Articles | Volume 18, issue 5
https://doi.org/10.5194/acp-18-3677-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-3677-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Mar 2018
Research article |
| 13 Mar 2018
| 13 Mar 2018
In situ measurements of desert dust particles above the western Mediterranean Sea with the balloon-borne Light Optical Aerosol Counter/sizer (LOAC) during the ChArMEx campaign of summer 2013
Jean-Baptiste Renard
CORRESPONDING AUTHOR
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace
(LPC2E), UMR CNRS-Université d'Orléans, 3A avenue de la recherche
scientifique, Orléans, France
François Dulac
Laboratoire des Sciences du Climat et de l'Environnement (LSCE), UMR
CEA-CNRS-UVSQ, IPSL, Université Paris-Saclay, CEA Saclay 701,
Gif-sur-Yvette, France
Pierre Durand
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UT3,
Toulouse, France
Quentin Bourgeois
Department of Meteorology and Bolin Centre for Climate Research,
Stockholm University, Stockholm, Sweden
Cyrielle Denjean
Centre National d'Etudes Spatiales (CNES), 18 Avenue Edouard Belin,
Toulouse, France
now at: Centre National de Recherches Météorologiques (CNRM),
UMR 3589 Météo-France-CNRS, OMP, Météo-France, Toulouse, France
Damien Vignelles
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace
(LPC2E), UMR CNRS-Université d'Orléans, 3A avenue de la recherche
scientifique, Orléans, France
Benoit Couté
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace
(LPC2E), UMR CNRS-Université d'Orléans, 3A avenue de la recherche
scientifique, Orléans, France
Matthieu Jeannot
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace
(LPC2E), UMR CNRS-Université d'Orléans, 3A avenue de la recherche
scientifique, Orléans, France
now at: MeteoModem company, Chemin du Moulin, Ury, France
Nicolas Verdier
Centre National d'Etudes Spatiales (CNES), 18 Avenue Edouard Belin,
Toulouse, France
Marc Mallet
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UT3,
Toulouse, France
now at: Centre National de Recherches Météorologiques (CNRM),
UMR 3589 Météo-France-CNRS, OMP, Météo-France, Toulouse, France
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Thomas Drugé, Pierre Nabat, Martine Michou, and Marc Mallet
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Patrick Dewald, Tobias Seubert, Simone T. Andersen, Gunther N. T. E. Türk, Jan Schuladen, Max R. McGillen, Cyrielle Denjean, Jean-Claude Etienne, Olivier Garrouste, Marina Jamar, Sergio Harb, Manuela Cirtog, Vincent Michoud, Mathieu Cazaunau, Antonin Bergé, Christopher Cantrell, Sebastien Dusanter, Bénédicte Picquet-Varrault, Alexandre Kukui, Chaoyang Xue, Abdelwahid Mellouki, Jos Lelieveld, and John N. Crowley
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Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Véronique Pont, Mathilde Arnaud, Thierry Bourrianne, Maria Dias Alves, and Eric Gardrat
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Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
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Philippe Ricaud, Massimo Del Guasta, Angelo Lupi, Romain Roehrig, Eric Bazile, Pierre Durand, Jean-Luc Attié, Alessia Nicosia, and Paolo Grigioni
Atmos. Chem. Phys., 24, 613–630, https://doi.org/10.5194/acp-24-613-2024, https://doi.org/10.5194/acp-24-613-2024, 2024
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Clouds affect the Earth's climate in ways that depend on the type of cloud (solid/liquid water). From observations at Concordia (Antarctica), we show that in supercooled liquid water (liquid water for temperatures below 0°C) clouds (SLWCs), temperature and SLWC radiative forcing increase with liquid water (up to 70 W m−2). We extrapolated that the maximum SLWC radiative forcing can reach 40 W m−2 over the Antarctic Peninsula, highlighting the importance of SLWCs for global climate prediction.
Florian Dupuy, Pierre Durand, and Thierry Hedde
Nonlin. Processes Geophys., 30, 553–570, https://doi.org/10.5194/npg-30-553-2023, https://doi.org/10.5194/npg-30-553-2023, 2023
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Forecasting near-surface winds over complex terrain requires high-resolution numerical weather prediction models, which drastically increase the duration of simulations and hinder them in running on a routine basis. A faster alternative is statistical downscaling. We explore different ways of calculating near-surface wind speed and direction using artificial intelligence algorithms based on various convolutional neural networks in order to find the best approach for wind downscaling.
Lambert Delbeke, Chien Wang, Pierre Tulet, Cyrielle Denjean, Maurin Zouzoua, Nicolas Maury, and Adrien Deroubaix
Atmos. Chem. Phys., 23, 13329–13354, https://doi.org/10.5194/acp-23-13329-2023, https://doi.org/10.5194/acp-23-13329-2023, 2023
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Low-level stratiform clouds (LLSCs) appear frequently over southern West Africa during the West African monsoon. Local and remote aerosol sources (biomass burning aerosols from central Africa) play a significant role in the LLSC life cycle. Based on measurements by the DACCIWA campaign, large-eddy simulation (LES) was conducted using different aerosol scenarios. The results show that both indirect and semi-direct effects can act individually or jointly to influence the life cycles of LLSCs.
Ian Chang, Lan Gao, Connor J. Flynn, Yohei Shinozuka, Sarah J. Doherty, Michael S. Diamond, Karla M. Longo, Gonzalo A. Ferrada, Gregory R. Carmichael, Patricia Castellanos, Arlindo M. da Silva, Pablo E. Saide, Calvin Howes, Zhixin Xue, Marc Mallet, Ravi Govindaraju, Qiaoqiao Wang, Yafang Cheng, Yan Feng, Sharon P. Burton, Richard A. Ferrare, Samuel E. LeBlanc, Meloë S. Kacenelenbogen, Kristina Pistone, Michal Segal-Rozenhaimer, Kerry G. Meyer, Ju-Mee Ryoo, Leonhard Pfister, Adeyemi A. Adebiyi, Robert Wood, Paquita Zuidema, Sundar A. Christopher, and Jens Redemann
Atmos. Chem. Phys., 23, 4283–4309, https://doi.org/10.5194/acp-23-4283-2023, https://doi.org/10.5194/acp-23-4283-2023, 2023
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Abundant aerosols are present above low-level liquid clouds over the southeastern Atlantic during late austral spring. The model simulation differences in the proportion of aerosol residing in the planetary boundary layer and in the free troposphere can greatly affect the regional aerosol radiative effects. This study examines the aerosol loading and fractional aerosol loading in the free troposphere among various models and evaluates them against measurements from the NASA ORACLES campaign.
Thomas Drugé, Pierre Nabat, Marc Mallet, Martine Michou, Samuel Rémy, and Oleg Dubovik
Atmos. Chem. Phys., 22, 12167–12205, https://doi.org/10.5194/acp-22-12167-2022, https://doi.org/10.5194/acp-22-12167-2022, 2022
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This study presents the implementation of brown carbon in the atmospheric component of the CNRM global climate model and particularly in its aerosol scheme TACTIC. Several simulations were carried out with this climate model, over the period 2000–2014, to evaluate the model by comparison with different reference datasets (PARASOL-GRASP, OMI-OMAERUVd, MACv2, FMI_SAT, AERONET) and to analyze the brown carbon radiative and climatic effects.
Marie Mazoyer, Frédéric Burnet, and Cyrielle Denjean
Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, https://doi.org/10.5194/acp-22-11305-2022, 2022
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The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
Michael John Weston, Stuart John Piketh, Frédéric Burnet, Stephen Broccardo, Cyrielle Denjean, Thierry Bourrianne, and Paola Formenti
Atmos. Chem. Phys., 22, 10221–10245, https://doi.org/10.5194/acp-22-10221-2022, https://doi.org/10.5194/acp-22-10221-2022, 2022
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An aerosol-aware microphysics scheme is evaluated for fog cases in Namibia. AEROCLO-sA campaign observations are used to access and parameterise the model. The model cloud condensation nuclei activation is lower than the observations. The scheme is designed for clouds with updrafts, while fog typically forms in stable conditions. A pseudo updraft speed assigned to the lowest model levels helps achieve more realistic cloud droplet number concentration and size distribution in the model.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Karine Desboeufs, Franck Fu, Matthieu Bressac, Antonio Tovar-Sánchez, Sylvain Triquet, Jean-François Doussin, Chiara Giorio, Patrick Chazette, Julie Disnaquet, Anaïs Feron, Paola Formenti, Franck Maisonneuve, Araceli Rodríguez-Romero, Pascal Zapf, François Dulac, and Cécile Guieu
Atmos. Chem. Phys., 22, 2309–2332, https://doi.org/10.5194/acp-22-2309-2022, https://doi.org/10.5194/acp-22-2309-2022, 2022
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This article reports the first concurrent sampling of wet deposition samples and surface seawater and was performed during the PEACETIME cruise in the remote Mediterranean (May–June 2017). Through the chemical composition of trace metals (TMs) in these samples, it emphasizes the decrease of atmospheric metal pollution in this area during the last few decades and the critical role of wet deposition as source of TMs for Mediterranean surface seawater, especially for intense dust deposition events.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Michal Segal Rozenhaimer, Meloë Kacenelenbogen, Yohei Shinozuka, Connor Flynn, Rich Ferrare, Sharon Burton, Chris Hostetler, Marc Mallet, and Paquita Zuidema
Atmos. Meas. Tech., 15, 61–77, https://doi.org/10.5194/amt-15-61-2022, https://doi.org/10.5194/amt-15-61-2022, 2022
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This work presents heating rates derived from aircraft observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS). We separate the total heating rates into aerosol and gas (primarily water vapor) absorption and explore some of the co-variability of heating rate profiles and their primary drivers, leading to the development of a new concept: the heating rate efficiency (HRE; the heating rate per unit aerosol extinction).
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Matthieu Bressac, Thibaut Wagener, Nathalie Leblond, Antonio Tovar-Sánchez, Céline Ridame, Vincent Taillandier, Samuel Albani, Sophie Guasco, Aurélie Dufour, Stéphanie H. M. Jacquet, François Dulac, Karine Desboeufs, and Cécile Guieu
Biogeosciences, 18, 6435–6453, https://doi.org/10.5194/bg-18-6435-2021, https://doi.org/10.5194/bg-18-6435-2021, 2021
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Phytoplankton growth is limited by the availability of iron in about 50 % of the ocean. Atmospheric deposition of desert dust represents a key source of iron. Here, we present direct observations of dust deposition in the Mediterranean Sea. A key finding is that the input of iron from dust primarily occurred in the deep ocean, while previous studies mainly focused on the ocean surface. This new insight will enable us to better represent controls on global marine productivity in models.
Sebastian Düsing, Albert Ansmann, Holger Baars, Joel C. Corbin, Cyrielle Denjean, Martin Gysel-Beer, Thomas Müller, Laurent Poulain, Holger Siebert, Gerald Spindler, Thomas Tuch, Birgit Wehner, and Alfred Wiedensohler
Atmos. Chem. Phys., 21, 16745–16773, https://doi.org/10.5194/acp-21-16745-2021, https://doi.org/10.5194/acp-21-16745-2021, 2021
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The work deals with optical properties of aerosol particles in dried and atmospheric states. Based on two measurement campaigns in the rural background of central Europe, different measurement approaches were compared with each other, such as modeling based on Mie theory and direct in situ or remote sensing measurements. Among others, it was shown that the aerosol extinction-to-backscatter ratio is relative humidity dependent, and refinement with respect to the model input parameters is needed.
Isabelle Chiapello, Paola Formenti, Lydie Mbemba Kabuiku, Fabrice Ducos, Didier Tanré, and François Dulac
Atmos. Chem. Phys., 21, 12715–12737, https://doi.org/10.5194/acp-21-12715-2021, https://doi.org/10.5194/acp-21-12715-2021, 2021
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The Mediterranean atmosphere is impacted by a variety of particle pollution, which exerts a complex pressure on climate and air quality. We analyze the 2005–2013 POLDER-3 satellite advanced aerosol data set over the Western Mediterranean Sea. Aerosols' spatial distribution and temporal evolution suggests a large-scale improvement of air quality related to the fine aerosol component, most probably resulting from reduction of anthropogenic particle emissions in the surrounding European countries.
Julien Jouanno, Rachid Benshila, Léo Berline, Antonin Soulié, Marie-Hélène Radenac, Guillaume Morvan, Frédéric Diaz, Julio Sheinbaum, Cristele Chevalier, Thierry Thibaut, Thomas Changeux, Frédéric Menard, Sarah Berthet, Olivier Aumont, Christian Ethé, Pierre Nabat, and Marc Mallet
Geosci. Model Dev., 14, 4069–4086, https://doi.org/10.5194/gmd-14-4069-2021, https://doi.org/10.5194/gmd-14-4069-2021, 2021
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The tropical Atlantic has been facing a massive proliferation of Sargassum since 2011, with severe environmental and socioeconomic impacts. We developed a modeling framework based on the NEMO ocean model, which integrates transport by currents and waves, and physiology of Sargassum with varying internal nutrient quota, and considers stranding at the coast. Results demonstrate the ability of the model to reproduce and forecast the seasonal cycle and large-scale distribution of Sargassum biomass.
