Articles | Volume 20, issue 23
https://doi.org/10.5194/acp-20-15015-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-15015-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Particle aging and aerosol–radiation interaction affect volcanic plume dispersion: evidence from the Raikoke 2019 eruption
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
Gholam Ali Hoshyaripour
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
Julia Bruckert
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
Ákos Horváth
Meteorological Institute, Universität Hamburg, Hamburg, Germany
Elizaveta Malinina
Institute of Environmental Physics, University of Bremen, Bremen, Germany
Sandra Wallis
Institute of Physics, Greifswald University, Greifswald, Germany
Fred J. Prata
AIRES Pty. Ltd., Mt Eliza, Victoria, Australia
Alexei Rozanov
Institute of Environmental Physics, University of Bremen, Bremen, Germany
Christian von Savigny
Institute of Physics, Greifswald University, Greifswald, Germany
Heike Vogel
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
Bernhard Vogel
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
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Anna Lange, Alexei Rozanov, and Christian von Savigny
Atmos. Chem. Phys., 23, 14829–14839, https://doi.org/10.5194/acp-23-14829-2023, https://doi.org/10.5194/acp-23-14829-2023, 2023
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We were able to demonstrate quantitatively that the blue colour of the sky cannot be solely attributed to Rayleigh scattering. The influence of ozone on the blue colour of the sky is calculated for different viewing geometries, total ozone columns and an enhanced stratospheric aerosol scenario. Furthermore, the effects of polarisation, surface albedo and observer height are investigated.
Michael Sigmond, James Anstey, Vivek Arora, Ruth Digby, Nathan Gillett, Viatcheslav Kharin, William Merryfield, Catherine Reader, John Scinocca, Neil Swart, John Virgin, Carsten Abraham, Jason Cole, Nicolas Lambert, Woo-Sung Lee, Yongxiao Liang, Elizaveta Malinina, Landon Rieger, Knut von Salzen, Christian Seiler, Clint Seinen, Andrew Shao, Reinel Sospedra-Alfonso, Libo Wang, and Duo Yang
Geosci. Model Dev., 16, 6553–6591, https://doi.org/10.5194/gmd-16-6553-2023, https://doi.org/10.5194/gmd-16-6553-2023, 2023
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John M. C. Plane, Jörg Gumbel, Konstantinos S. Kalogerakis, Daniel R. Marsh, and Christian von Savigny
Atmos. Chem. Phys., 23, 13255–13282, https://doi.org/10.5194/acp-23-13255-2023, https://doi.org/10.5194/acp-23-13255-2023, 2023
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Christoph G. Hoffmann, Lena G. Buth, and Christian von Savigny
Atmos. Chem. Phys., 23, 12781–12799, https://doi.org/10.5194/acp-23-12781-2023, https://doi.org/10.5194/acp-23-12781-2023, 2023
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The Madden–Julian oscillation is an important feature of weather in the tropics. Although it is mainly active in the troposphere, we show that it systematically influences the air temperature in the layers above, up to about 100 km altitude and from pole to pole. We have linked this to another known far-reaching process, interhemispheric coupling. This is basic research on atmospheric couplings and variability but might also be of interest for intraseasonal weather forecasting models.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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Felix Wrana, Ulrike Niemeier, Larry W. Thomason, Sandra Wallis, and Christian von Savigny
Atmos. Chem. Phys., 23, 9725–9743, https://doi.org/10.5194/acp-23-9725-2023, https://doi.org/10.5194/acp-23-9725-2023, 2023
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Sandra Wallis, Hauke Schmidt, and Christian von Savigny
Atmos. Chem. Phys., 23, 7001–7014, https://doi.org/10.5194/acp-23-7001-2023, https://doi.org/10.5194/acp-23-7001-2023, 2023
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Strong volcanic eruptions are able to alter the temperature and the circulation of the middle atmosphere. This study simulates the atmospheric response to an idealized strong tropical eruption and focuses on the impact on the mesosphere. The simulations show a warming of the polar summer mesopause in the first November after the eruption. Our study indicates that this is mainly due to dynamical coupling in the summer hemisphere with a potential contribution from interhemispheric coupling.
Axel Seifert, Vanessa Bachmann, Florian Filipitsch, Jochen Förstner, Christian M. Grams, Gholam Ali Hoshyaripour, Julian Quinting, Anika Rohde, Heike Vogel, Annette Wagner, and Bernhard Vogel
Atmos. Chem. Phys., 23, 6409–6430, https://doi.org/10.5194/acp-23-6409-2023, https://doi.org/10.5194/acp-23-6409-2023, 2023
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We investigate how mineral dust can lead to the formation of cirrus clouds. Dusty cirrus clouds lead to a reduction in solar radiation at the surface and, hence, a reduced photovoltaic power generation. Current weather prediction systems are not able to predict this interaction between mineral dust and cirrus clouds. We have developed a new physical description of the formation of dusty cirrus clouds. Overall we can show a considerable improvement in the forecast quality of clouds and radiation.
Linlu Mei, Vladimir Rozanov, Alexei Rozanov, and John P. Burrows
Geosci. Model Dev., 16, 1511–1536, https://doi.org/10.5194/gmd-16-1511-2023, https://doi.org/10.5194/gmd-16-1511-2023, 2023
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This paper summarizes recent developments of aerosol, cloud and surface reflectance databases and models in the framework of the software package SCIATRAN. These updates and developments extend the capabilities of the radiative transfer modeling, especially by accounting for different kinds of vertical inhomogeneties. Vertically inhomogeneous clouds and different aerosol types can be easily accounted for within SCIATRAN (V4.6). The widely used surface models and databases are now available.
Christian von Savigny, Anna Lange, Anne Hemkendreis, Christoph G. Hoffmann, and Alexei Rozanov
Clim. Past, 18, 2345–2356, https://doi.org/10.5194/cp-18-2345-2022, https://doi.org/10.5194/cp-18-2345-2022, 2022
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This study investigates the possibility of inferring information on aerosol optical depth from photographs of historic paintings. The idea – which has been applied in previous studies – is very interesting because it would provide an archive of the atmospheric aerosol loading covering many centuries. We show that twilight colours depend not only on the aerosol optical thickness, but also on several other parameters, making a quantitative estimate of aerosol optical depth very difficult.
Carlo Arosio, Alexei Rozanov, Victor Gorshelev, Alexandra Laeng, and John P. Burrows
Atmos. Meas. Tech., 15, 5949–5967, https://doi.org/10.5194/amt-15-5949-2022, https://doi.org/10.5194/amt-15-5949-2022, 2022
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This paper characterizes the uncertainties affecting the ozone profiles retrieved at the University of Bremen through OMPS limb satellite observations. An accurate knowledge of the uncertainties is relevant for the validation of the product and to correctly interpret the retrieval results. We investigate several sources of uncertainties, estimate a total random and systematic component, and verify the consistency of the combined OMPS-MLS total uncertainty.
