Articles | Volume 13, issue 7
https://doi.org/10.5194/acp-13-3679-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-3679-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
03 Apr 2013
Research article |
| 03 Apr 2013
CH4 and CO distributions over tropical fires during October 2006 as observed by the Aura TES satellite instrument and modeled by GEOS-Chem
J. Worden
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
K. Wecht
Harvard University, Cambridge, Massachusetts, USA
C. Frankenberg
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
M. Alvarado
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
K. Bowman
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
E. Kort
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
S. Kulawik
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
M. Lee
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
V. Payne
Jet Propulsion Laboratory/California Institute of Technology, Pasadena, California, USA
H. Worden
National Center for Atmospheric Research, Boulder, Colorado, USA
Related authors
John R. Worden, Susan S. Kulawik, Dejian Fu, Vivienne H. Payne, Alan E. Lipton, Igor Polonsky, Yuguang He, Karen Cady-Pereira, Jean-Luc Moncet, Robert L. Herman, Fredrick W. Irion, and Kevin W. Bowman
Atmos. Meas. Tech., 12, 2331–2339, https://doi.org/10.5194/amt-12-2331-2019, https://doi.org/10.5194/amt-12-2331-2019, 2019
Short summary
Short summary
In this paper we take the first steps towards generating a multi-decadal record of the deuterium content of water vapor, useful for evaluating the moisture sources and processes affecting water vapor, by estimating the deuterium content from thermal IR radiances from the AIRS instrument. We find the AIRS-based measurements are sensitive to the deuterium content of water vapor in the middle and lower troposphere with a single measurement uncertainty of ~ 3 % and an accuracy of ~ 0.7 %.
John R. Worden, Gary Doran, Susan Kulawik, Annmarie Eldering, David Crisp, Christian Frankenberg, Chris O'Dell, and Kevin Bowman
Atmos. Meas. Tech., 10, 2759–2771, https://doi.org/10.5194/amt-10-2759-2017, https://doi.org/10.5194/amt-10-2759-2017, 2017
Short summary
Short summary
This paper evaluates the uncertainties of the total column carbon dioxide (XCO2) measurements from the NASA OCO-2 instrument by comparing observed variations in small geographical regions to the calculated uncertainties of the data within this region. In general we find that the reported XCO2 precision is related to that expected from the XCO2 radiance noise. However, the reported accuracy is at least smaller than the actual accuracy by a factor of 2–4.
J. R. Worden, A. J. Turner, A. Bloom, S. S. Kulawik, J. Liu, M. Lee, R. Weidner, K. Bowman, C. Frankenberg, R. Parker, and V. H. Payne
Atmos. Meas. Tech., 8, 3433–3445, https://doi.org/10.5194/amt-8-3433-2015, https://doi.org/10.5194/amt-8-3433-2015, 2015
Short summary
Short summary
Here we demonstrate the potential for estimating lower tropospheric CH4 concentrations through the combination of free-tropospheric methane measurements from the Aura Tropospheric Emission Spectrometer (TES) and XCH4 (dry-mole air fraction of methane) from the Greenhouse Gases Observing Satellite - Thermal And Near-infrared for carbon Observation (GOSAT TANSO).
Joshua L. Laughner, Susan S. Kulawik, and Vivienne H. Payne
EGUsphere, https://doi.org/10.5194/egusphere-2025-2293, https://doi.org/10.5194/egusphere-2025-2293, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
We developed an algorithm to infer peroxyacyl nitrates from an instrument that has been in space for over 20 years. These nitrates can transport pollution significant distances downwind, thus having a long term record of their concentrations can help understand how transport of pollution changed over time. We were able to develop a product for this instrument that produces results compatible with a more recent instrument, allowing them to work together in future analyses.
Hannah Nesser, Kevin W. Bowman, Matthew D. Thill, Daniel J. Varon, Cynthia A. Randles, Ashutosh Tewari, Felipe J. Cardoso-Saldaña, Emily Reidy, Joannes D. Maasakkers, and Daniel J. Jacob
EGUsphere, https://doi.org/10.5194/egusphere-2025-2850, https://doi.org/10.5194/egusphere-2025-2850, 2025
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
Short summary
Short summary
Regional analyses of atmospheric trace gases can improve knowledge of fluxes and their trends at high resolution but rely on the specification of boundary conditions at the domain edges. Biases in the often-uncertain boundary conditions propagate to the inferred fluxes. We develop a framework to explain how errors in the boundary conditions influence the optimized fluxes, derive two metrics to estimate this influence, and compare two methods to correct for the biases.
Lucas A. Estrada, Daniel J. Varon, Melissa Sulprizio, Hannah Nesser, Zichong Chen, Nicholas Balasus, Sarah E. Hancock, Megan He, James D. East, Todd A. Mooring, Alexander Oort Alonso, Joannes D. Maasakkers, Ilse Aben, Sabour Baray, Kevin W. Bowman, John R. Worden, Felipe J. Cardoso-Saldaña, Emily Reidy, and Daniel J. Jacob
Geosci. Model Dev., 18, 3311–3330, https://doi.org/10.5194/gmd-18-3311-2025, https://doi.org/10.5194/gmd-18-3311-2025, 2025
Short summary
Short summary
Reducing emissions of methane, a powerful greenhouse gas, is a top policy concern for mitigating anthropogenic climate change. The Integrated Methane Inversion (IMI) is an advanced, cloud-based software that translates satellite observations into actionable emissions data. Here we present IMI version 2.0 with vastly expanded capabilities. These updates enable a wider range of scientific and stakeholder applications from individual basin to global scales with continuous emissions monitoring.
Raphaël Savelli, Dustin Carroll, Dimitris Menemenlis, Jonathan Lauderdale, Clément Bertin, Stephanie Dutkiewicz, Manfredi Manizza, Anthony Bloom, Karel Castro-Morales, Charles E. Miller, Marc Simard, Kevin W. Bowman, and Hong Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2025-1707, https://doi.org/10.5194/egusphere-2025-1707, 2025
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
Short summary
Short summary
Accounting for carbon and nutrients in rivers is essential for resolving carbon dioxide (CO2) exchanges between the ocean and the atmosphere. In this study, we add the effect of present-day rivers to a pioneering global-ocean biogeochemistry model. This study highlights the challenge for global ocean numerical models to cover the complexity of the flow of water and carbon across the Land-to-Ocean Aquatic Continuum.
Riley Duren, Daniel Cusworth, Alana Ayasse, Kate Howell, Alex Diamond, Tia Scarpelli, Jinsol Kim, Kelly O'neill, Judy Lai-Norling, Andrew Thorpe, Sander R. Zandbergen, Lucas Shaw, Mark Keremedjiev, Jeff Guido, Paul Giuliano, Malkam Goldstein, Ravi Nallapu, Geert Barentsen, David R. Thompson, Keely Roth, Daniel Jensen, Michael Eastwood, Frances Reuland, Taylor Adams, Adam Brandt, Eric A. Kort, James Mason, and Robert O. Green
EGUsphere, https://doi.org/10.5194/egusphere-2025-2275, https://doi.org/10.5194/egusphere-2025-2275, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
We describe the Carbon Mapper emissions monitoring system including methane and carbon dioxide observations from the constellation of Tanager hyperspectral satellites, a global monitoring strategy optimized for enabling mitigation impact at the scale of individual facilities, and a data platform that delivers timely and transparent information for diverse stakeholders. We present early findings from Tanager-1 including the use of our data to locate and repair a leaking oil and gas pipeline.
Rajesh Kumar, Piyush Bhardwaj, Cenlin He, Jennifer Boehnert, Forrest Lacey, Stefano Alessandrini, Kevin Sampson, Matthew Casali, Scott Swerdlin, Olga Wilhelmi, Gabriele G. Pfister, Benjamin Gaubert, and Helen Worden
Earth Syst. Sci. Data, 17, 1807–1834, https://doi.org/10.5194/essd-17-1807-2025, https://doi.org/10.5194/essd-17-1807-2025, 2025
Short summary
Short summary
We have created a 14-year hourly air quality dataset at 12 km resolution by combining satellite observations of atmospheric composition with air quality models over the contiguous United States (CONUS). The dataset has been found to reproduce key observed features of air quality over the CONUS. To enable easy visualization and interpretation of county-level air quality measures and trends by stakeholders, an ArcGIS air quality dashboard has also been developed.
Yu-Wen Chen, K. Sebastian Schmidt, Hong Chen, Steven T. Massie, Susan S. Kulawik, and Hironobu Iwabuchi
Atmos. Meas. Tech., 18, 1859–1884, https://doi.org/10.5194/amt-18-1859-2025, https://doi.org/10.5194/amt-18-1859-2025, 2025
Short summary
Short summary
CO2 column-averaged dry-air mole fractions can be retrieved from space using spectrometers like OCO-2. However, nearby clouds induce spectral distortions that bias these retrievals beyond the accuracy needed for global CO2 source and sink assessments. This study employs a physics-based linearization approach to represent 3D cloud effects and introduces radiance-level mitigation techniques for actual OCO-2 data, enabling the operational implementation of these corrections.
Edward Malina, Jure Brence, Jennifer Adams, Jovan Tanevski, Sašo Džeroski, Valentin Kantchev, and Kevin W. Bowman
Atmos. Meas. Tech., 18, 1689–1715, https://doi.org/10.5194/amt-18-1689-2025, https://doi.org/10.5194/amt-18-1689-2025, 2025
Short summary
Short summary
The large fleet of Earth observation satellites in orbit currently generate huge volumes of data, requiring significant computational resources to process these data in a timely manner. We present a method for predicting poor-quality measurements using machine learning. We find that machine learning methods can accurately predict poor-quality measurements and remove them from the processing chain, saving time and computational resources.
