Articles | Volume 13, issue 2
https://doi.org/10.5194/acp-13-917-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-917-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
22 Jan 2013
Research article |
| 22 Jan 2013
The first aerosol indirect effect quantified through airborne remote sensing during VOCALS-REx
D. Painemal
NASA Langley Research Center, Hampton, VA, USA
P. Zuidema
Rosenstiel School of Marine and Atmospheric Sciences, University of Miami, Key Biscayne, Fl, USA
Related authors
Florian Tornow, Ann Fridlind, George Tselioudis, Brian Cairns, Andrew Ackerman, Seethala Chellappan, David Painemal, Paquita Zuidema, Christiane Voigt, Simon Kirschler, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-3462, https://doi.org/10.5194/egusphere-2024-3462, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The recent NASA campaign ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) performed 71 tandem flights in mid-latitude marine cold-air outbreaks off the US Eastern seaboard. We provide meteorological and cloud transition stage context, allowing us to identify days that are most suitable for Lagrangian modeling and analysis. Surveyed cloud properties show signatures of cloud microphysical processes, such as cloud-top entrainment and secondary ice formation.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
Short summary
Short summary
Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Leong Wai Siu, Joseph S. Schlosser, David Painemal, Brian Cairns, Marta A. Fenn, Richard A. Ferrare, Johnathan W. Hair, Chris A. Hostetler, Longlei Li, Mary M. Kleb, Amy Jo Scarino, Taylor J. Shingler, Armin Sorooshian, Snorre A. Stamnes, and Xubin Zeng
Atmos. Meas. Tech., 17, 2739–2759, https://doi.org/10.5194/amt-17-2739-2024, https://doi.org/10.5194/amt-17-2739-2024, 2024
Short summary
Short summary
An unprecedented 3-year aerosol dataset was collected from a recent NASA field campaign over the western North Atlantic Ocean, which offers a special opportunity to evaluate two state-of-the-art remote sensing instruments, one lidar and the other polarimeter, on the same aircraft. Special attention has been paid to validate aerosol optical depth data and their uncertainties when no reference dataset is available. Physical reasons for the disagreement between two instruments are discussed.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
Short summary
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We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
Short summary
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
Short summary
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The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
Short summary
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
Short summary
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Edward Gryspeerdt, Daniel T. McCoy, Ewan Crosbie, Richard H. Moore, Graeme J. Nott, David Painemal, Jennifer Small-Griswold, Armin Sorooshian, and Luke Ziemba
Atmos. Meas. Tech., 15, 3875–3892, https://doi.org/10.5194/amt-15-3875-2022, https://doi.org/10.5194/amt-15-3875-2022, 2022
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Droplet number concentration is a key property of clouds, influencing a variety of cloud processes. It is also used for estimating the cloud response to aerosols. The satellite retrieval depends on a number of assumptions – different sampling strategies are used to select cases where these assumptions are most likely to hold. Here we investigate the impact of these strategies on the agreement with in situ data, the droplet number climatology and estimates of the indirect radiative forcing.
Zhujun Li, David Painemal, Gregory Schuster, Marian Clayton, Richard Ferrare, Mark Vaughan, Damien Josset, Jayanta Kar, and Charles Trepte
Atmos. Meas. Tech., 15, 2745–2766, https://doi.org/10.5194/amt-15-2745-2022, https://doi.org/10.5194/amt-15-2745-2022, 2022
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For more than 15 years, CALIPSO has revolutionized our understanding of the role of aerosols in climate. Here we evaluate CALIPSO aerosol typing over the ocean using an independent CALIPSO–CloudSat product. The analysis suggests that CALIPSO correctly categorizes clean marine aerosol over the open ocean, elevated smoke over the SE Atlantic, and dust over the tropical Atlantic. Similarities between clean and dusty marine over the open ocean implies that algorithm modifications are warranted.
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
David Painemal, Douglas Spangenberg, William L. Smith Jr., Patrick Minnis, Brian Cairns, Richard H. Moore, Ewan Crosbie, Claire Robinson, Kenneth L. Thornhill, Edward L. Winstead, and Luke Ziemba
Atmos. Meas. Tech., 14, 6633–6646, https://doi.org/10.5194/amt-14-6633-2021, https://doi.org/10.5194/amt-14-6633-2021, 2021
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Cloud properties derived from satellite sensors are critical for the global monitoring of climate. This study evaluates satellite-based cloud properties over the North Atlantic using airborne data collected during NAAMES. Satellite observations of droplet size and cloud optical depth tend to compare well with NAAMES data. The analysis indicates that the satellite pixel resolution and the specific viewing geometry need to be taken into account in research applications.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
David Painemal, Fu-Lung Chang, Richard Ferrare, Sharon Burton, Zhujun Li, William L. Smith Jr., Patrick Minnis, Yan Feng, and Marian Clayton
Atmos. Chem. Phys., 20, 7167–7177, https://doi.org/10.5194/acp-20-7167-2020, https://doi.org/10.5194/acp-20-7167-2020, 2020
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Aerosol–cloud interactions (ACIs) are the most uncertain aspect of anthropogenic forcing. Although satellites provide the observational dataset for the global ACI quantification, retrievals are limited to vertically integrated quantities (e.g., aerosol optical depth – AOD), which are typically used as an aerosol proxy. This study demonstrates that matching vertically resolved aerosol from CALIOP at the cloud-layer height with satellite cloud retrievals reduces uncertainties in ACI estimates.
David Painemal, Marian Clayton, Richard Ferrare, Sharon Burton, Damien Josset, and Mark Vaughan
Atmos. Meas. Tech., 12, 2201–2217, https://doi.org/10.5194/amt-12-2201-2019, https://doi.org/10.5194/amt-12-2201-2019, 2019
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We present 1 year of a new CALIOP-based aerosol extinction coefficient and lidar ratio over the ocean, with the goal of providing a flexible dataset for climate research as well as independent retrievals that can be helpful for refining CALIPSO Science Team algorithms. The retrievals are derived by constraining the lidar equation with an aerosol optical depth estimated from cross-calibrated CALIOP and CloudSat surface echos.
D. Painemal, P. Minnis, and S. Sun-Mack
Atmos. Chem. Phys., 13, 9997–10003, https://doi.org/10.5194/acp-13-9997-2013, https://doi.org/10.5194/acp-13-9997-2013, 2013
Haochi Che, Lu Zhang, Michal Segal-Rozenhaimer, Caroline Dang, Paquita Zuidema, and Arthur J. Sedlacek III
EGUsphere, https://doi.org/10.5194/egusphere-2024-3304, https://doi.org/10.5194/egusphere-2024-3304, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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We investigated how biomass burning (BB) affects cloud formation in the southeast Atlantic. We found that aerosol hygroscopicity, which influences cloud droplet formation, varied monthly and differed significantly between 2016 and 2017, due to changes in sulfate aerosols. These changes were driven by BB burning conditions, which were likely influenced by meteorological factors. This study highlights the important role of BB in shaping aerosol properties and clouds in the region.
Florian Tornow, Ann Fridlind, George Tselioudis, Brian Cairns, Andrew Ackerman, Seethala Chellappan, David Painemal, Paquita Zuidema, Christiane Voigt, Simon Kirschler, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-3462, https://doi.org/10.5194/egusphere-2024-3462, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The recent NASA campaign ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) performed 71 tandem flights in mid-latitude marine cold-air outbreaks off the US Eastern seaboard. We provide meteorological and cloud transition stage context, allowing us to identify days that are most suitable for Lagrangian modeling and analysis. Surveyed cloud properties show signatures of cloud microphysical processes, such as cloud-top entrainment and secondary ice formation.
Kira Zeider, Kayla McCauley, Sanja Dmitrovic, Leong Wai Siu, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Simon Kirschler, John B. Nowak, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, Paquita Zuidema, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-2743, https://doi.org/10.5194/egusphere-2024-2743, 2024
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In-situ aircraft data collected over the northwest Atlantic Ocean are utilized to compare aerosol conditions and turbulence between near-surface and below cloud base altitudes for different regimes of coupling strength between those two levels, along with how cloud microphysical properties vary across those regimes. Stronger coupling yields more homogenous aerosol structure vertically along with higher cloud drop concentrations and sea salt influence in clouds.
