Special issue  

The 2019 Raikoke eruption emitted an estimated 1.5±0.2 Tg of volcanic sulfur dioxide (SO₂) into the atmosphere, which makes it the largest volcanic SO₂ perturbation in the upper troposphere and lower stratosphere since the 2011 eruption of Nabro. The 2019 Raikoke eruption triggered numerous discussions among scientists involved in the SPARC Volcano Response (VolRes) initiative and provides an excellent opportunity to test our understanding of processes involved in the formation, growth and removal of volcanic aerosols in the atmosphere. Remote sensing measurements from geostationary and low-orbiting satellites with ultraviolet, visible, and infrared sensors (HIMAWARI-8, OMPS/NPP, OMI/Aura, TROPOMI/SP5, IASI/MeteopA-B-C, AIRS/Aqua, CALIOP/CALIPSO, SAGE III/ISS) provided a wealth of information on the SO₂ concentration, ash and sulfate aerosol particle optical properties from the initial injection through to the growth and removal of aerosols. This eruption therefore provides an excellent opportunity to inter-compare satellite observations and validate the different retrievals for SO₂ and volcanic aerosol properties from new satellite sensors such as TROPOMI. After the initial injection into altitudes up to 15–16 km, the plume reached 25–26 km altitude in late 2019, which corresponds to a fast vertical ascent that appears unusual compared to previous eruptions. The fast vertical ascent of the 2019 Raikoke plume may suggest an influence of smoke aerosol from large wildfires that took place in Canada and Siberia around the time of the eruption. The veil of aerosol particles from Raikoke 2019 has noticeably reduced the transparency of the stratosphere and detailed information and measurements on the aerosol properties will be useful to constrain atmospheric and climate model simulations.