Articles | Volume 14, issue 14
https://doi.org/10.5194/acp-14-7291-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-7291-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
17 Jul 2014
Research article |
| 17 Jul 2014
The effect of solar zenith angle on MODIS cloud optical and microphysical retrievals within marine liquid water clouds
D. P. Grosvenor
now at: School of Earth and Environment, University of Leeds, UK
Department of Atmospheric Science, University of Washington, Seattle, USA
Department of Atmospheric Science, University of Washington, Seattle, USA
Related authors
Masaru Yoshioka, Daniel P. Grosvenor, Amy H. Peace, Jim M. Haywood, Ying Chen, and Paul R. Field
EGUsphere, https://doi.org/10.5194/egusphere-2025-3244, https://doi.org/10.5194/egusphere-2025-3244, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
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We used advanced computer simulations to study how aerosol particles from a volcanic eruption in Iceland affected clouds. The eruption plume increased small droplets, but changes in cloud water and horizontal extent were not clear. Satellite comparisons between plume and non-plume regions can miss volcanic effects due to spatial variability in weather and aerosol, but simulations can isolate the impact by comparing cases with and without the eruption.
Emma Sands, Ruth M. Doherty, Fiona M. O'Connor, Richard J. Pope, James Weber, and Daniel P. Grosvenor
Atmos. Chem. Phys., 25, 7269–7297, https://doi.org/10.5194/acp-25-7269-2025, https://doi.org/10.5194/acp-25-7269-2025, 2025
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We perform a detailed satellite–model comparison for isoprene, formaldehyde and aerosol optical depth in an Earth system model. We quantify the impacts of several processes that affect how biosphere–atmosphere interactions influence atmospheric chemistry and aerosols. Our findings highlight that the aerosol direct effect is sensitive to the processes studied. These results can inform future investigations of how the biosphere can affect atmospheric composition and climate.
Xuemei Wang, Kenneth S. Carslaw, Daniel P. Grosvenor, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2025-132, https://doi.org/10.5194/egusphere-2025-132, 2025
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Anthropogenic emissions can influence aerosol particle number concentrations via new particle formation. Our model simulations predict around 10 % increase of the particle and cloud droplet number concentrations when doubling the emissions in the Manaus region in the Amazonian wet season. However, the corresponding changes in cloud water and rain mass are around 4 %. Such weak response implied that this convective environment is not sensitive to the localised anthropogenic emission changes here.
Xinyi Huang, Paul R. Field, Benjamin J. Murray, Daniel P. Grosvenor, Floortje van den Heuvel, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-4070, https://doi.org/10.5194/egusphere-2024-4070, 2025
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Short summary
Cold-air outbreak (CAO) clouds play a vital role in climate prediction. This study explores the responses of CAO clouds to aerosols and ice production under different environmental conditions. We found that CAO cloud responses vary with cloud temperature and are strongly controlled by the liquid-ice partitioning in these clouds, suggesting the importance of good representations of cloud microphysics properties to predict the behaviours of CAO clouds in a warming climate.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
Short summary
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
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A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Pratapaditya Ghosh, Katherine J. Evans, Daniel P. Grosvenor, Hyun-Gyu Kang, Salil Mahajan, Min Xu, Wei Zhang, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2024-2423, https://doi.org/10.5194/egusphere-2024-2423, 2024
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The most popular algorithm for calculating cloud droplet number concentrations in climate models is sensitive to parameters that control simulated aerosol particle number concentrations at different sizes. We recommend small modifications to functions in the algorithm to improve its performance. Implementing our changes in the UK Met Office climate model reduced average bias in simulated global droplet number concentrations, leading to more reflected solar radiation and a net cooling effect.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David M. H. Sexton, Christopher Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John W. Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 8749–8768, https://doi.org/10.5194/acp-23-8749-2023, https://doi.org/10.5194/acp-23-8749-2023, 2023
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Aerosol forcing of Earth’s energy balance has persisted as a major cause of uncertainty in climate simulations over generations of climate model development. We show that structural deficiencies in a climate model are exposed by comprehensively exploring parametric uncertainty and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. This provides a future pathway towards building models with greater physical realism and lower uncertainty.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 23, 6743–6773, https://doi.org/10.5194/acp-23-6743-2023, https://doi.org/10.5194/acp-23-6743-2023, 2023
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We determine what causes long-term trends in short-wave (SW) radiative fluxes in two climate models. A positive trend occurs between 1850 and 1970 (increasing SW reflection) and a negative trend between 1970 and 2014; the pre-1970 positive trend is mainly driven by an increase in cloud droplet number concentrations due to increases in aerosol, and the 1970–2014 trend is driven by a decrease in cloud fraction, which we attribute to changes in clouds caused by greenhouse gas-induced warming.
Xuemei Wang, Hamish Gordon, Daniel P. Grosvenor, Meinrat O. Andreae, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 4431–4461, https://doi.org/10.5194/acp-23-4431-2023, https://doi.org/10.5194/acp-23-4431-2023, 2023
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New particle formation in the upper troposphere is important for the global boundary layer aerosol population, and they can be transported downward in Amazonia. We use a global and a regional model to quantify the number of aerosols that are formed at high altitude and transported downward in a 1000 km region. We find that the majority of the aerosols are from outside the region. This suggests that the 1000 km region is unlikely to be a
closed loopfor aerosol formation, transport and growth.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David Sexton, Christopher C. Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2022-1330, https://doi.org/10.5194/egusphere-2022-1330, 2022
Preprint archived
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We show that potential structural deficiencies in a climate model can be exposed by comprehensively exploring its parametric uncertainty, and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. Combined consideration of parametric and structural uncertainties provides a future pathway towards building models that have greater physical realism and lower uncertainty.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
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Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 20, 15681–15724, https://doi.org/10.5194/acp-20-15681-2020, https://doi.org/10.5194/acp-20-15681-2020, 2020
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Particles arising from human activity interact with clouds and affect how much of the Sun's energy is reflected away. Lack of understanding about how to represent this in models leads to large uncertainties in climate predictions. We quantify cloud responses to particles in the latest UK Met Office climate model over the North Atlantic Ocean, showing that, in contrast to suggestions elsewhere, increases in cloud coverage and thickness are important over large areas.
Hamish Gordon, Paul R. Field, Steven J. Abel, Paul Barrett, Keith Bower, Ian Crawford, Zhiqiang Cui, Daniel P. Grosvenor, Adrian A. Hill, Jonathan Taylor, Jonathan Wilkinson, Huihui Wu, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, https://doi.org/10.5194/acp-20-10997-2020, 2020
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The Met Office's Unified Model is widely used both for weather forecasting and climate prediction. We present the first version of the model in which both aerosol and cloud particle mass and number concentrations are allowed to evolve separately and independently, which is important for studying how aerosols affect weather and climate. We test the model against aircraft observations near Ascension Island in the Atlantic, focusing on how aerosols can "activate" to become cloud droplets.
Leighton A. Regayre, Julia Schmale, Jill S. Johnson, Christian Tatzelt, Andrea Baccarini, Silvia Henning, Masaru Yoshioka, Frank Stratmann, Martin Gysel-Beer, Daniel P. Grosvenor, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10063–10072, https://doi.org/10.5194/acp-20-10063-2020, https://doi.org/10.5194/acp-20-10063-2020, 2020
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The amount of energy reflected back into space because of man-made particles is highly uncertain. Processes related to naturally occurring particles cause most of the uncertainty, but these processes are poorly constrained by present-day measurements. We show that measurements over the Southern Ocean, far from pollution sources, efficiently reduce climate model uncertainties. Our results pave the way to designing experiments and measurement campaigns that reduce this uncertainty even further.
Daniel T. McCoy, Paul Field, Hamish Gordon, Gregory S. Elsaesser, and Daniel P. Grosvenor
Atmos. Chem. Phys., 20, 4085–4103, https://doi.org/10.5194/acp-20-4085-2020, https://doi.org/10.5194/acp-20-4085-2020, 2020
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Incomplete understanding of how aerosol affects clouds degrades our ability to predict future climate. In particular, it is unclear how aerosol affects the lifetime of clouds. Does it increase or decrease it? This confusion is partially because causality flows from aerosol to clouds and clouds to aerosol, and it is hard to tell what is happening in observations. Here, we use simulations to tell us about how clouds affect aerosol and use this to interpret observations, showing increased lifetime.
Hamish Gordon, Paul R. Field, Steven J. Abel, Mohit Dalvi, Daniel P. Grosvenor, Adrian A. Hill, Ben T. Johnson, Annette K. Miltenberger, Masaru Yoshioka, and Ken S. Carslaw
Atmos. Chem. Phys., 18, 15261–15289, https://doi.org/10.5194/acp-18-15261-2018, https://doi.org/10.5194/acp-18-15261-2018, 2018
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Smoke from African fires is frequently transported across the Atlantic Ocean, where it interacts with clouds. We simulate the interaction of the smoke with the clouds, and the consequences of this for the solar radiation the clouds reflect. The simulations use a new regional configuration of the UK Met Office climate model. Our simulations indicate that the properties of the clouds, in particular their height and reflectivity, and the fractional cloud cover, are strongly affected by the smoke.
Daniel P. Grosvenor, Odran Sourdeval, and Robert Wood
Atmos. Meas. Tech., 11, 4273–4289, https://doi.org/10.5194/amt-11-4273-2018, https://doi.org/10.5194/amt-11-4273-2018, 2018
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We provide a parameterized correction to the retrieval of cloud effective radius from satellite instruments to account for the assumption that the retrieved value is representative of that at cloud top, whereas in reality it is representative of that lower down. The error leads to errors (which we quantify) in the retrieved cloud droplet concentrations of up to 38 % for stratocumulus regions and also to liquid water path errors, both of which can be corrected using our parameterizations.
