Articles | Volume 14, issue 18
https://doi.org/10.5194/acp-14-9583-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-9583-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
16 Sep 2014
Research article |
| 16 Sep 2014
Comparison of IASI water vapor retrieval with H2O-Raman lidar in the framework of the Mediterranean HyMeX and ChArMEx programs
P. Chazette
Laboratoire des Sciences du Climat et de l'Environnement (LSCE), UMR8212, Laboratoire mixte CEA-CNRS-UVSQ, CEA Saclay, 91191 Gif-sur-Yvette, France
F. Marnas
Laboratoire des Sciences du Climat et de l'Environnement (LSCE), UMR8212, Laboratoire mixte CEA-CNRS-UVSQ, CEA Saclay, 91191 Gif-sur-Yvette, France
J. Totems
Laboratoire des Sciences du Climat et de l'Environnement (LSCE), UMR8212, Laboratoire mixte CEA-CNRS-UVSQ, CEA Saclay, 91191 Gif-sur-Yvette, France
Laboratoire des Sciences du Climat et de l'Environnement (LSCE), UMR8212, Laboratoire mixte CEA-CNRS-UVSQ, CEA Saclay, 91191 Gif-sur-Yvette, France
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Atmos. Chem. Phys., 22, 5701–5724, https://doi.org/10.5194/acp-22-5701-2022, https://doi.org/10.5194/acp-22-5701-2022, 2022
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Sandrine Bony, Marie Lothon, Julien Delanoë, Pierre Coutris, Jean-Claude Etienne, Franziska Aemisegger, Anna Lea Albright, Thierry André, Hubert Bellec, Alexandre Baron, Jean-François Bourdinot, Pierre-Etienne Brilouet, Aurélien Bourdon, Jean-Christophe Canonici, Christophe Caudoux, Patrick Chazette, Michel Cluzeau, Céline Cornet, Jean-Philippe Desbios, Dominique Duchanoy, Cyrille Flamant, Benjamin Fildier, Christophe Gourbeyre, Laurent Guiraud, Tetyana Jiang, Claude Lainard, Christophe Le Gac, Christian Lendroit, Julien Lernould, Thierry Perrin, Frédéric Pouvesle, Pascal Richard, Nicolas Rochetin, Kevin Salaün, Alfons Schwarzenboeck, Guillaume Seurat, Bjorn Stevens, Julien Totems, Ludovic Touzé-Peiffer, Gilles Vergez, Jessica Vial, Leonie Villiger, and Raphaela Vogel
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Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Patrick Chazette, Cyrille Flamant, Harald Sodemann, Julien Totems, Anne Monod, Elsa Dieudonné, Alexandre Baron, Andrew Seidl, Hans Christian Steen-Larsen, Pascal Doira, Amandine Durand, and Sylvain Ravier
Atmos. Chem. Phys., 21, 10911–10937, https://doi.org/10.5194/acp-21-10911-2021, https://doi.org/10.5194/acp-21-10911-2021, 2021
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To gain understanding on the vertical structure of atmospheric water vapour above mountain lakes and to assess its link to the isotopic composition of the lake water and small-scale dynamics, the L-WAIVE field campaign was conducted in the Annecy valley in the French Alps in June 2019. Based on a synergy between ground-based, boat-borne, and airborne measuring platforms, significant gradients of isotopic content have been revealed at the transitions to the lake and to the free troposphere.
Patrick Chazette, Julien Totems, Alexandre Baron, Cyrille Flamant, and Sandrine Bony
Earth Syst. Sci. Data, 12, 2919–2936, https://doi.org/10.5194/essd-12-2919-2020, https://doi.org/10.5194/essd-12-2919-2020, 2020
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To characterize the trade-wind cumuli for climate change purposes, 20 ATR-42 flights were conducted over the tropical Atlantic, off the coast of Barbados from 23 January to 13 February 2020. These flights were conducted as part of the international EUREC4A (Elucidating the role of cloud–circulation coupling in climate) field campaign. A new sampling approach was applied, consisting in using a sidewards-staring lidar. The data are now made available to the international scientific community.
Patrick Chazette
Atmos. Meas. Tech., 13, 4461–4477, https://doi.org/10.5194/amt-13-4461-2020, https://doi.org/10.5194/amt-13-4461-2020, 2020
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By coupling lidar on board a ULA and ground-based lidar measurements, this paper highlights aerosol transport over the Strait of Gibraltar. It shows that the lidar-derived aerosol optical properties can be different from what is commonly accepted. It presents unprecedented vertical profiles over this region and relates them to the origin of air masses. The results are based on ground, airborne, and spaceborne observations, as well as multiple retro-trajectory analyses.
Alexandre Baron, Patrick Chazette, and Julien Totems
Atmos. Chem. Phys., 20, 6749–6768, https://doi.org/10.5194/acp-20-6749-2020, https://doi.org/10.5194/acp-20-6749-2020, 2020
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Two major winter aerosol pollution events have been sampled over the Paris area. They correspond to weather conditions with a high-pressure system. We show that during such events the ground-based particle matter content can be related to lidar-derived aerosol extinction coefficient within the atmospheric planetary boundary layer. This opens a new horizon for the monitoring of intense pollution events from space-borne active sensors.
Patrick Chazette, Cyrille Flamant, Julien Totems, Marco Gaetani, Gwendoline Smith, Alexandre Baron, Xavier Landsheere, Karine Desboeufs, Jean-François Doussin, and Paola Formenti
Atmos. Chem. Phys., 19, 14979–15005, https://doi.org/10.5194/acp-19-14979-2019, https://doi.org/10.5194/acp-19-14979-2019, 2019
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Evolution of the vertical distribution and optical properties of aerosols in the free troposphere is analysed for the first time over the Namibian coast, a region where uncertainties on aerosol–cloud coupling in climate simulations are significant. The high variability of atmospheric aerosol composition is highlighted using a combination of ground-based, airborne and space-borne lidar. Aerosols are mainly transported from Angola, but part of the highest aerosol layer may come from South America.
Valentin Duflot, Pierre Tulet, Olivier Flores, Christelle Barthe, Aurélie Colomb, Laurent Deguillaume, Mickael Vaïtilingom, Anne Perring, Alex Huffman, Mark T. Hernandez, Karine Sellegri, Ellis Robinson, David J. O'Connor, Odessa M. Gomez, Frédéric Burnet, Thierry Bourrianne, Dominique Strasberg, Manon Rocco, Allan K. Bertram, Patrick Chazette, Julien Totems, Jacques Fournel, Pierre Stamenoff, Jean-Marc Metzger, Mathilde Chabasset, Clothilde Rousseau, Eric Bourrianne, Martine Sancelme, Anne-Marie Delort, Rachel E. Wegener, Cedric Chou, and Pablo Elizondo
Atmos. Chem. Phys., 19, 10591–10618, https://doi.org/10.5194/acp-19-10591-2019, https://doi.org/10.5194/acp-19-10591-2019, 2019
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The Forests gAses aeRosols Clouds Exploratory (FARCE) campaign was conducted in March–April 2015 on the tropical island of La Réunion. For the first time, several scientific teams from different disciplines collaborated to provide reference measurements and characterization of La Réunion vegetation, volatile organic compounds (VOCs), biogenic VOCs (BVOCs), (bio)aerosols and composition of clouds, with a strong focus on the Maïdo mount slope area.
Nadia Fourrié, Mathieu Nuret, Pierre Brousseau, Olivier Caumont, Alexis Doerenbecher, Eric Wattrelot, Patrick Moll, Hervé Bénichou, Dominique Puech, Olivier Bock, Pierre Bosser, Patrick Chazette, Cyrille Flamant, Paolo Di Girolamo, Evelyne Richard, and Frédérique Saïd
Geosci. Model Dev., 12, 2657–2678, https://doi.org/10.5194/gmd-12-2657-2019, https://doi.org/10.5194/gmd-12-2657-2019, 2019
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The AROME-WMED (western Mediterranean) model is a dedicated version of the mesoscale Numerical Weather Prediction AROME-France model that ran in real time during the first special observation period of HyMeX. Two reanalyses were performed after the campaign. This paper depicts the main differences between the real-time version and the benefits brought by both HyMeX reanalyses. The second reanalysis is found to be closer to observations than the previous AROME-WMED analyses.
Patrick Chazette, Julien Totems, and Xiaoxia Shang
Atmos. Chem. Phys., 19, 3885–3904, https://doi.org/10.5194/acp-19-3885-2019, https://doi.org/10.5194/acp-19-3885-2019, 2019
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Using a backscatter N2-Raman lidar deployed on the western part of the French Riviera, we investigate the vertical aerosol structure below 5 km. By coupling these observations with spaceborne instruments and trajectory modeling, we highlight plumes of particulate pollutants moving towards the French Riviera. This pollution, mainly due to traffic and petrochemical activities, originates from the Spanish coast (Costa Blanca and Costa Brava–Daurada) and mixes with local emissions.
Xiaoxia Shang, Patrick Chazette, and Julien Totems
Atmos. Meas. Tech., 11, 6525–6538, https://doi.org/10.5194/amt-11-6525-2018, https://doi.org/10.5194/amt-11-6525-2018, 2018
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For the first time, a ground-based N2 Raman lidar sampled smoke plumes originating from a large accidental warehouse fire in the Paris area. We developed a new algorithm, dubbed top-down aerosol optical thickness matching, to characterize the optical properties of the smoke aerosols, without a pre-determined reference zone and in the presence of clouds. The industrial pollution episode was concomitant with the long-range transport of dust aerosols and the presence of an extended stratus cloud.
Patrick Chazette, Jean-Christophe Raut, and Julien Totems
Atmos. Chem. Phys., 18, 13075–13095, https://doi.org/10.5194/acp-18-13075-2018, https://doi.org/10.5194/acp-18-13075-2018, 2018
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We associate aerosol lidar measurements from the ground level and from an ultralight aircraft to improve our knowledge about aerosols above the Arctic circle; we highlight long-range transport of biomass burning aerosols and characterize the aerosol emissions from a flaring facility. The field experiment was performed as part of the Pollution in the ARCtic System (PARCS) project of the French Arctic Initiative, which took place from 13 to 26 May 2016 in northern Norway (over 70 °N).
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Laurent Menut, Cyrille Flamant, Solène Turquety, Adrien Deroubaix, Patrick Chazette, and Rémi Meynadier
Atmos. Chem. Phys., 18, 2687–2707, https://doi.org/10.5194/acp-18-2687-2018, https://doi.org/10.5194/acp-18-2687-2018, 2018
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During the DACCIWA project, the tropospheric chemical composition in large cities along the Gulf of Guinea is modelled using WRF and CHIMERE, with and without biomass burning emissions. The difference shows the net impact of fires on air quality in Lagos and Abidjan.
Gerard Ancellet, Jacques Pelon, Julien Totems, Patrick Chazette, Ariane Bazureau, Michaël Sicard, Tatiana Di Iorio, Francois Dulac, and Marc Mallet
Atmos. Chem. Phys., 16, 4725–4742, https://doi.org/10.5194/acp-16-4725-2016, https://doi.org/10.5194/acp-16-4725-2016, 2016
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A multi-lidar analysis conducted in the Mediterranean basin compares the impact of the long-range transport of North American biomass burning aerosols with the role of frequently observed Saharan dust outbreaks. This paper provides a detailed analysis of the potential North American aerosol sources, their transport to Europe and the mixing of different aerosol sources, using simulations of a particle dispersion model and lidar measurements of the aerosol optical properties.
