Articles | Volume 24, issue 16
https://doi.org/10.5194/acp-24-9045-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-9045-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Aug 2024
Research article |
| 20 Aug 2024
| 20 Aug 2024
International airport emissions and their impact on local air quality: chemical speciation of ambient aerosols at Madrid–Barajas Airport during the AVIATOR campaign
Saleh Alzahrani
CORRESPONDING AUTHOR
Department of Earth and Environmental Sciences, University of Manchester, Manchester, UK
Doğuşhan Kılıç
Department of Earth and Environmental Sciences, University of Manchester, Manchester, UK
National Centre for Atmospheric Science, University of Manchester, Manchester, UK
Michael Flynn
Department of Earth and Environmental Sciences, University of Manchester, Manchester, UK
Paul I. Williams
Department of Earth and Environmental Sciences, University of Manchester, Manchester, UK
National Centre for Atmospheric Science, University of Manchester, Manchester, UK
James Allan
Department of Earth and Environmental Sciences, University of Manchester, Manchester, UK
National Centre for Atmospheric Science, University of Manchester, Manchester, UK
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Chenjie Yu, Paola Formenti, Joel F. de Brito, Astrid Bauville, Antonin Bergé, Hichem Bouzidi, Mathieu Cazaunau, Manuela Cirtog, Claudia Di Biagio, Ludovico Di Antonio, Cécile Gaimoz, Franck Maisonneuve, Pascal Zapf, Tobias Seubert, Simone T. Andersen, Patrick Dewald, Gunther N. T. E. Türk, John N. Crowley, Alexandre Kukui, Chaoyang Xue, Cyrielle Denjean, Olivier Garrouste, Jean-Claude Etienne, Huihui Wu, James D. Allan, Dantong Liu, Yangzhou Wu, Christopher Cantrell, and Vincent Michoud
EGUsphere, https://doi.org/10.5194/egusphere-2025-2667, https://doi.org/10.5194/egusphere-2025-2667, 2025
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We presented a field measurement in a Paris suburban forest region to characterise the impacts of photochemical aging process on aerosol physical chemical properties. Photochemical production of organic aerosols increased forest fine particle mass and significantly enhanced absorption of short-wavelength sunlight. This study highlights the critical need to incorporate light absorbing carbonaceous particles formation mechanisms into models to accurately simulate their direct radiative impacts.
Huihui Wu, Nicholas Marsden, Paul Connolly, Michael Flynn, Paul I. Williams, Declan Finney, Kezhen Hu, Graeme J. Nott, Navaneeth Thamban, Keith Bower, Alan Blyth, Martin Gallagher, and Hugh Coe
EGUsphere, https://doi.org/10.5194/egusphere-2025-2600, https://doi.org/10.5194/egusphere-2025-2600, 2025
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Airborne observations over the Magdalena Mountains in New Mexico underscore the combined influence of meteorological conditions and aerosol characteristics on the development of deep-convective clouds under different flow regimes. Model-observation comparisons emphasize the critical role of aerosol entrainment in reproducing the observed broad cloud droplet spectra. This study provides valuable constraints for improving parameterizations of aerosol-cloud interactions in deep convective systems.
Sebastian Diez, Stuart Lacy, Hugh Coe, Josefina Urquiza, Max Priestman, Michael Flynn, Nicholas Marsden, Nicholas A. Martin, Stefan Gillott, Thomas Bannan, and Pete M. Edwards
Atmos. Meas. Tech., 17, 3809–3827, https://doi.org/10.5194/amt-17-3809-2024, https://doi.org/10.5194/amt-17-3809-2024, 2024
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In this paper we present an overview of the QUANT project, which to our knowledge is one of the largest evaluations of commercial sensors to date. The objective was to evaluate the performance of a range of commercial products and also to nourish the different applications in which these technologies can offer relevant information.
Gary Lloyd, Alan Blyth, Zhiqiang Cui, Thomas Choularton, Keith Bower, Martin Gallagher, Michael Flynn, Nicholas Marsden, Leif Denby, and Peter Gallimore
EGUsphere, https://doi.org/10.5194/egusphere-2024-142, https://doi.org/10.5194/egusphere-2024-142, 2024
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Clouds that develop in the tropical trade-wind regions are extensive and persistent in nature. They are important for understanding how the magnitude of warming by these cloud systems might change in a warming climate. This paper describes measurements of common cloud types in these regions (shallow cumulus clouds) and the way in which they produce rainfall. During different periods, with different amounts of particulate in the air, the characteristics of the clouds were very different.