Ákos Horváth, James L. Carr, Dong L. Wu, Julia Bruckert, Gholam Ali Hoshyaripour, and Stefan A. Buehler
Atmos. Chem. Phys., 22, 12311–12330, https://doi.org/10.5194/acp-22-12311-2022, https://doi.org/10.5194/acp-22-12311-2022, 2022
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We estimate plume heights for the April 2021 La Soufrière daytime eruptions using GOES-17 near-limb side views and GOES-16–MODIS stereo views. These geometric heights are then compared with brightness-temperature-based radiometric height estimates to characterize the biases of the latter. We also show that the side view method can be applied to infrared imagery and thus nighttime eruptions, albeit with larger uncertainty.
John T. Sullivan, Arnoud Apituley, Nora Mettig, Karin Kreher, K. Emma Knowland, Marc Allaart, Ankie Piters, Michel Van Roozendael, Pepijn Veefkind, Jerry R. Ziemke, Natalya Kramarova, Mark Weber, Alexei Rozanov, Laurence Twigg, Grant Sumnicht, and Thomas J. McGee
Atmos. Chem. Phys., 22, 11137–11153, https://doi.org/10.5194/acp-22-11137-2022, https://doi.org/10.5194/acp-22-11137-2022, 2022
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A TROPOspheric Monitoring Instrument (TROPOMI) validation campaign (TROLIX-19) was held in the Netherlands in September 2019. The research presented here focuses on using ozone lidars from NASA’s Goddard Space Flight Center to better evaluate the characterization of ozone throughout TROLIX-19 as compared to balloon-borne, space-borne and ground-based passive measurements, as well as a global coupled chemistry meteorology model.
Natalia E. Chubarova, Heike Vogel, Elizaveta E. Androsova, Alexander A. Kirsanov, Olga B. Popovicheva, Bernhard Vogel, and Gdaliy S. Rivin
Atmos. Chem. Phys., 22, 10443–10466, https://doi.org/10.5194/acp-22-10443-2022, https://doi.org/10.5194/acp-22-10443-2022, 2022
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Effects of urban aerosol pollution in Moscow were analyzed using the COSMO-ART chemical transport model and intensive measurement campaigns. We show that urban aerosol comprises about 15–20% of columnar aerosol content, consisting mainly of fine aerosol mode. The black carbon (BC) fraction is about 5 %, depending on particle dispersion intensity (IPD). The BC fraction low value explains weak absorbing properties of the Moscow atmosphere. IPD also defines the daily cycle of urban aerosol species.
Sandra Wallis, Christoph Gregor Hoffmann, and Christian von Savigny
Ann. Geophys., 40, 421–431, https://doi.org/10.5194/angeo-40-421-2022, https://doi.org/10.5194/angeo-40-421-2022, 2022
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Although the 1991 eruption of Mt Pinatubo had a severe impact on Earth's climate, the effect of this event on the mesosphere is not well understood. We investigated satellite-borne temperature measurements from the HALOE instrument and found indications that a positive temperature anomaly is present in the tropical upper mesosphere at the beginning of the HALOE time series, which may be related to the eruption of Mt. Pinatubo.
Anna Lange, Gerd Baumgarten, Alexei Rozanov, and Christian von Savigny
Ann. Geophys., 40, 407–419, https://doi.org/10.5194/angeo-40-407-2022, https://doi.org/10.5194/angeo-40-407-2022, 2022
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We investigate the influence of different parameters on the colour of noctilucent clouds (highest clouds in the atmosphere), using radiative transfer calculations. We determined the effect of the particle size, optical depth, single scattering/multiple scattering and ozone. For sufficiently large optical depth and for specific viewing geometries, ozone plays only a minor role in the blueish colour of noctilucent clouds (new result).
William G. Read, Gabriele Stiller, Stefan Lossow, Michael Kiefer, Farahnaz Khosrawi, Dale Hurst, Holger Vömel, Karen Rosenlof, Bianca M. Dinelli, Piera Raspollini, Gerald E. Nedoluha, John C. Gille, Yasuko Kasai, Patrick Eriksson, Christopher E. Sioris, Kaley A. Walker, Katja Weigel, John P. Burrows, and Alexei Rozanov
Atmos. Meas. Tech., 15, 3377–3400, https://doi.org/10.5194/amt-15-3377-2022, https://doi.org/10.5194/amt-15-3377-2022, 2022
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This paper attempts to provide an assessment of the accuracy of 21 satellite-based instruments that remotely measure atmospheric humidity in the upper troposphere of the Earth's atmosphere. The instruments made their measurements from 1984 to the present time; however, most of these instruments began operations after 2000, and only a few are still operational. The objective of this study is to quantify the accuracy of each satellite humidity data set.
Nora Mettig, Mark Weber, Alexei Rozanov, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Ryan M. Stauffer, Thierry Leblanc, Gerard Ancellet, Michael J. Newchurch, Shi Kuang, Rigel Kivi, Matthew B. Tully, Roeland Van Malderen, Ankie Piters, Bogumil Kois, René Stübi, and Pavla Skrivankova
Atmos. Meas. Tech., 15, 2955–2978, https://doi.org/10.5194/amt-15-2955-2022, https://doi.org/10.5194/amt-15-2955-2022, 2022
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Vertical ozone profiles from combined spectral measurements in the UV and IR spectral ranges were retrieved by using data from TROPOMI/S5P and CrIS/Suomi-NPP. The vertical resolution and accuracy of the ozone profiles are improved by combining both wavelength ranges compared to retrievals limited to UV or IR spectral data only. The advancement of our TOPAS algorithm for combined measurements is required because in the UV-only retrieval the vertical resolution in the troposphere is very limited.
Mireia Papke Chica, Valerian Hahn, Tiziana Braeuer, Elena de la Torre Castro, Florian Ewald, Mathias Gergely, Simon Kirschler, Luca Bugliaro Goggia, Stefanie Knobloch, Martina Kraemer, Johannes Lucke, Johanna Mayer, Raphael Maerkl, Manuel Moser, Laura Tomsche, Tina Jurkat-Witschas, Martin Zoeger, Christian von Savigny, and Christiane Voigt
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-255, https://doi.org/10.5194/acp-2022-255, 2022
Preprint withdrawn
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The mixed-phase temperature regime in convective clouds challenges our understanding of microphysical and radiative cloud properties. We provide a rare and unique dataset of aircraft in situ measurements in a strong mid-latitude convective system. We find that mechanisms initiating ice nucleation and growth strongly depend on temperature, relative humidity, and vertical velocity and variate within the measured system, resulting in altitude dependent changes of the cloud liquid and ice fraction.
