Articles | Volume 16, issue 16
https://doi.org/10.5194/acp-16-10385-2016
https://doi.org/10.5194/acp-16-10385-2016
Research article
 | 
17 Aug 2016
Research article |  | 17 Aug 2016

In-cloud measurements highlight the role of aerosol hygroscopicity in cloud droplet formation

Olli Väisänen, Antti Ruuskanen, Arttu Ylisirniö, Pasi Miettinen, Harri Portin, Liqing Hao, Ari Leskinen, Mika Komppula, Sami Romakkaniemi, Kari E. J. Lehtinen, and Annele Virtanen

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Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Cited articles

Ahmad, I., Mielonen, T., Grosvenor, D. P., Portin, H. J., Arola, A., Mikkonen, S., Kuhn, T., Leskinen, A., Joutsensaari, J., Komppula, M., Lehtinen, K. E. J., Laaksonen, A., and Romakkaniemi, S.: Long-term measurements of cloud droplet concentrations and aerosol-cloud interactions in continental boundary layer clouds, Tellus B, 65, 20138, https://doi.org/10.3402/Tellusb.V65i0.20138, 2013.
Almeida, G. P., Brito, J., Morales, C. A., Andrade, M. F., and Artaxo, P.: Measured and modelled cloud condensation nuclei (CCN) concentration in Sao Paulo, Brazil: the importance of aerosol size-resolved chemical composition on CCN concentration prediction, Atmos. Chem. Phys., 14, 7559–7572, https://doi.org/10.5194/acp-14-7559-2014, 2014.
Andreae, M. O. and Rosenfeld, D.: Aerosol-cloud-precipitation interactions. Part 1. The nature and sources of cloud-active aerosols, Earth.-Sci. Rev., 89, 13–41, https://doi.org/10.1016/j.earscirev.2008.03.001, 2008.
Anttila, T., Vaattovaara, P., Komppula, M., Hyvärinen, A.-P., Lihavainen, H., Kerminen, V.-M., and Laaksonen, A.: Size-dependent activation of aerosols into cloud droplets at a subarctic background site during the second Pallas Cloud Experiment (2nd PaCE): method development and data evaluation, Atmos. Chem. Phys., 9, 4841–4854, https://doi.org/10.5194/acp-9-4841-2009, 2009.
Asmi, E., Freney, E., Hervo, M., Picard, D., Rose, C., Colomb, A., and Sellegri, K.: Aerosol cloud activation in summer and winter at puy-de-Dome high altitude site in France, Atmos. Chem. Phys., 12, 11589–11607, https://doi.org/10.5194/acp-12-11589-2012, 2012.
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Short summary
In-cloud measurements of aerosol hygroscopicity and cloud droplet activation were conducted in Kuopio, Finland. According to the observations, the less hygroscopic accumulation mode particles were present in the non-activated aerosol, whereas the more hygroscopic particles were scavenged into cloud droplets. The results illustrate the sensitivity of cloud droplet formation to varying chemical composition and highlight the need for proper treatment of anthropogenic aerosols in CCN predictions.
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