate the biomass burning (BB) plume transported from Indochina and its impact on the downstream areas. The combination of BB aerosol enhancement with cloud water resulted in a reduction in incoming shortwave radiation at the surface in southern China and the East China Sea, which potentially has significant regional climate implications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Oliver Schneising, Michael Buchwitz, Jonas Hachmeister, Steffen Vanselow, Maximilian Reuter, Matthias Buschmann, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 16, 669–694, https://doi.org/10.5194/amt-16-669-2023, https://doi.org/10.5194/amt-16-669-2023, 2023
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Methane and carbon monoxide are important constituents of the atmosphere in the context of climate change and air pollution. We present the latest advances in the TROPOMI/WFMD algorithm to simultaneously retrieve atmospheric methane and carbon monoxide abundances from space. The changes in the latest product version are described in detail, and the resulting improvements are demonstrated. An overview of the products is provided including a discussion of annual increases and validation results.
Miriam Latsch, Andreas Richter, Henk Eskes, Maarten Sneep, Ping Wang, Pepijn Veefkind, Ronny Lutz, Diego Loyola, Athina Argyrouli, Pieter Valks, Thomas Wagner, Holger Sihler, Michel van Roozendael, Nicolas Theys, Huan Yu, Richard Siddans, and John P. Burrows
Atmos. Meas. Tech., 15, 6257–6283, https://doi.org/10.5194/amt-15-6257-2022, https://doi.org/10.5194/amt-15-6257-2022, 2022
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The article investigates different S5P TROPOMI cloud retrieval algorithms for tropospheric trace gas retrievals. The cloud products show differences primarily over snow and ice and for scenes under sun glint. Some issues regarding across-track dependence are found for the cloud fractions as well as for the cloud heights.
Carlo Arosio, Alexei Rozanov, Victor Gorshelev, Alexandra Laeng, and John P. Burrows
Atmos. Meas. Tech., 15, 5949–5967, https://doi.org/10.5194/amt-15-5949-2022, https://doi.org/10.5194/amt-15-5949-2022, 2022
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This paper characterizes the uncertainties affecting the ozone profiles retrieved at the University of Bremen through OMPS limb satellite observations. An accurate knowledge of the uncertainties is relevant for the validation of the product and to correctly interpret the retrieval results. We investigate several sources of uncertainties, estimate a total random and systematic component, and verify the consistency of the combined OMPS-MLS total uncertainty.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, Alba Lorente, Tobias Borsdorff, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Meas. Tech., 15, 4063–4074, https://doi.org/10.5194/amt-15-4063-2022, https://doi.org/10.5194/amt-15-4063-2022, 2022
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Sentinel-5P trace gas retrievals rely on elevation data in their calculations. Outdated or inaccurate data can lead to significant errors in e.g. dry-air mole fractions of methane (XCH4). We show that the use of inadequate elevation data leads to strong XCH4 anomalies in Greenland. Similar problems can be expected for other regions with inaccurate elevation data. However, we expect these to be more localized. We show that updating elevation data used in the retrieval solves this issue.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
William G. Read, Gabriele Stiller, Stefan Lossow, Michael Kiefer, Farahnaz Khosrawi, Dale Hurst, Holger Vömel, Karen Rosenlof, Bianca M. Dinelli, Piera Raspollini, Gerald E. Nedoluha, John C. Gille, Yasuko Kasai, Patrick Eriksson, Christopher E. Sioris, Kaley A. Walker, Katja Weigel, John P. Burrows, and Alexei Rozanov
Atmos. Meas. Tech., 15, 3377–3400, https://doi.org/10.5194/amt-15-3377-2022, https://doi.org/10.5194/amt-15-3377-2022, 2022
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This paper attempts to provide an assessment of the accuracy of 21 satellite-based instruments that remotely measure atmospheric humidity in the upper troposphere of the Earth's atmosphere. The instruments made their measurements from 1984 to the present time; however, most of these instruments began operations after 2000, and only a few are still operational. The objective of this study is to quantify the accuracy of each satellite humidity data set.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Oliver Schneising, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Robert J. Parker, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Cheng Liu, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, Christof Petri, David F. Pollard, Markus Rettinger, Coleen Roehl, Constantina Rousogenous, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Mihalis Vrekoussis, and Thorsten Warneke
Atmos. Meas. Tech., 15, 3401–3437, https://doi.org/10.5194/amt-15-3401-2022, https://doi.org/10.5194/amt-15-3401-2022, 2022
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We present a new version (v3) of the GOSAT and GOSAT-2 FOCAL products.
In addition to an increased number of XCO2 data, v3 also includes products for XCH4 (full-physics and proxy), XH2O and the relative ratio of HDO to H2O (δD). For GOSAT-2, we also present first XCO and XN2O results. All FOCAL data products show reasonable spatial distribution and temporal variations and agree well with TCCON. Global XN2O maps show a gradient from the tropics to higher latitudes on the order of 15 ppb.
Mark Weber, Carlo Arosio, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, Kleareti Tourpali, John P. Burrows, and Diego Loyola
Atmos. Chem. Phys., 22, 6843–6859, https://doi.org/10.5194/acp-22-6843-2022, https://doi.org/10.5194/acp-22-6843-2022, 2022
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Long-term trends in column ozone have been determined from five merged total ozone datasets spanning the period 1978–2020. We show that ozone recovery due to the decline in stratospheric halogens after the 1990s (as regulated by the Montreal Protocol) is evident outside the tropical region and amounts to half a percent per decade. The ozone recovery in the Northern Hemisphere is however compensated for by the negative long-term trend contribution from atmospheric dynamics since the year 2000.
Nora Mettig, Mark Weber, Alexei Rozanov, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Ryan M. Stauffer, Thierry Leblanc, Gerard Ancellet, Michael J. Newchurch, Shi Kuang, Rigel Kivi, Matthew B. Tully, Roeland Van Malderen, Ankie Piters, Bogumil Kois, René Stübi, and Pavla Skrivankova
Atmos. Meas. Tech., 15, 2955–2978, https://doi.org/10.5194/amt-15-2955-2022, https://doi.org/10.5194/amt-15-2955-2022, 2022
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Vertical ozone profiles from combined spectral measurements in the UV and IR spectral ranges were retrieved by using data from TROPOMI/S5P and CrIS/Suomi-NPP. The vertical resolution and accuracy of the ozone profiles are improved by combining both wavelength ranges compared to retrievals limited to UV or IR spectral data only. The advancement of our TOPAS algorithm for combined measurements is required because in the UV-only retrieval the vertical resolution in the troposphere is very limited.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Carlos Alberti, Qiansi Tu, Frank Hase, Maria V. Makarova, Konstantin Gribanov, Stefani C. Foka, Vyacheslav Zakharov, Thomas Blumenstock, Michael Buchwitz, Christopher Diekmann, Benjamin Ertl, Matthias M. Frey, Hamud Kh. Imhasin, Dmitry V. Ionov, Farahnaz Khosrawi, Sergey I. Osipov, Maximilian Reuter, Matthias Schneider, and Thorsten Warneke
Atmos. Meas. Tech., 15, 2199–2229, https://doi.org/10.5194/amt-15-2199-2022, https://doi.org/10.5194/amt-15-2199-2022, 2022
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Satellite and ground-based observations at high latitudes are much sparser than at low or mid latitudes, which makes direct coincident comparisons between remote-sensing observations more difficult. Therefore, a method of scaling continuous CAMS model data to the ground-based observations is developed and used for creating virtual COCCON observations. These adjusted CAMS data are then used for satellite inter-comparison, showing good agreement in both Peterhof and Yekaterinburg cities.
Kezia Lange, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys., 22, 2745–2767, https://doi.org/10.5194/acp-22-2745-2022, https://doi.org/10.5194/acp-22-2745-2022, 2022
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In this study, we investigated short time variability of NOx emissions and lifetimes on a global scale. We combined 2 years of satellite Sentinel-5P TROPOMI tropospheric NO2 column data with wind data. Fifty NOx sources distributed around the world are analyzed. The retrieved emissions show a clear seasonal dependence. NOx lifetime shows a latitudinal dependence but only a week seasonal dependence. NOx emissions show a clear weekly pattern which in contrast is not visible for NOx lifetimes.
Tobias Küchler, Stefan Noël, Heinrich Bovensmann, John Philip Burrows, Thomas Wagner, Christian Borger, Tobias Borsdorff, and Andreas Schneider
Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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We applied the air-mass-corrected differential optical absorption spectroscopy (AMC-DOAS) method to derive total column water vapour (TCWV) from Sentinel-5P measurements and compared it to independent data sets. The correlation coefficients of typically more than 0.9 and the small deviations up to 2.5 kg m−2 reveal good agreement between our data product and other TCWV data sets. In particular for the different Sentinel-5P water vapour products, the deviations are around 1 kg m−2.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michał Gałkowski, Justyna Swolkień, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys., 21, 17345–17371, https://doi.org/10.5194/acp-21-17345-2021, https://doi.org/10.5194/acp-21-17345-2021, 2021
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Quantification of anthropogenic CH4 emissions remains challenging, but it is essential for near-term climate mitigation strategies. We use airborne remote sensing observations to assess bottom-up estimates of coal mining emissions from one of Europe's largest CH4 emission hot spots located in Poland. The analysis reveals that emissions from small groups of shafts can be disentangled, but caution is advised when comparing observations to commonly reported annual emissions.
Yu-Wen Chen, Yi-Chun Chen, Charles C.-K. Chou, Hui-Ming Hung, Shih-Yu Chang, Lisa Eirenschmalz, Michael Lichtenstern, Helmut Ziereis, Hans Schlager, Greta Stratmann, Katharina Kaiser, Johannes Schneider, Stephan Borrmann, Florian Obersteiner, Eric Förster, Andreas Zahn, Wei-Nai Chen, Po-Hsiung Lin, Shuenn-Chin Chang, Maria Dolores Andrés Hernández, Pao-Kuan Wang, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-788, https://doi.org/10.5194/acp-2021-788, 2021
Preprint withdrawn
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By presenting an approach using EMeRGe-Asia airborne field measurements and surface observations, this study shows that the fraction of OH reactivity due to SO2-OH reaction has a significant correlation with the sulfate concentration. Approximately 30 % of sulfate is produced by SO2-OH reaction. Our results underline the importance of SO2-OH gas-phase oxidation in sulfate formation, and demonstrate that the method can be applied to other regions and under different meteorological conditions.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Nora Mettig, Mark Weber, Alexei Rozanov, Carlo Arosio, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Richard Querel, Thierry Leblanc, Sophie Godin-Beekmann, Rigel Kivi, and Matthew B. Tully
Atmos. Meas. Tech., 14, 6057–6082, https://doi.org/10.5194/amt-14-6057-2021, https://doi.org/10.5194/amt-14-6057-2021, 2021
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TROPOMI is a nadir-viewing satellite that has observed global atmospheric trace gases at unprecedented spatial resolution since 2017. The retrieval of ozone profiles with high accuracy has been demonstrated using the TOPAS (Tikhonov regularised Ozone Profile retrievAl with SCIATRAN) algorithm and applying appropriate spectral corrections to TROPOMI UV data. Ozone profiles from TROPOMI were compared to ozonesonde and lidar profiles, showing an agreement to within 5 % in the stratosphere.
Kai Krause, Folkard Wittrock, Andreas Richter, Stefan Schmitt, Denis Pöhler, Andreas Weigelt, and John P. Burrows
Atmos. Meas. Tech., 14, 5791–5807, https://doi.org/10.5194/amt-14-5791-2021, https://doi.org/10.5194/amt-14-5791-2021, 2021
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Ships are an important source of key pollutants. Usually, these are measured aboard the ship or on the coast using in situ instruments. This study shows how active optical remote sensing can be used to measure ship emissions and how to determine emission rates of individual ships out of those measurements. These emission rates are valuable input for the assessment of the influence of shipping emissions in regions close to the shipping lanes.
Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Mark Weber, Carlo Arosio, Annette Ladstätter-Weißenmayer, and John P. Burrows
Atmos. Meas. Tech., 14, 5771–5789, https://doi.org/10.5194/amt-14-5771-2021, https://doi.org/10.5194/amt-14-5771-2021, 2021
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OMPS/NPP (2012–present) allows obtaining the tropospheric ozone column by combining ozone data from limb and nadir observations from the same instrument platform. In a first step, the retrieval of the total ozone column from the OMPS Nadir Mapper using the weighting function fitting approach (WFFA) is described here. The OMPS total ozone was compared with ground-based and other satellite measurements, showing agreement within 2.5 %.
Lily N. Zhang, Susan Solomon, Kane A. Stone, Jonathan D. Shanklin, Joshua D. Eveson, Steve Colwell, John P. Burrows, Mark Weber, Pieternel F. Levelt, Natalya A. Kramarova, and David P. Haffner
Atmos. Chem. Phys., 21, 9829–9838, https://doi.org/10.5194/acp-21-9829-2021, https://doi.org/10.5194/acp-21-9829-2021, 2021
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In the 1980s, measurements at the British Antarctic Survey station in Halley, Antarctica, led to the discovery of the ozone hole. The Halley total ozone record continues to be uniquely valuable for studies of long-term changes in Antarctic ozone. Environmental conditions in 2017 forced a temporary cessation of operations, leading to a gap in the historic record. We develop and test a method for filling in the Halley record using satellite data and find evidence to further support ozone recovery.
Linlu Mei, Vladimir Rozanov, Christine Pohl, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2757–2780, https://doi.org/10.5194/tc-15-2757-2021, https://doi.org/10.5194/tc-15-2757-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 1 of two companion papers and shows the method description and sensitivity study. The paper investigates the major factors, including the assumptions of snow optical properties, snow particle distribution and atmospheric conditions (cloud and aerosol), impacting snow property retrievals from satellite observation.
Linlu Mei, Vladimir Rozanov, Evelyn Jäkel, Xiao Cheng, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2781–2802, https://doi.org/10.5194/tc-15-2781-2021, https://doi.org/10.5194/tc-15-2781-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 2 of two companion papers and shows the results and validation. The paper performs the new retrieval algorithm on the Sea and Land
Surface Temperature Radiometer (SLSTR) instrument and compares the retrieved snow properties with ground-based measurements, aircraft measurements and other satellite products.
Daniel Zawada, Ghislain Franssens, Robert Loughman, Antti Mikkonen, Alexei Rozanov, Claudia Emde, Adam Bourassa, Seth Dueck, Hannakaisa Lindqvist, Didier Ramon, Vladimir Rozanov, Emmanuel Dekemper, Erkki Kyrölä, John P. Burrows, Didier Fussen, and Doug Degenstein
Atmos. Meas. Tech., 14, 3953–3972, https://doi.org/10.5194/amt-14-3953-2021, https://doi.org/10.5194/amt-14-3953-2021, 2021
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Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, James R. Podolske, David F. Pollard, Mahesh Kumar Sha, Kei Shiomi, Ralf Sussmann, Yao Té, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech., 14, 3837–3869, https://doi.org/10.5194/amt-14-3837-2021, https://doi.org/10.5194/amt-14-3837-2021, 2021
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We present the first GOSAT and GOSAT-2 XCO2 data derived with the FOCAL retrieval algorithm. Comparisons of the GOSAT-FOCAL product with other data reveal long-term agreement within about 1 ppm over 1 decade, differences in seasonal variations of about 0.5 ppm, and a mean regional bias to ground-based TCCON data of 0.56 ppm with a mean scatter of 1.89 ppm. GOSAT-2-FOCAL data are preliminary only, but first comparisons show that they compare well with the GOSAT-FOCAL results and TCCON.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
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The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Ashique Vellalassery, Dhanyalekshmi Pillai, Julia Marshall, Christoph Gerbig, Michael Buchwitz, Oliver Schneising, and Aparnna Ravi
Atmos. Chem. Phys., 21, 5393–5414, https://doi.org/10.5194/acp-21-5393-2021, https://doi.org/10.5194/acp-21-5393-2021, 2021
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We investigate factors contributing to the severe and persistent air quality degradation in northern India that has worsened during every winter over the last decade. This is achieved by implementing atmospheric modelling and using recently available Sentinel-5 P satellite data for carbon monoxide. We see a minimal role of biomass burning, except for the state of Punjab. The aim is to focus on residential and industrial emission reduction strategies to tackle air pollution over northern India.
Michael Buchwitz, Maximilian Reuter, Stefan Noël, Klaus Bramstedt, Oliver Schneising, Michael Hilker, Blanca Fuentes Andrade, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hartmut Boesch, Lianghai Wu, Jochen Landgraf, Ilse Aben, Christian Retscher, Christopher W. O'Dell, and David Crisp
Atmos. Meas. Tech., 14, 2141–2166, https://doi.org/10.5194/amt-14-2141-2021, https://doi.org/10.5194/amt-14-2141-2021, 2021
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The COVID-19 pandemic resulted in reduced anthropogenic carbon dioxide (CO2) emissions during 2020 in large parts of the world. We have used a small ensemble of satellite retrievals of column-averaged CO2 (XCO2) to find out if a regional-scale reduction of atmospheric CO2 can be detected from space. We focus on East China and show that it is challenging to reliably detect and to accurately quantify the emission reduction, which only results in regional XCO2 reductions of about 0.1–0.2 ppm.