Julia Bruckert, Gholam Ali Hoshyaripour, Ákos Horváth, Lukas O. Muser, Fred J. Prata, Corinna Hoose, and Bernhard Vogel
Atmos. Chem. Phys., 22, 3535–3552, https://doi.org/10.5194/acp-22-3535-2022, https://doi.org/10.5194/acp-22-3535-2022, 2022
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Volcanic emissions endanger aviation and public health and also influence weather and climate. Forecasting the volcanic-plume dispersion is therefore a critical yet sophisticated task. Here, we show that explicit treatment of volcanic-plume dynamics and eruption source parameters significantly improves volcanic-plume dispersion forecasts. We further demonstrate the lofting of the SO2 due to a heating of volcanic particles by sunlight with major implications for volcanic aerosol research.
Julia Koch, Adam Bourassa, Nick Lloyd, Chris Roth, and Christian von Savigny
Atmos. Chem. Phys., 22, 3191–3202, https://doi.org/10.5194/acp-22-3191-2022, https://doi.org/10.5194/acp-22-3191-2022, 2022
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The mesopause, the region of the earth's atmosphere between 85 and 100 km, is hard to access by direct measurements. Therefore we look for parameters that can be measured using satellite or ground-based measurements. In this study we researched sodium airglow, a phenomenon that occurs when sodium atoms are excited by chemical reactions. We compared satellite measurements of the airglow and resulting sodium concentration profiles to gain a better understanding of the sodium in that region.
Sandip S. Dhomse, Carlo Arosio, Wuhu Feng, Alexei Rozanov, Mark Weber, and Martyn P. Chipperfield
Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, https://doi.org/10.5194/essd-13-5711-2021, 2021
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High-quality long-term ozone profile data sets are key to estimating short- and long-term ozone variability. Almost all the satellite (and chemical model) data sets show some kind of bias with respect to each other. This is because of differences in measurement methodologies as well as simplified processes in the models. We use satellite data sets and chemical model output to generate 42 years of ozone profile data sets using a random-forest machine-learning algorithm that is named ML-TOMCAT.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Nora Mettig, Mark Weber, Alexei Rozanov, Carlo Arosio, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Richard Querel, Thierry Leblanc, Sophie Godin-Beekmann, Rigel Kivi, and Matthew B. Tully
Atmos. Meas. Tech., 14, 6057–6082, https://doi.org/10.5194/amt-14-6057-2021, https://doi.org/10.5194/amt-14-6057-2021, 2021
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TROPOMI is a nadir-viewing satellite that has observed global atmospheric trace gases at unprecedented spatial resolution since 2017. The retrieval of ozone profiles with high accuracy has been demonstrated using the TOPAS (Tikhonov regularised Ozone Profile retrievAl with SCIATRAN) algorithm and applying appropriate spectral corrections to TROPOMI UV data. Ozone profiles from TROPOMI were compared to ozonesonde and lidar profiles, showing an agreement to within 5 % in the stratosphere.
Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Mark Weber, Carlo Arosio, Annette Ladstätter-Weißenmayer, and John P. Burrows
Atmos. Meas. Tech., 14, 5771–5789, https://doi.org/10.5194/amt-14-5771-2021, https://doi.org/10.5194/amt-14-5771-2021, 2021
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OMPS/NPP (2012–present) allows obtaining the tropospheric ozone column by combining ozone data from limb and nadir observations from the same instrument platform. In a first step, the retrieval of the total ozone column from the OMPS Nadir Mapper using the weighting function fitting approach (WFFA) is described here. The OMPS total ozone was compared with ground-based and other satellite measurements, showing agreement within 2.5 %.
Ákos Horváth, James L. Carr, Olga A. Girina, Dong L. Wu, Alexey A. Bril, Alexey A. Mazurov, Dmitry V. Melnikov, Gholam Ali Hoshyaripour, and Stefan A. Buehler
Atmos. Chem. Phys., 21, 12189–12206, https://doi.org/10.5194/acp-21-12189-2021, https://doi.org/10.5194/acp-21-12189-2021, 2021
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We give a detailed description of a new technique to estimate the height of volcanic eruption columns from near-limb geostationary imagery. Such oblique angle observations offer spectacular side views of eruption columns protruding from the Earth ellipsoid and thereby facilitate a height-by-angle estimation method. Due to its purely geometric nature, the new technique is unaffected by the limitations of traditional brightness-temperature-based height retrievals.
Ákos Horváth, Olga A. Girina, James L. Carr, Dong L. Wu, Alexey A. Bril, Alexey A. Mazurov, Dmitry V. Melnikov, Gholam Ali Hoshyaripour, and Stefan A. Buehler
Atmos. Chem. Phys., 21, 12207–12226, https://doi.org/10.5194/acp-21-12207-2021, https://doi.org/10.5194/acp-21-12207-2021, 2021
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We demonstrate the side view plume height estimation technique described in Part 1 on seven volcanic eruptions from 2019 and 2020, including the 2019 Raikoke eruption. We explore the strengths and limitations of the new technique in comparison to height estimation from brightness temperatures, stereo observations, and ground-based video footage.
Hengheng Zhang, Frank Wagner, Harald Saathoff, Heike Vogel, Gholam Ali Hoshyaripour, Vanessa Bachmann, Jochen Förstner, and Thomas Leisner
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-193, https://doi.org/10.5194/amt-2021-193, 2021
Revised manuscript not accepted
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The evolution and the properties of Saharan dust plume were characterized by LIDARs, a sun photometer, and a regional transport model. Comparison between LIDAR measurements, sun photometer and ICON-ART predictions shows a good agreement for dust arrival time, dust layer height, and dust structure but also that the model overestimates the backscatter coefficients by a factor of (2.2 ± 0.16) and underestimate aerosol optical depth by a factor of (1.5 ± 0.11).
Daniel Zawada, Ghislain Franssens, Robert Loughman, Antti Mikkonen, Alexei Rozanov, Claudia Emde, Adam Bourassa, Seth Dueck, Hannakaisa Lindqvist, Didier Ramon, Vladimir Rozanov, Emmanuel Dekemper, Erkki Kyrölä, John P. Burrows, Didier Fussen, and Doug Degenstein
Atmos. Meas. Tech., 14, 3953–3972, https://doi.org/10.5194/amt-14-3953-2021, https://doi.org/10.5194/amt-14-3953-2021, 2021
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Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
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An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Nellie Wullenweber, Anna Lange, Alexei Rozanov, and Christian von Savigny
Clim. Past, 17, 969–983, https://doi.org/10.5194/cp-17-969-2021, https://doi.org/10.5194/cp-17-969-2021, 2021
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This study investigates the physical processes leading to the rare phenomenon of the sun appearing blue or green. The phenomenon is caused by anomalous scattering by, e.g., volcanic or forest fire aerosols. Unlike most other studies, our study includes a full treatment of the effect of Rayleigh scattering on the colour of the sun. We investigate different factors and revisit a historic example, i.e. the Canadian forest fires in 1950, that led to blue sun events in different European countries.