Thomas Drugé, Pierre Nabat, Marc Mallet, and Samuel Somot
Atmos. Chem. Phys., 21, 7639–7669, https://doi.org/10.5194/acp-21-7639-2021, https://doi.org/10.5194/acp-21-7639-2021, 2021
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This study presents the surface mass concentration and AOD evolution of various aerosols over the Euro-Mediterranean region between the end of the 20th century and the mid-21st century. This study also describes the part of the expected climate change over the Euro-Mediterranean region that can be explained by the evolution of these different aerosols.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Cécile Debevec, Stéphane Sauvage, Valérie Gros, Thérèse Salameh, Jean Sciare, François Dulac, and Nadine Locoge
Atmos. Chem. Phys., 21, 1449–1484, https://doi.org/10.5194/acp-21-1449-2021, https://doi.org/10.5194/acp-21-1449-2021, 2021
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This study provides a better characterization of the seasonal variations in VOC sources impacting the western Mediterranean region, based on a comprehensive chemical composition measured over 25 months at a representative receptor site (Ersa) and by determining factors controlling their temporal variations. Some insights into dominant drivers for VOC concentration variations in Europe are also provided, built on comparisons of Ersa observations with the concomitant ones of 17 European sites.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Ghassan Taha, Mariam Tidiga, Maxim Eremenko, Adriana Bossolasco, Fabrice Jégou, Jean-Baptiste Renard, and Bernard Legras
Atmos. Chem. Phys., 21, 535–560, https://doi.org/10.5194/acp-21-535-2021, https://doi.org/10.5194/acp-21-535-2021, 2021
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The year 2019 was particularly rich for the stratospheric aerosol layer due to two volcanic eruptions (at Raikoke and Ulawun) and wildfire events. With satellite observations and models, we describe the exceptionally complex situation following the Raikoke eruption. The respective plume overwhelmed the Northern Hemisphere stratosphere in terms of aerosol load and resulted in the highest climate impact throughout the past decade.
Cécile Guieu, Fabrizio D'Ortenzio, François Dulac, Vincent Taillandier, Andrea Doglioli, Anne Petrenko, Stéphanie Barrillon, Marc Mallet, Pierre Nabat, and Karine Desboeufs
Biogeosciences, 17, 5563–5585, https://doi.org/10.5194/bg-17-5563-2020, https://doi.org/10.5194/bg-17-5563-2020, 2020
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We describe here the objectives and strategy of the PEACETIME project and cruise, dedicated to dust deposition and its impacts in the Mediterranean Sea. Our strategy to go a step further forward than in previous approaches in understanding these impacts by catching a real deposition event at sea is detailed. We summarize the work performed at sea, the type of data acquired and their valorization in the papers published in the special issue.
Marc Mallet, Fabien Solmon, Pierre Nabat, Nellie Elguindi, Fabien Waquet, Dominique Bouniol, Andrew Mark Sayer, Kerry Meyer, Romain Roehrig, Martine Michou, Paquita Zuidema, Cyrille Flamant, Jens Redemann, and Paola Formenti
Atmos. Chem. Phys., 20, 13191–13216, https://doi.org/10.5194/acp-20-13191-2020, https://doi.org/10.5194/acp-20-13191-2020, 2020
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This paper presents numerical simulations using two regional climate models to study the impact of biomass fire plumes from central Africa on the radiative balance of this region. The results indicate that biomass fires can either warm the regional climate when they are located above low clouds or cool it when they are located above land. They can also alter sea and land surface temperatures by decreasing solar radiation at the surface. Finally, they can also modify the atmospheric dynamics.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
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In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Pierre Nabat, Samuel Somot, Christophe Cassou, Marc Mallet, Martine Michou, Dominique Bouniol, Bertrand Decharme, Thomas Drugé, Romain Roehrig, and David Saint-Martin
Atmos. Chem. Phys., 20, 8315–8349, https://doi.org/10.5194/acp-20-8315-2020, https://doi.org/10.5194/acp-20-8315-2020, 2020
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The present work aims at better understanding regional climate–aerosol interactions over the Euro-Mediterranean region by studying the relationships between aerosols and atmospheric circulation. Based on 40-year regional climate simulations (1979–2018), our results show the role of the North Atlantic Oscillation in driving the interannual aerosol variability, and that of weather regimes for the daily variability, with ensuing effects on shortwave surface radiation and surface temperature.
Cyrielle Denjean, Thierry Bourrianne, Frederic Burnet, Marc Mallet, Nicolas Maury, Aurélie Colomb, Pamela Dominutti, Joel Brito, Régis Dupuy, Karine Sellegri, Alfons Schwarzenboeck, Cyrille Flamant, and Peter Knippertz
Atmos. Chem. Phys., 20, 4735–4756, https://doi.org/10.5194/acp-20-4735-2020, https://doi.org/10.5194/acp-20-4735-2020, 2020
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This paper presents aircraft measurements of aerosol optical properties over southern West Africa. We show that aerosol optical properties in the boundary layer were dominated by a persistent biomass burning loading from the Southern Hemisphere. Biomass burning aerosols were more light absorbing that those previously measured in other areas (Amazonia, North America). Our study suggests that lens-coated black carbon particles were the dominant absorber for these biomass burning aerosols.
Philippe Ricaud, Massimo Del Guasta, Eric Bazile, Niramson Azouz, Angelo Lupi, Pierre Durand, Jean-Luc Attié, Dana Veron, Vincent Guidard, and Paolo Grigioni
Atmos. Chem. Phys., 20, 4167–4191, https://doi.org/10.5194/acp-20-4167-2020, https://doi.org/10.5194/acp-20-4167-2020, 2020
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Thin (~ 100 m) supercooled liquid water (SLW, water staying in liquid phase below 0 °C) clouds have been detected, analysed, and modelled over the Dome C (Concordia, Antarctica) station during the austral summer 2018–2019 using observations and meteorological analyses. The SLW clouds were observed at the top of the planetary boundary layer and the SLW content was always strongly underestimated by the model indicating an incorrect simulation of the surface energy budget of the Antarctic Plateau.
Sophie L. Haslett, Jonathan W. Taylor, Mathew Evans, Eleanor Morris, Bernhard Vogel, Alima Dajuma, Joel Brito, Anneke M. Batenburg, Stephan Borrmann, Johannes Schneider, Christiane Schulz, Cyrielle Denjean, Thierry Bourrianne, Peter Knippertz, Régis Dupuy, Alfons Schwarzenböck, Daniel Sauer, Cyrille Flamant, James Dorsey, Ian Crawford, and Hugh Coe
Atmos. Chem. Phys., 19, 15217–15234, https://doi.org/10.5194/acp-19-15217-2019, https://doi.org/10.5194/acp-19-15217-2019, 2019
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Three aircraft datasets from the DACCIWA campaign in summer 2016 are used here to show there is a background mass of pollution present in the lower atmosphere in southern West Africa. We suggest that this likely comes from biomass burning in central and southern Africa, which has been carried into the region over the Atlantic Ocean. This would have a negative health impact on populations living near the coast and may alter the impact of growing city emissions on cloud formation and the monsoon.
Jean-Baptiste Renard, Gwenaël Berthet, Anny-Chantal Levasseur-Regourd, Sergey Beresnev, Alain Miffre, Patrick Rairoux, Damien Vignelles, and Fabrice Jégou
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-904, https://doi.org/10.5194/acp-2019-904, 2019
Revised manuscript not accepted
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Water and sulfuric acid droplets are the main component of stratospheric aerosols. Field measurements have shown that non-sulfate materials (NSPs) are also present. NSPs, released from Earth and from space, present a wide variety of sizes, compositions and shapes. New balloon counting measurements have shown the presence of enhanced-concentrations layers. We may conclude that the concentrations and the vertical distributions of NSPs are highly variable and mainly originate from Earth.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Erika Brattich, Encarnación Serrano Castillo, Fabrizio Giulietti, Jean-Baptiste Renard, Sachi N. Tripathi, Kunal Ghosh, Gwenael Berthet, Damien Vignelles, and Laura Tositti
Ann. Geophys., 37, 389–403, https://doi.org/10.5194/angeo-37-389-2019, https://doi.org/10.5194/angeo-37-389-2019, 2019
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This paper describes the aerosol measurement setup and results obtained from the BEXUS18 stratospheric balloon within the A5-Unib (Advanced Atmospheric Aerosol Acquisition and Analysis) experiment performed on 10 October 2014 in northern Sweden (Kiruna). The experiment and the results here presented broaden the understanding of the processes linking the presence of charges with particles all over the vertical heights from the ground to the stratosphere.
Marc Mallet, Pierre Nabat, Paquita Zuidema, Jens Redemann, Andrew Mark Sayer, Martin Stengel, Sebastian Schmidt, Sabrina Cochrane, Sharon Burton, Richard Ferrare, Kerry Meyer, Pablo Saide, Hiren Jethva, Omar Torres, Robert Wood, David Saint Martin, Romain Roehrig, Christina Hsu, and Paola Formenti
Atmos. Chem. Phys., 19, 4963–4990, https://doi.org/10.5194/acp-19-4963-2019, https://doi.org/10.5194/acp-19-4963-2019, 2019
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The model is able to represent LWP but not the LCF. AOD is consistent over the continent but also over ocean (ACAOD). Differences are observed in SSA due to the absence of internal mixing in ALADIN-Climate. A significant regional gradient of the forcing at TOA is observed. An intense positive forcing is simulated over Gabon. Results highlight the significant effect of enhanced moisture on BBA extinction. The surface dimming modifies the energy budget.
Marie Mazoyer, Frédéric Burnet, Cyrielle Denjean, Gregory C. Roberts, Martial Haeffelin, Jean-Charles Dupont, and Thierry Elias
Atmos. Chem. Phys., 19, 4323–4344, https://doi.org/10.5194/acp-19-4323-2019, https://doi.org/10.5194/acp-19-4323-2019, 2019
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In situ microphysical measurements collected during 23 fog events at SIRTA (south of Paris) are examined here. An original iterative method based on the κ-Köhler theory has been used to compute statistics of their activation properties. Useful information is provided to constrain and validate numerical simulations. The paper demonstrates that supersaturation encountered in these fogs is too low to observe a correlation between concentrations of aerosols > 200 nm and droplet concentrations.
Thomas Drugé, Pierre Nabat, Marc Mallet, and Samuel Somot
Atmos. Chem. Phys., 19, 3707–3731, https://doi.org/10.5194/acp-19-3707-2019, https://doi.org/10.5194/acp-19-3707-2019, 2019
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Among the different aerosols affecting the Euro-Mediterranean region, ammonium and nitrate (A&N) aerosols are expected to have a growing impact on regional climate. In this study, these aerosols have been introduced in the prognostic aerosol scheme of the ALADIN-Climate regional model. Results show that since 2005 over Europe, A&N aerosol optical depth is higher than sulfate and organics and they are responsible for a cooling of about −0.2 °C over Europe during summer.
Federica Pacifico, Claire Delon, Corinne Jambert, Pierre Durand, Eleanor Morris, Mat J. Evans, Fabienne Lohou, Solène Derrien, Venance H. E. Donnou, Arnaud V. Houeto, Irene Reinares Martínez, and Pierre-Etienne Brilouet
Atmos. Chem. Phys., 19, 2299–2325, https://doi.org/10.5194/acp-19-2299-2019, https://doi.org/10.5194/acp-19-2299-2019, 2019
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Biogenic fluxes from soil at a local and regional scale are crucial to study air pollution and climate. Here we present field measurements of soil fluxes of nitric oxide (NO) and ammonia (NH3) observed over four different land cover types, i.e. bare soil, grassland, maize field, and forest, at an inland rural site in Benin, West Africa, during the DACCIWA field campaign in
June and July 2016.
Camille Richon, Jean-Claude Dutay, Laurent Bopp, Briac Le Vu, James C. Orr, Samuel Somot, and François Dulac
Biogeosciences, 16, 135–165, https://doi.org/10.5194/bg-16-135-2019, https://doi.org/10.5194/bg-16-135-2019, 2019
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We evaluate the effects of climate change and biogeochemical forcing evolution on the nutrient and plankton cycles of the Mediterranean Sea for the first time. We use a high-resolution coupled physical and biogeochemical model and perform 120-year transient simulations. The results indicate that changes in external nutrient fluxes and climate change may have synergistic or antagonistic effects on nutrient concentrations, depending on the region and the scenario.
María José Granados-Muñoz, Michael Sicard, Roberto Román, Jose Antonio Benavent-Oltra, Rubén Barragán, Gerard Brogniez, Cyrielle Denjean, Marc Mallet, Paola Formenti, Benjamín Torres, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 19, 523–542, https://doi.org/10.5194/acp-19-523-2019, https://doi.org/10.5194/acp-19-523-2019, 2019
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The influence of mineral dust in the direct radiative effect is affected by a large uncertainty. This study investigates mineral dust radiative properties during an episode affecting southern Spain in June 2013 by using remote sensors and data collected on board an aircraft to feed a radiative transfer model. The study reveals the complexity of parameterizing these models, as characterizing mineral dust is still quite challenging, and the need for accurate mineral dust measurements.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Joel Brito, Cyrielle Denjean, Volker Dreiling, Andreas Fink, Corinne Jambert, Norbert Kalthoff, Peter Knippertz, Russ Ladkin, Sylvain Mailler, Marlon Maranan, Federica Pacifico, Bruno Piguet, Guillaume Siour, and Solène Turquety
Atmos. Chem. Phys., 19, 473–497, https://doi.org/10.5194/acp-19-473-2019, https://doi.org/10.5194/acp-19-473-2019, 2019
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This article presents a detailed analysis of anthropogenic and biomass burning pollutants over the Gulf of Guinea coastal region, using observations from the DACCIWA field campaign and modeling. The novelty is that we focus on how these two pollution sources are mixed and transported further inland. We show that during the day pollutants are accumulated along the coastline and transported northward as soon as the daytime convection in the atmospheric boundary layer ceases (16:00 UTC).
