Articles | Volume 19, issue 7
https://doi.org/10.5194/acp-19-5269-2019
https://doi.org/10.5194/acp-19-5269-2019
Research article
 | 
17 Apr 2019
Research article |  | 17 Apr 2019

Deriving stratospheric age of air spectra using an idealized set of chemically active trace gases

Marius Hauck, Frauke Fritsch, Hella Garny, and Andreas Engel

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Cited articles

Abalos, M., Legras, B., Ploeger, F., and Randel, W. J.: Evaluating the advective Brewer-Dobson circulation in three reanalyses for the period 1979–2012, J. Geophys. Res., 120, 7534–7554, https://doi.org/10.1002/2015JD023182, 2015. 
Andrews, A. E., Boering, K. A., Daube, B. C., Wofsy, S. C., Hintsa, E. J., Weinstock, E. M., and Bui, T. P.: Empirical age spectra for the lower tropical stratosphere from in situ observations of CO2: Implications for stratospheric transport, J. Geophys. Res., 104, 26581–26595, https://doi.org/10.1029/1999JD900150, 1999. 
Andrews, A. E., Boering, K. A., Wofsy, S. C., Daube, B. C., Jones, D. B., Alex, S., Loewenstein, M., Podolske, J. R., and Strahan, S. E.: Empirical age spectra for the midlatitude lower stratosphere from in situ observations of CO2: Quantitative evidence for a subtropical “barrier” to horizontal transport, J. Geophys. Res., 106, 10257–10274, https://doi.org/10.1029/2000JD900703, 2001b. 
Appenzeller, C., Holton, J. R., and Rosenlof, K. H.: Seasonal variation of mass transport across the tropopause, J. Geophys. Res., 101, 15071–15078, https://doi.org/10.1029/96JD00821, 1996. 
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The paper presents a modified method to invert mixing ratios of chemically active tracers into stratospheric age spectra. It features an imposed seasonal cycle to include transport seasonality into the spectra. An idealized set of tracers from a model is used as proof of concept and results are in good agreement with the model reference, except for the lowermost stratosphere. Applicability is studied with focus on number of tracers and error tolerance, providing a starting point for future work.
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