Felix Wrana, Christian von Savigny, Jacob Zalach, and Larry W. Thomason
Atmos. Meas. Tech., 14, 2345–2357, https://doi.org/10.5194/amt-14-2345-2021, https://doi.org/10.5194/amt-14-2345-2021, 2021
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In this paper, we describe a new method for calculating the size of naturally occurring droplets (aerosols) made mostly of sulfuric acid and water that can be found roughly at 20 km altitude in the atmosphere. We use data from the instrument SAGE III/ISS that is mounted on the International Space Station. We show that our method works well, and that the size parameters we calculate are reasonable and can be a valuable addition for a better understanding of aerosols and their effect on climate.
Harald Rybka, Ulrike Burkhardt, Martin Köhler, Ioanna Arka, Luca Bugliaro, Ulrich Görsdorf, Ákos Horváth, Catrin I. Meyer, Jens Reichardt, Axel Seifert, and Johan Strandgren
Atmos. Chem. Phys., 21, 4285–4318, https://doi.org/10.5194/acp-21-4285-2021, https://doi.org/10.5194/acp-21-4285-2021, 2021
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Estimating the impact of convection on the upper-tropospheric water budget remains a problem for models employing resolutions of several kilometers or more. A sub-kilometer high-resolution model is used to study summertime convection. The results suggest mostly close agreement with ground- and satellite-based observational data while slightly overestimating total frozen water path and anvil lifetime. The simulations are well suited to supplying information for parameterization development.
Larry W. Thomason, Mahesh Kovilakam, Anja Schmidt, Christian von Savigny, Travis Knepp, and Landon Rieger
Atmos. Chem. Phys., 21, 1143–1158, https://doi.org/10.5194/acp-21-1143-2021, https://doi.org/10.5194/acp-21-1143-2021, 2021
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Measurements of the impact of volcanic eruptions on stratospheric aerosol loading by space-based instruments show show a fairly well-behaved relationship between the magnitude and the apparent changes to aerosol size over several orders of magnitude. This directly measured relationship provides a unique opportunity to verify the performance of interactive aerosol models used in climate models.
Stefan Noël, Klaus Bramstedt, Alexei Rozanov, Elizaveta Malinina, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 13, 5643–5666, https://doi.org/10.5194/amt-13-5643-2020, https://doi.org/10.5194/amt-13-5643-2020, 2020
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A new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion-peeling method is presented. The resulting extinctions at 452, 525 and 750 nm compare well with other limb and occultation data from, e.g. SAGE and SCIAMACHY, but show small oscillating features which vanish in monthly anomalies. Major volcanic eruptions, polar stratospheric clouds and influences of the quasi-biennial oscillation can be identified in the time series.
Cited articles
Abdelkader, M., Metzger, S., Steil, B., Klingmüller, K., Tost, H., Pozzer, A., Stenchikov, G., Barrie, L., and Lelieveld, J.: Sensitivity of transatlantic dust transport to chemical aging and related atmospheric processes, Atmos. Chem. Phys., 17, 3799–3821, https://doi.org/10.5194/acp-17-3799-2017, 2017. a, b, c
Ayris, P. M. and Delmelle, P.: Volcanic and atmospheric controls on ash iron
solubility: A review, Phys. Chem. Earth, 45–46, 103–112,
https://doi.org/10.1016/j.pce.2011.04.013, 2012. a
Bagheri, G. and Bonadonna, C.: Aerodynamics of Volcanic Particles:
Characterization of Size, Shape, and Settling Velocity, in: Volcanic Ash
Hazard Observation, edited by: Mackie, S., Cashman, K., Ricketts, H., Rust,
A., and Watson, M., Elsevier, Volcanic Ash: hazard observation, ISBN 978-0-08-100405-0, available at: https://archive-ouverte.unige.ch/unige:86745 (last access: 10 April 2020), 2016. a
Bagnato, E., Aiuppa, A., Bertagnini, A., Bonadonna, C., Cioni, R., Pistolesi,
M., Pedone, M., and Hoskuldsson, A.: Scavenging of sulphur, halogens and
trace metals by volcanic ash: The 2010 Eyjafjallajökull eruption,
Geochim. Cosmochim. Ac., 103, 138–160, https://doi.org/10.1016/j.gca.2012.10.048, 2013. a, b
Bohren, C. F. and Huffman, D. R.: Absorption and Scattering of Light by Small
Particles, John Wiley & Sons, Ltd, New York, ISBN 9783527618156, 1983. a
Bonadonna, C. and Scollo, S.: IAVCEI Commission on Tephra Hazard Modelling, available at: http://www.ct.ingv.it/iavcei/results.htm (last access: 3 September 2020), 2013. a
Bond, T. C., Habib, G., and Bergstrom, R. W.: Limitations in the enhancement
of visible light absorption due to mixing state, J. Geophys. Res.-Atmos.,
111, https://doi.org/10.1029/2006JD007315, 2006. a
Brown, R. J., Bonadonna, C., and Durant, A. J.: A review of volcanic ash
aggregation, Phys. Chem. Earth, 45–46, 65–78,
https://doi.org/10.1016/j.pce.2011.11.001, 2012. a, b, c
Casadevall, T. J.: Volcanic ash and aviation safety: Proceedings of the first
international symposium on volcanic ash and aviation safety, Tech. rep., US
Geol. Surv., https://doi.org/10.3133/b2047, 1994. a
Clarisse, L. and Prata, F.: Infrared sounding of volcanic ash, in: Volcanic
Ash, edited by: Mackie, S., Cashman, K., Ricketts, H., Rust, A., and Watson, M., pp. 189–215, Elsevier, https://doi.org/10.1016/B978-0-08-100405-0.00017-3, ISBN 978-0-08-100405-0, 2016. a
Clarisse, L., Hurtmans, D., Prata, A. J., Karagulian, F., Clerbaux, C.,
De Mazière, M., and Coheur, P.-F.: Retrieving radius, concentration,
optical depth, and mass of different types of aerosols from high-resolution