Daniel T. McCoy, Paul R. Field, Anja Schmidt, Daniel P. Grosvenor, Frida A.-M. Bender, Ben J. Shipway, Adrian A. Hill, Jonathan M. Wilkinson, and Gregory S. Elsaesser
Atmos. Chem. Phys., 18, 5821–5846, https://doi.org/10.5194/acp-18-5821-2018, https://doi.org/10.5194/acp-18-5821-2018, 2018
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Here we use a combination of global convection-permitting models, satellite observations and the Holuhraun volcanic eruption to demonstrate that aerosol enhances the cloud liquid content and brightness of midlatitude cyclones. This is important because the strength of anthropogenic radiative forcing is uncertain, leading to uncertainty in the climate sensitivity consistent with observed temperature record.
Daniel T. McCoy, Frida A.-M. Bender, Daniel P. Grosvenor, Johannes K. Mohrmann, Dennis L. Hartmann, Robert Wood, and Paul R. Field
Atmos. Chem. Phys., 18, 2035–2047, https://doi.org/10.5194/acp-18-2035-2018, https://doi.org/10.5194/acp-18-2035-2018, 2018
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The interaction between clouds and aerosols represents the largest source of uncertainty in the anthropogenic radiative forcing. Cloud droplet number concentration (CDNC) is the state variable that moderates the interaction between aerosol and clouds. Here we show that CDNC decreases off the coasts of East Asia and North America due to controls on emissions. We support this analysis through an examination of volcanism in Hawaii and Vanuatu.
Daniel P. Grosvenor, Paul R. Field, Adrian A. Hill, and Benjamin J. Shipway
Atmos. Chem. Phys., 17, 5155–5183, https://doi.org/10.5194/acp-17-5155-2017, https://doi.org/10.5194/acp-17-5155-2017, 2017
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We used a weather model to simulate low-level layer clouds that lie off the coast of Chile and tested how they would be affected by airborne particulate matter (aerosols) according to the model. We found that as aerosols were increased, the clouds reflected more and more of the sun’s incoming energy due to the combined effects of the cloud droplets becoming smaller, the thickening of clouds, and increased areal coverage. However, the latter two effects were only important at low aerosol levels.
D. P. Grosvenor, J. C. King, T. W. Choularton, and T. Lachlan-Cope
Atmos. Chem. Phys., 14, 9481–9509, https://doi.org/10.5194/acp-14-9481-2014, https://doi.org/10.5194/acp-14-9481-2014, 2014
Masaru Yoshioka, Daniel P. Grosvenor, Amy H. Peace, Jim M. Haywood, Ying Chen, and Paul R. Field
EGUsphere, https://doi.org/10.5194/egusphere-2025-3244, https://doi.org/10.5194/egusphere-2025-3244, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We used advanced computer simulations to study how aerosol particles from a volcanic eruption in Iceland affected clouds. The eruption plume increased small droplets, but changes in cloud water and horizontal extent were not clear. Satellite comparisons between plume and non-plume regions can miss volcanic effects due to spatial variability in weather and aerosol, but simulations can isolate the impact by comparing cases with and without the eruption.
Emma Sands, Ruth M. Doherty, Fiona M. O'Connor, Richard J. Pope, James Weber, and Daniel P. Grosvenor
Atmos. Chem. Phys., 25, 7269–7297, https://doi.org/10.5194/acp-25-7269-2025, https://doi.org/10.5194/acp-25-7269-2025, 2025
Short summary
Short summary
We perform a detailed satellite–model comparison for isoprene, formaldehyde and aerosol optical depth in an Earth system model. We quantify the impacts of several processes that affect how biosphere–atmosphere interactions influence atmospheric chemistry and aerosols. Our findings highlight that the aerosol direct effect is sensitive to the processes studied. These results can inform future investigations of how the biosphere can affect atmospheric composition and climate.
Je-Yun Chun, Robert Wood, Peter N. Blossey, and Sarah J. Doherty
Atmos. Chem. Phys., 25, 5251–5271, https://doi.org/10.5194/acp-25-5251-2025, https://doi.org/10.5194/acp-25-5251-2025, 2025
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This study explores how aerosols affect clouds transitioning from stratocumulus to cumulus along trade winds under varying atmospheric conditions. We found that aerosols typically reduce precipitation and raise cloud height, but their impact changes when subsidence changes by aerosol enhancement are considered. Our findings indicate that the cooling effect of aerosols might be overestimated if these atmospheric changes are not accounted for.
Chris J. Wright, Joel A. Thornton, Lyatt Jaeglé, Yang Cao, Yannian Zhu, Jihu Liu, Randall Jones II, Robert Holzworth, Daniel Rosenfeld, Robert Wood, Peter Blossey, and Daehyun Kim
Atmos. Chem. Phys., 25, 2937–2946, https://doi.org/10.5194/acp-25-2937-2025, https://doi.org/10.5194/acp-25-2937-2025, 2025
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Aerosol particles influence clouds, which exert a large forcing on solar radiation and freshwater. To better understand the mechanisms by which aerosol influences thunderstorms, we look at the two busiest shipping lanes in the world, where recent regulations have reduced sulfur emissions by nearly an order of magnitude. We find that the reduction in emissions has been accompanied by a dramatic decrease in both lightning and the number of droplets in clouds over the shipping lanes.
Xuemei Wang, Kenneth S. Carslaw, Daniel P. Grosvenor, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2025-132, https://doi.org/10.5194/egusphere-2025-132, 2025
Short summary
Short summary
Anthropogenic emissions can influence aerosol particle number concentrations via new particle formation. Our model simulations predict around 10 % increase of the particle and cloud droplet number concentrations when doubling the emissions in the Manaus region in the Amazonian wet season. However, the corresponding changes in cloud water and rain mass are around 4 %. Such weak response implied that this convective environment is not sensitive to the localised anthropogenic emission changes here.
Xinyi Huang, Paul R. Field, Benjamin J. Murray, Daniel P. Grosvenor, Floortje van den Heuvel, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-4070, https://doi.org/10.5194/egusphere-2024-4070, 2025
Short summary
Short summary
Cold-air outbreak (CAO) clouds play a vital role in climate prediction. This study explores the responses of CAO clouds to aerosols and ice production under different environmental conditions. We found that CAO cloud responses vary with cloud temperature and are strongly controlled by the liquid-ice partitioning in these clouds, suggesting the importance of good representations of cloud microphysics properties to predict the behaviours of CAO clouds in a warming climate.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
Short summary
Short summary
Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
Short summary
Short summary
A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Philip J. Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah J. Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
Geosci. Model Dev., 17, 7963–7994, https://doi.org/10.5194/gmd-17-7963-2024, https://doi.org/10.5194/gmd-17-7963-2024, 2024
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We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming and climate impacts from greenhouse gas increases. This slightly changes clouds in six ocean regions to reflect more sunlight and cool the Earth. Example changes in clouds and climate are shown for three climate models. Cloud changes differ between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Lucas A. McMichael, Michael J. Schmidt, Robert Wood, Peter N. Blossey, and Lekha Patel
Geosci. Model Dev., 17, 7867–7888, https://doi.org/10.5194/gmd-17-7867-2024, https://doi.org/10.5194/gmd-17-7867-2024, 2024
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Marine cloud brightening (MCB) is a climate intervention technique to potentially cool the climate. Climate models used to gauge regional climate impacts associated with MCB often assume large areas of the ocean are uniformly perturbed. However, a more realistic representation of MCB application would require information about how an injected particle plume spreads. This work aims to develop such a plume-spreading model.
Ehsan Erfani, Robert Wood, Peter Blossey, Sarah J. Doherty, and Ryan Eastman
EGUsphere, https://doi.org/10.5194/egusphere-2024-3232, https://doi.org/10.5194/egusphere-2024-3232, 2024
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In this study, we explore how marine clouds interact with aerosols. We introduce a novel approach to identify a reduced number of representative cases from a wide array of observed environmental conditions prevalent in the Northeast Pacific. We created over 2200 trajectories from observations and used cloud-resolving simulations to investigate how marine low clouds evolve in two different cases. It is shown that aerosols can delay cloud breakup, but their impact depends on precipitation.
Pratapaditya Ghosh, Katherine J. Evans, Daniel P. Grosvenor, Hyun-Gyu Kang, Salil Mahajan, Min Xu, Wei Zhang, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2024-2423, https://doi.org/10.5194/egusphere-2024-2423, 2024
Short summary
Short summary
The most popular algorithm for calculating cloud droplet number concentrations in climate models is sensitive to parameters that control simulated aerosol particle number concentrations at different sizes. We recommend small modifications to functions in the algorithm to improve its performance. Implementing our changes in the UK Met Office climate model reduced average bias in simulated global droplet number concentrations, leading to more reflected solar radiation and a net cooling effect.
Ryan Eastman, Isabel L. McCoy, Hauke Schulz, and Robert Wood
Atmos. Chem. Phys., 24, 6613–6634, https://doi.org/10.5194/acp-24-6613-2024, https://doi.org/10.5194/acp-24-6613-2024, 2024
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for 1 year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is, in part, a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds' radiative effect. Future studies must account for differing properties and processes among cloud types.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David M. H. Sexton, Christopher Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John W. Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 8749–8768, https://doi.org/10.5194/acp-23-8749-2023, https://doi.org/10.5194/acp-23-8749-2023, 2023
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Aerosol forcing of Earth’s energy balance has persisted as a major cause of uncertainty in climate simulations over generations of climate model development. We show that structural deficiencies in a climate model are exposed by comprehensively exploring parametric uncertainty and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. This provides a future pathway towards building models with greater physical realism and lower uncertainty.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 23, 6743–6773, https://doi.org/10.5194/acp-23-6743-2023, https://doi.org/10.5194/acp-23-6743-2023, 2023
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We determine what causes long-term trends in short-wave (SW) radiative fluxes in two climate models. A positive trend occurs between 1850 and 1970 (increasing SW reflection) and a negative trend between 1970 and 2014; the pre-1970 positive trend is mainly driven by an increase in cloud droplet number concentrations due to increases in aerosol, and the 1970–2014 trend is driven by a decrease in cloud fraction, which we attribute to changes in clouds caused by greenhouse gas-induced warming.
