Articles | Volume 13, issue 18
https://doi.org/10.5194/acp-13-9379-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-9379-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
24 Sep 2013
Research article |
| 24 Sep 2013
Cloud and boundary layer interactions over the Arctic sea ice in late summer
M. D. Shupe
Cooperative Institute for Research in Environmental Sciences, University of Colorado and NOAA-Earth System Research Laboratory, Boulder, CO, USA
P. O. G. Persson
Cooperative Institute for Research in Environmental Sciences, University of Colorado and NOAA-Earth System Research Laboratory, Boulder, CO, USA
I. M. Brooks
Institute for Climate and Atmospheric Science, University of Leeds, Leeds, UK
M. Tjernström
Department of Meteorology and the Bert Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden
J. Sedlar
Swedish Meteorological and Hydrological Institute, Norrköping, Sweden
T. Mauritsen
Max Plank Institute for Meteorology, Hamburg, Germany
S. Sjogren
Department of Physics, Lund University, Lund, Sweden
C. Leck
Department of Meteorology and the Bert Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden
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Assia Arouf, Hélène Chepfer, Thibault Vaillant de Guélis, Marjolaine Chiriaco, Matthew D. Shupe, Rodrigo Guzman, Artem Feofilov, Patrick Raberanto, Tristan S. L'Ecuyer, Seiji Kato, and Michael R. Gallagher
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Ralf Bennartz, Frank Fell, Claire Pettersen, Matthew D. Shupe, and Dirk Schuettemeyer
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Christopher J. Cox, David C. Noone, Max Berkelhammer, Matthew D. Shupe, William D. Neff, Nathaniel B. Miller, Von P. Walden, and Konrad Steffen
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Amy Solomon, Gijs de Boer, Jessie M. Creamean, Allison McComiskey, Matthew D. Shupe, Maximilian Maahn, and Christopher Cox
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The results of this study indicate that perturbations in ice nucleating particles (INPs) dominate over cloud condensation nuclei (CCN) perturbations in Arctic mixed-phase stratocumulus; i.e., an equivalent fractional decrease in CCN and INPs results in an increase in the cloud-top longwave cooling rate, even though the droplet effective radius increases and the cloud emissivity decreases. In addition, cloud-processing causes layering of aerosols with increased concentrations of CCN at cloud top.
Matthew S. Norgren, Gijs de Boer, and Matthew D. Shupe
Atmos. Chem. Phys., 18, 13345–13361, https://doi.org/10.5194/acp-18-13345-2018, https://doi.org/10.5194/acp-18-13345-2018, 2018
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Arctic mixed-phase clouds are a critical component of the Arctic climate system because of their ability to influence the surface radiation budget. The radiative impact of an individual cloud is closely linked to the ability of the cloud to convert liquid drops to ice. In this paper, we show through an observational record that clouds present in polluted atmospheric conditions have lower amounts of ice than similar clouds found in clean conditions.
Claire Pettersen, Ralf Bennartz, Aronne J. Merrelli, Matthew D. Shupe, David D. Turner, and Von P. Walden
Atmos. Chem. Phys., 18, 4715–4735, https://doi.org/10.5194/acp-18-4715-2018, https://doi.org/10.5194/acp-18-4715-2018, 2018
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A novel method for classifying Arctic precipitation using ground based remote sensors is presented. The classification reveals two distinct, primary regimes of precipitation over the central Greenland Ice Sheet: snowfall coupled to deep, fully glaciated ice clouds or to shallow, mixed-phase clouds. The ice clouds are associated with low-pressure storm systems from the southeast, while the mixed-phase clouds slowly propagate from the southwest along a quiescent flow.
Robert A. Stillwell, Ryan R. Neely III, Jeffrey P. Thayer, Matthew D. Shupe, and David D. Turner
Atmos. Meas. Tech., 11, 835–859, https://doi.org/10.5194/amt-11-835-2018, https://doi.org/10.5194/amt-11-835-2018, 2018
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Yinghui Liu, Matthew D. Shupe, Zhien Wang, and Gerald Mace
Atmos. Chem. Phys., 17, 5973–5989, https://doi.org/10.5194/acp-17-5973-2017, https://doi.org/10.5194/acp-17-5973-2017, 2017
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Detailed and accurate vertical distributions of cloud properties are essential to accurately calculate the surface radiative flux and to depict the mean climate state, and such information is more desirable in the Arctic due to its recent rapid changes and the challenging observation conditions. This study presents a feasible way to provide such information by blending cloud observations from surface and space-based instruments with the understanding of their respective strength and limitations.
Nathaniel B. Miller, Matthew D. Shupe, Christopher J. Cox, David Noone, P. Ola G. Persson, and Konrad Steffen
The Cryosphere, 11, 497–516, https://doi.org/10.5194/tc-11-497-2017, https://doi.org/10.5194/tc-11-497-2017, 2017
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A comprehensive observational dataset is assembled to investigate atmosphere–Greenland ice sheet interactions and characterize surface temperature variability. The amount the surface temperature warms, due to increases in cloud presence and/or elevated sun angle, varies throughout the annual cycle and is modulated by the responses of latent, sensible and ground heat fluxes. This observationally based study provides process-based relationships, which are useful for evaluation of climate models.
Robert A. Stillwell, Ryan R. Neely III, Jeffrey P. Thayer, Matthew D. Shupe, and Michael O'Neill
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-303, https://doi.org/10.5194/amt-2016-303, 2016
Revised manuscript not accepted
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This work explores the observation of Arctic mixed phase clouds by lidar and the consequences of mishandling lidar signals linking the signals to their geophysical interpretation. It concludes 3 points: 1) cloud phase identification is not only linked to cloud phase but other cloud properties, 2) having more than two polarization signals can be used to quality control data not possible with only two signals, and 3) phase retrievals with more than two polarizations enhance retrieval flexibility.
Claire Pettersen, Ralf Bennartz, Mark S. Kulie, Aronne J. Merrelli, Matthew D. Shupe, and David D. Turner
Atmos. Chem. Phys., 16, 4743–4756, https://doi.org/10.5194/acp-16-4743-2016, https://doi.org/10.5194/acp-16-4743-2016, 2016
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We examined four summers of data from a ground-based atmospheric science instrument suite at Summit Station, Greenland, to isolate the signature of the ice precipitation. By using a combination of instruments with different specialities, we identified a passive microwave signature of the ice precipitation. This ice signature compares well to models using synthetic data characteristic of the site.
A. Solomon, G. Feingold, and M. D. Shupe
Atmos. Chem. Phys., 15, 10631–10643, https://doi.org/10.5194/acp-15-10631-2015, https://doi.org/10.5194/acp-15-10631-2015, 2015
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The maintenance of cloud ice production in Arctic mixed-phase stratocumulus is investigated in large eddy simulations that include a prognostic ice nuclei (IN) formulation and a diurnal cycle. It is demonstrated that IN recycling through subcloud sublimation prolongs ice production. Competing feedbacks between dynamical mixing and recycling are found to slow the rate of ice lost. The results of this study have important implications for the maintenance of phase partitioning in Arctic clouds.
G. Sotiropoulou, J. Sedlar, M. Tjernström, M. D. Shupe, I. M. Brooks, and P. O. G. Persson
Atmos. Chem. Phys., 14, 12573–12592, https://doi.org/10.5194/acp-14-12573-2014, https://doi.org/10.5194/acp-14-12573-2014, 2014
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During ASCOS, clouds are more frequently decoupled from the surface than coupled to it; when coupling occurs it is primary driven by the cloud. Decoupled clouds have a bimodal structure; they are either weakly or strongly decoupled from the surface; the enhancement of the decoupling is possibly due to sublimation of precipitation. Stable clouds (no cloud-driven mixing) are also observed; those are optically thin, often single-phase liquid, with no or negligible precipitation (e.g. fog).
J. M. Intrieri, G. de Boer, M. D. Shupe, J. R. Spackman, J. Wang, P. J. Neiman, G. A. Wick, T. F. Hock, and R. E. Hood
Atmos. Meas. Tech., 7, 3917–3926, https://doi.org/10.5194/amt-7-3917-2014, https://doi.org/10.5194/amt-7-3917-2014, 2014
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In winter 2011, the Global Hawk unmanned aircraft system (UAS) was deployed over the Arctic to evaluate a UAS dropsonde system at high latitudes. Dropsondes deployed from the Global Hawk successfully obtained high-resolution profiles of temperature, pressure, humidity, and wind speed and direction information between the stratosphere and surface. During the 25-hour polar flight, the Global Hawk released 35 sondes between the North Slope of Alaska and 85° N latitude.
J. Sedlar and M. D. Shupe
Atmos. Chem. Phys., 14, 3461–3478, https://doi.org/10.5194/acp-14-3461-2014, https://doi.org/10.5194/acp-14-3461-2014, 2014
M. Tjernström, C. Leck, C. E. Birch, J. W. Bottenheim, B. J. Brooks, I. M. Brooks, L. Bäcklin, R. Y.-W. Chang, G. de Leeuw, L. Di Liberto, S. de la Rosa, E. Granath, M. Graus, A. Hansel, J. Heintzenberg, A. Held, A. Hind, P. Johnston, J. Knulst, M. Martin, P. A. Matrai, T. Mauritsen, M. Müller, S. J. Norris, M. V. Orellana, D. A. Orsini, J. Paatero, P. O. G. Persson, Q. Gao, C. Rauschenberg, Z. Ristovski, J. Sedlar, M. D. Shupe, B. Sierau, A. Sirevaag, S. Sjogren, O. Stetzer, E. Swietlicki, M. Szczodrak, P. Vaattovaara, N. Wahlberg, M. Westberg, and C. R. Wheeler
Atmos. Chem. Phys., 14, 2823–2869, https://doi.org/10.5194/acp-14-2823-2014, https://doi.org/10.5194/acp-14-2823-2014, 2014
G. de Boer, M. D. Shupe, P. M. Caldwell, S. E. Bauer, O. Persson, J. S. Boyle, M. Kelley, S. A. Klein, and M. Tjernström
Atmos. Chem. Phys., 14, 427–445, https://doi.org/10.5194/acp-14-427-2014, https://doi.org/10.5194/acp-14-427-2014, 2014
James Douglas Annan, Julia Catherine Hargreaves, Thorsten Mauritsen, Erin McClymont, and Sze Ling Ho
EGUsphere, https://doi.org/10.5194/egusphere-2023-1941, https://doi.org/10.5194/egusphere-2023-1941, 2023
This preprint is open for discussion and under review for Climate of the Past (CP).
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We have created a new global surface temperature reconstruction of the climate of the mid-Pliocene Warm Period, representing the period roughly 3.2 million years before the present day. We estimate that the globally averaged mean temperature was around 3.6 °C warmer than it was in pre-industrial times, but there is significant uncertainty on this value.
Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
Atmos. Chem. Phys., 23, 9963–9992, https://doi.org/10.5194/acp-23-9963-2023, https://doi.org/10.5194/acp-23-9963-2023, 2023
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Lapse rate feedback (LRF) is a major driver of the Arctic amplification (AA) of climate change. It arises because the warming is stronger at the surface than aloft. Several processes can affect the LRF in the Arctic, such as the omnipresent temperature inversion. Here, we compare multimodel climate simulations to Arctic-based observations from a large research consortium to broaden our understanding of these processes, find synergy among them, and constrain the Arctic LRF and AA.
Manfred Wendisch, Johannes Stapf, Sebastian Becker, André Ehrlich, Evelyn Jäkel, Marcus Klingebiel, Christof Lüpkes, Michael Schäfer, and Matthew D. Shupe
Atmos. Chem. Phys., 23, 9647–9667, https://doi.org/10.5194/acp-23-9647-2023, https://doi.org/10.5194/acp-23-9647-2023, 2023
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Atmospheric radiation measurements have been conducted during two field campaigns using research aircraft. The data are analyzed to see if the near-surface air in the Arctic is warmed or cooled if warm–humid air masses from the south enter the Arctic or cold–dry air moves from the north from the Arctic to mid-latitude areas. It is important to study these processes and to check if climate models represent them well. Otherwise it is not possible to reliably forecast the future Arctic climate.
Sushant Das, Frida Bender, and Thorsten Mauritsen
EGUsphere, https://doi.org/10.5194/egusphere-2023-1605, https://doi.org/10.5194/egusphere-2023-1605, 2023
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Quantifying global and Indian precipitation responses to anthropogenic aerosol and CO2 forcings using multiple models is needed for reducing climate uncertainty. The response to global warming from CO2 increases precipitation both globally and over India, whereas the cooling response to sulfate aerosol leads to a reduction in precipitation in both cases. An opposite response to black carbon is noted i.e., a global decrease but an increase of precipitation over India implying changes in dynamics.