infrared nadir spectra, Appl. Optics, 49, 3713–3722, 2010. a
Copernicus: Sentinel-5P Pro-Operations Data Hub, available at: https://s5phub.copernicus.eu, last access: 23 November 2020. a
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi,
S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P.,
Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C.,
Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B.,
Hersbach, H., Hólm, E. V., Isaksen, L., Kållberg, P., Köhler, M.,
Matricardi, M., McNally, A. P., Monge-Sanz, B. M., Morcrette, J.-J., Park,
B.-K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J.-N., and Vitart,
F.: The ERA-Interim reanalysis: configuration and performance of the data
assimilation system, Quart. J. Roy. Meteorol. Soc., 137, 553–597,
https://doi.org/10.1002/qj.828, 2011. a
Delmelle, P., Lambert, M., Dufrêne, Y., Gerin, P., and Óskarsson,
N.: Gas/aerosol-ash interaction in volcanic plumes: New insights from
surface analyses of fine ash particles, Earth Planet Sc. Lett., 259, 159–170, https://doi.org/10.1016/j.epsl.2007.04.052, 2007. a
Durant, A. J., Bonadonna, C., and Horwell, C. J.: Atmospheric and
environmental impacts of volcanic particulates, Elements, 6, 235–240,
https://doi.org/10.2113/gselements.6.4.235, 2010. a, b
Folch, A., Costa, A., and Macedonio, G.: FPLUME-1.0: An integral volcanic
plume model accounting for ash aggregation, Geosci. Model. Dev., 9,
431–450, https://doi.org/10.5194/gmd-9-431-2016, 2016. a, b
Fountoukis, C. and Nenes, A.: ISORROPIA II: a computationally efficient thermodynamic equilibrium model for K+–Ca2+–Mg2+–NH4+–Na+–SO –NO –Cl−–H2O aerosols, Atmos. Chem. Phys., 7, 4639–4659, https://doi.org/10.5194/acp-7-4639-2007, 2007. a
Gasch, P., Rieger, D., Walter, C., Khain, P., Levi, Y., Knippertz, P., and Vogel, B.: Revealing the meteorological drivers of the September 2015 severe dust event in the Eastern Mediterranean, Atmos. Chem. Phys., 17, 13573–13604, https://doi.org/10.5194/acp-17-13573-2017, 2017. a, b
Gasteiger, J., Groß, S., Freudenthaler, V., and Wiegner, M.: Volcanic ash from Iceland over Munich: mass concentration retrieved from ground-based remote sensing measurements, Atmos. Chem. Phys., 11, 2209–2223, https://doi.org/10.5194/acp-11-2209-2011, 2011. a
Giorgetta, M. A., Brokopf, R., Crueger, T., Esch, M., Fiedler, S., Helmert, J.,
Hohenegger, C., Kornblueh, L., Köhler, M., Manzini, E., Mauritsen, T., Nam,
C., Raddatz, T., Rast, S., Reinert, D., Sakradzija, M., Schmidt, H., Schneck,
R., Schnur, R., Silvers, L., Wan, H., Zängl, G., and Stevens, B.: ICON-A,
the Atmosphere Component of the ICON Earth System Model: I. Model
Description, J. Adv. Model. Earth Sy., 10, 1613–1637,
https://doi.org/10.1029/2017MS001242, 2018. a
Gordon, I. E., Rothman, L. S., Hill, C., Kochanov, R. V., Tan, Y., Bernath,
P. F., Birk, M., Boudon, V., Campargue, A., Chance, K. V., Drouin, B. J.,
Flaud, J. M., Gamache, R. R., Hodges, J. T., Jacquemart, D., Perevalov,
V. I., Perrin, A., Shine, K. P., Smith, M. A., Tennyson, J., Toon, G. C.,
Tran, H., Tyuterev, V. G., Barbe, A., Császár, A. G., Devi,
V. M., Furtenbacher, T., Harrison, J. J., Hartmann, J. M., Jolly, A.,
Johnson, T. J., Karman, T., Kleiner, I., Kyuberis, A. A., Loos, J., Lyulin,
O. M., Massie, S. T., Mikhailenko, S. N., Moazzen-Ahmadi, N., Müller,
H. S., Naumenko, O. V., Nikitin, A. V., Polyansky, O. L., Rey, M., Rotger,
M., Sharpe, S. W., Sung, K., Starikova, E., Tashkun, S. A., Auwera, J. V.,
Wagner, G., Wilzewski, J., Wcisło, P., Yu, S., and Zak, E. J.: The
HITRAN2016 molecular spectroscopic database, J. Quant. Spectrosc. Ra., 203,
3–69, https://doi.org/10.1016/j.jqsrt.2017.06.038, 2017. a
Gouhier, M., Eychenne, J., Azzaoui, N., Guillin, A., Deslandes, M., Poret, M.,
Costa, A., and Husson, P.: Low efficiency of large volcanic eruptions in
transporting very fine ash into the atmosphere, Sci. Rep.-UK, 9, 1–12,
https://doi.org/10.1038/s41598-019-38595-7, 2019. a
Harvey, N. J., Huntley, N., Dacre, H. F., Goldstein, M., Thomson, D., and
Webster, H.: Multi-level emulation of a volcanic ash transport and dispersion
model to quantify sensitivity to uncertain parameters, Nat. Hazard. Earth
Sys., 18, 41–63, https://doi.org/10.5194/nhess-18-41-2018, 2018. a
Heidinger, A. and Li, Y.: Enterprise AWG Cloud Height Algorithm (ACHA) -
Algorithm Theoretical Basis Document, Tech. rep., NOAA NESDIS CENTER for
SATELLITE APPLICATIONS and RESEARCH, 77 pp., available at:
https://docs.google.com/document/d/1m2SatR91WIJcaAZweongcFCb6Wsx_xnRUcZxp94gXHk (last access: 10 April 2020),
2019. a
Heinze, R., Dipankar, A., Henken, C. C., Moseley, C., Sourdeval, O., Trömel,
S., Xie, X., Adamidis, P., Ament, F., Baars, H., Barthlott, C., Behrendt, A.,
Blahak, U., Bley, S., Brdar, S., Brueck, M., Crewell, S., Deneke, H.,
Di Girolamo, P., Evaristo, R., Fischer, J., Frank, C., Friederichs, P.,
Göcke, T., Gorges, K., Hande, L., Hanke, M., Hansen, A., Hege, H.-C., Hoose,
C., Jahns, T., Kalthoff, N., Klocke, D., Kneifel, S., Knippertz, P., Kuhn,
A., van Laar, T., Macke, A., Maurer, V., Mayer, B., Meyer, C. I., Muppa,
S. K., Neggers, R. A. J., Orlandi, E., Pantillon, F., Pospichal, B., Röber,
N., Scheck, L., Seifert, A., Seifert, P., Senf, F., Siligam, P., Simmer, C.,
Steinke, S., Stevens, B., Wapler, K., Weniger, M., Wulfmeyer, V., Zängl, G.,
Zhang, D., and Quaas, J.: Large-eddy simulations over Germany using ICON: a
comprehensive evaluation, Quart. J. Roy. Meteorol. Soc., 143, 69–100,
https://doi.org/10.1002/qj.2947, 2017. a
Hoshyaripour, G. A., Hort, M., and Langmann, B.: Ash iron mobilization through physicochemical processing in volcanic eruption plumes: a numerical modeling approach, Atmos. Chem. Phys., 15, 9361–9379, https://doi.org/10.5194/acp-15-9361-2015, 2015. a, b