Jakob Borchardt, Konstantin Gerilowski, Sven Krautwurst, Heinrich Bovensmann, Andrew K. Thorpe, David R. Thompson, Christian Frankenberg, Charles E. Miller, Riley M. Duren, and John Philip Burrows
Atmos. Meas. Tech., 14, 1267–1291, https://doi.org/10.5194/amt-14-1267-2021, https://doi.org/10.5194/amt-14-1267-2021, 2021
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The AVIRIS-NG hyperspectral imager has been used successfully to identify and quantify anthropogenic methane sources utilizing different retrieval and inversion methods. Here, we examine the adaption and application of the WFM-DOAS algorithm to AVIRIS-NG measurements to retrieve local methane column enhancements, compare the results with other retrievals, and quantify the uncertainties resulting from the retrieval method. Additionally, we estimate emissions from five detected methane plumes.
Soheila Jafariserajehlou, Vladimir V. Rozanov, Marco Vountas, Charles K. Gatebe, and John P. Burrows
Atmos. Meas. Tech., 14, 369–389, https://doi.org/10.5194/amt-14-369-2021, https://doi.org/10.5194/amt-14-369-2021, 2021
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In this work, we study retrieval of snow grain morphologies and their impact on the reflectance in a coupled snow–atmosphere system. We present a sensitivity study to highlight the importance of having adequate information about snow and atmosphere. A novel two-stage algorithm for retrieving the size and shape of snow grains is presented. The reflectance simulation results are compared to that of airborne measurements; high correlations of 0.98 at IR and 0.88–0.98 at VIS are achieved.
Maximilian Reuter, Heinrich Bovensmann, Michael Buchwitz, Jakob Borchardt, Sven Krautwurst, Konstantin Gerilowski, Matthias Lindauer, Dagmar Kubistin, and John P. Burrows
Atmos. Meas. Tech., 14, 153–172, https://doi.org/10.5194/amt-14-153-2021, https://doi.org/10.5194/amt-14-153-2021, 2021
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CO2 measurements from a small unmanned aircraft system (sUAS) can provide a cost-effective way to complement and validate satellite-based measurements of anthropogenic CO2 emissions. We introduce an sUAS which is capable of determining atmospheric CO2 mass fluxes from its own sensor data. We show results of validation flights at the ICOS atmospheric station in Steinkimmen and from demonstration flights downwind a CO2-emitting natural gas processing facility.
Bettina K. Gier, Michael Buchwitz, Maximilian Reuter, Peter M. Cox, Pierre Friedlingstein, and Veronika Eyring
Biogeosciences, 17, 6115–6144, https://doi.org/10.5194/bg-17-6115-2020, https://doi.org/10.5194/bg-17-6115-2020, 2020
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Models from Coupled Model Intercomparison Project (CMIP) phases 5 and 6 are compared to a satellite data product of column-averaged CO2 mole fractions (XCO2). The previously believed discrepancy of the negative trend in seasonal cycle amplitude in the satellite product, which is not seen in in situ data nor in the models, is attributed to a sampling characteristic. Furthermore, CMIP6 models are shown to have made progress in reproducing the observed XCO2 time series compared to CMIP5.
Yilong Wang, Grégoire Broquet, François-Marie Bréon, Franck Lespinas, Michael Buchwitz, Maximilian Reuter, Yasjka Meijer, Armin Loescher, Greet Janssens-Maenhout, Bo Zheng, and Philippe Ciais
Geosci. Model Dev., 13, 5813–5831, https://doi.org/10.5194/gmd-13-5813-2020, https://doi.org/10.5194/gmd-13-5813-2020, 2020
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Chem. Phys., 20, 12285–12312, https://doi.org/10.5194/acp-20-12285-2020, https://doi.org/10.5194/acp-20-12285-2020, 2020
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In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
Ilias Bougoudis, Anne-Marlene Blechschmidt, Andreas Richter, Sora Seo, John Philip Burrows, Nicolas Theys, and Annette Rinke
Atmos. Chem. Phys., 20, 11869–11892, https://doi.org/10.5194/acp-20-11869-2020, https://doi.org/10.5194/acp-20-11869-2020, 2020
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A 22-year (1996 to 2017) consistent Arctic tropospheric BrO dataset derived from four satellite remote sensing instruments is presented. An increase in tropospheric BrO VCDs over this period, and especially during polar springs, can be seen. Comparisons of tropospheric BrO VCDs with first-year sea ice reveal a moderate spatial and temporal correlation between the two, suggesting that the increase in first-year sea ice in the Arctic has an impact on tropospheric BrO abundancies.
Stefan Noël, Klaus Bramstedt, Alexei Rozanov, Elizaveta Malinina, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 13, 5643–5666, https://doi.org/10.5194/amt-13-5643-2020, https://doi.org/10.5194/amt-13-5643-2020, 2020
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A new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion-peeling method is presented. The resulting extinctions at 452, 525 and 750 nm compare well with other limb and occultation data from, e.g. SAGE and SCIAMACHY, but show small oscillating features which vanish in monthly anomalies. Major volcanic eruptions, polar stratospheric clouds and influences of the quasi-biennial oscillation can be identified in the time series.
Hirofumi Ohyama, Isamu Morino, Voltaire A. Velazco, Theresa Klausner, Gerry Bagtasa, Matthäus Kiel, Matthias Frey, Akihiro Hori, Osamu Uchino, Tsuneo Matsunaga, Nicholas M. Deutscher, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Sally E. Pusede, Alina Fiehn, Anke Roiger, Michael Lichtenstern, Hans Schlager, Pao K. Wang, Charles C.-K. Chou, Maria Dolores Andrés-Hernández, and John P. Burrows
Atmos. Meas. Tech., 13, 5149–5163, https://doi.org/10.5194/amt-13-5149-2020, https://doi.org/10.5194/amt-13-5149-2020, 2020
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Column-averaged dry-air mole fractions of CO2 and CH4 measured by a solar viewing portable Fourier transform spectrometer (EM27/SUN) were validated with in situ profile data obtained during the transfer flights of two aircraft campaigns. Atmospheric dynamical properties based on ERA5 and WRF-Chem were used as criteria for selecting the best aircraft profiles for the validation. The resulting air-mass-independent correction factors for the EM27/SUN data were 0.9878 for CO2 and 0.9829 for CH4.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Steffen Vanselow, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 20, 9169–9182, https://doi.org/10.5194/acp-20-9169-2020, https://doi.org/10.5194/acp-20-9169-2020, 2020
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The switch from the use of coal to natural gas or oil for energy generation potentially reduces the impact on global warming due to lower CO2 emissions with the same energy content. However, this climate benefit is offset by fugitive methane emissions during the production and distribution process. We quantify emission and leakage rates relative to production for several large production regions based on satellite observations to evaluate the climate footprint of the gas and oil industry.
Tina Hilbig, Klaus Bramstedt, Mark Weber, John P. Burrows, and Matthijs Krijger
Atmos. Meas. Tech., 13, 3893–3907, https://doi.org/10.5194/amt-13-3893-2020, https://doi.org/10.5194/amt-13-3893-2020, 2020
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One of the main limitations for long-term space-based measurements is
instrument degradation. We present an optimisation of the
degradation correction approach (Krijger et al. 2014) for SCIAMACHY
on-board Envisat, focusing on the improvement of the solar spectral
irradiance data. The main achievement of this study is the
successful integration of SCIAMACHY’s internal white light source
(WLS) into the existing degradation model and the
characterisation of WLS ageing in space.
Steven Compernolle, Tijl Verhoelst, Gaia Pinardi, José Granville, Daan Hubert, Arno Keppens, Sander Niemeijer, Bruno Rino, Alkis Bais, Steffen Beirle, Folkert Boersma, John P. Burrows, Isabelle De Smedt, Henk Eskes, Florence Goutail, François Hendrick, Alba Lorente, Andrea Pazmino, Ankie Piters, Enno Peters, Jean-Pierre Pommereau, Julia Remmers, Andreas Richter, Jos van Geffen, Michel Van Roozendael, Thomas Wagner, and Jean-Christopher Lambert
Atmos. Chem. Phys., 20, 8017–8045, https://doi.org/10.5194/acp-20-8017-2020, https://doi.org/10.5194/acp-20-8017-2020, 2020
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Tropospheric and stratospheric NO2 columns from the OMI QA4ECV NO2 satellite product are validated by comparison with ground-based measurements at 11 sites. The OMI stratospheric column has a small negative bias, and the OMI tropospheric column has a stronger negative bias relative to the ground-based data. Discrepancies are attributed to comparison errors (e.g. difference in horizontal smoothing) and measurement errors (e.g. clouds, aerosols, vertical smoothing and a priori profile assumptions).
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, and John Philip Burrows
Atmos. Meas. Tech., 13, 2577–2600, https://doi.org/10.5194/amt-13-2577-2020, https://doi.org/10.5194/amt-13-2577-2020, 2020
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The accurate measurement of peroxy radicals is essential for understanding the chemistry of air masses probed in the free troposphere. The PeRCEAS instrument has been designed, developed and thoroughly characterised for the measurement of the total sum of peroxy radicals (RO2*) aboard airborne platforms. Parameters expected to affect the precision and accuracy of the measurement have been investigated in detail.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 20, 3317–3332, https://doi.org/10.5194/acp-20-3317-2020, https://doi.org/10.5194/acp-20-3317-2020, 2020
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As a consequence of climate change, droughts in California are occurring more often, providing ample fuel for destructive wildfires. The associated smoke is reducing air quality as it contains pollutants considered harmful to public health and the environment such as carbon monoxide (CO). We analyse the statewide distribution of CO during the first days of two specific wildfires using satellite measurements and assess the corresponding air quality burden in major Californian cities.
Anne-Marlene Blechschmidt, Joaquim Arteta, Adriana Coman, Lyana Curier, Henk Eskes, Gilles Foret, Clio Gielen, Francois Hendrick, Virginie Marécal, Frédérik Meleux, Jonathan Parmentier, Enno Peters, Gaia Pinardi, Ankie J. M. Piters, Matthieu Plu, Andreas Richter, Arjo Segers, Mikhail Sofiev, Álvaro M. Valdebenito, Michel Van Roozendael, Julius Vira, Tim Vlemmix, and John P. Burrows
Atmos. Chem. Phys., 20, 2795–2823, https://doi.org/10.5194/acp-20-2795-2020, https://doi.org/10.5194/acp-20-2795-2020, 2020
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MAX-DOAS tropospheric NO2 vertical column retrievals from a set of European measurement stations are compared to regional air quality models which contribute to the operational Copernicus Atmosphere Monitoring Service (CAMS). Correlations are on the order of 35 %–75 %; large differences occur for individual pollution plumes. The results demonstrate that future model development needs to concentrate on improving representation of diurnal cycles and associated temporal scalings.
Leonardo M. A. Alvarado, Andreas Richter, Mihalis Vrekoussis, Andreas Hilboll, Anna B. Kalisz Hedegaard, Oliver Schneising, and John P. Burrows
Atmos. Chem. Phys., 20, 2057–2072, https://doi.org/10.5194/acp-20-2057-2020, https://doi.org/10.5194/acp-20-2057-2020, 2020
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We present CHOCHO and HCHO columns retrieved from measurements by TROPOMI. Elevated amounts of CHOCHO and HCHO are observed during the fire season in BC, Canada, where a large number of fires occurred in 2018. CHOCHO and HCHO plumes from individual fires are observed in air masses travelling over distances of up to 1500 km. Comparison with FLEXPART simulations with different lifetimes shows that effective lifetimes of 20 h and more are needed to explain the observations.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Stefan Noël, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Antonio Di Noia, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Lianghai Wu, Otto P. Hasekamp, Ilse Aben, Akihiko Kuze, Hiroshi Suto, Kei Shiomi, Yukio Yoshida, Isamu Morino, David Crisp, Christopher W. O'Dell, Justus Notholt, Christof Petri, Thorsten Warneke, Voltaire A. Velazco, Nicholas M. Deutscher, David W. T. Griffith, Rigel Kivi, David F. Pollard, Frank Hase, Ralf Sussmann, Yao V. Té, Kimberly Strong, Sébastien Roche, Mahesh K. Sha, Martine De Mazière, Dietrich G. Feist, Laura T. Iraci, Coleen M. Roehl, Christian Retscher, and Dinand Schepers
Atmos. Meas. Tech., 13, 789–819, https://doi.org/10.5194/amt-13-789-2020, https://doi.org/10.5194/amt-13-789-2020, 2020
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We present new satellite-derived data sets of atmospheric carbon dioxide (CO2) and methane (CH4). The data products are column-averaged dry-air mole fractions of CO2 and CH4, denoted XCO2 and XCH4. The products cover the years 2003–2018 and are merged Level 2 (satellite footprints) and merged Level 3 (gridded at monthly time and 5° x 5° spatial resolution) products obtained from combining several individual sensor products. We present the merging algorithms and product validation results.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, John P. Burrows, Tobias Borsdorff, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Christian Hermans, Laura T. Iraci, Rigel Kivi, Jochen Landgraf, Isamu Morino, Justus Notholt, Christof Petri, David F. Pollard, Sébastien Roche, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Voltaire A. Velazco, Thorsten Warneke, and Debra Wunch
Atmos. Meas. Tech., 12, 6771–6802, https://doi.org/10.5194/amt-12-6771-2019, https://doi.org/10.5194/amt-12-6771-2019, 2019
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We introduce an algorithm that is used to simultaneously derive the abundances of the important atmospheric constituents carbon monoxide and methane from the TROPOMI instrument onboard the Sentinel-5 Precursor satellite, which enables the determination of both gases with an unprecedented level of detail on a global scale. The quality of the resulting data sets is assessed and the first results are presented.
André Seyler, Andreas C. Meier, Folkard Wittrock, Lisa Kattner, Barbara Mathieu-Üffing, Enno Peters, Andreas Richter, Thomas Ruhtz, Anja Schönhardt, Stefan Schmolke, and John P. Burrows
Atmos. Meas. Tech., 12, 5959–5977, https://doi.org/10.5194/amt-12-5959-2019, https://doi.org/10.5194/amt-12-5959-2019, 2019
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This study describes a novel application of an
onion-peelingapproach to MAX-DOAS measurements of shipping emissions to study the inhomogeneous NO2 field above a shipping lane. It is shown how the method can be used to derive the approximate plume positions in the observed area, and, by using a simple Gaussian plume model, to calculate in-plume NO2 volume mixing ratios. For validation, a comparison to airborne imaging DOAS measurements during the NOSE campaign in July 2013 is included.
Lisa K. Behrens, Andreas Hilboll, Andreas Richter, Enno Peters, Leonardo M. A. Alvarado, Anna B. Kalisz Hedegaard, Folkard Wittrock, John P. Burrows, and Mihalis Vrekoussis
Atmos. Chem. Phys., 19, 10257–10278, https://doi.org/10.5194/acp-19-10257-2019, https://doi.org/10.5194/acp-19-10257-2019, 2019
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MAX-DOAS measurements were conducted on the research vessel Maria S. Merian during a cruise from the Azores to South Africa in October 2016. The measurements indicate enhanced levels of HCHO and CHOCHO over the remote Atlantic Ocean, which is unexpected due to their short lifetime. Precursors of these gases or gas–aerosol combinations might be transported. Model simulations indicate potential source regions over the African continent, probably related to biomass burning or biogenic emissions.
Enno Peters, Mareike Ostendorf, Tim Bösch, André Seyler, Anja Schönhardt, Stefan F. Schreier, Jeroen Sebastiaan Henzing, Folkard Wittrock, Andreas Richter, Mihalis Vrekoussis, and John P. Burrows
Atmos. Meas. Tech., 12, 4171–4190, https://doi.org/10.5194/amt-12-4171-2019, https://doi.org/10.5194/amt-12-4171-2019, 2019
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A novel imaging-DOAS instrument (IMPACT) is presented for measurements of nitrogen dioxide (NO2) in the atmosphere. The instrument combines full-azimuthal pointing (360°) with a large vertical coverage (40°). Complete panoramic scans and vertical NO2 profiles around the measurement site are acquired at a temporal resolution of 15 min. In addition, information about the aerosol phase function is retrieved from O4 slant columns along multiple almucantar scans measured simultaneously by IMPACT.