Declan L. Finney, Alan M. Blyth, Martin Gallagher, Huihui Wu, Graeme J. Nott, Michael I. Biggerstaff, Richard G. Sonnenfeld, Martin Daily, Dan Walker, David Dufton, Keith Bower, Steven Böing, Thomas Choularton, Jonathan Crosier, James Groves, Paul R. Field, Hugh Coe, Benjamin J. Murray, Gary Lloyd, Nicholas A. Marsden, Michael Flynn, Kezhen Hu, Navaneeth M. Thamban, Paul I. Williams, Paul J. Connolly, James B. McQuaid, Joseph Robinson, Zhiqiang Cui, Ralph R. Burton, Gordon Carrie, Robert Moore, Steven J. Abel, Dave Tiddeman, and Graydon Aulich
Earth Syst. Sci. Data, 16, 2141–2163, https://doi.org/10.5194/essd-16-2141-2024, https://doi.org/10.5194/essd-16-2141-2024, 2024
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The DCMEX (Deep Convective Microphysics Experiment) project undertook an aircraft- and ground-based measurement campaign of New Mexico deep convective clouds during July–August 2022. The campaign coordinated a broad range of instrumentation measuring aerosol, cloud physics, radar signals, thermodynamics, dynamics, electric fields, and weather. The project's objectives included the utilisation of these data with satellite observations to study the anvil cloud radiative effect.
Ernesto Reyes-Villegas, Douglas Lowe, Jill S. Johnson, Kenneth S. Carslaw, Eoghan Darbyshire, Michael Flynn, James D. Allan, Hugh Coe, Ying Chen, Oliver Wild, Scott Archer-Nicholls, Alex Archibald, Siddhartha Singh, Manish Shrivastava, Rahul A. Zaveri, Vikas Singh, Gufran Beig, Ranjeet Sokhi, and Gordon McFiggans
Atmos. Chem. Phys., 23, 5763–5782, https://doi.org/10.5194/acp-23-5763-2023, https://doi.org/10.5194/acp-23-5763-2023, 2023
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Organic aerosols (OAs), their sources and their processes remain poorly understood. The volatility basis set (VBS) approach, implemented in air quality models such as WRF-Chem, can be a useful tool to describe primary OA (POA) production and aging. However, the main disadvantage is its complexity. We used a Gaussian process simulator to reproduce model results and to estimate the sources of model uncertainty. We do this by comparing the outputs with OA observations made at Delhi, India, in 2018.
John W. Halfacre, Jordan Stewart, Scott C. Herndon, Joseph R. Roscioli, Christoph Dyroff, Tara I. Yacovitch, Michael Flynn, Stephen J. Andrews, Steven S. Brown, Patrick R. Veres, and Pete M. Edwards
Atmos. Meas. Tech., 16, 1407–1429, https://doi.org/10.5194/amt-16-1407-2023, https://doi.org/10.5194/amt-16-1407-2023, 2023
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This study details a new sampling method for the optical detection of hydrogen chloride (HCl). HCl is an important atmospheric reservoir for chlorine atoms, which can affect nitrogen oxide cycling and the lifetimes of volatile organic compounds and ozone. However, HCl has a high affinity for interacting with surfaces, thereby preventing fast, quantitative measurements. The sampling technique in this study minimizes these surface interactions and provides a high-quality measurement of HCl.
Aristeidis Voliotis, Mao Du, Yu Wang, Yunqi Shao, Thomas J. Bannan, Michael Flynn, Spyros N. Pandis, Carl J. Percival, M. Rami Alfarra, and Gordon McFiggans
Atmos. Chem. Phys., 22, 13677–13693, https://doi.org/10.5194/acp-22-13677-2022, https://doi.org/10.5194/acp-22-13677-2022, 2022
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The addition of a low-yield precursor to the reactive mixture of aVOC and bVOC can increase or decrease the SOA volatility that is system-dependent. Therefore, the SOA volatility of the mixtures cannot always be predicted based on the additivity. In complex mixtures the formation of lower-volatility products likely outweighs the formation of products with higher volatility. The unique products of each mixture contribute significantly to the signal, suggesting interactions can be important.
Sebastian Diez, Stuart E. Lacy, Thomas J. Bannan, Michael Flynn, Tom Gardiner, David Harrison, Nicholas Marsden, Nicholas A. Martin, Katie Read, and Pete M. Edwards
Atmos. Meas. Tech., 15, 4091–4105, https://doi.org/10.5194/amt-15-4091-2022, https://doi.org/10.5194/amt-15-4091-2022, 2022
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Regardless of the cost of the measuring instrument, there are no perfect measurements. For this reason, we compare the quality of the information provided by cheap devices when they are used to measure air pollutants and we try to emphasise that before judging the potential usefulness of the devices, the user must specify his own needs. Since commonly used performance indices/metrics can be misleading in qualifying this, we propose complementary visual analysis to the more commonly used metrics.
Chenjie Yu, Dantong Liu, Kang Hu, Ping Tian, Yangzhou Wu, Delong Zhao, Huihui Wu, Dawei Hu, Wenbo Guo, Qiang Li, Mengyu Huang, Deping Ding, and James D. Allan
Atmos. Chem. Phys., 22, 4375–4391, https://doi.org/10.5194/acp-22-4375-2022, https://doi.org/10.5194/acp-22-4375-2022, 2022
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In this study, we applied a new technique to investigate the aerosol properties on both a mass and number basis and CCN abilities in Beijing suburban regions. The size-resolved aerosol chemical compositions and CCN activation measurement enable a detailed analysis of BC-containing particle hygroscopicity and its size-dependent contribution to the CCN activation. The results presented in this study will affect future models and human health studies.