Amie Dobracki, Paquita Zuidema, Steven G. Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys., 23, 4775–4799, https://doi.org/10.5194/acp-23-4775-2023, https://doi.org/10.5194/acp-23-4775-2023, 2023
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Southern Africa produces approximately one-third of the world’s carbon from fires. The thick smoke layer can flow westward, interacting with the southeastern Atlantic cloud deck. The net radiative impact can alter regional circulation patterns, impacting rainfall over Africa. We find that the smoke is highly absorbing of sunlight, mostly because it contains more black carbon than smoke over the Northern Hemisphere.
Xuemei Wang, Hamish Gordon, Daniel P. Grosvenor, Meinrat O. Andreae, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 4431–4461, https://doi.org/10.5194/acp-23-4431-2023, https://doi.org/10.5194/acp-23-4431-2023, 2023
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New particle formation in the upper troposphere is important for the global boundary layer aerosol population, and they can be transported downward in Amazonia. We use a global and a regional model to quantify the number of aerosols that are formed at high altitude and transported downward in a 1000 km region. We find that the majority of the aerosols are from outside the region. This suggests that the 1000 km region is unlikely to be a
closed loopfor aerosol formation, transport and growth.
Ian Chang, Lan Gao, Connor J. Flynn, Yohei Shinozuka, Sarah J. Doherty, Michael S. Diamond, Karla M. Longo, Gonzalo A. Ferrada, Gregory R. Carmichael, Patricia Castellanos, Arlindo M. da Silva, Pablo E. Saide, Calvin Howes, Zhixin Xue, Marc Mallet, Ravi Govindaraju, Qiaoqiao Wang, Yafang Cheng, Yan Feng, Sharon P. Burton, Richard A. Ferrare, Samuel E. LeBlanc, Meloë S. Kacenelenbogen, Kristina Pistone, Michal Segal-Rozenhaimer, Kerry G. Meyer, Ju-Mee Ryoo, Leonhard Pfister, Adeyemi A. Adebiyi, Robert Wood, Paquita Zuidema, Sundar A. Christopher, and Jens Redemann
Atmos. Chem. Phys., 23, 4283–4309, https://doi.org/10.5194/acp-23-4283-2023, https://doi.org/10.5194/acp-23-4283-2023, 2023
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Abundant aerosols are present above low-level liquid clouds over the southeastern Atlantic during late austral spring. The model simulation differences in the proportion of aerosol residing in the planetary boundary layer and in the free troposphere can greatly affect the regional aerosol radiative effects. This study examines the aerosol loading and fractional aerosol loading in the free troposphere among various models and evaluates them against measurements from the NASA ORACLES campaign.
Francesca Gallo, Janek Uin, Kevin J. Sanchez, Richard H. Moore, Jian Wang, Robert Wood, Fan Mei, Connor Flynn, Stephen Springston, Eduardo B. Azevedo, Chongai Kuang, and Allison C. Aiken
Atmos. Chem. Phys., 23, 4221–4246, https://doi.org/10.5194/acp-23-4221-2023, https://doi.org/10.5194/acp-23-4221-2023, 2023
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This study provides a summary statistic of multiday aerosol plume transport event influences on aerosol physical properties and the cloud condensation nuclei budget at the U.S. Department of Energy Atmospheric Radiation Measurement Facility in the eastern North Atlantic (ENA). An algorithm that integrates aerosol properties is developed and applied to identify multiday aerosol transport events. The influence of the aerosol plumes on aerosol populations at the ENA is successively assessed.
Zhenquan Wang, Jian Yuan, Robert Wood, Yifan Chen, and Tiancheng Tong
Atmos. Chem. Phys., 23, 3247–3266, https://doi.org/10.5194/acp-23-3247-2023, https://doi.org/10.5194/acp-23-3247-2023, 2023
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This study develops a novel profile-based algorithm based on the ERA5 to estimate the inversion strength in the planetary boundary layer better than the previous inversion index, which is a key low-cloud-controlling factor. This improved measure is more effective at representing the meteorological influence on low-cloud variations. It can better constrain the meteorological influence on low clouds to better isolate cloud responses to aerosols or to estimate low cloud feedbacks in climate models.
Je-Yun Chun, Robert Wood, Peter Blossey, and Sarah J. Doherty
Atmos. Chem. Phys., 23, 1345–1368, https://doi.org/10.5194/acp-23-1345-2023, https://doi.org/10.5194/acp-23-1345-2023, 2023
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We investigate the impact of injected aerosol on subtropical low marine clouds under a variety of meteorological conditions using high-resolution model simulations. This study illustrates processes perturbed by aerosol injections and their impact on cloud properties (e.g., cloud number concentration, thickness, and cover). We show that those responses are highly sensitive to background meteorological conditions, such as precipitation, and background cloud properties.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David Sexton, Christopher C. Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2022-1330, https://doi.org/10.5194/egusphere-2022-1330, 2022
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We show that potential structural deficiencies in a climate model can be exposed by comprehensively exploring its parametric uncertainty, and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. Combined consideration of parametric and structural uncertainties provides a future pathway towards building models that have greater physical realism and lower uncertainty.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 22, 14209–14241, https://doi.org/10.5194/acp-22-14209-2022, https://doi.org/10.5194/acp-22-14209-2022, 2022
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The variability in the meteorological fields during each deployment is highly modulated at a daily to synoptic timescale. This paper, along with part 1, the climatological overview paper, provides a meteorological context for interpreting the airborne measurements gathered during the three ORACLES deployments. This study supports related studies focusing on the detailed investigation of the processes controlling stratocumulus decks, aerosol lifting, transport, and their interactions.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Jessica Danker, Odran Sourdeval, Isabel L. McCoy, Robert Wood, and Anna Possner
Atmos. Chem. Phys., 22, 10247–10265, https://doi.org/10.5194/acp-22-10247-2022, https://doi.org/10.5194/acp-22-10247-2022, 2022
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Using spaceborne lidar-radar retrievals, we show that seasonal changes in cloud phase outweigh changes in cloud-phase statistics across cloud morphologies at given cloud-top temperatures. These results show that cloud morphology does not seem to pose a primary constraint on cloud-phase statistics in the Southern Ocean. Meanwhile, larger changes in in-cloud albedo across cloud morphologies are observed in supercooled liquid rather than mixed-phase stratocumuli.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Amie Dobracki, Paquita Zuidema, Steve Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1081, https://doi.org/10.5194/acp-2021-1081, 2022
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The global maximum of shortwave-absorbing aerosol above cloud occurs above the southeast Atlantic, where the biomass-burning aerosol provides a distinct aerosol radiative warming of regional climate. The smoke aerosols are unusually highly absorbing of sunlight. This study seeks to understand the cause. We conclude the aerosol is already strongly absorbing at the fire emission source, but that chemical aging, through encouraging a net loss of organic aerosol, also contributes.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 21, 16689–16707, https://doi.org/10.5194/acp-21-16689-2021, https://doi.org/10.5194/acp-21-16689-2021, 2021
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Part 1 of the meteorological overview paper highlights the anomalous meteorological characteristics during the ORACLES deployment compared to the climatological mean at monthly timescales. The upper-level wave disturbance and the associated anomalous circulation explain the weakening of AEJ-S through the reduction of the strength of the heat low over the land during August 2017. This may also help explain the anomalously low aerosol optical depth observed in the August 2017 ORACLES deployment.
Rachel Atlas, Johannes Mohrmann, Joseph Finlon, Jeremy Lu, Ian Hsiao, Robert Wood, and Minghui Diao
Atmos. Meas. Tech., 14, 7079–7101, https://doi.org/10.5194/amt-14-7079-2021, https://doi.org/10.5194/amt-14-7079-2021, 2021
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Many clouds with temperatures between 0 °C and −40 °C contain both liquid and ice particles, and the ratio of liquid to ice particles influences how the clouds interact with radiation and moderate Earth's climate. We use a machine learning method called random forest to classify images of individual cloud particles as either liquid or ice. We apply our algorithm to images captured by aircraft within clouds overlying the Southern Ocean, and we find that it outperforms two existing algorithms.
Robert Wood
Atmos. Chem. Phys., 21, 14507–14533, https://doi.org/10.5194/acp-21-14507-2021, https://doi.org/10.5194/acp-21-14507-2021, 2021
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A simple model is described to assess the potential for increasing solar reflection by augmenting the aerosol population below marine low clouds, which increases the concentration of cloud droplets. The model is used to predict global cooling from marine cloud brightening climate intervention as a function of the quantity, size, and lifetime of salt particles injected per sprayer, the number of sprayers deployed, the cloud updraft speed, and unperturbed aerosol size distribution.
Yang Wang, Guangjie Zheng, Michael P. Jensen, Daniel A. Knopf, Alexander Laskin, Alyssa A. Matthews, David Mechem, Fan Mei, Ryan Moffet, Arthur J. Sedlacek, John E. Shilling, Stephen Springston, Amy Sullivan, Jason Tomlinson, Daniel Veghte, Rodney Weber, Robert Wood, Maria A. Zawadowicz, and Jian Wang
Atmos. Chem. Phys., 21, 11079–11098, https://doi.org/10.5194/acp-21-11079-2021, https://doi.org/10.5194/acp-21-11079-2021, 2021
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This paper reports the vertical profiles of trace gas and aerosol properties over the eastern North Atlantic, a region of persistent but diverse subtropical marine boundary layer (MBL) clouds. We examined the key processes that drive the cloud condensation nuclei (CCN) population and how it varies with season and synoptic conditions. This study helps improve the model representation of the aerosol processes in the remote MBL, reducing the simulated aerosol indirect effects.
Kristina Pistone, Paquita Zuidema, Robert Wood, Michael Diamond, Arlindo M. da Silva, Gonzalo Ferrada, Pablo E. Saide, Rei Ueyama, Ju-Mee Ryoo, Leonhard Pfister, James Podolske, David Noone, Ryan Bennett, Eric Stith, Gregory Carmichael, Jens Redemann, Connor Flynn, Samuel LeBlanc, Michal Segal-Rozenhaimer, and Yohei Shinozuka
Atmos. Chem. Phys., 21, 9643–9668, https://doi.org/10.5194/acp-21-9643-2021, https://doi.org/10.5194/acp-21-9643-2021, 2021
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Using aircraft-based measurements off the Atlantic coast of Africa, we found the springtime smoke plume was strongly correlated with the amount of water vapor in the atmosphere (more smoke indicated more humidity). We see the same general feature in satellite-assimilated and free-running models. Our analysis suggests this relationship is not caused by the burning but originates due to coincident continental meteorology plus fires. This air is transported over the ocean without further mixing.