Mounir Chrit, Karine Sartelet, Jean Sciare, Marwa Majdi, José Nicolas, Jean-Eudes Petit, and François Dulac
Atmos. Chem. Phys., 18, 18079–18100, https://doi.org/10.5194/acp-18-18079-2018, https://doi.org/10.5194/acp-18-18079-2018, 2018
Paola Formenti, Lydie Mbemba Kabuiku, Isabelle Chiapello, Fabrice Ducos, François Dulac, and Didier Tanré
Atmos. Meas. Tech., 11, 6761–6784, https://doi.org/10.5194/amt-11-6761-2018, https://doi.org/10.5194/amt-11-6761-2018, 2018
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Aerosol particles from natural and anthropogenic sources are climate regulators as they can counteract or amplify the warming effect of greenhouse gases, but are difficult to observe due to their temporal and spatial variability. Satellite sensors can provide the needed global coverage but need validation. In this paper we explore the capability of the POLDER-3 advanced space-borne sensor to observe aerosols over the western Mediterranean region.
Karine Desboeufs, Elisabeth Bon Nguyen, Servanne Chevaillier, Sylvain Triquet, and François Dulac
Atmos. Chem. Phys., 18, 14477–14492, https://doi.org/10.5194/acp-18-14477-2018, https://doi.org/10.5194/acp-18-14477-2018, 2018
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Atmospheric deposition is known to be a major source of nutrients for the marine biosphere in the Mediterranean Sea. The study of the origin of nutrients and trace metals in Corsica presented here shows that the dust events were the major sources of Si and Fe. Conversely, combustion sources predominated the inputs of N, P, and trace metals. This work showed the importance of considering background anthropogenic deposition for estimating the impact of atmospheric forcing on marine biota.
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Mounir Chrit, Karine Sartelet, Jean Sciare, Jorge Pey, José B. Nicolas, Nicolas Marchand, Evelyn Freney, Karine Sellegri, Matthias Beekmann, and François Dulac
Atmos. Chem. Phys., 18, 9631–9659, https://doi.org/10.5194/acp-18-9631-2018, https://doi.org/10.5194/acp-18-9631-2018, 2018
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Fine particulate matter (PM) in the atmosphere is of concern due to its effects on health, climate, ecosystems and biological cycles, and visibility.
These effects are especially important in the Mediterranean region. In this study, the air quality model Polyphemus is used to understand the
sources of inorganic and organic particles in the western Mediterranean and evaluate the uncertainties linked to the model parameters and hypotheses related to condensation/evaporation in the model.
Nizar Jaidan, Laaziz El Amraoui, Jean-Luc Attié, Philippe Ricaud, and François Dulac
Atmos. Chem. Phys., 18, 9351–9373, https://doi.org/10.5194/acp-18-9351-2018, https://doi.org/10.5194/acp-18-9351-2018, 2018
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The Mediterranean Basin, surrounded by three continents with diverse pollution sources, is particularly sensitive to climate change due to its location and diversity of ecosystems. In this work, we investigate the future change of surface ozone from 2000 to 2100 over this region using a set of atmospheric model outputs and ground-based observations. We also highlight how the future climate change and the increase of methane concentrations can offset the benefit of the pollution reduction policy.
Quentin Bourgeois, Annica M. L. Ekman, Jean-Baptiste Renard, Radovan Krejci, Abhay Devasthale, Frida A.-M. Bender, Ilona Riipinen, Gwenaël Berthet, and Jason L. Tackett
Atmos. Chem. Phys., 18, 7709–7720, https://doi.org/10.5194/acp-18-7709-2018, https://doi.org/10.5194/acp-18-7709-2018, 2018
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The altitude of aerosols is crucial as they can impact cloud formation and radiation. In this study, satellite observations have been used to characterize the global aerosol optical depth (AOD) in the boundary layer and the free troposphere. The free troposphere contributes 39 % to the global AOD during daytime. Overall, the results have implications for the description of budgets, sources, sinks and transport of aerosol particles as presently described in the atmospheric model.
Arineh Cholakian, Matthias Beekmann, Augustin Colette, Isabelle Coll, Guillaume Siour, Jean Sciare, Nicolas Marchand, Florian Couvidat, Jorge Pey, Valerie Gros, Stéphane Sauvage, Vincent Michoud, Karine Sellegri, Aurélie Colomb, Karine Sartelet, Helen Langley DeWitt, Miriam Elser, André S. H. Prévot, Sonke Szidat, and François Dulac
Atmos. Chem. Phys., 18, 7287–7312, https://doi.org/10.5194/acp-18-7287-2018, https://doi.org/10.5194/acp-18-7287-2018, 2018
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In this work, four schemes for the simulation of organic aerosols in the western Mediterranean basin are added to the CHIMERE chemistry–transport model; the resulting simulations are then compared to measurements obtained from ChArMEx. It is concluded that the scheme taking into account the fragmentation and the formation of nonvolatile organic aerosols corresponds better to measurements; the major source of this aerosol in the western Mediterranean is found to be of biogenic origin.
Evelyn Freney, Karine Sellegri, Mounir Chrit, Kouji Adachi, Joel Brito, Antoine Waked, Agnès Borbon, Aurélie Colomb, Régis Dupuy, Jean-Marc Pichon, Laetitia Bouvier, Claire Delon, Corinne Jambert, Pierre Durand, Thierry Bourianne, Cécile Gaimoz, Sylvain Triquet, Anaïs Féron, Matthias Beekmann, François Dulac, and Karine Sartelet
Atmos. Chem. Phys., 18, 7041–7056, https://doi.org/10.5194/acp-18-7041-2018, https://doi.org/10.5194/acp-18-7041-2018, 2018
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The focus of these experiments, within the ChArMEx project, were to better understand the chemical properties of ambient aerosols over the Mediterranean region. A series of airborne measurements were performed aboard the French research aircraft, the ATR42, during the summer period. Aerosol and gas-phase chemical mass spectrometry allowed us to understand the sources and formation of organic aerosols. Numerical models were incorporated into this study to help interpret our observations.
Vanessa Brocchi, Gisèle Krysztofiak, Valéry Catoire, Jonathan Guth, Virginie Marécal, Régina Zbinden, Laaziz El Amraoui, François Dulac, and Philippe Ricaud
Atmos. Chem. Phys., 18, 6887–6906, https://doi.org/10.5194/acp-18-6887-2018, https://doi.org/10.5194/acp-18-6887-2018, 2018
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The Mediterranean Basin still suffers from a limited amount of in situ measurements for a good characterization of its environmental state. This study shows that intercontinental transport of very high CO concentrations can affect the upper Mediterranean Basin troposphere. By using modeling, 5- to 12-day eastward transport of biomass burning starting from North America and Siberia impacts the mid-troposphere of the Mediterranean Basin.
Camille Richon, Jean-Claude Dutay, François Dulac, Rong Wang, and Yves Balkanski
Biogeosciences, 15, 2499–2524, https://doi.org/10.5194/bg-15-2499-2018, https://doi.org/10.5194/bg-15-2499-2018, 2018
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This work is part of the Mermex and ChArMEx projects of the MISTRALS program. It aims at studying the impacts of phosphorus deposition from contrasted sources on the biogeochemical cycles of the Mediterranean Sea.
The results show that combustion-related phosphorus deposition effects dominate P deposition over the northern Mediterranean, whereas dust-derived phosphorus deposition effects dominate in the southern part.
Daniela Meloni, Alcide di Sarra, Gérard Brogniez, Cyrielle Denjean, Lorenzo De Silvestri, Tatiana Di Iorio, Paola Formenti, José L. Gómez-Amo, Julian Gröbner, Natalia Kouremeti, Giuliano Liuzzi, Marc Mallet, Giandomenico Pace, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 18, 4377–4401, https://doi.org/10.5194/acp-18-4377-2018, https://doi.org/10.5194/acp-18-4377-2018, 2018
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This study examines how different aerosol optical properties determine the dust longwave radiative effects at the surface, in the atmosphere and at the top of the atmosphere, based on the combination of remote sensing and in situ observations from the ground, from airborne sensors, and from space, by means of radiative transfer modelling. The closure experiment is based on longwave irradiances and spectral brightness temperatures measured during the 2013 ChArMEx–ADRIMED campaign at Lampedusa.
Thibaut Lurton, Fabrice Jégou, Gwenaël Berthet, Jean-Baptiste Renard, Lieven Clarisse, Anja Schmidt, Colette Brogniez, and Tjarda J. Roberts
Atmos. Chem. Phys., 18, 3223–3247, https://doi.org/10.5194/acp-18-3223-2018, https://doi.org/10.5194/acp-18-3223-2018, 2018
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We quantify the chemical and microphysical effects of volcanic SO2 and HCl from the June 2009 Sarychev Peak eruption using a comprehensive aerosol–chemistry model combined with in situ measurements and satellite retrievals. Our results suggest that previous studies underestimated the eruption's atmospheric and climatic impact, mainly because previous model-to-satellite comparisons had to make assumptions about the aerosol size distribution and were based on biased satellite retrievals of AOD.
Nelson Bègue, Damien Vignelles, Gwenaël Berthet, Thierry Portafaix, Guillaume Payen, Fabrice Jégou, Hassan Benchérif, Julien Jumelet, Jean-Paul Vernier, Thibaut Lurton, Jean-Baptiste Renard, Lieven Clarisse, Vincent Duverger, Françoise Posny, Jean-Marc Metzger, and Sophie Godin-Beekmann
Atmos. Chem. Phys., 17, 15019–15036, https://doi.org/10.5194/acp-17-15019-2017, https://doi.org/10.5194/acp-17-15019-2017, 2017
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The space–time evolutions of the Calbuco plume are investigated by combining satellite, in situ aerosol counting and lidar observations, and a numerical model. All the data at Reunion Island reveal a twofold increase in the amount of aerosol with respect to the values observed before the eruption. The dynamic context has favored the spread of the plume exclusively in the Southern Hemisphere. This study highlights the role played by dynamical barriers in the transport of atmospheric species.
Jose A. Benavent-Oltra, Roberto Román, María J. Granados-Muñoz, Daniel Pérez-Ramírez, Pablo Ortiz-Amezcua, Cyrielle Denjean, Anton Lopatin, Hassan Lyamani, Benjamin Torres, Juan L. Guerrero-Rascado, David Fuertes, Oleg Dubovik, Anatoli Chaikovsky, Francisco J. Olmo, Marc Mallet, and Lucas Alados-Arboledas
Atmos. Meas. Tech., 10, 4439–4457, https://doi.org/10.5194/amt-10-4439-2017, https://doi.org/10.5194/amt-10-4439-2017, 2017
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In this study, vertical profiles and column integrated aerosol properties retrieved by GRASP (Generalized Retrieval of Atmosphere and Surface Properties) algorithm are evaluated with in situ airborne measurements made during the ChArMEx-ADRIMED field campaign in summer 2013. Differences between GRASP retrievals and airborne extinction profiles are in the range of 15 to 30 %. Also, the total volume concentration differences between in situ data and GRASP retrieval ranges from 15 to 36 %.
Yinghe Fu, Karine Desboeufs, Julie Vincent, Elisabeth Bon Nguyen, Benoit Laurent, Remi Losno, and François Dulac
Atmos. Meas. Tech., 10, 4389–4401, https://doi.org/10.5194/amt-10-4389-2017, https://doi.org/10.5194/amt-10-4389-2017, 2017
Uri Dayan, Philippe Ricaud, Régina Zbinden, and François Dulac
Atmos. Chem. Phys., 17, 13233–13263, https://doi.org/10.5194/acp-17-13233-2017, https://doi.org/10.5194/acp-17-13233-2017, 2017
Marine Claeys, Greg Roberts, Marc Mallet, Jovanna Arndt, Karine Sellegri, Jean Sciare, John Wenger, and Bastien Sauvage
Atmos. Chem. Phys., 17, 7891–7915, https://doi.org/10.5194/acp-17-7891-2017, https://doi.org/10.5194/acp-17-7891-2017, 2017
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Over a period of 5 days (summer 2013), the mass concentration of primary marine aerosols was dominant compared to other aerosols measured at a ground-based measuring site on Corsica. The characteristics of primary marine aerosols such as their size distribution, their optical properties and their direct radiative effect were studied as a function of their ageing and region of emission. These characteristics were compared to two other periods dominated by different aerosol regimes.