Julien Totems and Patrick Chazette
Atmos. Meas. Tech., 9, 1083–1094, https://doi.org/10.5194/amt-9-1083-2016, https://doi.org/10.5194/amt-9-1083-2016, 2016
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We present a calibration method for a water vapour Raman lidar, using a meteorological probe lifted by a kite, that was applied during the HyMeX and ChArMEx programs over the Mediterranean. It allowed measuring both the overlap factor of the lidar and the calibration constant with better precision than with simultaneous balloon radiosoundings, as balloons go up faster and can drift during the measurements. Comparisons to other moisture profiles demonstrate the accuracy of the calibrated lidar.
Patrick Chazette, Julien Totems, Gérard Ancellet, Jacques Pelon, and Michaël Sicard
Atmos. Chem. Phys., 16, 2863–2875, https://doi.org/10.5194/acp-16-2863-2016, https://doi.org/10.5194/acp-16-2863-2016, 2016
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We performed synergetic active and passive remote-sensing observations at Minorca (Spain), over more than 3 weeks in spring 2013. We characterized the aerosol optical properties and type using a combination of Rayleigh–Mie–Raman lidar and sun-photometer data. Results show a high variability due to changing atmospheric transport regimes and aerosol sources. Such variability significantly influences the radiative balance through the entire atmosphere and then the climate of the Mediterranean area.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
C. Flamant, J.-P. Chaboureau, P. Chazette, P. Di Girolamo, T. Bourrianne, J. Totems, and M. Cacciani
Atmos. Chem. Phys., 15, 12231–12249, https://doi.org/10.5194/acp-15-12231-2015, https://doi.org/10.5194/acp-15-12231-2015, 2015
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We analyze the direct radiative impact of an intense African dust plume on orographic precipitation in the western Mediterranean in the fall of 2012 using high-resolution simulations from a convection permitting mesoscale model validated against measurements acquired during the first special observation period of HyMeX. We show that the dust's direct radiative effect in such a dynamical environment is not sufficient to impact 24h of accumulated rainfall over the Cevennes in the dust simulation.
E. Dieudonné, P. Chazette, F. Marnas, J. Totems, and X. Shang
Atmos. Chem. Phys., 15, 5007–5026, https://doi.org/10.5194/acp-15-5007-2015, https://doi.org/10.5194/acp-15-5007-2015, 2015
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In June 2013, a ground-based mobile lidar performed the 10,000km ride from Paris to Ulan-Ude, near Lake Baikal. Aerosols have been characterized using two intensive properties: extinction-to-backscatter ratio and particle depolarization ratio. The results highlight spatial variations in the aerosol mix, with more terrigenous particles over Russia than Europe. Wildfire and desert dust plumes were also observed, offering the first optical characterization of dust from the Caspian–Aral region.
Y. Wang, K. N. Sartelet, M. Bocquet, P. Chazette, M. Sicard, G. D'Amico, J. F. Léon, L. Alados-Arboledas, A. Amodeo, P. Augustin, J. Bach, L. Belegante, I. Binietoglou, X. Bush, A. Comerón, H. Delbarre, D. García-Vízcaino, J. L. Guerrero-Rascado, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, F. Molero, N. Montoux, A. Muñoz, C. Muñoz, D. Nicolae, A. Papayannis, G. Pappalardo, J. Preissler, V. Rizi, F. Rocadenbosch, K. Sellegri, F. Wagner, and F. Dulac
Atmos. Chem. Phys., 14, 12031–12053, https://doi.org/10.5194/acp-14-12031-2014, https://doi.org/10.5194/acp-14-12031-2014, 2014
P. Chazette, F. Marnas, and J. Totems
Atmos. Meas. Tech., 7, 1629–1647, https://doi.org/10.5194/amt-7-1629-2014, https://doi.org/10.5194/amt-7-1629-2014, 2014
Y. Wang, K. N. Sartelet, M. Bocquet, and P. Chazette
Atmos. Chem. Phys., 14, 3511–3532, https://doi.org/10.5194/acp-14-3511-2014, https://doi.org/10.5194/acp-14-3511-2014, 2014
Y. Wang, K. N. Sartelet, M. Bocquet, and P. Chazette
Atmos. Chem. Phys., 13, 269–283, https://doi.org/10.5194/acp-13-269-2013, https://doi.org/10.5194/acp-13-269-2013, 2013
Patrick Chazette, Julien Totems, and Frédéric Laly
EGUsphere, https://doi.org/10.5194/egusphere-2024-3583, https://doi.org/10.5194/egusphere-2024-3583, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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The use of active remote sensing instruments to sample the atmospheric environment requires accurate calibration that is stable over time so that measurements are reproducible. This is the case for measurements of atmospheric water vapour using Raman lidar, which are of growing interest in the context of climate risks such as extreme precipitation. This study addresses this issue. It is based on 6 campaigns spread over a period of 7 years between 2016 and 2022.
Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
Atmos. Chem. Phys., 25, 183–197, https://doi.org/10.5194/acp-25-183-2025, https://doi.org/10.5194/acp-25-183-2025, 2025
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollen can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Daniele Zannoni, Hans Christian Steen-Larsen, Harald Sodemann, Iris Thurnherr, Cyrille Flamant, Patrick Chazette, Julien Totems, Martin Werner, and Myriam Raybaut
EGUsphere, https://doi.org/10.5194/egusphere-2024-3394, https://doi.org/10.5194/egusphere-2024-3394, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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High resolution airborne observations reveal that mixing between the free troposphere and surface evapotranspiration flux primarly modulates the water vapor isotopic composition in the lower troposphere. Water vapor isotopes structure variations occur on the scale of 100s of m, underlying the utility of stable isotopes for studying microscale atmospheric dynamics. This study also provides the basis for better validation of water vapor isotopes remote sensing retrievals with surface observations.
Xiaoxia Shang, Maria Filioglou, Julian Hofer, Moritz Haarig, Qiaoyun Hu, Philippe Goloub, Sami Romakkaniemi, and Mika Komppula
EGUsphere, https://doi.org/10.5194/egusphere-2024-3460, https://doi.org/10.5194/egusphere-2024-3460, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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We have developed a new method to analyze the aerosol components in the atmosphere. Using depolarization information of laser light measured by lidar instruments, we can separate the three aerosol types in an aerosol mixture. This method has been applied to study the mineral dust from different regions.
Frédéric Laly, Patrick Chazette, Julien Totems, Jérémy Lagarrigue, Laurent Forges, and Cyrille Flamant
Earth Syst. Sci. Data, 16, 5579–5602, https://doi.org/10.5194/essd-16-5579-2024, https://doi.org/10.5194/essd-16-5579-2024, 2024
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We present a dataset of water vapor mixing ratio profiles acquired during the Water Vapor Lidar Network Assimilation campaign in fall and winter 2022 and summer 2023, using three lidar systems deployed on the western Mediterranean coastline. This innovative campaign provides access to lower-tropospheric water vapor variability to constrain meteorological forecasting models. The scientific objective is to improve forecasting of heavy-precipation events that lead to flash floods and landslides.
Maria Filioglou, Petri Tiitta, Xiaoxia Shang, Ari Leskinen, Pasi Ahola, Sanna Pätsi, Annika Saarto, Ville Vakkari, Uula Isopahkala, and Mika Komppula
EGUsphere, https://doi.org/10.5194/egusphere-2024-3032, https://doi.org/10.5194/egusphere-2024-3032, 2024
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Every year a vast number of people experience allergic reactions due to exposure in airborne pollen. These symptoms are concentration-dependent thus, accurate information of the pollen load in the atmosphere is essential. Moreover, pollen grains and fragments of it are likely to contribute to cloud processes and suppress precipitation. In this work, we estimate the concentration and cloud-relevant parameters of birch pollen in the atmosphere using observations from a ceilometer instrument.
Maëlie Chazette, Patrick Chazette, Ilja M. Reiter, Xiaoxia Shang, Julien Totems, Jean-Philippe Orts, Irène Xueref-Remy, and Nicolas Montes
Biogeosciences, 21, 3289–3303, https://doi.org/10.5194/bg-21-3289-2024, https://doi.org/10.5194/bg-21-3289-2024, 2024
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The approach presented is original in its coupling between field observations and airborne lidar observations. It has been applied to an instrumented reference forest site in the south of France, which is heavily impacted by climate change. It leads to the evaluation of tree heights and ends with assessments of aerial and root carbon stocks. A detailed assessment of uncertainties is presented to add a level of reliability to the scientific products delivered.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
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EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
Patrick Chazette and Jean-Christophe Raut
Atmos. Meas. Tech., 16, 5847–5861, https://doi.org/10.5194/amt-16-5847-2023, https://doi.org/10.5194/amt-16-5847-2023, 2023
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The vertical profiles of the effective radii of ice crystals and ice water content in Arctic semi-transparent stratiform clouds were assessed using quantitative ground-based lidar measurements. The field campaign was part of the Pollution in the ARCtic System (PARCS) project which took place from 13 to 26 May 2016 in Hammerfest (70° 39′ 48″ N, 23° 41′ 00″ E). We show that under certain cloud conditions, lidar measurement combined with a dedicated algorithmic approach is an efficient tool.
Leonie Villiger, Marina Dütsch, Sandrine Bony, Marie Lothon, Stephan Pfahl, Heini Wernli, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Cyrille Flamant, Alfons Schwarzenboeck, Martin Werner, and Franziska Aemisegger
Atmos. Chem. Phys., 23, 14643–14672, https://doi.org/10.5194/acp-23-14643-2023, https://doi.org/10.5194/acp-23-14643-2023, 2023
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This study evaluates three numerical simulations performed with an isotope-enabled weather forecast model and investigates the coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. We show that the simulations reproduce key characteristics of shallow trade-wind clouds as observed during the field experiment EUREC4A and that the spatial distribution of stable-water-vapour isotopes is shaped by the overturning circulation associated with these clouds.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Cyrille Flamant, Marco Gaetani, Jean-Pierre Chaboureau, Patrick Chazette, Juan Cuesta, Stuart John Piketh, and Paola Formenti
Atmos. Chem. Phys., 22, 5701–5724, https://doi.org/10.5194/acp-22-5701-2022, https://doi.org/10.5194/acp-22-5701-2022, 2022
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Rivers of smoke extend from tropical southern Africa towards the Indian Ocean during the winter fire season, controlled by the interaction of tropical easterly waves, and westerly waves at mid latitudes. During the AEROCLO-sA field campaign in 2017, a river of smoke was directly observed over Namibia. In this paper, the evolution and atmospheric drivers of the river of smoke are described, and the role of a mid-latitude cut-off low in lifting the smoke to the upper troposphere is highlighted.
Sandrine Bony, Marie Lothon, Julien Delanoë, Pierre Coutris, Jean-Claude Etienne, Franziska Aemisegger, Anna Lea Albright, Thierry André, Hubert Bellec, Alexandre Baron, Jean-François Bourdinot, Pierre-Etienne Brilouet, Aurélien Bourdon, Jean-Christophe Canonici, Christophe Caudoux, Patrick Chazette, Michel Cluzeau, Céline Cornet, Jean-Philippe Desbios, Dominique Duchanoy, Cyrille Flamant, Benjamin Fildier, Christophe Gourbeyre, Laurent Guiraud, Tetyana Jiang, Claude Lainard, Christophe Le Gac, Christian Lendroit, Julien Lernould, Thierry Perrin, Frédéric Pouvesle, Pascal Richard, Nicolas Rochetin, Kevin Salaün, Alfons Schwarzenboeck, Guillaume Seurat, Bjorn Stevens, Julien Totems, Ludovic Touzé-Peiffer, Gilles Vergez, Jessica Vial, Leonie Villiger, and Raphaela Vogel
Earth Syst. Sci. Data, 14, 2021–2064, https://doi.org/10.5194/essd-14-2021-2022, https://doi.org/10.5194/essd-14-2021-2022, 2022
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The French ATR42 research aircraft participated in the EUREC4A international field campaign that took place in 2020 over the tropical Atlantic, east of Barbados. We present the extensive instrumentation of the aircraft, the research flights and the different measurements. We show that the ATR measurements of humidity, wind, aerosols and cloudiness in the lower atmosphere are robust and consistent with each other. They will make it possible to advance understanding of cloud–climate interactions.