Johannes Mohrmann, Robert Wood, Tianle Yuan, Hua Song, Ryan Eastman, and Lazaros Oreopoulos
Atmos. Chem. Phys., 21, 9629–9642, https://doi.org/10.5194/acp-21-9629-2021, https://doi.org/10.5194/acp-21-9629-2021, 2021
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Observations of marine-boundary-layer conditions are composited by cloud type, based on a new classification dataset. It is found that two cloud types, representing regions of clustered and suppressed low-level clouds, occur in very similar large-scale conditions but are distinguished from each other by considering low-level circulation and surface wind fields, validating prior results from modeling.
Maria A. Zawadowicz, Kaitlyn Suski, Jiumeng Liu, Mikhail Pekour, Jerome Fast, Fan Mei, Arthur J. Sedlacek, Stephen Springston, Yang Wang, Rahul A. Zaveri, Robert Wood, Jian Wang, and John E. Shilling
Atmos. Chem. Phys., 21, 7983–8002, https://doi.org/10.5194/acp-21-7983-2021, https://doi.org/10.5194/acp-21-7983-2021, 2021
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This paper describes the results of a recent field campaign in the eastern North Atlantic, where two mass spectrometers were deployed aboard a research aircraft to measure the chemistry of aerosols and trace gases. Very clean conditions were found, dominated by local sulfate-rich acidic aerosol and very aged organics. Evidence of
long-range transport of aerosols from the continents was also identified.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
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Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Tianle Yuan, Hua Song, Robert Wood, Johannes Mohrmann, Kerry Meyer, Lazaros Oreopoulos, and Steven Platnick
Atmos. Meas. Tech., 13, 6989–6997, https://doi.org/10.5194/amt-13-6989-2020, https://doi.org/10.5194/amt-13-6989-2020, 2020
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We use deep transfer learning techniques to classify satellite cloud images into different morphology types. It achieves the state-of-the-art results and can automatically process a large amount of satellite data. The algorithm will help low-cloud researchers to better understand their mesoscale organizations.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 20, 15681–15724, https://doi.org/10.5194/acp-20-15681-2020, https://doi.org/10.5194/acp-20-15681-2020, 2020
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Particles arising from human activity interact with clouds and affect how much of the Sun's energy is reflected away. Lack of understanding about how to represent this in models leads to large uncertainties in climate predictions. We quantify cloud responses to particles in the latest UK Met Office climate model over the North Atlantic Ocean, showing that, in contrast to suggestions elsewhere, increases in cloud coverage and thickness are important over large areas.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
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In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Hamish Gordon, Paul R. Field, Steven J. Abel, Paul Barrett, Keith Bower, Ian Crawford, Zhiqiang Cui, Daniel P. Grosvenor, Adrian A. Hill, Jonathan Taylor, Jonathan Wilkinson, Huihui Wu, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, https://doi.org/10.5194/acp-20-10997-2020, 2020
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The Met Office's Unified Model is widely used both for weather forecasting and climate prediction. We present the first version of the model in which both aerosol and cloud particle mass and number concentrations are allowed to evolve separately and independently, which is important for studying how aerosols affect weather and climate. We test the model against aircraft observations near Ascension Island in the Atlantic, focusing on how aerosols can "activate" to become cloud droplets.
Leighton A. Regayre, Julia Schmale, Jill S. Johnson, Christian Tatzelt, Andrea Baccarini, Silvia Henning, Masaru Yoshioka, Frank Stratmann, Martin Gysel-Beer, Daniel P. Grosvenor, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10063–10072, https://doi.org/10.5194/acp-20-10063-2020, https://doi.org/10.5194/acp-20-10063-2020, 2020
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The amount of energy reflected back into space because of man-made particles is highly uncertain. Processes related to naturally occurring particles cause most of the uncertainty, but these processes are poorly constrained by present-day measurements. We show that measurements over the Southern Ocean, far from pollution sources, efficiently reduce climate model uncertainties. Our results pave the way to designing experiments and measurement campaigns that reduce this uncertainty even further.
Francesca Gallo, Janek Uin, Stephen Springston, Jian Wang, Guangjie Zheng, Chongai Kuang, Robert Wood, Eduardo B. Azevedo, Allison McComiskey, Fan Mei, Adam Theisen, Jenni Kyrouac, and Allison C. Aiken
Atmos. Chem. Phys., 20, 7553–7573, https://doi.org/10.5194/acp-20-7553-2020, https://doi.org/10.5194/acp-20-7553-2020, 2020
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Continuous high-time-resolution ambient data can include periods when aerosol properties do not represent regional aerosol processes due to high-concentration local events. We develop a novel aerosol mask at the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) facility in the eastern North Atlantic (ENA). We use two ground sites to validate the mask, include a comparison with aircraft overflights, and provide guidance to increase data quality at ENA and other locations.
Daniel T. McCoy, Paul Field, Hamish Gordon, Gregory S. Elsaesser, and Daniel P. Grosvenor
Atmos. Chem. Phys., 20, 4085–4103, https://doi.org/10.5194/acp-20-4085-2020, https://doi.org/10.5194/acp-20-4085-2020, 2020
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Incomplete understanding of how aerosol affects clouds degrades our ability to predict future climate. In particular, it is unclear how aerosol affects the lifetime of clouds. Does it increase or decrease it? This confusion is partially because causality flows from aerosol to clouds and clouds to aerosol, and it is hard to tell what is happening in observations. Here, we use simulations to tell us about how clouds affect aerosol and use this to interpret observations, showing increased lifetime.
Mary Kacarab, K. Lee Thornhill, Amie Dobracki, Steven G. Howell, Joseph R. O'Brien, Steffen Freitag, Michael R. Poellot, Robert Wood, Paquita Zuidema, Jens Redemann, and Athanasios Nenes
Atmos. Chem. Phys., 20, 3029–3040, https://doi.org/10.5194/acp-20-3029-2020, https://doi.org/10.5194/acp-20-3029-2020, 2020
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We find that extensive biomass burning aerosol plumes from southern Africa can profoundly influence clouds in the southeastern Atlantic. Concurrent variations in vertical velocity, however, are found to magnify the relationship between boundary layer aerosol and the cloud droplet number. Neglecting these covariances may strongly bias the sign and magnitude of aerosol impacts on the cloud droplet number.
Sam Pennypacker, Michael Diamond, and Robert Wood
Atmos. Chem. Phys., 20, 2341–2351, https://doi.org/10.5194/acp-20-2341-2020, https://doi.org/10.5194/acp-20-2341-2020, 2020
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Using observations from instruments deployed to a small island in the southeast Atlantic, we study days when the atmospheric concentrations of particles near the surface are exceptionally low. Interestingly, these ultra-clean boundary layers occur in the same months as the smokiest boundary layers associated with biomass burning in Africa. We find evidence that enhancements in drizzle scavenging, on top of a seasonal maximum in cloudiness and precipitation, likely drive these conditions.
Samuel E. LeBlanc, Jens Redemann, Connor Flynn, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal-Rosenheimer, Yohei Shinozuka, Stephen Dunagan, Robert P. Dahlgren, Kerry Meyer, James Podolske, Steven G. Howell, Steffen Freitag, Jennifer Small-Griswold, Brent Holben, Michael Diamond, Robert Wood, Paola Formenti, Stuart Piketh, Gillian Maggs-Kölling, Monja Gerber, and Andreas Namwoonde
Atmos. Chem. Phys., 20, 1565–1590, https://doi.org/10.5194/acp-20-1565-2020, https://doi.org/10.5194/acp-20-1565-2020, 2020
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The southeast Atlantic during August–October experiences layers of smoke from biomass burning over marine stratocumulus clouds. Here we present the light attenuation of the smoke and its dependence in the spatial, vertical, and spectral domain through direct measurements from an airborne platform during September 2016. From our observations of this climatically important smoke, we found an average aerosol optical depth of 0.32 at 500 nm, slightly lower than comparative satellite measurements.
Marc Mallet, Pierre Nabat, Paquita Zuidema, Jens Redemann, Andrew Mark Sayer, Martin Stengel, Sebastian Schmidt, Sabrina Cochrane, Sharon Burton, Richard Ferrare, Kerry Meyer, Pablo Saide, Hiren Jethva, Omar Torres, Robert Wood, David Saint Martin, Romain Roehrig, Christina Hsu, and Paola Formenti
Atmos. Chem. Phys., 19, 4963–4990, https://doi.org/10.5194/acp-19-4963-2019, https://doi.org/10.5194/acp-19-4963-2019, 2019
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The model is able to represent LWP but not the LCF. AOD is consistent over the continent but also over ocean (ACAOD). Differences are observed in SSA due to the absence of internal mixing in ALADIN-Climate. A significant regional gradient of the forcing at TOA is observed. An intense positive forcing is simulated over Gabon. Results highlight the significant effect of enhanced moisture on BBA extinction. The surface dimming modifies the energy budget.
Guangjie Zheng, Yang Wang, Allison C. Aiken, Francesca Gallo, Michael P. Jensen, Pavlos Kollias, Chongai Kuang, Edward Luke, Stephen Springston, Janek Uin, Robert Wood, and Jian Wang
Atmos. Chem. Phys., 18, 17615–17635, https://doi.org/10.5194/acp-18-17615-2018, https://doi.org/10.5194/acp-18-17615-2018, 2018
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Here, we elucidate the key processes that drive marine boundary layer (MBL) aerosol size distribution in the eastern North Atlantic (ENA) using long-term measurements. The governing equations of particle concentration are established for different modes. Particles entrained from the free troposphere represent the major source of MBL cloud condensation nuclei (CCN), contributing both directly to CCN population and indirectly by supplying Aitken-mode particles that grow to CCN in the MBL.