Shijie Peng, Qinghua Yang, Matthew D. Shupe, Xingya Xi, Bo Han, Dake Chen, Sandro Dahlke, and Changwei Liu
Atmos. Chem. Phys., 23, 8683–8703, https://doi.org/10.5194/acp-23-8683-2023, https://doi.org/10.5194/acp-23-8683-2023, 2023
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Due to a lack of observations, the structure of the Arctic atmospheric boundary layer (ABL) remains to be further explored. By analyzing a year-round radiosonde dataset collected over the Arctic sea-ice surface, we found the annual cycle of the ABL height (ABLH) is primarily controlled by the evolution of ABL thermal structure, and the surface conditions also show a high correlation with ABLH variation. In addition, the Arctic ABLH is found to be decreased in summer compared with 20 years ago.
Michael Lonardi, Elisa F. Akansu, André Ehrlich, Mauro Mazzola, Christian Pilz, Matthew D. Shupe, Holger Siebert, and Manfred Wendisch
EGUsphere, https://doi.org/10.5194/egusphere-2023-1396, https://doi.org/10.5194/egusphere-2023-1396, 2023
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Profiles of thermal-infrared irradiance were measured at two Arctic sites. The presence or lack of clouds influences the vertical structure of these observations. In particular, the cloud top region is a source of radiative energy that can promote cooling and mixing in the cloud layer. Simulations are used to further characterize how the amount of water in the cloud modifies this forcing. Two case studies additionally showcase the evolution of the radiation profiles in a dynamic atmosphere.
Clare Marie Flynn, Linnea Huusko, Angshuman Modak, and Thorsten Mauritsen
EGUsphere, https://doi.org/10.5194/egusphere-2023-1613, https://doi.org/10.5194/egusphere-2023-1613, 2023
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The latest-generation climate models show surprisingly cold mid-20th century global-mean temperatures, often despite exhibiting more realistic late-20th/early-21st century temperatures. A too-strong aerosol forcing in many models was thought to the be primary cause of these too-cold mid-century temperatures, but this was found to only be a partial explanation. This also partly undermines the hope to construct a strong relationship between the mid-century temperatures and aerosol forcing.
Angshuman Modak and Thorsten Mauritsen
Atmos. Chem. Phys., 23, 7535–7549, https://doi.org/10.5194/acp-23-7535-2023, https://doi.org/10.5194/acp-23-7535-2023, 2023
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We provide an improved estimate of equilibrium climate sensitivity (ECS) constrained based on the instrumental temperature record including the corrections for the pattern effect. The improved estimate factors in the uncertainty caused by the underlying sea-surface temperature datasets used in the estimates of pattern effect. This together with the inter-model spread lifts the corresponding IPCC AR6 estimate to 3.2 K [1.8 to 11.0], which is lower and better constrained than in past studies.
Ines Bulatovic, Julien Savre, Michael Tjernström, Caroline Leck, and Annica M. L. Ekman
Atmos. Chem. Phys., 23, 7033–7055, https://doi.org/10.5194/acp-23-7033-2023, https://doi.org/10.5194/acp-23-7033-2023, 2023
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We use numerical modeling with detailed cloud microphysics to investigate a low-altitude cloud system consisting of two cloud layers – a type of cloud situation which was commonly observed during the summer of 2018 in the central Arctic (north of 80° N). The model generally reproduces the observed cloud layers and the thermodynamic structure of the lower atmosphere well. The cloud system is maintained unless there are low aerosol number concentrations or high large-scale wind speeds.
Kameswara S. Vinjamuri, Marco Vountas, Luca Lelli, Martin Stengel, Matthew D. Shupe, Kerstin Ebell, and John P. Burrows
Atmos. Meas. Tech., 16, 2903–2918, https://doi.org/10.5194/amt-16-2903-2023, https://doi.org/10.5194/amt-16-2903-2023, 2023
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Clouds play an important role in Arctic amplification. Cloud data from ground-based sites are valuable but cannot represent the whole Arctic. Therefore the use of satellite products is a measure to cover the entire Arctic. However, the quality of such cloud measurements from space is not well known. The paper discusses the differences and commonalities between satellite and ground-based measurements. We conclude that the satellite dataset, with a few exceptions, can be used in the Arctic.
John Prytherch, Sonja Murto, Ian Brown, Adam Ulfsbo, Brett F. Thornton, Volker Brüchert, Michael Tjernström, Anna Lunde Hermansson, Amanda T. Nylund, and Lina A. Holthusen
Biogeosciences Discuss., https://doi.org/10.5194/bg-2023-82, https://doi.org/10.5194/bg-2023-82, 2023
Preprint under review for BG
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We used chamber-flux systems to directly measure methane and carbon dioxide exchange between the ocean or sea ice and the atmosphere during an icebreaker-based expedition to the Central Arctic Ocean in summer 2021. These measurement-based constraints inform climate modeling and carbon budgets. The methane exchange measurements, the first such made in the CAO, are lower than previous estimates and imply that the CAO is an insignificant contributor to Arctic methane emission.
Ulrike Egerer, John J. Cassano, Matthew D. Shupe, Gijs de Boer, Dale Lawrence, Abhiram Doddi, Holger Siebert, Gina Jozef, Radiance Calmer, Jonathan Hamilton, Christian Pilz, and Michael Lonardi
Atmos. Meas. Tech., 16, 2297–2317, https://doi.org/10.5194/amt-16-2297-2023, https://doi.org/10.5194/amt-16-2297-2023, 2023
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This paper describes how measurements from a small uncrewed aircraft system can be used to estimate the vertical turbulent heat energy exchange between different layers in the atmosphere. This is particularly important for the atmosphere in the Arctic, as turbulent exchange in this region is often suppressed but is still important to understand how the atmosphere interacts with sea ice. We present three case studies from the MOSAiC field campaign in Arctic sea ice in 2020.
Gillian Young McCusker, Jutta Vüllers, Peggy Achtert, Paul Field, Jonathan J. Day, Richard Forbes, Ruth Price, Ewan O'Connor, Michael Tjernström, John Prytherch, Ryan Neely III, and Ian M. Brooks
Atmos. Chem. Phys., 23, 4819–4847, https://doi.org/10.5194/acp-23-4819-2023, https://doi.org/10.5194/acp-23-4819-2023, 2023
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In this study, we show that recent versions of two atmospheric models – the Unified Model and Integrated Forecasting System – overestimate Arctic cloud fraction within the lower troposphere by comparison with recent remote-sensing measurements made during the Arctic Ocean 2018 expedition. The overabundance of cloud is interlinked with the modelled thermodynamic structure, with strong negative temperature biases coincident with these overestimated cloud layers.
Maximilian Maahn, Dmitri Moisseev, Isabelle Steinke, Nina Maherndl, and Matthew D. Shupe
EGUsphere, https://doi.org/10.5194/egusphere-2023-655, https://doi.org/10.5194/egusphere-2023-655, 2023
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The open source Video In Situ Snowfall Sensor (VISSS) is a novel instrument for characterizing particle shape and size in snowfall. It allows accurate sizing of snow particles and combines a large observation volume with relatively high resolution and a design that limits wind perturbations. The open source nature of the VISSS hardware and software invites the community to contribute to the development of the instrument, which has many potential applications in atmospheric science and beyond.
Felix Pithan, Marylou Athanase, Sandro Dahlke, Antonio Sánchez-Benítez, Matthew D. Shupe, Anne Sledd, Jan Streffing, Gunilla Svensson, and Thomas Jung
Geosci. Model Dev., 16, 1857–1873, https://doi.org/10.5194/gmd-16-1857-2023, https://doi.org/10.5194/gmd-16-1857-2023, 2023
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Evaluating climate models usually requires long observational time series, but we present a method that also works for short field campaigns. We compare climate model output to observations from the MOSAiC expedition in the central Arctic Ocean. All models show how the arrival of a warm air mass warms the Arctic in April 2020, but two models do not show the response of snow temperature to the diurnal cycle. One model has too little liquid water and too much ice in clouds during cold days.
Ruth Price, Andrea Baccarini, Julia Schmale, Paul Zieger, Ian M. Brooks, Paul Field, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 2927–2961, https://doi.org/10.5194/acp-23-2927-2023, https://doi.org/10.5194/acp-23-2927-2023, 2023
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Arctic clouds can control how much energy is absorbed by the surface or reflected back to space. Using a computer model of the atmosphere we investigated the formation of atmospheric particles that allow cloud droplets to form. We found that particles formed aloft are transported to the lowest part of the Arctic atmosphere and that this is a key source of particles. Our results have implications for the way Arctic clouds will behave in the future as climate change continues to impact the region.
Martin Renoult, Navjit Sagoo, Jiang Zhu, and Thorsten Mauritsen
Clim. Past, 19, 323–356, https://doi.org/10.5194/cp-19-323-2023, https://doi.org/10.5194/cp-19-323-2023, 2023
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The relationship between the Last Glacial Maximum and the sensitivity of climate models to a doubling of CO2 can be used to estimate the true sensitivity of the Earth. However, this relationship has varied in successive model generations. In this study, we assess multiple processes at the Last Glacial Maximum which weaken this relationship. For example, how models respond to the presence of ice sheets is a large contributor of uncertainty.
Cathy Hohenegger, Peter Korn, Leonidas Linardakis, René Redler, Reiner Schnur, Panagiotis Adamidis, Jiawei Bao, Swantje Bastin, Milad Behravesh, Martin Bergemann, Joachim Biercamp, Hendryk Bockelmann, Renate Brokopf, Nils Brüggemann, Lucas Casaroli, Fatemeh Chegini, George Datseris, Monika Esch, Geet George, Marco Giorgetta, Oliver Gutjahr, Helmuth Haak, Moritz Hanke, Tatiana Ilyina, Thomas Jahns, Johann Jungclaus, Marcel Kern, Daniel Klocke, Lukas Kluft, Tobias Kölling, Luis Kornblueh, Sergey Kosukhin, Clarissa Kroll, Junhong Lee, Thorsten Mauritsen, Carolin Mehlmann, Theresa Mieslinger, Ann Kristin Naumann, Laura Paccini, Angel Peinado, Divya Sri Praturi, Dian Putrasahan, Sebastian Rast, Thomas Riddick, Niklas Roeber, Hauke Schmidt, Uwe Schulzweida, Florian Schütte, Hans Segura, Radomyra Shevchenko, Vikram Singh, Mia Specht, Claudia Christine Stephan, Jin-Song von Storch, Raphaela Vogel, Christian Wengel, Marius Winkler, Florian Ziemen, Jochem Marotzke, and Bjorn Stevens
Geosci. Model Dev., 16, 779–811, https://doi.org/10.5194/gmd-16-779-2023, https://doi.org/10.5194/gmd-16-779-2023, 2023
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Models of the Earth system used to understand climate and predict its change typically employ a grid spacing of about 100 km. Yet, many atmospheric and oceanic processes occur on much smaller scales. In this study, we present a new model configuration designed for the simulation of the components of the Earth system and their interactions at kilometer and smaller scales, allowing an explicit representation of the main drivers of the flow of energy and matter by solving the underlying equations.
Heather Guy, David D. Turner, Von P. Walden, Ian M. Brooks, and Ryan R. Neely
Atmos. Meas. Tech., 15, 5095–5115, https://doi.org/10.5194/amt-15-5095-2022, https://doi.org/10.5194/amt-15-5095-2022, 2022
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Fog formation is highly sensitive to near-surface temperatures and humidity profiles. Passive remote sensing instruments can provide continuous measurements of the vertical temperature and humidity profiles and liquid water content, which can improve fog forecasts. Here we compare the performance of collocated infrared and microwave remote sensing instruments and demonstrate that the infrared instrument is especially sensitive to the onset of thin radiation fog.
Océane Hames, Mahdi Jafari, David Nicholas Wagner, Ian Raphael, David Clemens-Sewall, Chris Polashenski, Matthew D. Shupe, Martin Schneebeli, and Michael Lehning
Geosci. Model Dev., 15, 6429–6449, https://doi.org/10.5194/gmd-15-6429-2022, https://doi.org/10.5194/gmd-15-6429-2022, 2022
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This paper presents an Eulerian–Lagrangian snow transport model implemented in the fluid dynamics software OpenFOAM, which we call snowBedFoam 1.0. We apply this model to reproduce snow deposition on a piece of ridged Arctic sea ice, which was produced during the MOSAiC expedition through scan measurements. The model appears to successfully reproduce the enhanced snow accumulation and deposition patterns, although some quantitative uncertainties were shown.