Anne Boynard, Catherine Wespes, Juliette Hadji-Lazaro, Selviga Sinnathamby, Daniel Hurtmans, Pierre-François Coheur, Marie Doutriaux-Boucher, Jacobus Onderwaater, Wolfgang Steinbrecht, Elyse A. Pennington, Kevin Bowman, and Cathy Clerbaux
EGUsphere, https://doi.org/10.5194/egusphere-2025-1054, https://doi.org/10.5194/egusphere-2025-1054, 2025
Short summary
Short summary
This study analyzes 16 years of global ozone data to assess its impact on air quality and climate. Using satellite measurements, we observed a global decrease in tropospheric ozone, particularly in tropical and European regions. The study highlights the importance of long-term data for tracking trends, especially during events like the pandemic. We emphasize the need for improved data processing and integrating multiple datasets to better understand ozone trends.
Mukesh Rai, Kazuyuki Miyazaki, Vivienne Payne, Bin Guan, and Duane Waliser
EGUsphere, https://doi.org/10.5194/egusphere-2025-399, https://doi.org/10.5194/egusphere-2025-399, 2025
Short summary
Short summary
This study introduces a novel method for quantifying extreme events of trace gas air pollutants by leveraging a tropospheric chemical reanalysis data set. The analysis revealed that while extreme events are infrequent, they contribute substantially (60 %) to the total transport of pollutants. This finding underscores the critical role of long-range transport events in determining global and regional air quality.
Takashi Sekiya, Emanuele Emili, Kazuyuki Miyazaki, Antje Inness, Zhen Qu, R. Bradley Pierce, Dylan Jones, Helen Worden, William Y. Y. Cheng, Vincent Huijnen, and Gerbrand Koren
Atmos. Chem. Phys., 25, 2243–2268, https://doi.org/10.5194/acp-25-2243-2025, https://doi.org/10.5194/acp-25-2243-2025, 2025
Short summary
Short summary
Five global chemical reanalysis datasets were used to assess the relative impacts of assimilating satellite ozone and its precursor measurements on tropospheric ozone analyses for 2010. The multiple reanalysis system comparison allows an evaluation of the dependency of the impacts on different reanalysis systems. The results suggested the importance of satellite ozone and its precursor measurements for improving ozone analysis in the whole troposphere, with varying magnitudes among the systems.
Kelley C. Wells, Dylan B. Millet, Jared F. Brewer, Vivienne H. Payne, Karen E. Cady-Pereira, Rick Pernak, Susan Kulawik, Corinne Vigouroux, Nicholas Jones, Emmanuel Mahieu, Maria Makarova, Tomoo Nagahama, Ivan Ortega, Mathias Palm, Kimberly Strong, Matthias Schneider, Dan Smale, Ralf Sussmann, and Minqiang Zhou
Atmos. Meas. Tech., 18, 695–716, https://doi.org/10.5194/amt-18-695-2025, https://doi.org/10.5194/amt-18-695-2025, 2025
Short summary
Short summary
Atmospheric volatile organic compounds (VOCs) affect both air quality and climate. Satellite measurements can help us to assess and predict their global impacts. We present new decadal (2012–2023) measurements of four key VOCs – methanol, ethene, ethyne, and hydrogen cyanide (HCN) – from the Cross-track Infrared Sounder. The measurements reflect emissions from major forests, wildfires, and industry and provide new information to advance understanding of these sources and their changes over time.
Min Huang, Gregory R. Carmichael, Kevin W. Bowman, Isabelle De Smedt, Andreas Colliander, Michael H. Cosh, Sujay V. Kumar, Alex B. Guenther, Scott J. Janz, Ryan M. Stauffer, Anne M. Thompson, Niko M. Fedkin, Robert J. Swap, John D. Bolten, and Alicia T. Joseph
Atmos. Chem. Phys., 25, 1449–1476, https://doi.org/10.5194/acp-25-1449-2025, https://doi.org/10.5194/acp-25-1449-2025, 2025
Short summary
Short summary
We use model simulations along with multiplatform, multidisciplinary observations and a range of analysis methods to estimate and understand the distributions, temporal changes, and impacts of reactive nitrogen and ozone over the most populous US region that has undergone significant environmental changes. Deposition, biogenic emissions, and extra-regional sources have been playing increasingly important roles in controlling pollutant budgets in this area as local anthropogenic emissions drop.
Dylan Jones, Lucas Prates, Zhen Qu, William Cheng, Kazuyuki Miyazaki, Takashi Sekiya, Antje Inness, Rajesh Kumar, Xiao Tang, Helen Worden, Gerbrand Koren, and Vincent Huijen
EGUsphere, https://doi.org/10.5194/egusphere-2024-3759, https://doi.org/10.5194/egusphere-2024-3759, 2025
Short summary
Short summary
We evaluate five chemical reanalysis products to assess their potential to provide useful information on tropospheric ozone variability. We find that the reanalyses produce consistent information on ozone variations in the free troposphere, but have large discrepancies at the surface. The results suggests that improvements in the reanalyses are needed to better exploit the assimilated observations to enhance the utility of the reanalysis products at the surface.
Kazuyuki Miyazaki, Yuliya Marchetti, James Montgomery, Steven Lu, and Kevin Bowman
EGUsphere, https://doi.org/10.5194/egusphere-2024-3753, https://doi.org/10.5194/egusphere-2024-3753, 2025
Short summary
Short summary
This study employs explainable machine learning to analyze the causes of significant biases in surface ozone estimates from chemical reanalysis. By analyzing global observations and chemical reanalysis outputs, key bias drivers such as meteorological conditions and precursor emissions were identified. This provides actionable insights to improve chemical transport models, observation systems, and emissions inventories, ultimately enhancing ozone reanalysis for better air pollution management.
Elyse A. Pennington, Gregory B. Osterman, Vivienne H. Payne, Kazuyuki Miyazaki, Kevin W. Bowman, and Jessica L. Neu
EGUsphere, https://doi.org/10.5194/egusphere-2024-3701, https://doi.org/10.5194/egusphere-2024-3701, 2024
Short summary
Short summary
Tropospheric ozone is a harmful pollutant & powerful greenhouse gas. For satellite products to accurately quantify trends in tropospheric ozone, they must have low bias compared to a reliable source of data. This study compares 3 TROPESS satellite products – CrIS, AIRS, & AIRSOMI – to ozonesonde data. They have low global measurement bias & thus can be used to detect global tropospheric ozone trends, but the measurement bias should be considered in certain regions & time periods.
Bryan N. Duncan, Daniel C. Anderson, Arlene M. Fiore, Joanna Joiner, Nickolay A. Krotkov, Can Li, Dylan B. Millet, Julie M. Nicely, Luke D. Oman, Jason M. St. Clair, Joshua D. Shutter, Amir H. Souri, Sarah A. Strode, Brad Weir, Glenn M. Wolfe, Helen M. Worden, and Qindan Zhu
Atmos. Chem. Phys., 24, 13001–13023, https://doi.org/10.5194/acp-24-13001-2024, https://doi.org/10.5194/acp-24-13001-2024, 2024
Short summary
Short summary
Trace gases emitted to or formed within the atmosphere may be chemically or physically removed from the atmosphere. One trace gas, the hydroxyl radical (OH), is responsible for initiating the chemical removal of many trace gases, including some greenhouse gases. Despite its importance, scientists have not been able to adequately measure OH. In this opinion piece, we discuss promising new methods to indirectly constrain OH using satellite data of trace gases that control the abundance of OH.
Yasin Elshorbany, Jerald R. Ziemke, Sarah Strode, Hervé Petetin, Kazuyuki Miyazaki, Isabelle De Smedt, Kenneth Pickering, Rodrigo J. Seguel, Helen Worden, Tamara Emmerichs, Domenico Taraborrelli, Maria Cazorla, Suvarna Fadnavis, Rebecca R. Buchholz, Benjamin Gaubert, Néstor Y. Rojas, Thiago Nogueira, Thérèse Salameh, and Min Huang
Atmos. Chem. Phys., 24, 12225–12257, https://doi.org/10.5194/acp-24-12225-2024, https://doi.org/10.5194/acp-24-12225-2024, 2024
Short summary
Short summary
We investigated tropospheric ozone spatial variability and trends from 2005 to 2019 and related those to ozone precursors on global and regional scales. We also investigate the spatiotemporal characteristics of the ozone formation regime in relation to ozone chemical sources and sinks. Our analysis is based on remote sensing products of the tropospheric column of ozone and its precursors, nitrogen dioxide, formaldehyde, and total column CO, as well as ozonesonde data and model simulations.
Cynthia D. Nevison, Qing Liang, Paul A. Newman, Britton B. Stephens, Geoff Dutton, Xin Lan, Roisin Commane, Yenny Gonzalez, and Eric Kort
Atmos. Chem. Phys., 24, 10513–10529, https://doi.org/10.5194/acp-24-10513-2024, https://doi.org/10.5194/acp-24-10513-2024, 2024
Short summary
Short summary
This study examines the drivers of interannual variability in tropospheric N2O. New insights are obtained from aircraft data and a chemistry–climate model that explicitly simulates stratospheric N2O. The stratosphere is found to be the dominant driver of N2O variability in the Northern Hemisphere, while both the stratosphere and El Niño cycles are important in the Southern Hemisphere. These results are consistent with known atmospheric dynamics and differences between the hemispheres.