Hoshyaripour, G. A., Bachmann, V., Förstner, J., Steiner, A., Vogel, H.,
Wagner, F., Walter, C., and Vogel, B.: Effects of Particle Non-Sphericity on
Dust Optical Properties in a Forecast System: Implications for
Model-Observation Comparison, J. Geophys. Res.-Atmos., 124, 7164–7178, https://doi.org/10.1029/2018JD030228, 2019. a
Jacobson, M. Z.: A physically-based treatment of elemental carbon optics:
Implications for global direct forcing of aerosols, Geophys. Res. Lett., 27, 217–220, https://doi.org/10.1029/1999GL010968, 2000. a, b
Kaiser, J. C., Hendricks, J., Righi, M., Riemer, N., Zaveri, R. A., Metzger, S., and Aquila, V.: The MESSy aerosol submodel MADE3 (v2.0b): description and a box model test, Geosci. Model Dev., 7, 1137–1157, https://doi.org/10.5194/gmd-7-1137-2014, 2014. a
Khaykin, S. M., Godin-Beekmann, S., Keckhut, P., Hauchecorne, A., Jumelet, J., Vernier, J.-P., Bourassa, A., Degenstein, D. A., Rieger, L. A., Bingen, C., Vanhellemont, F., Robert, C., DeLand, M., and Bhartia, P. K.: Variability and evolution of the midlatitude stratospheric aerosol budget from 22 years of ground-based lidar and satellite observations, Atmos. Chem. Phys., 17, 1829–1845, https://doi.org/10.5194/acp-17-1829-2017, 2017 a
Mackie, S. and Watson, M.: Probabilistic detection of volcanic ash using a
Bayesian approach, J. Geophys. Res.-Atmos., 119, 2409–2428, 2014. a
Malinina, E.: Retrieval of stratospheric aerosol characteristics from
spaceborne limb sounders, PhD Thesis, University of Bremen, available at:
http://nbn-resolving.de/urn:nbn:de:gbv:46-00107153-12 (last access: 23 November 2020), 2019. a
Malinina, E., Rozanov, A., Niemeier, U., Peglow, S., Arosio, C., Wrana, F., Timmreck, C., von Savigny, C., and Burrows, J. P.: Changes in stratospheric aerosol extinction coefficient after the 2018 Ambae eruption as seen by OMPS-LP and ECHAM5-HAM, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-749, in review, 2020. a
Marti, A., Folch, A., Jorba, O., and Janjic, Z.: Volcanic ash modeling with the online NMMB-MONARCH-ASH v1.0 model: model description, case simulation, and evaluation, Atmos. Chem. Phys., 17, 4005–4030, https://doi.org/10.5194/acp-17-4005-2017, 2017. a
Mastin, L. G.: A user-friendly one-dimensional model for wet volcanic plumes,
Geochem. Geophy. Geosy., 8, https://doi.org/10.1029/2006GC001455, 2007. a
Mastin, L., Guffanti, M., Servranckx, R., Webley, P., Barsotti, S., Dean, K.,
Durant, A., Ewert, J., Neri, A., Rose, W., Schneider, D., Siebert, L.,
Stunder, B., Swanson, G., Tupper, A., Volentik, A., and Waythomas, C.: A
multidisciplinary effort to assign realistic source parameters to models of
volcanic ash-cloud transport and dispersion during eruptions, J. Volcanol.
Geoth. Res., 186, 10–21, https://doi.org/10.1016/j.jvolgeores.2009.01.008, 2009. a
Mather, T. A.: Volcanism and the atmosphere: the potential role of the
atmosphere in unlocking the reactivity of volcanic emissions., Philos. T. Roy. Soc. A,, 366, 4581–4595, https://doi.org/10.1098/rsta.2008.0152, 2008. a
Mätzler, C.: MATLAB Functions for Mie Scattering and Absorption, Tech. rep., University of Bern, Research report No. 2002-08, https://doi.org/10.7892/boris.146551, 2002. a
Menzel, W., Frey, R., and Baum, B.: Cloud Top Properties and Cloud Phase –
Algorithm Theoretical Basis Document, Tech. rep., University of Wisconsin – Madison, 73 pp., available at: https://atmosphere-imager.gsfc.nasa.gov/sites/default/files/ModAtmo/MOD06-ATBD_2015_05_01_1.pdf (last access: 10 April 2020),
2015. a
Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S. A.:
Radiative transfer for inhomogeneous atmospheres: RRTM, a validated
correlated-k model for the longwave, J. Geophys. Res.-Atmos., 102,
16663–16682, https://doi.org/10.1029/97jd00237, 1997. a
NASA: LAADS DAAC, available at: https://ladsweb.modaps.eosdis.nasa.gov, last access: 10 April 2020a. a
NASA: Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations,
available at: https://eosweb.larc.nasa.gov/project/calipso/calipso_table/, last access: 23 November 2020b. a
Niemeier, U., Timmreck, C., Graf, H.-F., Kinne, S., Rast, S., and Self, S.: Initial fate of fine ash and sulfur from large volcanic eruptions, Atmos. Chem. Phys., 9, 9043–9057, https://doi.org/10.5194/acp-9-9043-2009, 2009. a, b, c
Pavolonis, M. J., Heidinger, A. K., and Sieglaff, J.: Automated retrievals of
volcanic ash and dust cloud properties from upwelling infrared measurements,
J. Geophys. Res.-Atmos., 118, 1436–1458, https://doi.org/10.1002/jgrd.50173, 2013. a
Pavolonis, M., Qi, H., and NOAA JPSS Program Office: NOAA JPSS Visible Infrared Imaging Radiometer Suite (VIIRS) Volcanic Ash Detection and Height Environmental Data Record (EDR) from NDE, NOAA National Centers for Environmental Information, https://doi.org/10.7289/V5BK19KS (last access: 10 April 2020), 2017. a
Platnick, S., Ackerman, S., King, M., et al.: MODIS Atmosphere L2 Cloud Product (06_L2), NASA MODIS Adaptive Processing System, Goddard Space Flight Center, USA, https://doi.org/10.5067/MODIS/MYD06_L2.061, 2015a. a
Platnick, S., Ackerman, S., King, M., et al.: MODIS Atmosphere L2 Cloud Product (06_L2), NASA MODIS Adaptive Processing System, Goddard Space Flight Center, USA, https://doi.org/10.5067/MODIS/MOD06_L2.061, 2015b. a
Platnick, S., Meyer, K. G., Heidinger, A. K., and Holz, R.: VIIRS Atmosphere L2 Cloud Properties Product, Version-1, NASA Level-1 and Atmosphere Archive & Distribution System (LAADS) Distributed Active Archive Center (DAAC), Goddard Space Flight Center, USA, https://doi.org/10.5067/VIIRS/CLDPROP_L2_VIIRS_SNPP.011, 2017. a