James D. Annan, Julia C. Hargreaves, and Thorsten Mauritsen
Clim. Past, 18, 1883–1896, https://doi.org/10.5194/cp-18-1883-2022, https://doi.org/10.5194/cp-18-1883-2022, 2022
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We have created a new global surface temperature reconstruction of the climate of the Last Glacial Maximum, representing the period 19–23 000 years before the present day. We find that the globally averaged mean temperature was roughly 4.5 °C colder than it was in pre-industrial times, albeit there is significant uncertainty on this value.
Assia Arouf, Hélène Chepfer, Thibault Vaillant de Guélis, Marjolaine Chiriaco, Matthew D. Shupe, Rodrigo Guzman, Artem Feofilov, Patrick Raberanto, Tristan S. L'Ecuyer, Seiji Kato, and Michael R. Gallagher
Atmos. Meas. Tech., 15, 3893–3923, https://doi.org/10.5194/amt-15-3893-2022, https://doi.org/10.5194/amt-15-3893-2022, 2022
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We proposed new estimates of the surface longwave (LW) cloud radiative effect (CRE) derived from observations collected by a space-based lidar on board the CALIPSO satellite and radiative transfer computations. Our estimate appropriately captures the surface LW CRE annual variability over bright polar surfaces, and it provides a dataset more than 13 years long.
Cheng You, Michael Tjernström, and Abhay Devasthale
Atmos. Chem. Phys., 22, 8037–8057, https://doi.org/10.5194/acp-22-8037-2022, https://doi.org/10.5194/acp-22-8037-2022, 2022
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In winter when solar radiation is absent in the Arctic, the poleward transport of heat and moisture into the high Arctic becomes the main contribution of Arctic warming. Over completely frozen ocean sectors, total surface energy budget is dominated by net long-wave heat, while over the Barents Sea, with an open ocean to the south, total net surface energy budget is dominated by the surface turbulent heat.
David N. Wagner, Matthew D. Shupe, Christopher Cox, Ola G. Persson, Taneil Uttal, Markus M. Frey, Amélie Kirchgaessner, Martin Schneebeli, Matthias Jaggi, Amy R. Macfarlane, Polona Itkin, Stefanie Arndt, Stefan Hendricks, Daniela Krampe, Marcel Nicolaus, Robert Ricker, Julia Regnery, Nikolai Kolabutin, Egor Shimanshuck, Marc Oggier, Ian Raphael, Julienne Stroeve, and Michael Lehning
The Cryosphere, 16, 2373–2402, https://doi.org/10.5194/tc-16-2373-2022, https://doi.org/10.5194/tc-16-2373-2022, 2022
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Based on measurements of the snow cover over sea ice and atmospheric measurements, we estimate snowfall and snow accumulation for the MOSAiC ice floe, between November 2019 and May 2020. For this period, we estimate 98–114 mm of precipitation. We suggest that about 34 mm of snow water equivalent accumulated until the end of April 2020 and that at least about 50 % of the precipitated snow was eroded or sublimated. Further, we suggest explanations for potential snowfall overestimation.
Helen Czerski, Ian M. Brooks, Steve Gunn, Robin Pascal, Adrian Matei, and Byron Blomquist
Ocean Sci., 18, 565–586, https://doi.org/10.5194/os-18-565-2022, https://doi.org/10.5194/os-18-565-2022, 2022
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The bubbles formed by breaking waves speed up the movement of gases like carbon dioxide and oxygen between the atmosphere and the ocean. Understanding where these gases go is an important part of understanding Earth's climate. In this paper we describe measurements of the bubbles close to the ocean surface during big storms in the North Atlantic. We observed small bubbles collecting in distinctive patterns which help us to understand the contribution they make to the ocean breathing.
Helen Czerski, Ian M. Brooks, Steve Gunn, Robin Pascal, Adrian Matei, and Byron Blomquist
Ocean Sci., 18, 587–608, https://doi.org/10.5194/os-18-587-2022, https://doi.org/10.5194/os-18-587-2022, 2022
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The bubbles formed by breaking waves at the ocean surface are important because they are thought to speed up the movement of gases like carbon dioxide and oxygen between the atmosphere and ocean. We collected data on the bubbles in the top few metres of the ocean which were created by storms in the North Atlantic. The focus in this paper is the bubble sizes and their position in the water. We saw that there are very predictable patterns and set out what happens to bubbles after a wave breaks.
Piyush Srivastava, Ian M. Brooks, John Prytherch, Dominic J. Salisbury, Andrew D. Elvidge, Ian A. Renfrew, and Margaret J. Yelland
Atmos. Chem. Phys., 22, 4763–4778, https://doi.org/10.5194/acp-22-4763-2022, https://doi.org/10.5194/acp-22-4763-2022, 2022
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The parameterization of surface turbulent fluxes over sea ice remains a weak point in weather forecast and climate models. Recent theoretical developments have introduced more extensive physics but these descriptions are poorly constrained due to a lack of observation data. Here we utilize a large dataset of measurements of turbulent fluxes over sea ice to tune the state-of-the-art parameterization of wind stress, and compare it with a previous scheme.
Michael R. Gallagher, Matthew D. Shupe, Hélène Chepfer, and Tristan L'Ecuyer
The Cryosphere, 16, 435–450, https://doi.org/10.5194/tc-16-435-2022, https://doi.org/10.5194/tc-16-435-2022, 2022
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By using direct observations of snowfall and mass changes, the variability of daily snowfall mass input to the Greenland ice sheet is quantified for the first time. With new methods we conclude that cyclones west of Greenland in summer contribute the most snowfall, with 1.66 Gt per occurrence. These cyclones are contextualized in the broader Greenland climate, and snowfall is validated against mass changes to verify the results. Snowfall and mass change observations are shown to agree well.
Tiina Nygård, Michael Tjernström, and Tuomas Naakka
Weather Clim. Dynam., 2, 1263–1282, https://doi.org/10.5194/wcd-2-1263-2021, https://doi.org/10.5194/wcd-2-1263-2021, 2021
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Temperature and humidity profiles in the Arctic atmosphere in winter are affected by both the large-scale dynamics and the local processes, such as radiation, cloud formation and turbulence. The results show that the influence of different large-scale flows on temperature and humidity profiles must be viewed as a progressing set of processes. Within the Arctic, there are notable regional differences in how large-scale flows affect the temperature and specific humidity profiles.
Heather Guy, Ian M. Brooks, Ken S. Carslaw, Benjamin J. Murray, Von P. Walden, Matthew D. Shupe, Claire Pettersen, David D. Turner, Christopher J. Cox, William D. Neff, Ralf Bennartz, and Ryan R. Neely III
Atmos. Chem. Phys., 21, 15351–15374, https://doi.org/10.5194/acp-21-15351-2021, https://doi.org/10.5194/acp-21-15351-2021, 2021
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We present the first full year of surface aerosol number concentration measurements from the central Greenland Ice Sheet. Aerosol concentrations here have a distinct seasonal cycle from those at lower-altitude Arctic sites, which is driven by large-scale atmospheric circulation. Our results can be used to help understand the role aerosols might play in Greenland surface melt through the modification of cloud properties. This is crucial in a rapidly changing region where observations are sparse.
Erik Johansson, Abhay Devasthale, Michael Tjernström, Annica M. L. Ekman, Klaus Wyser, and Tristan L'Ecuyer
Geosci. Model Dev., 14, 4087–4101, https://doi.org/10.5194/gmd-14-4087-2021, https://doi.org/10.5194/gmd-14-4087-2021, 2021
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Understanding the coupling of clouds to large-scale circulation is a grand challenge for the climate community. Cloud radiative heating (CRH) is a key parameter in this coupling and is therefore essential to model realistically. We, therefore, evaluate a climate model against satellite observations. Our findings indicate good agreement in the seasonal pattern of CRH even if the magnitude differs. We also find that increasing the horizontal resolution in the model has little effect on the CRH.
Ines Bulatovic, Adele L. Igel, Caroline Leck, Jost Heintzenberg, Ilona Riipinen, and Annica M. L. Ekman
Atmos. Chem. Phys., 21, 3871–3897, https://doi.org/10.5194/acp-21-3871-2021, https://doi.org/10.5194/acp-21-3871-2021, 2021
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We use detailed numerical modelling to show that small aerosol particles (diameters ~25–80 nm; so-called Aitken mode particles) significantly influence low-level cloud properties in the clean summertime high Arctic. The small particles can help sustain clouds when the concentration of larger particles is low (<10–20 cm-3). Measurements from four different observational campaigns in the high Arctic support the modelling results as they indicate that Aitken mode aerosols are frequently activated.
Jule Radtke, Thorsten Mauritsen, and Cathy Hohenegger
Atmos. Chem. Phys., 21, 3275–3288, https://doi.org/10.5194/acp-21-3275-2021, https://doi.org/10.5194/acp-21-3275-2021, 2021
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Shallow trade wind clouds are a key source of uncertainty to projections of the Earth's changing climate. We perform high-resolution simulations of trade cumulus and investigate how the representation and climate feedback of these clouds depend on the specific grid spacing. We find that the cloud feedback is positive when simulated with kilometre but near zero when simulated with hectometre grid spacing. These findings suggest that storm-resolving models may exaggerate the trade cloud feedback.
Jessie M. Creamean, Gijs de Boer, Hagen Telg, Fan Mei, Darielle Dexheimer, Matthew D. Shupe, Amy Solomon, and Allison McComiskey
Atmos. Chem. Phys., 21, 1737–1757, https://doi.org/10.5194/acp-21-1737-2021, https://doi.org/10.5194/acp-21-1737-2021, 2021
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Arctic clouds play a role in modulating sea ice extent. Importantly, aerosols facilitate cloud formation, and thus it is crucial to understand the interactions between aerosols and clouds. Vertical measurements of aerosols and clouds are needed to tackle this issue. We present results from balloon-borne measurements of aerosols and clouds over the course of 2 years in northern Alaska. These data shed light onto the vertical distributions of aerosols relative to clouds spanning multiple seasons.
Jutta Vüllers, Peggy Achtert, Ian M. Brooks, Michael Tjernström, John Prytherch, Annika Burzik, and Ryan Neely III
Atmos. Chem. Phys., 21, 289–314, https://doi.org/10.5194/acp-21-289-2021, https://doi.org/10.5194/acp-21-289-2021, 2021
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This paper provides interesting new results on the thermodynamic structure of the boundary layer, cloud conditions, and fog characteristics in the Arctic during the Arctic Ocean 2018 campaign. It provides information for interpreting further process studies on aerosol–cloud interactions and shows substantial differences in thermodynamic conditions and cloud characteristics based on comparison with previous campaigns. This certainly raises the question of whether it is just an exceptional year.
André Welti, E. Keith Bigg, Paul J. DeMott, Xianda Gong, Markus Hartmann, Mike Harvey, Silvia Henning, Paul Herenz, Thomas C. J. Hill, Blake Hornblow, Caroline Leck, Mareike Löffler, Christina S. McCluskey, Anne Marie Rauker, Julia Schmale, Christian Tatzelt, Manuela van Pinxteren, and Frank Stratmann
Atmos. Chem. Phys., 20, 15191–15206, https://doi.org/10.5194/acp-20-15191-2020, https://doi.org/10.5194/acp-20-15191-2020, 2020
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Ship-based measurements of maritime ice nuclei concentrations encompassing all oceans are compiled. From this overview it is found that maritime ice nuclei concentrations are typically 10–100 times lower than over continents, while concentrations are surprisingly similar in different oceanic regions. The analysis of the influence of ship emissions shows no effect on the data, making ship-based measurements an efficient strategy for the large-scale exploration of ice nuclei concentrations.
Peggy Achtert, Ewan J. O'Connor, Ian M. Brooks, Georgia Sotiropoulou, Matthew D. Shupe, Bernhard Pospichal, Barbara J. Brooks, and Michael Tjernström
Atmos. Chem. Phys., 20, 14983–15002, https://doi.org/10.5194/acp-20-14983-2020, https://doi.org/10.5194/acp-20-14983-2020, 2020
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We present observations of precipitating and non-precipitating Arctic liquid and mixed-phase clouds during a research cruise along the Russian shelf in summer and autumn of 2014. Active remote-sensing observations, radiosondes, and auxiliary measurements are combined in the synergistic Cloudnet retrieval. Cloud properties are analysed with respect to cloud-top temperature and boundary layer structure. About 8 % of all liquid clouds show a liquid water path below the infrared black body limit.