Edward Malina, Kevin W. Bowman, Valentin Kantchev, Le Kuai, Thomas P. Kurosu, Kazuyuki Miyazaki, Vijay Natraj, Gregory B. Osterman, Fabiano Oyafuso, and Matthew D. Thill
Atmos. Meas. Tech., 17, 5341–5371, https://doi.org/10.5194/amt-17-5341-2024, https://doi.org/10.5194/amt-17-5341-2024, 2024
Short summary
Short summary
Characterizing the distribution of ozone in the atmosphere is a challenging problem, with current Earth observation satellites using either thermal infrared (TIR) or ultraviolet (UV) instruments, sensitive to different portions of the atmosphere, making it difficult to gain a full picture. In this work, we combine measurements from the TIR and UV instruments Suomi NPP CrIS and Sentinel-5P/TROPOMI to improve sensitivity through the whole atmosphere and improve knowledge of ozone distribution.
David P. Edwards, Sara Martínez-Alonso, Duseong S. Jo, Ivan Ortega, Louisa K. Emmons, John J. Orlando, Helen M. Worden, Jhoon Kim, Hanlim Lee, Junsung Park, and Hyunkee Hong
Atmos. Chem. Phys., 24, 8943–8961, https://doi.org/10.5194/acp-24-8943-2024, https://doi.org/10.5194/acp-24-8943-2024, 2024
Short summary
Short summary
Until recently, satellite observations of atmospheric pollutants at any location could only be obtained once a day. New geostationary satellites stare at a region of the Earth to make hourly measurements, and the Geostationary Environment Monitoring Spectrometer is the first looking at Asia. These data and model simulations show how the change seen for one important pollutant that determines air quality depends on a combination of pollution emissions, atmospheric chemistry, and meteorology.
Yitong Yao, Philippe Ciais, Emilie Joetzjer, Wei Li, Lei Zhu, Yujie Wang, Christian Frankenberg, and Nicolas Viovy
Earth Syst. Dynam., 15, 763–778, https://doi.org/10.5194/esd-15-763-2024, https://doi.org/10.5194/esd-15-763-2024, 2024
Short summary
Short summary
Elevated CO2 concentration (eCO2) is critical for shaping the future path of forest carbon uptake, while uncertainties remain about concurrent carbon loss. Here, we found that eCO2 might amplify competition-induced carbon loss, while the extent of drought-induced carbon loss hinges on the balance between heightened biomass density and water-saving benefits. This is the first time that such carbon loss responses to ongoing climate change have been quantified separately over the Amazon rainforest.
Juliëtte C. S. Anema, Klaas Folkert Boersma, Piet Stammes, Gerbrand Koren, William Woodgate, Philipp Köhler, Christian Frankenberg, and Jacqui Stol
Biogeosciences, 21, 2297–2311, https://doi.org/10.5194/bg-21-2297-2024, https://doi.org/10.5194/bg-21-2297-2024, 2024
Short summary
Short summary
To keep the Paris agreement goals within reach, negative emissions are necessary. They can be achieved with mitigation techniques, such as reforestation, which remove CO2 from the atmosphere. While governments have pinned their hopes on them, there is not yet a good set of tools to objectively determine whether negative emissions do what they promise. Here we show how satellite measurements of plant fluorescence are useful in detecting carbon uptake due to reforestation and vegetation regrowth.
Ming Luo, Helen M. Worden, Robert D. Field, Kostas Tsigaridis, and Gregory S. Elsaesser
Atmos. Meas. Tech., 17, 2611–2624, https://doi.org/10.5194/amt-17-2611-2024, https://doi.org/10.5194/amt-17-2611-2024, 2024
Short summary
Short summary
The TROPESS CrIS single-pixel CO profile retrievals are compared to the MOPITT CO products in steps of adjusting them to the common a priori assumptions. The two data sets are found to agree within 5 %. We also demonstrated and analyzed the proper steps in evaluating GISS ModelE CO simulations using satellite CO retrieval products for the western US wildfire events in September 2020.
Russell Doughty, Yujie Wang, Jennifer Johnson, Nicholas Parazoo, Troy Magney, Zoe Pierrat, Xiangming Xiao, Luis Guanter, Philipp Köhler, Christian Frankenberg, Peter Somkuti, Shuang Ma, Yuanwei Qin, Sean Crowell, and Berrien Moore III
EGUsphere, https://doi.org/10.22541/essoar.168167172.20799710/v1, https://doi.org/10.22541/essoar.168167172.20799710/v1, 2024
Preprint archived
Short summary
Short summary
Here we present a novel model of global photosynthesis, ChloFluo, which uses spaceborne chlorophyll fluorescence to estimate the amount of photosynthetically active radiation absorbed by chlorophyll. Potential uses of our model are to advance our understanding of the timing and magnitude of photosynthesis, its effect on atmospheric carbon dioxide fluxes, and vegetation response to climate events and change.
Wenfu Tang, Benjamin Gaubert, Louisa Emmons, Daniel Ziskin, Debbie Mao, David Edwards, Avelino Arellano, Kevin Raeder, Jeffrey Anderson, and Helen Worden
Atmos. Meas. Tech., 17, 1941–1963, https://doi.org/10.5194/amt-17-1941-2024, https://doi.org/10.5194/amt-17-1941-2024, 2024
Short summary
Short summary
We assimilate different MOPITT CO products to understand the impact of (1) assimilating multispectral and joint retrievals versus single spectral products, (2) assimilating satellite profile products versus column products, and (3) assimilating multispectral and joint retrievals versus assimilating individual products separately.
Ke Liu, Yujie Wang, Troy S. Magney, and Christian Frankenberg
Biogeosciences, 21, 1501–1516, https://doi.org/10.5194/bg-21-1501-2024, https://doi.org/10.5194/bg-21-1501-2024, 2024
Short summary
Short summary
Stomata are pores on leaves that regulate gas exchange between plants and the atmosphere. Existing land models unrealistically assume stomata can jump between steady states when the environment changes. We implemented dynamic modeling to predict gradual stomatal responses at different scales. Results suggested that considering this effect on plant behavior patterns in diurnal cycles was important. Our framework also simplified simulations and can contribute to further efficiency improvements.
Nicole Jacobs, Christopher W. O'Dell, Thomas E. Taylor, Thomas L. Logan, Brendan Byrne, Matthäus Kiel, Rigel Kivi, Pauli Heikkinen, Aronne Merrelli, Vivienne H. Payne, and Abhishek Chatterjee
Atmos. Meas. Tech., 17, 1375–1401, https://doi.org/10.5194/amt-17-1375-2024, https://doi.org/10.5194/amt-17-1375-2024, 2024
Short summary
Short summary
The accuracy of trace gas retrievals from spaceborne observations, like those from the Orbiting Carbon Observatory 2 (OCO-2), are sensitive to the referenced digital elevation model (DEM). Therefore, we evaluate several global DEMs, used in versions 10 and 11 of the OCO-2 retrieval along with the Copernicus DEM. We explore the impacts of changing the DEM on biases in OCO-2-retrieved XCO2 and inferred CO2 fluxes. Our findings led to an update to OCO-2 v11.1 using the Copernicus DEM globally.
Magdalena Pühl, Anke Roiger, Alina Fiehn, Alan M. Gorchov Negron, Eric A. Kort, Stefan Schwietzke, Ignacio Pisso, Amy Foulds, James Lee, James L. France, Anna E. Jones, Dave Lowry, Rebecca E. Fisher, Langwen Huang, Jacob Shaw, Prudence Bateson, Stephen Andrews, Stuart Young, Pamela Dominutti, Tom Lachlan-Cope, Alexandra Weiss, and Grant Allen
Atmos. Chem. Phys., 24, 1005–1024, https://doi.org/10.5194/acp-24-1005-2024, https://doi.org/10.5194/acp-24-1005-2024, 2024
Short summary
Short summary
In April–May 2019 we carried out an airborne field campaign in the southern North Sea with the aim of studying methane emissions of offshore gas installations. We determined methane emissions from elevated methane measured downstream of the sampled installations. We compare our measured methane emissions with estimated methane emissions from national and global annual inventories. As a result, we find inconsistencies of inventories and large discrepancies between measurements and inventories.
Karen E. Cady-Pereira, Xuehui Guo, Rui Wang, April B. Leytem, Chase Calkins, Elizabeth Berry, Kang Sun, Markus Müller, Armin Wisthaler, Vivienne H. Payne, Mark W. Shephard, Mark A. Zondlo, and Valentin Kantchev
Atmos. Meas. Tech., 17, 15–36, https://doi.org/10.5194/amt-17-15-2024, https://doi.org/10.5194/amt-17-15-2024, 2024
Short summary
Short summary
Ammonia is a significant precursor of PM2.5 particles and thus contributes to poor air quality in many regions. Furthermore, ammonia concentrations are rising due to the increase of large-scale, intensive agricultural activities. Here we evaluate satellite measurements of ammonia against aircraft and surface network data, and show that there are differences in magnitude, but the satellite data are spatially and temporally well correlated with the in situ data.