Dan Weaver, Kimberly Strong, Kaley A. Walker, Chris Sioris, Matthias Schneider, C. Thomas McElroy, Holger Vömel, Michael Sommer, Katja Weigel, Alexei Rozanov, John P. Burrows, William G. Read, Evan Fishbein, and Gabriele Stiller
Atmos. Meas. Tech., 12, 4039–4063, https://doi.org/10.5194/amt-12-4039-2019, https://doi.org/10.5194/amt-12-4039-2019, 2019
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This work assesses water vapour profiles acquired by Atmospheric Chemistry Experiment (ACE) satellite instruments in the upper troposphere and lower stratosphere (UTLS) using comparisons to radiosondes and ground-based Fourier transform infrared spectrometer measurements acquired at a Canadian high Arctic measurement site in Eureka, Nunavut. Additional comparisons are made between these Eureka measurements and other water vapour satellite datasets for context, including AIRS, MLS, and others.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Sven Krautwurst, Christopher W. O'Dell, Andreas Richter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 19, 9371–9383, https://doi.org/10.5194/acp-19-9371-2019, https://doi.org/10.5194/acp-19-9371-2019, 2019
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The quantification of anthropogenic emissions with current CO2 satellite sensors is difficult, but NO2 is co-emitted, making it a suitable tracer of recently emitted CO2. We analyze enhancements of CO2 and NO2 observed by OCO-2 and S5P and estimate the CO2 plume cross-sectional fluxes that we compare with emission databases. Our results demonstrate the usefulness of simultaneous satellite observations of CO2 and NO2 as envisaged for the European Copernicus anthropogenic CO2 monitoring mission
Hyeong-Ahn Kwon, Rokjin J. Park, Gonzalo González Abad, Kelly Chance, Thomas P. Kurosu, Jhoon Kim, Isabelle De Smedt, Michel Van Roozendael, Enno Peters, and John Burrows
Atmos. Meas. Tech., 12, 3551–3571, https://doi.org/10.5194/amt-12-3551-2019, https://doi.org/10.5194/amt-12-3551-2019, 2019
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The Geostationary Environment Monitoring Spectrometer (GEMS) will be launched by South Korea in 2019, and it will measure radiances ranging from 300 to 500 nm every hour with a fine spatial resolution of 7 km x 8 km over Seoul in South Korea to monitor column concentrations of air pollutants including O3, NO2, SO2, and HCHO, as well as aerosol optical properties. This paper describes a GEMS formaldehyde retrieval algorithm including a number of sensitivity tests for algorithm evaluation.
Elizaveta Malinina, Alexei Rozanov, Landon Rieger, Adam Bourassa, Heinrich Bovensmann, John P. Burrows, and Doug Degenstein
Atmos. Meas. Tech., 12, 3485–3502, https://doi.org/10.5194/amt-12-3485-2019, https://doi.org/10.5194/amt-12-3485-2019, 2019
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This paper covers the problems related to the derivation of aerosol extinction coefficients and Ångström exponents from space-borne instruments working in limb and occultation viewing geometries. Aerosol extinction coefficients and Ångström exponents were calculated from the SCIAMACHY aerosol particle size data set. The results were compared with the data from SAGE II and OSIRIS. The Ångström exponent in the tropical regions and its dependency on particle size parameters are discussed.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Meas. Tech., 12, 2913–2932, https://doi.org/10.5194/amt-12-2913-2019, https://doi.org/10.5194/amt-12-2913-2019, 2019
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TROPOMI on board the Copernicus Sentinel-5 Precursor platform can measure various atmospheric compositions at high spatial resolution and improved spectral resolution compared to its predecessors. Bromine monoxide (BrO) is one of the gases that can be derived from the measured radiances of TROPOMI using the differential optical absorption spectroscopy method. In this paper, we present the first retrieval results of BrO column amounts from TROPOMI observations on global and regional scales.
Stefan Lossow, Farahnaz Khosrawi, Michael Kiefer, Kaley A. Walker, Jean-Loup Bertaux, Laurent Blanot, James M. Russell, Ellis E. Remsberg, John C. Gille, Takafumi Sugita, Christopher E. Sioris, Bianca M. Dinelli, Enzo Papandrea, Piera Raspollini, Maya García-Comas, Gabriele P. Stiller, Thomas von Clarmann, Anu Dudhia, William G. Read, Gerald E. Nedoluha, Robert P. Damadeo, Joseph M. Zawodny, Katja Weigel, Alexei Rozanov, Faiza Azam, Klaus Bramstedt, Stefan Noël, John P. Burrows, Hideo Sagawa, Yasuko Kasai, Joachim Urban, Patrick Eriksson, Donal P. Murtagh, Mark E. Hervig, Charlotta Högberg, Dale F. Hurst, and Karen H. Rosenlof
Atmos. Meas. Tech., 12, 2693–2732, https://doi.org/10.5194/amt-12-2693-2019, https://doi.org/10.5194/amt-12-2693-2019, 2019
Stefan F. Schreier, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys., 19, 5853–5879, https://doi.org/10.5194/acp-19-5853-2019, https://doi.org/10.5194/acp-19-5853-2019, 2019
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In this case stuy, we have coupled ground-based remote-sensing measurements with surface in situ measurements to investigate NO2 distributions in the planetary boundary layer in the Viennese metropolitan area. We find that the application of a novel linear regression analysis for the conversion of tropospheric NO2 vertical columns into near-surface NO2 mixing ratios is promising and thus the method needs to be further explored and tested on satellite observations in future studies.
Carlo Arosio, Alexei Rozanov, Elizaveta Malinina, Mark Weber, and John P. Burrows
Atmos. Meas. Tech., 12, 2423–2444, https://doi.org/10.5194/amt-12-2423-2019, https://doi.org/10.5194/amt-12-2423-2019, 2019
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The aim of this study is the merging of stratospheric ozone profiles from three satellite data sets. The merged time series is used to compute long-term changes as a function of altitude, latitude and longitude to study the evolution of the ozone layer over 1985–2018. During the last 16 years we found positive trends in the upper stratosphere at mid latitudes, a large variability of the ozone changes as a function of longitude and a fluctuation in the tropical middle stratospheric trend.
Soheila Jafariserajehlou, Linlu Mei, Marco Vountas, Vladimir Rozanov, John P. Burrows, and Rainer Hollmann
Atmos. Meas. Tech., 12, 1059–1076, https://doi.org/10.5194/amt-12-1059-2019, https://doi.org/10.5194/amt-12-1059-2019, 2019
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We developed a new algorithm for cloud identification over the Arctic. This algorithm called ASCIA, utilizes time-series measurements of Advanced Along-Track Scanning Radiometer (AATSR) on Envisat and Sea and Land Surface Temperature Radiometer (SLSTR) on Sentinel-3A and -3B.
The data product of ASCIA is compared with three satellite products: ASCIA shows an improved performance compared to them. We validated ASCIA by ground-based measurements and a promising agreement is achieved.
Stefan Bender, Miriam Sinnhuber, Patrick J. Espy, and John P. Burrows
Atmos. Chem. Phys., 19, 2135–2147, https://doi.org/10.5194/acp-19-2135-2019, https://doi.org/10.5194/acp-19-2135-2019, 2019
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We present an empirical model for nitric oxide (NO) in the mesosphere (60–90 km) derived from SCIAMACHY limb scan data. Our model relates the daily (longitudinally) averaged NO number densities from SCIAMACHY as a function of geomagnetic latitude to the solar Lyman-alpha and the geomagnetic AE indices. We use a non-linear regression model, incorporating a finite and seasonally varying lifetime for the geomagnetically induced NO.
Evgenia Galytska, Alexey Rozanov, Martyn P. Chipperfield, Sandip. S. Dhomse, Mark Weber, Carlo Arosio, Wuhu Feng, and John P. Burrows
Atmos. Chem. Phys., 19, 767–783, https://doi.org/10.5194/acp-19-767-2019, https://doi.org/10.5194/acp-19-767-2019, 2019
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In this study we analysed ozone changes in the tropical mid-stratosphere as observed by the SCIAMACHY instrument during 2004–2012. We used simulations from TOMCAT model with different chemical and dynamical forcings to reveal primary causes of ozone changes. We also considered measured NO2 and modelled NOx, NOx, and N2O data. With modelled AoA data we identified seasonal changes in the upwelling speed and explained how those changes affect N2O chemistry which leads to observed ozone changes.
Tim Bösch, Vladimir Rozanov, Andreas Richter, Enno Peters, Alexei Rozanov, Folkard Wittrock, Alexis Merlaud, Johannes Lampel, Stefan Schmitt, Marijn de Haij, Stijn Berkhout, Bas Henzing, Arnoud Apituley, Mirjam den Hoed, Jan Vonk, Martin Tiefengraber, Moritz Müller, and John Philip Burrows
Atmos. Meas. Tech., 11, 6833–6859, https://doi.org/10.5194/amt-11-6833-2018, https://doi.org/10.5194/amt-11-6833-2018, 2018
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A new MAX-DOAS profiling algorithm for aerosols and trace
gases was developed.
The performance of this novel algorithm was tested with the help of
synthetic data and measurements from the CINDI-2 campaign in Cabauw, the
Netherlands, in 2016.
Michael Buchwitz, Maximilian Reuter, Oliver Schneising, Stefan Noël, Bettina Gier, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Akihiko Kuze, Hiroshi Suto, Yukio Yoshida, David Crisp, and Christopher O'Dell
Atmos. Chem. Phys., 18, 17355–17370, https://doi.org/10.5194/acp-18-17355-2018, https://doi.org/10.5194/acp-18-17355-2018, 2018
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We present a new satellite data set of column-averaged mixing ratios of carbon dioxide (CO2), which covers the time period 2003 to 2016. We used this data set to compute annual mean atmospheric CO2 growth rates. We show that the growth rate is highest during 2015 and 2016 despite nearly constant CO2 emissions from fossil fuel burning in recent years. The high growth rates are attributed to year 2015-2016 El Nino episodes. We present correlations with fossil fuel emissions and ENSO indices.
Farahnaz Khosrawi, Stefan Lossow, Gabriele P. Stiller, Karen H. Rosenlof, Joachim Urban, John P. Burrows, Robert P. Damadeo, Patrick Eriksson, Maya García-Comas, John C. Gille, Yasuko Kasai, Michael Kiefer, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Alexei Rozanov, Christopher E. Sioris, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 11, 4435–4463, https://doi.org/10.5194/amt-11-4435-2018, https://doi.org/10.5194/amt-11-4435-2018, 2018
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Time series of stratospheric and lower mesospheric water vapour using 33 data sets from 15 satellite instruments were compared in the framework of the second SPARC water vapour assessment. We find that most data sets can be considered in observational and modelling studies addressing, e.g. stratospheric and lower mesospheric water vapour variability and trends if data-set-specific characteristics (e.g. a drift) and restrictions (e.g. temporal and spatial coverage) are taken into account.
Landon A. Rieger, Elizaveta P. Malinina, Alexei V. Rozanov, John P. Burrows, Adam E. Bourassa, and Doug A. Degenstein
Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, https://doi.org/10.5194/amt-11-3433-2018, 2018
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This paper compares aerosol extinction records from two limb scattering instruments, OSIRIS and SCIAMACHY, to that from the occultation instrument SAGE II. Differences are investigated through modelling and retrieval studies and important sources of systematic errors are quantified. It is found that the largest biases come from uncertainties in the aerosol size distribution and the aerosol particle concentration at altitudes above 30 km.
Lisa K. Behrens, Andreas Hilboll, Andreas Richter, Enno Peters, Henk Eskes, and John P. Burrows
Atmos. Meas. Tech., 11, 2769–2795, https://doi.org/10.5194/amt-11-2769-2018, https://doi.org/10.5194/amt-11-2769-2018, 2018
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We developed a novel NO2 DOAS retrieval for the GOME-2A instrument in the UV spectral range, which is compared with a NO2 retrieval in the visible and model values. Regions representative for both anthropogenic and biomass burning NO2 pollution are investigated. Anthropogenic air pollution is mostly located in the boundary layer close to the surface. In contrast, biomass burning NO2 is often uplifted into elevated layers.
Carlo Arosio, Alexei Rozanov, Elizaveta Malinina, Kai-Uwe Eichmann, Thomas von Clarmann, and John P. Burrows
Atmos. Meas. Tech., 11, 2135–2149, https://doi.org/10.5194/amt-11-2135-2018, https://doi.org/10.5194/amt-11-2135-2018, 2018
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This paper describes the development of a retrieval algorithm at the University of Bremen which derives stratospheric ozone profiles from limb observations performed by the OMPS satellite instrument. Here we present the implementation of the algorithm and the validation of our results (1 year of data against independent satellite and ground-based measurements). Good agreement is generally found between 20 and 55 km, mostly within 10 % at all latitudes.
Evgenia Galytska, Vassyl Danylevsky, René Hommel, and John P. Burrows
Atmos. Meas. Tech., 11, 2101–2118, https://doi.org/10.5194/amt-11-2101-2018, https://doi.org/10.5194/amt-11-2101-2018, 2018
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This research assesses the influence of biomass burning during forest fires throughout summer 2010 on aerosol load over Ukraine, the European territory of Russia (ETR) and Eastern Europe. We apply and compare ground-based and satellite measurements to determine aerosol content, dynamics, and properties. With the application of modeling techniques (HYSPLIT), we show that the maximum AOD in August 2010 over Ukraine was caused by particle transport from the forest fires in the ETR.
Elizaveta Malinina, Alexei Rozanov, Vladimir Rozanov, Patricia Liebing, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 11, 2085–2100, https://doi.org/10.5194/amt-11-2085-2018, https://doi.org/10.5194/amt-11-2085-2018, 2018
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Stratospheric aerosols play an important role in climate change. This paper presents the retrieval algorithm of two aerosol particle size distribution parameters in the stratosphere from remote sensing instruments. A unique data set was created by implementing this algorithm on SCIAMACHY limb measurements. The general behaviour of the aerosol particle size parameters was revealed. Comparison of the retrieved parameters with another instrument showed good agreement.
Stefan Noël, Katja Weigel, Klaus Bramstedt, Alexei Rozanov, Mark Weber, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 18, 4463–4476, https://doi.org/10.5194/acp-18-4463-2018, https://doi.org/10.5194/acp-18-4463-2018, 2018
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The combined analysis of stratospheric methane and water vapour data derived from SCIAMACHY solar occultation measurements shows the expected anti-correlation and a clear temporal variation related to waves in equatorial zonal winds. Above about 20 km most of the additional water vapour is attributed to the oxidation of methane. The SCIAMACHY data confirm that at lower altitudes water vapour and methane are transported from the tropics to higher latitudes.
Linlu Mei, Vladimir Rozanov, Marco Vountas, John P. Burrows, and Andreas Richter
Atmos. Chem. Phys., 18, 2511–2523, https://doi.org/10.5194/acp-18-2511-2018, https://doi.org/10.5194/acp-18-2511-2018, 2018
Mark Weber, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, John P. Burrows, Craig S. Long, and Diego Loyola
Atmos. Chem. Phys., 18, 2097–2117, https://doi.org/10.5194/acp-18-2097-2018, https://doi.org/10.5194/acp-18-2097-2018, 2018
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This paper commemorates the 30-year anniversary of the initial signing of the Montreal Protocol (MP) on substances that deplete the ozone layer. The MP is so far successful in reducing ozone-depleting substances, and total ozone decline was successfully stopped by the late 1990s. Total ozone levels have been mostly stable since then. In some regions, barely significant upward trends are observed that suggest an emergence into the expected ozone recovery phase.
Thomas Krings, Bruno Neininger, Konstantin Gerilowski, Sven Krautwurst, Michael Buchwitz, John P. Burrows, Carsten Lindemann, Thomas Ruhtz, Dirk Schüttemeyer, and Heinrich Bovensmann
Atmos. Meas. Tech., 11, 721–739, https://doi.org/10.5194/amt-11-721-2018, https://doi.org/10.5194/amt-11-721-2018, 2018
Grégoire Broquet, François-Marie Bréon, Emmanuel Renault, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Frédéric Chevallier, Lin Wu, and Philippe Ciais
Atmos. Meas. Tech., 11, 681–708, https://doi.org/10.5194/amt-11-681-2018, https://doi.org/10.5194/amt-11-681-2018, 2018
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This study assesses the potential of space-borne imagery of CO2 atmospheric concentrations for monitoring the emissions from the Paris area. Such imagery could be provided by European and American missions in the next decade. It highlights the difficulty to improve current knowledge on CO2 emissions for urban areas with CO2 observations from satellites, and calls for more technological innovations in the remote sensing of CO2 and in the models that exploit it.
Amirmahdi Zarboo, Stefan Bender, John P. Burrows, Johannes Orphal, and Miriam Sinnhuber
Atmos. Meas. Tech., 11, 473–487, https://doi.org/10.5194/amt-11-473-2018, https://doi.org/10.5194/amt-11-473-2018, 2018
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We present the retrieved volume emission rates (VERs) from the airglow of both the daytime and twilight O2(1Σ) band and O2(1Δ) band emissions in the mesosphere and lower thermosphere (MLT). We have investigated the daily mean latitudinal distributions and the time series of the retrieved VER in the altitude range from 53 to 149 km. These observations provide information about the chemistry and dynamics and can be used to infer ozone, solar heating rates, and temperature in the MLT.