Jovanna Arndt, Jean Sciare, Marc Mallet, Greg C. Roberts, Nicolas Marchand, Karine Sartelet, Karine Sellegri, François Dulac, Robert M. Healy, and John C. Wenger
Atmos. Chem. Phys., 17, 6975–7001, https://doi.org/10.5194/acp-17-6975-2017, https://doi.org/10.5194/acp-17-6975-2017, 2017
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The chemical composition of individual PM2.5 particles was measured at a background site on Corsica in the Mediterranean to determine the contribution of different sources to background aerosol in the region. Most of the particles were from fossil fuel combustion and biomass burning, transported to the site from France, Italy and eastern Europe, and also accumulated other species en route. This work shows that largest impact on air quality in the Mediterranean is from anthropogenic emissions.
Juan Antonio Bravo-Aranda, Gregori de Arruda Moreira, Francisco Navas-Guzmán, María José Granados-Muñoz, Juan Luis Guerrero-Rascado, David Pozo-Vázquez, Clara Arbizu-Barrena, Francisco José Olmo Reyes, Marc Mallet, and Lucas Alados Arboledas
Atmos. Chem. Phys., 17, 6839–6851, https://doi.org/10.5194/acp-17-6839-2017, https://doi.org/10.5194/acp-17-6839-2017, 2017
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The automatic detection of the planetary boundary layer height (PBL height) by means of lidar measurements still presents difficulties. This work shows an improvement in the PBL height detection using lidar depolarization measurements. To our knowledge, it is the first time that the lidar depolarization technique is used for this purpose. Also, the PBL height derived from the WRF model is compared with the PBL heights of this new method and from a microwave radiometer during CHARMEX campaigns.
Pierre Tulet, Andréa Di Muro, Aurélie Colomb, Cyrielle Denjean, Valentin Duflot, Santiago Arellano, Brice Foucart, Jérome Brioude, Karine Sellegri, Aline Peltier, Alessandro Aiuppa, Christelle Barthe, Chatrapatty Bhugwant, Soline Bielli, Patrice Boissier, Guillaume Boudoire, Thierry Bourrianne, Christophe Brunet, Fréderic Burnet, Jean-Pierre Cammas, Franck Gabarrot, Bo Galle, Gaetano Giudice, Christian Guadagno, Fréderic Jeamblu, Philippe Kowalski, Jimmy Leclair de Bellevue, Nicolas Marquestaut, Dominique Mékies, Jean-Marc Metzger, Joris Pianezze, Thierry Portafaix, Jean Sciare, Arnaud Tournigand, and Nicolas Villeneuve
Atmos. Chem. Phys., 17, 5355–5378, https://doi.org/10.5194/acp-17-5355-2017, https://doi.org/10.5194/acp-17-5355-2017, 2017
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The STRAP campaign was conducted in 2015 to investigate the volcanic plumes of Piton de La Fournaise (La Réunion, France). For the first time, measurements were conducted at the local (near the vent) and regional scales around the island. The STRAP 2015 campaign gave a unique set of multi-disciplinary data that can now be used by modellers to improve the numerical parameterisations of the physical and chemical evolution of the volcanic plumes.
Gwenaël Berthet, Fabrice Jégou, Valéry Catoire, Gisèle Krysztofiak, Jean-Baptiste Renard, Adam E. Bourassa, Doug A. Degenstein, Colette Brogniez, Marcel Dorf, Sebastian Kreycy, Klaus Pfeilsticker, Bodo Werner, Franck Lefèvre, Tjarda J. Roberts, Thibaut Lurton, Damien Vignelles, Nelson Bègue, Quentin Bourgeois, Daniel Daugeron, Michel Chartier, Claude Robert, Bertrand Gaubicher, and Christophe Guimbaud
Atmos. Chem. Phys., 17, 2229–2253, https://doi.org/10.5194/acp-17-2229-2017, https://doi.org/10.5194/acp-17-2229-2017, 2017
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Since the last major volcanic event, i.e. the Pinatubo eruption in 1991, only
moderateeruptions have regularly injected sulfur into the stratosphere, typically enhancing the aerosol loading for several months. We investigate here for the first time the chemical perturbation associated with the Sarychev eruption in June 2009, using balloon-borne instruments and model calculations. Some chemical compounds are significantly affected by the aerosols, but the impact on stratospheric ozone is weak.
François Gheusi, Pierre Durand, Nicolas Verdier, François Dulac, Jean-Luc Attié, Philippe Commun, Brice Barret, Claude Basdevant, Antoine Clenet, Solène Derrien, Alexis Doerenbecher, Laaziz El Amraoui, Alain Fontaine, Emeric Hache, Corinne Jambert, Elodie Jaumouillé, Yves Meyerfeld, Laurent Roblou, and Flore Tocquer
Atmos. Meas. Tech., 9, 5811–5832, https://doi.org/10.5194/amt-9-5811-2016, https://doi.org/10.5194/amt-9-5811-2016, 2016
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Boundary-layer pressurised balloons allow for horizontal multi-day flights in the lower atmosphere, carrying light scientific payloads. Ozonesondes, usually used for balloon soundings have too short a lifetime for such flights. An adaptation is proposed, whereby conventional sondes are operated with short measurement phases alternating with longer periods of dormancy. The sondes were operated over the western Mediterranean, offering an original perspective on tropospheric ozone.
Michaël Sicard, Rubén Barragan, François Dulac, Lucas Alados-Arboledas, and Marc Mallet
Atmos. Chem. Phys., 16, 12177–12203, https://doi.org/10.5194/acp-16-12177-2016, https://doi.org/10.5194/acp-16-12177-2016, 2016
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The seasonal variability of the aerosol optical, microphysical and radiative properties at three insular sites in the western Mediterranean Basin is presented. The main drivers of the observed annual cycles and NE–SW gradients are mineral dust outbreaks in summer and European continental aerosols in spring. The lack of NE–W gradients of some aerosol properties is attributed to a homogeneous spatial distribution of the fine particle load and absorption low values in the southwesternmost site.
Jean-Baptiste Renard, François Dulac, Gwenaël Berthet, Thibaut Lurton, Damien Vignelles, Fabrice Jégou, Thierry Tonnelier, Matthieu Jeannot, Benoit Couté, Rony Akiki, Nicolas Verdier, Marc Mallet, François Gensdarmes, Patrick Charpentier, Samuel Mesmin, Vincent Duverger, Jean-Charles Dupont, Thierry Elias, Vincent Crenn, Jean Sciare, Paul Zieger, Matthew Salter, Tjarda Roberts, Jérôme Giacomoni, Matthieu Gobbi, Eric Hamonou, Haraldur Olafsson, Pavla Dagsson-Waldhauserova, Claude Camy-Peyret, Christophe Mazel, Thierry Décamps, Martin Piringer, Jérémy Surcin, and Daniel Daugeron
Atmos. Meas. Tech., 9, 3673–3686, https://doi.org/10.5194/amt-9-3673-2016, https://doi.org/10.5194/amt-9-3673-2016, 2016
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We illustrate the first Light Optical Aerosol Counter (LOAC) airborne results obtained from an unmanned aerial vehicle (UAV) and a variety of scientific balloons: tethered balloons deployed in urban environments, pressurized balloons drifting in the lower troposphere over the western Mediterranean during the Chemistry-Aerosol Mediterranean Experiment (ChArMEx), and meteorological sounding balloons launched in the western Mediterranean region and in the south-west of France.
Julie Vincent, Benoit Laurent, Rémi Losno, Elisabeth Bon Nguyen, Pierre Roullet, Stéphane Sauvage, Servanne Chevaillier, Patrice Coddeville, Noura Ouboulmane, Alcide Giorgio di Sarra, Antonio Tovar-Sánchez, Damiano Sferlazzo, Ana Massanet, Sylvain Triquet, Rafael Morales Baquero, Michel Fornier, Cyril Coursier, Karine Desboeufs, François Dulac, and Gilles Bergametti
Atmos. Chem. Phys., 16, 8749–8766, https://doi.org/10.5194/acp-16-8749-2016, https://doi.org/10.5194/acp-16-8749-2016, 2016
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To investigate dust deposition dynamics at the regional scale, five automatic deposition collectors named CARAGA have been deployed in the western Mediterranean basin (Lampedusa, Majorca, Corsica, Frioul and Le Casset) during 1 to 3 years depending on the station. Complementary observations provided by both satellite and air mass trajectories are used to identify the dust provenance areas and the transport pathways from the Sahara to the stations for the studied period.
Fabrice Chane Ming, Damien Vignelles, Fabrice Jegou, Gwenael Berthet, Jean-Baptiste Renard, François Gheusi, and Yuriy Kuleshov
Atmos. Chem. Phys., 16, 8023–8042, https://doi.org/10.5194/acp-16-8023-2016, https://doi.org/10.5194/acp-16-8023-2016, 2016
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Coupled balloon-borne observations of Light Optical Aerosol Counter (LOAC), M10 meteorological GPS sondes, ozonesondes, and GPS radio occultation data are examined to identify gravity-wave (GW)-induced fluctuations on tracer gases and on the vertical distribution of stratospheric aerosol concentrations during the 2013 ChArMEx campaign. Observed mesoscale GWs induce a strong modulation of the amplitude of tracer gases and the stratospheric aerosol background.
María José Granados-Muñoz, Francisco Navas-Guzmán, Juan Luis Guerrero-Rascado, Juan Antonio Bravo-Aranda, Ioannis Binietoglou, Sergio Nepomuceno Pereira, Sara Basart, José María Baldasano, Livio Belegante, Anatoli Chaikovsky, Adolfo Comerón, Giuseppe D'Amico, Oleg Dubovik, Luka Ilic, Panos Kokkalis, Constantino Muñoz-Porcar, Slobodan Nickovic, Doina Nicolae, Francisco José Olmo, Alexander Papayannis, Gelsomina Pappalardo, Alejandro Rodríguez, Kerstin Schepanski, Michaël Sicard, Ana Vukovic, Ulla Wandinger, François Dulac, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 16, 7043–7066, https://doi.org/10.5194/acp-16-7043-2016, https://doi.org/10.5194/acp-16-7043-2016, 2016
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This study provides a detailed overview of the Mediterranean region regarding aerosol microphysical properties during the ChArMEx/EMEP campaign in July 2012. An in-depth analysis of the horizontal, vertical, and temporal dimensions is performed using LIRIC, proving the algorithm's ability in automated retrieval of microphysical property profiles within a network. A validation of four dust models is included, obtaining fair good agreement, especially for the vertical distribution of the aerosol.
Stefanie Augustin-Bauditz, Heike Wex, Cyrielle Denjean, Susan Hartmann, Johannes Schneider, Susann Schmidt, Martin Ebert, and Frank Stratmann
Atmos. Chem. Phys., 16, 5531–5543, https://doi.org/10.5194/acp-16-5531-2016, https://doi.org/10.5194/acp-16-5531-2016, 2016
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In this study, we mixed a pure mineral dust sample with ice active biological material and quantified the immersion freezing behavior of the resulting particles utilizing the Leipzig Aerosol Cloud Interaction Simulator (LACIS). Furthermore, we used different methods to investigate the mixing state of our generated aerosol.
We found that internally mixed particles, containing ice active biological material, follow the ice nucleation behavior observed for the pure biological particles.
Jean-Baptiste Renard, François Dulac, Gwenaël Berthet, Thibaut Lurton, Damien Vignelles, Fabrice Jégou, Thierry Tonnelier, Matthieu Jeannot, Benoit Couté, Rony Akiki, Nicolas Verdier, Marc Mallet, François Gensdarmes, Patrick Charpentier, Samuel Mesmin, Vincent Duverger, Jean-Charles Dupont, Thierry Elias, Vincent Crenn, Jean Sciare, Paul Zieger, Matthew Salter, Tjarda Roberts, Jérôme Giacomoni, Matthieu Gobbi, Eric Hamonou, Haraldur Olafsson, Pavla Dagsson-Waldhauserova, Claude Camy-Peyret, Christophe Mazel, Thierry Décamps, Martin Piringer, Jérémy Surcin, and Daniel Daugeron
Atmos. Meas. Tech., 9, 1721–1742, https://doi.org/10.5194/amt-9-1721-2016, https://doi.org/10.5194/amt-9-1721-2016, 2016
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LOAC is a light aerosols counter for performing measurements at the surface and under all kinds of atmospheric balloons. LOAC performs observations at two scattering angles. The first one at 12° is insensitive to the refractive index of the particles; the second one at 60° is strongly sensitive to the refractive index. By combining the measurements, it is possible to retrieve the size distribution between 0.2 and 100 micrometeres and to estimate the nature of the dominant particles.
Gerard Ancellet, Jacques Pelon, Julien Totems, Patrick Chazette, Ariane Bazureau, Michaël Sicard, Tatiana Di Iorio, Francois Dulac, and Marc Mallet
Atmos. Chem. Phys., 16, 4725–4742, https://doi.org/10.5194/acp-16-4725-2016, https://doi.org/10.5194/acp-16-4725-2016, 2016
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A multi-lidar analysis conducted in the Mediterranean basin compares the impact of the long-range transport of North American biomass burning aerosols with the role of frequently observed Saharan dust outbreaks. This paper provides a detailed analysis of the potential North American aerosol sources, their transport to Europe and the mixing of different aerosol sources, using simulations of a particle dispersion model and lidar measurements of the aerosol optical properties.