Cynthia H. Whaley, Tim Butler, Jose A. Adame, Rupal Ambulkar, Stephen R. Arnold, Rebecca R. Buchholz, Benjamin Gaubert, Douglas S. Hamilton, Min Huang, Hayley Hung, Johannes W. Kaiser, Jacek W. Kaminski, Christophe Knote, Gerbrand Koren, Jean-Luc Kouassi, Meiyun Lin, Tianjia Liu, Jianmin Ma, Kasemsan Manomaiphiboon, Elisa Bergas Masso, Jessica L. McCarty, Mariano Mertens, Mark Parrington, Helene Peiro, Pallavi Saxena, Saurabh Sonwani, Vanisa Surapipith, Damaris Tan, Wenfu Tang, Veerachai Tanpipat, Kostas Tsigaridis, Christine Wiedinmyer, Oliver Wild, Yuanyu Xie, and Paquita Zuidema
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-126, https://doi.org/10.5194/gmd-2024-126, 2024
Preprint under review for GMD
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The multi-model experiment design of the HTAP3 Fires project takes a multi-pollutant approach to improving our understanding of transboundary transport of wildland fire and agricultural burning emissions and their impacts. The experiments are designed with the goal of answering science policy questions related to fires. The options for the multi-model approach, including inputs, outputs, and model set up are discussed, and the official recommendations for the project are presented.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Amie Dobracki, Ernie Lewis, Arthur Sedlacek III, Tyler Tatro, Maria Zawadowicz, and Paquita Zuidema
EGUsphere, https://doi.org/10.5194/egusphere-2024-1347, https://doi.org/10.5194/egusphere-2024-1347, 2024
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Biomass-burning aerosol is commonly present in the marine boundary layer of the southeast Atlantic Ocean between June and October. Our research indicates that burning conditions, aerosol transport pathways, and prolonged oxidation processes, both heterogeneous and aqueous-phase determine the chemical, microphysical, and optical properties of the boundary layer aerosol. Notably, we find that the aerosol optical properties can be estimated from the chemical properties alone.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
Short summary
Short summary
Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Leong Wai Siu, Joseph S. Schlosser, David Painemal, Brian Cairns, Marta A. Fenn, Richard A. Ferrare, Johnathan W. Hair, Chris A. Hostetler, Longlei Li, Mary M. Kleb, Amy Jo Scarino, Taylor J. Shingler, Armin Sorooshian, Snorre A. Stamnes, and Xubin Zeng
Atmos. Meas. Tech., 17, 2739–2759, https://doi.org/10.5194/amt-17-2739-2024, https://doi.org/10.5194/amt-17-2739-2024, 2024
Short summary
Short summary
An unprecedented 3-year aerosol dataset was collected from a recent NASA field campaign over the western North Atlantic Ocean, which offers a special opportunity to evaluate two state-of-the-art remote sensing instruments, one lidar and the other polarimeter, on the same aircraft. Special attention has been paid to validate aerosol optical depth data and their uncertainties when no reference dataset is available. Physical reasons for the disagreement between two instruments are discussed.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
Short summary
Short summary
We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
Short summary
Short summary
We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
Short summary
Short summary
The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
Short summary
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Amie Dobracki, Paquita Zuidema, Steven G. Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys., 23, 4775–4799, https://doi.org/10.5194/acp-23-4775-2023, https://doi.org/10.5194/acp-23-4775-2023, 2023
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Southern Africa produces approximately one-third of the world’s carbon from fires. The thick smoke layer can flow westward, interacting with the southeastern Atlantic cloud deck. The net radiative impact can alter regional circulation patterns, impacting rainfall over Africa. We find that the smoke is highly absorbing of sunlight, mostly because it contains more black carbon than smoke over the Northern Hemisphere.
Ian Chang, Lan Gao, Connor J. Flynn, Yohei Shinozuka, Sarah J. Doherty, Michael S. Diamond, Karla M. Longo, Gonzalo A. Ferrada, Gregory R. Carmichael, Patricia Castellanos, Arlindo M. da Silva, Pablo E. Saide, Calvin Howes, Zhixin Xue, Marc Mallet, Ravi Govindaraju, Qiaoqiao Wang, Yafang Cheng, Yan Feng, Sharon P. Burton, Richard A. Ferrare, Samuel E. LeBlanc, Meloë S. Kacenelenbogen, Kristina Pistone, Michal Segal-Rozenhaimer, Kerry G. Meyer, Ju-Mee Ryoo, Leonhard Pfister, Adeyemi A. Adebiyi, Robert Wood, Paquita Zuidema, Sundar A. Christopher, and Jens Redemann
Atmos. Chem. Phys., 23, 4283–4309, https://doi.org/10.5194/acp-23-4283-2023, https://doi.org/10.5194/acp-23-4283-2023, 2023
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Abundant aerosols are present above low-level liquid clouds over the southeastern Atlantic during late austral spring. The model simulation differences in the proportion of aerosol residing in the planetary boundary layer and in the free troposphere can greatly affect the regional aerosol radiative effects. This study examines the aerosol loading and fractional aerosol loading in the free troposphere among various models and evaluates them against measurements from the NASA ORACLES campaign.
Haley M. Royer, Mira L. Pöhlker, Ovid Krüger, Edmund Blades, Peter Sealy, Nurun Nahar Lata, Zezhen Cheng, Swarup China, Andrew P. Ault, Patricia K. Quinn, Paquita Zuidema, Christopher Pöhlker, Ulrich Pöschl, Meinrat Andreae, and Cassandra J. Gaston
Atmos. Chem. Phys., 23, 981–998, https://doi.org/10.5194/acp-23-981-2023, https://doi.org/10.5194/acp-23-981-2023, 2023
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This paper presents atmospheric particle chemical composition and measurements of aerosol water uptake properties collected at Ragged Point, Barbados, during the winter of 2020. The result of this study indicates the importance of small African smoke particles for cloud droplet formation in the tropical North Atlantic and highlights the large spatial and temporal pervasiveness of smoke over the Atlantic Ocean.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 22, 14209–14241, https://doi.org/10.5194/acp-22-14209-2022, https://doi.org/10.5194/acp-22-14209-2022, 2022
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The variability in the meteorological fields during each deployment is highly modulated at a daily to synoptic timescale. This paper, along with part 1, the climatological overview paper, provides a meteorological context for interpreting the airborne measurements gathered during the three ORACLES deployments. This study supports related studies focusing on the detailed investigation of the processes controlling stratocumulus decks, aerosol lifting, transport, and their interactions.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Caroline Dang, Michal Segal-Rozenhaimer, Haochi Che, Lu Zhang, Paola Formenti, Jonathan Taylor, Amie Dobracki, Sara Purdue, Pui-Shan Wong, Athanasios Nenes, Arthur Sedlacek III, Hugh Coe, Jens Redemann, Paquita Zuidema, Steven Howell, and James Haywood
Atmos. Chem. Phys., 22, 9389–9412, https://doi.org/10.5194/acp-22-9389-2022, https://doi.org/10.5194/acp-22-9389-2022, 2022
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Transmission electron microscopy was used to analyze aged African smoke particles and how the smoke interacts with the marine atmosphere. We found that the volatility of organic aerosol increases with biomass burning plume age, that black carbon is often mixed with potassium salts and that the marine atmosphere can incorporate Na and Cl into smoke particles. Marine salts are more processed when mixed with smoke plumes, and there are interesting Cl-rich yet Na-absent marine particles.
Haochi Che, Michal Segal-Rozenhaimer, Lu Zhang, Caroline Dang, Paquita Zuidema, Arthur J. Sedlacek III, Xiaoye Zhang, and Connor Flynn
Atmos. Chem. Phys., 22, 8767–8785, https://doi.org/10.5194/acp-22-8767-2022, https://doi.org/10.5194/acp-22-8767-2022, 2022
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A 17-month in situ study on Ascension Island found low single-scattering albedo and strong absorption enhancement of the marine boundary layer aerosols during biomass burnings on the African continent, along with apparent patterns of regular monthly variability. We further discuss the characteristics and drivers behind these changes and find that biomass burning conditions in Africa may be the main factor influencing the optical properties of marine boundary aerosols.
Edward Gryspeerdt, Daniel T. McCoy, Ewan Crosbie, Richard H. Moore, Graeme J. Nott, David Painemal, Jennifer Small-Griswold, Armin Sorooshian, and Luke Ziemba
Atmos. Meas. Tech., 15, 3875–3892, https://doi.org/10.5194/amt-15-3875-2022, https://doi.org/10.5194/amt-15-3875-2022, 2022
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Droplet number concentration is a key property of clouds, influencing a variety of cloud processes. It is also used for estimating the cloud response to aerosols. The satellite retrieval depends on a number of assumptions – different sampling strategies are used to select cases where these assumptions are most likely to hold. Here we investigate the impact of these strategies on the agreement with in situ data, the droplet number climatology and estimates of the indirect radiative forcing.