Xiaoxia Shang, Holger Baars, Iwona S. Stachlewska, Ina Mattis, and Mika Komppula
Atmos. Chem. Phys., 22, 3931–3944, https://doi.org/10.5194/acp-22-3931-2022, https://doi.org/10.5194/acp-22-3931-2022, 2022
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This study reports pollen observations at four lidar stations (Hohenpeißenberg, Germany; Kuopio, Finland; Leipzig, Germany; and Warsaw, Poland) during the intensive observation campaign organized in May 2020. A novel simple method for the characterization of the pure pollen is proposed, based on lidar measurements. It was applied to evaluate the pollen depolarization ratio and for the aerosol classifications.
Karine Desboeufs, Franck Fu, Matthieu Bressac, Antonio Tovar-Sánchez, Sylvain Triquet, Jean-François Doussin, Chiara Giorio, Patrick Chazette, Julie Disnaquet, Anaïs Feron, Paola Formenti, Franck Maisonneuve, Araceli Rodríguez-Romero, Pascal Zapf, François Dulac, and Cécile Guieu
Atmos. Chem. Phys., 22, 2309–2332, https://doi.org/10.5194/acp-22-2309-2022, https://doi.org/10.5194/acp-22-2309-2022, 2022
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This article reports the first concurrent sampling of wet deposition samples and surface seawater and was performed during the PEACETIME cruise in the remote Mediterranean (May–June 2017). Through the chemical composition of trace metals (TMs) in these samples, it emphasizes the decrease of atmospheric metal pollution in this area during the last few decades and the critical role of wet deposition as source of TMs for Mediterranean surface seawater, especially for intense dust deposition events.
Patrick Chazette, Alexandre Baron, and Cyrille Flamant
Atmos. Chem. Phys., 22, 1271–1292, https://doi.org/10.5194/acp-22-1271-2022, https://doi.org/10.5194/acp-22-1271-2022, 2022
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Within the framework of the international EUREC4A project, horizontal lidar measurements were carried out over Barbados from the French research aircraft ATR-42. These measurements highlighted the strong heterogeneity of the aerosol field (mainly dust and biomass burning aerosols) and therefore of the associated optical properties. This heterogeneity varies according to meteorological conditions and could significantly modulate the climatic impact of aerosols trapped over the tropical Atlantic.
Julien Totems, Patrick Chazette, and Alexandre Baron
Atmos. Meas. Tech., 14, 7525–7544, https://doi.org/10.5194/amt-14-7525-2021, https://doi.org/10.5194/amt-14-7525-2021, 2021
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We describe in detail the design and calibration of the new Raman channels for the WALI system, going over the important sources of bias and uncertainty on retrieved temperature profiles. For the first time, their impact is investigated using horizontal shots in a homogenous atmosphere: the magnitude of the highlighted biases can be much larger than the targeted absolute accuracy of 1° C. Actual measurement errors are quantified using radiosoundings launched close to the lidar site.
Jonas Hamperl, Clément Capitaine, Jean-Baptiste Dherbecourt, Myriam Raybaut, Patrick Chazette, Julien Totems, Bruno Grouiez, Laurence Régalia, Rosa Santagata, Corinne Evesque, Jean-Michel Melkonian, Antoine Godard, Andrew Seidl, Harald Sodemann, and Cyrille Flamant
Atmos. Meas. Tech., 14, 6675–6693, https://doi.org/10.5194/amt-14-6675-2021, https://doi.org/10.5194/amt-14-6675-2021, 2021
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Laser active remote sensing of tropospheric water vapor is a promising technology for enhancing our understanding of processes governing the global hydrological cycle. We investigate the potential of a ground-based lidar to monitor the main water vapor isotopes at high spatio-temporal resolutions in the lower troposphere. Using a realistic end-to-end simulator, we show that high-precision measurements can be achieved within a range of 1.5 km, in mid-latitude or tropical environments.
Xiaoxia Shang, Tero Mielonen, Antti Lipponen, Elina Giannakaki, Ari Leskinen, Virginie Buchard, Anton S. Darmenov, Antti Kukkurainen, Antti Arola, Ewan O'Connor, Anne Hirsikko, and Mika Komppula
Atmos. Meas. Tech., 14, 6159–6179, https://doi.org/10.5194/amt-14-6159-2021, https://doi.org/10.5194/amt-14-6159-2021, 2021
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The long-range-transported smoke particles from a Canadian wildfire event were observed with a multi-wavelength Raman polarization lidar and a ceilometer over Kuopio, Finland, in June 2019. The optical properties and the mass concentration estimations were reported for such aged smoke aerosols over northern Europe.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Patrick Chazette, Cyrille Flamant, Harald Sodemann, Julien Totems, Anne Monod, Elsa Dieudonné, Alexandre Baron, Andrew Seidl, Hans Christian Steen-Larsen, Pascal Doira, Amandine Durand, and Sylvain Ravier
Atmos. Chem. Phys., 21, 10911–10937, https://doi.org/10.5194/acp-21-10911-2021, https://doi.org/10.5194/acp-21-10911-2021, 2021
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To gain understanding on the vertical structure of atmospheric water vapour above mountain lakes and to assess its link to the isotopic composition of the lake water and small-scale dynamics, the L-WAIVE field campaign was conducted in the Annecy valley in the French Alps in June 2019. Based on a synergy between ground-based, boat-borne, and airborne measuring platforms, significant gradients of isotopic content have been revealed at the transitions to the lake and to the free troposphere.
Stephanie Bohlmann, Xiaoxia Shang, Ville Vakkari, Elina Giannakaki, Ari Leskinen, Kari E. J. Lehtinen, Sanna Pätsi, and Mika Komppula
Atmos. Chem. Phys., 21, 7083–7097, https://doi.org/10.5194/acp-21-7083-2021, https://doi.org/10.5194/acp-21-7083-2021, 2021
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Measurements of the multi-wavelength Raman polarization lidar PollyXT and a Halo Photonics StreamLine Doppler lidar have been combined with measurements of pollen type and concentration using a traditional pollen trap at the rural forest site in Vehmasmäki, Finland. Depolarization ratios were measured at three wavelengths. High depolarization ratios were detected during an event with high birch and spruce pollen concentrations and a wavelength dependence of the depolarization ratio was observed.
Xiaoxia Shang, Elina Giannakaki, Stephanie Bohlmann, Maria Filioglou, Annika Saarto, Antti Ruuskanen, Ari Leskinen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 15323–15339, https://doi.org/10.5194/acp-20-15323-2020, https://doi.org/10.5194/acp-20-15323-2020, 2020
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Measurements of the multi-wavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at a rural forest site in Kuopio, Finland. The depolarization ratio was enhanced when there were pollen grains in the atmosphere, illustrating the potential of lidar to track pollen grains in the atmosphere. The depolarization ratio of pure pollen particles was assessed for birch and pine pollen using a novel algorithm.
Patrick Chazette, Julien Totems, Alexandre Baron, Cyrille Flamant, and Sandrine Bony
Earth Syst. Sci. Data, 12, 2919–2936, https://doi.org/10.5194/essd-12-2919-2020, https://doi.org/10.5194/essd-12-2919-2020, 2020
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To characterize the trade-wind cumuli for climate change purposes, 20 ATR-42 flights were conducted over the tropical Atlantic, off the coast of Barbados from 23 January to 13 February 2020. These flights were conducted as part of the international EUREC4A (Elucidating the role of cloud–circulation coupling in climate) field campaign. A new sampling approach was applied, consisting in using a sidewards-staring lidar. The data are now made available to the international scientific community.
Patrick Chazette
Atmos. Meas. Tech., 13, 4461–4477, https://doi.org/10.5194/amt-13-4461-2020, https://doi.org/10.5194/amt-13-4461-2020, 2020
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By coupling lidar on board a ULA and ground-based lidar measurements, this paper highlights aerosol transport over the Strait of Gibraltar. It shows that the lidar-derived aerosol optical properties can be different from what is commonly accepted. It presents unprecedented vertical profiles over this region and relates them to the origin of air masses. The results are based on ground, airborne, and spaceborne observations, as well as multiple retro-trajectory analyses.
Maria Filioglou, Elina Giannakaki, John Backman, Jutta Kesti, Anne Hirsikko, Ronny Engelmann, Ewan O'Connor, Jari T. T. Leskinen, Xiaoxia Shang, Hannele Korhonen, Heikki Lihavainen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 8909–8922, https://doi.org/10.5194/acp-20-8909-2020, https://doi.org/10.5194/acp-20-8909-2020, 2020
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Dust optical properties are region-dependent. Saharan, Asian, and Arabian dusts do not pose similar optical properties in terms of lidar ratios; thus, a universal lidar ratio for dust particles will lead to biases. The present study analyses observations over the United Arab Emirates, quantifying the optical and geometrical extents of the aerosol layers in the area, providing at the same time the Arabian dust properties along with chemical analysis of dust samples collected in the region.
Alexandre Baron, Patrick Chazette, and Julien Totems
Atmos. Chem. Phys., 20, 6749–6768, https://doi.org/10.5194/acp-20-6749-2020, https://doi.org/10.5194/acp-20-6749-2020, 2020
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Two major winter aerosol pollution events have been sampled over the Paris area. They correspond to weather conditions with a high-pressure system. We show that during such events the ground-based particle matter content can be related to lidar-derived aerosol extinction coefficient within the atmospheric planetary boundary layer. This opens a new horizon for the monitoring of intense pollution events from space-borne active sensors.
Patrick Chazette, Cyrille Flamant, Julien Totems, Marco Gaetani, Gwendoline Smith, Alexandre Baron, Xavier Landsheere, Karine Desboeufs, Jean-François Doussin, and Paola Formenti
Atmos. Chem. Phys., 19, 14979–15005, https://doi.org/10.5194/acp-19-14979-2019, https://doi.org/10.5194/acp-19-14979-2019, 2019
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Evolution of the vertical distribution and optical properties of aerosols in the free troposphere is analysed for the first time over the Namibian coast, a region where uncertainties on aerosol–cloud coupling in climate simulations are significant. The high variability of atmospheric aerosol composition is highlighted using a combination of ground-based, airborne and space-borne lidar. Aerosols are mainly transported from Angola, but part of the highest aerosol layer may come from South America.
Stephanie Bohlmann, Xiaoxia Shang, Elina Giannakaki, Maria Filioglou, Annika Saarto, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 19, 14559–14569, https://doi.org/10.5194/acp-19-14559-2019, https://doi.org/10.5194/acp-19-14559-2019, 2019
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Measurements of the multiwavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at the rural forest site in Vehmasmäki, Finland. High particle depolarization ratios were observed during an intense pollination event of birch pollen occasionally mixed with spruce pollen. Our observations illustrate the potential of the particle depolarization ratio to track pollen grains in the atmosphere.