Wenfu Tang, Louisa K. Emmons, Helen M. Worden, Rajesh Kumar, Cenlin He, Benjamin Gaubert, Zhonghua Zheng, Simone Tilmes, Rebecca R. Buchholz, Sara-Eva Martinez-Alonso, Claire Granier, Antonin Soulie, Kathryn McKain, Bruce C. Daube, Jeff Peischl, Chelsea Thompson, and Pieternel Levelt
Geosci. Model Dev., 16, 6001–6028, https://doi.org/10.5194/gmd-16-6001-2023, https://doi.org/10.5194/gmd-16-6001-2023, 2023
Short summary
Short summary
The new MUSICAv0 model enables the study of atmospheric chemistry across all relevant scales. We develop a MUSICAv0 grid for Africa. We evaluate MUSICAv0 with observations and compare it with a previously used model – WRF-Chem. Overall, the performance of MUSICAv0 is comparable to WRF-Chem. Based on model–satellite discrepancies, we find that future field campaigns in an eastern African region (30°E–45°E, 5°S–5°N) could substantially improve the predictive skill of air quality models.
Drew C. Pendergrass, Daniel J. Jacob, Hannah Nesser, Daniel J. Varon, Melissa Sulprizio, Kazuyuki Miyazaki, and Kevin W. Bowman
Geosci. Model Dev., 16, 4793–4810, https://doi.org/10.5194/gmd-16-4793-2023, https://doi.org/10.5194/gmd-16-4793-2023, 2023
Short summary
Short summary
We have built a tool called CHEEREIO that allows scientists to use observations of pollutants or gases in the atmosphere, such as from satellites or surface stations, to update supercomputer models that simulate the Earth. CHEEREIO uses the difference between the model simulations of the atmosphere and real-world observations to come up with a good guess for the actual composition of our atmosphere, the true emissions of various pollutants, and whatever else they may want to study.
Thomas E. Taylor, Christopher W. O'Dell, David Baker, Carol Bruegge, Albert Chang, Lars Chapsky, Abhishek Chatterjee, Cecilia Cheng, Frédéric Chevallier, David Crisp, Lan Dang, Brian Drouin, Annmarie Eldering, Liang Feng, Brendan Fisher, Dejian Fu, Michael Gunson, Vance Haemmerle, Graziela R. Keller, Matthäus Kiel, Le Kuai, Thomas Kurosu, Alyn Lambert, Joshua Laughner, Richard Lee, Junjie Liu, Lucas Mandrake, Yuliya Marchetti, Gregory McGarragh, Aronne Merrelli, Robert R. Nelson, Greg Osterman, Fabiano Oyafuso, Paul I. Palmer, Vivienne H. Payne, Robert Rosenberg, Peter Somkuti, Gary Spiers, Cathy To, Brad Weir, Paul O. Wennberg, Shanshan Yu, and Jia Zong
Atmos. Meas. Tech., 16, 3173–3209, https://doi.org/10.5194/amt-16-3173-2023, https://doi.org/10.5194/amt-16-3173-2023, 2023
Short summary
Short summary
NASA's Orbiting Carbon Observatory 2 and 3 (OCO-2 and OCO-3, respectively) provide complementary spatiotemporal coverage from a sun-synchronous and precession orbit, respectively. Estimates of total column carbon dioxide (XCO2) derived from the two sensors using the same retrieval algorithm show broad consistency over a 2.5-year overlapping time record. This suggests that data from the two satellites may be used together for scientific analysis.
Emma L. Yates, Laura T. Iraci, Susan S. Kulawik, Ju-Mee Ryoo, Josette E. Marrero, Caroline L. Parworth, Jason M. St. Clair, Thomas F. Hanisco, Thao Paul V. Bui, Cecilia S. Chang, and Jonathan M. Dean-Day
Earth Syst. Sci. Data, 15, 2375–2389, https://doi.org/10.5194/essd-15-2375-2023, https://doi.org/10.5194/essd-15-2375-2023, 2023
Short summary
Short summary
The Alpha Jet Atmospheric eXperiment (AJAX) flew scientific flights between 2011 and 2018 providing measurements of carbon dioxide, methane, ozone, formaldehyde, water vapor and meteorological parameters over California and Nevada, USA. AJAX was a multi-year, multi-objective, multi-instrument program with a variety of sampling strategies resulting in an extensive dataset of interest to a wide variety of users. AJAX measurements have been published at https://asdc.larc.nasa.gov/project/AJAX.
Vincent Humphrey and Christian Frankenberg
Biogeosciences, 20, 1789–1811, https://doi.org/10.5194/bg-20-1789-2023, https://doi.org/10.5194/bg-20-1789-2023, 2023
Short summary
Short summary
Microwave satellites can be used to monitor how vegetation biomass changes over time or how droughts affect the world's forests. However, such satellite data are still difficult to validate and interpret because of a lack of comparable field observations. Here, we present a remote sensing technique that uses the Global Navigation Satellite System (GNSS) as a makeshift radar, making it possible to observe canopy transmissivity at any existing environmental research site in a cost-efficient way.
Brendan Byrne, David F. Baker, Sourish Basu, Michael Bertolacci, Kevin W. Bowman, Dustin Carroll, Abhishek Chatterjee, Frédéric Chevallier, Philippe Ciais, Noel Cressie, David Crisp, Sean Crowell, Feng Deng, Zhu Deng, Nicholas M. Deutscher, Manvendra K. Dubey, Sha Feng, Omaira E. García, David W. T. Griffith, Benedikt Herkommer, Lei Hu, Andrew R. Jacobson, Rajesh Janardanan, Sujong Jeong, Matthew S. Johnson, Dylan B. A. Jones, Rigel Kivi, Junjie Liu, Zhiqiang Liu, Shamil Maksyutov, John B. Miller, Scot M. Miller, Isamu Morino, Justus Notholt, Tomohiro Oda, Christopher W. O'Dell, Young-Suk Oh, Hirofumi Ohyama, Prabir K. Patra, Hélène Peiro, Christof Petri, Sajeev Philip, David F. Pollard, Benjamin Poulter, Marine Remaud, Andrew Schuh, Mahesh K. Sha, Kei Shiomi, Kimberly Strong, Colm Sweeney, Yao Té, Hanqin Tian, Voltaire A. Velazco, Mihalis Vrekoussis, Thorsten Warneke, John R. Worden, Debra Wunch, Yuanzhi Yao, Jeongmin Yun, Andrew Zammit-Mangion, and Ning Zeng
Earth Syst. Sci. Data, 15, 963–1004, https://doi.org/10.5194/essd-15-963-2023, https://doi.org/10.5194/essd-15-963-2023, 2023
Short summary
Short summary
Changes in the carbon stocks of terrestrial ecosystems result in emissions and removals of CO2. These can be driven by anthropogenic activities (e.g., deforestation), natural processes (e.g., fires) or in response to rising CO2 (e.g., CO2 fertilization). This paper describes a dataset of CO2 emissions and removals derived from atmospheric CO2 observations. This pilot dataset informs current capabilities and future developments towards top-down monitoring and verification systems.
Madison J. Shogrin, Vivienne H. Payne, Susan S. Kulawik, Kazuyuki Miyazaki, and Emily V. Fischer
Atmos. Chem. Phys., 23, 2667–2682, https://doi.org/10.5194/acp-23-2667-2023, https://doi.org/10.5194/acp-23-2667-2023, 2023
Short summary
Short summary
We evaluate the spatiotemporal variability of peroxy acyl nitrates (PANs), important photochemical pollutants, over Mexico City using satellite observations. PANs exhibit a seasonal cycle that maximizes in spring. Wildfires contribute to observed interannual variability, and the satellite indicates several areas of frequent outflow. Recent changes in NOx emissions are not accompanied by changes in PANs. This work demonstrates analysis approaches that can be applied to other megacities.
Ali Jalali, Kaley A. Walker, Kimberly Strong, Rebecca R. Buchholz, Merritt N. Deeter, Debra Wunch, Sébastien Roche, Tyler Wizenberg, Erik Lutsch, Erin McGee, Helen M. Worden, Pierre Fogal, and James R. Drummond
Atmos. Meas. Tech., 15, 6837–6863, https://doi.org/10.5194/amt-15-6837-2022, https://doi.org/10.5194/amt-15-6837-2022, 2022
Short summary
Short summary
This study validates MOPITT version 8 carbon monoxide measurements over the Canadian high Arctic for the period 2006 to 2019. The MOPITT products from different detector pixels and channels are compared with ground-based measurements from the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Nunavut, Canada. These results show good consistency between the satellite and ground-based measurements and provide guidance on the usage of these MOPITT data at high latitudes.
Stijn Naus, Lucas G. Domingues, Maarten Krol, Ingrid T. Luijkx, Luciana V. Gatti, John B. Miller, Emanuel Gloor, Sourish Basu, Caio Correia, Gerbrand Koren, Helen M. Worden, Johannes Flemming, Gabrielle Pétron, and Wouter Peters
Atmos. Chem. Phys., 22, 14735–14750, https://doi.org/10.5194/acp-22-14735-2022, https://doi.org/10.5194/acp-22-14735-2022, 2022
Short summary
Short summary
We assimilate MOPITT CO satellite data in the TM5-4D-Var inverse modelling framework to estimate Amazon fire CO emissions for 2003–2018. We show that fire emissions have decreased over the analysis period, coincident with a decrease in deforestation rates. However, interannual variations in fire emissions are large, and they correlate strongly with soil moisture. Our results reveal an important role for robust, top-down fire CO emissions in quantifying and attributing Amazon fire intensity.