Anna Possner, Hailong Wang, Robert Wood, Ken Caldeira, and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 17475–17488, https://doi.org/10.5194/acp-18-17475-2018, https://doi.org/10.5194/acp-18-17475-2018, 2018
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We quantify aerosol–cloud radiative interactions in a regime of deep open-cell stratocumuli (boundary layer depth 1.5 km), a regime which remains largely unexplored within this context and yet is more dominant than cases of shallow stratocumuli previously studied. We simulate substantial increases in albedo in a regime where ship tracks are not found and argue that such changes may escape detection and attribution through remote sensing due to the large natural variability in the system.
Hamish Gordon, Paul R. Field, Steven J. Abel, Mohit Dalvi, Daniel P. Grosvenor, Adrian A. Hill, Ben T. Johnson, Annette K. Miltenberger, Masaru Yoshioka, and Ken S. Carslaw
Atmos. Chem. Phys., 18, 15261–15289, https://doi.org/10.5194/acp-18-15261-2018, https://doi.org/10.5194/acp-18-15261-2018, 2018
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Smoke from African fires is frequently transported across the Atlantic Ocean, where it interacts with clouds. We simulate the interaction of the smoke with the clouds, and the consequences of this for the solar radiation the clouds reflect. The simulations use a new regional configuration of the UK Met Office climate model. Our simulations indicate that the properties of the clouds, in particular their height and reflectivity, and the fractional cloud cover, are strongly affected by the smoke.
Michael S. Diamond, Amie Dobracki, Steffen Freitag, Jennifer D. Small Griswold, Ashley Heikkila, Steven G. Howell, Mary E. Kacarab, James R. Podolske, Pablo E. Saide, and Robert Wood
Atmos. Chem. Phys., 18, 14623–14636, https://doi.org/10.5194/acp-18-14623-2018, https://doi.org/10.5194/acp-18-14623-2018, 2018
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Smoke from Africa can mix into clouds over the southeast Atlantic and create new droplets, which brightens the clouds, reflects more sunlight, and thus cools the region. Using aircraft data from a NASA field campaign, we find that cloud properties are correlated with smoke as expected when the smoke is below the clouds but not when smoke is above the clouds because it takes several days for clouds to mix smoke downward. We recommend methods that can track clouds as they move for future studies.
Daniel P. Grosvenor, Odran Sourdeval, and Robert Wood
Atmos. Meas. Tech., 11, 4273–4289, https://doi.org/10.5194/amt-11-4273-2018, https://doi.org/10.5194/amt-11-4273-2018, 2018
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We provide a parameterized correction to the retrieval of cloud effective radius from satellite instruments to account for the assumption that the retrieved value is representative of that at cloud top, whereas in reality it is representative of that lower down. The error leads to errors (which we quantify) in the retrieved cloud droplet concentrations of up to 38 % for stratocumulus regions and also to liquid water path errors, both of which can be corrected using our parameterizations.
Daniel T. McCoy, Paul R. Field, Anja Schmidt, Daniel P. Grosvenor, Frida A.-M. Bender, Ben J. Shipway, Adrian A. Hill, Jonathan M. Wilkinson, and Gregory S. Elsaesser
Atmos. Chem. Phys., 18, 5821–5846, https://doi.org/10.5194/acp-18-5821-2018, https://doi.org/10.5194/acp-18-5821-2018, 2018
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Here we use a combination of global convection-permitting models, satellite observations and the Holuhraun volcanic eruption to demonstrate that aerosol enhances the cloud liquid content and brightness of midlatitude cyclones. This is important because the strength of anthropogenic radiative forcing is uncertain, leading to uncertainty in the climate sensitivity consistent with observed temperature record.
Daniel T. McCoy, Frida A.-M. Bender, Daniel P. Grosvenor, Johannes K. Mohrmann, Dennis L. Hartmann, Robert Wood, and Paul R. Field
Atmos. Chem. Phys., 18, 2035–2047, https://doi.org/10.5194/acp-18-2035-2018, https://doi.org/10.5194/acp-18-2035-2018, 2018
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The interaction between clouds and aerosols represents the largest source of uncertainty in the anthropogenic radiative forcing. Cloud droplet number concentration (CDNC) is the state variable that moderates the interaction between aerosol and clouds. Here we show that CDNC decreases off the coasts of East Asia and North America due to controls on emissions. We support this analysis through an examination of volcanism in Hawaii and Vanuatu.
Xiaoli Zhou, Andrew S. Ackerman, Ann M. Fridlind, Robert Wood, and Pavlos Kollias
Atmos. Chem. Phys., 17, 12725–12742, https://doi.org/10.5194/acp-17-12725-2017, https://doi.org/10.5194/acp-17-12725-2017, 2017
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Shallow maritime clouds make a well-known transition from stratocumulus to trade cumulus with flow from the subtropics equatorward. Three-day large-eddy simulations that investigate the potential influence of overlying African biomass burning plumes during that transition indicate that cloud-related impacts are likely substantially cooling to negligible at the top of the atmosphere, with magnitude sensitive to background and perturbation aerosol and cloud properties.
Daniel P. Grosvenor, Paul R. Field, Adrian A. Hill, and Benjamin J. Shipway
Atmos. Chem. Phys., 17, 5155–5183, https://doi.org/10.5194/acp-17-5155-2017, https://doi.org/10.5194/acp-17-5155-2017, 2017
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We used a weather model to simulate low-level layer clouds that lie off the coast of Chile and tested how they would be affected by airborne particulate matter (aerosols) according to the model. We found that as aerosols were increased, the clouds reflected more and more of the sun’s incoming energy due to the combined effects of the cloud droplets becoming smaller, the thickening of clouds, and increased areal coverage. However, the latter two effects were only important at low aerosol levels.
Kuan-Ting O and Robert Wood
Atmos. Chem. Phys., 16, 7239–7249, https://doi.org/10.5194/acp-16-7239-2016, https://doi.org/10.5194/acp-16-7239-2016, 2016
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In this work, based on the well-known formulae of classical nucleation theory (CNT), the temperature at which the mean number of critical embryos inside a droplet is unity is derived from the Boltzmann distribution function and explored as a new simplified approximation for homogeneous freezing temperature. It thus appears that the simplicity of this approximation makes it potentially useful for predicting homogeneous freezing temperatures of water droplets in the atmosphere.
D. P. Grosvenor, J. C. King, T. W. Choularton, and T. Lachlan-Cope
Atmos. Chem. Phys., 14, 9481–9509, https://doi.org/10.5194/acp-14-9481-2014, https://doi.org/10.5194/acp-14-9481-2014, 2014
C. R. Terai, C. S. Bretherton, R. Wood, and G. Painter
Atmos. Chem. Phys., 14, 8071–8088, https://doi.org/10.5194/acp-14-8071-2014, https://doi.org/10.5194/acp-14-8071-2014, 2014
A. Muhlbauer, I. L. McCoy, and R. Wood
Atmos. Chem. Phys., 14, 6695–6716, https://doi.org/10.5194/acp-14-6695-2014, https://doi.org/10.5194/acp-14-6695-2014, 2014
A. H. Berner, C. S. Bretherton, R. Wood, and A. Muhlbauer
Atmos. Chem. Phys., 13, 12549–12572, https://doi.org/10.5194/acp-13-12549-2013, https://doi.org/10.5194/acp-13-12549-2013, 2013
C. R. Terai and R. Wood
Atmos. Chem. Phys., 13, 9899–9914, https://doi.org/10.5194/acp-13-9899-2013, https://doi.org/10.5194/acp-13-9899-2013, 2013
A. Gettelman, H. Morrison, C. R. Terai, and R. Wood
Atmos. Chem. Phys., 13, 9855–9867, https://doi.org/10.5194/acp-13-9855-2013, https://doi.org/10.5194/acp-13-9855-2013, 2013
R. C. George, R. Wood, C. S. Bretherton, and G. Painter
Atmos. Chem. Phys., 13, 6305–6328, https://doi.org/10.5194/acp-13-6305-2013, https://doi.org/10.5194/acp-13-6305-2013, 2013
C. H. Twohy, J. R. Anderson, D. W. Toohey, M. Andrejczuk, A. Adams, M. Lytle, R. C. George, R. Wood, P. Saide, S. Spak, P. Zuidema, and D. Leon
Atmos. Chem. Phys., 13, 2541–2562, https://doi.org/10.5194/acp-13-2541-2013, https://doi.org/10.5194/acp-13-2541-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Impact of weather systems on observed precipitation at Ny-Ålesund (Svalbard)
Analysis of ship emission effects on clouds over the southeastern Atlantic using geostationary satellite observations
Relationship between latent and radiative heating fields of tropical cloud systems using synergistic satellite observations
Shallow cloud variability in Houston, Texas, during the ESCAPE and TRACER field experiments
How does the lifetime of detrained cirrus impact the high-cloud radiative effect in the tropics?