Waldemar Schledewitch, Gary Lloyd, Keith Bower, Thomas Choularton, Michael Flynn, and Martin Gallagher
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-69, https://doi.org/10.5194/acp-2022-69, 2022
Publication in ACP not foreseen
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Ice crystals on the surface of ice and snow covered terrain are thought to be transported into clouds that cover the surface. This has important implications for the properties of clouds in these regions. This research measured the potential transport of surface based ice crystals into the surrounding clouds at a mountain top site.
Dawei Hu, M. Rami Alfarra, Kate Szpek, Justin M. Langridge, Michael I. Cotterell, Claire Belcher, Ian Rule, Zixia Liu, Chenjie Yu, Yunqi Shao, Aristeidis Voliotis, Mao Du, Brett Smith, Greg Smallwood, Prem Lobo, Dantong Liu, Jim M. Haywood, Hugh Coe, and James D. Allan
Atmos. Chem. Phys., 21, 16161–16182, https://doi.org/10.5194/acp-21-16161-2021, https://doi.org/10.5194/acp-21-16161-2021, 2021
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Here, we developed new techniques for investigating these properties in the laboratory and applied these to BC and BrC from different sources, including diesel exhaust, inverted propane flame and wood combustion. These have allowed us to quantify the changes in shape and chemical composition of different soots according to source and variables such as the moisture content of wood.
Ernesto Reyes-Villegas, Upasana Panda, Eoghan Darbyshire, James M. Cash, Rutambhara Joshi, Ben Langford, Chiara F. Di Marco, Neil J. Mullinger, Mohammed S. Alam, Leigh R. Crilley, Daniel J. Rooney, W. Joe F. Acton, Will Drysdale, Eiko Nemitz, Michael Flynn, Aristeidis Voliotis, Gordon McFiggans, Hugh Coe, James Lee, C. Nicholas Hewitt, Mathew R. Heal, Sachin S. Gunthe, Tuhin K. Mandal, Bhola R. Gurjar, Shivani, Ranu Gadi, Siddhartha Singh, Vijay Soni, and James D. Allan
Atmos. Chem. Phys., 21, 11655–11667, https://doi.org/10.5194/acp-21-11655-2021, https://doi.org/10.5194/acp-21-11655-2021, 2021
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This paper shows the first multisite online measurements of PM1 in Delhi, India, with measurements over different seasons in Old Delhi and New Delhi in 2018. Organic aerosol (OA) source apportionment was performed using positive matrix factorisation (PMF). Traffic was the main primary aerosol source for both OAs and black carbon, seen with PMF and Aethalometer model analysis, indicating that control of primary traffic exhaust emissions would make a significant reduction to Delhi air pollution.
Benjamin A. Nault, Duseong S. Jo, Brian C. McDonald, Pedro Campuzano-Jost, Douglas A. Day, Weiwei Hu, Jason C. Schroder, James Allan, Donald R. Blake, Manjula R. Canagaratna, Hugh Coe, Matthew M. Coggon, Peter F. DeCarlo, Glenn S. Diskin, Rachel Dunmore, Frank Flocke, Alan Fried, Jessica B. Gilman, Georgios Gkatzelis, Jacqui F. Hamilton, Thomas F. Hanisco, Patrick L. Hayes, Daven K. Henze, Alma Hodzic, James Hopkins, Min Hu, L. Greggory Huey, B. Thomas Jobson, William C. Kuster, Alastair Lewis, Meng Li, Jin Liao, M. Omar Nawaz, Ilana B. Pollack, Jeffrey Peischl, Bernhard Rappenglück, Claire E. Reeves, Dirk Richter, James M. Roberts, Thomas B. Ryerson, Min Shao, Jacob M. Sommers, James Walega, Carsten Warneke, Petter Weibring, Glenn M. Wolfe, Dominique E. Young, Bin Yuan, Qiang Zhang, Joost A. de Gouw, and Jose L. Jimenez
Atmos. Chem. Phys., 21, 11201–11224, https://doi.org/10.5194/acp-21-11201-2021, https://doi.org/10.5194/acp-21-11201-2021, 2021
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Secondary organic aerosol (SOA) is an important aspect of poor air quality for urban regions around the world, where a large fraction of the population lives. However, there is still large uncertainty in predicting SOA in urban regions. Here, we used data from 11 urban campaigns and show that the variability in SOA production in these regions is predictable and is explained by key emissions. These results are used to estimate the premature mortality associated with SOA in urban regions.
Zainab Bibi, Hugh Coe, James Brooks, Paul I. Williams, Ernesto Reyes-Villegas, Michael Priestley, Carl J. Percival, and James D. Allan
Atmos. Chem. Phys., 21, 10763–10777, https://doi.org/10.5194/acp-21-10763-2021, https://doi.org/10.5194/acp-21-10763-2021, 2021
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We are presenting a new method to apportion black carbon/soot into multiple sources through the inclusion of fullerene and metal data into HR-SP-AMS factorisation. While this itself would be considered a technical development, we can present a budget of contributions to measured BC during the event studied, including the conclusion that fireworks contributed little compared to the bonfire, traffic, and domestic wood-burning emissions.