Zhujun Li, David Painemal, Gregory Schuster, Marian Clayton, Richard Ferrare, Mark Vaughan, Damien Josset, Jayanta Kar, and Charles Trepte
Atmos. Meas. Tech., 15, 2745–2766, https://doi.org/10.5194/amt-15-2745-2022, https://doi.org/10.5194/amt-15-2745-2022, 2022
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For more than 15 years, CALIPSO has revolutionized our understanding of the role of aerosols in climate. Here we evaluate CALIPSO aerosol typing over the ocean using an independent CALIPSO–CloudSat product. The analysis suggests that CALIPSO correctly categorizes clean marine aerosol over the open ocean, elevated smoke over the SE Atlantic, and dust over the tropical Atlantic. Similarities between clean and dusty marine over the open ocean implies that algorithm modifications are warranted.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Michal Segal Rozenhaimer, Meloë Kacenelenbogen, Yohei Shinozuka, Connor Flynn, Rich Ferrare, Sharon Burton, Chris Hostetler, Marc Mallet, and Paquita Zuidema
Atmos. Meas. Tech., 15, 61–77, https://doi.org/10.5194/amt-15-61-2022, https://doi.org/10.5194/amt-15-61-2022, 2022
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This work presents heating rates derived from aircraft observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS). We separate the total heating rates into aerosol and gas (primarily water vapor) absorption and explore some of the co-variability of heating rate profiles and their primary drivers, leading to the development of a new concept: the heating rate efficiency (HRE; the heating rate per unit aerosol extinction).
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Amie Dobracki, Paquita Zuidema, Steve Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1081, https://doi.org/10.5194/acp-2021-1081, 2022
Preprint withdrawn
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The global maximum of shortwave-absorbing aerosol above cloud occurs above the southeast Atlantic, where the biomass-burning aerosol provides a distinct aerosol radiative warming of regional climate. The smoke aerosols are unusually highly absorbing of sunlight. This study seeks to understand the cause. We conclude the aerosol is already strongly absorbing at the fire emission source, but that chemical aging, through encouraging a net loss of organic aerosol, also contributes.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 21, 16689–16707, https://doi.org/10.5194/acp-21-16689-2021, https://doi.org/10.5194/acp-21-16689-2021, 2021
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Part 1 of the meteorological overview paper highlights the anomalous meteorological characteristics during the ORACLES deployment compared to the climatological mean at monthly timescales. The upper-level wave disturbance and the associated anomalous circulation explain the weakening of AEJ-S through the reduction of the strength of the heat low over the land during August 2017. This may also help explain the anomalously low aerosol optical depth observed in the August 2017 ORACLES deployment.
Raphaela Vogel, Heike Konow, Hauke Schulz, and Paquita Zuidema
Atmos. Chem. Phys., 21, 16609–16630, https://doi.org/10.5194/acp-21-16609-2021, https://doi.org/10.5194/acp-21-16609-2021, 2021
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The shallow cumulus clouds that populate the trade-wind regions can produce substantial amounts of rain. Before reaching the surface, part of the rain can evaporate and form pools of cold air that spread at the surface as density currents. We use 10 years of data from Barbados to show that such cold pools occur on 3 out of 4 d, that cold-pool periods are 90 % cloudier relative to the average winter conditions, and that they are connected to specific patterns of mesoscale cloud organization.
David Painemal, Douglas Spangenberg, William L. Smith Jr., Patrick Minnis, Brian Cairns, Richard H. Moore, Ewan Crosbie, Claire Robinson, Kenneth L. Thornhill, Edward L. Winstead, and Luke Ziemba
Atmos. Meas. Tech., 14, 6633–6646, https://doi.org/10.5194/amt-14-6633-2021, https://doi.org/10.5194/amt-14-6633-2021, 2021
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Cloud properties derived from satellite sensors are critical for the global monitoring of climate. This study evaluates satellite-based cloud properties over the North Atlantic using airborne data collected during NAAMES. Satellite observations of droplet size and cloud optical depth tend to compare well with NAAMES data. The analysis indicates that the satellite pixel resolution and the specific viewing geometry need to be taken into account in research applications.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Jianhao Zhang and Paquita Zuidema
Atmos. Chem. Phys., 21, 11179–11199, https://doi.org/10.5194/acp-21-11179-2021, https://doi.org/10.5194/acp-21-11179-2021, 2021
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The subtropical Atlantic hosts one of the planet's largest marine low cloud decks and interacts with biomass burning aerosol from approximately July through October. This study clarifies how the monthly evolution in meteorology and the biomass burning aerosol vertical structure affects the seasonal cycle in its low cloud fraction, such that the July–October evolution in low cloud cover and morphology are reinforced, when compared to scenarios with less aerosol present.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Robert Pincus, Chris W. Fairall, Adriana Bailey, Haonan Chen, Patrick Y. Chuang, Gijs de Boer, Graham Feingold, Dean Henze, Quinn T. Kalen, Jan Kazil, Mason Leandro, Ashley Lundry, Ken Moran, Dana A. Naeher, David Noone, Akshar J. Patel, Sergio Pezoa, Ivan PopStefanija, Elizabeth J. Thompson, James Warnecke, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 3281–3296, https://doi.org/10.5194/essd-13-3281-2021, https://doi.org/10.5194/essd-13-3281-2021, 2021
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This paper describes observations taken from a research aircraft during a field experiment in the western Atlantic Ocean during January and February 2020. The plane made 11 flights, most 8-9 h long, and measured the properties of the atmosphere and ocean with a combination of direct measurements, sensors falling from the plane to profile the atmosphere and ocean, and remote sensing measurements of clouds and the ocean surface.
Kristina Pistone, Paquita Zuidema, Robert Wood, Michael Diamond, Arlindo M. da Silva, Gonzalo Ferrada, Pablo E. Saide, Rei Ueyama, Ju-Mee Ryoo, Leonhard Pfister, James Podolske, David Noone, Ryan Bennett, Eric Stith, Gregory Carmichael, Jens Redemann, Connor Flynn, Samuel LeBlanc, Michal Segal-Rozenhaimer, and Yohei Shinozuka
Atmos. Chem. Phys., 21, 9643–9668, https://doi.org/10.5194/acp-21-9643-2021, https://doi.org/10.5194/acp-21-9643-2021, 2021
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Using aircraft-based measurements off the Atlantic coast of Africa, we found the springtime smoke plume was strongly correlated with the amount of water vapor in the atmosphere (more smoke indicated more humidity). We see the same general feature in satellite-assimilated and free-running models. Our analysis suggests this relationship is not caused by the burning but originates due to coincident continental meteorology plus fires. This air is transported over the ocean without further mixing.