Patricia Liebing, Matthijs Krijger, Ralph Snel, Klaus Bramstedt, Stefan Noël, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 11, 265–289, https://doi.org/10.5194/amt-11-265-2018, https://doi.org/10.5194/amt-11-265-2018, 2018
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This article describes a method to determine the polarization sensitivity of SCIAMACHY, a spectrometer on Envisat, from in-orbit data. Polarization is a preference of a direction in which light oscillates, and many optical instruments suffer from a dependence of their measured signals on this. To measure and correct for this effect, a statistical analysis of in-flight data combined with a model of the atmosphere and the instrument was performed, showing that the instrument changed after launch.
Sven Krautwurst, Konstantin Gerilowski, Haflidi H. Jonsson, David R. Thompson, Richard W. Kolyer, Laura T. Iraci, Andrew K. Thorpe, Markus Horstjann, Michael Eastwood, Ira Leifer, Samuel A. Vigil, Thomas Krings, Jakob Borchardt, Michael Buchwitz, Matthew M. Fladeland, John P. Burrows, and Heinrich Bovensmann
Atmos. Meas. Tech., 10, 3429–3452, https://doi.org/10.5194/amt-10-3429-2017, https://doi.org/10.5194/amt-10-3429-2017, 2017
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This study investigates a subset of data collected during the CO2 and Methane EXperiment (COMEX) in 2014. It focuses on airborne measurements to quantify the emissions from landfills in the Los Angeles Basin. Airborne remote sensing data have been used to estimate the emission rate of one particular landfill on four different days. The results have been compared to airborne in situ measurements. Airborne imaging spectroscopy has been used to identify emission hotspots across the landfill.
André Seyler, Folkard Wittrock, Lisa Kattner, Barbara Mathieu-Üffing, Enno Peters, Andreas Richter, Stefan Schmolke, and John P. Burrows
Atmos. Chem. Phys., 17, 10997–11023, https://doi.org/10.5194/acp-17-10997-2017, https://doi.org/10.5194/acp-17-10997-2017, 2017
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Shipping accounts for a significant part of the emissions from the transportation sector. We have analyzed 3 years of MAX-DOAS measurements of NO2 and SO2 from a small island in the German Bight, showing that despite the vicinity to the shipping lane, the contribution of shipping sources to air pollution is only about 40 %. The implementation of stricter fuel sulfur limits led to a significant reduction in SO2-to-NO2 ratios in shipping emissions and ambient SO2 levels at the German coast.
Martin P. Langowski, Christian von Savigny, John P. Burrows, Didier Fussen, Erin C. M. Dawkins, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Meas. Tech., 10, 2989–3006, https://doi.org/10.5194/amt-10-2989-2017, https://doi.org/10.5194/amt-10-2989-2017, 2017
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Meteoric metals form metal layers in the upper atmosphere anandplay a role in the formation of middle-atmospheric clouds and aerosols. However, the total metal influx rate is not well known. Global Na datasets from measurements and a model are available, which had not been compared yet on a global scale until this paper. Overall the agreement is good, and many differences between measurements are also found in the model simulations. However, the modeled layer altitude is too low.
Christopher J. Merchant, Frank Paul, Thomas Popp, Michael Ablain, Sophie Bontemps, Pierre Defourny, Rainer Hollmann, Thomas Lavergne, Alexandra Laeng, Gerrit de Leeuw, Jonathan Mittaz, Caroline Poulsen, Adam C. Povey, Max Reuter, Shubha Sathyendranath, Stein Sandven, Viktoria F. Sofieva, and Wolfgang Wagner
Earth Syst. Sci. Data, 9, 511–527, https://doi.org/10.5194/essd-9-511-2017, https://doi.org/10.5194/essd-9-511-2017, 2017
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Climate data records (CDRs) contain data describing Earth's climate and should address uncertainty in the data to communicate what is known about climate variability or change and what range of doubt exists. This paper discusses good practice for including uncertainty information in CDRs for the essential climate variables (ECVs) derived from satellite data. Recommendations emerge from the shared experience of diverse ECV projects within the European Space Agency Climate Change Initiative.
Marko Scholze, Michael Buchwitz, Wouter Dorigo, Luis Guanter, and Shaun Quegan
Biogeosciences, 14, 3401–3429, https://doi.org/10.5194/bg-14-3401-2017, https://doi.org/10.5194/bg-14-3401-2017, 2017
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This paper briefly reviews data assimilation techniques in carbon cycle data assimilation and the requirements of data assimilation systems on observations. We provide a non-exhaustive overview of current observations and their uncertainties for use in terrestrial carbon cycle data assimilation, focussing on relevant space-based observations.
Klaus Bramstedt, Thomas C. Stone, Manfred Gottwald, Stefan Noël, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 10, 2413–2423, https://doi.org/10.5194/amt-10-2413-2017, https://doi.org/10.5194/amt-10-2413-2017, 2017
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The satellite instrument SCIAMACHY on board the ESA's platform Envisat
(2002–2012) performed observations of the Earth's atmosphere. Using sun and moon observations of the instrument itself, we derived a set of correction
parameters for the determination of the viewing directions of the
instrument. From this work, all vertical profiles of atmospheric parameters
from SCIAMACHY's limb and occultation measurements will be improved by a more
accurate altitude information.
Andreas Carlos Meier, Anja Schönhardt, Tim Bösch, Andreas Richter, André Seyler, Thomas Ruhtz, Daniel-Eduard Constantin, Reza Shaiganfar, Thomas Wagner, Alexis Merlaud, Michel Van Roozendael, Livio Belegante, Doina Nicolae, Lucian Georgescu, and John Philip Burrows
Atmos. Meas. Tech., 10, 1831–1857, https://doi.org/10.5194/amt-10-1831-2017, https://doi.org/10.5194/amt-10-1831-2017, 2017
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We present airborne remote sensing measurements of NO2 in the urban area of Bucharest. NO2 is a harmful pollutant, which is emitted in combustion processes. The measurements presented here enable the creation of maps, showing the horizontal NO2 distribution across the whole city within a relatively short time window of 1.5 h. These data provide new insight into urban pollution levels and their spatial distribution.
Michael Buchwitz, Oliver Schneising, Maximilian Reuter, Jens Heymann, Sven Krautwurst, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Christian Frankenberg, and Alexander J. Turner
Atmos. Chem. Phys., 17, 5751–5774, https://doi.org/10.5194/acp-17-5751-2017, https://doi.org/10.5194/acp-17-5751-2017, 2017
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Methane is an important greenhouse gas and increasing atmospheric concentrations result in global warming. We present a simple method to derive annual methane emission estimates of methane hotspot areas from satellite data. We present results for four source areas. We found that our estimates are in good agreement with other studies/data sets for the Four Corners region in the USA and for Azerbaijan but we also found higher emissions for parts of California and Turkmenistan.
Jia Jia, Annette Ladstätter-Weißenmayer, Xuewei Hou, Alexei Rozanov, and John P. Burrows
Atmos. Chem. Phys., 17, 4915–4930, https://doi.org/10.5194/acp-17-4915-2017, https://doi.org/10.5194/acp-17-4915-2017, 2017
Anja Schönhardt, Andreas Richter, Nicolas Theys, and John P. Burrows
Atmos. Chem. Phys., 17, 4857–4870, https://doi.org/10.5194/acp-17-4857-2017, https://doi.org/10.5194/acp-17-4857-2017, 2017
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Iodine monoxide, IO, is observed in satellite measurements following the eruption of the Kasatochi volcano, Alaska, in August 2008. Large IO columns are detected by SCIAMACHY on ENVISAT and by GOME-2 on MetOp-A for several days. IO amounts are approximately 1 order of magnitude smaller than those of BrO. Details in the spatial distributions differ between IO, BrO and sulfur dioxide, SO2. The total mass of IO in the volcanic plume is determined to be on the order of 10 Mg.
Stefan Lossow, Farahnaz Khosrawi, Gerald E. Nedoluha, Faiza Azam, Klaus Bramstedt, John. P. Burrows, Bianca M. Dinelli, Patrick Eriksson, Patrick J. Espy, Maya García-Comas, John C. Gille, Michael Kiefer, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Gabriele P. Stiller, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 10, 1111–1137, https://doi.org/10.5194/amt-10-1111-2017, https://doi.org/10.5194/amt-10-1111-2017, 2017
Enno Peters, Gaia Pinardi, André Seyler, Andreas Richter, Folkard Wittrock, Tim Bösch, Michel Van Roozendael, François Hendrick, Theano Drosoglou, Alkiviadis F. Bais, Yugo Kanaya, Xiaoyi Zhao, Kimberly Strong, Johannes Lampel, Rainer Volkamer, Theodore Koenig, Ivan Ortega, Olga Puentedura, Mónica Navarro-Comas, Laura Gómez, Margarita Yela González, Ankie Piters, Julia Remmers, Yang Wang, Thomas Wagner, Shanshan Wang, Alfonso Saiz-Lopez, David García-Nieto, Carlos A. Cuevas, Nuria Benavent, Richard Querel, Paul Johnston, Oleg Postylyakov, Alexander Borovski, Alexander Elokhov, Ilya Bruchkouski, Haoran Liu, Cheng Liu, Qianqian Hong, Claudia Rivera, Michel Grutter, Wolfgang Stremme, M. Fahim Khokhar, Junaid Khayyam, and John P. Burrows
Atmos. Meas. Tech., 10, 955–978, https://doi.org/10.5194/amt-10-955-2017, https://doi.org/10.5194/amt-10-955-2017, 2017
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This work is about harmonization of differential optical absorption spectroscopy retrieval codes, which is a remote sensing technique widely used to derive atmospheric trace gas amounts. The study is based on ground-based measurements performed during the Multi-Axis DOAS Comparison campaign for Aerosols and Trace gases (MAD-CAT) in Mainz, Germany, in summer 2013. In total, 17 international groups working in the field of the DOAS technique participated in this study.
Andreas Hilboll, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-101, https://doi.org/10.5194/acp-2017-101, 2017
Revised manuscript has not been submitted
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We investigate the temporal evolution of the important tropospheric air pollutant nitrogen dioxide (NO2) since the early 2000s, and correlate NO2 abundances with indicators of economic development. Until 2012, NO2 pollution and economic growth are strongly correlated, with annual increases of up to 4.4 %. Since then, tropospheric NO2 pollution has stabilized or is even declining, probably as a result of a slow-down in Indian economic growth combined with the implementation of cleaner technology.
Ruixiong Zhang, Yuhang Wang, Qiusheng He, Laiguo Chen, Yuzhong Zhang, Hang Qu, Charles Smeltzer, Jianfeng Li, Leonardo M. A. Alvarado, Mihalis Vrekoussis, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 17, 3083–3095, https://doi.org/10.5194/acp-17-3083-2017, https://doi.org/10.5194/acp-17-3083-2017, 2017
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We use short-lived reactive aromatics as proxies to diagnose transport of pollutants to Tibet. In situ observations of short-lived reactive aromatics across the Tibetan Plateau are analyzed using a regional chemistry and transport model. Our results suggest that the cut-off low system is a major pathway for long-range transport of pollutants such as black carbon. The modeling analysis reveals that even the state-of-the-science reanalysis cannot simulate this cut-off system accurately.
Stefan Bender, Miriam Sinnhuber, Martin Langowski, and John P. Burrows
Atmos. Meas. Tech., 10, 209–220, https://doi.org/10.5194/amt-10-209-2017, https://doi.org/10.5194/amt-10-209-2017, 2017
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We present the retrieval of NO number densities from 60 km to 85 km from measurements of SCIAMACHY/Envisat in its nominal limb mode (0–91 km). We derive the densities from the NO gamma bands (230–300 nm). Using prior input reduces the incorrect attribution of NO from the lower thermosphere. The SCIAMACHY nominal limb scans provide almost 10 years of daily NO data in this altitude range, a unique data record to constrain NO in the mesosphere for testing and validating chemistry climate models.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Chris A. McLinden, Peter F. Bernath, Adam E. Bourassa, John P. Burrows, Doug A. Degenstein, Bernd Funke, Didier Fussen, Gloria L. Manney, C. Thomas McElroy, Donal Murtagh, Cora E. Randall, Piera Raspollini, Alexei Rozanov, James M. Russell III, Makoto Suzuki, Masato Shiotani, Joachim Urban, Thomas von Clarmann, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 5781–5810, https://doi.org/10.5194/amt-9-5781-2016, https://doi.org/10.5194/amt-9-5781-2016, 2016
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This study validates version 3.5 of the ACE-FTS NOy species data sets by comparing diurnally scaled ACE-FTS data to correlative data from 11 other satellite limb sounders. For all five species examined (NO, NO2, HNO3, N2O5, and ClONO2), there is good agreement between ACE-FTS and the other data sets in various regions of the atmosphere. In these validated regions, these NOy data products can be used for further investigation into the composition, dynamics, and climate of the stratosphere.
Dhanyalekshmi Pillai, Michael Buchwitz, Christoph Gerbig, Thomas Koch, Maximilian Reuter, Heinrich Bovensmann, Julia Marshall, and John P. Burrows
Atmos. Chem. Phys., 16, 9591–9610, https://doi.org/10.5194/acp-16-9591-2016, https://doi.org/10.5194/acp-16-9591-2016, 2016
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Approximately 70 % of total CO2 emissions arise from cities; however, there exist large uncertainties in quantifying urban emissions. The present study investigates the potential of a satellite mission like CarbonSat to retrieve the city emissions via inverse modelling techniques. The study makes a valid conclusion that an instrument like CarbonSat has high potential to provide important information on city emissions when exploiting the observations using a high-resolution modelling system.
Elpida Leventidou, Kai-Uwe Eichmann, Mark Weber, and John P. Burrows
Atmos. Meas. Tech., 9, 3407–3427, https://doi.org/10.5194/amt-9-3407-2016, https://doi.org/10.5194/amt-9-3407-2016, 2016
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Here, we present a 17 years tropical tropospheric ozone columns dataset (1996–2012) using GOME, SCIAMACHY, and GOME-2 data, developed as part of the verification algorithm for TROPOMI on S5p mission.The uncertainty is less than 2 DU. Validation with SHADOZ ozonesonde data showed biases within 5 DU and RMS errors less than 10 DU. Comparisons with tropospheric ozone columns derived from limb–nadir matching showed that the bias and RMS are within the range of the CCD_IUP comparison with the sondes.
Stefan Noël, Klaus Bramstedt, Michael Hilker, Patricia Liebing, Johannes Plieninger, Max Reuter, Alexei Rozanov, Christopher E. Sioris, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 9, 1485–1503, https://doi.org/10.5194/amt-9-1485-2016, https://doi.org/10.5194/amt-9-1485-2016, 2016
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Stratospheric methane (CH4) and carbon dioxide (CO2) profiles have been derived from solar occultation measurements of the SCIAMACHY satellite instrument. The accuracy of these profiles is estimated to be about 5–10 % for CH4 and 2–3 % for CO2, mainly limited by unexpected vertical oscillations. Results are available for August 2002 to April 2012 and latitudes between about 50 and 70° N. From these, time series trends have been estimated, which are in reasonable agreement with total column trends.
Stefan F. Schreier, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 16, 2803–2817, https://doi.org/10.5194/acp-16-2803-2016, https://doi.org/10.5194/acp-16-2803-2016, 2016
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Mixing ratios of NO2 and HCHO in the free troposphere are obtained from MAX-DOAS measurements at two mountain stations at midlatitudes and in the tropics using a modified geometrical approach. The method is applied in the UV wavelength range and, thus, allows the detection of HCHO mixing ratios, in addition to NO2. We find that mixing ratios of both species are increased in the tropical free troposphere due to biomass burning.
Kai-Uwe Eichmann, Luca Lelli, Christian von Savigny, Harjinder Sembhi, and John P. Burrows
Atmos. Meas. Tech., 9, 793–815, https://doi.org/10.5194/amt-9-793-2016, https://doi.org/10.5194/amt-9-793-2016, 2016
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Height-resolved limb radiance spectra of the satellite instrument SCIAMACHY are used to retrieve cloud top heights with a colour index method. Clouds are detectable from the lower to the uppermost troposphere. These cloud heights help to improve the trace gas retrieval for the upper troposphere and lower stratosphere. Comparisons with other data sets have shown good agreement. As clouds and aerosols are not distinguishable, lower stratospheric volcanic aerosol clouds are detected in some years.
Susan Kulawik, Debra Wunch, Christopher O'Dell, Christian Frankenberg, Maximilian Reuter, Tomohiro Oda, Frederic Chevallier, Vanessa Sherlock, Michael Buchwitz, Greg Osterman, Charles E. Miller, Paul O. Wennberg, David Griffith, Isamu Morino, Manvendra K. Dubey, Nicholas M. Deutscher, Justus Notholt, Frank Hase, Thorsten Warneke, Ralf Sussmann, John Robinson, Kimberly Strong, Matthias Schneider, Martine De Mazière, Kei Shiomi, Dietrich G. Feist, Laura T. Iraci, and Joyce Wolf
Atmos. Meas. Tech., 9, 683–709, https://doi.org/10.5194/amt-9-683-2016, https://doi.org/10.5194/amt-9-683-2016, 2016
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To accurately estimate source and sink locations of carbon dioxide, systematic errors in satellite measurements and models must be characterized. This paper examines two satellite data sets (GOSAT, launched 2009, and SCIAMACHY, launched 2002), and two models (CarbonTracker and MACC) vs. the TCCON CO2 validation data set. We assess biases and errors by season and latitude, satellite performance under averaging, and diurnal variability. Our findings are useful for assimilation of satellite data.