Luisa Ickes, Grace C. E. Porter, Robert Wagner, Michael P. Adams, Sascha Bierbauer, Allan K. Bertram, Merete Bilde, Sigurd Christiansen, Annica M. L. Ekman, Elena Gorokhova, Kristina Höhler, Alexei A. Kiselev, Caroline Leck, Ottmar Möhler, Benjamin J. Murray, Thea Schiebel, Romy Ullrich, and Matthew E. Salter
Atmos. Chem. Phys., 20, 11089–11117, https://doi.org/10.5194/acp-20-11089-2020, https://doi.org/10.5194/acp-20-11089-2020, 2020
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The Arctic is a region where aerosols are scarce. Sea spray might be a potential source of aerosols acting as ice-nucleating particles. We investigate two common phytoplankton species (Melosira arctica and Skeletonema marinoi) and present their ice nucleation activity in comparison with Arctic seawater microlayer samples from different field campaigns. We also aim to understand the aerosolization process of marine biological samples and the potential effect on the ice nucleation activity.
Martin Renoult, James Douglas Annan, Julia Catherine Hargreaves, Navjit Sagoo, Clare Flynn, Marie-Luise Kapsch, Qiang Li, Gerrit Lohmann, Uwe Mikolajewicz, Rumi Ohgaito, Xiaoxu Shi, Qiong Zhang, and Thorsten Mauritsen
Clim. Past, 16, 1715–1735, https://doi.org/10.5194/cp-16-1715-2020, https://doi.org/10.5194/cp-16-1715-2020, 2020
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Interest in past climates as sources of information for the climate system has grown in recent years. In particular, studies of the warm mid-Pliocene and cold Last Glacial Maximum showed relationships between the tropical surface temperature of the Earth and its sensitivity to an abrupt doubling of atmospheric CO2. In this study, we develop a new and promising statistical method and obtain similar results as previously observed, wherein the sensitivity does not seem to exceed extreme values.
James D. Annan, Julia C. Hargreaves, Thorsten Mauritsen, and Bjorn Stevens
Earth Syst. Dynam., 11, 709–719, https://doi.org/10.5194/esd-11-709-2020, https://doi.org/10.5194/esd-11-709-2020, 2020
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In this paper we explore the potential of variability for constraining the equilibrium response of the climate system to external forcing. We show that the constraint is inherently skewed, with a long tail to high sensitivity, and that while the variability may contain some useful information, it is unlikely to generate a tight constraint.
Clare Marie Flynn and Thorsten Mauritsen
Atmos. Chem. Phys., 20, 7829–7842, https://doi.org/10.5194/acp-20-7829-2020, https://doi.org/10.5194/acp-20-7829-2020, 2020
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The range of climate sensitivity of models participating in CMIP6 has increased relative to models participating in CMIP5 due to decreases in the total feedback parameter. This is caused by increases in the shortwave all-sky and clear-sky feedbacks, particularly over the Southern Ocean. These shifts between CMIP6 and CMIP5 did not arise by chance. Both CMIP5 and CMIP6 models are found to exhibit aerosol forcing that is too strong, causing too much cooling relative to observations.
Grace C. E. Porter, Sebastien N. F. Sikora, Michael P. Adams, Ulrike Proske, Alexander D. Harrison, Mark D. Tarn, Ian M. Brooks, and Benjamin J. Murray
Atmos. Meas. Tech., 13, 2905–2921, https://doi.org/10.5194/amt-13-2905-2020, https://doi.org/10.5194/amt-13-2905-2020, 2020
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Ice-nucleating particles affect cloud development, lifetime, and radiative properties. Hence it is important to know the abundance of INPs throughout the atmosphere. Here we present the development and application of a radio-controlled payload capable of collecting size-resolved aerosol from a tethered balloon for the primary purpose of offline INP analysis. Test data are presented from four locations: southern Finland, northern England, Svalbard, and southern England.
Rosa Gierens, Stefan Kneifel, Matthew D. Shupe, Kerstin Ebell, Marion Maturilli, and Ulrich Löhnert
Atmos. Chem. Phys., 20, 3459–3481, https://doi.org/10.5194/acp-20-3459-2020, https://doi.org/10.5194/acp-20-3459-2020, 2020
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Multiyear statistics of persistent low-level mixed-phase clouds observed at an Arctic fjord environment in Svalbard are presented. The effects the local boundary layer (i.e. the fjords' wind climate and surface coupling), regional wind direction, and seasonality have on the cloud occurrence and properties are evaluated using a synergy of ground-based remote sensing methods and auxiliary data. The phenomena considered were found to modify the amount of liquid and ice in the studied clouds.
Markus M. Frey, Sarah J. Norris, Ian M. Brooks, Philip S. Anderson, Kouichi Nishimura, Xin Yang, Anna E. Jones, Michelle G. Nerentorp Mastromonaco, David H. Jones, and Eric W. Wolff
Atmos. Chem. Phys., 20, 2549–2578, https://doi.org/10.5194/acp-20-2549-2020, https://doi.org/10.5194/acp-20-2549-2020, 2020
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A winter sea ice expedition to Antarctica provided the first direct observations of sea salt aerosol (SSA) production during snow storms above sea ice, thereby validating a model hypothesis to account for winter time SSA maxima in Antarctica not explained otherwise. Defining SSA sources is important given the critical roles that aerosol plays for climate, for air quality and as a potential ice core proxy for sea ice conditions in the past.
Mingxi Yang, Sarah J. Norris, Thomas G. Bell, and Ian M. Brooks
Atmos. Chem. Phys., 19, 15271–15284, https://doi.org/10.5194/acp-19-15271-2019, https://doi.org/10.5194/acp-19-15271-2019, 2019
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This work reports direct measurements of sea spray fluxes from a coastal site in the UK, which are relevant for atmospheric chemistry as well as coastal air quality. Sea spray fluxes from this location are roughly an order of magnitude greater than over the open ocean at similar wind conditions, comparable to previous coastal measurements. Unlike previous open ocean measurements that are largely wind speed dependent, we find that sea spray fluxes near the coast depend more strongly on waves.
Gijs de Boer, Darielle Dexheimer, Fan Mei, John Hubbe, Casey Longbottom, Peter J. Carroll, Monty Apple, Lexie Goldberger, David Oaks, Justin Lapierre, Michael Crume, Nathan Bernard, Matthew D. Shupe, Amy Solomon, Janet Intrieri, Dale Lawrence, Abhiram Doddi, Donna J. Holdridge, Michael Hubbell, Mark D. Ivey, and Beat Schmid
Earth Syst. Sci. Data, 11, 1349–1362, https://doi.org/10.5194/essd-11-1349-2019, https://doi.org/10.5194/essd-11-1349-2019, 2019
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This paper provides a summary of observations collected at Oliktok Point, Alaska, as part of the Profiling at Oliktok Point to Enhance YOPP Experiments (POPEYE) campaign. The Year of Polar Prediction (YOPP) is a multi-year concentrated effort to improve forecasting capabilities at high latitudes across a variety of timescales. POPEYE observations include atmospheric data collected using unmanned aircraft, tethered balloons, and radiosondes, made in parallel with routine measurements at the site.
Xin Yang, Markus M. Frey, Rachael H. Rhodes, Sarah J. Norris, Ian M. Brooks, Philip S. Anderson, Kouichi Nishimura, Anna E. Jones, and Eric W. Wolff
Atmos. Chem. Phys., 19, 8407–8424, https://doi.org/10.5194/acp-19-8407-2019, https://doi.org/10.5194/acp-19-8407-2019, 2019
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This is a comprehensive model–data comparison aiming to evaluate the proposed mechanism of sea salt aerosol (SSA) production from blowing snow on sea ice. Some key parameters such as snow salinity and blowing-snow size distribution were constrained by data collected in the Weddell Sea. The good agreement between modelled SSA and the cruise data strongly indicates that sea ice surface is a large SSA source in polar regions, a process which has not been considered in current climate models.
Ralf Bennartz, Frank Fell, Claire Pettersen, Matthew D. Shupe, and Dirk Schuettemeyer
Atmos. Chem. Phys., 19, 8101–8121, https://doi.org/10.5194/acp-19-8101-2019, https://doi.org/10.5194/acp-19-8101-2019, 2019
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The Greenland Ice Sheet (GrIS) is rapidly melting. Snowfall is the only source of ice mass over the GrIS. We use satellite observations to assess how much snow on average falls over the GrIS and what the annual cycle and spatial distribution of snowfall is. We find the annual mean snowfall over the GrIS inferred from CloudSat to be 34 ± 7.5 cm yr−1 liquid equivalent.
Maximilian Maahn, Fabian Hoffmann, Matthew D. Shupe, Gijs de Boer, Sergey Y. Matrosov, and Edward P. Luke
Atmos. Meas. Tech., 12, 3151–3171, https://doi.org/10.5194/amt-12-3151-2019, https://doi.org/10.5194/amt-12-3151-2019, 2019
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Cloud radars are unique instruments for observing cloud processes, but uncertainties in radar calibration have frequently limited data quality. Here, we present three novel methods for calibrating vertically pointing cloud radars. These calibration methods are based on microphysical processes of liquid clouds, such as the transition of cloud droplets to drizzle drops. We successfully apply the methods to cloud radar data from the North Slope of Alaska (NSA) and Oliktok Point (OLI) ARM sites.
Christopher J. Cox, David C. Noone, Max Berkelhammer, Matthew D. Shupe, William D. Neff, Nathaniel B. Miller, Von P. Walden, and Konrad Steffen
Atmos. Chem. Phys., 19, 7467–7485, https://doi.org/10.5194/acp-19-7467-2019, https://doi.org/10.5194/acp-19-7467-2019, 2019
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Fogs are frequently reported by observers on the Greenland Ice Sheet. Fogs play a role in the hydrological and energetic balances of the ice sheet surface, but as yet the properties of Greenland fogs are not well known. We observed fogs in all months from Summit Station for 2 years and report their properties. Annually, fogs impart a slight warming to the surface and a case study suggests that they are particularly influential by providing insulation during the coldest part of the day in summer.
Daniel T. McCoy, Paul R. Field, Gregory S. Elsaesser, Alejandro Bodas-Salcedo, Brian H. Kahn, Mark D. Zelinka, Chihiro Kodama, Thorsten Mauritsen, Benoit Vanniere, Malcolm Roberts, Pier L. Vidale, David Saint-Martin, Aurore Voldoire, Rein Haarsma, Adrian Hill, Ben Shipway, and Jonathan Wilkinson
Atmos. Chem. Phys., 19, 1147–1172, https://doi.org/10.5194/acp-19-1147-2019, https://doi.org/10.5194/acp-19-1147-2019, 2019
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The largest single source of uncertainty in the climate sensitivity predicted by global climate models is how much low-altitude clouds change as the climate warms. Models predict that the amount of liquid within and the brightness of low-altitude clouds increase in the extratropics with warming. We show that increased fluxes of moisture into extratropical storms in the midlatitudes explain the majority of the observed trend and the modeled increase in liquid water within these storms.
Amy Solomon, Gijs de Boer, Jessie M. Creamean, Allison McComiskey, Matthew D. Shupe, Maximilian Maahn, and Christopher Cox
Atmos. Chem. Phys., 18, 17047–17059, https://doi.org/10.5194/acp-18-17047-2018, https://doi.org/10.5194/acp-18-17047-2018, 2018
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The results of this study indicate that perturbations in ice nucleating particles (INPs) dominate over cloud condensation nuclei (CCN) perturbations in Arctic mixed-phase stratocumulus; i.e., an equivalent fractional decrease in CCN and INPs results in an increase in the cloud-top longwave cooling rate, even though the droplet effective radius increases and the cloud emissivity decreases. In addition, cloud-processing causes layering of aerosols with increased concentrations of CCN at cloud top.
Matthew S. Norgren, Gijs de Boer, and Matthew D. Shupe
Atmos. Chem. Phys., 18, 13345–13361, https://doi.org/10.5194/acp-18-13345-2018, https://doi.org/10.5194/acp-18-13345-2018, 2018
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Arctic mixed-phase clouds are a critical component of the Arctic climate system because of their ability to influence the surface radiation budget. The radiative impact of an individual cloud is closely linked to the ability of the cloud to convert liquid drops to ice. In this paper, we show through an observational record that clouds present in polluted atmospheric conditions have lower amounts of ice than similar clouds found in clean conditions.