James M. Cash, Ben Langford, Chiara Di Marco, Neil J. Mullinger, James Allan, Ernesto Reyes-Villegas, Ruthambara Joshi, Mathew R. Heal, W. Joe F. Acton, C. Nicholas Hewitt, Pawel K. Misztal, Will Drysdale, Tuhin K. Mandal, Shivani, Ranu Gadi, Bhola Ram Gurjar, and Eiko Nemitz
Atmos. Chem. Phys., 21, 10133–10158, https://doi.org/10.5194/acp-21-10133-2021, https://doi.org/10.5194/acp-21-10133-2021, 2021
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We present the first real-time composition of submicron particulate matter (PM1) in Old Delhi using high-resolution aerosol mass spectrometry. Seasonal analysis shows peak concentrations occur during the post-monsoon, and novel-tracers reveal the largest sources are a combination of local open and regional crop residue burning. Strong links between increased chloride aerosol concentrations and burning sources of PM1 suggest burning sources are responsible for the post-monsoon chloride peak.
Huihui Wu, Jonathan W. Taylor, Justin M. Langridge, Chenjie Yu, James D. Allan, Kate Szpek, Michael I. Cotterell, Paul I. Williams, Michael Flynn, Patrick Barker, Cathryn Fox, Grant Allen, James Lee, and Hugh Coe
Atmos. Chem. Phys., 21, 9417–9440, https://doi.org/10.5194/acp-21-9417-2021, https://doi.org/10.5194/acp-21-9417-2021, 2021
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Seasonal biomass burning over West Africa is a globally significant source of carbonaceous particles in the atmosphere, which have important climate impacts but are poorly constrained. We conducted in situ airborne measurements to investigate the evolution of smoke aerosol properties in this region. We observed absorption enhancement for both black carbon and brown carbon after emission, which provides new field results and constraints on aerosol parameterizations for future climate models.
Sobhan Kumar Kompalli, Surendran Nair Suresh Babu, Krishnaswamy Krishna Moorthy, Sreedharan Krishnakumari Satheesh, Mukunda Madhab Gogoi, Vijayakumar S. Nair, Venugopalan Nair Jayachandran, Dantong Liu, Michael J. Flynn, and Hugh Coe
Atmos. Chem. Phys., 21, 9173–9199, https://doi.org/10.5194/acp-21-9173-2021, https://doi.org/10.5194/acp-21-9173-2021, 2021
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The first observations of refractory black carbon aerosol size distributions and mixing state in South Asian outflow to the northern Indian Ocean were carried out as a part of the ICARB-2018 experiment during winter. Size distributions indicated mixed sources of BC particles in the outflow, which are thickly coated. The coating thickness of BC is controlled mainly by the availability of condensable species in the outflow.
Rutambhara Joshi, Dantong Liu, Eiko Nemitz, Ben Langford, Neil Mullinger, Freya Squires, James Lee, Yunfei Wu, Xiaole Pan, Pingqing Fu, Simone Kotthaus, Sue Grimmond, Qiang Zhang, Ruili Wu, Oliver Wild, Michael Flynn, Hugh Coe, and James Allan
Atmos. Chem. Phys., 21, 147–162, https://doi.org/10.5194/acp-21-147-2021, https://doi.org/10.5194/acp-21-147-2021, 2021
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Black carbon (BC) is a component of particulate matter which has significant effects on climate and human health. Sources of BC include biomass burning, transport, industry and domestic cooking and heating. In this study, we measured BC emissions in Beijing, finding a dominance of traffic emissions over all other sources. The quantitative method presented here has benefits for revising widely used emissions inventories and for understanding BC sources with impacts on air quality and climate.
Douglas Morrison, Ian Crawford, Nicholas Marsden, Michael Flynn, Katie Read, Luis Neves, Virginia Foot, Paul Kaye, Warren Stanley, Hugh Coe, David Topping, and Martin Gallagher
Atmos. Chem. Phys., 20, 14473–14490, https://doi.org/10.5194/acp-20-14473-2020, https://doi.org/10.5194/acp-20-14473-2020, 2020
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We provide conservative estimates of the concentrations of bacteria within transatlantic dust clouds, originating from the African continent. We observe significant seasonal differences in the overall concentrations of particles but no seasonal variation in the ratio between bacteria and dust. With bacteria contributing to ice formation at warmer temperatures than dust, our observations should improve the accuracy of climate models.
Huihui Wu, Jonathan W. Taylor, Kate Szpek, Justin M. Langridge, Paul I. Williams, Michael Flynn, James D. Allan, Steven J. Abel, Joseph Pitt, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 12697–12719, https://doi.org/10.5194/acp-20-12697-2020, https://doi.org/10.5194/acp-20-12697-2020, 2020
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Airborne measurements of highly aged biomass burning aerosols (BBAs) over the remote southeast Atlantic provide unique aerosol parameters for climate models. Our observations demonstrate the persistence of strongly absorbing BBAs across wide regions of the South Atlantic. We also found significant vertical variation in the single-scattering albedo of these BBAs, as a function of relative chemical composition and size. Aerosol properties in the marine BL are suggested to be separated from the FT.