Patricia K. Quinn, Elizabeth J. Thompson, Derek J. Coffman, Sunil Baidar, Ludovic Bariteau, Timothy S. Bates, Sebastien Bigorre, Alan Brewer, Gijs de Boer, Simon P. de Szoeke, Kyla Drushka, Gregory R. Foltz, Janet Intrieri, Suneil Iyer, Chris W. Fairall, Cassandra J. Gaston, Friedhelm Jansen, James E. Johnson, Ovid O. Krüger, Richard D. Marchbanks, Kenneth P. Moran, David Noone, Sergio Pezoa, Robert Pincus, Albert J. Plueddemann, Mira L. Pöhlker, Ulrich Pöschl, Estefania Quinones Melendez, Haley M. Royer, Malgorzata Szczodrak, Jim Thomson, Lucia M. Upchurch, Chidong Zhang, Dongxiao Zhang, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 1759–1790, https://doi.org/10.5194/essd-13-1759-2021, https://doi.org/10.5194/essd-13-1759-2021, 2021
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ATOMIC took place in the northwestern tropical Atlantic during January and February of 2020 to gather information on shallow atmospheric convection, the effects of aerosols and clouds on the ocean surface energy budget, and mesoscale oceanic processes. Measurements made from the NOAA RV Ronald H. Brown and assets it deployed (instrumented mooring and uncrewed seagoing vehicles) are described herein to advance widespread use of the data by the ATOMIC and broader research communities.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal Rozenhaimer, Yohei Shinozuka, Connor Flynn, Amie Dobracki, Paquita Zuidema, Steven Howell, Steffen Freitag, and Sarah Doherty
Atmos. Meas. Tech., 14, 567–593, https://doi.org/10.5194/amt-14-567-2021, https://doi.org/10.5194/amt-14-567-2021, 2021
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Based on observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS), this work establishes an observationally driven link from mid-visible aerosol optical depth (AOD) and other scene parameters to broadband shortwave irradiance (and by extension the direct aerosol radiative effect, DARE). The majority of the case-to-case DARE variability within the ORACLES dataset is attributable to the dependence on AOD and scene albedo.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Marc Mallet, Fabien Solmon, Pierre Nabat, Nellie Elguindi, Fabien Waquet, Dominique Bouniol, Andrew Mark Sayer, Kerry Meyer, Romain Roehrig, Martine Michou, Paquita Zuidema, Cyrille Flamant, Jens Redemann, and Paola Formenti
Atmos. Chem. Phys., 20, 13191–13216, https://doi.org/10.5194/acp-20-13191-2020, https://doi.org/10.5194/acp-20-13191-2020, 2020
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This paper presents numerical simulations using two regional climate models to study the impact of biomass fire plumes from central Africa on the radiative balance of this region. The results indicate that biomass fires can either warm the regional climate when they are located above low clouds or cool it when they are located above land. They can also alter sea and land surface temperatures by decreasing solar radiation at the surface. Finally, they can also modify the atmospheric dynamics.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
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In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Yohei Shinozuka, Meloë S. Kacenelenbogen, Sharon P. Burton, Steven G. Howell, Paquita Zuidema, Richard A. Ferrare, Samuel E. LeBlanc, Kristina Pistone, Stephen Broccardo, Jens Redemann, K. Sebastian Schmidt, Sabrina P. Cochrane, Marta Fenn, Steffen Freitag, Amie Dobracki, Michal Segal-Rosenheimer, and Connor J. Flynn
Atmos. Chem. Phys., 20, 11275–11285, https://doi.org/10.5194/acp-20-11275-2020, https://doi.org/10.5194/acp-20-11275-2020, 2020
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To help satellite retrieval of aerosols and studies of their radiative effects, we demonstrate that daytime aerosol optical depth over low-level clouds is similar to that in neighboring clear skies at the same heights. Based on recent airborne lidar and sun photometer observations above the southeast Atlantic, the mean AOD difference at 532 nm is between 0 and -0.01, when comparing the cloudy and clear sides of cloud edges, with each up to 20 km wide.
Adeyemi A. Adebiyi, Paquita Zuidema, Ian Chang, Sharon P. Burton, and Brian Cairns
Atmos. Chem. Phys., 20, 11025–11043, https://doi.org/10.5194/acp-20-11025-2020, https://doi.org/10.5194/acp-20-11025-2020, 2020
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Over the southeast Atlantic, interactions between the low-level clouds and the overlying smoke aerosols have previously been highlighted, but no study has yet focused on the presence of the mid-level clouds that complicate the aerosol–cloud interactions. Here we show that these optically thin super-cooled mid-level clouds are relatively common, and they frequently occur at the top of the smoke layer between August and October with significant radiative impacts on the low-level clouds.
Samantha J. Kramer, Claudia Alvarez, Anne E. Barkley, Peter R. Colarco, Lillian Custals, Rodrigo Delgadillo, Cassandra J. Gaston, Ravi Govindaraju, and Paquita Zuidema
Atmos. Chem. Phys., 20, 10047–10062, https://doi.org/10.5194/acp-20-10047-2020, https://doi.org/10.5194/acp-20-10047-2020, 2020
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Comparisons of sea salt and size-resolved dust mass concentration measurements over southeast Florida to those from the MERRA-2/GEOS-5 FP aerosol reanalysis show the reanalysis depicts excessive sea salt and puts too much dust in larger intermediate sizes than do the measurements. The vertical distribution of the dust mass is approximately correct. The incorrect reanalysis aerosol speciation and dust sizes have implications for the modeling of their transport, deposition, and radiative impact.
David Painemal, Fu-Lung Chang, Richard Ferrare, Sharon Burton, Zhujun Li, William L. Smith Jr., Patrick Minnis, Yan Feng, and Marian Clayton
Atmos. Chem. Phys., 20, 7167–7177, https://doi.org/10.5194/acp-20-7167-2020, https://doi.org/10.5194/acp-20-7167-2020, 2020
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Aerosol–cloud interactions (ACIs) are the most uncertain aspect of anthropogenic forcing. Although satellites provide the observational dataset for the global ACI quantification, retrievals are limited to vertically integrated quantities (e.g., aerosol optical depth – AOD), which are typically used as an aerosol proxy. This study demonstrates that matching vertically resolved aerosol from CALIOP at the cloud-layer height with satellite cloud retrievals reduces uncertainties in ACI estimates.
Steven J. Abel, Paul A. Barrett, Paquita Zuidema, Jianhao Zhang, Matt Christensen, Fanny Peers, Jonathan W. Taylor, Ian Crawford, Keith N. Bower, and Michael Flynn
Atmos. Chem. Phys., 20, 4059–4084, https://doi.org/10.5194/acp-20-4059-2020, https://doi.org/10.5194/acp-20-4059-2020, 2020
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In situ measurements of a free-tropospheric (FT) biomass burning aerosol plume in contact with the boundary layer inversion overriding a pocket of open cells (POC) and surrounding stratiform cloud are presented. The data highlight the contrasting thermodynamic, aerosol and cloud properties in the two cloud regimes and further demonstrate that the cloud regime plays a key role in regulating the flow of FT aerosols into the boundary layer, which has implications for the aerosol indirect effect.
Mary Kacarab, K. Lee Thornhill, Amie Dobracki, Steven G. Howell, Joseph R. O'Brien, Steffen Freitag, Michael R. Poellot, Robert Wood, Paquita Zuidema, Jens Redemann, and Athanasios Nenes
Atmos. Chem. Phys., 20, 3029–3040, https://doi.org/10.5194/acp-20-3029-2020, https://doi.org/10.5194/acp-20-3029-2020, 2020
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We find that extensive biomass burning aerosol plumes from southern Africa can profoundly influence clouds in the southeastern Atlantic. Concurrent variations in vertical velocity, however, are found to magnify the relationship between boundary layer aerosol and the cloud droplet number. Neglecting these covariances may strongly bias the sign and magnitude of aerosol impacts on the cloud droplet number.
Jianhao Zhang and Paquita Zuidema
Atmos. Chem. Phys., 19, 14493–14516, https://doi.org/10.5194/acp-19-14493-2019, https://doi.org/10.5194/acp-19-14493-2019, 2019
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Boundary layer (BL) semi-direct effects in the remote SE Atlantic are investigated using LASIC field measurements and satellite retrievals. Low-cloud cover and cloud liquid water path decrease with increasing smoke loadings in the BL. Daily-mean surface-based mixed layer is warmer by 0.5 K, moisture accumulates near the surface throughout the night, and the BL deepens by 200 m, with LWPs and cloud top heights increasing, in the sunlit morning hours, as part of the smoke-altered BL diurnal cycle.
Kristina Pistone, Jens Redemann, Sarah Doherty, Paquita Zuidema, Sharon Burton, Brian Cairns, Sabrina Cochrane, Richard Ferrare, Connor Flynn, Steffen Freitag, Steven G. Howell, Meloë Kacenelenbogen, Samuel LeBlanc, Xu Liu, K. Sebastian Schmidt, Arthur J. Sedlacek III, Michal Segal-Rozenhaimer, Yohei Shinozuka, Snorre Stamnes, Bastiaan van Diedenhoven, Gerard Van Harten, and Feng Xu
Atmos. Chem. Phys., 19, 9181–9208, https://doi.org/10.5194/acp-19-9181-2019, https://doi.org/10.5194/acp-19-9181-2019, 2019
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Understanding how smoke particles interact with sunlight is important in calculating their effects on climate, since some smoke is more scattering (cooling) and some is more absorbing (heating). Knowing this proportion is important for both satellite observations and climate models. We measured smoke properties in a recent aircraft-based field campaign off the west coast of Africa and present a comparison of these properties as measured using the six different, independent techniques available.
Marc Mallet, Pierre Nabat, Paquita Zuidema, Jens Redemann, Andrew Mark Sayer, Martin Stengel, Sebastian Schmidt, Sabrina Cochrane, Sharon Burton, Richard Ferrare, Kerry Meyer, Pablo Saide, Hiren Jethva, Omar Torres, Robert Wood, David Saint Martin, Romain Roehrig, Christina Hsu, and Paola Formenti
Atmos. Chem. Phys., 19, 4963–4990, https://doi.org/10.5194/acp-19-4963-2019, https://doi.org/10.5194/acp-19-4963-2019, 2019
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The model is able to represent LWP but not the LCF. AOD is consistent over the continent but also over ocean (ACAOD). Differences are observed in SSA due to the absence of internal mixing in ALADIN-Climate. A significant regional gradient of the forcing at TOA is observed. An intense positive forcing is simulated over Gabon. Results highlight the significant effect of enhanced moisture on BBA extinction. The surface dimming modifies the energy budget.