A.-M. Blechschmidt, A. Richter, J. P. Burrows, L. Kaleschke, K. Strong, N. Theys, M. Weber, X. Zhao, and A. Zien
Atmos. Chem. Phys., 16, 1773–1788, https://doi.org/10.5194/acp-16-1773-2016, https://doi.org/10.5194/acp-16-1773-2016, 2016
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A comprehensive case study of a comma-shaped bromine monoxide plume in the Arctic, which was transported by a polar cyclone and was observed by the GOME-2 satellite sensor over several days, is presented. By making combined use of different kinds of satellite data and numerical models, we demonstrate the important role of the frontal weather system in favouring the bromine activation cycle and blowing snow production, which may have acted as a bromine source during the bromine explosion event.
Sébastien Massart, Anna Agustí-Panareda, Jens Heymann, Michael Buchwitz, Frédéric Chevallier, Maximilian Reuter, Michael Hilker, John P. Burrows, Nicholas M. Deutscher, Dietrich G. Feist, Frank Hase, Ralf Sussmann, Filip Desmet, Manvendra K. Dubey, David W. T. Griffith, Rigel Kivi, Christof Petri, Matthias Schneider, and Voltaire A. Velazco
Atmos. Chem. Phys., 16, 1653–1671, https://doi.org/10.5194/acp-16-1653-2016, https://doi.org/10.5194/acp-16-1653-2016, 2016
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This study presents the European Centre for Medium-Range Weather Forecasts (ECMWF) monitoring of atmospheric CO2 using measurements from the Greenhouse gases Observing Satellite (GOSAT). We show that the modelled CO2 has a better precision than standard CO2 satellite products compared to ground-based measurements. We also present the CO2 forecast based on our best knowledge of the atmospheric CO2 distribution. We show that it has skill to forecast the largest scale CO2 patterns up to day 5.
M. P. Langowski, C. von Savigny, J. P. Burrows, V. V. Rozanov, T. Dunker, U.-P. Hoppe, M. Sinnhuber, and A. C. Aikin
Atmos. Meas. Tech., 9, 295–311, https://doi.org/10.5194/amt-9-295-2016, https://doi.org/10.5194/amt-9-295-2016, 2016
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An algorithm has been developed for the retrieval of sodium atom (Na) number density on a latitude and altitude grid from SCIAMACHY limb measurements of the Na resonance fluorescence (multiannual means 2008–2012). The Na layer peaks at 90 to 93 km altitude and has a FWHM of 5 to 15 km. A summer minimum in peak density and width is observed at high latitudes. At low latitudes, a semiannual oscillation is found. The results are compared with other measurements and models and agree well with these.
F. Ebojie, J. P. Burrows, C. Gebhardt, A. Ladstätter-Weißenmayer, C. von Savigny, A. Rozanov, M. Weber, and H. Bovensmann
Atmos. Chem. Phys., 16, 417–436, https://doi.org/10.5194/acp-16-417-2016, https://doi.org/10.5194/acp-16-417-2016, 2016
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The goal of this study is to determine the global and zonal changes in the tropospheric ozone data product derived from SCIAMACHY limb-nadir-matching (LNM) observations during the period 2003–2011.
Tropospheric O3 shows statistically significant increases over some regions of South Asia, the South American continent, Alaska, around Congo in Africa and over some continental outflows. Significant decrease in TOC is observed over some continents and oceans.
K. Weigel, A. Rozanov, F. Azam, K. Bramstedt, R. Damadeo, K.-U. Eichmann, C. Gebhardt, D. Hurst, M. Kraemer, S. Lossow, W. Read, N. Spelten, G. P. Stiller, K. A. Walker, M. Weber, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 9, 133–158, https://doi.org/10.5194/amt-9-133-2016, https://doi.org/10.5194/amt-9-133-2016, 2016
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The SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) aboard the Envisat satellite provided measurements between 2002 and 2012 with different viewing geometries. The limb viewing geometry allows the retrieval of water vapour profiles in the UTLS (upper troposphere and lower stratosphere) from the near-infrared spectral range (1353–1410 nm). Here, we present data version 3.01 and compare it to other water vapour data.
F. Khosrawi, J. Urban, S. Lossow, G. Stiller, K. Weigel, P. Braesicke, M. C. Pitts, A. Rozanov, J. P. Burrows, and D. Murtagh
Atmos. Chem. Phys., 16, 101–121, https://doi.org/10.5194/acp-16-101-2016, https://doi.org/10.5194/acp-16-101-2016, 2016
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Our sensitivity studies based on air parcel trajectories confirm that Polar stratospheric cloud (PSC) formation is quite sensitive to water vapour and temperature changes. Considering water vapour time series from satellite measurements we do not find a consistent, significant trend in water vapour in the lower stratosphere during the past 15 years (2000–2014). Thus, the severe dentrification observed in 2010/2011 cannot be directly related to increases in stratospheric water vapour.
C. von Savigny, F. Ernst, A. Rozanov, R. Hommel, K.-U. Eichmann, V. Rozanov, J. P. Burrows, and L. W. Thomason
Atmos. Meas. Tech., 8, 5223–5235, https://doi.org/10.5194/amt-8-5223-2015, https://doi.org/10.5194/amt-8-5223-2015, 2015
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This article presents validation results for stratospheric aerosol extinction profiles retrieved from limb-scatter measurements with the SCIAMACHY instrument on the Envisat satellite. The SCIAMACHY retrievals are compared to co-located measurements with the SAGE II instrument. Very good agreement to within about 15% is found in a global average sense at altitudes above 15 km. The article also presents sample results on the global morphology of the stratospheric aerosol layer from 2003 to 2011.
A. Schönhardt, P. Altube, K. Gerilowski, S. Krautwurst, J. Hartmann, A. C. Meier, A. Richter, and J. P. Burrows
Atmos. Meas. Tech., 8, 5113–5131, https://doi.org/10.5194/amt-8-5113-2015, https://doi.org/10.5194/amt-8-5113-2015, 2015
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The study reports on the application of an aircraft-based instrument (AirMAP) measuring atmospheric nitrogen dioxide. Two-dimensional maps are produced at a spatial resolution of 28m x 30m and with wide spatial coverage. The instrument characteristics are explained and the detailed mapping of a power plant emission plume is demonstrated. Small-scale enhanced amounts of nitrogen dioxide from traffic are observed above a motorway.
A. Butz, J. Orphal, R. Checa-Garcia, F. Friedl-Vallon, T. von Clarmann, H. Bovensmann, O. Hasekamp, J. Landgraf, T. Knigge, D. Weise, O. Sqalli-Houssini, and D. Kemper
Atmos. Meas. Tech., 8, 4719–4734, https://doi.org/10.5194/amt-8-4719-2015, https://doi.org/10.5194/amt-8-4719-2015, 2015
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The Geostationary Emission Explorer for Europe (G3E) is a mission concept for a greenhouse gas sounder in geostationary orbit. It is designed to provide column-average concentrations of carbon dioxide, methane, and carbon monoxide with high spatial and 2-hour temporal resolution throughout the central European continent. The prospective data density, precision and accuracy suggest G3E as a key component of a future carbon emission monitoring system.
D. R. Thompson, I. Leifer, H. Bovensmann, M. Eastwood, M. Fladeland, C. Frankenberg, K. Gerilowski, R. O. Green, S. Kratwurst, T. Krings, B. Luna, and A. K. Thorpe
Atmos. Meas. Tech., 8, 4383–4397, https://doi.org/10.5194/amt-8-4383-2015, https://doi.org/10.5194/amt-8-4383-2015, 2015
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We discuss principles for real-time infrared spectral signature detection and measurement, and report performance onboard the NASA Airborne Visible Infrared Spectrometer - Next Generation (AVIRIS-NG). We describe a case study of the NASA/ESA CO2 and MEthane eXperiment (COMEX), a multi-platform campaign to measure CH4 plumes released from anthropogenic sources including oil and gas infrastructure. AVIRIS-NG successfully detected CH4 plumes in concert with other in situ and remote instruments.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
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The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
S. Bender, M. Sinnhuber, T. von Clarmann, G. Stiller, B. Funke, M. López-Puertas, J. Urban, K. Pérot, K. A. Walker, and J. P. Burrows
Atmos. Meas. Tech., 8, 4171–4195, https://doi.org/10.5194/amt-8-4171-2015, https://doi.org/10.5194/amt-8-4171-2015, 2015
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We compare the nitric oxide (NO) daily zonal mean number density data sets in the mesosphere and lower thermosphere (MLT, 60km to 150km) from four instruments: ACE-FTS (2004--2010), MIPAS (2005--2012), SCIAMACHY (2008--2012), and SMR (2003--2012). We find that these data sets from different instruments consistently constrain NO in the MLT. Thus, they offer reliable forcing inputs for climate and chemistry climate models as an initial step to include solar and geomagnetic activity.
L. Kattner, B. Mathieu-Üffing, J. P. Burrows, A. Richter, S. Schmolke, A. Seyler, and F. Wittrock
Atmos. Chem. Phys., 15, 10087–10092, https://doi.org/10.5194/acp-15-10087-2015, https://doi.org/10.5194/acp-15-10087-2015, 2015
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On 1 January 2015, the International Maritime Organisation tightened the regulations for sulfur content of shipping fuels in Sulfur Emission Control Areas. Here we present data from a station near Hamburg harbour in the North Sea SECA, which uses in situ measurements of atmospheric trace gases to deduce the sulphur fuel content of passing ships. We compare data from 2014 before the regulation change and from January 2015 and show how this method can be used for compliance monitoring.
J. Jia, A. Rozanov, A. Ladstätter-Weißenmayer, and J. P. Burrows
Atmos. Meas. Tech., 8, 3369–3383, https://doi.org/10.5194/amt-8-3369-2015, https://doi.org/10.5194/amt-8-3369-2015, 2015
J. Heymann, M. Reuter, M. Hilker, M. Buchwitz, O. Schneising, H. Bovensmann, J. P. Burrows, A. Kuze, H. Suto, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, S. Kawakami, R. Kivi, I. Morino, C. Petri, C. Roehl, M. Schneider, V. Sherlock, R. Sussmann, V. A. Velazco, T. Warneke, and D. Wunch
Atmos. Meas. Tech., 8, 2961–2980, https://doi.org/10.5194/amt-8-2961-2015, https://doi.org/10.5194/amt-8-2961-2015, 2015
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Long-term data sets of global atmospheric carbon dioxide concentrations based on observations from different satellite instruments may suffer from inconsistencies originating from the use of different retrieval algorithms. This issue has been addressed by applying the Bremen Optimal Estimation DOAS retrieval algorithm to SCIAMACHY and TANSO-FTS observations. Detailed comparisons with TCCON and CarbonTracker show good consistency between the SCIAMACHY and TANSO-FTS data sets.
T. Dinter, V. V. Rozanov, J. P. Burrows, and A. Bracher
Ocean Sci., 11, 373–389, https://doi.org/10.5194/os-11-373-2015, https://doi.org/10.5194/os-11-373-2015, 2015
M. P. Langowski, C. von Savigny, J. P. Burrows, W. Feng, J. M. C. Plane, D. R. Marsh, D. Janches, M. Sinnhuber, A. C. Aikin, and P. Liebing
Atmos. Chem. Phys., 15, 273–295, https://doi.org/10.5194/acp-15-273-2015, https://doi.org/10.5194/acp-15-273-2015, 2015
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Global concentration fields of Mg and Mg+ in the Earth's upper mesosphere and lower thermosphere (70-150km) are presented. These are retrieved from SCIAMACHY/Envisat satellite grating spectrometer measurements in limb viewing geometry between 2008 and 2012.
These were compared with WACCM-Mg model results and a large fraction of the available measurement results for these species, and an interpretation of the results is done. The variation of these species during NLC presence is discussed.
M. Reuter, M. Buchwitz, M. Hilker, J. Heymann, O. Schneising, D. Pillai, H. Bovensmann, J. P. Burrows, H. Bösch, R. Parker, A. Butz, O. Hasekamp, C. W. O'Dell, Y. Yoshida, C. Gerbig, T. Nehrkorn, N. M. Deutscher, T. Warneke, J. Notholt, F. Hase, R. Kivi, R. Sussmann, T. Machida, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 13739–13753, https://doi.org/10.5194/acp-14-13739-2014, https://doi.org/10.5194/acp-14-13739-2014, 2014
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Current knowledge about the European terrestrial biospheric carbon sink relies upon bottom-up and global surface flux inverse model estimates using in situ measurements. Our analysis of five satellite data sets comprises a regional inversion designed to be insensitive to potential retrieval biases and transport errors. We show that the satellite-derived sink is larger (1.0±0.3GtC/a) than previous estimates (0.4±0.4GtC/a).
G. D. Hayman, F. M. O'Connor, M. Dalvi, D. B. Clark, N. Gedney, C. Huntingford, C. Prigent, M. Buchwitz, O. Schneising, J. P. Burrows, C. Wilson, N. Richards, and M. Chipperfield
Atmos. Chem. Phys., 14, 13257–13280, https://doi.org/10.5194/acp-14-13257-2014, https://doi.org/10.5194/acp-14-13257-2014, 2014
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Globally, wetlands are a major source of methane, which is the second most important greenhouse gas. We find the JULES wetland methane scheme to perform well in general, although there is a tendency for it to overpredict emissions in the tropics and underpredict them in northern latitudes. Our study highlights novel uses of satellite data as a major tool to constrain land-atmosphere methane flux models in a warming world.
J. Aschmann, J. P. Burrows, C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, and A. M. Thompson
Atmos. Chem. Phys., 14, 12803–12814, https://doi.org/10.5194/acp-14-12803-2014, https://doi.org/10.5194/acp-14-12803-2014, 2014
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This study compares observations and simulation results of ozone in the lower tropical stratosphere. It shows that ozone in this region decreased from 1985 up to about 2002, which is consistent with an increase in tropical upwelling predicted by climate models. However, the decrease effectively stops after 2002, indicating that significant changes in tropical upwelling have occurred. The most important factor appears to be that the vertical ascent in the tropics is no longer accelerating.
E. Peters, F. Wittrock, A. Richter, L. M. A. Alvarado, V. V. Rozanov, and J. P. Burrows
Atmos. Meas. Tech., 7, 4203–4221, https://doi.org/10.5194/amt-7-4203-2014, https://doi.org/10.5194/amt-7-4203-2014, 2014
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In this study, a correction spectrum accounting for insufficiencies in commonly used liquid water absorption spectra in DOAS applications is retrieved from ship-borne field measurements. The correction spectrum compensates at the same time for broadband parts of vibrational Raman scattering. With this, an entire compensation of liquid water spectral effects in DOAS applications was achieved.
L. M. A. Alvarado, A. Richter, M. Vrekoussis, F. Wittrock, A. Hilboll, S. F. Schreier, and J. P. Burrows
Atmos. Meas. Tech., 7, 4133–4150, https://doi.org/10.5194/amt-7-4133-2014, https://doi.org/10.5194/amt-7-4133-2014, 2014
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An improved glyoxal retrieval for OMI measurements using the DOAS method has been developed. The retrieval is based on sensitivity tests for the selection of most appropriate retrieval parameters. Also, corrections for reduction of interferences with other species have been applied. In addition, the link between pyrogenic emissions and glyoxal over regions with large wildfires have been investigated, and showed that fires are an important source of glyoxal.