Valentin Duflot, Pierre Tulet, Olivier Flores, Christelle Barthe, Aurélie Colomb, Laurent Deguillaume, Mickael Vaïtilingom, Anne Perring, Alex Huffman, Mark T. Hernandez, Karine Sellegri, Ellis Robinson, David J. O'Connor, Odessa M. Gomez, Frédéric Burnet, Thierry Bourrianne, Dominique Strasberg, Manon Rocco, Allan K. Bertram, Patrick Chazette, Julien Totems, Jacques Fournel, Pierre Stamenoff, Jean-Marc Metzger, Mathilde Chabasset, Clothilde Rousseau, Eric Bourrianne, Martine Sancelme, Anne-Marie Delort, Rachel E. Wegener, Cedric Chou, and Pablo Elizondo
Atmos. Chem. Phys., 19, 10591–10618, https://doi.org/10.5194/acp-19-10591-2019, https://doi.org/10.5194/acp-19-10591-2019, 2019
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The Forests gAses aeRosols Clouds Exploratory (FARCE) campaign was conducted in March–April 2015 on the tropical island of La Réunion. For the first time, several scientific teams from different disciplines collaborated to provide reference measurements and characterization of La Réunion vegetation, volatile organic compounds (VOCs), biogenic VOCs (BVOCs), (bio)aerosols and composition of clouds, with a strong focus on the Maïdo mount slope area.
Nadia Fourrié, Mathieu Nuret, Pierre Brousseau, Olivier Caumont, Alexis Doerenbecher, Eric Wattrelot, Patrick Moll, Hervé Bénichou, Dominique Puech, Olivier Bock, Pierre Bosser, Patrick Chazette, Cyrille Flamant, Paolo Di Girolamo, Evelyne Richard, and Frédérique Saïd
Geosci. Model Dev., 12, 2657–2678, https://doi.org/10.5194/gmd-12-2657-2019, https://doi.org/10.5194/gmd-12-2657-2019, 2019
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The AROME-WMED (western Mediterranean) model is a dedicated version of the mesoscale Numerical Weather Prediction AROME-France model that ran in real time during the first special observation period of HyMeX. Two reanalyses were performed after the campaign. This paper depicts the main differences between the real-time version and the benefits brought by both HyMeX reanalyses. The second reanalysis is found to be closer to observations than the previous AROME-WMED analyses.
Sieglinde Callewaert, Sophie Vandenbussche, Nicolas Kumps, Arve Kylling, Xiaoxia Shang, Mika Komppula, Philippe Goloub, and Martine De Mazière
Atmos. Meas. Tech., 12, 3673–3698, https://doi.org/10.5194/amt-12-3673-2019, https://doi.org/10.5194/amt-12-3673-2019, 2019
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This article presents the updated MAPIR algorithm, which uses infrared satellite data to obtain the global 3-D distribution of mineral aerosols. A description of the method together with its technical improvements is given. Additionally, a 10-year data set was generated and used to evaluate this new algorithm against AERONET, CALIOP, CATS and two ground-based lidar stations. We have shown that the new MAPIR algorithm provides reliable aerosol optical depth and dust layer mean altitude profiles.
Patrick Chazette, Julien Totems, and Xiaoxia Shang
Atmos. Chem. Phys., 19, 3885–3904, https://doi.org/10.5194/acp-19-3885-2019, https://doi.org/10.5194/acp-19-3885-2019, 2019
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Using a backscatter N2-Raman lidar deployed on the western part of the French Riviera, we investigate the vertical aerosol structure below 5 km. By coupling these observations with spaceborne instruments and trajectory modeling, we highlight plumes of particulate pollutants moving towards the French Riviera. This pollution, mainly due to traffic and petrochemical activities, originates from the Spanish coast (Costa Blanca and Costa Brava–Daurada) and mixes with local emissions.
Xiaoxia Shang, Patrick Chazette, and Julien Totems
Atmos. Meas. Tech., 11, 6525–6538, https://doi.org/10.5194/amt-11-6525-2018, https://doi.org/10.5194/amt-11-6525-2018, 2018
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For the first time, a ground-based N2 Raman lidar sampled smoke plumes originating from a large accidental warehouse fire in the Paris area. We developed a new algorithm, dubbed top-down aerosol optical thickness matching, to characterize the optical properties of the smoke aerosols, without a pre-determined reference zone and in the presence of clouds. The industrial pollution episode was concomitant with the long-range transport of dust aerosols and the presence of an extended stratus cloud.
Yoann Tellier, Clémence Pierangelo, Martin Wirth, Fabien Gibert, and Fabien Marnas
Atmos. Meas. Tech., 11, 5865–5884, https://doi.org/10.5194/amt-11-5865-2018, https://doi.org/10.5194/amt-11-5865-2018, 2018
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The French and German space agencies (CNES, DLR) are currently developing MERLIN, a satellite that will measure atmospheric concentration of methane, a powerful greenhouse gas. To reach the desired precision, horizontally averaging the measurements along the satellite track is performed but leads to a processing bias due to non-linear equations. This article studies the processing biases for several averaging schemes and bias correction algorithms and recommends a best approach to limit biases.
Patrick Chazette, Jean-Christophe Raut, and Julien Totems
Atmos. Chem. Phys., 18, 13075–13095, https://doi.org/10.5194/acp-18-13075-2018, https://doi.org/10.5194/acp-18-13075-2018, 2018
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We associate aerosol lidar measurements from the ground level and from an ultralight aircraft to improve our knowledge about aerosols above the Arctic circle; we highlight long-range transport of biomass burning aerosols and characterize the aerosol emissions from a flaring facility. The field experiment was performed as part of the Pollution in the ARCtic System (PARCS) project of the French Arctic Initiative, which took place from 13 to 26 May 2016 in northern Norway (over 70 °N).
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Laurent Menut, Cyrille Flamant, Solène Turquety, Adrien Deroubaix, Patrick Chazette, and Rémi Meynadier
Atmos. Chem. Phys., 18, 2687–2707, https://doi.org/10.5194/acp-18-2687-2018, https://doi.org/10.5194/acp-18-2687-2018, 2018
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During the DACCIWA project, the tropospheric chemical composition in large cities along the Gulf of Guinea is modelled using WRF and CHIMERE, with and without biomass burning emissions. The difference shows the net impact of fires on air quality in Lagos and Abidjan.
Jean-Pierre Chaboureau, Cyrille Flamant, Thibaut Dauhut, Cécile Kocha, Jean-Philippe Lafore, Chistophe Lavaysse, Fabien Marnas, Mohamed Mokhtari, Jacques Pelon, Irene Reinares Martínez, Kerstin Schepanski, and Pierre Tulet
Atmos. Chem. Phys., 16, 6977–6995, https://doi.org/10.5194/acp-16-6977-2016, https://doi.org/10.5194/acp-16-6977-2016, 2016
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The Fennec field campaign conducted in June 2011 led to the first observational data set ever obtained that documents the Saharan atmospheric boundary layer under the influence of the heat low. In addition to the aircraft operation, four dust forecasts were run at low and high resolutions with convection-parameterizing and convection-permitting models, respectively. The unique airborne and ground-based data sets allowed the first ever intercomparison of dust forecasts over the western Sahara.
Gerard Ancellet, Jacques Pelon, Julien Totems, Patrick Chazette, Ariane Bazureau, Michaël Sicard, Tatiana Di Iorio, Francois Dulac, and Marc Mallet
Atmos. Chem. Phys., 16, 4725–4742, https://doi.org/10.5194/acp-16-4725-2016, https://doi.org/10.5194/acp-16-4725-2016, 2016
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A multi-lidar analysis conducted in the Mediterranean basin compares the impact of the long-range transport of North American biomass burning aerosols with the role of frequently observed Saharan dust outbreaks. This paper provides a detailed analysis of the potential North American aerosol sources, their transport to Europe and the mixing of different aerosol sources, using simulations of a particle dispersion model and lidar measurements of the aerosol optical properties.
Julien Totems and Patrick Chazette
Atmos. Meas. Tech., 9, 1083–1094, https://doi.org/10.5194/amt-9-1083-2016, https://doi.org/10.5194/amt-9-1083-2016, 2016
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We present a calibration method for a water vapour Raman lidar, using a meteorological probe lifted by a kite, that was applied during the HyMeX and ChArMEx programs over the Mediterranean. It allowed measuring both the overlap factor of the lidar and the calibration constant with better precision than with simultaneous balloon radiosoundings, as balloons go up faster and can drift during the measurements. Comparisons to other moisture profiles demonstrate the accuracy of the calibrated lidar.
Patrick Chazette, Julien Totems, Gérard Ancellet, Jacques Pelon, and Michaël Sicard
Atmos. Chem. Phys., 16, 2863–2875, https://doi.org/10.5194/acp-16-2863-2016, https://doi.org/10.5194/acp-16-2863-2016, 2016
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We performed synergetic active and passive remote-sensing observations at Minorca (Spain), over more than 3 weeks in spring 2013. We characterized the aerosol optical properties and type using a combination of Rayleigh–Mie–Raman lidar and sun-photometer data. Results show a high variability due to changing atmospheric transport regimes and aerosol sources. Such variability significantly influences the radiative balance through the entire atmosphere and then the climate of the Mediterranean area.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
C. Flamant, J.-P. Chaboureau, P. Chazette, P. Di Girolamo, T. Bourrianne, J. Totems, and M. Cacciani
Atmos. Chem. Phys., 15, 12231–12249, https://doi.org/10.5194/acp-15-12231-2015, https://doi.org/10.5194/acp-15-12231-2015, 2015
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We analyze the direct radiative impact of an intense African dust plume on orographic precipitation in the western Mediterranean in the fall of 2012 using high-resolution simulations from a convection permitting mesoscale model validated against measurements acquired during the first special observation period of HyMeX. We show that the dust's direct radiative effect in such a dynamical environment is not sufficient to impact 24h of accumulated rainfall over the Cevennes in the dust simulation.
E. Dieudonné, P. Chazette, F. Marnas, J. Totems, and X. Shang
Atmos. Chem. Phys., 15, 5007–5026, https://doi.org/10.5194/acp-15-5007-2015, https://doi.org/10.5194/acp-15-5007-2015, 2015
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In June 2013, a ground-based mobile lidar performed the 10,000km ride from Paris to Ulan-Ude, near Lake Baikal. Aerosols have been characterized using two intensive properties: extinction-to-backscatter ratio and particle depolarization ratio. The results highlight spatial variations in the aerosol mix, with more terrigenous particles over Russia than Europe. Wildfire and desert dust plumes were also observed, offering the first optical characterization of dust from the Caspian–Aral region.
