Articles | Volume 15, issue 5
Research article
02 Mar 2015
Research article |  | 02 Mar 2015

Aerosol size distribution and radiative forcing response to anthropogenically driven historical changes in biogenic secondary organic aerosol formation

S. D. D'Andrea, J. C. Acosta Navarro, S. C. Farina, C. E. Scott, A. Rap, D. K. Farmer, D. V. Spracklen, I. Riipinen, and J. R. Pierce

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Cited articles

Acosta Navarro, J. C., Smolander, S., Struthers, H., Zorita, E., Ekman, A. M. L., Kaplan, J. O., Guenther, A., Arneth, A. and Riipinen, I.: Global emissions of terpenoid VOCs from terrestrial vegetation in the last millennium, J. Geophys. Res.-Atmos., 119, 6867–6885,, 2014
Adams, P. J. and Seinfeld, J. H.: Disproportionate impact of particulate emissions on global cloud condensation nuclei concentrations, Geophys. Res. Lett., 30, 1210–1239,, 2003.
Arneth, A., Niinemets, Ü., Pressley, S., Bäck, J., Hari, P., Karl, T., Noe, S., Prentice, I. C., Serça, D., Hickler, T., Wolf, A., and Smith, B.: Process-based estimates of terrestrial ecosystem isoprene emissions: incorporating the effects of a direct CO2-isoprene interaction, Atmos. Chem. Phys., 7, 31–53,, 2007.
Arneth, A., Schurgers, G., Lathiere, J., Duhl, T., Beerling, D. J., Hewitt, C. N., Martin, M., and Guenther, A.: Global terrestrial isoprene emission models: sensitivity to variability in climate and vegetation, Atmos. Chem. Phys., 11, 8037–8052,, 2011.
Bellouin, N., Rae, J., Jones, A., Johnson, C., Haywood, J., and Boucher, O.: Aerosol forcing in the Climate Model Intercomparison Project (CMIP5) simulations by HadGEM2-ES and the role of ammonium nitrate, J. Geophys. Res.-Atmos., 116, D20206,, 2011.
Short summary
We use modeled estimates of BVOCs from the years 1000 to 2000 to test the effect of anthropogenic BVOC emission changes on SOA formation, aerosol size distributions, and radiative effects using the GEOS-Chem-TOMAS model. Changes of >25% in the number of particles with diameters >80nm are predicted regionally due to extensive land-use changes, leading to increases in combined radiative effect of >0.5 Wm-2. This change in radiative forcing could be an overlooked anthropogenic effect on climate.
Final-revised paper