David Painemal, Marian Clayton, Richard Ferrare, Sharon Burton, Damien Josset, and Mark Vaughan
Atmos. Meas. Tech., 12, 2201–2217, https://doi.org/10.5194/amt-12-2201-2019, https://doi.org/10.5194/amt-12-2201-2019, 2019
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We present 1 year of a new CALIOP-based aerosol extinction coefficient and lidar ratio over the ocean, with the goal of providing a flexible dataset for climate research as well as independent retrievals that can be helpful for refining CALIPSO Science Team algorithms. The retrievals are derived by constraining the lidar equation with an aerosol optical depth estimated from cross-calibrated CALIOP and CloudSat surface echos.
Eunsil Jung, Bruce A. Albrecht, Armin Sorooshian, Paquita Zuidema, and Haflidi H. Jonsson
Atmos. Chem. Phys., 16, 11395–11413, https://doi.org/10.5194/acp-16-11395-2016, https://doi.org/10.5194/acp-16-11395-2016, 2016
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We calculate the qualitative behavior of precipitation response to aerosol loadings with cloud depths for warm boundary layer clouds (stratocumulus and shallow marine cumulus), using aircraft measurements across four field campaigns. The finding shows that precipitation responds similarly to aerosol loadings for both stratocumulus and cumulus clouds, regardless of cloud type. Precipitation is most susceptible to aerosol perturbations in the medium–deep depth of clouds.
D. Painemal, P. Minnis, and S. Sun-Mack
Atmos. Chem. Phys., 13, 9997–10003, https://doi.org/10.5194/acp-13-9997-2013, https://doi.org/10.5194/acp-13-9997-2013, 2013
C. H. Twohy, J. R. Anderson, D. W. Toohey, M. Andrejczuk, A. Adams, M. Lytle, R. C. George, R. Wood, P. Saide, S. Spak, P. Zuidema, and D. Leon
Atmos. Chem. Phys., 13, 2541–2562, https://doi.org/10.5194/acp-13-2541-2013, https://doi.org/10.5194/acp-13-2541-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
How does riming influence the observed spatial variability of ice water in mixed-phase clouds?
Microphysical view of the development and ice production of mid-latitude stratiform clouds with embedded convection during an extratropical cyclone
Clouds and precipitation in the initial phase of marine cold-air outbreaks as observed by airborne remote sensing
Estimating the snow density using collocated Parsivel and Micro-Rain Radar measurements: a preliminary study from ICE-POP 2017/2018
Technical note: On the ice microphysics of isolated thunderstorms and non-thunderstorms in southern China – a radar polarimetric perspective
Distinctive aerosol–cloud–precipitation interactions in marine boundary layer clouds from the ACE-ENA and SOCRATES aircraft field campaigns
Theoretical Framework for Measuring Cloud Effective Supersaturation Fluctuations with an Advanced Optical System
Drivers of droplet formation in east Mediterranean orographic clouds
Objectively identified mesoscale surface air pressure waves in the context of winter storm environments and radar reflectivity features: a 3+ year analysis
Observability of moisture transport divergence in Arctic atmospheric rivers by dropsondes
Elucidating the boundary layer turbulence dissipation rate using high-resolution measurements from a radar wind profiler network over the Tibetan Plateau
Environmental controls on isolated convection during the Amazonian wet season
Isotopic composition of convective rainfall in the inland tropics of Brazil
Measurement report: Cloud and environmental properties associated with aggregated shallow marine cumulus and cumulus congestus
Lifecycle of updrafts and mass flux in isolated deep convection over the Amazon rainforest: insights from cell tracking
Thermodynamic and cloud evolution in a cold-air outbreak during HALO-(AC)3: quasi-Lagrangian observations compared to the ERA5 and CARRA reanalyses
Powering aircraft with 100 % sustainable aviation fuel reduces ice crystals in contrails
Supercooled liquid water clouds observed over Dome C, Antarctica: temperature sensitivity and cloud radiative forcing
Role of thermodynamic and turbulence processes on the fog life cycle during SOFOG3D experiment
Characterizing the near-global cloud vertical structures over land using high-resolution radiosonde measurements
Differences in microphysical properties of cirrus at high and mid-latitudes
Sub-cloud rain evaporation in the North Atlantic winter trade winds derived by pairing isotopic data with a bin-resolved microphysical model
Overview and statistical analysis of boundary layer clouds and precipitation over the western North Atlantic Ocean
A set of methods to evaluate the below-cloud evaporation effect on local precipitation isotopic composition: a case study for Xi'an, China
Earth-system-model evaluation of cloud and precipitation occurrence for supercooled and warm clouds over the Southern Ocean's Macquarie Island
Pollution slightly enhances atmospheric cooling by low-level clouds in tropical West Africa
Investigating an indirect aviation effect on mid-latitude cirrus clouds – linking lidar-derived optical properties to in situ measurements
Investigating the vertical extent and short-wave radiative effects of the ice phase in Arctic summertime low-level clouds
Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer
Aircraft observations of gravity wave activity and turbulence in the tropical tropopause layer: prevalence, influence on cirrus clouds, and comparison with global storm-resolving models
Influence of air mass origin on microphysical properties of low-level clouds in a subarctic environment
Sensitivity of convectively driven tropical tropopause cirrus properties to ice habits in high-resolution simulations
Upper-tropospheric slightly ice-subsaturated regions: frequency of occurrence and statistical evidence for the appearance of contrail cirrus
Examination of aerosol indirect effects during cirrus cloud evolution
In situ microphysics observations of intense pyroconvection from a large wildfire
Conditions favorable for secondary ice production in Arctic mixed-phase clouds
Interaction between cloud–radiation, atmospheric dynamics and thermodynamics based on observational data from GoAmazon 2014/15 and a cloud-resolving model
Snowfall in Northern Finland derives mostly from ice clouds
Observation of secondary ice production in clouds at low temperatures
In situ and satellite-based estimates of cloud properties and aerosol–cloud interactions over the southeast Atlantic Ocean
Ice fog observed at cirrus temperatures at Dome C, Antarctic Plateau
Life cycle of stratocumulus clouds over 1 year at the coast of the Atacama Desert
Experimental study on the evolution of droplet size distribution during the fog life cycle
Significant continental source of ice-nucleating particles at the tip of Chile's southernmost Patagonia region
Retrieving ice-nucleating particle concentration and ice multiplication factors using active remote sensing validated by in situ observations
Temporal and vertical distributions of the occurrence of cirrus clouds over a coastal station in the Indian monsoon region
Continental thunderstorm ground enhancement observed at an exceptionally low altitude
Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions
In situ observation of riming in mixed-phase clouds using the PHIPS probe
Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice-nucleating particles and instrument inter-comparison in the Hyytiälä boreal forest
Nina Maherndl, Manuel Moser, Imke Schirmacher, Aaron Bansemer, Johannes Lucke, Christiane Voigt, and Maximilian Maahn
Atmos. Chem. Phys., 24, 13935–13960, https://doi.org/10.5194/acp-24-13935-2024, https://doi.org/10.5194/acp-24-13935-2024, 2024
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It is not clear why ice crystals in clouds occur in clusters. Here, airborne measurements of clouds in mid-latitudes and high latitudes are used to study the spatial variability of ice. Further, we investigate the influence of riming, which occurs when liquid droplets freeze onto ice crystals. We find that riming enhances the occurrence of ice clusters. In the Arctic, riming leads to ice clustering at spatial scales of 3–5 km. This is due to updrafts and not higher amounts of liquid water.
Yuanmou Du, Dantong Liu, Delong Zhao, Mengyu Huang, Ping Tian, Dian Wen, Wei Xiao, Wei Zhou, Hui He, Baiwan Pan, Dongfei Zuo, Xiange Liu, Yingying Jing, Rong Zhang, Jiujiang Sheng, Fei Wang, Yu Huang, Yunbo Chen, and Deping Ding
Atmos. Chem. Phys., 24, 13429–13444, https://doi.org/10.5194/acp-24-13429-2024, https://doi.org/10.5194/acp-24-13429-2024, 2024
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By conducting in situ measurements, we investigated ice production processes in stratiform clouds with embedded convection over the North China Plain. The results show that the ice number concentration is strongly related to the distance to the cloud top, and the level with a larger distance to the cloud top has more graupel falling from upper levels, which promotes collision and coalescence between graupel and droplets and enhances secondary ice production.
