Articles | Volume 23, issue 9
https://doi.org/10.5194/acp-23-5419-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-5419-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Multiple pathways for the formation of secondary organic aerosol in the North China Plain in summer
Yifang Gu
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
University of Chinese Academy of Sciences, Beijing 100049, China
Ru-Jin Huang
CORRESPONDING AUTHOR
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
Institute of Global Environmental Change, Xi'an Jiaotong University, Xi'an 710049, China
University of Chinese Academy of Sciences, Beijing 100049, China
Jing Duan
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
Chunshui Lin
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
Haobin Zhong
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
University of Chinese Academy of Sciences, Beijing 100049, China
Ying Wang
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
Haiyan Ni
SKLLQG, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China
State Key Laboratory of Severe Weather & Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Ruiguang Xu
Department of Environmental Engineering, School of Energy and Environmental Engineering, Hebei University of Engineering, Handan 056038, China
Hebei Key Laboratory of Air Pollution Cause and Impact, Handan 056038, China
Litao Wang
Department of Environmental Engineering, School of Energy and Environmental Engineering, Hebei University of Engineering, Handan 056038, China
Hebei Key Laboratory of Air Pollution Cause and Impact, Handan 056038, China
Yong Jie Li
Department of Civil and Environmental Engineering, Faculty of Science and Technology, University of Macau, Taipa, Macau SAR 999078, China
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24 citations as recorded by crossref.
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- Source apportionment and secondary organic aerosol formation potential of VOCs in urban and suburban areas of South Korea K. Kim et al.
- Aerosol and precipitation composition at a coastal New England site (Acadia National Park): implications for air quality and aerosol composition during cold air outbreaks A. Seckar-Martinez et al.
- Rapid formation of secondary aerosol precursors from the autoxidation of C5–C8 n-aldehydes S. Barua et al.
- Mixing state and evolutionary mechanism of oxalic acid homologs in Liaocheng, East China: Insights from seasonal and hourly observations J. Ma et al.
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- Atmospheric aqueous-phase reactions of organics in dark: A review Y. Sha et al.
- Fossil-dominated secondary organic aerosol (SOA) formation in coastal China: size-divergent pathways of aqueous Fenton reactions versus gas-phase volatile organic compound (VOC) autoxidation J. Wang et al.
- Divergent changes in aerosol optical hygroscopicity and new particle formation during a heatwave of summer 2022 Y. Hao et al.
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al.
- Influence of anthropogenic pollution on the molecular composition of organic aerosols over a forest site in the Qinling Mountains region of central China X. Zhang et al.
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- Drivers of biogenic secondary organic aerosols in Eastern China: Evidence from machine learning and high-resolution measurements K. Zhang et al.
- Evaluating simulations of organic aerosol volatility and degree of oxygenation in eastern China Y. Li et al.
- Influence of atmospheric ammonia on secondary inorganic aerosol formation in PM2.5 during spring 2024 in the Hongseong area, Republic of Korea J. Jang et al.
- Variations in polycyclic aromatic hydrocarbons concentrations and their contribution to aerosol optical depth during the COVID-19 outbreak: A study in Yokohama using generalized additive model W. Jing et al.
24 citations as recorded by crossref.
- The semi-solid phase of atmospheric particles facilitates the formation of secondary brown carbon: Possible contribution of ionic strength to Maillard-like reactions J. Xie et al.
- Characteristics and processing of aqueous secondary organic aerosols during autumn in suburban Eastern China: role of aerosol liquid water, aerosol acidity, and photochemistry Q. Wang et al.
- Characteristics of airborne bacteria over inland and coastal atmosphere influenced by systemic air mass in northern China Z. Wang et al.
- Source apportionment and secondary organic aerosol formation potential of VOCs in urban and suburban areas of South Korea K. Kim et al.
- Aerosol and precipitation composition at a coastal New England site (Acadia National Park): implications for air quality and aerosol composition during cold air outbreaks A. Seckar-Martinez et al.
- Rapid formation of secondary aerosol precursors from the autoxidation of C5–C8 n-aldehydes S. Barua et al.
- Mixing state and evolutionary mechanism of oxalic acid homologs in Liaocheng, East China: Insights from seasonal and hourly observations J. Ma et al.
- Emission Characteristics, Environmental Impacts, and Health Risks of Volatile Organic Compounds from Asphalt Materials: A State-of-the-Art Review J. Li et al.
- Measurement report: Size-resolved secondary organic aerosol formation modulated by aerosol water uptake in wintertime haze J. Duan et al.
- Wintertime fine aerosol particles composition and its evolution in two megacities of southern and northern China Y. Cheng et al.
- Current challenges in the visibility improvement of urban Chongqing in Southwest China: From the perspective of PM2.5-bound water uptake property over 2015–2021 Y. Hao et al.
- Unveiling seasonal dynamics of nitrate aerosols: A crucial step in understanding atmospheric pollution Q. Wang et al.
- Atmospheric aqueous-phase reactions of organics in dark: A review Y. Sha et al.
- Fossil-dominated secondary organic aerosol (SOA) formation in coastal China: size-divergent pathways of aqueous Fenton reactions versus gas-phase volatile organic compound (VOC) autoxidation J. Wang et al.
- Divergent changes in aerosol optical hygroscopicity and new particle formation during a heatwave of summer 2022 Y. Hao et al.
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al.
- Influence of anthropogenic pollution on the molecular composition of organic aerosols over a forest site in the Qinling Mountains region of central China X. Zhang et al.
- Sources of PM2.5 exposure and health benefits of clean air actions in Shanghai Y. Gu et al.
- Unveiling the key drivers and formation pathways for secondary organic aerosols in an eastern China megacity F. Zhang et al.
- Influence of ozone pollution on the mixing state and formation of oxygenated organics containing single particles S. Liu et al.
- Drivers of biogenic secondary organic aerosols in Eastern China: Evidence from machine learning and high-resolution measurements K. Zhang et al.
- Evaluating simulations of organic aerosol volatility and degree of oxygenation in eastern China Y. Li et al.
- Influence of atmospheric ammonia on secondary inorganic aerosol formation in PM2.5 during spring 2024 in the Hongseong area, Republic of Korea J. Jang et al.
- Variations in polycyclic aromatic hydrocarbons concentrations and their contribution to aerosol optical depth during the COVID-19 outbreak: A study in Yokohama using generalized additive model W. Jing et al.
Saved (final revised paper)
Latest update: 06 May 2026
Short summary
Secondary organic aerosol (SOA) can be produced by various pathways, but its formation mechanisms are unclear. Observations were conducted in the North China Plain during a highly oxidizing atmosphere in summer. We found that fast photochemistry dominated SOA formation during daytime. Two types of aqueous-phase chemistry (nocturnal and daytime processing) take place at high relative humidity. The potential transformation from primary organic aerosol (POA) to SOA was also an important pathway.
Secondary organic aerosol (SOA) can be produced by various pathways, but its formation...
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