Jonathan W. Taylor, Huihui Wu, Kate Szpek, Keith Bower, Ian Crawford, Michael J. Flynn, Paul I. Williams, James Dorsey, Justin M. Langridge, Michael I. Cotterell, Cathryn Fox, Nicholas W. Davies, Jim M. Haywood, and Hugh Coe
Atmos. Chem. Phys., 20, 11201–11221, https://doi.org/10.5194/acp-20-11201-2020, https://doi.org/10.5194/acp-20-11201-2020, 2020
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Every year, huge plumes of smoke hundreds of miles wide travel over the south Atlantic Ocean from fires in central and southern Africa. These plumes absorb the sun’s energy and warm the climate. We used airborne optical instrumentation to determine how absorbing the smoke was as well as the relative importance of black and brown carbon. We also tested different ways of simulating these properties that could be used in a climate model.
Cited articles
Alfarra, M. R., Prevot, A. S., Szidat, S., Sandradewi, J., Weimer, S., Lanz, V. A., Schreiber, D., Mohr, M., and Baltensperger, U.: Identification of the mass spectral signature of organic aerosols from wood burning emissions, Environ. Sci. Technol., 41, 5770–5777, 2007.
Amato, F., Moreno, T., Pandolfi, M., Querol, X., Alastuey, A., Delgado, A., Pedrero, M., and Cots, N.: Concentrations, sources and geochemistry of airborne particulate matter at a major European airport, J. Environ. Monitor., 12, 854–862, https://doi.org/10.1039/B925439K, 2010.
Anderson, B. E., Chen, G., and Blake, D. R.: Hydrocarbon emissions from a modern commercial airliner, Atmos. Environ., 40, 3601–3612, https://doi.org/10.1016/j.atmosenv.2005.09.072, 2006.
Anderson, B. E., Beyersdorf, A. J., Hudgins, C. H., Plant, J. V., Thornhill, K. L., Winstead, E. L., Ziemba, L. D., Howard, R., Corporan, E., Miake-Lye, R. C., and Herndon, S. C.: Alternative aviation fuel experiment (AAFEX), NASA, No. NASA/TM-2011-217059, 2011.
Boldo, E., Medina, S., Le Tertre, A., Hurley, F., Mücke, H. G., Ballester, F., Aguilera, I., and Eilstein, D., on behalf of the Apheis group: Apheis: Health impact assessment of long-term exposure to PM2.5 in 23 European cities, Eur. J. Epidemiol., 21, 449–458, https://doi.org/10.1007/s10654-006-9014-0, 2006.
Bond, T. C., Streets, D. G., Yarber, K. F., Nelson, S. M., Woo, J. H., and Klimont, Z.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geophys. Res.-Atmos., 109, D14203, https://doi.org/10.1029/2003JD003697, 2004.
Canagaratna, M. R., Jayne, J. T., Jimenez, J. L., Allan, J. D., Alfarra, M. R., Zhang, Q., Onasch, T. B., Drewnick, F., Coe, H., Middlebrook, A., and Delia, A.: Chemical and microphysical characterization of ambient aerosols with the aerodyne aerosol mass spectrometer, Mass Spectrom. Rev., 26, 185–222, https://doi.org/10.1002/mas.20115, 2007.
Canonaco, F., Crippa, M., Slowik, J. G., Baltensperger, U., and Prévôt, A. S. H.: SoFi, an IGOR-based interface for the efficient use of the generalized multilinear engine (ME-2) for the source apportionment: ME-2 application to aerosol mass spectrometer data, Atmos. Meas. Tech., 6, 3649–3661, https://doi.org/10.5194/amt-6-3649-2013, 2013.
Carslaw, D. C. and Ropkins, K.: Openair – an R package for air quality data analysis, Environ. Modell. Softw., 27, 52–61, https://doi.org/10.1016/j.envsoft.2011.09.008, 2012.
Carslaw, D. C., Beevers, S. D., Ropkins, K., and Bell, M. C.: Detecting and quantifying aircraft and other on-airport contributions to ambient nitrogen oxides in the vicinity of a large international airport, Atmos. Environ., 40, 5424–5434, https://doi.org/10.1016/j.atmosenv.2006.04.062, 2006.
Crilley, L. R., Bloss, W. J., Yin, J., Beddows, D. C. S., Harrison, R. M., Allan, J. D., Young, D. E., Flynn, M., Williams, P., Zotter, P., Prevot, A. S. H., Heal, M. R., Barlow, J. F., Halios, C. H., Lee, J. D., Szidat, S., and Mohr, C.: Sources and contributions of wood smoke during winter in London: assessing local and regional influences, Atmos. Chem. Phys., 15, 3149–3171, https://doi.org/10.5194/acp-15-3149-2015, 2015.
Eurostat Database: Air transport statistics, https://european-union.europa.eu/index_en (last access: September 2023), 2022.
Fushimi, A., Saitoh, K., Fujitani, Y., and Takegawa, N.: Identification of jet lubrication oil as a major component of aircraft exhaust nanoparticles, Atmos. Chem. Phys., 19, 6389–6399, https://doi.org/10.5194/acp-19-6389-2019, 2019.
He, R. W., Shirmohammadi, F., Gerlofs-Nijland, M. E., Sioutas, C., and Cassee, F. R.: Pro-inflammatory responses to PM0.25 from airport and urban traffic emissions, Sci. Total Environ., 640, 997–1003, https://doi.org/10.1016/j.scitotenv.2018.05.382, 2018.