Peterson, P. K., Pöhler, D., Sihler, H., Zielcke, J., General, S., Frieß, U., Platt, U., Simpson, W. R., Nghiem, S. V., Shepson, P. B., Stirm, B. H., Dhaniyala, S., Wagner, T., Caulton, D. R., Fuentes, J. D., and Pratt, K. A.: Observations of bromine monoxide transport in the Arctic sustained on aerosol particles, Atmos. Chem. Phys., 17, 7567–7579, https://doi.org/10.5194/acp-17-7567-2017, 2017. a, b
Prata, A.: Infrared radiative transfer calculations for volcanic ash clouds,
Geophys. Res. Lett., 16, 1293–1296, 1989. a
Prata, F., Bluth, G., Rose, B., Schneider, D., and Tupper, A.: Comments on
Failures in detecting volcanic ash from a satellite-based technique, Remote
Sens. Environ., 78, 341–346, 2001. a
Prata, A. J., Rose, W. I., Self, S., and O'Brien, D. M.: Global, Long-Term Sulphur Dioxide Measurements from TOVS Data: A New Tool for Studying Explosive Volcanism and Climate, in: Volcanism and the Earth's Atmosphere, 75–92, American Geophysical Union (AGU), ISBN 9781118668542, https://doi.org/10.1029/139GM05, 2004. a
Prata, A. T., Dacre, H. F., Irvine, E. A., Mathieu, E., Shine, K. P., and
Clarkson, R. J.: Calculating and communicating ensemble-based volcanic ash
dosage and concentration risk for aviation, Meteorol. Appl., 26, 253–266,
https://doi.org/10.1002/met.1759, 2019. a
Rieger, D., Bangert, M., Bischoff-Gauss, I., Förstner, J., Lundgren, K., Reinert, D., Schröter, J., Vogel, H., Zängl, G., Ruhnke, R., and Vogel, B.: ICON–ART 1.0 – a new online-coupled model system from the global to regional scale, Geosci. Model Dev., 8, 1659–1676, https://doi.org/10.5194/gmd-8-1659-2015, 2015. a, b, c
Rieger, L. A., Malinina, E. P., Rozanov, A. V., Burrows, J. P., Bourassa, A. E., and Degenstein, D. A.: A study of the approaches used to retrieve aerosol extinction, as applied to limb observations made by OSIRIS and SCIAMACHY, Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, 2018. 2018. a
Riemer, N., Vogel, H., Vogel, B., and Fiedler, F.: Modeling aerosols on the
mesoscale-γ: Treatment of soot aerosol and its radiative effects, J.
Geophys. Res.-Atmos., 108, https://doi.org/10.1029/2003jd003448, 2003. a
Riemer, N., Ault, A. P., West, M., Craig, R. L., and Curtis, J. H.: Aerosol
Mixing State: Measurements, Modeling, and Impacts, Rev. Geophys., 57,
187–249, https://doi.org/10.1029/2018RG000615, 2019. a
Robock, A.: Volcanic eruptions and climate, Rev. Geophys., 38, 191–219,
https://doi.org/10.1029/1998RG000054, 2000. a
Rose, W. and Durant, A.: Fine ash content of explosive eruptions, J. Volcanol.
Geoth. Res., 186, 32–39,
https://doi.org/10.1016/j.jvolgeores.2009.01.010, 2009. a, b
Rozanov, A., Malinina, E., and Vountas, M.: IUP data limb sets, available at: http://www.iup.uni-bremen.de/DataRequest/, last access: 24 November 2020. a
Schmidt, A., Witham, C. S., Theys, N., Richards, N. A. D., Thordarson, T.,
Szpek, K., Feng, W., Hort, M. C., Woolley, A. M., Jones, A. R., Redington,
A. L., Johnson, B. T., Hayward, C. L., and Carslaw, K. S.: Assessing hazards
to aviation from sulfur dioxide emitted by explosive Icelandic eruptions, J.
Geophys. Res.-Atmos., 119, 14180–14196, https://doi.org/10.1002/2014jd022070, 2014. a, b
Schröter, J., Rieger, D., Stassen, C., Vogel, H., Weimer, M., Werchner, S., Förstner, J., Prill, F., Reinert, D., Zängl, G., Giorgetta, M., Ruhnke, R., Vogel, B., and Braesicke, P.: ICON-ART 2.1: a flexible tracer framework and its application for composition studies in numerical weather forecasting and climate simulations, Geosci. Model Dev., 11, 4043–4068, https://doi.org/10.5194/gmd-11-4043-2018, 2018. a
Seinfeld, J. H. and Pandis, S. N.: Atmospheric Chemistry and Physics, Wiley
John & Sons, 3rd edition, 1152 pp., ISBN 978-1-118-94740-1, 2016. a
Shao, Y., Wyrwoll, K.-H., Chappell, A., Huang, J., Lin, Z., Mctainsh, G. H.,
Mikami, M., Tanaka, T. Y., Wang, X., and Yoon, S.: Dust cycle: An emerging
core theme in Earth system science, Aeolian Res., 2, 181–204,
https://doi.org/10.1016/j.aeolia.2011.02.001, 2011. a
Tabazadeh, A. and Turco, R. P.: Stratospheric Chlorine Injection by Volcanic
Eruptions: HCI Scavenging and Implications for Ozone, Science (New York,
N.Y.), 260, 1082–1086, https://doi.org/10.1126/science.260.5111.1082, 1993. a
Textor, C., Graf, H.-F., Timmreck, C., and Robock, A.: Emissions from
volcanoes, in: Emissions of Atmospheric Trace Compounds, edited by: Granier, C., Artaxo, P., and Reeves, C. E., pp. 269–303, Springer Netherlands, Dordrecht, ISBN 978-1-4020-2167-1, https://doi.org/10.1007/978-1-4020-2167-1, 2004. a
Textor, C., Graf, H. F., Herzog, M., Oberhuber, J. M., Rose, W. I., and Ernst, G. G. J.: Volcanic particle aggregation in explosive eruption columns Part II: Numerical experiments, J. Volcanol. Geoth. Res., 150, 378–394,
https://doi.org/10.1016/j.jvolgeores.2005.09.008, 2006. a
Theys, N., De Smedt, I., Yu, H., Danckaert, T., van Gent, J., Hörmann, C., Wagner, T., Hedelt, P., Bauer, H., Romahn, F., Pedergnana, M., Loyola, D., and Van Roozendael, M.: Sulfur dioxide retrievals from TROPOMI onboard Sentinel-5 Precursor: algorithm theoretical basis, Atmos. Meas. Tech., 10, 119–153, https://doi.org/10.5194/amt-10-119-2017, 2017. a
Theys, N., Hedelt, P., De Smedt, I., Lerot, C., Yu, H., Vlietinck, J.,
Pedergnana, M., Arellano, S., Galle, B., Fernandez, D., Carlito, C.,
Barrington, C., Taisne, B., Delgado Granados, H., Loyola, D., and
Van Roozendael, M.: Global monitoring of volcanic SO2 degassing with
unprecedented resolution from TROPOMI onboard Sentinel-5 Precursor, Sci.