Anvil–radiation diurnal interaction: shortwave radiative-heating destabilization driving the diurnal variation of convective anvil outflow and its modulation on the radiative cancellation
Impact of wildfire smoke on Arctic cirrus formation – Part 1: Analysis of MOSAiC 2019–2020 observations
A new aggregation and riming discrimination algorithm based on polarimetric weather radars
Study of optical scattering properties and direct radiative effects of high-altitude cirrus clouds in Barcelona, Spain, with 4 years of lidar measurements
Co-variability drives the inverted-V sensitivity between liquid water path and droplet concentrations
Life cycle studies and liquid-phase characterization of Arctic mixed-phase clouds: MOSAiC 2019–2020 results
Lightning declines over shipping lanes following regulation of fuel sulfur emissions
Post-return stroke VHF electromagnetic activity in north-western Mediterranean cloud-to-ground lightning flashes
A machine learning-based perspective on deep convective clouds and their organisation in 3D. Part I: Influence of deep convective cores on the cloud life-cycle
A machine learning-based perspective on deep convective clouds and their organisation in 3D. Part II: Spatial-temporal patterns of convective organisation
Technical note: Applicability of physics-based and machine-learning-based algorithms of a geostationary satellite in retrieving the diurnal cycle of cloud base height
Observing convective activities in complex convective organizations and their contributions to precipitation and anvil cloud amounts
Weak liquid water path response in ship tracks
Air mass history linked to the development of Arctic mixed-phase clouds
Distinct structure, radiative effects, and precipitation characteristics of deep convection systems in the Tibetan Plateau compared to the tropical Indian Ocean
The correlation between Arctic sea ice, cloud phase and radiation using A-Train satellites
Technical note: Retrieval of the supercooled liquid fraction in mixed-phase clouds from Himawari-8 observations
Characterisation of low-base and mid-base clouds and their thermodynamic phase over the Southern Ocean and Arctic marine regions
A survey of radiative and physical properties of North Atlantic mesoscale cloud morphologies from multiple identification methodologies
Extensive coverage of ultrathin tropical tropopause layer cirrus clouds revealed by balloon-borne lidar observations
The effects of warm-air intrusions in the high Arctic on cirrus clouds
The characteristics of cloud macro-parameters caused by the seeder–feeder process inside clouds measured by millimeter-wave cloud radar in Xi'an, China
Shallow- and deep-convection characteristics in the greater Houston, Texas, area using cell tracking methodology
Observations of the macrophysical properties of cumulus cloud fields over the tropical western Pacific and their connection to meteorological variables
A Lagrangian perspective on the lifecycle and cloud radiative effect of deep convective clouds over Africa
Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic
Technical note: Bimodal parameterizations of in situ ice cloud particle size distributions
Inter-relations of precipitation, aerosols, and clouds over Andalusia, southern Spain, revealed by the Andalusian Global ObseRvatory of the Atmosphere (AGORA)
On the relationship between mesoscale cellular convection and meteorological forcing: comparing the Southern Ocean against the North Pacific
Aerosol-related effects on the occurrence of heterogeneous ice formation over Lauder, New Zealand ∕ Aotearoa
Low-level Arctic clouds: a blind zone in our knowledge of the radiation budget
Climatologically invariant scale invariance seen in distributions of cloud horizontal sizes
Variability and properties of liquid-dominated clouds over the ice-free and sea-ice-covered Arctic Ocean
Asymmetries in cloud microphysical properties ascribed to sea ice leads via water vapour transport in the central Arctic
Quantifying the dependence of drop spectrum width on cloud drop number concentration for cloud remote sensing
The evolution of deep convective systems and their associated cirrus outflows
Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean
Rapid saturation of cloud water adjustments to shipping emissions
Sensitivities of cloud radiative effects to large-scale meteorology and aerosols from global observations
Distinct secondary ice production processes observed in radar Doppler spectra: insights from a case study
Investigating the development of clouds within marine cold-air outbreaks
Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations
Examining cloud vertical structure and radiative effects from satellite retrievals and evaluation of CMIP6 scenarios
Influence of cloud microphysics schemes on weather model predictions of heavy precipitation
Convective organization and 3D structure of tropical cloud systems deduced from synergistic A-Train observations and machine learning
Kerstin Ebell, Christian Buhren, Rosa Gierens, Giovanni Chellini, Melanie Lauer, Andreas Walbröl, Sandro Dahlke, Pavel Krobot, and Mario Mech
Atmos. Chem. Phys., 25, 7315–7342, https://doi.org/10.5194/acp-25-7315-2025, https://doi.org/10.5194/acp-25-7315-2025, 2025
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Ground-based observations of precipitation are rare in the Arctic. Since 2017, additional temporally highly resolved precipitation measurements have been carried out by a precipitation gauge and an optical precipitation sensor at Ny-Ålesund, Svalbard. These new data facilitate the distinction between liquid and solid precipitation. Using reanalysis data, we also find that water vapor transport contributes strongly to precipitation and especially to extreme precipitation events.
Nikos Benas, Jan Fokke Meirink, Rob Roebeling, and Martin Stengel
Atmos. Chem. Phys., 25, 6957–6973, https://doi.org/10.5194/acp-25-6957-2025, https://doi.org/10.5194/acp-25-6957-2025, 2025
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This study examines how ship emissions affect clouds over a shipping corridor in the southeastern Atlantic. Using satellite data from 2004 to 2023, we find that ship emissions increase the number of cloud droplets while reducing their size and slightly decrease cloud water content. Effects on seasonal and daily patterns vary based on regional factors. The impact of emissions weakened after stricter regulations were implemented in 2020.
Xiaoting Chen, Claudia J. Stubenrauch, and Giulio Mandorli
Atmos. Chem. Phys., 25, 6857–6880, https://doi.org/10.5194/acp-25-6857-2025, https://doi.org/10.5194/acp-25-6857-2025, 2025
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Strongly precipitating mesoscale convective systems produce a large amount of diabatic heating of the atmosphere, influencing atmospheric circulation. Their complete 3D description, attained by machine learning techniques in combination with satellite observations, has enabled a detailed study of the relationship between latent and radiative heating in these cloud systems. Convective organization increases both the average and the vertical gradient of radiative effects of the mesoscale convective systems.
Zackary Mages, Pavlos Kollias, Bernat Puigdomènech Treserras, Paloma Borque, and Mariko Oue
Atmos. Chem. Phys., 25, 6025–6045, https://doi.org/10.5194/acp-25-6025-2025, https://doi.org/10.5194/acp-25-6025-2025, 2025
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Convective clouds are a key component of the climate system. Using remote sensing observations during two field experiments in Houston, Texas, we identify four diurnal patterns of shallow convective clouds. We find areas more frequently experiencing shallow convective clouds, and we find areas where the vertical extent of shallow convective clouds is higher and where they are more likely to precipitate. This provides insight into the complicated environment that forms these clouds in Houston.
George Horner and Edward Gryspeerdt
Atmos. Chem. Phys., 25, 5617–5631, https://doi.org/10.5194/acp-25-5617-2025, https://doi.org/10.5194/acp-25-5617-2025, 2025
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This work tracks the life cycle of thin cirrus clouds that flow out of tropical convective storms. These cirrus clouds are found to have a warming effect on the atmosphere over their whole lifetime. Thin cirrus that originate from land origin convection warm more than those of ocean origin. Moreover, if the lifetime of these cirrus clouds increase, the warming they exert over their whole lifetime also increases. These results help us understand how these clouds might change in a future climate.
Zhenquan Wang
Atmos. Chem. Phys., 25, 5021–5039, https://doi.org/10.5194/acp-25-5021-2025, https://doi.org/10.5194/acp-25-5021-2025, 2025
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Convective anvil outflow directly driven by the shortwave radiative-heating destabilization is strong during the daytime, whereas the outflow contributed by the longwave radiative cooling through radiative destabilization and circulation is weak. This leads to the diurnal variation in the convection-producing anvil clouds, which in turn can influence the radiative energy budget.
Albert Ansmann, Cristofer Jimenez, Johanna Roschke, Johannes Bühl, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Daniel A. Knopf, Sandro Dahlke, Tom Gaudek, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 25, 4847–4866, https://doi.org/10.5194/acp-25-4847-2025, https://doi.org/10.5194/acp-25-4847-2025, 2025
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In this study, we focus on the potential impact of wildfire smoke on cirrus formation. For the first time, state-of-the-art aerosol and cirrus observations with lidar and radar, presented in this paper (Part 1 of a series of two articles), are closely linked to the comprehensive modeling of gravity-wave-induced ice nucleation in cirrus evolution processes, presented in a companion paper (Part 2). We found a clear impact of wildfire smoke on cirrus evolution.
Armin Blanke, Mathias Gergely, and Silke Trömel
Atmos. Chem. Phys., 25, 4167–4184, https://doi.org/10.5194/acp-25-4167-2025, https://doi.org/10.5194/acp-25-4167-2025, 2025
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The area-wide radar-based distinction between riming and aggregation is crucial for model microphysics and data assimilation. This study introduces a discrimination algorithm based on polarimetric radar networks only. Exploiting the unique opportunity to link fall velocities from Doppler spectra to polarimetric variables in an operational setting enables us to set up and evaluate a well-performing machine learning algorithm.
Cristina Gil-Díaz, Michäel Sicard, Odran Sourdeval, Athulya Saiprakash, Constantino Muñoz-Porcar, Adolfo Comerón, Alejandro Rodríguez-Gómez, and Daniel Camilo Fortunato dos Santos Oliveira
Atmos. Chem. Phys., 25, 3445–3464, https://doi.org/10.5194/acp-25-3445-2025, https://doi.org/10.5194/acp-25-3445-2025, 2025
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This study presents a comprehensive analysis of optical scattering properties and direct radiative effects of cirrus clouds based on 4 years of continuous ground-based lidar measurements with the Barcelona MPLNET lidar. A novel approach of the self-consistent scattering model for cirrus clouds is presented to determine their optical scattering properties at different wavelengths, and their direct radiative effects are calculated with the discrete ordinates method embedded in the ARTDECO package.
Tom Goren, Goutam Choudhury, Jan Kretzschmar, and Isabel McCoy
Atmos. Chem. Phys., 25, 3413–3423, https://doi.org/10.5194/acp-25-3413-2025, https://doi.org/10.5194/acp-25-3413-2025, 2025
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Many studies have identified an inverted-V relationship between the liquid water path (LWP) and droplet concentration (Nd), where LWP increases and then decreases with Nd. Using satellite observations and meteorological data, we demonstrate that the inverted V primarily reflects co-variability between LWP and Nd. We suggest taking a holistic approach that considers this co-variability when assessing the climatological sensitivity of LWP to anthropogenic aerosols.
Cristofer Jimenez, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Ronny Engelmann, Martin Radenz, Julian Hofer, Dietrich Althausen, Daniel Alexander Knopf, Sandro Dahlke, Johannes Bühl, Holger Baars, Patric Seifert, and Ulla Wandinger
EGUsphere, https://doi.org/10.5194/egusphere-2025-967, https://doi.org/10.5194/egusphere-2025-967, 2025
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Using advanced remote sensing on the icebreaker Polarstern, we studied mixed-phase clouds (MPCs) in the central Arctic during the 2019–2020 MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) campaign. For the first time, lidar and radar techniques tracked the year-round evolution of liquid and ice phases in MPCs. The study provides cloud statistics and explores key processes driving cloud longevity, offering new insights into Arctic cloud formation and persistence.