Imke Schirmacher, Sabrina Schnitt, Marcus Klingebiel, Nina Maherndl, Benjamin Kirbus, André Ehrlich, Mario Mech, and Susanne Crewell
Atmos. Chem. Phys., 24, 12823–12842, https://doi.org/10.5194/acp-24-12823-2024, https://doi.org/10.5194/acp-24-12823-2024, 2024
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During Arctic marine cold-air outbreaks, cold air flows from sea ice over open water. Roll circulations evolve, forming cloud streets. We investigate the initial circulation and cloud development using high-resolution airborne measurements. We compute the distance an air mass traveled over water (fetch) from back trajectories. Cloud streets form at 15 km fetch, cloud cover strongly increases at around 20 km, and precipitation forms at around 30 km.
Wei-Yu Chang, Yung-Chuan Yang, Chen-Yu Hung, Kwonil Kim, Gyuwon Lee, and Ali Tokay
Atmos. Chem. Phys., 24, 11955–11979, https://doi.org/10.5194/acp-24-11955-2024, https://doi.org/10.5194/acp-24-11955-2024, 2024
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Snow density is derived by collocated Micro-Rain Radar (MRR) and Parsivel (ICE-POP 2017/2018). We apply the particle size distribution from Parsivel to a T-matrix backscattering simulation and compare with ZHH from MRR. Bulk density and bulk water fractions are derived from comparing simulated and calculated ZHH. Retrieved bulk density is validated by comparing snowfall rate measurements from Pluvio and the Precipitation Imaging Package. Snowfall rate consistency confirms the algorithm.
Chuanhong Zhao, Yijun Zhang, Dong Zheng, Haoran Li, Sai Du, Xueyan Peng, Xiantong Liu, Pengguo Zhao, Jiafeng Zheng, and Juan Shi
Atmos. Chem. Phys., 24, 11637–11651, https://doi.org/10.5194/acp-24-11637-2024, https://doi.org/10.5194/acp-24-11637-2024, 2024
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Understanding lightning activity is important for meteorology and atmospheric chemistry. However, the occurrence of lightning activity in clouds is uncertain. In this study, we quantified the difference between isolated thunderstorms and non-thunderstorms. We showed that lightning activity was more likely to occur with more graupel volume and/or riming. A deeper ZDR column was associated with lightning occurrence. This information can aid in a deeper understanding of lighting physics.
Xiaojian Zheng, Xiquan Dong, Baike Xi, Timothy Logan, and Yuan Wang
Atmos. Chem. Phys., 24, 10323–10347, https://doi.org/10.5194/acp-24-10323-2024, https://doi.org/10.5194/acp-24-10323-2024, 2024
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The marine boundary layer aerosol–cloud interactions (ACIs) are examined using in situ measurements from two aircraft campaigns over the eastern North Atlantic (ACE-ENA) and Southern Ocean (SOCRATES). The SOCRATES clouds have more and smaller cloud droplets. The ACE-ENA clouds exhibit stronger drizzle formation and growth. Results found distinctive aerosol–cloud interactions for two campaigns. The drizzle processes significantly alter sub-cloud aerosol budgets and impact the ACI assessments.
Ye Kuang, Jiangchuan Tao, Hanbin Xu, Li Liu, Pengfei Liu, Wanyun Xu, Weiqi Xu, Yele Sun, and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-2698, https://doi.org/10.5194/egusphere-2024-2698, 2024
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This study presents a novel optical framework to measure supersaturation, a fundamental parameter in cloud physics, by observing the scattering properties of particles that have or have not grown into cloud droplets. The technique offers high-resolution measurements, capturing essential fluctuations in supersaturation necessary for understanding cloud physics.
Romanos Foskinis, Ghislain Motos, Maria I. Gini, Olga Zografou, Kunfeng Gao, Stergios Vratolis, Konstantinos Granakis, Ville Vakkari, Kalliopi Violaki, Andreas Aktypis, Christos Kaltsonoudis, Zongbo Shi, Mika Komppula, Spyros N. Pandis, Konstantinos Eleftheriadis, Alexandros Papayannis, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9827–9842, https://doi.org/10.5194/acp-24-9827-2024, https://doi.org/10.5194/acp-24-9827-2024, 2024
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Analysis of modeling, in situ, and remote sensing measurements reveals the microphysical state of orographic clouds and their response to aerosol from the boundary layer and free troposphere. We show that cloud response to aerosol is robust, as predicted supersaturation and cloud droplet number levels agree with those determined from in-cloud measurements. The ability to determine if clouds are velocity- or aerosol-limited allows for novel model constraints and remote sensing products.
Luke R. Allen, Sandra E. Yuter, Matthew A. Miller, and Laura M. Tomkins
EGUsphere, https://doi.org/10.5194/egusphere-2024-2160, https://doi.org/10.5194/egusphere-2024-2160, 2024
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Atmospheric gravity waves are air oscillations in which buoyancy is the restoring force, which can enhance precipitation production. We used 3+ seasons of pressure data to identify gravity waves with wavelengths ≤ 170 km in the Toronto and New York metropolitan areas in the context of snow storms. Of 79 snow events, only 6 had detectable gravity wave events, suggesting that gravity waves on the scales of typical radar reflectivity features are uncommon in those two locations during snow storms.
Henning Dorff, Heike Konow, Vera Schemann, and Felix Ament
Atmos. Chem. Phys., 24, 8771–8795, https://doi.org/10.5194/acp-24-8771-2024, https://doi.org/10.5194/acp-24-8771-2024, 2024
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Using synthetic dropsondes, we assess how discrete spatial sampling and temporal evolution during flight affect the accuracy of real sonde-based moisture transport divergence in Arctic atmospheric rivers (ARs). Non-instantaneous sampling during temporal AR evolution deteriorates the divergence values more than spatial undersampling. Moisture advection is the dominating factor but most sensitive to the sampling method. We suggest a minimum of seven sondes to resolve the AR divergence components.
Deli Meng, Jianping Guo, Xiaoran Guo, Yinjun Wang, Ning Li, Yuping Sun, Zhen Zhang, Na Tang, Haoran Li, Fan Zhang, Bing Tong, Hui Xu, and Tianmeng Chen
Atmos. Chem. Phys., 24, 8703–8720, https://doi.org/10.5194/acp-24-8703-2024, https://doi.org/10.5194/acp-24-8703-2024, 2024
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The turbulence in the planetary boundary layer (PBL) over the Tibetan Plateau (TP) remains unclear. Here we elucidate the vertical profile of and temporal variation in the turbulence dissipation rate in the PBL over the TP based on a radar wind profiler (RWP) network. To the best of our knowledge, this is the first time that the turbulence profile over the whole TP has been revealed. Furthermore, the possible mechanisms of clouds acting on the PBL turbulence structure are investigated.
Leandro Alex Moreira Viscardi, Giuseppe Torri, David K. Adams, and Henrique de Melo Jorge Barbosa
Atmos. Chem. Phys., 24, 8529–8548, https://doi.org/10.5194/acp-24-8529-2024, https://doi.org/10.5194/acp-24-8529-2024, 2024
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We evaluate the environmental conditions that control how clouds grow from fair weather cumulus into severe thunderstorms during the Amazonian wet season. Days with rain clouds begin with more moisture in the air and have strong convergence in the afternoon, while precipitation intensity increases with large-scale vertical velocity, moisture, and low-level wind. These results contribute to understanding how clouds form over the rainforest.