Angela Benedetti, Jeffrey S. Reid, Peter Knippertz, John H. Marsham, Francesca Di Giuseppe, Samuel Rémy, Sara Basart, Olivier Boucher, Ian M. Brooks, Laurent Menut, Lucia Mona, Paolo Laj, Gelsomina Pappalardo, Alfred Wiedensohler, Alexander Baklanov, Malcolm Brooks, Peter R. Colarco, Emilio Cuevas, Arlindo da Silva, Jeronimo Escribano, Johannes Flemming, Nicolas Huneeus, Oriol Jorba, Stelios Kazadzis, Stefan Kinne, Thomas Popp, Patricia K. Quinn, Thomas T. Sekiyama, Taichu Tanaka, and Enric Terradellas
Atmos. Chem. Phys., 18, 10615–10643, https://doi.org/10.5194/acp-18-10615-2018, https://doi.org/10.5194/acp-18-10615-2018, 2018
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Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centers. This development is due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation authorities, solar energy plant managers, climate service providers, and health professionals. This paper describes the advances in the field and sets out requirements for observations for the sustainability of these activities.
Andrew E. Dessler, Thorsten Mauritsen, and Bjorn Stevens
Atmos. Chem. Phys., 18, 5147–5155, https://doi.org/10.5194/acp-18-5147-2018, https://doi.org/10.5194/acp-18-5147-2018, 2018
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One of the most important parameters in climate science is the equilibrium climate sensitivity (ECS). Estimates of this quantity based on 20th-century observations suggest low values of ECS (below 2 °C). We show that these calculations may be significantly in error. Together with other recent work on this problem, it seems probable that the ECS is larger than suggested by the 20th-century observations.
Claire Pettersen, Ralf Bennartz, Aronne J. Merrelli, Matthew D. Shupe, David D. Turner, and Von P. Walden
Atmos. Chem. Phys., 18, 4715–4735, https://doi.org/10.5194/acp-18-4715-2018, https://doi.org/10.5194/acp-18-4715-2018, 2018
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A novel method for classifying Arctic precipitation using ground based remote sensors is presented. The classification reveals two distinct, primary regimes of precipitation over the central Greenland Ice Sheet: snowfall coupled to deep, fully glaciated ice clouds or to shallow, mixed-phase clouds. The ice clouds are associated with low-pressure storm systems from the southeast, while the mixed-phase clouds slowly propagate from the southwest along a quiescent flow.
Robert A. Stillwell, Ryan R. Neely III, Jeffrey P. Thayer, Matthew D. Shupe, and David D. Turner
Atmos. Meas. Tech., 11, 835–859, https://doi.org/10.5194/amt-11-835-2018, https://doi.org/10.5194/amt-11-835-2018, 2018
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This work focuses on making unambiguous measurements of Arctic cloud phase and assessing those measurements within the context of cloud radiative effects. It is found that effects related to lidar data recording systems can cause retrieval ambiguities that alter the interpretation of cloud phase in as much as 30 % of the available data. This misinterpretation of cloud-phase data can cause a misinterpretation of the effect of cloud phase on the surface radiation budget by as much as 10 to 30 %.
Katharina Loewe, Annica M. L. Ekman, Marco Paukert, Joseph Sedlar, Michael Tjernström, and Corinna Hoose
Atmos. Chem. Phys., 17, 6693–6704, https://doi.org/10.5194/acp-17-6693-2017, https://doi.org/10.5194/acp-17-6693-2017, 2017
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Processes that affect Arctic mixed-phase cloud life cycle are extremely important for the surface energy budget. Three different sensitivity experiments mimic changes in the advection of air masses with different thermodynamic profiles and aerosol properties to find the potential mechanisms leading to the dissipation of the cloud. We found that the reduction of the cloud droplet number concentration was likely the primary contributor to the dissipation of the observed Arctic mixed-phase cloud.
Jost Heintzenberg, Peter Tunved, Martí Galí, and Caroline Leck
Atmos. Chem. Phys., 17, 6153–6175, https://doi.org/10.5194/acp-17-6153-2017, https://doi.org/10.5194/acp-17-6153-2017, 2017
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Events of new particle formation (NPF) were analyzed objectively in a 10-year data set of hourly particle size distributions recorded on Mt. Zeppelin, Spitsbergen, Svalbard. Three different types of NPF events were identified that were hypothesized to be different expressions of related source processes. Back trajectories and ancillary atmospheric and marine data strongly point to marine biogenic sources causing new particle formation in the summer Arctic.
Yinghui Liu, Matthew D. Shupe, Zhien Wang, and Gerald Mace
Atmos. Chem. Phys., 17, 5973–5989, https://doi.org/10.5194/acp-17-5973-2017, https://doi.org/10.5194/acp-17-5973-2017, 2017
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Detailed and accurate vertical distributions of cloud properties are essential to accurately calculate the surface radiative flux and to depict the mean climate state, and such information is more desirable in the Arctic due to its recent rapid changes and the challenging observation conditions. This study presents a feasible way to provide such information by blending cloud observations from surface and space-based instruments with the understanding of their respective strength and limitations.
Nathaniel B. Miller, Matthew D. Shupe, Christopher J. Cox, David Noone, P. Ola G. Persson, and Konrad Steffen
The Cryosphere, 11, 497–516, https://doi.org/10.5194/tc-11-497-2017, https://doi.org/10.5194/tc-11-497-2017, 2017
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A comprehensive observational dataset is assembled to investigate atmosphere–Greenland ice sheet interactions and characterize surface temperature variability. The amount the surface temperature warms, due to increases in cloud presence and/or elevated sun angle, varies throughout the annual cycle and is modulated by the responses of latent, sensible and ground heat fluxes. This observationally based study provides process-based relationships, which are useful for evaluation of climate models.
Bjorn Stevens, Stephanie Fiedler, Stefan Kinne, Karsten Peters, Sebastian Rast, Jobst Müsse, Steven J. Smith, and Thorsten Mauritsen
Geosci. Model Dev., 10, 433–452, https://doi.org/10.5194/gmd-10-433-2017, https://doi.org/10.5194/gmd-10-433-2017, 2017
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A simple analytic description of aerosol optical properties and their main effects on clouds is developed and described. The analytic description is easy to use and easy to modify and should aid experimentation to help understand how aerosol radiative and cloud interactions effect climate and circulation. The climatology is recommended for adoption by models participating in the sixth phase of the Coupled Model Intercomparison Project.
Robert A. Stillwell, Ryan R. Neely III, Jeffrey P. Thayer, Matthew D. Shupe, and Michael O'Neill
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-303, https://doi.org/10.5194/amt-2016-303, 2016
Revised manuscript not accepted
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This work explores the observation of Arctic mixed phase clouds by lidar and the consequences of mishandling lidar signals linking the signals to their geophysical interpretation. It concludes 3 points: 1) cloud phase identification is not only linked to cloud phase but other cloud properties, 2) having more than two polarization signals can be used to quality control data not possible with only two signals, and 3) phase retrievals with more than two polarizations enhance retrieval flexibility.
Evelyne Hamacher-Barth, Caroline Leck, and Kjell Jansson
Atmos. Chem. Phys., 16, 6577–6593, https://doi.org/10.5194/acp-16-6577-2016, https://doi.org/10.5194/acp-16-6577-2016, 2016
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Aerosol particles collected during the ASCOS expedition in the high Arctic in summer 2008 were examined with electron microscopy and elemental dispersive X-ray spectroscopy. The majority of particles consisted of marine gel matter accompanied by minor fractions of ammonium (bi)sulfate and internally mixed sulfur containing particles. Depending on their morphology, marine gel particles showed prevalence for either the ions Na+/K+ or Ca2+/Mg2+.
Mingxi Yang, Thomas G. Bell, Frances E. Hopkins, Vassilis Kitidis, Pierre W. Cazenave, Philip D. Nightingale, Margaret J. Yelland, Robin W. Pascal, John Prytherch, Ian M. Brooks, and Timothy J. Smyth
Atmos. Chem. Phys., 16, 5745–5761, https://doi.org/10.5194/acp-16-5745-2016, https://doi.org/10.5194/acp-16-5745-2016, 2016
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Coastal seas are sources of methane in the atmosphere and can fluctuate from emitting to absorbing carbon dioxide. Direct air–sea transport measurements of these two greenhouse gases in near shore regions remain scarce. From a recently established coastal atmospheric station on the south-west coast of the UK, we observed that the oceanic absorption of carbon dioxide peaked during the phytoplankton bloom, while methane emission varied with the tidal cycle, likely due to an estuary influence.
Claire Pettersen, Ralf Bennartz, Mark S. Kulie, Aronne J. Merrelli, Matthew D. Shupe, and David D. Turner
Atmos. Chem. Phys., 16, 4743–4756, https://doi.org/10.5194/acp-16-4743-2016, https://doi.org/10.5194/acp-16-4743-2016, 2016
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We examined four summers of data from a ground-based atmospheric science instrument suite at Summit Station, Greenland, to isolate the signature of the ice precipitation. By using a combination of instruments with different specialities, we identified a passive microwave signature of the ice precipitation. This ice signature compares well to models using synthetic data characteristic of the site.
P. Achtert, I. M. Brooks, B. J. Brooks, B. I. Moat, J. Prytherch, P. O. G. Persson, and M. Tjernström
Atmos. Meas. Tech., 8, 4993–5007, https://doi.org/10.5194/amt-8-4993-2015, https://doi.org/10.5194/amt-8-4993-2015, 2015
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Doppler lidar wind measurements were obtained during a 3-month Arctic cruise in summer 2014. Ship-motion effects were compensated by combining a commercial Doppler lidar with a custom-made motion-stabilisation platform. This enables the retrieval of wind profiles in the Arctic boundary layer with uncertainties comparable to land-based lidar measurements and standard radiosondes. The presented set-up has the potential to facilitate continuous ship-based wind profile measurements over the oceans.
E. Johansson, A. Devasthale, T. L'Ecuyer, A. M. L. Ekman, and M. Tjernström
Atmos. Chem. Phys., 15, 11557–11570, https://doi.org/10.5194/acp-15-11557-2015, https://doi.org/10.5194/acp-15-11557-2015, 2015
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Both radiative and latent heat components of total diabatic heating influence Indian monsoon dynamics. This study investigates radiative component in detail, focusing on various cloud types that have largest radiative impact during summer monsoon over the Indian subcontinent. The vertical structure of radiative heating and its intra-seasonal variability is investigated with particular emphasis on the upper troposphere and lower stratosphere (UTLS) region.
A. Solomon, G. Feingold, and M. D. Shupe
Atmos. Chem. Phys., 15, 10631–10643, https://doi.org/10.5194/acp-15-10631-2015, https://doi.org/10.5194/acp-15-10631-2015, 2015
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The maintenance of cloud ice production in Arctic mixed-phase stratocumulus is investigated in large eddy simulations that include a prognostic ice nuclei (IN) formulation and a diurnal cycle. It is demonstrated that IN recycling through subcloud sublimation prolongs ice production. Competing feedbacks between dynamical mixing and recycling are found to slow the rate of ice lost. The results of this study have important implications for the maintenance of phase partitioning in Arctic clouds.
J. Prytherch, M. J. Yelland, I. M. Brooks, D. J. Tupman, R. W. Pascal, B. I. Moat, and S. J. Norris
Atmos. Chem. Phys., 15, 10619–10629, https://doi.org/10.5194/acp-15-10619-2015, https://doi.org/10.5194/acp-15-10619-2015, 2015
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Signals at scales associated with wave and platform motion are often apparent in ship-based turbulent flux measurements, but it has been uncertain whether this is due to measurement error or to wind-wave interactions. We show that the signal has a dependence on horizontal ship velocity and that removing the signal reduces the dependence of the momentum flux on the orientation of the ship to the wind. We conclude that the signal is a bias due to time-varying motion-dependent flow distortion.
J. Heintzenberg, C. Leck, and P. Tunved
Atmos. Chem. Phys., 15, 6487–6502, https://doi.org/10.5194/acp-15-6487-2015, https://doi.org/10.5194/acp-15-6487-2015, 2015
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Particle size distributions from four summer cruises of the Swedish icebreaker Oden were combined with back trajectories and pack ice information in a cluster algorithm to investigate source areas and aerosol formation in the central Arctic. Five source regions and three aerosol types resulted. Long travel times over ice, combined with more open water conditions shortly before air mass arrival, seem to control the formation of ultrafine particles over the central Arctic pack ice.
C. Leck and E. Svensson
Atmos. Chem. Phys., 15, 2545–2568, https://doi.org/10.5194/acp-15-2545-2015, https://doi.org/10.5194/acp-15-2545-2015, 2015
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In the Arctic clouds are very important for determining the melting of the sea ice. The radiative properties of the optically thin Arctic clouds strongly depend on the number of particles available for water uptake. This study argues that the Köhler equation commonly used for simulating cloud droplet activation is not fully complete for describing the condensational growth of the interaction of the hydrophilic and hydrophobic entities on the structures of the airborne polymer gels present.