J. Strandgren, L. Mei, M. Vountas, J. P. Burrows, A. Lyapustin, and Y. Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-25869-2014, https://doi.org/10.5194/acpd-14-25869-2014, 2014
Revised manuscript not accepted
K. Noguchi, A. Richter, V. Rozanov, A. Rozanov, J. P. Burrows, H. Irie, and K. Kita
Atmos. Meas. Tech., 7, 3497–3508, https://doi.org/10.5194/amt-7-3497-2014, https://doi.org/10.5194/amt-7-3497-2014, 2014
A. Spolaor, P. Vallelonga, J. Gabrieli, T. Martma, M. P. Björkman, E. Isaksson, G. Cozzi, C. Turetta, H. A. Kjær, M. A. J. Curran, A. D. Moy, A. Schönhardt, A.-M. Blechschmidt, J. P. Burrows, J. M. C. Plane, and C. Barbante
Atmos. Chem. Phys., 14, 9613–9622, https://doi.org/10.5194/acp-14-9613-2014, https://doi.org/10.5194/acp-14-9613-2014, 2014
L. L. Mei, Y. Xue, A. A. Kokhanovsky, W. von Hoyningen-Huene, G. de Leeuw, and J. P. Burrows
Atmos. Meas. Tech., 7, 2411–2420, https://doi.org/10.5194/amt-7-2411-2014, https://doi.org/10.5194/amt-7-2411-2014, 2014
A. W. Zien, A. Richter, A. Hilboll, A.-M. Blechschmidt, and J. P. Burrows
Atmos. Chem. Phys., 14, 7367–7396, https://doi.org/10.5194/acp-14-7367-2014, https://doi.org/10.5194/acp-14-7367-2014, 2014
W. Chehade, M. Weber, and J. P. Burrows
Atmos. Chem. Phys., 14, 7059–7074, https://doi.org/10.5194/acp-14-7059-2014, https://doi.org/10.5194/acp-14-7059-2014, 2014
F. Ebojie, C. von Savigny, A. Ladstätter-Weißenmayer, A. Rozanov, M. Weber, K.-U. Eichmann, S. Bötel, N. Rahpoe, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 7, 2073–2096, https://doi.org/10.5194/amt-7-2073-2014, https://doi.org/10.5194/amt-7-2073-2014, 2014
J. Yoon, J. P. Burrows, M. Vountas, W. von Hoyningen-Huene, D. Y. Chang, A. Richter, and A. Hilboll
Atmos. Chem. Phys., 14, 6881–6902, https://doi.org/10.5194/acp-14-6881-2014, https://doi.org/10.5194/acp-14-6881-2014, 2014
P. Ciais, A. J. Dolman, A. Bombelli, R. Duren, A. Peregon, P. J. Rayner, C. Miller, N. Gobron, G. Kinderman, G. Marland, N. Gruber, F. Chevallier, R. J. Andres, G. Balsamo, L. Bopp, F.-M. Bréon, G. Broquet, R. Dargaville, T. J. Battin, A. Borges, H. Bovensmann, M. Buchwitz, J. Butler, J. G. Canadell, R. B. Cook, R. DeFries, R. Engelen, K. R. Gurney, C. Heinze, M. Heimann, A. Held, M. Henry, B. Law, S. Luyssaert, J. Miller, T. Moriyama, C. Moulin, R. B. Myneni, C. Nussli, M. Obersteiner, D. Ojima, Y. Pan, J.-D. Paris, S. L. Piao, B. Poulter, S. Plummer, S. Quegan, P. Raymond, M. Reichstein, L. Rivier, C. Sabine, D. Schimel, O. Tarasova, R. Valentini, R. Wang, G. van der Werf, D. Wickland, M. Williams, and C. Zehner
Biogeosciences, 11, 3547–3602, https://doi.org/10.5194/bg-11-3547-2014, https://doi.org/10.5194/bg-11-3547-2014, 2014
B. Dils, M. Buchwitz, M. Reuter, O. Schneising, H. Boesch, R. Parker, S. Guerlet, I. Aben, T. Blumenstock, J. P. Burrows, A. Butz, N. M. Deutscher, C. Frankenberg, F. Hase, O. P. Hasekamp, J. Heymann, M. De Mazière, J. Notholt, R. Sussmann, T. Warneke, D. Griffith, V. Sherlock, and D. Wunch
Atmos. Meas. Tech., 7, 1723–1744, https://doi.org/10.5194/amt-7-1723-2014, https://doi.org/10.5194/amt-7-1723-2014, 2014
L. Lelli, A. A. Kokhanovsky, V. V. Rozanov, M. Vountas, and J. P. Burrows
Atmos. Chem. Phys., 14, 5679–5692, https://doi.org/10.5194/acp-14-5679-2014, https://doi.org/10.5194/acp-14-5679-2014, 2014
M. Horstjann, M. D. Andrés Hernández, V. Nenakhov, A. Chrobry, and J. P. Burrows
Atmos. Meas. Tech., 7, 1245–1257, https://doi.org/10.5194/amt-7-1245-2014, https://doi.org/10.5194/amt-7-1245-2014, 2014
R. Hommel, K.-U. Eichmann, J. Aschmann, K. Bramstedt, M. Weber, C. von Savigny, A. Richter, A. Rozanov, F. Wittrock, F. Khosrawi, R. Bauer, and J. P. Burrows
Atmos. Chem. Phys., 14, 3247–3276, https://doi.org/10.5194/acp-14-3247-2014, https://doi.org/10.5194/acp-14-3247-2014, 2014
S. F. Schreier, A. Richter, J. W. Kaiser, and J. P. Burrows
Atmos. Chem. Phys., 14, 2447–2466, https://doi.org/10.5194/acp-14-2447-2014, https://doi.org/10.5194/acp-14-2447-2014, 2014
V. Gorshelev, A. Serdyuchenko, M. Weber, W. Chehade, and J. P. Burrows
Atmos. Meas. Tech., 7, 609–624, https://doi.org/10.5194/amt-7-609-2014, https://doi.org/10.5194/amt-7-609-2014, 2014
A. Serdyuchenko, V. Gorshelev, M. Weber, W. Chehade, and J. P. Burrows
Atmos. Meas. Tech., 7, 625–636, https://doi.org/10.5194/amt-7-625-2014, https://doi.org/10.5194/amt-7-625-2014, 2014
C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, H. Bovensmann, J. P. Burrows, D. Degenstein, L. Froidevaux, and A. M. Thompson
Atmos. Chem. Phys., 14, 831–846, https://doi.org/10.5194/acp-14-831-2014, https://doi.org/10.5194/acp-14-831-2014, 2014
M. Langowski, M. Sinnhuber, A. C. Aikin, C. von Savigny, and J. P. Burrows
Atmos. Meas. Tech., 7, 29–48, https://doi.org/10.5194/amt-7-29-2014, https://doi.org/10.5194/amt-7-29-2014, 2014
O. Schneising, M. Reuter, M. Buchwitz, J. Heymann, H. Bovensmann, and J. P. Burrows
Atmos. Chem. Phys., 14, 133–141, https://doi.org/10.5194/acp-14-133-2014, https://doi.org/10.5194/acp-14-133-2014, 2014
M. Buchwitz, M. Reuter, H. Bovensmann, D. Pillai, J. Heymann, O. Schneising, V. Rozanov, T. Krings, J. P. Burrows, H. Boesch, C. Gerbig, Y. Meijer, and A. Löscher
Atmos. Meas. Tech., 6, 3477–3500, https://doi.org/10.5194/amt-6-3477-2013, https://doi.org/10.5194/amt-6-3477-2013, 2013
W. Chehade, V. Gorshelev, A. Serdyuchenko, J. P. Burrows, and M. Weber
Atmos. Meas. Tech., 6, 3055–3065, https://doi.org/10.5194/amt-6-3055-2013, https://doi.org/10.5194/amt-6-3055-2013, 2013
N. Rahpoe, C. von Savigny, M. Weber, A.V. Rozanov, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 6, 2825–2837, https://doi.org/10.5194/amt-6-2825-2013, https://doi.org/10.5194/amt-6-2825-2013, 2013
S. Bender, M. Sinnhuber, J. P. Burrows, M. Langowski, B. Funke, and M. López-Puertas
Atmos. Meas. Tech., 6, 2521–2531, https://doi.org/10.5194/amt-6-2521-2013, https://doi.org/10.5194/amt-6-2521-2013, 2013
W. Chehade, B. Gür, P. Spietz, V. Gorshelev, A. Serdyuchenko, J. P. Burrows, and M. Weber
Atmos. Meas. Tech., 6, 1623–1632, https://doi.org/10.5194/amt-6-1623-2013, https://doi.org/10.5194/amt-6-1623-2013, 2013
M. D. Andrés-Hernández, D. Kartal, J. N. Crowley, V. Sinha, E. Regelin, M. Martínez-Harder, V. Nenakhov, J. Williams, H. Harder, H. Bozem, W. Song, J. Thieser, M. J. Tang, Z. Hosaynali Beigi, and J. P. Burrows
Atmos. Chem. Phys., 13, 5731–5749, https://doi.org/10.5194/acp-13-5731-2013, https://doi.org/10.5194/acp-13-5731-2013, 2013
A. Hilboll, A. Richter, and J. P. Burrows
Atmos. Chem. Phys., 13, 4145–4169, https://doi.org/10.5194/acp-13-4145-2013, https://doi.org/10.5194/acp-13-4145-2013, 2013
A. Hilboll, A. Richter, A. Rozanov, Ø. Hodnebrog, A. Heckel, S. Solberg, F. Stordal, and J. P. Burrows
Atmos. Meas. Tech., 6, 565–584, https://doi.org/10.5194/amt-6-565-2013, https://doi.org/10.5194/amt-6-565-2013, 2013
M. Reuter, H. Bösch, H. Bovensmann, A. Bril, M. Buchwitz, A. Butz, J. P. Burrows, C. W. O'Dell, S. Guerlet, O. Hasekamp, J. Heymann, N. Kikuchi, S. Oshchepkov, R. Parker, S. Pfeifer, O. Schneising, T. Yokota, and Y. Yoshida
Atmos. Chem. Phys., 13, 1771–1780, https://doi.org/10.5194/acp-13-1771-2013, https://doi.org/10.5194/acp-13-1771-2013, 2013
T. Krings, K. Gerilowski, M. Buchwitz, J. Hartmann, T. Sachs, J. Erzinger, J. P. Burrows, and H. Bovensmann
Atmos. Meas. Tech., 6, 151–166, https://doi.org/10.5194/amt-6-151-2013, https://doi.org/10.5194/amt-6-151-2013, 2013
Related subject area
Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Water vapour isotopes over West Africa as observed from space: which processes control tropospheric H2O ∕ HDO pair distributions?
Evidence of successful methane mitigation in one of Europe's most important oil production region
SO2 emissions derived from TROPOMI observations over India using a flux-divergence method with variable lifetimes
Evaluation of the WRF-Chem performance for the air pollutants over the United Arab Emirates
Analysis of the long-range transport of the volcanic plume from the 2021 Tajogaite/Cumbre Vieja eruption to Europe using TROPOMI and ground-based measurements
Development of a high-spatial-resolution annual emission inventory of greenhouse gases from open straw burning in Northeast China from 2001 to 2020
Evaluating spatiotemporal variations and exposure risk of ground-level ozone concentrations across China from 2000 to 2020 using satellite-derived high-resolution data
Quantifying large methane emissions from the Nord Stream pipeline gas leak of September 2022 using IASI satellite observations and inverse modelling
Automated detection of regions with persistently enhanced methane concentrations using Sentinel-5 Precursor satellite data
Biomass burning CO emissions: exploring insights through TROPOMI-derived emissions and emission coefficients
Measurement report: Combined use of MAX-DOAS and AERONET ground-based measurements in Montevideo, Uruguay, for the detection of distant biomass burning
Quantifying CH4 emissions from coal mine aggregation areas in Shanxi, China, using TROPOMI observations and the wind-assigned anomaly method
Identifying episodic carbon monoxide emission events in the MOPITT measurement dataset
Quantifying effects of long-range transport of NO2 over Delhi using back trajectories and satellite data
Measurement report: Ammonia in Paris derived from ground-based open-path and satellite observations
Anthropogenic CO2 emission estimates in the Tokyo metropolitan area from ground-based CO2 column observations
Characterizing the tropospheric water vapor spatial variation and trend using 2007–2018 COSMIC radio occultation and ECMWF reanalysis data
Detecting nitrogen oxide emissions in Qatar and quantifying emission factors of gas-fired power plants – a 4-year study
Identifying and accounting for the Coriolis effect in satellite NO2 observations and emission estimates
Characterisations of Europe's integrated water vapour and assessments of atmospheric reanalyses using more than 2 decades of ground-based GPS
Ground-level gaseous pollutants (NO2, SO2, and CO) in China: daily seamless mapping and spatiotemporal variations
NH3 spatiotemporal variability over Paris, Mexico City, and Toronto, and its link to PM2.5 during pollution events
Multi-axis differential optical absorption spectroscopy (MAX-DOAS) observations of formaldehyde and nitrogen dioxide at three sites in Asia and comparison with the global chemistry transport model CHASER
Quantifying CH4 emissions in hard coal mines from TROPOMI and IASI observations using the wind-assigned anomaly method
Estimation of surface ammonia concentrations and emissions in China from the polar-orbiting Infrared Atmospheric Sounding Interferometer and the FY-4A Geostationary Interferometric Infrared Sounder
Interannual variability in the Australian carbon cycle over 2015–2019, based on assimilation of Orbiting Carbon Observatory-2 (OCO-2) satellite data
Source and variability of formaldehyde (HCHO) at northern high latitudes: an integrated satellite, aircraft, and model study
Volcanic SO2 layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
Spaceborne tropospheric nitrogen dioxide (NO2) observations from 2005–2020 over the Yangtze River Delta (YRD), China: variabilities, implications, and drivers
Novel assessment of numerical forecasting model relative humidity with satellite probabilistic estimates
Influence of springtime atmospheric circulation types on the distribution of air pollutants in the Arctic
Technical note: Evaluation of profile retrievals of aerosols and trace gases for MAX-DOAS measurements under different aerosol scenarios based on radiative transfer simulations
Diurnal evolution of total column and surface atmospheric ammonia in the megacity of Paris, France, during an intense springtime pollution episode
The reduction in C2H6 from 2015 to 2020 over Hefei, eastern China, points to air quality improvement in China
Mapping the drivers of formaldehyde (HCHO) variability from 2015 to 2019 over eastern China: insights from Fourier transform infrared observation and GEOS-Chem model simulation
The impact of Los Angeles Basin pollution and stratospheric intrusions on the surrounding San Gabriel Mountains as seen by surface measurements, lidar, and numerical models
Sudden changes in nitrogen dioxide emissions over Greece due to lockdown after the outbreak of COVID-19
Monitoring CO emissions of the metropolis Mexico City using TROPOMI CO observations
Pollution trace gas distributions and their transport in the Asian monsoon upper troposphere and lowermost stratosphere during the StratoClim campaign 2017
Spatial distribution of enhanced BrO and its relation to meteorological parameters in Arctic and Antarctic sea ice regions
Trends of atmospheric water vapour in Switzerland from ground-based radiometry, FTIR and GNSS data
A Raman lidar tropospheric water vapour climatology and height-resolved trend analysis over Payerne, Switzerland
The potential of Orbiting Carbon Observatory-2 data to reduce the uncertainties in CO2 surface fluxes over Australia using a variational assimilation scheme
Observing carbon dioxide emissions over China's cities and industrial areas with the Orbiting Carbon Observatory-2
Observational evidence of moistening the lowermost stratosphere via isentropic mixing across the subtropical jet
Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution
NH3 emissions from large point sources derived from CrIS and IASI satellite observations
Diurnal cycle of short-term fluctuations of integrated water vapour above Switzerland
Retrieval of total column and surface NO2 from Pandora zenith-sky measurements
MAX-DOAS measurements of tropospheric NO2 and HCHO in Nanjing and a comparison to ozone monitoring instrument observations
Christopher Johannes Diekmann, Matthias Schneider, Peter Knippertz, Tim Trent, Hartmut Boesch, Amelie Ninja Roehling, John Worden, Benjamin Ertl, Farahnaz Khosrawi, and Frank Hase
Atmos. Chem. Phys., 25, 5409–5431, https://doi.org/10.5194/acp-25-5409-2025, https://doi.org/10.5194/acp-25-5409-2025, 2025
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The West African Monsoon is the main source of rainfall over West Africa, and understanding the development of the monsoon remains challenging due to complex interactions of atmospheric processes. We make use of new satellite datasets of isotopes in tropospheric water vapour to characterize processes controlling the monsoon convection. We find that comparing different water vapour isotopes reveals effects of rain–vapour interactions and air mass transport.
Gerrit Kuhlmann, Foteini Stavropoulou, Stefan Schwietzke, Daniel Zavala-Araiza, Andrew Thorpe, Andreas Hueni, Lukas Emmenegger, Andreea Calcan, Thomas Röckmann, and Dominik Brunner
Atmos. Chem. Phys., 25, 5371–5385, https://doi.org/10.5194/acp-25-5371-2025, https://doi.org/10.5194/acp-25-5371-2025, 2025
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A measurement campaign in 2019 found that methane emissions from oil and gas in Romania were significantly higher than reported. In 2021, our follow-up campaign using airborne remote sensing showed a marked decreases in emissions by 20 %–60 % due to improved infrastructure. The study highlights the importance of measurement-based emission monitoring and illustrates the value of a multi-scale assessment integrating ground-based observations with large-scale airborne remote sensing campaigns.
Yutao Chen, Ronald J. van der A, Jieying Ding, Henk Eskes, Jason E. Williams, Nicolas Theys, Athanasios Tsikerdekis, and Pieternel F. Levelt
Atmos. Chem. Phys., 25, 1851–1868, https://doi.org/10.5194/acp-25-1851-2025, https://doi.org/10.5194/acp-25-1851-2025, 2025
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There is a lack of local SO2 top-down emission inventories in India. With the improvement in the divergence method and the derivation of SO2 local lifetime, gridded SO2 emissions over a large area can be estimated efficiently. This method can be applied to any region in the world to derive SO2 emissions. Especially for regions with high latitudes, our methodology has the potential to significantly improve the top-down derivation of SO2 emissions.