Helin, A., Niemi, J. V., Virkkula, A., Pirjola, L., Teinilä, K., Backman, J., Aurela, M., Saarikoski, S., Rönkkö, T., Asmi, E., and Timonen, H.: Characteristics and source apportionment of black carbon in the Helsinki metropolitan area, Finland, Atmos. Environ., 190, 87–98, https://doi.org/10.1016/j.atmosenv.2018.07.022, 2018.
Herndon, S. C., Jayne, J. T., Lobo, P., Onasch, T. B., Fleming, G., Hagen, D. E., Whitefield, P. D., and Miake-Lye, R. C.: Commercial aircraft engine emissions characterization of in-use aircraft at Hartsfield-Jackson Atlanta International Airport, Environ. Sci. Technol., 42, 1877–1883, https://doi.org/10.1021/es072029+, 2008.
Hu, S., Fruin, S., Kozawa, K., Mara, S., Winer, A. M., and Paulson, S. E.: Aircraft emission impacts in a neighborhood adjacent to a general aviation airport in Southern California, Environ. Sci. Technol., 43, 8039–8045, https://doi.org/10.1021/es900975f, 2009.
Hudda, N. and Fruin, S. A.: International airport impacts to air quality: size and related properties of large increases in ultrafine particle number concentrations, Environ. Sci. Technol., 50, 3362–3370, https://doi.org/10.1021/acs.est.5b05313, 2016.
Hudda, N., Gould, T., Hartin, K., Larson, T. V., and Fruin, S. A.: Emissions from an international airport increase particle number concentrations 4-fold at 10 km downwind, Environ. Sci. Technol., 48, 6628–6635, https://doi.org/10.1021/es5001566, 2014.
Hudda, N., Simon, M. C., Zamore, W., Brugge, D., and Durant, J. L.: Aviation emissions impact ambient ultrafine particle concentrations in the greater Boston area, Environ. Sci. Technol., 50, 8514–8521, https://doi.org/10.1021/acs.est.6b01815, 2016.
International Civil Aviation Organization (ICAO): Environmental protection. Annex 16 to the Convention on International Civil Aviation, Volume II aircraft engine emissions, ICAO, Montreal, 2016.
Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., and Aiken, A. C.: Evolution of organic aerosols in the atmosphere, Science, 326, 1525–1529, https://doi.org/10.1126/science.1180353, 2009.
Jonsdottir, H. R., Delaval, M., Leni, Z., Keller, A., Brem, B. T., Siegerist, F., Schönenberger, D., Durdina, L., Elser, M., Burtscher, H., and Liati, A.: Non-volatile particle emissions from aircraft turbine engines at ground-idle induce oxidative stress in bronchial cells, Communications Biology, 2, 90, https://doi.org/10.1038/s42003-019-0332-7, 2019.
Kinsey, J. S.: Characterization of emissions from commercial aircraft engines during the Aircraft Particle Emissions eXperiment (APEX) 1 to 3, U.S. Environmental Protection Agency, Washington, DC, EPA/600/R-09/130, 2009.
Kinsey, J. S., Dong, Y., Williams, D. C., and Logan, R.: Physical characterization of the fine particle emissions from commercial aircraft engines during the Aircraft Particle Emissions eXperiment (APEX) 1–3, Atmos. Environ., 44, 2147–2156, https://doi.org/10.1016/j.atmosenv.2010.02.010, 2010.
Kinsey, J. S., Hays, M. D., Dong, Y., Williams, D. C., and Logan, R.: Chemical characterization of the fine particle emissions from commercial aircraft engines during the Aircraft Particle Emissions eXperiment (APEX) 1 to 3, Environ. Sci. Technol., 45, 3415–3421, https://doi.org/10.1021/es103880d, 2011.
Lee, D. S., Pitari, G., Grewe, V., Gierens, K., Penner, J. E., Petzold, A., Prather, M. J., Schumann, U., Bais, A., Berntsen, T., and Iachetti, D.: Transport impacts on atmosphere and climate: Aviation, Atmos. Environ., 44, 4678–4734, https://doi.org/10.1016/j.atmosenv.2009.06.005, 2010.
Li, N., Hao, M., Phalen, R. F., Hinds, W. C., and Nel, A. E.: Particulate air pollutants and asthma: a paradigm for the role of oxidative stress in PM-induced adverse health effects, Clin. Immunol., 109, 250–265, https://doi.org/10.1016/j.clim.2003.08.006, 2003.
Liu, G., Yan, B., and Chen, G.: Technical review on jet fuel production, Renew. Sust. Energ. Rev., 25, 59–70, 2013.
Masiol, M. and Harrison, R. M.: Aircraft engine exhaust emissions and other airport-related contributions to ambient air pollution: A review, Atmos. Environ., 95, 409–455, https://doi.org/10.1016/j.atmosenv.2014.05.070, 2014.
Mazaheri, M., Johnson, G. R., and Morawska, L.: An inventory of particle and gaseous emissions from large aircraft thrust engine operations at an airport, Atmos. Environ., 45, 3500–3507, https://doi.org/10.1016/j.atmosenv.2010.12.012, 2011.