Chris J. Wright, Joel A. Thornton, Lyatt Jaeglé, Yang Cao, Yannian Zhu, Jihu Liu, Randall Jones II, Robert Holzworth, Daniel Rosenfeld, Robert Wood, Peter Blossey, and Daehyun Kim
Atmos. Chem. Phys., 25, 2937–2946, https://doi.org/10.5194/acp-25-2937-2025, https://doi.org/10.5194/acp-25-2937-2025, 2025
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Aerosol particles influence clouds, which exert a large forcing on solar radiation and freshwater. To better understand the mechanisms by which aerosol influences thunderstorms, we look at the two busiest shipping lanes in the world, where recent regulations have reduced sulfur emissions by nearly an order of magnitude. We find that the reduction in emissions has been accompanied by a dramatic decrease in both lightning and the number of droplets in clouds over the shipping lanes.
Andrea Kolínská, Ivana Kolmašová, Eric Defer, Ondřej Santolík, and Stéphane Pédeboy
Atmos. Chem. Phys., 25, 1791–1803, https://doi.org/10.5194/acp-25-1791-2025, https://doi.org/10.5194/acp-25-1791-2025, 2025
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We contribute to understanding differences in lightning flashes of opposite polarity by explaining distinct in-cloud processes after return strokes. Using data from multiple sensors, including individual Lightning Mapping Array stations, we reveal that positive flashes sustain strong high-frequency radiation due to the recharging of their in-cloud leader; this is in contrast to negative flashes, for which this activity declines rapidly.
Sarah Brüning and Holger Tost
EGUsphere, https://doi.org/10.5194/egusphere-2025-374, https://doi.org/10.5194/egusphere-2025-374, 2025
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This study analyses the temporal variability and life-cycle of spatially organised convective clouds, frequently associated with severe weather. We derive the data from a machine learning-based 3D extrapolation of 2D satellite data. The results highlight the impact of convective organisation on horizontal and vertical cloud properties and a prolonged cloud life-cycle. Overall, our findings emphasise a more intense activity over land but enhanced seasonal changes over the ocean.
Sarah Brüning and Holger Tost
EGUsphere, https://doi.org/10.5194/egusphere-2025-376, https://doi.org/10.5194/egusphere-2025-376, 2025
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The connection between convective cloud organisation and severe weather demands a robust characterisation of hazardous clouds. This study sets on to investigate spatio-temporal patterns and regional hotspots of convective organisation using machine learning-based 3D data and combining different organisation indices. While limitations arise due to overlapping effects of isolated and clustered convection, we emphasise the impact of a surface-specific seasonality that depends on the hemisphere.
Mengyuan Wang, Min Min, Jun Li, Han Lin, Yongen Liang, Binlong Chen, Zhigang Yao, Na Xu, and Miao Zhang
Atmos. Chem. Phys., 24, 14239–14256, https://doi.org/10.5194/acp-24-14239-2024, https://doi.org/10.5194/acp-24-14239-2024, 2024
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Although machine learning technology is advanced in the field of satellite remote sensing, the physical inversion algorithm based on cloud base height can better capture the daily variation in the characteristics of the cloud base.
Zhenquan Wang and Jian Yuan
Atmos. Chem. Phys., 24, 13811–13831, https://doi.org/10.5194/acp-24-13811-2024, https://doi.org/10.5194/acp-24-13811-2024, 2024
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Tropical convection organizations are normally connected complexes of many convective activities. In this work, a novel variable-brightness-temperature segment tracking algorithm is established to partition the complex convective organizations into structural components of single cold cores for tracking separately. The duration, precipitation and anvil amount of the tracked organization segments have strong loglinear relationships with brightness temperature structures.
Anna Tippett, Edward Gryspeerdt, Peter Manshausen, Philip Stier, and Tristan W. P. Smith
Atmos. Chem. Phys., 24, 13269–13283, https://doi.org/10.5194/acp-24-13269-2024, https://doi.org/10.5194/acp-24-13269-2024, 2024
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Ship emissions can form artificially brightened clouds, known as ship tracks, and provide us with an opportunity to investigate how aerosols interact with clouds. Previous studies that used ship tracks suggest that clouds can experience large increases in the amount of water (LWP) from aerosols. Here, we show that there is a bias in previous research and that, when we account for this bias, the LWP response to aerosols is much weaker than previously reported.
Rebecca J. Murray-Watson and Edward Gryspeerdt
Atmos. Chem. Phys., 24, 11115–11132, https://doi.org/10.5194/acp-24-11115-2024, https://doi.org/10.5194/acp-24-11115-2024, 2024
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The formation of mixed-phase clouds during marine cold-air outbreaks is not well understood. Our study, using satellite data and Lagrangian trajectories, reveals that the occurrence of these clouds depends on both time and temperature, influenced partly by the presence of biological ice-nucleating particles. This highlights the importance of comprehending local aerosol dynamics for precise modelling of cloud-phase transitions in the Arctic.
Yuxin Zhao, Jiming Li, Deyu Wen, Yarong Li, Yuan Wang, and Jianping Huang
Atmos. Chem. Phys., 24, 9435–9457, https://doi.org/10.5194/acp-24-9435-2024, https://doi.org/10.5194/acp-24-9435-2024, 2024
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This study identifies deep convection systems (DCSs), including deep convection cores and anvils, over the Tibetan Plateau (TP) and tropical Indian Ocean (TO). The DCSs over the TP are less frequent, showing narrower and thinner cores and anvils compared to those over the TO. TP DCSs show a stronger longwave cloud radiative effect at the surface and in the low-level atmosphere. Distinct aerosol–cloud–precipitation interaction is found in TP DCSs, probably due to the cold cloud bases.
Grégory V. Cesana, Olivia Pierpaoli, Matteo Ottaviani, Linh Vu, Zhonghai Jin, and Israel Silber
Atmos. Chem. Phys., 24, 7899–7909, https://doi.org/10.5194/acp-24-7899-2024, https://doi.org/10.5194/acp-24-7899-2024, 2024
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Better characterizing the relationship between sea ice and clouds is key to understanding Arctic climate because clouds and sea ice affect surface radiation and modulate Arctic surface warming. Our results indicate that Arctic liquid clouds robustly increase in response to sea ice decrease. This increase has a cooling effect on the surface because more solar radiation is reflected back to space, and it should contribute to dampening future Arctic surface warming.
Ziming Wang, Husi Letu, Huazhe Shang, and Luca Bugliaro
Atmos. Chem. Phys., 24, 7559–7574, https://doi.org/10.5194/acp-24-7559-2024, https://doi.org/10.5194/acp-24-7559-2024, 2024
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The supercooled liquid fraction (SLF) in mixed-phase clouds is retrieved for the first time using passive geostationary satellite observations based on differences in liquid droplet and ice particle radiative properties. The retrieved results are comparable to global distributions observed by active instruments, and the feasibility of the retrieval method to analyze the observed trends of the SLF has been validated.
Barbara Dietel, Odran Sourdeval, and Corinna Hoose
Atmos. Chem. Phys., 24, 7359–7383, https://doi.org/10.5194/acp-24-7359-2024, https://doi.org/10.5194/acp-24-7359-2024, 2024
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Uncertainty with respect to cloud phases over the Southern Ocean and Arctic marine regions leads to large uncertainties in the radiation budget of weather and climate models. This study investigates the phases of low-base and mid-base clouds using satellite-based remote sensing data. A comprehensive analysis of the correlation of cloud phase with various parameters, such as temperature, aerosols, sea ice, vertical and horizontal cloud extent, and cloud radiative effect, is presented.
Ryan Eastman, Isabel L. McCoy, Hauke Schulz, and Robert Wood
Atmos. Chem. Phys., 24, 6613–6634, https://doi.org/10.5194/acp-24-6613-2024, https://doi.org/10.5194/acp-24-6613-2024, 2024
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for 1 year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is, in part, a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds' radiative effect. Future studies must account for differing properties and processes among cloud types.
Thomas Lesigne, François Ravetta, Aurélien Podglajen, Vincent Mariage, and Jacques Pelon
Atmos. Chem. Phys., 24, 5935–5952, https://doi.org/10.5194/acp-24-5935-2024, https://doi.org/10.5194/acp-24-5935-2024, 2024
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Upper tropical clouds have a strong impact on Earth's climate but are challenging to observe. We report the first long-duration observations of tropical clouds from lidars flying on board stratospheric balloons. Comparisons with spaceborne observations reveal the enhanced sensitivity of balloon-borne lidar to optically thin cirrus. These clouds, which have a significant coverage and lie in the uppermost troposphere, are linked with the dehydration of air masses on their way to the stratosphere.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
Atmos. Chem. Phys., 24, 5971–5987, https://doi.org/10.5194/acp-24-5971-2024, https://doi.org/10.5194/acp-24-5971-2024, 2024
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For decades the earth's temperature has been rising. The Arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm-air intrusions, air masses are transported into the Arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Huige Di and Yun Yuan
Atmos. Chem. Phys., 24, 5783–5801, https://doi.org/10.5194/acp-24-5783-2024, https://doi.org/10.5194/acp-24-5783-2024, 2024
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We observed the seeder–feeder process among double-layer clouds using a cloud radar and microwave radiometer. By defining the parameters of the seeding depth and seeding time of the upper cloud affecting the lower cloud, we find that the cloud particle terminal velocity is significantly enhanced during the seeder–feeder period, and the lower the height and thinner the thickness of the height difference between double-layer clouds, the lower the height and thicker the thickness of seeding depth.