Tai-Long He, Dylan B. A. Jones, Kazuyuki Miyazaki, Kevin W. Bowman, Zhe Jiang, Xiaokang Chen, Rui Li, Yuxiang Zhang, and Kunna Li
Atmos. Chem. Phys., 22, 14059–14074, https://doi.org/10.5194/acp-22-14059-2022, https://doi.org/10.5194/acp-22-14059-2022, 2022
Short summary
Short summary
We use a deep-learning (DL) model to estimate Chinese NOx emissions by combining satellite analysis and in situ measurements. Our results are consistent with conventional analyses of Chinese NOx emissions. Comparison with mobility data shows that the DL model has a better capability to capture changes in NOx. We analyse Chinese NOx emissions during the COVID-19 pandemic lockdown period. Our results illustrate the potential use of DL as a complementary tool for conventional air quality studies.
Brendan Byrne, Junjie Liu, Yonghong Yi, Abhishek Chatterjee, Sourish Basu, Rui Cheng, Russell Doughty, Frédéric Chevallier, Kevin W. Bowman, Nicholas C. Parazoo, David Crisp, Xing Li, Jingfeng Xiao, Stephen Sitch, Bertrand Guenet, Feng Deng, Matthew S. Johnson, Sajeev Philip, Patrick C. McGuire, and Charles E. Miller
Biogeosciences, 19, 4779–4799, https://doi.org/10.5194/bg-19-4779-2022, https://doi.org/10.5194/bg-19-4779-2022, 2022
Short summary
Short summary
Plants draw CO2 from the atmosphere during the growing season, while respiration releases CO2 to the atmosphere throughout the year, driving seasonal variations in atmospheric CO2 that can be observed by satellites, such as the Orbiting Carbon Observatory 2 (OCO-2). Using OCO-2 XCO2 data and space-based constraints on plant growth, we show that permafrost-rich northeast Eurasia has a strong seasonal release of CO2 during the autumn, hinting at an unexpectedly large respiration signal from soils.
Yujie Wang and Christian Frankenberg
Biogeosciences, 19, 4705–4714, https://doi.org/10.5194/bg-19-4705-2022, https://doi.org/10.5194/bg-19-4705-2022, 2022
Short summary
Short summary
Plant hydraulics is often misrepresented in topical research. We highlight the commonly seen ambiguities and/or mistakes, with equations and figures to help visualize the potential biases. We recommend careful thinking when using or modifying existing plant hydraulic terms, methods, and models.
Nicole A. June, Anna L. Hodshire, Elizabeth B. Wiggins, Edward L. Winstead, Claire E. Robinson, K. Lee Thornhill, Kevin J. Sanchez, Richard H. Moore, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Matthew M. Coggon, Jonathan M. Dean-Day, T. Paul Bui, Jeff Peischl, Robert J. Yokelson, Matthew J. Alvarado, Sonia M. Kreidenweis, Shantanu H. Jathar, and Jeffrey R. Pierce
Atmos. Chem. Phys., 22, 12803–12825, https://doi.org/10.5194/acp-22-12803-2022, https://doi.org/10.5194/acp-22-12803-2022, 2022
Short summary
Short summary
The evolution of organic aerosol composition and size is uncertain due to variability within and between smoke plumes. We examine the impact of plume concentration on smoke evolution from smoke plumes sampled by the NASA DC-8 during FIREX-AQ. We find that observed organic aerosol and size distribution changes are correlated to plume aerosol mass concentrations. Additionally, coagulation explains the majority of the observed growth.
Helen M. Worden, Gene L. Francis, Susan S. Kulawik, Kevin W. Bowman, Karen Cady-Pereira, Dejian Fu, Jennifer D. Hegarty, Valentin Kantchev, Ming Luo, Vivienne H. Payne, John R. Worden, Róisín Commane, and Kathryn McKain
Atmos. Meas. Tech., 15, 5383–5398, https://doi.org/10.5194/amt-15-5383-2022, https://doi.org/10.5194/amt-15-5383-2022, 2022
Short summary
Short summary
Satellite observations of global carbon monoxide (CO) are essential for understanding atmospheric chemistry and pollution sources. This paper describes a new data product using radiance measurements from the Cross-track Infrared Sounder (CrIS) instrument on the Suomi National Polar-orbiting Partnership (SNPP) satellite that provides vertical profiles of CO from single-field-of-view observations. We show how these satellite CO profiles compare to aircraft observations and evaluate their biases.
Yujie Wang and Christian Frankenberg
Biogeosciences Discuss., https://doi.org/10.5194/bg-2022-172, https://doi.org/10.5194/bg-2022-172, 2022
Revised manuscript not accepted
Short summary
Short summary
Leaf light absorption coefficient is often not measured along with leaf gas exchange, but assumed to be constant. This potentially causes biases in estimated photosynthetic capacity and modeled photosynthetic rates. We explored how leaf light absorption features and light source may impact the photosynthesis modeling, and found that the biases are dependent of model assumptions. Researchers need to be more cautious with these inaccurate assumptions in photosynthesis models.
Sara Martínez-Alonso, Merritt N. Deeter, Bianca C. Baier, Kathryn McKain, Helen Worden, Tobias Borsdorff, Colm Sweeney, and Ilse Aben
Atmos. Meas. Tech., 15, 4751–4765, https://doi.org/10.5194/amt-15-4751-2022, https://doi.org/10.5194/amt-15-4751-2022, 2022
Short summary
Short summary
AirCore is a novel balloon sampling system that can measure, among others, vertical profiles of carbon monoxide (CO) from 25–30 km of altitude to near the surface. Our analyses of AirCore and satellite CO data show that AirCore profiles are suited for satellite data validation, the use of shorter aircraft vertical profiles in satellite validation results in small errors (1–3 percent points) mostly at 300 hPa and above, and the error introduced by clouds in TROPOMI land data is small (1–2 %).
Daniel J. Jacob, Daniel J. Varon, Daniel H. Cusworth, Philip E. Dennison, Christian Frankenberg, Ritesh Gautam, Luis Guanter, John Kelley, Jason McKeever, Lesley E. Ott, Benjamin Poulter, Zhen Qu, Andrew K. Thorpe, John R. Worden, and Riley M. Duren
Atmos. Chem. Phys., 22, 9617–9646, https://doi.org/10.5194/acp-22-9617-2022, https://doi.org/10.5194/acp-22-9617-2022, 2022
Short summary
Short summary
We review the capability of satellite observations of atmospheric methane to quantify methane emissions on all scales. We cover retrieval methods, precision requirements, inverse methods for inferring emissions, source detection thresholds, and observations of system completeness. We show that current instruments already enable quantification of regional and national emissions including contributions from large point sources. Coverage and resolution will increase significantly in coming years.
Vivienne H. Payne, Susan S. Kulawik, Emily V. Fischer, Jared F. Brewer, L. Gregory Huey, Kazuyuki Miyazaki, John R. Worden, Kevin W. Bowman, Eric J. Hintsa, Fred Moore, James W. Elkins, and Julieta Juncosa Calahorrano
Atmos. Meas. Tech., 15, 3497–3511, https://doi.org/10.5194/amt-15-3497-2022, https://doi.org/10.5194/amt-15-3497-2022, 2022
Short summary
Short summary
We compare new satellite measurements of peroxyacetyl nitrate (PAN) with reference aircraft measurements from two different instruments flown on the same platform. While there is a systematic difference between the two aircraft datasets, both show the same large-scale distribution of PAN and the discrepancy between aircraft datasets is small compared to the satellite uncertainties. The satellite measurements show skill in capturing large-scale variations in PAN.
Min Huang, James H. Crawford, Gregory R. Carmichael, Kevin W. Bowman, Sujay V. Kumar, and Colm Sweeney
Atmos. Chem. Phys., 22, 7461–7487, https://doi.org/10.5194/acp-22-7461-2022, https://doi.org/10.5194/acp-22-7461-2022, 2022
Short summary
Short summary
This study demonstrates that ozone dry-deposition modeling can be improved by revising the model's dry-deposition parameterizations to better represent the effects of environmental conditions including the soil moisture fields. Applying satellite soil moisture data assimilation is shown to also have added value. Such advancements in coupled modeling and data assimilation can benefit the assessments of ozone impacts on human and vegetation health.
Dustin Roten, John C. Lin, Lewis Kunik, Derek Mallia, Dien Wu, Tomohiro Oda, and Eric A. Kort
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-315, https://doi.org/10.5194/acp-2022-315, 2022
Revised manuscript not accepted
Short summary
Short summary
The systems used to monitor carbon dioxide (CO2) emissions from urban areas provides a means to observe and quantify emissions reductions from policy-related reduction efforts. Space-based instruments, such as NASA's Orbiting Carbon Observatory-3 (OCO-3), provides detailed "snapshots" of CO2 emissions from many megacities around the world. This work quantifies the amount of emission "information" contained in these snapshots and uses this information to update previous estimates of urban CO2.
Merritt Deeter, Gene Francis, John Gille, Debbie Mao, Sara Martínez-Alonso, Helen Worden, Dan Ziskin, James Drummond, Róisín Commane, Glenn Diskin, and Kathryn McKain
Atmos. Meas. Tech., 15, 2325–2344, https://doi.org/10.5194/amt-15-2325-2022, https://doi.org/10.5194/amt-15-2325-2022, 2022
Short summary
Short summary
The MOPITT (Measurements of Pollution in the Troposphere) satellite instrument uses remote sensing to obtain retrievals (measurements) of carbon monoxide (CO) in the atmosphere. This paper describes the latest MOPITT data product, Version 9. Globally, the number of daytime MOPITT retrievals over land has increased by 30 %–40 % compared to the previous product. The reported improvements in the MOPITT product should benefit a wide variety of applications including studies of pollution sources.