Rep.-UK, 9, 2643, https://doi.org/10.1038/s41598-019-39279-y, 2019. a
Timmreck, C.: Modeling the climatic effects of large explosive volcanic
eruptions, Wires, Clim. Change, 3, 545–564, https://doi.org/10.1002/wcc.192, 2012. a
Van Eaton, A. R., Mastin, L. G., Herzog, M., Schwaiger, H. F., Schneider,
D. J., Wallace, K. L., and Clarke, A. B.: Hail formation triggers rapid ash
aggregation in volcanic plumes, Nat. Commun., 6, 1–7,
https://doi.org/10.1038/ncomms8860, 2015. a
van Kempen, T. A., van Hees, R. M., Tol, P. J. J., Aben, I., and Hoogeveen, R. W. M.: In-flight calibration and monitoring of the Tropospheric Monitoring Instrument (TROPOMI) short-wave infrared (SWIR) module, Atmos. Meas. Tech., 12, 6827–6844, https://doi.org/10.5194/amt-12-6827-2019, 2019. a
Vernier, J.-P., Fairlie, T. D., Deshler, T., Natarajan, M., Knepp, T., Foster, K., Wienhold, F. G., Bedka, K. M., Thomason, L., and Trepte, C.: In situ and space-based observations of the Kelud volcanic plume: The persistence of ash in the lower stratosphere, J. Geophys. Res.-Atmos., 121, 11104–11118, https://doi.org/10.1002/2016JD025344, 2016. a
Vogel, A., Diplas, S., Durant, A. J., Azar, A. S., Sunding, M. F., Rose, W. I., Sytchkova, A., Bonadonna, C., Krüger, K., and Stohl, A.: Reference data set of volcanic ash physicochemical and optical properties, J. Geophys. Res.-Atmos., 122, 9485–9514, https://doi.org/10.1002/2016JD026328, 2017. a, b
Vogel, B., Vogel, H., Bäumer, D., Bangert, M., Lundgren, K., Rinke, R., and Stanelle, T.: The comprehensive model system COSMO-ART – Radiative impact of aerosol on the state of the atmosphere on the regional scale, Atmos. Chem. Phys., 9, 8661–8680, https://doi.org/10.5194/acp-9-8661-2009, 2009. a
von Savigny, C., Timmreck, C., Buehler, S., Burrows, J., Giorgetta, M., Hegerl, G., Horvath, A., Hoshyaripour, G. A., Hoose, C., Quaas, J., Malinina, E., Rozanov, A., Schmidt, H., Thomason, L., Toohey, M., and Vogel, B.: The
Research Unit VolImpact: Revisiting the volcanic impact on atmosphere and
climate? preparations for the next big volcanic eruption, Meteorol.
Z., 29, 3–18, https://doi.org/10.1127/metz/2019/0999, 2020. a
Walter, C.: Simulationen der Ausbreitung von Vulkanasche unter expliziter
Berücksichtigung der optischen Eigenschaften der Aschepartikel, Ph.D.
thesis, Karlsruher Institut für Technologie (KIT), 80, 194 pp., https://doi.org/10.5445/KSP/1000095717, ISBN 978-3-7315-0939-4, 2019. a
Weimer, M., Schröter, J., Eckstein, J., Deetz, K., Neumaier, M., Fischbeck, G., Hu, L., Millet, D. B., Rieger, D., Vogel, H., Vogel, B., Reddmann, T., Kirner, O., Ruhnke, R., and Braesicke, P.: An emission module for ICON-ART 2.0: implementation and simulations of acetone, Geosci. Model Dev., 10, 2471–2494, https://doi.org/10.5194/gmd-10-2471-2017, 2017. a
Weingartner, E., Burtscher, H., and Baltensperger, U.: Hygroscopic properties
of carbon and diesel soot particles, Atmos. Environ., 31, 2311–2327,
https://doi.org/10.1016/S1352-2310(97)00023-X, 1997. a
Wen, S. and Rose, W. I.: Retrieval of sizes and total masses of particles in
volcanic clouds using AVHRR bands 4 and 5, J. Geophys. Res.-Atmos., 99,
5421–5431, 1994. a
Wernli, H., Paulat, M., Hagen, M., and Frei, C.: SAL-A Novel Quality Measure
for the Verification of Quantitative Precipitation Forecasts, Mon. Weather
Rev., 136, 4470–4487, https://doi.org/10.1175/2008MWR2415.1, 2008.
a, b
Wernli, H., Hofmann, C., and Zimmer, M.: Spatial Forecast Verification Methods Intercomparison Project: Application of the SAL Technique, Weather Forecast., 24, 1472–1484, https://doi.org/10.1175/2009WAF2222271.1, 2009. a
Western, L. M., Watson, M. I., and Francis, P. N.: Uncertainty in two-channel
infrared remote sensing retrievals of a well-characterised volcanic ash
cloud, B. Volcanol., 77, 67, https://doi.org/10.1007/s00445-015-0950-y, 2015. a
Yu, P., Toon, O. B., Bardeen, C. G., Zhu, Y., Rosenlof, K. H., Portmann, R. W., Thornberry, T. D., Gao, R.-S., Davis, S. M., Wolf, E. T., de Gouw, J.,
Peterson, D. A., Fromm, M. D., and Robock, A.: Black carbon lofts wildfire
smoke high into the stratosphere to form a persistent plume, Science, 365,
587–590, https://doi.org/10.1126/science.aax1748, 2019. a, b
Zängl, G., Reinert, D., Rípodas, P., and Baldauf, M.: The ICON
(ICOsahedral Non-hydrostatic) modelling framework of DWD and MPI-M:
Description of the non-hydrostatic dynamical core, Q. J. Roy. Meteor.
Soc., 141, 563–579, https://doi.org/10.1002/qj.2378, 2015. a, b, c
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Short summary
Volcanic aerosols endanger aircraft and thus disrupt air travel globally. For aviation safety, it is vital to know the location and lifetime of such aerosols in the atmosphere. Here we show that the interaction of volcanic particles with each other eventually reduces their atmospheric lifetime. Moreover, we demonstrate that sunlight heats these particles, which lifts them several kilometers in the atmosphere. These findings support a more reliable forecast of volcanic aerosol dispersion.
Volcanic aerosols endanger aircraft and thus disrupt air travel globally. For aviation safety,...
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