Y. Wang, K. N. Sartelet, M. Bocquet, P. Chazette, M. Sicard, G. D'Amico, J. F. Léon, L. Alados-Arboledas, A. Amodeo, P. Augustin, J. Bach, L. Belegante, I. Binietoglou, X. Bush, A. Comerón, H. Delbarre, D. García-Vízcaino, J. L. Guerrero-Rascado, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, F. Molero, N. Montoux, A. Muñoz, C. Muñoz, D. Nicolae, A. Papayannis, G. Pappalardo, J. Preissler, V. Rizi, F. Rocadenbosch, K. Sellegri, F. Wagner, and F. Dulac
Atmos. Chem. Phys., 14, 12031–12053, https://doi.org/10.5194/acp-14-12031-2014, https://doi.org/10.5194/acp-14-12031-2014, 2014
P. Chazette, F. Marnas, and J. Totems
Atmos. Meas. Tech., 7, 1629–1647, https://doi.org/10.5194/amt-7-1629-2014, https://doi.org/10.5194/amt-7-1629-2014, 2014
Y. Wang, K. N. Sartelet, M. Bocquet, and P. Chazette
Atmos. Chem. Phys., 14, 3511–3532, https://doi.org/10.5194/acp-14-3511-2014, https://doi.org/10.5194/acp-14-3511-2014, 2014
Y. Wang, K. N. Sartelet, M. Bocquet, and P. Chazette
Atmos. Chem. Phys., 13, 269–283, https://doi.org/10.5194/acp-13-269-2013, https://doi.org/10.5194/acp-13-269-2013, 2013
Related subject area
Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The ZiCOS-M CO2 sensor network: measurement performance and CO2 variability across Zürich
Interannual variations in the Δ(17O) signature of atmospheric CO2 at two mid-latitude sites suggest a close link to stratosphere–troposphere exchange
Atmospheric NH3 in urban Beijing: long-term variations and implications for secondary inorganic aerosol control
How rainfall events modify trace gas mixing ratios in central Amazonia
Airborne in-situ quantification of methane emissions from oil and gas production in Romania
Uncertainty in continuous ΔCO-based ΔffCO2 estimates derived from 14C flask and bottom-up ΔCO ∕ ΔffCO2 ratios
Measurement Report: The effects of SECA regulations on the atmospheric SO2 concentrations in the Baltic Sea, based on long-term observations at the Finnish Utö Island
Dynamical drivers of free-tropospheric ozone increases over equatorial Southeast Asia
Air mass transport to the tropical western Pacific troposphere inferred from ozone and relative humidity balloon observations above Palau
Mixing-layer-height-referenced ozone vertical distribution in the lower troposphere of Chinese megacities: stratification, classification, and meteorological and photochemical mechanisms
Six years of continuous carbon isotope composition measurements of methane in Heidelberg (Germany) – a study of source contributions and comparison to emission inventories
What caused large ozone variabilities in three megacity clusters in eastern China during 2015–2020?
Atmospheric turbulence observed during a fuel-bed-scale low-intensity surface fire
Fingerprints of the COVID-19 economic downturn and recovery on ozone anomalies at high-elevation sites in North America and western Europe
Ozone in the boreal forest in the Alberta Oil Sands Region
Zugspitze ozone 1970–2020: the role of stratosphere–troposphere transport
High sulfur dioxide deposition velocities measured with the flux–gradient technique in a boreal forest in the Alberta Oil Sands Region
Quantification of methane emissions in Hamburg using a network of FTIR spectrometers and an inverse modeling approach
Local-to-regional methane emissions from the Upper Silesian Coal Basin (USCB) quantified using UAV-based atmospheric measurements
Transport pathways of carbon monoxide from Indonesian fire pollution to a subtropical high-altitude mountain site in the western North Pacific
Global warming will largely increase waste treatment CH4 emissions in Chinese megacities: insight from the first city-scale CH4 concentration observation network in Hangzhou, China
Disentangling methane and carbon dioxide sources and transport across the Russian Arctic from aircraft measurements
Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations
Mercury in the free troposphere and bidirectional atmosphere–vegetation exchanges – insights from Maïdo mountain observatory in the Southern Hemisphere tropics
Diurnal variability of atmospheric O2, CO2, and their exchange ratio above a boreal forest in southern Finland
How adequately are elevated moist layers represented in reanalysis and satellite observations?
Quantitative impacts of vertical transport on the long-term trend of nocturnal ozone increase over the Pearl River Delta region during 2006–2019
Factors influencing the temporal variability of atmospheric methane emissions from Upper Silesia coal mines: a case study from the CoMet mission
Enhanced natural releases of mercury in response to the reduction in anthropogenic emissions during the COVID-19 lockdown by explainable machine learning
Temporal variability of tropospheric ozone and ozone profiles in the Korean Peninsula during the East Asian summer monsoon: insights from multiple measurements and reanalysis datasets
Retrieving CH4-emission rates from coal mine ventilation shafts using UAV-based AirCore observations and the genetic algorithm–interior point penalty function (GA-IPPF) model
Measurement report: Atmospheric mercury in a coastal city of Southeast China – inter-annual variations and influencing factors
Tropospheric and stratospheric ozone profiles during the 2019 TROpomi vaLIdation eXperiment (TROLIX-19)
Evaluation of correlated Pandora column NO2 and in situ surface NO2 measurements during GMAP campaign
Transport of substantial stratospheric ozone to the surface by a dying typhoon and shallow convection
Observational constraints on methane emissions from Polish coal mines using a ground-based remote sensing network
Continuous CH4 and δ13CH4 measurements in London demonstrate under-reported natural gas leakage
Long-term fluxes of carbonyl sulfide and their seasonality and interannual variability in a boreal forest
Declines and peaks in NO2 pollution during the multiple waves of the COVID-19 pandemic in the New York metropolitan area
Measurement report: Characterization of uncertainties in fluxes and fuel sulfur content from ship emissions in the Baltic Sea
Limitations of the radon tracer method (RTM) to estimate regional greenhouse gas (GHG) emissions – a case study for methane in Heidelberg
Positive and negative influences of typhoons on tropospheric ozone over southern China
Spatial and temporal variations of CO2 mole fractions observed at Beijing, Xianghe, and Xinglong in North China
The CO2 integral emission by the megacity of St Petersburg as quantified from ground-based FTIR measurements combined with dispersion modelling
Anthropogenic and natural controls on atmospheric δ13C-CO2 variations in the Yangtze River delta: insights from a carbon isotope modeling framework
Quantifying variability, source, and transport of CO in the urban areas over the Himalayas and Tibetan Plateau
New methodology shows short atmospheric lifetimes of oxidized sulfur and nitrogen due to dry deposition
Uncertainties in eddy covariance air–sea CO2 flux measurements and implications for gas transfer velocity parameterisations
Convergent evidence for the pervasive but limited contribution of biomass burning to atmospheric ammonia in peninsular Southeast Asia
Concurrent variation in oil and gas methane emissions and oil price during the COVID-19 pandemic
Stuart K. Grange, Pascal Rubli, Andrea Fischer, Dominik Brunner, Christoph Hueglin, and Lukas Emmenegger
EGUsphere, https://doi.org/10.5194/egusphere-2024-2925, https://doi.org/10.5194/egusphere-2024-2925, 2024
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Carbon dioxide (CO2) is a very important atmospheric pollutant and to better understand the gas's source and sink dynamics, a mid-cost sensor network hosting 26 sites was deployed in and around Zürich, Switzerland. The sensors' measurement performance was quantified and natural and anthropogenic CO2 emission sources were explored with a focus on what drives high CO2 levels. The observations will be used further by others to validate what is thought to be known about CO2 emissions in the region.
Pharahilda M. Steur, Hubertus A. Scheeren, Gerbrand Koren, Getachew A. Adnew, Wouter Peters, and Harro A. J. Meijer
Atmos. Chem. Phys., 24, 11005–11027, https://doi.org/10.5194/acp-24-11005-2024, https://doi.org/10.5194/acp-24-11005-2024, 2024
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We present records of the triple oxygen isotope signature (Δ(17O)) of atmospheric CO2 obtained with laser absorption spectroscopy from two mid-latitude stations. Significant interannual variability is observed in both records. A model sensitivity study suggests that stratosphere–troposphere exchange, which carries high-Δ(17O) CO2 from the stratosphere into the troposphere, causes most of the variability. This makes Δ(17O) a potential tracer for stratospheric intrusions into the troposphere.
Ziru Lan, Xiaoyi Zhang, Weili Lin, Xiaobin Xu, Zhiqiang Ma, Jun Jin, Lingyan Wu, and Yangmei Zhang
Atmos. Chem. Phys., 24, 9355–9368, https://doi.org/10.5194/acp-24-9355-2024, https://doi.org/10.5194/acp-24-9355-2024, 2024
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Our study examined the long-term trends of atmospheric ammonia in urban Beijing from 2009 to 2020. We found that the trends did not match satellite data or emission estimates, revealing complexities in ammonia sources. While seasonal variations in ammonia were temperature-dependent, daily variations were correlated with water vapor. We also found an increasing contribution of ammonia reduction, emphasizing its importance in mitigating the effects of fine particulate matter in Beijing.
Luiz A. T. Machado, Jürgen Kesselmeier, Santiago Botía, Hella van Asperen, Meinrat O. Andreae, Alessandro C. de Araújo, Paulo Artaxo, Achim Edtbauer, Rosaria R. Ferreira, Marco A. Franco, Hartwig Harder, Sam P. Jones, Cléo Q. Dias-Júnior, Guido G. Haytzmann, Carlos A. Quesada, Shujiro Komiya, Jost Lavric, Jos Lelieveld, Ingeborg Levin, Anke Nölscher, Eva Pfannerstill, Mira L. Pöhlker, Ulrich Pöschl, Akima Ringsdorf, Luciana Rizzo, Ana M. Yáñez-Serrano, Susan Trumbore, Wanda I. D. Valenti, Jordi Vila-Guerau de Arellano, David Walter, Jonathan Williams, Stefan Wolff, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 8893–8910, https://doi.org/10.5194/acp-24-8893-2024, https://doi.org/10.5194/acp-24-8893-2024, 2024
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Composite analysis of gas concentration before and after rainfall, during the day and night, gives insight into the complex relationship between trace gas variability and precipitation. The analysis helps us to understand the sources and sinks of trace gases within a forest ecosystem. It elucidates processes that are not discernible under undisturbed conditions and contributes to a deeper understanding of the trace gas life cycle and its intricate interactions with cloud dynamics in the Amazon.
Hossein Maazallahi, Foteini Stavropoulou, Samuel Jonson Sutanto, Michael Steiner, Dominik Brunner, Mariano Mertens, Patrick Jöckel, Antoon Visschedijk, Hugo Denier van der Gon, Stijn Dellaert, Nataly Velandia Salinas, Stefan Schwietzke, Daniel Zavala-Araiza, Sorin Ghemulet, Alexandru Pana, Magdalena Ardelean, Marius Corbu, Andreea Calcan, Stephen A. Conley, Mackenzie L. Smith, and Thomas Röckmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-2135, https://doi.org/10.5194/egusphere-2024-2135, 2024
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This article provide insights from airborne in-situ measurements during the ROMEO campaign with support from two model simulations. The results from the evaluations performed for this article are independently consistent with the results from previously published article which was based on ground-based measurements during the ROMEO campaign. The results show that reported methane emissions from oil and gas industry in Romania are largely under-reported to UNFCCC in 2019.
Fabian Maier, Ingeborg Levin, Sébastien Conil, Maksym Gachkivskyi, Hugo Denier van der Gon, and Samuel Hammer
Atmos. Chem. Phys., 24, 8205–8223, https://doi.org/10.5194/acp-24-8205-2024, https://doi.org/10.5194/acp-24-8205-2024, 2024
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We assess the uncertainty in continuous fossil fuel carbon dioxide (ffCO2) estimates derived from carbon monoxide (CO) observations and radiocarbon (14CO2) flask measurements from an urban and a rural site. This study provides the basis for using continuous CO-based ffCO2 observations in atmospheric transport inversion frameworks to derive ffCO2 emission estimates. We also compare the flask-based CO / ffCO2 ratios with modeled ratios to validate an emission inventory for central Europe.
Androniki Maragkidou, Tiia Grönholm, Laura Rautiainen, Juha Nikmo, Jukka-Pekka Jalkanen, Timo Mäkelä, Timo Anttila, Lauri Laakso, and Jaakko Kukkonen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1703, https://doi.org/10.5194/egusphere-2024-1703, 2024
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The Baltic Sea's designation as a Sulphur Emission Control Area in 2006, with subsequent regulations, significantly reduced sulphur emissions from shipping. Our study analyzed air quality data from 2003 to 2020 at Utö island and employed modelling, showing a continuous decrease in SO2 concentrations since 2003 and evidencing, thus, the effectiveness of such regulations in improving air quality. It also underscored the importance of long-term, high-resolution monitoring at remote marine sites.
Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Ninong Komala, Habib Khirzin Al-Ghazali, Dian Yudha Risdianto, Ambun Dindang, Ahmad Fairudz bin Jamaluddin, Mohan Kumar Sammathuria, Norazura Binti Zakaria, Bryan J. Johnson, and Patrick D. Cullis
Atmos. Chem. Phys., 24, 5221–5234, https://doi.org/10.5194/acp-24-5221-2024, https://doi.org/10.5194/acp-24-5221-2024, 2024
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SHADOZ balloon-borne ozone measurements over equatorial Southeast Asia from 1998–2022 reveal that ozone increases during the early months of the year are linked to reduced convective storm activity, which typically redistributes and cleans the atmosphere of ozone. These findings challenge models to replicate the trends produced by the SHADOZ and meteorological observations and emphasize the importance of studying monthly or seasonal instead of annual changes for understanding ozone trends.
Katrin Müller, Peter von der Gathen, and Markus Rex
Atmos. Chem. Phys., 24, 4693–4716, https://doi.org/10.5194/acp-24-4693-2024, https://doi.org/10.5194/acp-24-4693-2024, 2024
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The transport history of tropospheric air masses above the tropical western Pacific is studied by local ozone and relative humidity profile measurements from Palau. A prominent anti-correlation between both tracers separates air masses of different origin and genesis. Back trajectories confirm a local convective origin of the year-round humid ozone-poor background. Anomalously dry ozone-rich air is generated in tropical Asia by pollution and dehydrated during transport via radiative cooling.
Zhiheng Liao, Meng Gao, Jinqiang Zhang, Jiaren Sun, Jiannong Quan, Xingcan Jia, Yubing Pan, and Shaojia Fan
Atmos. Chem. Phys., 24, 3541–3557, https://doi.org/10.5194/acp-24-3541-2024, https://doi.org/10.5194/acp-24-3541-2024, 2024
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This study collected 1897 ozonesondes from two Chinese megacities (Beijing and Hong Kong) in 2000–2022 to investigate the climatological vertical heterogeneity of lower-tropospheric ozone distribution with a mixing-layer-height-referenced (h-referenced) vertical coordinate system. This vertical coordinate system highlighted O3 stratification features existing at the mixing layer–free troposphere interface and provided a better understanding of O3 pollution in urban regions.
Antje Hoheisel and Martina Schmidt
Atmos. Chem. Phys., 24, 2951–2969, https://doi.org/10.5194/acp-24-2951-2024, https://doi.org/10.5194/acp-24-2951-2024, 2024
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In Heidelberg, Germany, methane and its stable carbon isotope composition have been measured continuously with a cavity ring-down spectroscopy (CRDS) analyser since April 2014. These 6-year time series are analysed with the Keeling plot method for the isotopic composition of the sources, as well as seasonal variations and trends in methane emissions. The source contributions derived from atmospheric measurements were used to evaluate global and regional emission inventories of methane.
Tingting Hu, Yu Lin, Run Liu, Yuepeng Xu, Shanshan Ouyang, Boguang Wang, Yuanhang Zhang, and Shaw Chen Liu
Atmos. Chem. Phys., 24, 1607–1626, https://doi.org/10.5194/acp-24-1607-2024, https://doi.org/10.5194/acp-24-1607-2024, 2024
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We hypothesize that the cause of the worsening O3 trends in the Beijing–Tianjin–Hebei region, the Yangtze River Delta, and Pearl River Delta from 2015 to 2020 is attributable to the increased occurrence of meteorological conditions of high solar radiation and a positive temperature anomaly under the influence of West Pacific subtropical high, tropical cyclones, and mid–high-latitude wave activities.
Joseph Seitz, Shiyuan Zhong, Joseph J. Charney, Warren E. Heilman, Kenneth L. Clark, Xindi Bian, Nicholas S. Skowronski, Michael R. Gallagher, Matthew Patterson, Jason Cole, Michael T. Kiefer, Rory Hadden, and Eric Mueller
Atmos. Chem. Phys., 24, 1119–1142, https://doi.org/10.5194/acp-24-1119-2024, https://doi.org/10.5194/acp-24-1119-2024, 2024
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Atmospheric turbulence affects wildland fire behaviors and heat and smoke transfer. Turbulence data collected during an experimental fire on a 10 m x 10 m densely instrumented burn plot are analyzed, and the results reveal substantial heterogeneity in fire-induced turbulence characteristics across the small plot, which highlights the necessity for coupled atmosphere–fire behavior models to have 1–2 m grid spacing so that adequate simulations of fire behavior and smoke transfer can be achieved.
Davide Putero, Paolo Cristofanelli, Kai-Lan Chang, Gaëlle Dufour, Gregory Beachley, Cédric Couret, Peter Effertz, Daniel A. Jaffe, Dagmar Kubistin, Jason Lynch, Irina Petropavlovskikh, Melissa Puchalski, Timothy Sharac, Barkley C. Sive, Martin Steinbacher, Carlos Torres, and Owen R. Cooper
Atmos. Chem. Phys., 23, 15693–15709, https://doi.org/10.5194/acp-23-15693-2023, https://doi.org/10.5194/acp-23-15693-2023, 2023
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We investigated the impact of societal restriction measures during the COVID-19 pandemic on surface ozone at 41 high-elevation sites worldwide. Negative ozone anomalies were observed for spring and summer 2020 for all of the regions considered. In 2021, negative anomalies continued for Europe and partially for the eastern US, while western US sites showed positive anomalies due to wildfires. IASI satellite data and the Carbon Monitor supported emission reductions as a cause of the anomalies.
Xuanyi Zhang, Mark Gordon, Paul A. Makar, Timothy Jiang, Jonathan Davies, and David Tarasick
Atmos. Chem. Phys., 23, 13647–13664, https://doi.org/10.5194/acp-23-13647-2023, https://doi.org/10.5194/acp-23-13647-2023, 2023
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Measurements of ozone in the atmosphere were made in a forest downwind of oil sands mining and production facilities in northern Alberta. These measurements show that the emissions of other pollutants from oil sands production and processing reduce the amount of ozone in the forest. By using an atmospheric model combined with measurements, we find that the rate at which ozone is absorbed by the forest is lower than typical rates from similar measurements in other forests.
Thomas Trickl, Cédric Couret, Ludwig Ries, and Hannes Vogelmann
Atmos. Chem. Phys., 23, 8403–8427, https://doi.org/10.5194/acp-23-8403-2023, https://doi.org/10.5194/acp-23-8403-2023, 2023
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Downward atmospheric transport from the stratosphere (STT) is the most important natural source of tropospheric ozone. We analyse the stratospheric influence on the long-term series of ozone and carbon monoxide measured on the Zugspitze in the Bavarian Alps (2962 m a.s.l.). Since the 1970s, there has been a pronounced ozone rise that has been ascribed to an increase in STT. We determine the stratospheric influence from the observational data alone (humidity and 7Be).
Mark Gordon, Dane Blanchard, Timothy Jiang, Paul A. Makar, Ralf M. Staebler, Julian Aherne, Cris Mihele, and Xuanyi Zhang
Atmos. Chem. Phys., 23, 7241–7255, https://doi.org/10.5194/acp-23-7241-2023, https://doi.org/10.5194/acp-23-7241-2023, 2023
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Measurements of the gas sulfur dioxide (SO2) were made in a forest downwind of oil sands mining and production facilities in northern Alberta. These measurements tell us the rate at which SO2 is absorbed by the forest. The measured rate is much higher than what is currently used by air quality models, which is supported by a previous study in this region. This suggests that SO2 may have a much shorter lifetime in the atmosphere at this location than currently predicted by models.
Andreas Forstmaier, Jia Chen, Florian Dietrich, Juan Bettinelli, Hossein Maazallahi, Carsten Schneider, Dominik Winkler, Xinxu Zhao, Taylor Jones, Carina van der Veen, Norman Wildmann, Moritz Makowski, Aydin Uzun, Friedrich Klappenbach, Hugo Denier van der Gon, Stefan Schwietzke, and Thomas Röckmann
Atmos. Chem. Phys., 23, 6897–6922, https://doi.org/10.5194/acp-23-6897-2023, https://doi.org/10.5194/acp-23-6897-2023, 2023
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Large cities emit greenhouse gases which contribute to global warming. In this study, we measured the release of one important green house gas, methane, in Hamburg. Multiple sources that contribute to methane emissions were located and quantified. Methane sources were found to be mainly caused by human activity (e.g., by release from oil and gas refineries). Moreover, potential natural sources have been located, such as the Elbe River and lakes.
Truls Andersen, Zhao Zhao, Marcel de Vries, Jaroslaw Necki, Justyna Swolkien, Malika Menoud, Thomas Röckmann, Anke Roiger, Andreas Fix, Wouter Peters, and Huilin Chen
Atmos. Chem. Phys., 23, 5191–5216, https://doi.org/10.5194/acp-23-5191-2023, https://doi.org/10.5194/acp-23-5191-2023, 2023
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The Upper Silesian Coal Basin, Poland, is one of the hot spots of methane emissions in Europe. Using an uncrewed aerial vehicle (UAV), we performed atmospheric measurements of methane concentrations downwind of five ventilation shafts in this region and determined the emission rates from the individual shafts. We found a strong correlation between quantified shaft-averaged emission rates and hourly inventory data, which also allows us to estimate the methane emissions from the entire region.
Saginela Ravindra Babu, Chang-Feng Ou-Yang, Stephen M. Griffith, Shantanu Kumar Pani, Steven Soon-Kai Kong, and Neng-Huei Lin
Atmos. Chem. Phys., 23, 4727–4740, https://doi.org/10.5194/acp-23-4727-2023, https://doi.org/10.5194/acp-23-4727-2023, 2023
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In October 2006 and 2015, extensive fire episodes occurred in Indonesia, releasing an enormous amount of CO emissions. By combining in situ and satellite CO measurements and reanalysis products, we reported plausible transport pathways of CO from Indonesia to the Lulin Atmospheric Background Station (LABS; 23.47° N, 120.87° E; 2862 m a.s.l.) in Taiwan. We identified (i) horizontal transport in the free troposphere and (ii) vertical transport through the Hadley circulation.
Cheng Hu, Junqing Zhang, Bing Qi, Rongguang Du, Xiaofei Xu, Haoyu Xiong, Huili Liu, Xinyue Ai, Yiyi Peng, and Wei Xiao
Atmos. Chem. Phys., 23, 4501–4520, https://doi.org/10.5194/acp-23-4501-2023, https://doi.org/10.5194/acp-23-4501-2023, 2023
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We build the first city-scale tower-based atmospheric CH4 concentration observation network in China. The a priori total annual anthropogenic CH4 emissions and emissions from waste treatment were overestimated by 36.0 % and 47.1 %, respectively, in Hangzhou. Global warming will largely enhance the CH4 emission factor of waste treatment, which will increase by 17.6 %, 9.6 %, 5.6 % and 4.0 % for Representative Concentration Pathway (RCP) 8.5, RCP6.0, RCP4.5 and RCP2.6, respectively, by 2100.