Vinicius dos Santos, Didier Gastmans, Ana María Durán-Quesada, Ricardo Sánchez-Murillo, Kazimierz Rozanski, Oliver Kracht, and Demilson de Assis Quintão
Atmos. Chem. Phys., 24, 6663–6680, https://doi.org/10.5194/acp-24-6663-2024, https://doi.org/10.5194/acp-24-6663-2024, 2024
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We present novel findings on convective rainfall, summer rain in the late afternoon, by coupling water stable isotopes, micro rain radar, and satellite data. We found the tallest clouds in the afternoon and much smaller clouds at night, resulting in differences in day–night ratios in water stable isotopes. We sampled rain and meteorological variables every 5–10 min, allowing us to evaluate the development of convective rainfall, contributing to knowledge of rainfall related to extreme events.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
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Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Siddhant Gupta, Dié Wang, Scott E. Giangrande, Thiago S. Biscaro, and Michael P. Jensen
Atmos. Chem. Phys., 24, 4487–4510, https://doi.org/10.5194/acp-24-4487-2024, https://doi.org/10.5194/acp-24-4487-2024, 2024
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We examine the lifecycle of isolated deep convective clouds (DCCs) in the Amazon rainforest. Weather radar echoes from the DCCs are tracked to evaluate their lifecycle. The DCC size and intensity increase, reach a peak, and then decrease over the DCC lifetime. Vertical profiles of air motion and mass transport from different seasons are examined to understand the transport of energy and momentum within DCC cores and to address the deficiencies in simulating DCCs using weather and climate models.
Benjamin Kirbus, Imke Schirmacher, Marcus Klingebiel, Michael Schäfer, André Ehrlich, Nils Slättberg, Johannes Lucke, Manuel Moser, Hanno Müller, and Manfred Wendisch
Atmos. Chem. Phys., 24, 3883–3904, https://doi.org/10.5194/acp-24-3883-2024, https://doi.org/10.5194/acp-24-3883-2024, 2024
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A research aircraft is used to track the changes in air temperature, moisture, and cloud properties for air that moves from cold Arctic sea ice onto warmer oceanic waters. The measurements are compared to two reanalysis models named ERA5 and CARRA. The biggest differences are found for air temperature over the sea ice and moisture over the ocean. CARRA data are more accurate than ERA5 because they better simulate the sea ice, the transition from sea ice to open ocean, and the forming clouds.
Raphael Satoru Märkl, Christiane Voigt, Daniel Sauer, Rebecca Katharina Dischl, Stefan Kaufmann, Theresa Harlaß, Valerian Hahn, Anke Roiger, Cornelius Weiß-Rehm, Ulrike Burkhardt, Ulrich Schumann, Andreas Marsing, Monika Scheibe, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Reetu Sallinen, Tobias Schripp, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 3813–3837, https://doi.org/10.5194/acp-24-3813-2024, https://doi.org/10.5194/acp-24-3813-2024, 2024
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In situ measurements of contrails from a large passenger aircraft burning 100 % sustainable aviation fuel (SAF) show a 56 % reduction in contrail ice crystal numbers compared to conventional Jet A-1. Results from a climate model initialized with the observations suggest a significant decrease in radiative forcing from contrails. Our study confirms that future increased use of low aromatic SAF can reduce the climate impact from aviation.
Philippe Ricaud, Massimo Del Guasta, Angelo Lupi, Romain Roehrig, Eric Bazile, Pierre Durand, Jean-Luc Attié, Alessia Nicosia, and Paolo Grigioni
Atmos. Chem. Phys., 24, 613–630, https://doi.org/10.5194/acp-24-613-2024, https://doi.org/10.5194/acp-24-613-2024, 2024
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Clouds affect the Earth's climate in ways that depend on the type of cloud (solid/liquid water). From observations at Concordia (Antarctica), we show that in supercooled liquid water (liquid water for temperatures below 0°C) clouds (SLWCs), temperature and SLWC radiative forcing increase with liquid water (up to 70 W m−2). We extrapolated that the maximum SLWC radiative forcing can reach 40 W m−2 over the Antarctic Peninsula, highlighting the importance of SLWCs for global climate prediction.
Cheikh Dione, Martial Haeffelin, Frédéric Burnet, Christine Lac, Guylaine Canut, Julien Delanoë, Jean-Charles Dupont, Susana Jorquera, Pauline Martinet, Jean-François Ribaud, and Felipe Toledo
Atmos. Chem. Phys., 23, 15711–15731, https://doi.org/10.5194/acp-23-15711-2023, https://doi.org/10.5194/acp-23-15711-2023, 2023
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This paper documents the role of thermodynamics and turbulence in the fog life cycle over southwestern France. It is based on a unique dataset collected during the SOFOG3D field campaign in autumn and winter 2019–2020. The paper gives a threshold for turbulence driving the different phases of the fog life cycle and the role of advection in the night-time dissipation of fog. The results can be operationalised to nowcast fog and improve short-range forecasts in numerical weather prediction models.
Hui Xu, Jianping Guo, Bing Tong, Jinqiang Zhang, Tianmeng Chen, Xiaoran Guo, Jian Zhang, and Wenqing Chen
Atmos. Chem. Phys., 23, 15011–15038, https://doi.org/10.5194/acp-23-15011-2023, https://doi.org/10.5194/acp-23-15011-2023, 2023
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The radiative effect of cloud remains one of the largest uncertain factors in climate change, largely due to the lack of cloud vertical structure (CVS) observations. The study presents the first near-global CVS climatology using high-vertical-resolution soundings. Single-layer cloud mainly occurs over arid regions. As the number of cloud layers increases, clouds tend to have lower bases and thinner layer thicknesses. The occurrence frequency of cloud exhibits a pronounced seasonal diurnal cycle.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
Atmos. Chem. Phys., 23, 13167–13189, https://doi.org/10.5194/acp-23-13167-2023, https://doi.org/10.5194/acp-23-13167-2023, 2023
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In this study, we show the differences in the microphysical properties between high-latitude (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region on cloud formation. We show that HL cirrus are characterized by a lower concentration of larger ice crystals when compared to ML cirrus.
Mampi Sarkar, Adriana Bailey, Peter Blossey, Simon P. de Szoeke, David Noone, Estefanía Quiñones Meléndez, Mason D. Leandro, and Patrick Y. Chuang
Atmos. Chem. Phys., 23, 12671–12690, https://doi.org/10.5194/acp-23-12671-2023, https://doi.org/10.5194/acp-23-12671-2023, 2023
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We study rain evaporation characteristics below shallow cumulus clouds over the North Atlantic Ocean by pairing isotope observations with a microphysical model. The modeled fraction of rain mass that evaporates below the cloud strongly depends on the raindrop size and distribution width. Moreover, the higher the rain mass fraction evaporated, the greater the change in deuterium excess. In this way, rain evaporation could be studied independently using only isotope and microphysical observations.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Meng Xing, Weiguo Liu, Jing Hu, and Zheng Wang
Atmos. Chem. Phys., 23, 9123–9136, https://doi.org/10.5194/acp-23-9123-2023, https://doi.org/10.5194/acp-23-9123-2023, 2023
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The below-cloud evaporation effect (BCE) on precipitation largely impacts the final isotopic composition. However, determining the BCE effect remains poorly constrained. Our work used a ΔdΔδ diagram to differentiate the below-cloud processes. Moreover, by comparing two different computing methods, we considered that both methods are suitable for evaluation the BCE, except for snowfall events. Overall, our work compiled a set of effective methods to evaluate the BCE effect.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
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Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
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The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Rachel Atlas and Christopher S. Bretherton
Atmos. Chem. Phys., 23, 4009–4030, https://doi.org/10.5194/acp-23-4009-2023, https://doi.org/10.5194/acp-23-4009-2023, 2023
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The tropical tropopause layer exists between the troposphere and the stratosphere in the tropics. Very thin cirrus clouds cool Earth's surface by scrubbing water vapor (a greenhouse gas) out of air parcels as they ascend through the tropical tropopause layer on their way to the stratosphere. We show observational evidence from aircraft that small-scale (< 100 km) gravity waves and turbulence increase the amount of ice in these clouds and may allow them to remove more water vapor from the air.
Konstantinos Matthaios Doulgeris, Ville Vakkari, Ewan J. O'Connor, Veli-Matti Kerminen, Heikki Lihavainen, and David Brus
Atmos. Chem. Phys., 23, 2483–2498, https://doi.org/10.5194/acp-23-2483-2023, https://doi.org/10.5194/acp-23-2483-2023, 2023
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We investigated how different long-range-transported air masses can affect the microphysical properties of low-level clouds in a clean subarctic environment. A connection was revealed. Higher values of cloud droplet number concentrations were related to continental air masses, whereas the lowest values of number concentrations were related to marine air masses. These were characterized by larger cloud droplets. Clouds in all regions were sensitive to increases in cloud number concentration.