C. Denjean, F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, G. Momboisse, K. Sellegri, A. Schwarzenbock, E. Freney, M. Mallet, and P. Formenti
Atmos. Chem. Phys., 16, 1081–1104, https://doi.org/10.5194/acp-16-1081-2016, https://doi.org/10.5194/acp-16-1081-2016, 2016
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This study investigates the size distribution, chemical composition, and optical properties of Saharan mineral dust transported over the western Mediterranean using in situ measurements collected from aircraft. Their variability due to altitude, time of transport, and mixing rate with pollution particles are discussed. We found moderate light absorption of the dust plumes even in the presence of pollution particles and the persistence of large dust particles after transport in the Mediterranean.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
C. Darbieu, F. Lohou, M. Lothon, J. Vilà-Guerau de Arellano, F. Couvreux, P. Durand, D. Pino, E. G. Patton, E. Nilsson, E. Blay-Carreras, and B. Gioli
Atmos. Chem. Phys., 15, 10071–10086, https://doi.org/10.5194/acp-15-10071-2015, https://doi.org/10.5194/acp-15-10071-2015, 2015
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A case study of the BLLAST experiment is considered to explore the decay of turbulence that occurs in the convective boundary layer over land during the afternoon. Based on observations and on a large-eddy simulation, the analysis reveals two phases in the afternoon: a first quasi-stationary phase when the turbulent kinetic energy slowly decays without significant change in the turbulence structure and a second phase of more rapid decay with a change in spectral turbulence characteristics.
H. P. Pietersen, J. Vilà-Guerau de Arellano, P. Augustin, A. van de Boer, O. de Coster, H. Delbarre, P. Durand, M. Fourmentin, B. Gioli, O. Hartogensis, F. Lohou, M. Lothon, H. G. Ouwersloot, D. Pino, and J. Reuder
Atmos. Chem. Phys., 15, 4241–4257, https://doi.org/10.5194/acp-15-4241-2015, https://doi.org/10.5194/acp-15-4241-2015, 2015
J.-F. Léon, P. Augustin, M. Mallet, T. Bourrianne, V. Pont, F. Dulac, M. Fourmentin, D. Lambert, and B. Sauvage
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-9507-2015, https://doi.org/10.5194/acpd-15-9507-2015, 2015
Preprint withdrawn
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This paper presents the aerosol vertical distribution observed by lidar soundings in Corsica (western Mediterranean) between February 2012 and August 2013. A seasonal cycle is observed in the extinction coefficient profiles and aerosol optical thickness with minima in winter and maxima in spring-summer. Less than 10% of the daily observations show high AOD corresponding to the large-scale advection of desert dust from Northern Africa or pollution aerosols from Europe.
J.-B. Renard, F. Dulac, G. Berthet, T. Lurton, D. Vignelles, F. Jégou, T. Tonnelier, C. Thaury, M. Jeannot, B. Couté, R. Akiki, J.-L. Mineau, N. Verdier, M. Mallet, F. Gensdarmes, P. Charpentier, S. Mesmin, V. Duverger, J.-C. Dupont, T. Elias, V. Crenn, J. Sciare, J. Giacomoni, M. Gobbi, E. Hamonou, H. Olafsson, P. Dagsson-Waldhauserova, C. Camy-Peyret, C. Mazel, T. Décamps, M. Piringer, J. Surcin, and D. Daugeron
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-8-1203-2015, https://doi.org/10.5194/amtd-8-1203-2015, 2015
Revised manuscript not accepted
J.-B. Renard, F. Dulac, G. Berthet, T. Lurton, D. Vignelle, F. Jégou, T. Tonnelier, C. Thaury, M. Jeannot, B. Couté, R. Akiki, J.-L. Mineau, N. Verdier, M. Mallet, F. Gensdarmes, P. Charpentier, S. Mesmin, V. Duverger, J.-C. Dupont, T. Elias, V. Crenn, J. Sciare, J. Giacomoni, M. Gobbi, E. Hamonou, H. Olafsson, P. Dagsson-Waldhauserova, C. Camy-Peyret, C. Mazel, T. Décamps, M. Piringer, J. Surcin, and D. Daugeron
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-8-1261-2015, https://doi.org/10.5194/amtd-8-1261-2015, 2015
Revised manuscript not accepted
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We present exemples of measurements obtained by the new light optical aerosol counter LOAC. The measurement were conducted from different kinds of balloons in the troposphre and stratosphere.
C. Denjean, P. Formenti, B. Picquet-Varrault, M. Camredon, E. Pangui, P. Zapf, Y. Katrib, C. Giorio, A. Tapparo, B. Temime-Roussel, A. Monod, B. Aumont, and J. F. Doussin
Atmos. Chem. Phys., 15, 883–897, https://doi.org/10.5194/acp-15-883-2015, https://doi.org/10.5194/acp-15-883-2015, 2015
Y. Wang, K. N. Sartelet, M. Bocquet, P. Chazette, M. Sicard, G. D'Amico, J. F. Léon, L. Alados-Arboledas, A. Amodeo, P. Augustin, J. Bach, L. Belegante, I. Binietoglou, X. Bush, A. Comerón, H. Delbarre, D. García-Vízcaino, J. L. Guerrero-Rascado, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, F. Molero, N. Montoux, A. Muñoz, C. Muñoz, D. Nicolae, A. Papayannis, G. Pappalardo, J. Preissler, V. Rizi, F. Rocadenbosch, K. Sellegri, F. Wagner, and F. Dulac
Atmos. Chem. Phys., 14, 12031–12053, https://doi.org/10.5194/acp-14-12031-2014, https://doi.org/10.5194/acp-14-12031-2014, 2014
M. Lothon, F. Lohou, D. Pino, F. Couvreux, E. R. Pardyjak, J. Reuder, J. Vilà-Guerau de Arellano, P Durand, O. Hartogensis, D. Legain, P. Augustin, B. Gioli, D. H. Lenschow, I. Faloona, C. Yagüe, D. C. Alexander, W. M. Angevine, E Bargain, J. Barrié, E. Bazile, Y. Bezombes, E. Blay-Carreras, A. van de Boer, J. L. Boichard, A. Bourdon, A. Butet, B. Campistron, O. de Coster, J. Cuxart, A. Dabas, C. Darbieu, K. Deboudt, H. Delbarre, S. Derrien, P. Flament, M. Fourmentin, A. Garai, F. Gibert, A. Graf, J. Groebner, F. Guichard, M. A. Jiménez, M. Jonassen, A. van den Kroonenberg, V. Magliulo, S. Martin, D. Martinez, L. Mastrorillo, A. F. Moene, F. Molinos, E. Moulin, H. P. Pietersen, B. Piguet, E. Pique, C. Román-Cascón, C. Rufin-Soler, F. Saïd, M. Sastre-Marugán, Y. Seity, G. J. Steeneveld, P. Toscano, O. Traullé, D. Tzanos, S. Wacker, N. Wildmann, and A. Zaldei
Atmos. Chem. Phys., 14, 10931–10960, https://doi.org/10.5194/acp-14-10931-2014, https://doi.org/10.5194/acp-14-10931-2014, 2014
C. Guieu, C. Ridame, E. Pulido-Villena, M. Bressac, K. Desboeufs, and F. Dulac
Biogeosciences, 11, 5621–5635, https://doi.org/10.5194/bg-11-5621-2014, https://doi.org/10.5194/bg-11-5621-2014, 2014
C. Aghnatios, R. Losno, and F. Dulac
Biogeosciences, 11, 4627–4633, https://doi.org/10.5194/bg-11-4627-2014, https://doi.org/10.5194/bg-11-4627-2014, 2014
T. Lurton, J.-B. Renard, D. Vignelles, M. Jeannot, R. Akiki, J.-L. Mineau, and T. Tonnelier
Atmos. Meas. Tech., 7, 931–939, https://doi.org/10.5194/amt-7-931-2014, https://doi.org/10.5194/amt-7-931-2014, 2014
C. Guieu, F. Dulac, C. Ridame, and P. Pondaven
Biogeosciences, 11, 425–442, https://doi.org/10.5194/bg-11-425-2014, https://doi.org/10.5194/bg-11-425-2014, 2014
M. Mallet, O. Dubovik, P. Nabat, F. Dulac, R. Kahn, J. Sciare, D. Paronis, and J. F. Léon
Atmos. Chem. Phys., 13, 9195–9210, https://doi.org/10.5194/acp-13-9195-2013, https://doi.org/10.5194/acp-13-9195-2013, 2013
D. Legain, O. Bousquet, T. Douffet, D. Tzanos, E. Moulin, J. Barrie, and J.-B. Renard
Atmos. Meas. Tech., 6, 2195–2205, https://doi.org/10.5194/amt-6-2195-2013, https://doi.org/10.5194/amt-6-2195-2013, 2013
F. Jégou, G. Berthet, C. Brogniez, J.-B. Renard, P. François, J. M. Haywood, A. Jones, Q. Bourgeois, T. Lurton, F. Auriol, S. Godin-Beekmann, C. Guimbaud, G. Krysztofiak, B. Gaubicher, M. Chartier, L. Clarisse, C. Clerbaux, J. Y. Balois, C. Verwaerde, and D. Daugeron
Atmos. Chem. Phys., 13, 6533–6552, https://doi.org/10.5194/acp-13-6533-2013, https://doi.org/10.5194/acp-13-6533-2013, 2013
G. Wetzel, H. Oelhaf, G. Berthet, A. Bracher, C. Cornacchia, D. G. Feist, H. Fischer, A. Fix, M. Iarlori, A. Kleinert, A. Lengel, M. Milz, L. Mona, S. C. Müller, J. Ovarlez, G. Pappalardo, C. Piccolo, P. Raspollini, J.-B. Renard, V. Rizi, S. Rohs, C. Schiller, G. Stiller, M. Weber, and G. Zhang
Atmos. Chem. Phys., 13, 5791–5811, https://doi.org/10.5194/acp-13-5791-2013, https://doi.org/10.5194/acp-13-5791-2013, 2013
P. Nabat, S. Somot, M. Mallet, I. Chiapello, J. J. Morcrette, F. Solmon, S. Szopa, F. Dulac, W. Collins, S. Ghan, L. W. Horowitz, J. F. Lamarque, Y. H. Lee, V. Naik, T. Nagashima, D. Shindell, and R. Skeie
Atmos. Meas. Tech., 6, 1287–1314, https://doi.org/10.5194/amt-6-1287-2013, https://doi.org/10.5194/amt-6-1287-2013, 2013
R. Baghi, P. Durand, C. Jambert, C. Jarnot, C. Delon, D. Serça, N. Striebig, M. Ferlicoq, and P. Keravec
Atmos. Meas. Tech., 5, 3119–3132, https://doi.org/10.5194/amt-5-3119-2012, https://doi.org/10.5194/amt-5-3119-2012, 2012
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions
Hygroscopic aerosols amplify longwave downward radiation in the Arctic
Measurement report: Optical and structural properties of atmospheric water-soluble organic carbon in China – insights from multi-site spectroscopic measurements
Measurement report: The variation properties of aerosol hygroscopic growth related to chemical composition during new particle formation days in a coastal city of Southeast China
In situ vertical observations of the layered structure of air pollution in a continental high-latitude urban boundary layer during winter
Size-resolved hygroscopicity and volatility properties of ambient urban aerosol particles measured by a volatility hygroscopicity tandem differential mobility analyzer system in Beijing
Terrestrial runoff is an important source of biological ice-nucleating particles in Arctic marine systems
Characterization of aerosol over the eastern Mediterranean by polarization-sensitive Raman lidar measurements during A-LIFE – aerosol type classification and type separation
Aerosol spectral optical properties in the Paris urban area and its peri-urban and forested surroundings during summer 2022 from ACROSS surface observations
Measurement report: An investigation of the spatiotemporal variability in aerosols in the mountainous terrain of the upper Colorado River basin using SAIL-Net
Contributions of the synoptic meteorology to the seasonal cloud condensation nuclei cycle over the Southern Ocean
Measurement report: Cloud condensation nuclei (CCN) activity in the South China Sea from shipborne observations during the summer and winter of 2021 – seasonal variation and anthropogenic influence
Measurement report: A comparative analysis of an intensive incursion of fluorescing African dust particles over Puerto Rico and another over Spain
Measurement report: Analysis of aerosol optical depth variation at Zhongshan Station in Antarctica
External particle mixing influences hygroscopicity in a sub-urban area
Long-term observations of black carbon and carbon monoxide in the Poker Flat Research Range, central Alaska, with a focus on forest wildfire emissions
High ice-nucleating particle concentrations associated with Arctic haze in springtime cold-air outbreaks
CCN estimations at a high-altitude remote site: role of organic aerosol variability and hygroscopicity
Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement
Spatial, temporal, and meteorological impact of the 26 February 2023 dust storm: increase in particulate matter concentrations across New Mexico and West Texas
Large spatiotemporal variability in aerosol properties over central Argentina during the CACTI field campaign
Quantification and characterization of primary biological aerosol particles and microbes aerosolized from Baltic seawater
Brownness of organics in anthropogenic biomass burning aerosols over South Asia
Measurement report: size-resolved particle effective density measured by the AAC-SMPS and implications for chemical composition
Source apportionment of particle number size distribution at the street canyon and urban background sites
Long-range transport of coarse mineral dust: an evaluation of the Met Office Unified Model against aircraft observations
Extreme Saharan dust events expand northward over the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 episodes
Atmospheric black carbon in the metropolitan area of La Paz and El Alto, Bolivia: concentration levels and emission sources
Changing optical properties of black carbon and brown carbon aerosols during long-range transport from the Indo-Gangetic Plain to the equatorial Indian Ocean
The evolution of aerosols mixing state derived from a field campaign in Beijing: implications to the particles aging time scale in urban atmosphere
Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic
Ice-nucleating particles active below −24 °C in a Finnish boreal forest and their relationship to bioaerosols
Measurement report: The influence of particle number size distribution and hygroscopicity on the microphysical properties of cloud droplets at a mountain site
Measurements of particle emissions of an A350-941 burning 100 % sustainable aviation fuels in cruise
Vertical distribution of ice nucleating particles over the boreal forest of Hyytiälä, Finland
Multi-year gradient measurements of sea spray fluxes over the Baltic Sea and the North Atlantic Ocean
Measurement report: In situ vertical profiles of below-cloud aerosol over the central Greenland Ice Sheet
Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US
Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe
Simulated contrail-processed aviation soot aerosols are poor ice-nucleating particles at cirrus temperatures
Biological and dust aerosols as sources of ice-nucleating particles in the eastern Mediterranean: source apportionment, atmospheric processing and parameterization
Quantifying the dust direct radiative effect in the southwestern United States: findings from multiyear measurements
How horizontal transport and turbulent mixing impact aerosol particle and precursor concentrations at a background site in the UAE
Markedly different impacts of primary emissions and secondary aerosol formation on aerosol mixing states revealed by simultaneous measurements of CCNC, H(/V)TDMA, and SP2
Phase matrix characterization of long-range transported Saharan dust using multiwavelength polarized polar imaging nephelometry
Vertically resolved aerosol variability at the Amazon Tall Tower Observatory under wet-season conditions
Vertical structure of a springtime smoky and humid troposphere over the southeast Atlantic from aircraft and reanalysis
Measurement Report: Long-term Assessment of Primary and Secondary Organic Aerosols in Shanghai Megacity throughout China’s Clean Air Actions since 2010
Shipborne observations of black carbon aerosols in the western Arctic Ocean during summer and autumn 2016–2020: impact of boreal fires
Attribution of aerosol particle number size distributions to main sources using an 11-year urban dataset
Sihan Liu, Honglei Wang, Delong Zhao, Wei Zhou, Yuanmou Du, Zhengguo Zhang, Peng Cheng, Tianliang Zhao, Yue Ke, Zihao Wu, and Mengyu Huang
Atmos. Chem. Phys., 25, 4151–4165, https://doi.org/10.5194/acp-25-4151-2025, https://doi.org/10.5194/acp-25-4151-2025, 2025
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To understand the effect of aerosols on the vertical distribution of stratocumulus microphysical quantities in southwest China, the daily variation characteristics and formation mechanism of the vertical profiles of stratocumulus microphysical characteristics in this region were described using the data of nine cloud-crossing aircraft observations over Guangxi from 10 October to 3 November 2020.
