Articles | Volume 15, issue 5
https://doi.org/10.5194/acp-15-2247-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-2247-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
02 Mar 2015
Research article |
| 02 Mar 2015
Aerosol size distribution and radiative forcing response to anthropogenically driven historical changes in biogenic secondary organic aerosol formation
S. D. D'Andrea
Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
J. C. Acosta Navarro
Department of Applied Environmental Science and Bert Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden
S. C. Farina
Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
C. E. Scott
School of Earth and Environment, University of Leeds, Leeds, UK
School of Earth and Environment, University of Leeds, Leeds, UK
D. K. Farmer
Department of Chemistry, Colorado State University, Fort Collins, CO, USA
D. V. Spracklen
School of Earth and Environment, University of Leeds, Leeds, UK
I. Riipinen
Department of Applied Environmental Science and Bert Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden
Center for Atmospheric Particle Studies, Carnegie Mellon University, Pittsburgh, PA, USA
J. R. Pierce
Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
Department of Physics and Atmospheric Science, Dalhousie University, Halifax, NS, Canada
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Cited
13 citations as recorded by crossref.
- Causes and importance of new particle formation in the present‐day and preindustrial atmospheres H. Gordon et al. 10.1002/2017JD026844
- Assessing the climate benefits of afforestation in the Canadian Northern Boreal and Southern Arctic K. Dsouza et al. 10.1038/s41467-025-56699-9
- Impact of gas-to-particle partitioning approaches on the simulated radiative effects of biogenic secondary organic aerosol C. Scott et al. 10.5194/acp-15-12989-2015
- The Present and Future of Secondary Organic Aerosol Direct Forcing on Climate K. Tsigaridis & M. Kanakidou 10.1007/s40641-018-0092-3
- Re-evaluating the distribution and variation characteristics of haze in China using different distinguishing methods during recent years L. Gao et al. 10.1016/j.scitotenv.2020.138905
- Reviewing the links and feedbacks between climate change and air pollution in Europe U. Im et al. 10.3389/fenvs.2022.954045
- Mechanism of SOA formation determines magnitude of radiative effects J. Zhu et al. 10.1073/pnas.1712273114
- Impact on short-lived climate forcers (SLCFs) from a realistic land-use change scenario via changes in biogenic emissions C. Scott et al. 10.1039/C7FD00028F
- The Tree Drought Emission MONitor (Tree DEMON), an innovative system for assessing biogenic volatile organic compounds emission from plants M. Lüpke et al. 10.1186/s13007-017-0166-6
- Biotic stress accelerates formation of climate-relevant aerosols in boreal forests J. Joutsensaari et al. 10.5194/acp-15-12139-2015
- Impact on short-lived climate forcers increases projected warming due to deforestation C. Scott et al. 10.1038/s41467-017-02412-4
- The aerosol radiative effects of uncontrolled combustion of domestic waste J. Kodros et al. 10.5194/acp-16-6771-2016
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
13 citations as recorded by crossref.
- Causes and importance of new particle formation in the present‐day and preindustrial atmospheres H. Gordon et al. 10.1002/2017JD026844
- Assessing the climate benefits of afforestation in the Canadian Northern Boreal and Southern Arctic K. Dsouza et al. 10.1038/s41467-025-56699-9
- Impact of gas-to-particle partitioning approaches on the simulated radiative effects of biogenic secondary organic aerosol C. Scott et al. 10.5194/acp-15-12989-2015
- The Present and Future of Secondary Organic Aerosol Direct Forcing on Climate K. Tsigaridis & M. Kanakidou 10.1007/s40641-018-0092-3
- Re-evaluating the distribution and variation characteristics of haze in China using different distinguishing methods during recent years L. Gao et al. 10.1016/j.scitotenv.2020.138905
- Reviewing the links and feedbacks between climate change and air pollution in Europe U. Im et al. 10.3389/fenvs.2022.954045
- Mechanism of SOA formation determines magnitude of radiative effects J. Zhu et al. 10.1073/pnas.1712273114
- Impact on short-lived climate forcers (SLCFs) from a realistic land-use change scenario via changes in biogenic emissions C. Scott et al. 10.1039/C7FD00028F
- The Tree Drought Emission MONitor (Tree DEMON), an innovative system for assessing biogenic volatile organic compounds emission from plants M. Lüpke et al. 10.1186/s13007-017-0166-6
- Biotic stress accelerates formation of climate-relevant aerosols in boreal forests J. Joutsensaari et al. 10.5194/acp-15-12139-2015
- Impact on short-lived climate forcers increases projected warming due to deforestation C. Scott et al. 10.1038/s41467-017-02412-4
- The aerosol radiative effects of uncontrolled combustion of domestic waste J. Kodros et al. 10.5194/acp-16-6771-2016
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
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Latest update: 01 Jul 2025
Short summary
We use modeled estimates of BVOCs from the years 1000 to 2000 to test the effect of anthropogenic BVOC emission changes on SOA formation, aerosol size distributions, and radiative effects using the GEOS-Chem-TOMAS model. Changes of >25% in the number of particles with diameters >80nm are predicted regionally due to extensive land-use changes, leading to increases in combined radiative effect of >0.5 Wm-2. This change in radiative forcing could be an overlooked anthropogenic effect on climate.
We use modeled estimates of BVOCs from the years 1000 to 2000 to test the effect of...
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