Russell Doughty, Thomas P. Kurosu, Nicholas Parazoo, Philipp Köhler, Yujie Wang, Ying Sun, and Christian Frankenberg
Earth Syst. Sci. Data, 14, 1513–1529, https://doi.org/10.5194/essd-14-1513-2022, https://doi.org/10.5194/essd-14-1513-2022, 2022
Short summary
Short summary
We describe and compare solar-induced chlorophyll fluorescence data produced by NASA from the Greenhouse Gases Observing Satellite (GOSAT) and the Orbiting Carbon Observatory-2 (OCO-2) and OCO-3 platforms.
Johannes Gensheimer, Alexander J. Turner, Philipp Köhler, Christian Frankenberg, and Jia Chen
Biogeosciences, 19, 1777–1793, https://doi.org/10.5194/bg-19-1777-2022, https://doi.org/10.5194/bg-19-1777-2022, 2022
Short summary
Short summary
We develop a convolutional neural network, named SIFnet, that increases the spatial resolution of SIF from TROPOMI by a factor of 10 to a spatial resolution of 0.005°. SIFnet utilizes coarse SIF observations, together with a broad range of high-resolution auxiliary data. The insights gained from interpretable machine learning techniques allow us to make quantitative claims about the relationships between SIF and other common parameters related to photosynthesis.
Vijay Natraj, Ming Luo, Jean-Francois Blavier, Vivienne H. Payne, Derek J. Posselt, Stanley P. Sander, Zhao-Cheng Zeng, Jessica L. Neu, Denis Tremblay, Longtao Wu, Jacola A. Roman, Yen-Hung Wu, and Leonard I. Dorsky
Atmos. Meas. Tech., 15, 1251–1267, https://doi.org/10.5194/amt-15-1251-2022, https://doi.org/10.5194/amt-15-1251-2022, 2022
Short summary
Short summary
High-fidelity monitoring and forecast of air quality and the hydrological cycle require understanding the vertical distribution of temperature, humidity, and trace gases at high spatiotemporal resolution. We describe a new instrument concept, called the JPL GEO-IR Sounder, that would provide this information for the first time from a single instrument platform. Simulations demonstrate the benefits of combining measurements from multiple wavelengths for this purpose from geostationary orbit.
Heba S. Marey, James R. Drummond, Dylan B. A. Jones, Helen Worden, Merritt N. Deeter, John Gille, and Debbie Mao
Atmos. Meas. Tech., 15, 701–719, https://doi.org/10.5194/amt-15-701-2022, https://doi.org/10.5194/amt-15-701-2022, 2022
Short summary
Short summary
In this study, an analysis has been performed to understand the improvements in observational coverage over Canada in the new MOPITT V9 product. Temporal and spatial analysis of V9 indicates a general coverage gain of 15–20 % relative to V8, which varies regionally and seasonally; e.g., the number of successful MOPITT retrievals in V9 was doubled over Canada in winter. Also, comparison with the corresponding IASI instrument indicated generally good agreement, with about a 5–10 % positive bias.
Jennifer D. Hegarty, Karen E. Cady-Pereira, Vivienne H. Payne, Susan S. Kulawik, John R. Worden, Valentin Kantchev, Helen M. Worden, Kathryn McKain, Jasna V. Pittman, Róisín Commane, Bruce C. Daube Jr., and Eric A. Kort
Atmos. Meas. Tech., 15, 205–223, https://doi.org/10.5194/amt-15-205-2022, https://doi.org/10.5194/amt-15-205-2022, 2022
Short summary
Short summary
Carbon monoxide (CO) is produced by combustion of substances such as fossil fuels and plays an important role in atmospheric pollution and climate. We evaluated estimates of atmospheric CO derived from outgoing radiation measurements of the Atmospheric Infrared Sounder (AIRS) on a satellite orbiting the Earth against CO measurements from aircraft to show that these satellite measurements are reliable for continuous global monitoring of atmospheric CO concentrations.
Yujie Wang and Christian Frankenberg
Biogeosciences, 19, 29–45, https://doi.org/10.5194/bg-19-29-2022, https://doi.org/10.5194/bg-19-29-2022, 2022
Short summary
Short summary
Modeling vegetation canopy is important in predicting whether the land remains a carbon sink to mitigate climate change in the near future. Vegetation canopy model complexity, however, impacts the model-predicted carbon and water fluxes as well as canopy fluorescence, even if the same suite of model inputs is used. Given the biases caused by canopy model complexity, we recommend not misusing parameters inverted using different models or assumptions.
Alexander J. Turner, Philipp Köhler, Troy S. Magney, Christian Frankenberg, Inez Fung, and Ronald C. Cohen
Biogeosciences, 18, 6579–6588, https://doi.org/10.5194/bg-18-6579-2021, https://doi.org/10.5194/bg-18-6579-2021, 2021
Short summary
Short summary
This work builds a high-resolution estimate (500 m) of gross primary productivity (GPP) over the US using satellite measurements of solar-induced chlorophyll fluorescence (SIF) from the TROPOspheric Monitoring Instrument (TROPOMI) between 2018 and 2020. We identify ecosystem-specific scaling factors for estimating gross primary productivity (GPP) from TROPOMI SIF. Extreme precipitation events drive four regional GPP anomalies that account for 28 % of year-to-year GPP differences across the US.
Siraput Jongaramrungruang, Georgios Matheou, Andrew K. Thorpe, Zhao-Cheng Zeng, and Christian Frankenberg
Atmos. Meas. Tech., 14, 7999–8017, https://doi.org/10.5194/amt-14-7999-2021, https://doi.org/10.5194/amt-14-7999-2021, 2021
Short summary
Short summary
This study shows how precision error and bias in column methane retrieval change with different instrument specifications and the impact of spectrally complex surface albedos on retrievals. We show how surface interferences can be mitigated with an optimal spectral resolution and a higher polynomial degree in a retrieval process. The findings can inform future satellite instrument designs to have robust observations capable of separating real CH4 plume enhancements from surface interferences.
Luis Guanter, Cédric Bacour, Andreas Schneider, Ilse Aben, Tim A. van Kempen, Fabienne Maignan, Christian Retscher, Philipp Köhler, Christian Frankenberg, Joanna Joiner, and Yongguang Zhang
Earth Syst. Sci. Data, 13, 5423–5440, https://doi.org/10.5194/essd-13-5423-2021, https://doi.org/10.5194/essd-13-5423-2021, 2021
Short summary
Short summary
Sun-induced chlorophyll fluorescence (SIF) is an electromagnetic signal emitted by plants in the red and far-red parts of the spectrum. It has a functional link to photosynthesis and can be measured by satellite instruments, which makes it an important variable for the remote monitoring of the photosynthetic activity of vegetation ecosystems around the world. In this contribution we present a SIF dataset derived from the new Sentinel-5P TROPOMI missions.
Yujie Wang, Philipp Köhler, Liyin He, Russell Doughty, Renato K. Braghiere, Jeffrey D. Wood, and Christian Frankenberg
Geosci. Model Dev., 14, 6741–6763, https://doi.org/10.5194/gmd-14-6741-2021, https://doi.org/10.5194/gmd-14-6741-2021, 2021
Short summary
Short summary
We present the first step in testing a new land model as part of a new Earth system model. Our model links plant hydraulics, stomatal optimization theory, and a comprehensive canopy radiation scheme. We compared model-predicted carbon and water fluxes to flux tower observations and model-predicted sun-induced chlorophyll fluorescence to satellite retrievals. Our model quantitatively predicted the carbon and water fluxes as well as the canopy fluorescence yield.
Eric J. Hintsa, Fred L. Moore, Dale F. Hurst, Geoff S. Dutton, Bradley D. Hall, J. David Nance, Ben R. Miller, Stephen A. Montzka, Laura P. Wolton, Audra McClure-Begley, James W. Elkins, Emrys G. Hall, Allen F. Jordan, Andrew W. Rollins, Troy D. Thornberry, Laurel A. Watts, Chelsea R. Thompson, Jeff Peischl, Ilann Bourgeois, Thomas B. Ryerson, Bruce C. Daube, Yenny Gonzalez Ramos, Roisin Commane, Gregory W. Santoni, Jasna V. Pittman, Steven C. Wofsy, Eric Kort, Glenn S. Diskin, and T. Paul Bui
Atmos. Meas. Tech., 14, 6795–6819, https://doi.org/10.5194/amt-14-6795-2021, https://doi.org/10.5194/amt-14-6795-2021, 2021
Short summary
Short summary
We built UCATS to study atmospheric chemistry and transport. It has measured trace gases including CFCs, N2O, SF6, CH4, CO, and H2 with gas chromatography, as well as ozone and water vapor. UCATS has been part of missions to study the tropical tropopause; transport of air into the stratosphere; greenhouse gases, transport, and chemistry in the troposphere; and ozone chemistry, on both piloted and unmanned aircraft. Its design, capabilities, and some results are shown and described here.