G. Sotiropoulou, J. Sedlar, M. Tjernström, M. D. Shupe, I. M. Brooks, and P. O. G. Persson
Atmos. Chem. Phys., 14, 12573–12592, https://doi.org/10.5194/acp-14-12573-2014, https://doi.org/10.5194/acp-14-12573-2014, 2014
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During ASCOS, clouds are more frequently decoupled from the surface than coupled to it; when coupling occurs it is primary driven by the cloud. Decoupled clouds have a bimodal structure; they are either weakly or strongly decoupled from the surface; the enhancement of the decoupling is possibly due to sublimation of precipitation. Stable clouds (no cloud-driven mixing) are also observed; those are optically thin, often single-phase liquid, with no or negligible precipitation (e.g. fog).
J. M. Intrieri, G. de Boer, M. D. Shupe, J. R. Spackman, J. Wang, P. J. Neiman, G. A. Wick, T. F. Hock, and R. E. Hood
Atmos. Meas. Tech., 7, 3917–3926, https://doi.org/10.5194/amt-7-3917-2014, https://doi.org/10.5194/amt-7-3917-2014, 2014
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In winter 2011, the Global Hawk unmanned aircraft system (UAS) was deployed over the Arctic to evaluate a UAS dropsonde system at high latitudes. Dropsondes deployed from the Global Hawk successfully obtained high-resolution profiles of temperature, pressure, humidity, and wind speed and direction information between the stratosphere and surface. During the 25-hour polar flight, the Global Hawk released 35 sondes between the North Slope of Alaska and 85° N latitude.
T. Vihma, R. Pirazzini, I. Fer, I. A. Renfrew, J. Sedlar, M. Tjernström, C. Lüpkes, T. Nygård, D. Notz, J. Weiss, D. Marsan, B. Cheng, G. Birnbaum, S. Gerland, D. Chechin, and J. C. Gascard
Atmos. Chem. Phys., 14, 9403–9450, https://doi.org/10.5194/acp-14-9403-2014, https://doi.org/10.5194/acp-14-9403-2014, 2014
J. Browse, K. S. Carslaw, G. W. Mann, C. E. Birch, S. R. Arnold, and C. Leck
Atmos. Chem. Phys., 14, 7543–7557, https://doi.org/10.5194/acp-14-7543-2014, https://doi.org/10.5194/acp-14-7543-2014, 2014
B. Sierau, R. Y.-W. Chang, C. Leck, J. Paatero, and U. Lohmann
Atmos. Chem. Phys., 14, 7409–7430, https://doi.org/10.5194/acp-14-7409-2014, https://doi.org/10.5194/acp-14-7409-2014, 2014
J. Sedlar and M. D. Shupe
Atmos. Chem. Phys., 14, 3461–3478, https://doi.org/10.5194/acp-14-3461-2014, https://doi.org/10.5194/acp-14-3461-2014, 2014
M. I. A. Berghof, G. P. Frank, S. Sjogren, and B. G. Martinsson
Atmos. Meas. Tech., 7, 877–886, https://doi.org/10.5194/amt-7-877-2014, https://doi.org/10.5194/amt-7-877-2014, 2014
M. Tjernström, C. Leck, C. E. Birch, J. W. Bottenheim, B. J. Brooks, I. M. Brooks, L. Bäcklin, R. Y.-W. Chang, G. de Leeuw, L. Di Liberto, S. de la Rosa, E. Granath, M. Graus, A. Hansel, J. Heintzenberg, A. Held, A. Hind, P. Johnston, J. Knulst, M. Martin, P. A. Matrai, T. Mauritsen, M. Müller, S. J. Norris, M. V. Orellana, D. A. Orsini, J. Paatero, P. O. G. Persson, Q. Gao, C. Rauschenberg, Z. Ristovski, J. Sedlar, M. D. Shupe, B. Sierau, A. Sirevaag, S. Sjogren, O. Stetzer, E. Swietlicki, M. Szczodrak, P. Vaattovaara, N. Wahlberg, M. Westberg, and C. R. Wheeler
Atmos. Chem. Phys., 14, 2823–2869, https://doi.org/10.5194/acp-14-2823-2014, https://doi.org/10.5194/acp-14-2823-2014, 2014
C. Wesslén, M. Tjernström, D. H. Bromwich, G. de Boer, A. M. L. Ekman, L.-S. Bai, and S.-H. Wang
Atmos. Chem. Phys., 14, 2605–2624, https://doi.org/10.5194/acp-14-2605-2014, https://doi.org/10.5194/acp-14-2605-2014, 2014
G. de Boer, M. D. Shupe, P. M. Caldwell, S. E. Bauer, O. Persson, J. S. Boyle, M. Kelley, S. A. Klein, and M. Tjernström
Atmos. Chem. Phys., 14, 427–445, https://doi.org/10.5194/acp-14-427-2014, https://doi.org/10.5194/acp-14-427-2014, 2014
C. Leck, Q. Gao, F. Mashayekhy Rad, and U. Nilsson
Atmos. Chem. Phys., 13, 12573–12588, https://doi.org/10.5194/acp-13-12573-2013, https://doi.org/10.5194/acp-13-12573-2013, 2013
P. Kupiszewski, C. Leck, M. Tjernström, S. Sjogren, J. Sedlar, M. Graus, M. Müller, B. Brooks, E. Swietlicki, S. Norris, and A. Hansel
Atmos. Chem. Phys., 13, 12405–12431, https://doi.org/10.5194/acp-13-12405-2013, https://doi.org/10.5194/acp-13-12405-2013, 2013
E. Hamacher-Barth, K. Jansson, and C. Leck
Atmos. Meas. Tech., 6, 3459–3475, https://doi.org/10.5194/amt-6-3459-2013, https://doi.org/10.5194/amt-6-3459-2013, 2013
A. Devasthale, J. Sedlar, T. Koenigk, and E. J. Fetzer
Atmos. Chem. Phys., 13, 7441–7450, https://doi.org/10.5194/acp-13-7441-2013, https://doi.org/10.5194/acp-13-7441-2013, 2013
K.-G. Karlsson, A. Riihelä, R. Müller, J. F. Meirink, J. Sedlar, M. Stengel, M. Lockhoff, J. Trentmann, F. Kaspar, R. Hollmann, and E. Wolters
Atmos. Chem. Phys., 13, 5351–5367, https://doi.org/10.5194/acp-13-5351-2013, https://doi.org/10.5194/acp-13-5351-2013, 2013
S. J. Norris, I. M. Brooks, B. I. Moat, M. J. Yelland, G. de Leeuw, R. W. Pascal, and B. Brooks
Ocean Sci., 9, 133–145, https://doi.org/10.5194/os-9-133-2013, https://doi.org/10.5194/os-9-133-2013, 2013
S. Sjogren, G. P. Frank, M. I. A. Berghof, and B. G. Martinsson
Atmos. Meas. Tech., 6, 349–357, https://doi.org/10.5194/amt-6-349-2013, https://doi.org/10.5194/amt-6-349-2013, 2013
D. A. J. Sproson, I. M. Brooks, and S. J. Norris
Atmos. Meas. Tech., 6, 323–335, https://doi.org/10.5194/amt-6-323-2013, https://doi.org/10.5194/amt-6-323-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
A set of methods to evaluate the below-cloud evaporation effect on local precipitation isotopic composition: a case study for Xi'an, China
Earth-system-model evaluation of cloud and precipitation occurrence for supercooled and warm clouds over the Southern Ocean's Macquarie Island
Pollution slightly enhances atmospheric cooling by low-level clouds in tropical West Africa
Investigating an indirect aviation effect on mid-latitude cirrus clouds – linking lidar-derived optical properties to in situ measurements
Investigating the vertical extent and short-wave radiative effects of the ice phase in Arctic summertime low-level clouds
Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer
Overview and statistical analysis of boundary layer clouds and precipitation over the western North-Atlantic Ocean
Aircraft observations of gravity wave activity and turbulence in the tropical tropopause layer: prevalence, influence on cirrus clouds, and comparison with global storm-resolving models
Differences in microphysical properties of cirrus at high and mid-latitudes
Influence of air mass origin on microphysical properties of low-level clouds in a subarctic environment
Sensitivity of convectively driven tropical tropopause cirrus properties to ice habits in high-resolution simulations
Upper-tropospheric slightly ice-subsaturated regions: frequency of occurrence and statistical evidence for the appearance of contrail cirrus
Examination of aerosol indirect effects during cirrus cloud evolution
In situ microphysics observations of intense pyroconvection from a large wildfire
Conditions favorable for secondary ice production in Arctic mixed-phase clouds
Interaction between cloud–radiation, atmospheric dynamics and thermodynamics based on observational data from GoAmazon 2014/15 and a cloud-resolving model
Sub-cloud Rain Evaporation in the North Atlantic Ocean
Snowfall in Northern Finland derives mostly from ice clouds
Observation of secondary ice production in clouds at low temperatures
In situ and satellite-based estimates of cloud properties and aerosol–cloud interactions over the southeast Atlantic Ocean
Ice fog observed at cirrus temperatures at Dome C, Antarctic Plateau
Life cycle of stratocumulus clouds over 1 year at the coast of the Atacama Desert
Experimental study on the evolution of droplet size distribution during the fog life cycle
Significant continental source of ice-nucleating particles at the tip of Chile's southernmost Patagonia region
Retrieving ice-nucleating particle concentration and ice multiplication factors using active remote sensing validated by in situ observations
Temporal and vertical distributions of the occurrence of cirrus clouds over a coastal station in the Indian monsoon region
Continental thunderstorm ground enhancement observed at an exceptionally low altitude
Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions
In situ observation of riming in mixed-phase clouds using the PHIPS probe
Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice-nucleating particles and instrument inter-comparison in the Hyytiälä boreal forest
North Atlantic Ocean SST-gradient-driven variations in aerosol and cloud evolution along Lagrangian cold-air outbreak trajectories
Factors affecting precipitation formation and precipitation susceptibility of marine stratocumulus with variable above- and below-cloud aerosol concentrations over the Southeast Atlantic
An assessment of macrophysical and microphysical cloud properties driving radiative forcing of shallow trade-wind clouds
High concentrations of ice crystals in upper-tropospheric tropical clouds: is there a link to biomass and fossil fuel combustion?
Atmospheric rivers and associated precipitation patterns during the ACLOUD and PASCAL campaigns near Svalbard (May–June 2017): case studies using observations, reanalyses, and a regional climate model
Mass of different snow crystal shapes derived from fall speed measurements
Measurement report: Impact of African aerosol particles on cloud evolution in a tropical montane cloud forest in the Caribbean
Annual exposure to polycyclic aromatic hydrocarbons in urban environments linked to wintertime wood-burning episodes
Reduced ice number concentrations in contrails from low-aromatic biofuel blends
Distinct impacts on precipitation by aerosol radiative effect over three different megacity regions of eastern China
Estimation of the terms acting on local 1 h surface temperature variations in Paris region: the specific contribution of clouds
Contrasting characteristics of open- and closed-cellular stratocumulus cloud in the eastern North Atlantic
Mass and density of individual frozen hydrometeors
Linear relationship between effective radius and precipitation water content near the top of convective clouds: measurement results from ACRIDICON–CHUVA campaign
Supercooled liquid water and secondary ice production in Kelvin–Helmholtz instability as revealed by radar Doppler spectra observations
Morning boundary layer conditions for shallow to deep convective cloud evolution during the dry season in the central Amazon
Analysis of aerosol–cloud interactions and their implications for precipitation formation using aircraft observations over the United Arab Emirates
Impact of wind pattern and complex topography on snow microphysics during International Collaborative Experiment for PyeongChang 2018 Olympic and Paralympic winter games (ICE-POP 2018)
Evaluation of simulated cloud liquid water in low clouds over the Beaufort Sea in the Arctic System Reanalysis using ARISE airborne in situ observations
Comprehensive quantification of height dependence of entrainment mixing between stratiform cloud top and environment
Meng Xing, Weiguo Liu, Jing Hu, and Zheng Wang
Atmos. Chem. Phys., 23, 9123–9136, https://doi.org/10.5194/acp-23-9123-2023, https://doi.org/10.5194/acp-23-9123-2023, 2023
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The below-cloud evaporation effect (BCE) on precipitation largely impacts the final isotopic composition. However, determining the BCE effect remains poorly constrained. Our work used a ΔdΔδ diagram to differentiate the below-cloud processes. Moreover, by comparing two different computing methods, we considered that both methods are suitable for evaluation the BCE, except for snowfall events. Overall, our work compiled a set of effective methods to evaluate the BCE effect.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
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Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
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The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2023-898, https://doi.org/10.5194/egusphere-2023-898, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North-Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study is well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice and precipitation.