Yesobu Yarragunta, Diana Francis, Ricardo Fonseca, and Narendra Nelli
Atmos. Chem. Phys., 25, 1685–1709, https://doi.org/10.5194/acp-25-1685-2025, https://doi.org/10.5194/acp-25-1685-2025, 2025
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This study evaluates the Weather Research and Forecasting model with chemistry (WRF-Chem) in simulating air pollutants over the United Arab Emirates using satellite observations. The model accurately captured ozone and carbon monoxide but showed discrepancies for nitrogen dioxide. WRF-Chem was moderately correlated with aerosol optical depth observations and performed well in simulating meteorological parameters, demonstrating its suitability for atmospheric modelling.
Pascal Hedelt, Jens Reichardt, Felix Lauermann, Benjamin Weiß, Nicolas Theys, Alberto Redondas, Africa Barreto, Omaira Garcia, and Diego Loyola
Atmos. Chem. Phys., 25, 1253–1272, https://doi.org/10.5194/acp-25-1253-2025, https://doi.org/10.5194/acp-25-1253-2025, 2025
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The 2021 volcanic eruption of Tajogaite on La Palma is investigated using ground-based and satellite measurements. In addition, the atmospheric transport of the volcanic cloud towards Europe is studied in detail. The amount of SO2 released during the eruption and the height of the volcanic plume are in excellent agreement among the different measurements. Furthermore, volcanic aerosol microphysical properties could be retrieved using a new retrieval approach based on lidar measurements.
Zihan Song, Leiming Zhang, Chongguo Tian, Qiang Fu, Zhenxing Shen, Renjian Zhang, Dong Liu, and Song Cui
Atmos. Chem. Phys., 24, 13101–13113, https://doi.org/10.5194/acp-24-13101-2024, https://doi.org/10.5194/acp-24-13101-2024, 2024
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A novel concept integrating crop cycle information into fire spot extraction was proposed. Spatiotemporal variations of open straw burning in Northeast China are revealed. Open straw burning in Northeast China emitted a total of 218 Tg of CO2-eq during 2001–2020. The policy of banning straw burning effectively reduced greenhouse gas emissions.
Qingqing He, Jingru Cao, Pablo E. Saide, Tong Ye, and Weihang Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3310, https://doi.org/10.5194/egusphere-2024-3310, 2024
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We explored variations in ground ozone and exposure risk hotspots across China (2000–2020) at multiple spatiotemporal scales using a high-resolution dataset derived from satellite LST via a machine-learning hindcast framework. The dataset was validated using cross-validation and external measurements. A non-monotonous trend emerged, with turning points around 2007 and 2015, showing regional variation. Ozone levels >100 μg/m3 shifted from June to May, while levels >160 μg/m3 expanded in the NCP.
Chris Wilson, Brian J. Kerridge, Richard Siddans, David P. Moore, Lucy J. Ventress, Emily Dowd, Wuhu Feng, Martyn P. Chipperfield, and John J. Remedios
Atmos. Chem. Phys., 24, 10639–10653, https://doi.org/10.5194/acp-24-10639-2024, https://doi.org/10.5194/acp-24-10639-2024, 2024
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The leaks from the Nord Stream gas pipelines in September 2022 released a large amount of methane (CH4) into the atmosphere. We provide observational data from a satellite instrument that shows a large CH4 plume over the North Sea off the coast of Scandinavia. We use this together with atmospheric models to quantify the CH4 leaked into the atmosphere from the pipelines. We find that 219–427 Gg CH4 was emitted, making this the largest individual fossil-fuel-related CH4 leak on record.
Steffen Vanselow, Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Hartmut Boesch, and John P. Burrows
Atmos. Chem. Phys., 24, 10441–10473, https://doi.org/10.5194/acp-24-10441-2024, https://doi.org/10.5194/acp-24-10441-2024, 2024
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We developed an algorithm to automatically detect persistent methane source regions, to quantify their emissions and to determine their source types, by analyzing TROPOMI data from 2018–2021. The over 200 globally detected natural and anthropogenic source regions include small-scale point sources such as individual coal mines and larger-scale source regions such as wetlands and large oil and gas fields.
Debora Griffin, Jack Chen, Kerry Anderson, Paul Makar, Chris A. McLinden, Enrico Dammers, and Andre Fogal
Atmos. Chem. Phys., 24, 10159–10186, https://doi.org/10.5194/acp-24-10159-2024, https://doi.org/10.5194/acp-24-10159-2024, 2024
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Satellite-derived CO emissions provide new insights into the understanding of global CO emission rates from wildfires. We use TROPOMI satellite data to create a global inventory database of wildfire CO emissions. These satellite-derived wildfire emissions are used for the evaluation and improvement of existing fire emission inventories and to examine how the wildfire CO emissions have changed over the past 2 decades.
Matías Osorio, Alejandro Agesta, Tim Bösch, Nicolás Casaballe, Andreas Richter, Leonardo M. A. Alvarado, and Erna Frins
Atmos. Chem. Phys., 24, 7447–7465, https://doi.org/10.5194/acp-24-7447-2024, https://doi.org/10.5194/acp-24-7447-2024, 2024
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This study concerns the detection and quantification of long-transport emissions of a biomass burning event, which represents a major source of air pollutants, due to the release of large amounts of aerosols and chemical species into the atmosphere. The quantification was done using ground-based observations (which play an important role in assessing the abundance of trace gases and aerosols) over Montevideo (Uruguay) and using satellite observations.
Qiansi Tu, Frank Hase, Kai Qin, Jason Blake Cohen, Farahnaz Khosrawi, Xinrui Zou, Matthias Schneider, and Fan Lu
Atmos. Chem. Phys., 24, 4875–4894, https://doi.org/10.5194/acp-24-4875-2024, https://doi.org/10.5194/acp-24-4875-2024, 2024
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Four-year satellite observations of XCH4 are used to derive CH4 emissions in three regions of China’s coal-rich Shanxi province. The wind-assigned anomalies for two opposite wind directions are calculated, and the estimated emission rates are comparable to the current bottom-up inventory but lower than the CAMS and EDGAR inventories. This research enhances the understanding of emissions in Shanxi and supports climate mitigation strategies by validating emission inventories.
Paul S. Jeffery, James R. Drummond, Jiansheng Zou, and Kaley A. Walker
Atmos. Chem. Phys., 24, 4253–4263, https://doi.org/10.5194/acp-24-4253-2024, https://doi.org/10.5194/acp-24-4253-2024, 2024
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The MOPITT instrument has been monitoring carbon monoxide (CO) since March 2000. This dataset has been used for many applications; however, episodic emission events, which release large amounts of CO into the atmosphere, are a major source of uncertainty. This study presents a method for identifying these events by determining measurements that are unlikely to have typically arisen. The distribution and frequency of these flagged measurements in the MOPITT dataset are presented and discussed.
Ailish M. Graham, Richard J. Pope, Martyn P. Chipperfield, Sandip S. Dhomse, Matilda Pimlott, Wuhu Feng, Vikas Singh, Ying Chen, Oliver Wild, Ranjeet Sokhi, and Gufran Beig
Atmos. Chem. Phys., 24, 789–806, https://doi.org/10.5194/acp-24-789-2024, https://doi.org/10.5194/acp-24-789-2024, 2024
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Our paper uses novel satellite datasets and high-resolution emissions datasets alongside a back-trajectory model to investigate the balance of local and external sources influencing NOx air pollution changes in Delhi. We find in the post-monsoon season that NOx from local and non-local transport emissions contributes most to poor air quality in Delhi. Therefore, air quality mitigation strategies in Delhi and surrounding regions are used to control this issue.
Camille Viatte, Nadir Guendouz, Clarisse Dufaux, Arjan Hensen, Daan Swart, Martin Van Damme, Lieven Clarisse, Pierre Coheur, and Cathy Clerbaux
Atmos. Chem. Phys., 23, 15253–15267, https://doi.org/10.5194/acp-23-15253-2023, https://doi.org/10.5194/acp-23-15253-2023, 2023
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Ammonia (NH3) is an important air pollutant which, as a precursor of fine particulate matter, raises public health concerns. Models have difficulty predicting events of pollution associated with NH3 since ground-based observations of this gas are still relatively sparse and difficult to implement. We present the first relatively long (2.5 years) and continuous record of hourly NH3 concentrations in Paris to determine its temporal variabilities at different scales to unravel emission sources.
Hirofumi Ohyama, Matthias M. Frey, Isamu Morino, Kei Shiomi, Masahide Nishihashi, Tatsuya Miyauchi, Hiroko Yamada, Makoto Saito, Masanobu Wakasa, Thomas Blumenstock, and Frank Hase
Atmos. Chem. Phys., 23, 15097–15119, https://doi.org/10.5194/acp-23-15097-2023, https://doi.org/10.5194/acp-23-15097-2023, 2023
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We conducted a field campaign for CO2 column measurements in the Tokyo metropolitan area with three ground-based Fourier transform spectrometers. The model simulations using prior CO2 fluxes were generally in good agreement with the observations. We developed an urban-scale inversion system in which spatially resolved CO2 fluxes and a scaling factor of large point source emissions were estimated. The posterior total CO2 emissions agreed with emission inventories within the posterior uncertainty.
Xi Shao, Shu-Peng Ho, Xin Jing, Xinjia Zhou, Yong Chen, Tung-Chang Liu, Bin Zhang, and Jun Dong
Atmos. Chem. Phys., 23, 14187–14218, https://doi.org/10.5194/acp-23-14187-2023, https://doi.org/10.5194/acp-23-14187-2023, 2023
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Atmospheric water vapor plays an essential role in the global energy balance, hydrological cycle, and climate system. This paper characterizes and compares the global, latitudinal, and regional variabilities of COSMIC and ERA5 water vapor distribution, as well as the seasonality and long-term trends at selected pressure levels from 2007 to 2018. Evaluation of spatiotemporal variabilities of atmospheric water vapor ensures the qualities of COSMIC and reanalysis water vapor for climate studies.
Anthony Rey-Pommier, Frédéric Chevallier, Philippe Ciais, Jonilda Kushta, Theodoros Christoudias, I. Safak Bayram, and Jean Sciare
Atmos. Chem. Phys., 23, 13565–13583, https://doi.org/10.5194/acp-23-13565-2023, https://doi.org/10.5194/acp-23-13565-2023, 2023
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We use four years (2019–2022) of TROPOMI NO2 data to map NOx emissions in Qatar. We estimate average monthly emissions for the country and industrial facilities and derive an emission factor for the power sector. Monthly emissions have a weekly cycle reflecting the social norms in Qatar and an annual cycle consistent with the electricity production by gas-fired power plants. Their mean value is lower than the NOx emissions in global inventories but similar to the emissions reported for 2007.
Daniel A. Potts, Roger Timmis, Emma J. S. Ferranti, and Joshua D. Vande Hey
Atmos. Chem. Phys., 23, 4577–4593, https://doi.org/10.5194/acp-23-4577-2023, https://doi.org/10.5194/acp-23-4577-2023, 2023
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With the launch of the TROPOspheric Monitoring Instrument (TROPOMI) in 2017, it is now possible to observe pollutants emitted from individual industrial facilities on a daily basis around the globe. By using observations of nitrogen dioxide (NO2) from 16 different industrial sites, we show how the Coriolis effect influences the trajectory of these emission plumes as well as how the additional curvature can lead to a substantial underestimation of the calculated emissions.
Peng Yuan, Roeland Van Malderen, Xungang Yin, Hannes Vogelmann, Weiping Jiang, Joseph Awange, Bernhard Heck, and Hansjörg Kutterer
Atmos. Chem. Phys., 23, 3517–3541, https://doi.org/10.5194/acp-23-3517-2023, https://doi.org/10.5194/acp-23-3517-2023, 2023
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Water vapour plays an important role in various weather and climate processes. However, due to its large spatiotemporal variability, its high-accuracy quantification remains a challenge. In this study, 20+ years of GPS-derived integrated water vapour (IWV) retrievals in Europe were obtained. They were then used to characterise the temporal features of Europe's IWV and assess six atmospheric reanalyses. Results show that ERA5 outperforms the other reanalyses at most temporal scales.
Jing Wei, Zhanqing Li, Jun Wang, Can Li, Pawan Gupta, and Maureen Cribb
Atmos. Chem. Phys., 23, 1511–1532, https://doi.org/10.5194/acp-23-1511-2023, https://doi.org/10.5194/acp-23-1511-2023, 2023
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This study estimated the daily seamless 10 km ambient gaseous pollutants (NO2, SO2, and CO) across China using machine learning with extensive input variables measured on monitors, satellites, and models. Our dataset yields a high data quality via cross-validation at varying spatiotemporal scales and outperforms most previous related studies, making it most helpful to future (especially short-term) air pollution and environmental health-related studies.
Camille Viatte, Rimal Abeed, Shoma Yamanouchi, William C. Porter, Sarah Safieddine, Martin Van Damme, Lieven Clarisse, Beatriz Herrera, Michel Grutter, Pierre-Francois Coheur, Kimberly Strong, and Cathy Clerbaux
Atmos. Chem. Phys., 22, 12907–12922, https://doi.org/10.5194/acp-22-12907-2022, https://doi.org/10.5194/acp-22-12907-2022, 2022
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Large cities can experience high levels of fine particulate matter (PM2.5) pollution linked to ammonia (NH3) mainly emitted from agricultural activities. Using a combination of PM2.5 and NH3 measurements from in situ instruments, satellite infrared spectrometers, and atmospheric model simulations, we have demonstrated the role of NH3 and meteorological conditions on pollution events occurring over Paris, Toronto, and Mexico City.
Hossain Mohammed Syedul Hoque, Kengo Sudo, Hitoshi Irie, Alessandro Damiani, Manish Naja, and Al Mashroor Fatmi
Atmos. Chem. Phys., 22, 12559–12589, https://doi.org/10.5194/acp-22-12559-2022, https://doi.org/10.5194/acp-22-12559-2022, 2022
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Nitrogen dioxide (NO2) and formaldehyde (HCHO) are essential trace graces regulating tropospheric ozone chemistry. These trace constituents are measured using an optical passive remote sensing technique. In addition, NO2 and HCHO are simulated with a computer model and evaluated against the observations. Such evaluations are essential to assess model uncertainties and improve their predictability. The results yielded good agreement between the two datasets with some discrepancies.
Qiansi Tu, Matthias Schneider, Frank Hase, Farahnaz Khosrawi, Benjamin Ertl, Jaroslaw Necki, Darko Dubravica, Christopher J. Diekmann, Thomas Blumenstock, and Dianjun Fang
Atmos. Chem. Phys., 22, 9747–9765, https://doi.org/10.5194/acp-22-9747-2022, https://doi.org/10.5194/acp-22-9747-2022, 2022
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Three-year satellite observations and high-resolution model forecast of XCH4 are used to derive CH4 emissions in the USCB region, Poland – a region of intense coal mining activities. The wind-assigned anomalies for two opposite wind directions are calculated and the estimated emission rates are very close to the inventories and in reasonable agreement with the previous studies. Our method is quite robust and can serve as a simple method to estimate CH4 or CO2 emissions for other regions.
Pu Liu, Jia Ding, Lei Liu, Wen Xu, and Xuejun Liu
Atmos. Chem. Phys., 22, 9099–9110, https://doi.org/10.5194/acp-22-9099-2022, https://doi.org/10.5194/acp-22-9099-2022, 2022
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Ammonia (NH3) is the important alkaline gas and the key component of fine particulate matter. We used satellite-based observations to analyze the changes in hourly NH3 concentrations and estimated surface NH3 concentrations and NH3 emissions in China. This study shows enormous potential for using satellite data to estimate surface NH3 concentrations and NH3 emissions and provides an important reference for understanding NH3 variation in China.
Yohanna Villalobos, Peter J. Rayner, Jeremy D. Silver, Steven Thomas, Vanessa Haverd, Jürgen Knauer, Zoë M. Loh, Nicholas M. Deutscher, David W. T. Griffith, and David F. Pollard
Atmos. Chem. Phys., 22, 8897–8934, https://doi.org/10.5194/acp-22-8897-2022, https://doi.org/10.5194/acp-22-8897-2022, 2022
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We study the interannual variability in Australian carbon fluxes for 2015–2019 derived from OCO-2 satellite data. Our results suggest that Australia's semi-arid ecosystems are highly responsive to variations in climate drivers such as rainfall and temperature. We found that high rainfall and low temperatures recorded in 2016 led to an anomalous carbon sink over savanna and sparsely vegetated regions, while unprecedented dry and hot weather in 2019 led to anomalous carbon release.