Denghui Ji, Mathias Palm, Matthias Buschmann, Kerstin Ebell, Marion Maturilli, Xiaoyu Sun, and Justus Notholt
Atmos. Chem. Phys., 25, 3889–3904, https://doi.org/10.5194/acp-25-3889-2025, https://doi.org/10.5194/acp-25-3889-2025, 2025
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Our study explores how certain aerosols, like sea salt, affect infrared heat radiation in the Arctic, potentially speeding up warming. We used advanced technology to measure aerosol composition and found that these particles grow with humidity, significantly increasing their heat-trapping effect in the infrared region, especially in winter. Our findings suggest these aerosols could be a key factor in Arctic warming, emphasizing the importance of understanding aerosols for climate prediction.
Haibiao Chen, Caiqing Yan, Liubin Huang, Lin Du, Yang Yue, Xinfeng Wang, Qingcai Chen, Mingjie Xie, Junwen Liu, Fengwen Wang, Shuhong Fang, Qiaoyun Yang, Hongya Niu, Mei Zheng, Yan Wu, and Likun Xue
Atmos. Chem. Phys., 25, 3647–3667, https://doi.org/10.5194/acp-25-3647-2025, https://doi.org/10.5194/acp-25-3647-2025, 2025
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A comprehensive understanding of the optical properties of brown carbon (BrC) is essential to accurately assess its climatic effects. Based on multi-site spectroscopic measurements, this study demonstrated the significant spatial heterogeneity in the optical and structural properties of water-soluble organic carbon (WSOC) in different regions of China and revealed factors affecting WSOC light absorption and the relationship between fluorophores and light absorption of WSOC.
Lingjun Li, Mengren Li, Xiaolong Fan, Yuping Chen, Ziyi Lin, Anqi Hou, Siqing Zhang, Ronghua Zheng, and Jinsheng Chen
Atmos. Chem. Phys., 25, 3669–3685, https://doi.org/10.5194/acp-25-3669-2025, https://doi.org/10.5194/acp-25-3669-2025, 2025
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Here, we show differences and variations in the aerosol scattering hygroscopic growth factor (f(RH)) between new particle formation (NPF) and non-NPF days and the effect of aerosol chemical compositions on f(RH) in Xiamen with in situ observations. The findings are helpful for the further understanding of aerosol hygroscopicity in a coastal city and the use of hygroscopic growth factors in models of air quality and climate change.
Roman Pohorsky, Andrea Baccarini, Natalie Brett, Brice Barret, Slimane Bekki, Gianluca Pappaccogli, Elsa Dieudonné, Brice Temime-Roussel, Barbara D'Anna, Meeta Cesler-Maloney, Antonio Donateo, Stefano Decesari, Kathy S. Law, William R. Simpson, Javier Fochesatto, Steve R. Arnold, and Julia Schmale
Atmos. Chem. Phys., 25, 3687–3715, https://doi.org/10.5194/acp-25-3687-2025, https://doi.org/10.5194/acp-25-3687-2025, 2025
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This study presents an analysis of vertical measurements of pollution in an Alaskan city during winter. It investigates the relationship between the atmospheric structure and the layering of aerosols and trace gases. Results indicate an overall very shallow surface mixing layer. The height of this layer is strongly influenced by a local shallow wind. The study also provides information on the pollution chemical composition at different altitudes, including pollution signatures from power plants.
Aoyuan Yu, Xiaojing Shen, Qianli Ma, Jiayuan Lu, Xinyao Hu, Yangmei Zhang, Quan Liu, Linlin Liang, Lei Liu, Shuo Liu, Hongfei Tong, Huizheng Che, Xiaoye Zhang, and Junying Sun
Atmos. Chem. Phys., 25, 3389–3412, https://doi.org/10.5194/acp-25-3389-2025, https://doi.org/10.5194/acp-25-3389-2025, 2025
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In this work, we utilized a volatility hygroscopicity tandem differential mobility analyzer (VH-TDMA) to investigate, for the first time, the hygroscopicity and volatility of submicron aerosols, as well as their hygroscopicity after heating, in urban Beijing during the autumn of 2023. We analyzed the size-resolved characteristics of hygroscopicity and volatility, the relationship between hygroscopic and volatile properties, and the hygroscopicity of heated submicron aerosols.
Corina Wieber, Lasse Z. Jensen, Leendert Vergeynst, Lorenz Meire, Thomas Juul-Pedersen, Kai Finster, and Tina Šantl-Temkiv
Atmos. Chem. Phys., 25, 3327–3346, https://doi.org/10.5194/acp-25-3327-2025, https://doi.org/10.5194/acp-25-3327-2025, 2025
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The Arctic region is subject to profound changes due to a warming climate. Ice-nucleating particles (INPs) in the seawater can get transported to the atmosphere and impact cloud formation. However, the sources of characteristics of INPs in the marine areas are poorly understood. We investigated the INPs in seawater from Greenlandic fjords and identified a seasonal variability, with highly active INPs originating from terrestrial sources such as glacial and soil runoff.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
Atmos. Chem. Phys., 25, 3191–3211, https://doi.org/10.5194/acp-25-3191-2025, https://doi.org/10.5194/acp-25-3191-2025, 2025
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Aerosols contribute to the largest uncertainties in climate change predictions. The eastern Mediterranean is a hotspot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during A-LIFE (Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics) to characterize aerosols and aerosol mixtures. We extend current lidar classification and separation schemes and compare them to classification schemes using different methods.
Ludovico Di Antonio, Claudia Di Biagio, Paola Formenti, Aline Gratien, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Patrice Coll, Barbara D'Anna, Joel F. de Brito, David O. De Haan, Juliette R. Dignum, Shravan Deshmukh, Olivier Favez, Pierre-Marie Flaud, Cecile Gaimoz, Lelia N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Emilie Perraudin, Jean-Eudes Petit, Prodip Acharja, Laurent Poulain, Pauline Pouyes, Eva Drew Pronovost, Véronique Riffault, Kanuri I. Roundtree, Marwa Shahin, Guillaume Siour, Eric Villenave, Pascal Zapf, Gilles Foret, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 25, 3161–3189, https://doi.org/10.5194/acp-25-3161-2025, https://doi.org/10.5194/acp-25-3161-2025, 2025
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The spectral complex refractive index (CRI) and single scattering albedo were retrieved from submicron aerosol measurements at three sites within the greater Paris area during the ACROSS field campaign (June–July 2022). Measurements revealed urban emission impact on surrounding areas. CRI full period averages at 520 nm were 1.41 – 0.037i (urban), 1.52 – 0.038i (peri-urban), and 1.50 – 0.025i (rural). Organic aerosols dominated the aerosol mass and contributed up to 22 % of absorption at 370 nm.
Leah D. Gibson, Ezra J. T. Levin, Ethan Emerson, Nick Good, Anna Hodshire, Gavin McMeeking, Kate Patterson, Bryan Rainwater, Tom Ramin, and Ben Swanson
Atmos. Chem. Phys., 25, 2745–2762, https://doi.org/10.5194/acp-25-2745-2025, https://doi.org/10.5194/acp-25-2745-2025, 2025
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From fall 2021 to summer 2023, SAIL-Net, a network of six aerosol measurement nodes, was deployed in the East River watershed (Colorado, USA) to study aerosol variability across space and time in mountainous terrain. We found that aerosol variability is influenced by elevation differences, with the most representative site in the region changing seasonally, suggesting aerosol spatial variability also varies seasonally. This work offers a blueprint for future studies in other mountainous regions.
Tahereh Alinejadtabrizi, Yi Huang, Francisco Lang, Steven Siems, Michael Manton, Luis Ackermann, Melita Keywood, Ruhi Humphries, Paul Krummel, Alastair Williams, and Greg Ayers
Atmos. Chem. Phys., 25, 2631–2648, https://doi.org/10.5194/acp-25-2631-2025, https://doi.org/10.5194/acp-25-2631-2025, 2025
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Clouds over the Southern Ocean are crucial to Earth's energy balance, but understanding the factors that control them is complex. Our research examines how weather patterns affect tiny particles called cloud condensation nuclei (CCN), which influence cloud properties. Using data from Kennaook / Cape Grim, we found that winter air from Antarctica brings cleaner conditions with lower CCN, while summer patterns from Australia transport more particles. Precipitation also helps reduce CCN in winter.
Hengjia Ou, Mingfu Cai, Yongyun Zhang, Xue Ni, Baoling Liang, Qibin Sun, Shixin Mai, Cuizhi Sun, Shengzhen Zhou, Haichao Wang, Jiaren Sun, and Jun Zhao
Atmos. Chem. Phys., 25, 2495–2513, https://doi.org/10.5194/acp-25-2495-2025, https://doi.org/10.5194/acp-25-2495-2025, 2025
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Two shipborne observations in the South China Sea (SCS) in summer and winter 2021 were conducted. Our study found aerosol hygroscopicity is higher in the SCS in summer than winter, with significant influences from various terrestrial air masses. Aerosol size distribution had a stronger effect on activation ratio than aerosol hygroscopicity in summer and vice versa in winter. Our study provides valuable information to enhance our understanding of cloud condensation nuclei activities in the SCS.
Bighnaraj Sarangi, Darrel Baumgardner, Ana Isabel Calvo, Benjamin Bolaños-Rosero, Roberto Fraile, Alberto Rodríguez-Fernández, Delia Fernández-González, Carlos Blanco-Alegre, Cátia Gonçalves, Estela D. Vicente, and Olga L. Mayol-Bracero
Atmos. Chem. Phys., 25, 843–865, https://doi.org/10.5194/acp-25-843-2025, https://doi.org/10.5194/acp-25-843-2025, 2025
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Measurements of fluorescing aerosol particle properties have been made during two major African dust events, one over the island of Puerto Rico and the other over the city of León, Spain. The measurements were made with two wideband integrated bioaerosol spectrometers. A significant change in the background aerosol properties, at both locations, is observed when the dust is in the respective regions.
