Articles | Volume 23, issue 9
https://doi.org/10.5194/acp-23-5419-2023
https://doi.org/10.5194/acp-23-5419-2023
Research article
 | 
16 May 2023
Research article |  | 16 May 2023

Multiple pathways for the formation of secondary organic aerosol in the North China Plain in summer

Yifang Gu, Ru-Jin Huang, Jing Duan, Wei Xu, Chunshui Lin, Haobin Zhong, Ying Wang, Haiyan Ni, Quan Liu, Ruiguang Xu, Litao Wang, and Yong Jie Li

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Cited articles

An, Z., Huang, R. J., Zhang, R., Tie, X., Li, G., Cao, J., Zhou, W., Shi, Z., Han, Y., Gu, Z., and Ji, Y.: Severe haze in northern China: A synergy of anthropogenic emissions and atmospheric processes, P. Natl. Acad. Sci. USA, 116, 8657–8666, https://doi.org/10.1073/pnas.1900125116, 2019. 
Bikkina, S., Kawamura, K., and Sarin, M.: Secondary Organic Aerosol Formation over Coastal Ocean: Inferences from Atmospheric Water-Soluble Low Molecular Weight Organic Compounds, Environ. Sci. Technol., 51, 4347–4357, https://doi.org/10.1021/acs.est.6b05986, 2017. 
Canagaratna, M. R., Jimenez, J. L., Kroll, J. H., Chen, Q., Kessler, S. H., Massoli, P., Hildebrandt Ruiz, L., Fortner, E., Williams, L. R., Wilson, K. R., Surratt, J. D., Donahue, N. M., Jayne, J. T., and Worsnop, D. R.: Elemental ratio measurements of organic compounds using aerosol mass spectrometry: characterization, improved calibration, and implications, Atmos. Chem. Phys., 15, 253–272, https://doi.org/10.5194/acp-15-253-2015, 2015. 
Canonaco, F., Crippa, M., Slowik, J. G., Baltensperger, U., and Prévôt, A. S. H.: SoFi, an IGOR-based interface for the efficient use of the generalized multilinear engine (ME-2) for the source apportionment: ME-2 application to aerosol mass spectrometer data, Atmos. Meas. Tech., 6, 3649–3661, https://doi.org/10.5194/amt-6-3649-2013, 2013. 
Carlton, A. G., Turpin, B. J., Altieri, K. E., Seitzinger, S., Reff, A., Lim, H. J., and Ervens, B.: Atmospheric oxalic acid and SOA production from glyoxal: Results of aqueous photooxidation experiments, Atmos. Environ., 41, 7588–7602, https://doi.org/10.1016/j.atmosenv.2007.05.035, 2007. 
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Short summary
Secondary organic aerosol (SOA) can be produced by various pathways, but its formation mechanisms are unclear. Observations were conducted in the North China Plain during a highly oxidizing atmosphere in summer. We found that fast photochemistry dominated SOA formation during daytime. Two types of aqueous-phase chemistry (nocturnal and daytime processing) take place at high relative humidity. The potential transformation from primary organic aerosol (POA) to SOA was also an important pathway.
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