Articles | Volume 18, issue 18
https://doi.org/10.5194/acp-18-13305-2018
https://doi.org/10.5194/acp-18-13305-2018
Research article
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17 Sep 2018
Research article | Highlight paper |  | 17 Sep 2018

Inverse modelling of CF4 and NF3 emissions in East Asia

Tim Arnold, Alistair J. Manning, Jooil Kim, Shanlan Li, Helen Webster, David Thomson, Jens Mühle, Ray F. Weiss, Sunyoung Park, and Simon O'Doherty

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Cited articles

Arnold, T., Mühle, J., Salameh, P. K., Harth, C. M., Ivy, D. J., and Weiss, R. F.: Automated measurement of nitrogen trifluoride in ambient air, Anal. Chem., 84, 4798–4804, https://doi.org/10.1021/ac300373e, 2012. 
Arnold, T., Harth, C., Mühle, J., Manning, A. J., Salameh, P., Kim, J., Ivy, D. J., Steele, L. P., Petrenko, V. V., Severinghaus, J. P., Baggenstos, D., and Weiss, R. F.: Nitrogen trifluoride global emissions estimated from updated atmospheric measurements, P. Natl. Acad. Sci. USA, 110, 2019–2034, 2013. 
Bronfin, B. R. and Hazlett, R. N.: Synthesis of nitrogen fluorides in a plasma jet, Ind. Eng. Chem. Fund., 5, 472–478, https://doi.org/10.1021/i160020a007, 1966. 
Chang, M. B. and Chang, J.-S.: Abatement of PFCs from Semiconductor Manufacturing Processes by Nonthermal Plasma Technologies:? A Critical Review, Ind. Eng. Chem. Res., 45, 4101–4109, https://doi.org/10.1021/ie051227b, 2006. 
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Short summary
Emissions of carbon tetrafluoride CF4, NF3 and CHF3 in east Asia have been calculated using atmospheric measurements and an atmospheric transport model. We calculate emissions of CF4 to be quite constant between the years 2008 and 2015 for both China and South Korea, with 2015 emissions calculated at 4.33 ± 2.65 Gg yr-1 and 0.36 ± 0.11 Gg yr-1, respectively. Emission estimates of NF3 from South Korea could be made with relatively small uncertainty at 0.6 ± 0.07 Gg yr-1 in 2015.
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