Yi Yin, Frederic Chevallier, Philippe Ciais, Philippe Bousquet, Marielle Saunois, Bo Zheng, John Worden, A. Anthony Bloom, Robert J. Parker, Daniel J. Jacob, Edward J. Dlugokencky, and Christian Frankenberg
Atmos. Chem. Phys., 21, 12631–12647, https://doi.org/10.5194/acp-21-12631-2021, https://doi.org/10.5194/acp-21-12631-2021, 2021
Short summary
Short summary
The growth of methane, the second-most important anthropogenic greenhouse gas after carbon dioxide, has been accelerating in recent years. Using an ensemble of multi-tracer atmospheric inversions constrained by surface or satellite observations, we show that global methane emissions increased by nearly 1 % per year from 2010–2017, with leading contributions from the tropics and East Asia.
Min Huang, James H. Crawford, Joshua P. DiGangi, Gregory R. Carmichael, Kevin W. Bowman, Sujay V. Kumar, and Xiwu Zhan
Atmos. Chem. Phys., 21, 11013–11040, https://doi.org/10.5194/acp-21-11013-2021, https://doi.org/10.5194/acp-21-11013-2021, 2021
Short summary
Short summary
This study evaluates the impact of satellite soil moisture data assimilation on modeled weather and ozone fields at various altitudes above the southeastern US during the summer. It emphasizes the importance of soil moisture in the understanding of surface ozone pollution and upper tropospheric chemistry, as well as air pollutants’ source–receptor relationships between the US and its downwind areas.
Wenfu Tang, David P. Edwards, Louisa K. Emmons, Helen M. Worden, Laura M. Judd, Lok N. Lamsal, Jassim A. Al-Saadi, Scott J. Janz, James H. Crawford, Merritt N. Deeter, Gabriele Pfister, Rebecca R. Buchholz, Benjamin Gaubert, and Caroline R. Nowlan
Atmos. Meas. Tech., 14, 4639–4655, https://doi.org/10.5194/amt-14-4639-2021, https://doi.org/10.5194/amt-14-4639-2021, 2021
Short summary
Short summary
We use high-resolution airborne mapping spectrometer measurements to assess sub-grid variability within satellite pixels over urban regions. The sub-grid variability within satellite pixels increases with increasing satellite pixel sizes. Temporal variability within satellite pixels decreases with increasing satellite pixel sizes. This work is particularly relevant and useful for future satellite design, satellite data interpretation, and point-grid data comparisons.
Dien Wu, John C. Lin, Henrique F. Duarte, Vineet Yadav, Nicholas C. Parazoo, Tomohiro Oda, and Eric A. Kort
Geosci. Model Dev., 14, 3633–3661, https://doi.org/10.5194/gmd-14-3633-2021, https://doi.org/10.5194/gmd-14-3633-2021, 2021
Short summary
Short summary
A model (SMUrF) is presented that estimates biogenic CO2 fluxes over cities around the globe to separate out biogenic fluxes from anthropogenic emissions. The model leverages satellite-based solar-induced fluorescence data and a machine-learning technique. We evaluate the biogenic fluxes against flux observations and show contrasts between biogenic and anthropogenic fluxes over cities, revealing urban–rural flux gradients, diurnal cycles, and the resulting imprints on atmospheric-column CO2.
Zhe Jiang, Hongrong Shi, Bin Zhao, Yu Gu, Yifang Zhu, Kazuyuki Miyazaki, Xin Lu, Yuqiang Zhang, Kevin W. Bowman, Takashi Sekiya, and Kuo-Nan Liou
Atmos. Chem. Phys., 21, 8693–8708, https://doi.org/10.5194/acp-21-8693-2021, https://doi.org/10.5194/acp-21-8693-2021, 2021
Short summary
Short summary
We use the COVID-19 pandemic as a unique natural experiment to obtain a more robust understanding of the effectiveness of emission reductions toward air quality improvement by combining chemical transport simulations and observations. Our findings imply a shift from current control policies in California: a strengthened control on primary PM2.5 emissions and a well-balanced control on NOx and volatile organic compounds are needed to effectively and sustainably alleviate PM2.5 and O3 pollution.
Anna L. Hodshire, Emily Ramnarine, Ali Akherati, Matthew L. Alvarado, Delphine K. Farmer, Shantanu H. Jathar, Sonia M. Kreidenweis, Chantelle R. Lonsdale, Timothy B. Onasch, Stephen R. Springston, Jian Wang, Yang Wang, Lawrence I. Kleinman, Arthur J. Sedlacek III, and Jeffrey R. Pierce
Atmos. Chem. Phys., 21, 6839–6855, https://doi.org/10.5194/acp-21-6839-2021, https://doi.org/10.5194/acp-21-6839-2021, 2021
Short summary
Short summary
Biomass burning emits particles and vapors that can impact both health and climate. Here, we investigate the role of dilution in the evolution of aerosol size and composition in observed US wildfire smoke plumes. Centers of plumes dilute more slowly than edges. We see differences in concentrations and composition between the centers and edges both in the first measurement and in subsequent measurements. Our findings support the hypothesis that plume dilution influences smoke aging.
David R. Lyon, Benjamin Hmiel, Ritesh Gautam, Mark Omara, Katherine A. Roberts, Zachary R. Barkley, Kenneth J. Davis, Natasha L. Miles, Vanessa C. Monteiro, Scott J. Richardson, Stephen Conley, Mackenzie L. Smith, Daniel J. Jacob, Lu Shen, Daniel J. Varon, Aijun Deng, Xander Rudelis, Nikhil Sharma, Kyle T. Story, Adam R. Brandt, Mary Kang, Eric A. Kort, Anthony J. Marchese, and Steven P. Hamburg
Atmos. Chem. Phys., 21, 6605–6626, https://doi.org/10.5194/acp-21-6605-2021, https://doi.org/10.5194/acp-21-6605-2021, 2021
Short summary
Short summary
The Permian Basin (USA) is the world’s largest oil field. We use tower- and aircraft-based approaches to measure how methane emissions in the Permian Basin changed throughout 2020. In early 2020, 3.3 % of the region’s gas was emitted; then in spring 2020, the loss rate temporarily dropped to 1.9 % as oil price crashed. We find this short-term reduction to be a result of reduced well development, less gas flaring, and fewer abnormal events despite minimal reductions in oil and gas production.
Joannes D. Maasakkers, Daniel J. Jacob, Melissa P. Sulprizio, Tia R. Scarpelli, Hannah Nesser, Jianxiong Sheng, Yuzhong Zhang, Xiao Lu, A. Anthony Bloom, Kevin W. Bowman, John R. Worden, and Robert J. Parker
Atmos. Chem. Phys., 21, 4339–4356, https://doi.org/10.5194/acp-21-4339-2021, https://doi.org/10.5194/acp-21-4339-2021, 2021
Short summary
Short summary
We use 2010–2015 GOSAT satellite observations of atmospheric methane over North America in a high-resolution inversion to estimate methane emissions. We find general consistency with the gridded EPA inventory but higher oil and gas production emissions, with oil production emissions twice as large as in the latest EPA Greenhouse Gas Inventory. We find lower wetland emissions than predicted by WetCHARTs and a small increasing trend in the eastern US, apparently related to unconventional oil/gas.
Jakob Borchardt, Konstantin Gerilowski, Sven Krautwurst, Heinrich Bovensmann, Andrew K. Thorpe, David R. Thompson, Christian Frankenberg, Charles E. Miller, Riley M. Duren, and John Philip Burrows
Atmos. Meas. Tech., 14, 1267–1291, https://doi.org/10.5194/amt-14-1267-2021, https://doi.org/10.5194/amt-14-1267-2021, 2021
Short summary
Short summary
The AVIRIS-NG hyperspectral imager has been used successfully to identify and quantify anthropogenic methane sources utilizing different retrieval and inversion methods. Here, we examine the adaption and application of the WFM-DOAS algorithm to AVIRIS-NG measurements to retrieve local methane column enhancements, compare the results with other retrievals, and quantify the uncertainties resulting from the retrieval method. Additionally, we estimate emissions from five detected methane plumes.
Junjie Liu, Latha Baskaran, Kevin Bowman, David Schimel, A. Anthony Bloom, Nicholas C. Parazoo, Tomohiro Oda, Dustin Carroll, Dimitris Menemenlis, Joanna Joiner, Roisin Commane, Bruce Daube, Lucianna V. Gatti, Kathryn McKain, John Miller, Britton B. Stephens, Colm Sweeney, and Steven Wofsy
Earth Syst. Sci. Data, 13, 299–330, https://doi.org/10.5194/essd-13-299-2021, https://doi.org/10.5194/essd-13-299-2021, 2021
Short summary
Short summary
On average, the terrestrial biosphere carbon sink is equivalent to ~ 20 % of fossil fuel emissions. Understanding where and why the terrestrial biosphere absorbs carbon from the atmosphere is pivotal to any mitigation policy. Here we present a regionally resolved satellite-constrained net biosphere exchange (NBE) dataset with corresponding uncertainties between 2010–2018: CMS-Flux NBE 2020. The dataset provides a unique perspective on monitoring regional contributions to the CO2 growth rate.
Xueying Yu, Dylan B. Millet, Kelley C. Wells, Daven K. Henze, Hansen Cao, Timothy J. Griffis, Eric A. Kort, Genevieve Plant, Malte J. Deventer, Randall K. Kolka, D. Tyler Roman, Kenneth J. Davis, Ankur R. Desai, Bianca C. Baier, Kathryn McKain, Alan C. Czarnetzki, and A. Anthony Bloom
Atmos. Chem. Phys., 21, 951–971, https://doi.org/10.5194/acp-21-951-2021, https://doi.org/10.5194/acp-21-951-2021, 2021
Short summary
Short summary
Methane concentrations have doubled since 1750. The US Upper Midwest is a key region contributing to such trends, but sources are poorly understood. We collected and analyzed aircraft data to resolve spatial and timing biases in wetland and livestock emission estimates and uncover errors in inventory treatment of manure management. We highlight the importance of intensive agriculture for the regional and US methane budgets and the potential for methane mitigation through improved management.