Lijing Chen, Lei Zhang, Yong She, Zhaoliang Zeng, Yu Zheng, Biao Tian, Wenqian Zhang, Zhaohui Liu, Huizheng Che, and Minghu Ding
Atmos. Chem. Phys., 25, 727–739, https://doi.org/10.5194/acp-25-727-2025, https://doi.org/10.5194/acp-25-727-2025, 2025
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Aerosol optical depth (AOD) at Zhongshan Station varies seasonally, with lower values in summer and higher values in winter. Winter and spring AOD increases due to reduced fine-mode particles, while summer and autumn increases are linked to particle growth. Diurnal AOD variation correlates positively with temperature but negatively with wind speed and humidity. Backward trajectories show that aerosols on high-AOD (low-AOD) days primarily originate from the ocean (interior Antarctica).
Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Silvia Henning, Jean-Eudes Petit, Pauline Fombelle, Olivier Favez, Hartmut Herrmann, and Mira Pöhlker
Atmos. Chem. Phys., 25, 741–758, https://doi.org/10.5194/acp-25-741-2025, https://doi.org/10.5194/acp-25-741-2025, 2025
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Aerosol hygroscopicity has been investigated at a sub-urban site in Paris; analysis shows the sub-saturated regime's measured hygroscopicity and the chemically derived hygroscopic growth, shedding light on the large effect of external particle mixing and its influence on predicting hygroscopicity.
Takeshi Kinase, Fumikazu Taketani, Masayuki Takigawa, Chunmao Zhu, Yongwon Kim, Petr Mordovskoi, and Yugo Kanaya
Atmos. Chem. Phys., 25, 143–156, https://doi.org/10.5194/acp-25-143-2025, https://doi.org/10.5194/acp-25-143-2025, 2025
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Boreal forest wildfires in interior Alaska represent an important black carbon (BC) source for the Arctic and surrounding regions. We observed BC and carbon monoxide (CO) concentrations in the Poker Flat Research Range since 2016 and found a positive correlation between the observed BC / ∆CO ratio and fire radiative power (FRP) observed in Alaska and Canada. Our finding suggests the BC emission factor and/or inventory could be potentially improved by using FRP.
Erin N. Raif, Sarah L. Barr, Mark D. Tarn, James B. McQuaid, Martin I. Daily, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Paul R. Field, Kenneth S. Carslaw, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 14045–14072, https://doi.org/10.5194/acp-24-14045-2024, https://doi.org/10.5194/acp-24-14045-2024, 2024
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Ice-nucleating particles (INPs) allow ice to form in clouds at temperatures warmer than −35°C. We measured INP concentrations over the Norwegian and Barents seas in weather events where cold air is ejected from the Arctic. These concentrations were among the highest measured in the Arctic. It is likely that the INPs were transported to the Arctic from distant regions. These results show it is important to consider hemispheric-scale INP processes to understand INP concentrations in the Arctic.
Fernando Rejano, Andrea Casans, Marta Via, Juan Andrés Casquero-Vera, Sonia Castillo, Hassan Lyamani, Alberto Cazorla, Elisabeth Andrews, Daniel Pérez-Ramírez, Andrés Alastuey, Francisco Javier Gómez-Moreno, Lucas Alados-Arboledas, Francisco José Olmo, and Gloria Titos
Atmos. Chem. Phys., 24, 13865–13888, https://doi.org/10.5194/acp-24-13865-2024, https://doi.org/10.5194/acp-24-13865-2024, 2024
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This study provides valuable insights to improve cloud condensation nuclei (CCN) estimations at a high-altitude remote site which is influenced by nearby urban pollution. Understanding the factors that affect CCN estimations is essential to improve the CCN data coverage worldwide and assess aerosol–cloud interactions on a global scale. This is crucial for improving climate models, since aerosol–cloud interactions are the most important source of uncertainty in climate projections.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven G. Howell
Atmos. Chem. Phys., 24, 13849–13864, https://doi.org/10.5194/acp-24-13849-2024, https://doi.org/10.5194/acp-24-13849-2024, 2024
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Using airborne measurements over the southeast Atlantic Ocean, we examined how much moisture aerosols take up during Africa’s biomass burning season. Our study revealed the important role of organic aerosols and introduced a predictive model for moisture uptake, accounting for organics, sulfate, and black carbon, summarizing results from various campaigns. These findings improve our understanding of aerosol–moisture interactions and their radiative effects in this climatically critical region.
Mary C. Robinson, Kaitlin Schueth, and Karin Ardon-Dryer
Atmos. Chem. Phys., 24, 13733–13750, https://doi.org/10.5194/acp-24-13733-2024, https://doi.org/10.5194/acp-24-13733-2024, 2024
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On 26 February 2023, New Mexico and West Texas were impacted by a severe dust storm. To analyze this storm, 28 meteorological stations and 19 PM2.5 and PM10 stations were used. Dust particles were in the air for 16 h, and dust storm conditions lasted for up to 120 min. Hourly PM2.5 and PM10 concentrations were up to 518 and 9983 µg m−3, respectively. For Lubbock, Texas, the maximum PM2.5 concentrations were the highest ever recorded.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa Emmons
Atmos. Chem. Phys., 24, 13477–13502, https://doi.org/10.5194/acp-24-13477-2024, https://doi.org/10.5194/acp-24-13477-2024, 2024
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Aerosol property measurements recently collected on the ground and by a research aircraft in central Argentina during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable data set needed to evaluate and improve model predictions of aerosols in a traditionally data-sparse region of South America.
Julika Zinke, Gabriel Pereira Freitas, Rachel Ann Foster, Paul Zieger, Ernst Douglas Nilsson, Piotr Markuszewski, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 13413–13428, https://doi.org/10.5194/acp-24-13413-2024, https://doi.org/10.5194/acp-24-13413-2024, 2024
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Bioaerosols, which can influence climate and human health, were studied in the Baltic Sea. In May and August 2021, we used a sea spray simulation chamber during two ship-based campaigns to collect and measure these aerosols. We found that microbes were enriched in air compared to seawater. Bacterial diversity was analysed using DNA sequencing. Our methods provided consistent estimates of microbial emission fluxes, aligning with previous studies.
Chimurkar Navinya, Taveen Singh Kapoor, Gupta Anurag, Chandra Venkataraman, Harish C. Phuleria, and Rajan K. Chakrabarty
Atmos. Chem. Phys., 24, 13285–13297, https://doi.org/10.5194/acp-24-13285-2024, https://doi.org/10.5194/acp-24-13285-2024, 2024
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Brown carbon (BrC) aerosols show an order-of-magnitude variation in their light absorption strength. Our understanding of BrC from real-world biomass burning remains limited, complicating the determination of its radiative impact. Our study reports absorption properties of BrC emitted from four major biomass burning sources using field measurements in India. It develops an absorption parameterization for BrC and examines the spatial variability in BrC's absorption strength across India.
Yao Song, Jing Wei, Wenlong Zhao, Jinmei Ding, Xiangyu Pei, Fei Zhang, Zhengning Xu, Ruifang Shi, Ya Wei, Lu Zhang, Lingling Jin, and Zhibin Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3298, https://doi.org/10.5194/egusphere-2024-3298, 2024
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This study investigates the size-resolved effective density (ρeff) of aerosol particles in Hangzhou using an AAC-SMPS. The ρeff values ranged from 1.47 to 1.63 g/cm3, increasing with particle diameter. Smaller particles showed significant diurnal density variations. The relationship between ρeff and particle diameter varies due to differences in the chemical composition of the particles. A new method to derive size-resolved chemical composition of particles from ρeff was proposed.
Sami D. Harni, Minna Aurela, Sanna Saarikoski, Jarkko V. Niemi, Harri Portin, Hanna Manninen, Ville Leinonen, Pasi Aalto, Phil K. Hopke, Tuukka Petäjä, Topi Rönkkö, and Hilkka Timonen
Atmos. Chem. Phys., 24, 12143–12160, https://doi.org/10.5194/acp-24-12143-2024, https://doi.org/10.5194/acp-24-12143-2024, 2024
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In this study, particle number size distribution data were used in a novel way in positive matrix factorization analysis to find aerosol source profiles in the area. Measurements were made in Helsinki at a street canyon and urban background sites between February 2015 and June 2019. Five different aerosol sources were identified. These sources underline the significance of traffic-related emissions in urban environments despite recent improvements in emission reduction technologies.
Natalie G. Ratcliffe, Claire L. Ryder, Nicolas Bellouin, Stephanie Woodward, Anthony Jones, Ben Johnson, Lisa-Maria Wieland, Maximilian Dollner, Josef Gasteiger, and Bernadett Weinzierl
Atmos. Chem. Phys., 24, 12161–12181, https://doi.org/10.5194/acp-24-12161-2024, https://doi.org/10.5194/acp-24-12161-2024, 2024
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Large mineral dust particles are more abundant in the atmosphere than expected and have different impacts on the environment than small particles, which are better represented in climate models. We use aircraft measurements to assess a climate model representation of large-dust transport. We find that the model underestimates the amount of large dust at all stages of transport and that fast removal of the large particles increases this underestimation with distance from the Sahara.
Sergio Rodríguez and Jessica López-Darias
Atmos. Chem. Phys., 24, 12031–12053, https://doi.org/10.5194/acp-24-12031-2024, https://doi.org/10.5194/acp-24-12031-2024, 2024
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Extreme Saharan dust events expanded northward to the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 events. These episodes are caused by low-to-high dipole meteorology during hemispheric anomalies characterized by subtropical anticyclones shifting to higher latitudes, anomalous low pressures beyond the tropics and amplified Rossby waves. Extreme dust events occur in a paradoxical context of a multidecadal decrease in dust emissions, a topic that requires further investigation.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin L. Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Wiedensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
Atmos. Chem. Phys., 24, 12055–12077, https://doi.org/10.5194/acp-24-12055-2024, https://doi.org/10.5194/acp-24-12055-2024, 2024
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Levels of black carbon (BC) are scarcely reported in the Southern Hemisphere, especially in high-altitude conditions. This study provides insight into the concentration level, variability, and optical properties of BC in La Paz and El Alto and at the Chacaltaya Global Atmosphere Watch Station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, in addition to biomass and open waste burning.
Krishnakant Budhavant, Mohanan Remani Manoj, Hari Ram Chandrika Rajendran Nair, Samuel Mwaniki Gaita, Henry Holmstrand, Abdus Salam, Ahmed Muslim, Sreedharan Krishnakumari Satheesh, and Örjan Gustafsson
Atmos. Chem. Phys., 24, 11911–11925, https://doi.org/10.5194/acp-24-11911-2024, https://doi.org/10.5194/acp-24-11911-2024, 2024
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The South Asian Pollution Experiment 2018 used access to three strategically located receptor observatories. Observational constraints revealed opposing trends in the mass absorption cross sections of black carbon (BC MAC) and brown carbon (BrC MAC) during long-range transport. Models estimating the climate effects of BC aerosols may have underestimated the ambient BC MAC over distant receptor areas, leading to discrepancies in aerosol absorption predicted by observation-constrained models.
Jieyao Liu, Fang Zhang, Jingye Ren, and Lu Chen
EGUsphere, https://doi.org/10.5194/egusphere-2024-2999, https://doi.org/10.5194/egusphere-2024-2999, 2024
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The particles mixing states and aging time scale are important for the evaluation of aerosols climate effects, but they are poorly parameterized in current models. We unravel the evolution of real-time mixing states and aging time scale of size-resolved particles based on field measurement in urban Beijing. This study provides observational basis for accurately parameterizing the aging time scale of aerosol particles in climate models.
Abigail S. Williams, Jeramy L. Dedrick, Lynn M. Russell, Florian Tornow, Israel Silber, Ann M. Fridlind, Benjamin Swanson, Paul J. DeMott, Paul Zieger, and Radovan Krejci
Atmos. Chem. Phys., 24, 11791–11805, https://doi.org/10.5194/acp-24-11791-2024, https://doi.org/10.5194/acp-24-11791-2024, 2024
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The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentrations, smaller Hoppel minima, lower effective supersaturations, and accumulation-mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol–cloud interactions in order to improve their accurate representation in models.
Franziska Vogel, Michael P. Adams, Larissa Lacher, Polly B. Foster, Grace C. E. Porter, Barbara Bertozzi, Kristina Höhler, Julia Schneider, Tobias Schorr, Nsikanabasi S. Umo, Jens Nadolny, Zoé Brasseur, Paavo Heikkilä, Erik S. Thomson, Nicole Büttner, Martin I. Daily, Romy Fösig, Alexander D. Harrison, Jorma Keskinen, Ulrike Proske, Jonathan Duplissy, Markku Kulmala, Tuukka Petäjä, Ottmar Möhler, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 11737–11757, https://doi.org/10.5194/acp-24-11737-2024, https://doi.org/10.5194/acp-24-11737-2024, 2024
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Primary ice formation in clouds strongly influences their properties; hence, it is important to understand the sources of ice-nucleating particles (INPs) and their variability. We present 2 months of INP measurements in a Finnish boreal forest using a new semi-autonomous INP counting device based on gas expansion. These results show strong variability in INP concentrations, and we present a case that the INPs we observe are, at least some of the time, of biological origin.