Rachel Atlas and Christopher S. Bretherton
Atmos. Chem. Phys., 23, 4009–4030, https://doi.org/10.5194/acp-23-4009-2023, https://doi.org/10.5194/acp-23-4009-2023, 2023
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The tropical tropopause layer exists between the troposphere and the stratosphere in the tropics. Very thin cirrus clouds cool Earth's surface by scrubbing water vapor (a greenhouse gas) out of air parcels as they ascend through the tropical tropopause layer on their way to the stratosphere. We show observational evidence from aircraft that small-scale (< 100 km) gravity waves and turbulence increase the amount of ice in these clouds and may allow them to remove more water vapor from the air.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
EGUsphere, https://doi.org/10.5194/egusphere-2023-374, https://doi.org/10.5194/egusphere-2023-374, 2023
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In this study we show the differences in the microphysical properties between high latitudes (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and Central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region of cloud formation. We show that HL cirrus are characterized by lower concentration of larger ice crystals compared to ML cirrus.
Konstantinos Matthaios Doulgeris, Ville Vakkari, Ewan J. O'Connor, Veli-Matti Kerminen, Heikki Lihavainen, and David Brus
Atmos. Chem. Phys., 23, 2483–2498, https://doi.org/10.5194/acp-23-2483-2023, https://doi.org/10.5194/acp-23-2483-2023, 2023
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We investigated how different long-range-transported air masses can affect the microphysical properties of low-level clouds in a clean subarctic environment. A connection was revealed. Higher values of cloud droplet number concentrations were related to continental air masses, whereas the lowest values of number concentrations were related to marine air masses. These were characterized by larger cloud droplets. Clouds in all regions were sensitive to increases in cloud number concentration.
Fayçal Lamraoui, Martina Krämer, Armin Afchine, Adam B. Sokol, Sergey Khaykin, Apoorva Pandey, and Zhiming Kuang
Atmos. Chem. Phys., 23, 2393–2419, https://doi.org/10.5194/acp-23-2393-2023, https://doi.org/10.5194/acp-23-2393-2023, 2023
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Cirrus in the tropical tropopause layer (TTL) can play a key role in vertical transport. We investigate the role of different cloud regimes and the associated ice habits in regulating the properties of the TTL. We use high-resolution numerical experiments at the scales of large-eddy simulations (LESs) and aircraft measurements. We found that LES-scale parameterizations that predict ice shape are crucial for an accurate representation of TTL cirrus and thus the associated (de)hydration process.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Flor Vanessa Maciel, Minghui Diao, and Ryan Patnaude
Atmos. Chem. Phys., 23, 1103–1129, https://doi.org/10.5194/acp-23-1103-2023, https://doi.org/10.5194/acp-23-1103-2023, 2023
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Aerosol indirect effects on cirrus clouds are investigated during cirrus evolution, using global-scale in situ observations and climate model simulations. As cirrus evolves, the mechanisms to form ice crystals also change with time. Both small and large aerosols are found to affect cirrus properties. Southern Hemisphere cirrus appears to be more sensitive to additional aerosols. The climate model underestimates ice crystal mass, likely due to biases of relative humidity and vertical velocity.
David E. Kingsmill, Jeffrey R. French, and Neil P. Lareau
Atmos. Chem. Phys., 23, 1–21, https://doi.org/10.5194/acp-23-1-2023, https://doi.org/10.5194/acp-23-1-2023, 2023
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This study uses in situ aircraft measurements to characterize the size and shape distributions of 10 µm to 6 mm diameter particles observed during six penetrations of wildfire-induced pyroconvection. Particles sampled in one penetration of a smoke plume are most likely pyrometeors composed of ash. The other penetrations are through pyrocumulus clouds where particle composition is most likely a combination of hydrometeors (ice particles) and pyrometeors (ash).
Julie Thérèse Pasquier, Jan Henneberger, Fabiola Ramelli, Annika Lauber, Robert Oscar David, Jörg Wieder, Tim Carlsen, Rosa Gierens, Marion Maturilli, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 15579–15601, https://doi.org/10.5194/acp-22-15579-2022, https://doi.org/10.5194/acp-22-15579-2022, 2022
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It is important to understand how ice crystals and cloud droplets form in clouds, as their concentrations and sizes determine the exact radiative properties of the clouds. Normally, ice crystals form from aerosols, but we found evidence for the formation of additional ice crystals from the original ones over a large temperature range within Arctic clouds. In particular, additional ice crystals were formed during collisions of several ice crystals or during the freezing of large cloud droplets.
Layrson J. M. Gonçalves, Simone M. S. C. Coelho, Paulo Y. Kubota, and Dayana C. Souza
Atmos. Chem. Phys., 22, 15509–15526, https://doi.org/10.5194/acp-22-15509-2022, https://doi.org/10.5194/acp-22-15509-2022, 2022
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This research aims to study the environmental conditions that are favorable and not favorable to cloud formation, in this case specifically for the Amazon region. The results found in this research will be used to improve the representation of clouds in numerical models that are used in weather and climate prediction. In general, it is expected that with better knowledge regarding the cloud–radiation interaction, it is possible to make a better forecast of weather and climate.
Mampi Sarkar, Adriana Bailey, Peter Blossey, Simon P. de Szoeke, David Noone, Estefania Quinones Melendez, Mason Leandro, and Patrick Chuang
EGUsphere, https://doi.org/10.5194/egusphere-2022-1143, https://doi.org/10.5194/egusphere-2022-1143, 2022
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We study rain evaporation below marine clouds using observations collected during the Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC). 65 % of the rain evaporate completely due to smaller raindrops falling in a dry surface layer. Similarly, heavier rain only reaches the surface if larger raindrops at cloud base were to fall into a moister surface layer, showing that rain evaporation is controlled by both microphysical and thermodynamic processes in the sub-cloud layer.
Claudia Mignani, Lukas Zimmermann, Rigel Kivi, Alexis Berne, and Franz Conen
Atmos. Chem. Phys., 22, 13551–13568, https://doi.org/10.5194/acp-22-13551-2022, https://doi.org/10.5194/acp-22-13551-2022, 2022
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We determined over the course of 8 winter months the phase of clouds associated with snowfall in Northern Finland using radiosondes and observations of ice particle habits at ground level. We found that precipitating clouds were extending from near ground to at least 2.7 km altitude and approximately three-quarters of them were likely glaciated. Possible moisture sources and ice formation processes are discussed.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
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The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Étienne Vignon, Lea Raillard, Christophe Genthon, Massimo Del Guasta, Andrew J. Heymsfield, Jean-Baptiste Madeleine, and Alexis Berne
Atmos. Chem. Phys., 22, 12857–12872, https://doi.org/10.5194/acp-22-12857-2022, https://doi.org/10.5194/acp-22-12857-2022, 2022
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The near-surface atmosphere over the Antarctic Plateau is cold and pristine and resembles to a certain extent the high troposphere where cirrus clouds form. In this study, we use innovative humidity measurements at Concordia Station to study the formation of ice fogs at temperatures <−40°C. We provide observational evidence that ice fogs can form through the homogeneous freezing of solution aerosols, a common nucleation pathway for cirrus clouds.
Jan H. Schween, Camilo del Rio, Juan-Luis García, Pablo Osses, Sarah Westbrook, and Ulrich Löhnert
Atmos. Chem. Phys., 22, 12241–12267, https://doi.org/10.5194/acp-22-12241-2022, https://doi.org/10.5194/acp-22-12241-2022, 2022
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Marine stratocumulus clouds of the eastern Pacific play an essential role in the Earth's climate. These clouds form the major source of water to parts of the extreme dry Atacama Desert at the northern coast of Chile. For the first time these clouds are observed over a whole year with three remote sensing instruments. It is shown how these clouds are influenced by the land–sea wind system and the distribution of ocean temperatures.
Marie Mazoyer, Frédéric Burnet, and Cyrielle Denjean
Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, https://doi.org/10.5194/acp-22-11305-2022, 2022
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The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
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Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Saleem Ali, Sanjay Kumar Mehta, Aravindhavel Ananthavel, and Tondapu Venkata Ramesh Reddy
Atmos. Chem. Phys., 22, 8321–8342, https://doi.org/10.5194/acp-22-8321-2022, https://doi.org/10.5194/acp-22-8321-2022, 2022
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Multiple cirrus clouds frequently occur over regions of deep convection in the tropics. Tropical convection has a strong diurnal pattern, with peaks in the afternoon to early evening, over the continents. Continuous micropulse lidar observations over a coastal station in the Indian monsoon region enable us, for the first time, to demonstrate a robust diurnal pattern of single and multiple cirrus occurrences, with peaks during the late afternoon and early morning hours, respectively.
Ivana Kolmašová, Ondřej Santolík, Jakub Šlegl, Jana Popová, Zbyněk Sokol, Petr Zacharov, Ondřej Ploc, Gerhard Diendorfer, Ronald Langer, Radek Lán, and Igor Strhárský
Atmos. Chem. Phys., 22, 7959–7973, https://doi.org/10.5194/acp-22-7959-2022, https://doi.org/10.5194/acp-22-7959-2022, 2022
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Gamma ray radiation related to thunderstorms was previously observed at the high-altitude mountain observatories or on the western coast of Japan, usually being terminated by lightning discharges. We show unusual observations of gamma rays at an altitude below 1000 m, coinciding with peculiar rapid variations in the vertical electric field, which are linked to inverted intracloud lightning discharges. This indicates that a strong, lower positive-charge region was present inside the thundercloud.
Cuiqi Zhang, Zhijun Wu, Jingchuan Chen, Jie Chen, Lizi Tang, Wenfei Zhu, Xiangyu Pei, Shiyi Chen, Ping Tian, Song Guo, Limin Zeng, Min Hu, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7539–7556, https://doi.org/10.5194/acp-22-7539-2022, https://doi.org/10.5194/acp-22-7539-2022, 2022
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The immersion ice nucleation effectiveness of aerosols from multiple sources in the urban environment remains elusive. In this study, we demonstrate that the immersion ice-nucleating particle (INP) concentration increased dramatically during a dust event in an urban atmosphere. Pollutant aerosols, including inorganic salts formed through secondary transformation (SIA) and black carbon (BC), might not act as effective INPs under mixed-phase cloud conditions.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Chem. Phys., 22, 7087–7103, https://doi.org/10.5194/acp-22-7087-2022, https://doi.org/10.5194/acp-22-7087-2022, 2022
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Riming, i.e., the accretion of small droplets on the surface of ice particles via collision, is one of the major uncertainties in model prediction of mixed-phase clouds. We discuss the occurrence (up to 50% of particles) and aging of rimed ice particles and show correlations of the occurrence and the degree of riming with ambient meteorological parameters using data gathered by the Particle Habit Imaging and Polar Scattering (PHIPS) probe during three airborne in situ field campaigns.
Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 5117–5145, https://doi.org/10.5194/acp-22-5117-2022, https://doi.org/10.5194/acp-22-5117-2022, 2022
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The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Matthew D. Brown, Ewan C. Crosbie, Francesca Gallo, Johnathan W. Hair, Chris A. Hostetler, Carolyn E. Jordan, Claire E. Robinson, Amy Jo Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Luke D. Ziemba, Georges Saliba, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Peter Gaube, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 22, 2795–2815, https://doi.org/10.5194/acp-22-2795-2022, https://doi.org/10.5194/acp-22-2795-2022, 2022
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Atmospheric particle concentrations impact clouds, which strongly impact the amount of sunlight reflected back into space and the overall climate. Measurements of particles over the ocean are rare and expensive to collect, so models are necessary to fill in the gaps by simulating both particle and clouds. However, some measurements are needed to test the accuracy of the models. Here, we measure changes in particles in different weather conditions, which are ideal for comparison with models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Rose M. Miller, and Jennifer D. Small Griswold
Atmos. Chem. Phys., 22, 2769–2793, https://doi.org/10.5194/acp-22-2769-2022, https://doi.org/10.5194/acp-22-2769-2022, 2022
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This study evaluates the impact of biomass burning aerosols on precipitation in marine stratocumulus clouds using observations from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign over the Southeast Atlantic. Instances of contact and separation between aerosol and cloud layers show polluted clouds have a lower precipitation rate and a lower precipitation susceptibility. This information will help improve cloud representation in Earth system models.
Anna E. Luebke, André Ehrlich, Michael Schäfer, Kevin Wolf, and Manfred Wendisch
Atmos. Chem. Phys., 22, 2727–2744, https://doi.org/10.5194/acp-22-2727-2022, https://doi.org/10.5194/acp-22-2727-2022, 2022
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A combination of aircraft and satellite observations is used to show how the characteristics of tropical shallow clouds interact with incoming and outgoing energy. A complete depiction of these clouds is challenging to obtain, but such data are useful for understanding how models can correctly represent them. The amount of cloud is found to be the most important factor, while other cloud characteristics become increasingly impactful when more cloud is present.