Clément Narbaud, Jean-Daniel Paris, Sophie Wittig, Antoine Berchet, Marielle Saunois, Philippe Nédélec, Boris D. Belan, Mikhail Y. Arshinov, Sergei B. Belan, Denis Davydov, Alexander Fofonov, and Artem Kozlov
Atmos. Chem. Phys., 23, 2293–2314, https://doi.org/10.5194/acp-23-2293-2023, https://doi.org/10.5194/acp-23-2293-2023, 2023
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We measured CH4 and CO2 from aircraft over the Russian Arctic. Analyzing our data with the Lagrangian model FLEXPART, we find a sharp east–west gradient in atmospheric composition. Western Siberia is influenced by strong wetland CH4 emissions, deep CO2 gradient from biospheric uptake, and long-range transport from Europe and North America. Eastern flights document less variability. Over the Arctic Ocean, we find a small influence from marine CH4 emissions compatible with reasonable inventories.
Flora Kluge, Tilman Hüneke, Christophe Lerot, Simon Rosanka, Meike K. Rotermund, Domenico Taraborrelli, Benjamin Weyland, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 1369–1401, https://doi.org/10.5194/acp-23-1369-2023, https://doi.org/10.5194/acp-23-1369-2023, 2023
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Using airborne glyoxal concentration and vertical column density measurements, vertical profiles are inferred for eight global regions in aged biomass burning plumes and the tropical marine boundary layer. Using TROPOMI observations, an analysis of space- and airborne measurements is performed. A comparison to EMAC simulations shows a general glyoxal underprediction, which points to various missing sources and precursors from anthropogenic activities, biomass burning, and the sea surface.
Alkuin M. Koenig, Olivier Magand, Bert Verreyken, Jerome Brioude, Crist Amelynck, Niels Schoon, Aurélie Colomb, Beatriz Ferreira Araujo, Michel Ramonet, Mahesh K. Sha, Jean-Pierre Cammas, Jeroen E. Sonke, and Aurélien Dommergue
Atmos. Chem. Phys., 23, 1309–1328, https://doi.org/10.5194/acp-23-1309-2023, https://doi.org/10.5194/acp-23-1309-2023, 2023
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The global distribution of mercury, a potent neurotoxin, depends on atmospheric transport, chemistry, and interactions between the Earth’s surface and the air. Our understanding of these processes is still hampered by insufficient observations. Here, we present new data from a mountain observatory in the Southern Hemisphere. We give insights into mercury concentrations in air masses coming from aloft, and we show that tropical mountain vegetation may be a daytime source of mercury to the air.
Kim A. P. Faassen, Linh N. T. Nguyen, Eadin R. Broekema, Bert A. M. Kers, Ivan Mammarella, Timo Vesala, Penelope A. Pickers, Andrew C. Manning, Jordi Vilà-Guerau de Arellano, Harro A. J. Meijer, Wouter Peters, and Ingrid T. Luijkx
Atmos. Chem. Phys., 23, 851–876, https://doi.org/10.5194/acp-23-851-2023, https://doi.org/10.5194/acp-23-851-2023, 2023
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The exchange ratio (ER) between atmospheric O2 and CO2 provides a useful tracer for separately estimating photosynthesis and respiration processes in the forest carbon balance. This is highly relevant to better understand the expected biosphere sink, which determines future atmospheric CO2 levels. We therefore measured O2, CO2, and their ER above a boreal forest in Finland and investigated their diurnal behaviour for a representative day, and we show the most suitable way to determine the ER.
Marc Prange, Stefan A. Buehler, and Manfred Brath
Atmos. Chem. Phys., 23, 725–741, https://doi.org/10.5194/acp-23-725-2023, https://doi.org/10.5194/acp-23-725-2023, 2023
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We investigate the representation of elevated moist layers (EMLs) in two satellite retrieval products and ERA5 reanalysis. EMLs occur in the vicinity of tropical convective storms and are thought to have an impact on their evolution through radiative heating. We provide a first dedicated assessment of EMLs in long-term data products in terms of moist layer strength, vertical thickness and altitude by comparing to collocated radiosondes over the western Pacific, a region where EMLs often occur.
Yongkang Wu, Weihua Chen, Yingchang You, Qianqian Xie, Shiguo Jia, and Xuemei Wang
Atmos. Chem. Phys., 23, 453–469, https://doi.org/10.5194/acp-23-453-2023, https://doi.org/10.5194/acp-23-453-2023, 2023
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Relying on observed and simulated data, we determine the spatiotemporal characteristics of nocturnal O3 increase (NOI) events in the Pearl River Delta region during 2006–2019. Low-level jets and convective storms are the main meteorological processes causing NOI. Daytime O3 is another essential influencing factor. More importantly, a more prominent role of meteorological processes in NOI has been demonstrated. Our study highlights the important role of meteorology in nocturnal O3 pollution.
Justyna Swolkień, Andreas Fix, and Michał Gałkowski
Atmos. Chem. Phys., 22, 16031–16052, https://doi.org/10.5194/acp-22-16031-2022, https://doi.org/10.5194/acp-22-16031-2022, 2022
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Determination of emissions from coal mines on a local scale requires instantaneous data. We analysed temporal emission data for ventilation shafts and factors influencing their variability. They were saturation of the seams with methane, the permeability of the rock mass, and coal output. The data for the verification should reflect the actual values of emissions from point sources. It is recommended to achieve this by using a standardised emission measurement system for all coal mines.
Xiaofei Qin, Shengqian Zhou, Hao Li, Guochen Wang, Cheng Chen, Chengfeng Liu, Xiaohao Wang, Juntao Huo, Yanfen Lin, Jia Chen, Qingyan Fu, Yusen Duan, Kan Huang, and Congrui Deng
Atmos. Chem. Phys., 22, 15851–15865, https://doi.org/10.5194/acp-22-15851-2022, https://doi.org/10.5194/acp-22-15851-2022, 2022
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Using artificial neural network modeling and an explainable analysis approach, natural surface emissions (NSEs) were identified as a main driver of gaseous elemental mercury (GEM) variations during the COVID-19 lockdown. A sharp drop in GEM concentrations due to a significant reduction in anthropogenic emissions may disrupt the surface–air exchange balance of Hg, leading to increases in NSEs. This implies that NSEs may pose challenges to the future control of Hg pollution.
Juseon Bak, Eun-Ji Song, Hyo-Jung Lee, Xiong Liu, Ja-Ho Koo, Joowan Kim, Wonbae Jeon, Jae-Hwan Kim, and Cheol-Hee Kim
Atmos. Chem. Phys., 22, 14177–14187, https://doi.org/10.5194/acp-22-14177-2022, https://doi.org/10.5194/acp-22-14177-2022, 2022
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Our study investigates the temporal variations of ozone profiles at Pohang in the Korean Peninsula from multiple ozone products. We discuss the quantitative relationships between daily surface measurements and key meteorological variables, different seasonality of ozone between the troposphere and stratosphere, and interannual changes in the lower tropospheric ozone, linked by the weather pattern driven by the East Asian summer monsoon.
Tianqi Shi, Zeyu Han, Ge Han, Xin Ma, Huilin Chen, Truls Andersen, Huiqin Mao, Cuihong Chen, Haowei Zhang, and Wei Gong
Atmos. Chem. Phys., 22, 13881–13896, https://doi.org/10.5194/acp-22-13881-2022, https://doi.org/10.5194/acp-22-13881-2022, 2022
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CH4 works as the second-most important greenhouse gas, its reported emission inventories being far less than CO2. In this study, we developed a self-adjusted model to estimate the CH4 emission rate from strong point sources by the UAV-based AirCore system. This model would reduce the uncertainty in CH4 emission rate quantification accrued by errors in measurements of wind and concentration. Actual measurements on Pniówek coal demonstrate the high accuracy and stability of our developed model.
Jiayan Shi, Yuping Chen, Lingling Xu, Youwei Hong, Mengren Li, Xiaolong Fan, Liqian Yin, Yanting Chen, Chen Yang, Gaojie Chen, Taotao Liu, Xiaoting Ji, and Jinsheng Chen
Atmos. Chem. Phys., 22, 11187–11202, https://doi.org/10.5194/acp-22-11187-2022, https://doi.org/10.5194/acp-22-11187-2022, 2022
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Gaseous elemental mercury (GEM) was observed in Southeast China over the period 2012–2020. The observed GEM concentrations showed no distinct inter-annual variation trends. The interpretation rate of transportation and meteorology on GEM variations displayed an increasing trend. In contrast, anthropogenic emissions have shown a decreasing interpretation rate since 2012, indicating the effectiveness of emission mitigation measures in reducing GEM concentrations in the study region.
John T. Sullivan, Arnoud Apituley, Nora Mettig, Karin Kreher, K. Emma Knowland, Marc Allaart, Ankie Piters, Michel Van Roozendael, Pepijn Veefkind, Jerry R. Ziemke, Natalya Kramarova, Mark Weber, Alexei Rozanov, Laurence Twigg, Grant Sumnicht, and Thomas J. McGee
Atmos. Chem. Phys., 22, 11137–11153, https://doi.org/10.5194/acp-22-11137-2022, https://doi.org/10.5194/acp-22-11137-2022, 2022
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A TROPOspheric Monitoring Instrument (TROPOMI) validation campaign (TROLIX-19) was held in the Netherlands in September 2019. The research presented here focuses on using ozone lidars from NASA’s Goddard Space Flight Center to better evaluate the characterization of ozone throughout TROLIX-19 as compared to balloon-borne, space-borne and ground-based passive measurements, as well as a global coupled chemistry meteorology model.
Lim-Seok Chang, Donghee Kim, Hyunkee Hong, Deok-Rae Kim, Jeong-Ah Yu, Kwangyul Lee, Hanlim Lee, Daewon Kim, Jinkyu Hong, Hyun-Young Jo, and Cheol-Hee Kim
Atmos. Chem. Phys., 22, 10703–10720, https://doi.org/10.5194/acp-22-10703-2022, https://doi.org/10.5194/acp-22-10703-2022, 2022
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Our study explored the synergy of combined column and surface measurements during GMAP (GEMS Map of Air Pollution) campaign. It has several points to note for vertical distribution analysis. Particularly under prevailing local wind meteorological conditions, Pandora-based vertical structures sometimes showed negative correlations between column and surface measurements. Vertical analysis should be done carefully in some local meteorological conditions when employing either surface or columns.
Zhixiong Chen, Jane Liu, Xiushu Qie, Xugeng Cheng, Yukun Shen, Mengmiao Yang, Rubin Jiang, and Xiangke Liu
Atmos. Chem. Phys., 22, 8221–8240, https://doi.org/10.5194/acp-22-8221-2022, https://doi.org/10.5194/acp-22-8221-2022, 2022
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A vigorous surface ozone surge event of stratospheric origin occurred in the North China Plain at night. Surface ozone concentrations were 40–50 ppbv higher than the corresponding monthly mean, whereas surface carbon monoxide concentrations declined abruptly, which confirmed the direct stratospheric intrusions to the surface. We further addressed the notion that a combined effect of the dying typhoon and mesoscale convective systems was responsible for this vigorous ozone surge.
Andreas Luther, Julian Kostinek, Ralph Kleinschek, Sara Defratyka, Mila Stanisavljević, Andreas Forstmaier, Alexandru Dandocsi, Leon Scheidweiler, Darko Dubravica, Norman Wildmann, Frank Hase, Matthias M. Frey, Jia Chen, Florian Dietrich, Jarosław Nȩcki, Justyna Swolkień, Christoph Knote, Sanam N. Vardag, Anke Roiger, and André Butz
Atmos. Chem. Phys., 22, 5859–5876, https://doi.org/10.5194/acp-22-5859-2022, https://doi.org/10.5194/acp-22-5859-2022, 2022
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Coal mining is an extensive source of anthropogenic methane emissions. In order to reduce and mitigate methane emissions, it is important to know how much and where the methane is emitted. We estimated coal mining methane emissions in Poland based on atmospheric methane measurements and particle dispersion modeling. In general, our emission estimates suggest higher emissions than expected by previous annual emission reports.