Fayçal Lamraoui, Martina Krämer, Armin Afchine, Adam B. Sokol, Sergey Khaykin, Apoorva Pandey, and Zhiming Kuang
Atmos. Chem. Phys., 23, 2393–2419, https://doi.org/10.5194/acp-23-2393-2023, https://doi.org/10.5194/acp-23-2393-2023, 2023
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Cirrus in the tropical tropopause layer (TTL) can play a key role in vertical transport. We investigate the role of different cloud regimes and the associated ice habits in regulating the properties of the TTL. We use high-resolution numerical experiments at the scales of large-eddy simulations (LESs) and aircraft measurements. We found that LES-scale parameterizations that predict ice shape are crucial for an accurate representation of TTL cirrus and thus the associated (de)hydration process.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Flor Vanessa Maciel, Minghui Diao, and Ryan Patnaude
Atmos. Chem. Phys., 23, 1103–1129, https://doi.org/10.5194/acp-23-1103-2023, https://doi.org/10.5194/acp-23-1103-2023, 2023
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Aerosol indirect effects on cirrus clouds are investigated during cirrus evolution, using global-scale in situ observations and climate model simulations. As cirrus evolves, the mechanisms to form ice crystals also change with time. Both small and large aerosols are found to affect cirrus properties. Southern Hemisphere cirrus appears to be more sensitive to additional aerosols. The climate model underestimates ice crystal mass, likely due to biases of relative humidity and vertical velocity.
David E. Kingsmill, Jeffrey R. French, and Neil P. Lareau
Atmos. Chem. Phys., 23, 1–21, https://doi.org/10.5194/acp-23-1-2023, https://doi.org/10.5194/acp-23-1-2023, 2023
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This study uses in situ aircraft measurements to characterize the size and shape distributions of 10 µm to 6 mm diameter particles observed during six penetrations of wildfire-induced pyroconvection. Particles sampled in one penetration of a smoke plume are most likely pyrometeors composed of ash. The other penetrations are through pyrocumulus clouds where particle composition is most likely a combination of hydrometeors (ice particles) and pyrometeors (ash).
Julie Thérèse Pasquier, Jan Henneberger, Fabiola Ramelli, Annika Lauber, Robert Oscar David, Jörg Wieder, Tim Carlsen, Rosa Gierens, Marion Maturilli, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 15579–15601, https://doi.org/10.5194/acp-22-15579-2022, https://doi.org/10.5194/acp-22-15579-2022, 2022
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It is important to understand how ice crystals and cloud droplets form in clouds, as their concentrations and sizes determine the exact radiative properties of the clouds. Normally, ice crystals form from aerosols, but we found evidence for the formation of additional ice crystals from the original ones over a large temperature range within Arctic clouds. In particular, additional ice crystals were formed during collisions of several ice crystals or during the freezing of large cloud droplets.
Layrson J. M. Gonçalves, Simone M. S. C. Coelho, Paulo Y. Kubota, and Dayana C. Souza
Atmos. Chem. Phys., 22, 15509–15526, https://doi.org/10.5194/acp-22-15509-2022, https://doi.org/10.5194/acp-22-15509-2022, 2022
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This research aims to study the environmental conditions that are favorable and not favorable to cloud formation, in this case specifically for the Amazon region. The results found in this research will be used to improve the representation of clouds in numerical models that are used in weather and climate prediction. In general, it is expected that with better knowledge regarding the cloud–radiation interaction, it is possible to make a better forecast of weather and climate.
Claudia Mignani, Lukas Zimmermann, Rigel Kivi, Alexis Berne, and Franz Conen
Atmos. Chem. Phys., 22, 13551–13568, https://doi.org/10.5194/acp-22-13551-2022, https://doi.org/10.5194/acp-22-13551-2022, 2022
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We determined over the course of 8 winter months the phase of clouds associated with snowfall in Northern Finland using radiosondes and observations of ice particle habits at ground level. We found that precipitating clouds were extending from near ground to at least 2.7 km altitude and approximately three-quarters of them were likely glaciated. Possible moisture sources and ice formation processes are discussed.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
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The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Étienne Vignon, Lea Raillard, Christophe Genthon, Massimo Del Guasta, Andrew J. Heymsfield, Jean-Baptiste Madeleine, and Alexis Berne
Atmos. Chem. Phys., 22, 12857–12872, https://doi.org/10.5194/acp-22-12857-2022, https://doi.org/10.5194/acp-22-12857-2022, 2022
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The near-surface atmosphere over the Antarctic Plateau is cold and pristine and resembles to a certain extent the high troposphere where cirrus clouds form. In this study, we use innovative humidity measurements at Concordia Station to study the formation of ice fogs at temperatures <−40°C. We provide observational evidence that ice fogs can form through the homogeneous freezing of solution aerosols, a common nucleation pathway for cirrus clouds.
Jan H. Schween, Camilo del Rio, Juan-Luis García, Pablo Osses, Sarah Westbrook, and Ulrich Löhnert
Atmos. Chem. Phys., 22, 12241–12267, https://doi.org/10.5194/acp-22-12241-2022, https://doi.org/10.5194/acp-22-12241-2022, 2022
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Marine stratocumulus clouds of the eastern Pacific play an essential role in the Earth's climate. These clouds form the major source of water to parts of the extreme dry Atacama Desert at the northern coast of Chile. For the first time these clouds are observed over a whole year with three remote sensing instruments. It is shown how these clouds are influenced by the land–sea wind system and the distribution of ocean temperatures.
Marie Mazoyer, Frédéric Burnet, and Cyrielle Denjean
Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, https://doi.org/10.5194/acp-22-11305-2022, 2022
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The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
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Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Saleem Ali, Sanjay Kumar Mehta, Aravindhavel Ananthavel, and Tondapu Venkata Ramesh Reddy
Atmos. Chem. Phys., 22, 8321–8342, https://doi.org/10.5194/acp-22-8321-2022, https://doi.org/10.5194/acp-22-8321-2022, 2022
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Multiple cirrus clouds frequently occur over regions of deep convection in the tropics. Tropical convection has a strong diurnal pattern, with peaks in the afternoon to early evening, over the continents. Continuous micropulse lidar observations over a coastal station in the Indian monsoon region enable us, for the first time, to demonstrate a robust diurnal pattern of single and multiple cirrus occurrences, with peaks during the late afternoon and early morning hours, respectively.
Ivana Kolmašová, Ondřej Santolík, Jakub Šlegl, Jana Popová, Zbyněk Sokol, Petr Zacharov, Ondřej Ploc, Gerhard Diendorfer, Ronald Langer, Radek Lán, and Igor Strhárský
Atmos. Chem. Phys., 22, 7959–7973, https://doi.org/10.5194/acp-22-7959-2022, https://doi.org/10.5194/acp-22-7959-2022, 2022
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Gamma ray radiation related to thunderstorms was previously observed at the high-altitude mountain observatories or on the western coast of Japan, usually being terminated by lightning discharges. We show unusual observations of gamma rays at an altitude below 1000 m, coinciding with peculiar rapid variations in the vertical electric field, which are linked to inverted intracloud lightning discharges. This indicates that a strong, lower positive-charge region was present inside the thundercloud.
Cuiqi Zhang, Zhijun Wu, Jingchuan Chen, Jie Chen, Lizi Tang, Wenfei Zhu, Xiangyu Pei, Shiyi Chen, Ping Tian, Song Guo, Limin Zeng, Min Hu, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7539–7556, https://doi.org/10.5194/acp-22-7539-2022, https://doi.org/10.5194/acp-22-7539-2022, 2022
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The immersion ice nucleation effectiveness of aerosols from multiple sources in the urban environment remains elusive. In this study, we demonstrate that the immersion ice-nucleating particle (INP) concentration increased dramatically during a dust event in an urban atmosphere. Pollutant aerosols, including inorganic salts formed through secondary transformation (SIA) and black carbon (BC), might not act as effective INPs under mixed-phase cloud conditions.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Chem. Phys., 22, 7087–7103, https://doi.org/10.5194/acp-22-7087-2022, https://doi.org/10.5194/acp-22-7087-2022, 2022
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Riming, i.e., the accretion of small droplets on the surface of ice particles via collision, is one of the major uncertainties in model prediction of mixed-phase clouds. We discuss the occurrence (up to 50% of particles) and aging of rimed ice particles and show correlations of the occurrence and the degree of riming with ambient meteorological parameters using data gathered by the Particle Habit Imaging and Polar Scattering (PHIPS) probe during three airborne in situ field campaigns.
Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 5117–5145, https://doi.org/10.5194/acp-22-5117-2022, https://doi.org/10.5194/acp-22-5117-2022, 2022
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The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
Cited articles
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Bennartz, R.: Global assessment of marine boundary layer cloud droplet number concentration from satellite, J. Geophys. Res., 112, D02201, https://doi.org/10.1029/2006JD007547, 2007.
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