Tianlang Zhao, Jingqiu Mao, William R. Simpson, Isabelle De Smedt, Lei Zhu, Thomas F. Hanisco, Glenn M. Wolfe, Jason M. St. Clair, Gonzalo González Abad, Caroline R. Nowlan, Barbara Barletta, Simone Meinardi, Donald R. Blake, Eric C. Apel, and Rebecca S. Hornbrook
Atmos. Chem. Phys., 22, 7163–7178, https://doi.org/10.5194/acp-22-7163-2022, https://doi.org/10.5194/acp-22-7163-2022, 2022
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Monitoring formaldehyde (HCHO) can help us understand Arctic vegetation change. Here, we compare satellite data and model and show that Alaska summertime HCHO is largely dominated by a background from methane oxidation during mild wildfire years and is dominated by wildfire (largely from direct emission of fire) during strong fire years. Consequently, it is challenging to use satellite HCHO to study vegetation change in the Arctic region.
Maria-Elissavet Koukouli, Konstantinos Michailidis, Pascal Hedelt, Isabelle A. Taylor, Antje Inness, Lieven Clarisse, Dimitris Balis, Dmitry Efremenko, Diego Loyola, Roy G. Grainger, and Christian Retscher
Atmos. Chem. Phys., 22, 5665–5683, https://doi.org/10.5194/acp-22-5665-2022, https://doi.org/10.5194/acp-22-5665-2022, 2022
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Volcanic eruptions eject large amounts of ash and trace gases into the atmosphere. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. The main aim of this paper is to present its extensive verification, accomplished within the ESA S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements, as well as assess its impact on the forecasts provided by CAMS.
Hao Yin, Youwen Sun, Justus Notholt, Mathias Palm, and Cheng Liu
Atmos. Chem. Phys., 22, 4167–4185, https://doi.org/10.5194/acp-22-4167-2022, https://doi.org/10.5194/acp-22-4167-2022, 2022
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In this study, we quantity the long-term variabilities and the underlying drivers of NO2 from 2005 to 2020 over the Yangtze River Delta (YRD), one of the most densely populated and highly industrialized city clusters in China. We reveal the significant effect of the Action Plan on the Prevention and Control of Air Pollution since 2013 adopted by the Chinese government to reduce NOx pollution. Our study can improve the understanding of pollution control measures on a regional scale.
Chloé Radice, Hélène Brogniez, Pierre-Emmanuel Kirstetter, and Philippe Chambon
Atmos. Chem. Phys., 22, 3811–3825, https://doi.org/10.5194/acp-22-3811-2022, https://doi.org/10.5194/acp-22-3811-2022, 2022
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A novel probabilistic approach is proposed to evaluate relative humidity (RH) profiles simulated by an atmospheric model with respect to satellite-based RH defined from probability distributions. It improves upon deterministic comparisons by enhancing the information content to enable a finer assessment of each model–observation discrepancy, highlighting significant departures within a deterministic confidence range. Geographical and vertical distributions of the model biases are discussed.
Manu Anna Thomas, Abhay Devasthale, and Tiina Nygård
Atmos. Chem. Phys., 21, 16593–16608, https://doi.org/10.5194/acp-21-16593-2021, https://doi.org/10.5194/acp-21-16593-2021, 2021
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The impact of transported pollutants and their spatial distribution in the Arctic are governed by the local atmospheric circulation or weather states. Therefore, we investigated eight different atmospheric circulation types observed during the spring season in the Arctic. Using satellite and reanalysis datasets, this study provides a comprehensive assessment of the typical circulation patterns that can lead to enhanced or reduced pollution concentrations in the different sectors of the Arctic.
Xin Tian, Yang Wang, Steffen Beirle, Pinhua Xie, Thomas Wagner, Jin Xu, Ang Li, Steffen Dörner, Bo Ren, and Xiaomei Li
Atmos. Chem. Phys., 21, 12867–12894, https://doi.org/10.5194/acp-21-12867-2021, https://doi.org/10.5194/acp-21-12867-2021, 2021
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The performances of two MAX-DOAS inversion algorithms were evaluated for various aerosol pollution scenarios. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. The evaluation results can effectively guide the application of the two inversion algorithms in the actual atmosphere and improve the accuracy of the actual inversion.
Rebecca D. Kutzner, Juan Cuesta, Pascale Chelin, Jean-Eudes Petit, Mokhtar Ray, Xavier Landsheere, Benoît Tournadre, Jean-Charles Dupont, Amandine Rosso, Frank Hase, Johannes Orphal, and Matthias Beekmann
Atmos. Chem. Phys., 21, 12091–12111, https://doi.org/10.5194/acp-21-12091-2021, https://doi.org/10.5194/acp-21-12091-2021, 2021
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Our work investigates the diurnal evolution of atmospheric ammonia concentrations during a major pollution event. It analyses it in regard of both chemical (gas–particle conversion) and physical (vertical mixing, meteorology) processes in the atmosphere. These mechanisms are key for understanding the evolution of the physicochemical state of the atmosphere; therefore, it clearly fits into the scope of Atmospheric Chemistry and Physics.
Youwen Sun, Hao Yin, Cheng Liu, Emmanuel Mahieu, Justus Notholt, Yao Té, Xiao Lu, Mathias Palm, Wei Wang, Changgong Shan, Qihou Hu, Min Qin, Yuan Tian, and Bo Zheng
Atmos. Chem. Phys., 21, 11759–11779, https://doi.org/10.5194/acp-21-11759-2021, https://doi.org/10.5194/acp-21-11759-2021, 2021
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The variability, sources, and transport of ethane (C2H6) over eastern China from 2015 to 2020 were studied using ground-based Fourier transform infrared (FTIR) spectroscopy and GEOS-Chem simulations. C2H6 variability is driven by both meteorological and emission factors. The reduction in C2H6 in recent years over eastern China points to air quality improvement in China.
Youwen Sun, Hao Yin, Cheng Liu, Lin Zhang, Yuan Cheng, Mathias Palm, Justus Notholt, Xiao Lu, Corinne Vigouroux, Bo Zheng, Wei Wang, Nicholas Jones, Changong Shan, Min Qin, Yuan Tian, Qihou Hu, Fanhao Meng, and Jianguo Liu
Atmos. Chem. Phys., 21, 6365–6387, https://doi.org/10.5194/acp-21-6365-2021, https://doi.org/10.5194/acp-21-6365-2021, 2021
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This study mapped the drivers of HCHO variability from 2015 to 2019 over eastern China. Hydroxyl (OH) radical production rates from HCHO photolysis were evaluated. The relative contributions of emitted and photochemical sources to the observed HCHO abundance were analyzed. Contributions of various emission sources and geographical regions to the observed HCHO summertime enhancements were determined.
Fernando Chouza, Thierry Leblanc, Mark Brewer, Patrick Wang, Sabino Piazzolla, Gabriele Pfister, Rajesh Kumar, Carl Drews, Simone Tilmes, Louisa Emmons, and Matthew Johnson
Atmos. Chem. Phys., 21, 6129–6153, https://doi.org/10.5194/acp-21-6129-2021, https://doi.org/10.5194/acp-21-6129-2021, 2021
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The tropospheric ozone lidar at the JPL Table Mountain Facility (TMF) was used to investigate the impact of Los Angeles (LA) Basin pollution transport and stratospheric intrusions in the planetary boundary layer on the San Gabriel Mountains. The results of this study indicate a dominant role of the LA Basin pollution on days when high ozone levels were observed at TMF (March–October period).
Maria-Elissavet Koukouli, Ioanna Skoulidou, Andreas Karavias, Isaak Parcharidis, Dimitris Balis, Astrid Manders, Arjo Segers, Henk Eskes, and Jos van Geffen
Atmos. Chem. Phys., 21, 1759–1774, https://doi.org/10.5194/acp-21-1759-2021, https://doi.org/10.5194/acp-21-1759-2021, 2021
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In recent years, satellite observations have contributed to monitoring air quality. During the first COVID-19 lockdown, lower levels of nitrogen dioxide were observed over Greece by S5P/TROPOMI for March and April 2020 (than the preceding year) due to decreased transport emissions. Taking meteorology into account, using LOTOS-EUROS CTM simulations, the resulting decline due to the lockdown was estimated to range between 0 % and −37 % for the five largest Greek cities, with an average of ~ −10 %.
Tobias Borsdorff, Agustín García Reynoso, Gilberto Maldonado, Bertha Mar-Morales, Wolfgang Stremme, Michel Grutter, and Jochen Landgraf
Atmos. Chem. Phys., 20, 15761–15774, https://doi.org/10.5194/acp-20-15761-2020, https://doi.org/10.5194/acp-20-15761-2020, 2020
Sören Johansson, Michael Höpfner, Oliver Kirner, Ingo Wohltmann, Silvia Bucci, Bernard Legras, Felix Friedl-Vallon, Norbert Glatthor, Erik Kretschmer, Jörn Ungermann, and Gerald Wetzel
Atmos. Chem. Phys., 20, 14695–14715, https://doi.org/10.5194/acp-20-14695-2020, https://doi.org/10.5194/acp-20-14695-2020, 2020
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We present high-resolution measurements of pollutant trace gases (PAN, C2H2, and HCOOH) in the Asian monsoon UTLS from the airborne limb imager GLORIA during StratoClim 2017. Enhancements are observed up to 16 km altitude, and PAN and C2H2 even up to 18 km. Two atmospheric models, CAMS and EMAC, reproduce the pollutant's large-scale structures but not finer structures. Convection is investigated using backward trajectories of the models ATLAS and TRACZILLA with advanced detection of convection.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Chem. Phys., 20, 12285–12312, https://doi.org/10.5194/acp-20-12285-2020, https://doi.org/10.5194/acp-20-12285-2020, 2020
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In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
Leonie Bernet, Elmar Brockmann, Thomas von Clarmann, Niklaus Kämpfer, Emmanuel Mahieu, Christian Mätzler, Gunter Stober, and Klemens Hocke
Atmos. Chem. Phys., 20, 11223–11244, https://doi.org/10.5194/acp-20-11223-2020, https://doi.org/10.5194/acp-20-11223-2020, 2020
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With global warming, water vapour increases in the atmosphere. Water vapour is an important gas because it is a natural greenhouse gas and affects the formation of clouds, rain and snow. How much water vapour increases can vary in different regions of the world. To verify if it increases as expected on a regional scale, we analysed water vapour measurements in Switzerland. We found that water vapour generally increases as expected from temperature changes, except in winter.
Shannon Hicks-Jalali, Robert J. Sica, Giovanni Martucci, Eliane Maillard Barras, Jordan Voirin, and Alexander Haefele
Atmos. Chem. Phys., 20, 9619–9640, https://doi.org/10.5194/acp-20-9619-2020, https://doi.org/10.5194/acp-20-9619-2020, 2020
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We have calculated an 11.5-year water vapour climatology using the Raman Lidar for Meteorological Observations (RALMO), located in Payerne, Switzerland. The climatology shows that the highest water vapour concentrations are in the summer months and the lowest in the winter months. We present for the first time height-resolved water vapour trends, which show that water vapour increases specific humidity by between 5 % and 15 % per decade depending on the altitude.
Yohanna Villalobos, Peter Rayner, Steven Thomas, and Jeremy Silver
Atmos. Chem. Phys., 20, 8473–8500, https://doi.org/10.5194/acp-20-8473-2020, https://doi.org/10.5194/acp-20-8473-2020, 2020
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Estimated carbon fluxes for Australia are subject to considerable uncertainty. We ran simulation experiments over Australia to determine how much these uncertainties can be constrained using satellite data. We found that the satellite data has the potential to reduce these uncertainties up to 80 % across the whole continent. For 1 month, this percentage corresponds to 0.51 Pg C y-1 for Australia. This method could lead to significantly more accurate estimates of Australia's carbon budget.
Bo Zheng, Frédéric Chevallier, Philippe Ciais, Grégoire Broquet, Yilong Wang, Jinghui Lian, and Yuanhong Zhao
Atmos. Chem. Phys., 20, 8501–8510, https://doi.org/10.5194/acp-20-8501-2020, https://doi.org/10.5194/acp-20-8501-2020, 2020
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The Paris Climate Agreement requires all parties to report CO2 emissions regularly. Given the self-reporting nature of this system, it is critical to evaluate the emission reports with independent observation systems. Here we present the direct observations of city CO2 plumes from space and the quantification of CO2 emissions from these observations over the largest emitter country China. The emissions from 46 hot-spot regions representing 13 % of China's total emissions can be well constrained.
Jeffery Langille, Adam Bourassa, Laura L. Pan, Daniel Letros, Brian Solheim, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 20, 5477–5486, https://doi.org/10.5194/acp-20-5477-2020, https://doi.org/10.5194/acp-20-5477-2020, 2020
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Water vapour (WV) is a highly variable and extremely important trace gas in Earth’s atmosphere. Due to its radiative and chemical properties, it is coupled to the climate in an extremely complex manner. This is especially true in the lowermost stratosphere (LMS). Despite its importance, the physical processes that control mixing and the distribution of WV in the LMS are poorly understood. This study provides observational evidence of moistening the LMS via mixing across the subtropical jet.
Youwen Sun, Cheng Liu, Lin Zhang, Mathias Palm, Justus Notholt, Hao Yin, Corinne Vigouroux, Erik Lutsch, Wei Wang, Changong Shan, Thomas Blumenstock, Tomoo Nagahama, Isamu Morino, Emmanuel Mahieu, Kimberly Strong, Bavo Langerock, Martine De Mazière, Qihou Hu, Huifang Zhang, Christof Petri, and Jianguo Liu
Atmos. Chem. Phys., 20, 5437–5456, https://doi.org/10.5194/acp-20-5437-2020, https://doi.org/10.5194/acp-20-5437-2020, 2020
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We present multiyear time series of ground-based Fourier-transform infrared spectroscopy measurements of HCN in densely populated eastern China. The seasonality and interannual variability of tropospheric HCN columns were investigated. The potential sources that drive the observed HCN seasonality and interannual variability were determined using a GEOS-Chem tagged CO simulation, global fire maps, and potential source contribution function values calculated using HYSPLIT back trajectories.
Enrico Dammers, Chris A. McLinden, Debora Griffin, Mark W. Shephard, Shelley Van Der Graaf, Erik Lutsch, Martijn Schaap, Yonatan Gainairu-Matz, Vitali Fioletov, Martin Van Damme, Simon Whitburn, Lieven Clarisse, Karen Cady-Pereira, Cathy Clerbaux, Pierre Francois Coheur, and Jan Willem Erisman
Atmos. Chem. Phys., 19, 12261–12293, https://doi.org/10.5194/acp-19-12261-2019, https://doi.org/10.5194/acp-19-12261-2019, 2019
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Ammonia is an essential molecule in the environment, but at its current levels it is unsustainable. However, the emissions are highly uncertain. We explore the use of satellites to estimate the ammonia lifetime and emissions around point sources to help improve the budget. The same method applied to different satellite instruments shows consistent results. Comparison to the emission inventories shows that those are underestimating emissions of point sources by on average a factor of 2.5.
Klemens Hocke, Leonie Bernet, Jonas Hagen, Axel Murk, Matthias Renker, and Christian Mätzler
Atmos. Chem. Phys., 19, 12083–12090, https://doi.org/10.5194/acp-19-12083-2019, https://doi.org/10.5194/acp-19-12083-2019, 2019
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The Tropospheric Water Radiometer (TROWARA) observed an enhanced intensity of short-term integrated water vapour (IWV) fluctuations during daytime in summer. These IWV fluctuations are possibly related to latent heat flux and thermal convective activity in the lower troposphere. The observed climatology and spectra of IWV fluctuations might be useful for modelling studies of water vapour convection in the atmospheric boundary layer at mid latitudes.
Xiaoyi Zhao, Debora Griffin, Vitali Fioletov, Chris McLinden, Jonathan Davies, Akira Ogyu, Sum Chi Lee, Alexandru Lupu, Michael D. Moran, Alexander Cede, Martin Tiefengraber, and Moritz Müller
Atmos. Chem. Phys., 19, 10619–10642, https://doi.org/10.5194/acp-19-10619-2019, https://doi.org/10.5194/acp-19-10619-2019, 2019
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New nitrogen dioxide (NO2) retrieval algorithms are developed for Pandora zenith-sky measurements. A column-to-surface conversion look-up table was produced for the Pandora instruments; therefore, quick and practical Pandora-based surface NO2 concentration data can be obtained for air quality monitoring purposes. It is demonstrated that the surface NO2 concentration is controlled not only by the planetary boundary layer height but also by both boundary layer dynamics and photochemistry.
Ka Lok Chan, Zhuoru Wang, Aijun Ding, Klaus-Peter Heue, Yicheng Shen, Jing Wang, Feng Zhang, Yining Shi, Nan Hao, and Mark Wenig
Atmos. Chem. Phys., 19, 10051–10071, https://doi.org/10.5194/acp-19-10051-2019, https://doi.org/10.5194/acp-19-10051-2019, 2019
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The paper presents long-term observations of atmospheric nitrogen dioxide (NO2) and formaldehyde (HCHO) in Nanjing using a MAX-DOAS instrument. The measurements were performed from April 2013 to February 2017. The MAX-DOAS measurements of NO2 and HCHO are used to validate OMI satellite observations and to investigate the influences of region transport of air pollutants on the air quality in Nanjing.
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