NIST Mass Spectrometry Data Center: Decane, US Secretary of Commerce, https://webbook.nist.gov/cgi/cbook.cgi?ID=C124185&Mask=200#Mass-Spec (last access: September 2023), 1990.
Onasch, T. B., Jayne, J. T., Herndon, S., Worsnop, D. R., Miake-Lye, R. C., Mortimer, I. P., and Anderson, B. E.: Chemical properties of aircraft engine particulate exhaust emissions, J. Propul. Power, 25, 1121–1137, https://doi.org/10.2514/1.36371, 2009.
Paatero, P.: The multilinear engine – a table-driven, least squares program for solving multilinear problems, including the n-way parallel factor analysis model, J. Comput. Graph. Stat., 8, 854–888, https://doi.org/10.1080/10618600.1999.10474853, 1999.
Paatero, P. and Tapper, U.: Positive matrix factorization: A non-negative factor model with optimal utilization of error estimates of data values, Environmetrics, 5, 111–126, https://doi.org/10.1002/env.3170050203, 1994.
Petzold, A. and Schönlinner, M.: Multi-angle absorption photometry – a new method for the measurement of aerosol light absorption and atmospheric black carbon, J. Aerosol Sci., 35, 421–441, https://doi.org/10.1016/j.jaerosci.2003.09.005, 2004.
Pope III, C. A. and Dockery, D. W.: Health effects of fine particulate air pollution: lines that connect, J. Air Waste Manage., 56, 709–742, https://doi.org/10.1080/10473289.2006.10464485, 2006.
Reyes-Villegas, E., Green, D. C., Priestman, M., Canonaco, F., Coe, H., Prévôt, A. S. H., and Allan, J. D.: Organic aerosol source apportionment in London 2013 with ME-2: exploring the solution space with annual and seasonal analysis, Atmos. Chem. Phys., 16, 15545–15559, https://doi.org/10.5194/acp-16-15545-2016, 2016.
Reyes-Villegas, E., Priestley, M., Ting, Y.-C., Haslett, S., Bannan, T., Le Breton, M., Williams, P. I., Bacak, A., Flynn, M. J., Coe, H., Percival, C., and Allan, J. D.: Simultaneous aerosol mass spectrometry and chemical ionisation mass spectrometry measurements during a biomass burning event in the UK: insights into nitrate chemistry, Atmos. Chem. Phys., 18, 4093–4111, https://doi.org/10.5194/acp-18-4093-2018, 2018.
Rissman, J., Arunachalam, S., Woody, M., West, J. J., BenDor, T., and Binkowski, F. S.: A plume-in-grid approach to characterize air quality impacts of aircraft emissions at the Hartsfield–Jackson Atlanta International Airport, Atmos. Chem. Phys., 13, 9285–9302, https://doi.org/10.5194/acp-13-9285-2013, 2013.
Salihu, A. L., Lloyd, S. M., and Akgunduz, A.: Electrification of airport taxiway operations: A simulation framework for analyzing congestion and cost, Transportation Res. D-Tr. E., 97, 102962, https://doi.org/10.1016/j.trd.2021.102962, 2021.
Schripp, T., Anderson, B. E., Bauder, U., Rauch, B., Corbin, J. C., Smallwood, G. J., Lobo, P., Crosbie, E. C., Shook, M. A., Miake-Lye, R. C., and Yu, Z.: Aircraft engine particulate matter emissions from sustainable aviation fuels: Results from ground-based measurements during the NASA/DLR campaign ECLIF2/ND-MAX, Fuel, 325, 124764, https://doi.org/10.1016/j.fuel.2022.124764, 2022.
Schwarze, P. E., Øvrevik, J., Låg, M., Refsnes, M., Nafstad, P., Hetland, R. B., and Dybing, E.: Particulate matter properties and health effects: consistency of epidemiological and toxicological studies, Hum. Exp. Toxicol., 25, 559–579, https://doi.org/10.1177/096032706072520, 2006.
Smith, L. D., Allan, J., Coe, H., Reyes-Villegas, E., Johnson, M. P., Crayford, A., Durand, E., and Williams, P. I.: Examining chemical composition of gas turbine-emitted organic aerosol using positive matrix factorisation (PMF), J. Aerosol Sci., 159, 105869, https://doi.org/10.1016/j.jaerosci.2021.105869, 2022.
Stettler, M. E. J., Eastham, S., and Barrett, S. R. H.: Air quality and public health impacts of UK airports. Part I: Emissions, Atmos. Environ., 45, 5415–5424, https://doi.org/10.1016/j.atmosenv.2011.07.012, 2011.
Timko, M. T., Onasch, T. B., Northway, M. J., Jayne, J. T., Canagaratna, M. R., Herndon, S. C., Wood, E. C., Miake-Lye, R. C., and Knighton, W. B.: Gas turbine engine emissions – Part II: chemical properties of particulate matter, J. Eng. Gas Turbines Power, 132, 061505, https://doi.org/10.1115/1.4000132, 2010.