Graciela B. Raga, Darrel Baumgardner, Blanca Rios, Yanet Díaz-Esteban, Alejandro Jaramillo, Martin Gallagher, Bastien Sauvage, Pawel Wolff, and Gary Lloyd
Atmos. Chem. Phys., 22, 2269–2292, https://doi.org/10.5194/acp-22-2269-2022, https://doi.org/10.5194/acp-22-2269-2022, 2022
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The In-Service Aircraft for a Global Observing System (IAGOS) is a small fleet of commercial aircraft that carry a suite of meteorological, gas, aerosol, and cloud sensors and have been measuring worldwide for almost 9 years, since late 2011. Extreme ice events (EIEs) have been identified from the IAGOS cloud measurements and linked to surface emissions for biomass and fossil fuel consumption. The results reported here are highly relevant for climate change and flight operations forecasting.
Carolina Viceto, Irina V. Gorodetskaya, Annette Rinke, Marion Maturilli, Alfredo Rocha, and Susanne Crewell
Atmos. Chem. Phys., 22, 441–463, https://doi.org/10.5194/acp-22-441-2022, https://doi.org/10.5194/acp-22-441-2022, 2022
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We focus on anomalous moisture transport events known as atmospheric rivers (ARs). During ACLOUD and PASCAL, three AR events were identified: 30 May, 6 June, and 9 June 2017. We explore their spatio-temporal evolution and precipitation patterns using measurements, reanalyses, and a model. We show the importance of the following: Atlantic and Siberian pathways during spring–summer in the Arctic, AR-associated heat/moisture increase, precipitation phase transition, and high-resolution datasets.
Sandra Vázquez-Martín, Thomas Kuhn, and Salomon Eliasson
Atmos. Chem. Phys., 21, 18669–18688, https://doi.org/10.5194/acp-21-18669-2021, https://doi.org/10.5194/acp-21-18669-2021, 2021
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High-resolution top- and side-view images of snow ice particles taken by the D-ICI instrument are used to determine the shape; size; cross-sectional area; fall speed; and, based upon these properties, the mass of the individual snow particles. The study analyses the relationships between these fundamental properties as a function of particle shape and highlights that the choice of size parameter, maximum dimension or another characteristic length, is crucial when relating fall speed to mass.
Elvis Torres-Delgado, Darrel Baumgardner, and Olga L. Mayol-Bracero
Atmos. Chem. Phys., 21, 18011–18027, https://doi.org/10.5194/acp-21-18011-2021, https://doi.org/10.5194/acp-21-18011-2021, 2021
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African dust aerosols can travel thousands of kilometers and reach the Caribbean and other places, where they can serve as ice and cloud condensation nuclei and alter precipitation patterns. Cloud microphysical properties (droplet number and size) were measured in a Caribbean tropical montane cloud forest along with models and satellite products. The results of the study suggest that meteorology and air mass history are more important for cloud processes than aerosols transported from Africa.
Irini Tsiodra, Georgios Grivas, Kalliopi Tavernaraki, Aikaterini Bougiatioti, Maria Apostolaki, Despina Paraskevopoulou, Alexandra Gogou, Constantine Parinos, Konstantina Oikonomou, Maria Tsagkaraki, Pavlos Zarmpas, Athanasios Nenes, and Nikolaos Mihalopoulos
Atmos. Chem. Phys., 21, 17865–17883, https://doi.org/10.5194/acp-21-17865-2021, https://doi.org/10.5194/acp-21-17865-2021, 2021
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We analyze observations from year-long measurements at Athens, Greece. Nighttime wintertime PAH levels are 4 times higher than daytime, and wintertime values are 15 times higher than summertime. Biomass burning aerosol during wintertime pollution events is responsible for these significant wintertime enhancements and accounts for 43 % of the population exposure to PAH carcinogenic risk. Biomass burning poses additional health risks beyond those associated with the high PM levels that develop.
Tiziana Bräuer, Christiane Voigt, Daniel Sauer, Stefan Kaufmann, Valerian Hahn, Monika Scheibe, Hans Schlager, Felix Huber, Patrick Le Clercq, Richard H. Moore, and Bruce E. Anderson
Atmos. Chem. Phys., 21, 16817–16826, https://doi.org/10.5194/acp-21-16817-2021, https://doi.org/10.5194/acp-21-16817-2021, 2021
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Over half of aviation climate impact is caused by contrails. Biofuels can reduce the ice crystal numbers in contrails and mitigate the climate impact. The experiment ECLIF II/NDMAX in 2018 assessed the effects of biofuels on contrails and aviation emissions. The NASA DC-8 aircraft performed measurements inside the contrail of the DLR A320. One reference fuel and two blends of the biofuel HEFA and kerosene are analysed. We find a max reduction of contrail ice numbers through biofuel use of 40 %.
Yue Sun and Chuanfeng Zhao
Atmos. Chem. Phys., 21, 16555–16574, https://doi.org/10.5194/acp-21-16555-2021, https://doi.org/10.5194/acp-21-16555-2021, 2021
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Using high-resolution multi-year warm season data, the influence of aerosol on precipitation time over the North China Plain (NCP), Yangtze River Delta (YRD), and Pearl River Delta (PRD) is investigated. Aerosol amount and type have significant influence on precipitation time: precipitation start time is advanced by 3 h in the NCP, delayed 2 h in the PRD, and negligibly changed in the YRD. Aerosol impact on precipitation is also influenced by precipitation type and meteorological conditions.
Oscar Javier Rojas Muñoz, Marjolaine Chiriaco, Sophie Bastin, and Justine Ringard
Atmos. Chem. Phys., 21, 15699–15723, https://doi.org/10.5194/acp-21-15699-2021, https://doi.org/10.5194/acp-21-15699-2021, 2021
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A method is developed and evaluated to quantify each process that affects hourly 2 m temperature variations on a local scale, based almost exclusively on observations retrieved from an observatory near the Paris region. Each term involved in surface temperature variations is estimated, and its contribution and importance are also assessed. It is found that clouds are the main modulator on hourly temperature variations for most hours of the day, and thus their characterization is addressed.
Michael P. Jensen, Virendra P. Ghate, Dié Wang, Diana K. Apoznanski, Mary J. Bartholomew, Scott E. Giangrande, Karen L. Johnson, and Mandana M. Thieman
Atmos. Chem. Phys., 21, 14557–14571, https://doi.org/10.5194/acp-21-14557-2021, https://doi.org/10.5194/acp-21-14557-2021, 2021
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This work compares the large-scale meteorology, cloud, aerosol, precipitation, and thermodynamics of closed- and open-cell cloud organizations using long-term observations from the astern North Atlantic. Open-cell cases are associated with cold-air outbreaks and occur in deeper boundary layers, with stronger winds and higher rain rates compared to closed-cell cases. These results offer important benchmarks for model representation of boundary layer clouds in this climatically important region.
Karlie N. Rees, Dhiraj K. Singh, Eric R. Pardyjak, and Timothy J. Garrett
Atmos. Chem. Phys., 21, 14235–14250, https://doi.org/10.5194/acp-21-14235-2021, https://doi.org/10.5194/acp-21-14235-2021, 2021
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Accurate predictions of weather and climate require descriptions of the mass and density of snowflakes as a function of their size. Few measurements have been obtained to date because snowflakes are so small and fragile. This article describes results from a new instrument that automatically measures individual snowflake size, mass, and density. Key findings are that small snowflakes have much lower densities than is often assumed and that snowflake density increases with temperature.
Ramon Campos Braga, Daniel Rosenfeld, Ovid O. Krüger, Barbara Ervens, Bruna A. Holanda, Manfred Wendisch, Trismono Krisna, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 14079–14088, https://doi.org/10.5194/acp-21-14079-2021, https://doi.org/10.5194/acp-21-14079-2021, 2021
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Quantifying the precipitation within clouds is crucial for our understanding of the Earth's hydrological cycle. Using in situ measurements of cloud and rain properties over the Amazon Basin and Atlantic Ocean, we show here a linear relationship between the effective radius (re) and precipitation water content near the tops of convective clouds for different pollution states and temperature levels. Our results emphasize the role of re to determine both initiation and amount of precipitation.
Haoran Li, Alexei Korolev, and Dmitri Moisseev
Atmos. Chem. Phys., 21, 13593–13608, https://doi.org/10.5194/acp-21-13593-2021, https://doi.org/10.5194/acp-21-13593-2021, 2021
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Kelvin–Helmholtz (K–H) clouds embedded in a stratiform precipitation event were uncovered via radar Doppler spectral analysis. Given the unprecedented detail of the observations, we show that multiple populations of secondary ice columns were generated in the pockets where larger cloud droplets are formed and not at some constant level within the cloud. Our results highlight that the K–H instability is favorable for liquid droplet growth and secondary ice formation.
Alice Henkes, Gilberto Fisch, Luiz A. T. Machado, and Jean-Pierre Chaboureau
Atmos. Chem. Phys., 21, 13207–13225, https://doi.org/10.5194/acp-21-13207-2021, https://doi.org/10.5194/acp-21-13207-2021, 2021
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The Amazonian boundary layer is investigated during the dry season in order to better understand the processes that occur between night and day until the stage where shallow cumulus clouds become deep. Observations show that shallow to deep clouds are characterized by a shorter morning transition stage (e.g., the time needed to eliminate the stable boundary layer inversion), while higher humidity above the boundary layer favors the evolution from shallow to deep cumulus clouds.
Youssef Wehbe, Sarah A. Tessendorf, Courtney Weeks, Roelof Bruintjes, Lulin Xue, Roy Rasmussen, Paul Lawson, Sarah Woods, and Marouane Temimi
Atmos. Chem. Phys., 21, 12543–12560, https://doi.org/10.5194/acp-21-12543-2021, https://doi.org/10.5194/acp-21-12543-2021, 2021
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The role of dust aerosols as ice-nucleating particles is well established in the literature, whereas their role as cloud condensation nuclei is less understood, particularly in polluted desert environments. We analyze coincident aerosol size distributions and cloud particle imagery collected over the UAE with a research aircraft. Despite the presence of ultra-giant aerosol sizes associated with dust, an active collision–coalescence process is not observed within the limited depths of warm cloud.
Kwonil Kim, Wonbae Bang, Eun-Chul Chang, Francisco J. Tapiador, Chia-Lun Tsai, Eunsil Jung, and Gyuwon Lee
Atmos. Chem. Phys., 21, 11955–11978, https://doi.org/10.5194/acp-21-11955-2021, https://doi.org/10.5194/acp-21-11955-2021, 2021
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This study analyzes the microphysical characteristics of snow in complex terrain and the nearby ocean according to topography and wind pattern during the ICE-POP 2018 campaign. The observations from collocated vertically pointing radars and disdrometers indicate that the riming in the mountainous region is likely caused by a strong shear and turbulence. The different behaviors of aggregation and riming were found by three different synoptic patterns (air–sea interaction, cold low, and warm low).
J. Brant Dodson, Patrick C. Taylor, Richard H. Moore, David H. Bromwich, Keith M. Hines, Kenneth L. Thornhill, Chelsea A. Corr, Bruce E. Anderson, Edward L. Winstead, and Joseph R. Bennett
Atmos. Chem. Phys., 21, 11563–11580, https://doi.org/10.5194/acp-21-11563-2021, https://doi.org/10.5194/acp-21-11563-2021, 2021
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Aircraft in situ observations of low-level Beaufort Sea cloud properties and thermodynamics from the ARISE campaign are compared with the Arctic System Reanalysis (ASR) to better understand deficiencies in simulated clouds. ASR produces too little cloud water, which coincides with being too warm and dry. In addition, ASR struggles to produce cloud water even in favorable thermodynamic conditions. A random sampling experiment also shows the effects of the limited aircraft sampling on the results.
Sinan Gao, Chunsong Lu, Yangang Liu, Seong Soo Yum, Jiashan Zhu, Lei Zhu, Neel Desai, Yongfeng Ma, and Shang Wu
Atmos. Chem. Phys., 21, 11225–11241, https://doi.org/10.5194/acp-21-11225-2021, https://doi.org/10.5194/acp-21-11225-2021, 2021
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Only a few studies have been focused on the vertical variation of entrainment mixing with low resolutions which are crucial to cloud-related processes. A sawtooth pattern allows for an examination of mixing with high vertical resolution. A new measure is introduced to estimate entrainment mixing to overcome difficulties in existing measures, where vertical profile indicates that entrainment mixing becomes more homogeneous with decreasing altitudes, consistent with the dynamical measures.
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