Xiaojing Shen, Quan Liu, Junying Sun, Wanlin Kong, Qianli Ma, Bing Qi, Lujie Han, Yangmei Zhang, Linlin Liang, Lei Liu, Shuo Liu, Xinyao Hu, Jiayuan Lu, Aoyuan Yu, Huizheng Che, and Xiaoye Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2850, https://doi.org/10.5194/egusphere-2024-2850, 2024
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In this work, an automatic switched inlet system was developed and employed to investigate the aerosols and cloud droplets at a mountain site with frequent cloud processes. It showed different characteristics of cloud residual and interstitial particles. Stronger particle hygroscopicity reduced liquid water content and smaller cloud droplet diameters. This investigation contributes to understanding aerosol-cloud interactions by assessing the impact of aerosol particles on cloud microphysics.
Rebecca Dischl, Daniel Sauer, Christiane Voigt, Theresa Harlaß, Felicitas Sakellariou, Raphael Märkl, Ulrich Schumann, Monika Scheibe, Stefan Kaufmann, Anke Roiger, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Mark Johnson, Denise Ahrens, Reetu Sallinen, Tobias Schripp, Georg Eckel, Uwe Bauder, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 11255–11273, https://doi.org/10.5194/acp-24-11255-2024, https://doi.org/10.5194/acp-24-11255-2024, 2024
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In-flight measurements of aircraft emissions burning 100 % sustainable aviation fuel (SAF) show reduced particle number concentrations up to 41 % compared to conventional jet fuel. Particle emissions are dependent on engine power setting, flight altitude, and fuel composition. Engine models show a good correlation with measurement results. Future increased prevalence of SAF can positively influence the climate impact of aviation.
Zoé Brasseur, Julia Schneider, Janne Lampilahti, Ville Vakkari, Victoria A. Sinclair, Christina J. Williamson, Carlton Xavier, Dmitri Moisseev, Markus Hartmann, Pyry Poutanen, Markus Lampimäki, Markku Kulmala, Tuukka Petäjä, Katrianne Lehtipalo, Erik S. Thomson, Kristina Höhler, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 24, 11305–11332, https://doi.org/10.5194/acp-24-11305-2024, https://doi.org/10.5194/acp-24-11305-2024, 2024
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Ice-nucleating particles (INPs) strongly influence the formation of clouds by initiating the formation of ice crystals. However, very little is known about the vertical distribution of INPs in the atmosphere. Here, we present aircraft measurements of INP concentrations above the Finnish boreal forest. Results show that near-surface INPs are efficiently transported and mixed within the boundary layer and occasionally reach the free troposphere.
Piotr Markuszewski, E. Douglas Nilsson, Julika Zinke, E. Monica Mårtensson, Matthew Salter, Przemysław Makuch, Małgorzata Kitowska, Iwona Niedźwiecka-Wróbel, Violetta Drozdowska, Dominik Lis, Tomasz Petelski, Luca Ferrero, and Jacek Piskozub
Atmos. Chem. Phys., 24, 11227–11253, https://doi.org/10.5194/acp-24-11227-2024, https://doi.org/10.5194/acp-24-11227-2024, 2024
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Our research provides new insights into the study of sea spray aerosol (SSA) emissions in the Baltic Sea and North Atlantic. We observed that SSA flux is suppressed during increased marine biological activity in the Baltic Sea. At the same time, the influence of wave age showed higher SSA emissions in the Baltic Sea for younger waves compared to the Atlantic Ocean. These insights underscore the complex interplay between biological activity and physical dynamics in regulating SSA emissions.
Heather Guy, Andrew S. Martin, Erik Olson, Ian M. Brooks, and Ryan R. Neely III
Atmos. Chem. Phys., 24, 11103–11114, https://doi.org/10.5194/acp-24-11103-2024, https://doi.org/10.5194/acp-24-11103-2024, 2024
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Aerosol particles impact cloud properties which influence Greenland Ice Sheet melt. Understanding the aerosol population that interacts with clouds is important for constraining future melt. Measurements of aerosols at cloud height over Greenland are rare, and surface measurements are often used to investigate cloud–aerosol interactions. We use a tethered balloon to measure aerosols up to cloud base and show that surface measurements are often not equivalent to those just below the cloud.
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
Atmos. Chem. Phys., 24, 10985–11004, https://doi.org/10.5194/acp-24-10985-2024, https://doi.org/10.5194/acp-24-10985-2024, 2024
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We examined aerosol particles from wildfires and identified tarballs (TBs) from the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign. This study reveals the compositions, abundance, sizes, and mixing states of TBs and shows that TBs formed as the smoke aged for up to 5 h. This study provides measurements of TBs from various biomass-burning events and ages, enhancing our knowledge of TB emissions and our understanding of their climate impact.
Jia Sun, Markus Hermann, Kay Weinhold, Maik Merkel, Wolfram Birmili, Yifan Yang, Thomas Tuch, Harald Flentje, Björn Briel, Ludwig Ries, Cedric Couret, Michael Elsasser, Ralf Sohmer, Klaus Wirtz, Frank Meinhardt, Maik Schütze, Olaf Bath, Bryan Hellack, Veli-Matti Kerminen, Markku Kulmala, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 24, 10667–10687, https://doi.org/10.5194/acp-24-10667-2024, https://doi.org/10.5194/acp-24-10667-2024, 2024
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We investigated the characteristics of new particle formation (NPF) for various environments from urban background to high Alpine and the impacts of NPF on cloud condensation nuclei and aerosol radiative forcing. NPF features differ between site categories, implying the crucial role of local environmental factors such as the degree of emissions and meteorological conditions. The results also underscore the importance of local environments when assessing the impact of NPF on climate in models.
Baptiste Testa, Lukas Durdina, Jacinta Edebeli, Curdin Spirig, and Zamin A. Kanji
Atmos. Chem. Phys., 24, 10409–10424, https://doi.org/10.5194/acp-24-10409-2024, https://doi.org/10.5194/acp-24-10409-2024, 2024
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Aviation soot residuals released from contrails can become compacted upon sublimation of the ice crystals, generating new voids in the aggregates where ice nucleation can occur. Here we show that contrail-processed soot is highly compact but that it remains unable to form ice at a relative humidity different from that required for the formation of background cirrus from the more ubiquitous aqueous solution droplets, suggesting that it will not perturb cirrus cloud formation via ice nucleation.
Kunfeng Gao, Franziska Vogel, Romanos Foskinis, Stergios Vratolis, Maria I. Gini, Konstantinos Granakis, Anne-Claire Billault-Roux, Paraskevi Georgakaki, Olga Zografou, Prodromos Fetfatzis, Alexis Berne, Alexandros Papayannis, Konstantinos Eleftheridadis, Ottmar Möhler, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9939–9974, https://doi.org/10.5194/acp-24-9939-2024, https://doi.org/10.5194/acp-24-9939-2024, 2024
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Ice nucleating particle (INP) concentrations are required for correct predictions of clouds and precipitation in a changing climate, but they are poorly constrained in climate models. We unravel source contributions to INPs in the eastern Mediterranean and find that biological particles are important, regardless of their origin. The parameterizations developed exhibit superior performance and enable models to consider biological-particle effects on INPs.
Alexandra Kuwano, Amato T. Evan, Blake Walkowiak, and Robert Frouin
Atmos. Chem. Phys., 24, 9843–9868, https://doi.org/10.5194/acp-24-9843-2024, https://doi.org/10.5194/acp-24-9843-2024, 2024
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The dust direct radiative effect is highly uncertain. Here we used new measurements collected over 3 years and during dust storms at a field site in a desert region in the southwestern United States to estimate the regional dust direct radiative effect. We also used novel soil mineralogy retrieved from an airborne spectrometer to estimate this parameter with model output. We find that, in this region, dust has a minimal net cooling effect on this region's climate.
Jutta Kesti, Ewan J. O'Connor, Anne Hirsikko, John Backman, Maria Filioglou, Anu-Maija Sundström, Juha Tonttila, Heikki Lihavainen, Hannele Korhonen, and Eija Asmi
Atmos. Chem. Phys., 24, 9369–9386, https://doi.org/10.5194/acp-24-9369-2024, https://doi.org/10.5194/acp-24-9369-2024, 2024
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The study combines aerosol particle measurements at the surface and vertical profiling of the atmosphere with a scanning Doppler lidar to investigate how particle transportation together with boundary layer evolution can affect particle and SO2 concentrations at the surface in the Arabian Peninsula region. The instrumentation enabled us to see elevated nucleation mode particle and SO2 concentrations at the surface when air masses transported from polluted areas are mixed in the boundary layer.
Jiangchuan Tao, Biao Luo, Weiqi Xu, Gang Zhao, Hanbin Xu, Biao Xue, Miaomiao Zhai, Wanyun Xu, Huarong Zhao, Sanxue Ren, Guangsheng Zhou, Li Liu, Ye Kuang, and Yele Sun
Atmos. Chem. Phys., 24, 9131–9154, https://doi.org/10.5194/acp-24-9131-2024, https://doi.org/10.5194/acp-24-9131-2024, 2024
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Using simultaneous measurements of DMA–CCNC, H(/V)TDMA, and DMA–SP2, impacts of primary emissions and secondary aerosol formations on changes in aerosol physicochemical properties were comprehensively investigated. It was found that intercomparisons among aerosol mixing-state parameters derived from different techniques can help us gain more insight into aerosol physical properties which, in turn, will aid the investigation of emission characteristics and secondary aerosol formation pathways.
Elena Bazo, Daniel Perez-Ramirez, Antonio Valenzuela, Vanderlei Martins, Gloria Titos, Alberto Cazorla, Fernando Rejano, Diego Patrón, Arlett Diaz-Zurita, Francisco Jose Garcia-Izquierdo, David Fuertes, Lucas Alados-Arboledas, and Francisco Jose Olmo
EGUsphere, https://doi.org/10.5194/egusphere-2024-2080, https://doi.org/10.5194/egusphere-2024-2080, 2024
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This works analyses aerosol scattering phase function for transported Saharan dust to the city of Granada – located in southwestern Europe. We use the novel technique polar imaging nephelometry that helps to determine the phase functions using a CCD camara. The capability of measuring with polarized light helps to inferr new properties about the mixture of Saharan dust particles with other of anthropogenic origin.
Marco A. Franco, Rafael Valiati, Bruna A. Holanda, Bruno B. Meller, Leslie A. Kremper, Luciana V. Rizzo, Samara Carbone, Fernando G. Morais, Janaína P. Nascimento, Meinrat O. Andreae, Micael A. Cecchini, Luiz A. T. Machado, Milena Ponczek, Ulrich Pöschl, David Walter, Christopher Pöhlker, and Paulo Artaxo
Atmos. Chem. Phys., 24, 8751–8770, https://doi.org/10.5194/acp-24-8751-2024, https://doi.org/10.5194/acp-24-8751-2024, 2024
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The Amazon wet-season atmosphere was studied at the Amazon Tall Tower Observatory site, revealing vertical variations (between 60 and 325 m) in natural aerosols. Daytime mixing contrasted with nighttime stratification, with distinct rain-induced changes in aerosol populations. Notably, optical property recovery at higher levels was faster, while near-canopy aerosols showed higher scattering efficiency. These findings enhance our understanding of aerosol impacts on climate dynamics.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Haifeng Yu, Yunhua Chang, Lin Cheng, Yusen Duan, and Jianlin Hu
EGUsphere, https://doi.org/10.5194/egusphere-2024-1488, https://doi.org/10.5194/egusphere-2024-1488, 2024
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This study presents long-term measurements and comprehensive analysis of carbonaceous aerosols in PM2.5 in Shanghai. We further estimated POC and SOC levels, examining their temporal variations on interannual, monthly, seasonal, and diurnal scales. Through rigorous statistical analysis and correlation studies with meteorological parameters and pollutant concentrations, the origins, formation mechanisms, and spatial distribution patterns of SOC were elucidated.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
Atmos. Chem. Phys., 24, 6339–6357, https://doi.org/10.5194/acp-24-6339-2024, https://doi.org/10.5194/acp-24-6339-2024, 2024
Short summary
Short summary
Black carbon (BC) aerosols play important roles in Arctic climate change, yet they are not well understood because of limited observational data. We observed BC mass concentrations (mBC) in the western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high-BC events in the Arctic Ocean.
Máté Vörösmarty, Philip K. Hopke, and Imre Salma
Atmos. Chem. Phys., 24, 5695–5712, https://doi.org/10.5194/acp-24-5695-2024, https://doi.org/10.5194/acp-24-5695-2024, 2024
Short summary
Short summary
The World Health Organization identified ultrafine particles, which make up most of the particle number concentrations, as a potential risk factor for humans. The sources of particle numbers are very different from those of the particulate matter mass. We performed source apportionment of size-segregated particle number concentrations over the diameter range of 6–1000 nm in Budapest for 11 full years. Six source types were identified, characterized and quantified.
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Short summary
A campaign was performed in the summer of 2013 above the Mediterranean basin, including in situ counting balloon-borne aerosol measurements (LOAC), for the detection of mineral dust. Three modes in the dust particle volume size distributions were detected, at roughly 0.2, 4, and 30 mm. Particles larger than 40 mm were often observed. They were lifted several days before and their persistence after transport over long distances is in conflict with dust sedimentation calculations.
A campaign was performed in the summer of 2013 above the Mediterranean basin, including in situ...
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