Timko, M. T., Albo, S. E., Onasch, T. B., Fortner, E. C., Yu, Z., Miake-Lye, R. C., Canagaratna, M. R., Ng, N. L., and Worsnop, D. R.: Composition and sources of the organic particle emissions from aircraft engines, Aerosol Sci. Tech., 48, 61–73, https://doi.org/10.1080/02786826.2013.857758, 2014.
Ulbrich, I. M., Canagaratna, M. R., Zhang, Q., Worsnop, D. R., and Jimenez, J. L.: Interpretation of organic components from Positive Matrix Factorization of aerosol mass spectrometric data, Atmos. Chem. Phys., 9, 2891–2918, https://doi.org/10.5194/acp-9-2891-2009, 2009.
Ungeheuer, F., Caudillo, L., Ditas, F., Simon, M., van Pinxteren, D., Kılıç, D., Rose, D., Jacobi, S., Kürten, A., Curtius, J., and Vogel, A. L.: Nucleation of jet engine oil vapours is a large source of aviation-related ultrafine particles, Communications Earth & Environment, 3, 319, https://doi.org/10.1038/s43247-022-00653-w, 2022.
van Baaren, E.: The Feasibility of a Fully Electric Aircraft Towing System, Master's thesis, Delft University of Technology, Delft, Netherlands, 2019.
Westerdahl, D., Fruin, S. A., Fine, P. L., and Sioutas, C.: The Los Angeles International Airport as a source of ultrafine particles and other pollutants to nearby communities, Atmos. Environ., 42, 3143–3155, https://doi.org/10.1016/j.atmosenv.2007.09.006, 2008.
Yang, X., Cheng, S., Lang, J., Xu, R., and Lv, Z.: Characterization of aircraft emissions and air quality impacts of an international airport, J. Environ. Sci.-China, 72, 198–207, https://doi.org/10.1016/j.jes.2018.01.007, 2018.
Yim, S. H., Stettler, M. E., and Barrett, S. R.: Air quality and public health impacts of UK airports. Part II: Impacts and policy assessment, Atmos. Environ., 67, 184–192, https://doi.org/10.1016/j.atmosenv.2012.10.017, 2013.
Yu, K. N., Cheung, Y. P., Cheung, T., and Henry, R. C.: Identifying the impact of large urban airports on local air quality by nonparametric regression, Atmos. Environ., 38, 4501–4507, https://doi.org/10.1016/j.atmosenv.2004.05.034, 2004.
Yu, Z., Liscinsky, D. S., Winstead, E. L., True, B. S., Timko, M. T., Bhargava, A., Herndon, S. C., Miake-Lye, R. C., and Anderson, B. E.: Characterization of lubrication oil emissions from aircraft engines, Environ. Sci. Technol., 44, 9530–9534, https://doi.org/10.1021/es102145z, 2010.
Yu, Z., Herndon, S. C., Ziemba, L. D., Timko, M. T., Liscinsky, D. S., Anderson, B. E., and Miake-Lye, R. C.: Identification of lubrication oil in the particulate matter emissions from engine exhaust of in-service commercial aircraft, Environ. Sci. Technol., 46, 9630–9637, https://doi.org/10.1021/es301692t, 2012.
Yu, Z., Timko, M. T., Herndon, S. C., Richard, C., Beyersdorf, A. J., Ziemba, L. D., Winstead, E. L., and Anderson, B. E.: Mode-specific, semi-volatile chemical composition of particulate matter emissions from a commercial gas turbine aircraft engine, Atmos. Environ., 218, 116974, https://doi.org/10.1016/j.atmosenv.2019.116974, 2019.
Yunos, S. N. M. M., Ghafir, M. F. A., and Wahab, A. A.: Aircraft LTO emissions regulations and implementations at European airports, AIP Conference Proceedings, 1831, 020006, https://doi.org/10.1063/1.4981147, 2017.
Zhang, Q., Jimenez, J. L., Allan, J., Coe, H., Ulbrich, I. M., Alfarra, M. R., Takami, A., Middlebrook, A. M., Sun, Y. L., Dzepina, K., Dunlea, E. J., Docherty, K. S., DeCarlo, P. F., Salcedo, D., Onasch, T. B., Jayne, J. T., Miyoshi, T., Shimono, A., and Worsnop, D. R.: Ubiquity and dominance of oxygenated species in organic aerosols in anthropogenically-influenced Northern Hemisphere midlatitudes, Geophys. Res. Lett., 34, L13801, https://doi.org/10.1029/2007GL029979, 2007.
Zhu, Y., Fanning, E., Yu, R. C., Zhang, Q., and Froines, J. R.: Aircraft emissions and local air quality impacts from takeoff activities at a large International Airport, Atmos. Environ., 45, 6526–6533, https://doi.org/10.1016/j.atmosenv.2011.08.062, 2011.
Short summary
This paper investigates emissions from aviation activities at an international airport to evaluate their impact on local air quality. The study provides detailed insights into the chemical composition of aerosols and key pollutants in the airport environment. Source apportionment analysis using positive matrix factorisation (PMF) identified three significant sources: less oxidised oxygenated organic aerosol, alkane organic aerosol, and more oxidised oxygenated organic aerosol.
This paper investigates emissions from aviation activities at an international airport to...
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