Eric Saboya, Giulia Zazzeri, Heather Graven, Alistair J. Manning, and Sylvia Englund Michel
Atmos. Chem. Phys., 22, 3595–3613, https://doi.org/10.5194/acp-22-3595-2022, https://doi.org/10.5194/acp-22-3595-2022, 2022
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Continuous measurements of atmospheric methane concentrations and its carbon-13 isotope have been made in central London since early 2018. These measurements were used to evaluate methane emissions reported in global and UK-specific emission inventories for the London area. Compared to atmospheric methane measurements from March 2018 to October 2020, both inventories are under-reporting natural gas leakage for the London area.
Timo Vesala, Kukka-Maaria Kohonen, Linda M. J. Kooijmans, Arnaud P. Praplan, Lenka Foltýnová, Pasi Kolari, Markku Kulmala, Jaana Bäck, David Nelson, Dan Yakir, Mark Zahniser, and Ivan Mammarella
Atmos. Chem. Phys., 22, 2569–2584, https://doi.org/10.5194/acp-22-2569-2022, https://doi.org/10.5194/acp-22-2569-2022, 2022
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Carbonyl sulfide (COS) provides new insights into carbon cycle research. We present an easy-to-use flux parameterization and the longest existing time series of forest–atmosphere COS exchange measurements, which allow us to study both seasonal and interannual variability. We observed only uptake of COS by the forest on an annual basis, with 37 % variability between years. Upscaling the boreal COS uptake using a biosphere model indicates a significant missing COS sink at high latitudes.
Maria Tzortziou, Charlotte F. Kwong, Daniel Goldberg, Luke Schiferl, Róisín Commane, Nader Abuhassan, James J. Szykman, and Lukas C. Valin
Atmos. Chem. Phys., 22, 2399–2417, https://doi.org/10.5194/acp-22-2399-2022, https://doi.org/10.5194/acp-22-2399-2022, 2022
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The COVID-19 pandemic created an extreme natural experiment in which sudden changes in human behavior significantly impacted urban air quality. Using a combination of model, satellite, and ground-based data, we examine the impact of multiple waves and phases of the pandemic on atmospheric nitrogen pollution in the New York metropolitan area, and address the role of weather as a key driver of high pollution episodes observed even during – and despite – the stringent early lockdowns.
Jari Walden, Liisa Pirjola, Tuomas Laurila, Juha Hatakka, Heidi Pettersson, Tuomas Walden, Jukka-Pekka Jalkanen, Harri Nordlund, Toivo Truuts, Miika Meretoja, and Kimmo K. Kahma
Atmos. Chem. Phys., 21, 18175–18194, https://doi.org/10.5194/acp-21-18175-2021, https://doi.org/10.5194/acp-21-18175-2021, 2021
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Ship emissions play an important role in the deposition of gaseous compounds and nanoparticles (Ntot), affecting climate, human health (especially in coastal areas), and eutrophication. Micrometeorological methods showed that ship emissions were mainly responsible for the deposition of Ntot, whereas they only accounted for a minor proportion of CO2 deposition. An uncertainty analysis applied to the fluxes and fuel sulfur content results demonstrated the reliability of the results.
Ingeborg Levin, Ute Karstens, Samuel Hammer, Julian DellaColetta, Fabian Maier, and Maksym Gachkivskyi
Atmos. Chem. Phys., 21, 17907–17926, https://doi.org/10.5194/acp-21-17907-2021, https://doi.org/10.5194/acp-21-17907-2021, 2021
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The radon tracer method is applied to atmospheric methane and radon observations from the upper Rhine valley to independently estimate methane emissions from the region. Comparison of our top-down results with bottom-up inventory data requires high-resolution footprint modelling and representative radon flux data. In agreement with inventories, observed emissions decreased, but only until 2005. A limitation of this method is that point-source emissions are not captured or not fully captured.
Zhixiong Chen, Jane Liu, Xugeng Cheng, Mengmiao Yang, and Hong Wang
Atmos. Chem. Phys., 21, 16911–16923, https://doi.org/10.5194/acp-21-16911-2021, https://doi.org/10.5194/acp-21-16911-2021, 2021
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Using a large ensemble of typhoons, we investigate the impacts of evolving typhoons on tropospheric ozone and address the linkages between typhoon-affected meteorological conditions and ozone variations. The influences of typhoon-induced stratospheric intrusions on lower-troposphere ozone are also quantified. Thus, the results obtained in this study have important implications for a full understanding of the multifaced roles of typhoons in modulating tropospheric ozone variation.
Yang Yang, Minqiang Zhou, Ting Wang, Bo Yao, Pengfei Han, Denghui Ji, Wei Zhou, Yele Sun, Gengchen Wang, and Pucai Wang
Atmos. Chem. Phys., 21, 11741–11757, https://doi.org/10.5194/acp-21-11741-2021, https://doi.org/10.5194/acp-21-11741-2021, 2021
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This study introduces the in situ CO2 measurement system installed in Beijing (urban), Xianghe (suburban), and Xinglong (rural) in North China for the first time. The spatial and temporal variations in CO2 mole fractions at the three sites between June 2018 and April 2020 are discussed on both seasonal and diurnal scales.
Dmitry V. Ionov, Maria V. Makarova, Frank Hase, Stefani C. Foka, Vladimir S. Kostsov, Carlos Alberti, Thomas Blumenstock, Thorsten Warneke, and Yana A. Virolainen
Atmos. Chem. Phys., 21, 10939–10963, https://doi.org/10.5194/acp-21-10939-2021, https://doi.org/10.5194/acp-21-10939-2021, 2021
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Megacities are a significant source of emissions of various substances in the atmosphere, including carbon dioxide, which is the most important anthropogenic greenhouse gas. In 2019–2020, the Emission Monitoring Mobile Experiment was carried out in St Petersburg, which is the second-largest industrial city in Russia. The results of this experiment, coupled with numerical modelling, helped to estimate the amount of CO2 emitted by the city. This value was twice as high as predicted.
Cheng Hu, Jiaping Xu, Cheng Liu, Yan Chen, Dong Yang, Wenjing Huang, Lichen Deng, Shoudong Liu, Timothy J. Griffis, and Xuhui Lee
Atmos. Chem. Phys., 21, 10015–10037, https://doi.org/10.5194/acp-21-10015-2021, https://doi.org/10.5194/acp-21-10015-2021, 2021
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Seventy percent of global CO2 emissions were emitted from urban landscapes. The Yangtze River delta (YRD) ranks as one of the most densely populated regions in the world and is an anthropogenic CO2 hotspot. Besides anthropogenic factors, natural ecosystems and croplands act as significant CO2 sinks and sources. Independent quantification of the fossil and cement CO2 emission and assessment of their impact on atmospheric δ13C-CO2 have potential to improve our understanding of urban CO2 cycling.
Youwen Sun, Hao Yin, Yuan Cheng, Qianggong Zhang, Bo Zheng, Justus Notholt, Xiao Lu, Cheng Liu, Yuan Tian, and Jianguo Liu
Atmos. Chem. Phys., 21, 9201–9222, https://doi.org/10.5194/acp-21-9201-2021, https://doi.org/10.5194/acp-21-9201-2021, 2021
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We quantified the variability, source, and transport of urban CO over the Himalayas and Tibetan Plateau (HTP) by using measurement, model simulation, and the analysis of meteorological fields. Urban CO over the HTP is dominated by anthropogenic and biomass burning emissions from local, South Asia and East Asia, and oxidation sources. The decreasing trends in surface CO since 2015 in most cities over the HTP are attributed to the reduction in local and transported CO emissions in recent years.
Katherine Hayden, Shao-Meng Li, Paul Makar, John Liggio, Samar G. Moussa, Ayodeji Akingunola, Robert McLaren, Ralf M. Staebler, Andrea Darlington, Jason O'Brien, Junhua Zhang, Mengistu Wolde, and Leiming Zhang
Atmos. Chem. Phys., 21, 8377–8392, https://doi.org/10.5194/acp-21-8377-2021, https://doi.org/10.5194/acp-21-8377-2021, 2021
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We developed a method using aircraft measurements to determine lifetimes with respect to dry deposition for oxidized sulfur and nitrogen compounds over the boreal forest in Alberta, Canada. Atmospheric lifetimes were significantly shorter than derived from chemical transport models with differences related to modelled dry deposition velocities. The shorter lifetimes suggest models need to reassess dry deposition treatment and predictions of sulfur and nitrogen in the atmosphere and ecosystems.
Yuanxu Dong, Mingxi Yang, Dorothee C. E. Bakker, Vassilis Kitidis, and Thomas G. Bell
Atmos. Chem. Phys., 21, 8089–8110, https://doi.org/10.5194/acp-21-8089-2021, https://doi.org/10.5194/acp-21-8089-2021, 2021
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Eddy covariance (EC) is the most direct method for measuring air–sea CO2 flux from ships. However, uncertainty in EC air–sea CO2 fluxes has not been well quantified. Here we show that with the state-of-the-art gas analysers, instrumental noise no longer contributes significantly to the CO2 flux uncertainty. Applying an appropriate averaging timescale (1–3 h) and suitable air–sea CO2 fugacity threshold (at least 20 µatm) to EC flux data enables an optimal analysis of the gas transfer velocity.
Yunhua Chang, Yan-Lin Zhang, Sawaeng Kawichai, Qian Wang, Martin Van Damme, Lieven Clarisse, Tippawan Prapamontol, and Moritz F. Lehmann
Atmos. Chem. Phys., 21, 7187–7198, https://doi.org/10.5194/acp-21-7187-2021, https://doi.org/10.5194/acp-21-7187-2021, 2021
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In this study, we integrated satellite constraints on atmospheric NH3 levels and fire intensity, discrete NH3 concentration measurement, and N isotopic analysis of NH3 in order to assess the regional-scale contribution of biomass burning to ambient atmospheric NH3 in the heartland of Southeast Asia. The combined approach provides a valuable cross-validation framework for source apportioning of NH3 in the lower atmosphere and will thus help to ameliorate predictions of biomass burning emissions.
David R. Lyon, Benjamin Hmiel, Ritesh Gautam, Mark Omara, Katherine A. Roberts, Zachary R. Barkley, Kenneth J. Davis, Natasha L. Miles, Vanessa C. Monteiro, Scott J. Richardson, Stephen Conley, Mackenzie L. Smith, Daniel J. Jacob, Lu Shen, Daniel J. Varon, Aijun Deng, Xander Rudelis, Nikhil Sharma, Kyle T. Story, Adam R. Brandt, Mary Kang, Eric A. Kort, Anthony J. Marchese, and Steven P. Hamburg
Atmos. Chem. Phys., 21, 6605–6626, https://doi.org/10.5194/acp-21-6605-2021, https://doi.org/10.5194/acp-21-6605-2021, 2021
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The Permian Basin (USA) is the world’s largest oil field. We use tower- and aircraft-based approaches to measure how methane emissions in the Permian Basin changed throughout 2020. In early 2020, 3.3 % of the region’s gas was emitted; then in spring 2020, the loss rate temporarily dropped to 1.9 % as oil price crashed. We find this short-term reduction to be a result of reduced well development, less gas flaring, and fewer abnormal events despite minimal reductions in oil and gas production.
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