Kristofer S. Tuftedal, Bernat Puigdomènech Treserras, Mariko Oue, and Pavlos Kollias
Atmos. Chem. Phys., 24, 5637–5657, https://doi.org/10.5194/acp-24-5637-2024, https://doi.org/10.5194/acp-24-5637-2024, 2024
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This study analyzed coastal convective cells from June through September 2018–2021. The cells were classified and their lifecycles were analyzed to better understand their characteristics. Features such as convective-core growth, for example, are shown. The study found differences in the initiation location of shallow convection and in the aerosol loading in deep convective environments. This work provides a foundation for future analyses of convection or other tracked events elsewhere.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
William K. Jones, Martin Stengel, and Philip Stier
Atmos. Chem. Phys., 24, 5165–5180, https://doi.org/10.5194/acp-24-5165-2024, https://doi.org/10.5194/acp-24-5165-2024, 2024
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Storm clouds cover large areas of the tropics. These clouds both reflect incoming sunlight and trap heat from the atmosphere below, regulating the temperature of the tropics. Over land, storm clouds occur in the late afternoon and evening and so exist both during the daytime and at night. Changes in this timing could upset the balance of the respective cooling and heating effects of these clouds. We find that isolated storms have a larger effect on this balance than their small size suggests.
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
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The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Irene Bartolomé García, Odran Sourdeval, Reinhold Spang, and Martina Krämer
Atmos. Chem. Phys., 24, 1699–1716, https://doi.org/10.5194/acp-24-1699-2024, https://doi.org/10.5194/acp-24-1699-2024, 2024
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How many ice crystals of each size are in a cloud is a key parameter for the retrieval of cloud properties. The distribution of ice crystals is obtained from in situ measurements and used to create parameterizations that can be used when analyzing the remote-sensing data. Current parameterizations are based on data sets that do not include reliable measurements of small crystals, but in our study we use a data set that includes very small ice crystals to improve these parameterizations.
Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, Lucas Alados-Arboledas, Agustín Millares, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 24, 1571–1585, https://doi.org/10.5194/acp-24-1571-2024, https://doi.org/10.5194/acp-24-1571-2024, 2024
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The south-central interior of Andalusia experiences complex precipitation patterns as a result of the semi-arid Mediterranean climate and the influence of Saharan dust. This study monitored the inter-relations between aerosols, clouds, meteorological variables, and precipitation systems using ground-based remote sensing and in situ instruments.
Francisco Lang, Steven T. Siems, Yi Huang, Tahereh Alinejadtabrizi, and Luis Ackermann
Atmos. Chem. Phys., 24, 1451–1466, https://doi.org/10.5194/acp-24-1451-2024, https://doi.org/10.5194/acp-24-1451-2024, 2024
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Marine low-level clouds play a crucial role in the Earth's energy balance, trapping heat from the surface and reflecting sunlight back into space. These clouds are distinguishable by their large-scale spatial structures, primarily characterized as hexagonal patterns with either filled (closed) or empty (open) cells. Utilizing satellite observations, these two cloud type patterns have been categorized over the Southern Ocean and North Pacific Ocean through a pattern recognition program.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
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An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Hannes Jascha Griesche, Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 24, 597–612, https://doi.org/10.5194/acp-24-597-2024, https://doi.org/10.5194/acp-24-597-2024, 2024
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The Arctic is strongly affected by climate change and the role of clouds therein is not yet completely understood. Measurements from the Arctic expedition PS106 were used to simulate radiative fluxes with and without clouds at very low altitudes (below 165 m), and their radiative effect was calculated to be 54 Wm-2. The low heights of these clouds make them hard to observe. This study shows the importance of accurate measurements and simulations of clouds and gives suggestions for improvements.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Viewed from space, a defining feature of Earth's atmosphere is the wide spectrum of cloud sizes. A recent study predicted the distribution of cloud sizes, and this paper compares the prediction to observations. Although there is nuance in viewing perspective, we find robust agreement with theory across different climatological conditions, including land–ocean contrasts, time of year, or latitude, suggesting a minor role for Coriolis forces, aerosol loading, or surface temperature.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Pablo Saavedra Garfias, Heike Kalesse-Los, Luisa von Albedyll, Hannes Griesche, and Gunnar Spreen
Atmos. Chem. Phys., 23, 14521–14546, https://doi.org/10.5194/acp-23-14521-2023, https://doi.org/10.5194/acp-23-14521-2023, 2023
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An important Arctic climate process is the release of heat fluxes from sea ice openings to the atmosphere that influence the clouds. The characterization of this process is the objective of this study. Using synergistic observations from the MOSAiC expedition, we found that single-layer cloud properties show significant differences when clouds are coupled or decoupled to the water vapour transport which is used as physical link between the upwind sea ice openings and the cloud under observation.
Matthew D. Lebsock and Mikael Witte
Atmos. Chem. Phys., 23, 14293–14305, https://doi.org/10.5194/acp-23-14293-2023, https://doi.org/10.5194/acp-23-14293-2023, 2023
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This paper evaluates measurements of cloud drop size distributions made from airplanes. We find that as the number of cloud drops increases the distribution of the cloud drop sizes narrows. The data are used to develop a simple equation that relates the drop number to the width of the drop sizes. We then use this equation to demonstrate that existing approaches to observe the drop number from satellites contain errors that can be corrected by including the new relationship.
George Horner and Edward Gryspeerdt
Atmos. Chem. Phys., 23, 14239–14253, https://doi.org/10.5194/acp-23-14239-2023, https://doi.org/10.5194/acp-23-14239-2023, 2023
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Tropical deep convective clouds, and the thin cirrus (ice) clouds that flow out from them, are important for modulating the energy budget of the tropical atmosphere. This work uses a new method to track the evolution of the properties of these clouds across their entire lifetimes. We find these clouds cool the atmosphere in the first 6 h before switching to a warming regime after the deep convective core has dissipated, which is sustained beyond 120 h from the initial convective event.
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
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For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
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Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
Hendrik Andersen, Jan Cermak, Alyson Douglas, Timothy A. Myers, Peer Nowack, Philip Stier, Casey J. Wall, and Sarah Wilson Kemsley
Atmos. Chem. Phys., 23, 10775–10794, https://doi.org/10.5194/acp-23-10775-2023, https://doi.org/10.5194/acp-23-10775-2023, 2023
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This study uses an observation-based cloud-controlling factor framework to study near-global sensitivities of cloud radiative effects to a large number of meteorological and aerosol controls. We present near-global sensitivity patterns to selected thermodynamic, dynamic, and aerosol factors and discuss the physical mechanisms underlying the derived sensitivities. Our study hopes to guide future analyses aimed at constraining cloud feedbacks and aerosol–cloud interactions.
Anne-Claire Billault-Roux, Paraskevi Georgakaki, Josué Gehring, Louis Jaffeux, Alfons Schwarzenboeck, Pierre Coutris, Athanasios Nenes, and Alexis Berne
Atmos. Chem. Phys., 23, 10207–10234, https://doi.org/10.5194/acp-23-10207-2023, https://doi.org/10.5194/acp-23-10207-2023, 2023
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Secondary ice production plays a key role in clouds and precipitation. In this study, we analyze radar measurements from a snowfall event in the Jura Mountains. Complex signatures are observed, which reveal that ice crystals were formed through various processes. An analysis of multi-sensor data suggests that distinct ice multiplication processes were taking place. Both the methods used and the insights gained through this case study contribute to a better understanding of snowfall microphysics.
Rebecca J. Murray-Watson, Edward Gryspeerdt, and Tom Goren
Atmos. Chem. Phys., 23, 9365–9383, https://doi.org/10.5194/acp-23-9365-2023, https://doi.org/10.5194/acp-23-9365-2023, 2023
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Clouds formed in Arctic marine cold air outbreaks undergo a distinct evolution, but the factors controlling their transition from high-coverage to broken cloud fields are poorly understood. We use satellite and reanalysis data to study how these clouds develop in time and the different influences on their evolution. The aerosol concentration is correlated with cloud break-up; more aerosol is linked to prolonged coverage and a stronger cooling effect, with implications for a more polluted Arctic.
Michael S. Diamond
Atmos. Chem. Phys., 23, 8259–8269, https://doi.org/10.5194/acp-23-8259-2023, https://doi.org/10.5194/acp-23-8259-2023, 2023
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Fuel sulfur regulations were implemented for ships in 2020 to improve air quality but may also accelerate global warming. We use spatial statistics and satellite retrievals to detect changes in the size of cloud droplets and find evidence for a resulting decrease in cloud brightness within a major shipping corridor after the sulfur limits went into effect. Our results confirm both that the regulations are being followed and that they are having a warming influence via their effect on clouds.
Hao Luo, Johannes Quaas, and Yong Han
Atmos. Chem. Phys., 23, 8169–8186, https://doi.org/10.5194/acp-23-8169-2023, https://doi.org/10.5194/acp-23-8169-2023, 2023
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Clouds exhibit a wide range of vertical structures with varying microphysical and radiative properties. We show a global survey of spatial distribution, vertical extent and radiative effect of various classified cloud vertical structures using joint satellite observations from the new CCCM datasets during 2007–2010. Moreover, the long-term trends in CVSs are investigated based on different CMIP6 future scenarios to capture the cloud variations with different, increasing anthropogenic forcings.
Gregor Köcher, Tobias Zinner, and Christoph Knote
Atmos. Chem. Phys., 23, 6255–6269, https://doi.org/10.5194/acp-23-6255-2023, https://doi.org/10.5194/acp-23-6255-2023, 2023
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Polarimetric radar observations of 30 d of convective precipitation events are used to statistically analyze 5 state-of-the-art microphysics schemes of varying complexity. The frequency and area of simulated heavy-precipitation events are in some cases significantly different from those observed, depending on the microphysics scheme. Analysis of simulated particle size distributions and reflectivities shows that some schemes have problems reproducing the correct particle size distributions.
Claudia J. Stubenrauch, Giulio Mandorli, and Elisabeth Lemaitre
Atmos. Chem. Phys., 23, 5867–5884, https://doi.org/10.5194/acp-23-5867-2023, https://doi.org/10.5194/acp-23-5867-2023, 2023
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Organized convection leads to large convective cloud systems and intense rain and may change with a warming climate. Their complete 3D description, attained by machine learning techniques in combination with various satellite observations, together with a cloud system concept, link convection to anvil properties, while convective organization can be identified by the horizontal structure of intense rain.
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