Susan S. Kulawik, John R. Worden, Vivienne H. Payne, Dejian Fu, Steven C. Wofsy, Kathryn McKain, Colm Sweeney, Bruce C. Daube Jr., Alan Lipton, Igor Polonsky, Yuguang He, Karen E. Cady-Pereira, Edward J. Dlugokencky, Daniel J. Jacob, and Yi Yin
Atmos. Meas. Tech., 14, 335–354, https://doi.org/10.5194/amt-14-335-2021, https://doi.org/10.5194/amt-14-335-2021, 2021
Short summary
Short summary
This paper shows comparisons of a new single-footprint methane product from the AIRS satellite to aircraft-based observations. We show that this AIRS methane product provides useful information to study seasonal and global methane trends of this important greenhouse gas.
A. Anthony Bloom, Kevin W. Bowman, Junjie Liu, Alexandra G. Konings, John R. Worden, Nicholas C. Parazoo, Victoria Meyer, John T. Reager, Helen M. Worden, Zhe Jiang, Gregory R. Quetin, T. Luke Smallman, Jean-François Exbrayat, Yi Yin, Sassan S. Saatchi, Mathew Williams, and David S. Schimel
Biogeosciences, 17, 6393–6422, https://doi.org/10.5194/bg-17-6393-2020, https://doi.org/10.5194/bg-17-6393-2020, 2020
Short summary
Short summary
We use a model of the 2001–2015 tropical land carbon cycle, with satellite measurements of land and atmospheric carbon, to disentangle lagged and concurrent effects (due to past and concurrent meteorological events, respectively) on annual land–atmosphere carbon exchanges. The variability of lagged effects explains most 2001–2015 inter-annual carbon flux variations. We conclude that concurrent and lagged effects need to be accurately resolved to better predict the world's land carbon sink.
Benjamin Gaubert, Louisa K. Emmons, Kevin Raeder, Simone Tilmes, Kazuyuki Miyazaki, Avelino F. Arellano Jr., Nellie Elguindi, Claire Granier, Wenfu Tang, Jérôme Barré, Helen M. Worden, Rebecca R. Buchholz, David P. Edwards, Philipp Franke, Jeffrey L. Anderson, Marielle Saunois, Jason Schroeder, Jung-Hun Woo, Isobel J. Simpson, Donald R. Blake, Simone Meinardi, Paul O. Wennberg, John Crounse, Alex Teng, Michelle Kim, Russell R. Dickerson, Hao He, Xinrong Ren, Sally E. Pusede, and Glenn S. Diskin
Atmos. Chem. Phys., 20, 14617–14647, https://doi.org/10.5194/acp-20-14617-2020, https://doi.org/10.5194/acp-20-14617-2020, 2020
Short summary
Short summary
This study investigates carbon monoxide pollution in East Asia during spring using a numerical model, satellite remote sensing, and aircraft measurements. We found an underestimation of emission sources. Correcting the emission bias can improve air quality forecasting of carbon monoxide and other species including ozone. Results also suggest that controlling VOC and CO emissions, in addition to widespread NOx controls, can improve ozone pollution over East Asia.
Chantelle R. Lonsdale, Matthew J. Alvarado, Anna L. Hodshire, Emily Ramnarine, and Jeffrey R. Pierce
Geosci. Model Dev., 13, 4579–4593, https://doi.org/10.5194/gmd-13-4579-2020, https://doi.org/10.5194/gmd-13-4579-2020, 2020
Short summary
Short summary
The System for Atmospheric Modelling (SAM) has been coupled with the detailed gas/aerosol chemistry model, the Aerosol Simulation Program (ASP), to capture cross-plume concentration gradients as fire plumes evolve downwind. SAM-ASP v1.0 will lead to the development of parameterizations of near-source biomass burning chemistry that can be used to more accurately simulate biomass burning chemical and physical transformations of trace gases and aerosols within coarser chemical transport models.
Kazuyuki Miyazaki, Kevin Bowman, Takashi Sekiya, Henk Eskes, Folkert Boersma, Helen Worden, Nathaniel Livesey, Vivienne H. Payne, Kengo Sudo, Yugo Kanaya, Masayuki Takigawa, and Koji Ogochi
Earth Syst. Sci. Data, 12, 2223–2259, https://doi.org/10.5194/essd-12-2223-2020, https://doi.org/10.5194/essd-12-2223-2020, 2020
Short summary
Short summary
This study presents the results from the Tropospheric Chemistry Reanalysis version 2 (TCR-2) for 2005–2018 obtained from the assimilation of multiple satellite measurements of ozone, CO, NO2, HNO3, and SO2 from the OMI, SCIAMACHY, GOME-2, TES, MLS, and MOPITT instruments. The evaluation results demonstrate the capability of the reanalysis products to improve understanding of the processes controlling variations in atmospheric composition, including long-term changes in air quality and emissions.
Rui Cheng, Troy S. Magney, Debsunder Dutta, David R. Bowling, Barry A. Logan, Sean P. Burns, Peter D. Blanken, Katja Grossmann, Sophia Lopez, Andrew D. Richardson, Jochen Stutz, and Christian Frankenberg
Biogeosciences, 17, 4523–4544, https://doi.org/10.5194/bg-17-4523-2020, https://doi.org/10.5194/bg-17-4523-2020, 2020
Short summary
Short summary
We measured reflected sunlight from an evergreen canopy for a year to detect changes in pigments that play an important role in regulating the seasonality of photosynthesis. Results show a strong mechanistic link between spectral reflectance features and pigment content, which is validated using a biophysical model. Our results show spectrally where, why, and when spectral features change over the course of the season and show promise for estimating photosynthesis remotely.
Sara Martínez-Alonso, Merritt Deeter, Helen Worden, Tobias Borsdorff, Ilse Aben, Róisin Commane, Bruce Daube, Gene Francis, Maya George, Jochen Landgraf, Debbie Mao, Kathryn McKain, and Steven Wofsy
Atmos. Meas. Tech., 13, 4841–4864, https://doi.org/10.5194/amt-13-4841-2020, https://doi.org/10.5194/amt-13-4841-2020, 2020
Short summary
Short summary
CO is of great importance in climate and air quality studies. To understand newly available TROPOMI data in the frame of the global CO record, we compared those to satellite (MOPITT) and airborne (ATom) CO datasets. The MOPITT dataset is the longest to date (2000–present) and is well-characterized. We used ATom to validate cloudy TROPOMI data over oceans and investigate TROPOMI's vertical sensitivity to CO. Our results show that TROPOMI CO data are in excellent agreement with the other datasets.
Wenfu Tang, Benjamin Gaubert, Louisa Emmons, Yonghoon Choi, Joshua P. DiGangi, Glenn S. Diskin, Xiaomei Xu, Cenlin He, Helen Worden, Simone Tilmes, Rebecca Buchholz, Hannah S. Halliday, and Avelino F. Arellano
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-864, https://doi.org/10.5194/acp-2020-864, 2020
Revised manuscript not accepted
Short summary
Short summary
A specific demonstration of the potential use of correlative information from carbon monoxide to refine estimates of regional carbon dioxide emissions from fossil fuel combustion.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
Short summary
Short summary
Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Nicholas C. Parazoo, Troy Magney, Alex Norton, Brett Raczka, Cédric Bacour, Fabienne Maignan, Ian Baker, Yongguang Zhang, Bo Qiu, Mingjie Shi, Natasha MacBean, Dave R. Bowling, Sean P. Burns, Peter D. Blanken, Jochen Stutz, Katja Grossmann, and Christian Frankenberg
Biogeosciences, 17, 3733–3755, https://doi.org/10.5194/bg-17-3733-2020, https://doi.org/10.5194/bg-17-3733-2020, 2020
Short summary
Short summary
Satellite measurements of solar-induced chlorophyll fluorescence (SIF) provide a global measure of photosynthetic change. This enables scientists to better track carbon cycle responses to environmental change and tune biochemical processes in vegetation models for an improved simulation of future change. We use tower-instrumented SIF measurements and controlled model experiments to assess the state of the art in terrestrial biosphere SIF modeling and find a wide range of sensitivities to light.
Marielle Saunois, Ann R. Stavert, Ben Poulter, Philippe Bousquet, Josep G. Canadell, Robert B. Jackson, Peter A. Raymond, Edward J. Dlugokencky, Sander Houweling, Prabir K. Patra, Philippe Ciais, Vivek K. Arora, David Bastviken, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Kimberly M. Carlson, Mark Carrol, Simona Castaldi, Naveen Chandra, Cyril Crevoisier, Patrick M. Crill, Kristofer Covey, Charles L. Curry, Giuseppe Etiope, Christian Frankenberg, Nicola Gedney, Michaela I. Hegglin, Lena Höglund-Isaksson, Gustaf Hugelius, Misa Ishizawa, Akihiko Ito, Greet Janssens-Maenhout, Katherine M. Jensen, Fortunat Joos, Thomas Kleinen, Paul B. Krummel, Ray L. Langenfelds, Goulven G. Laruelle, Licheng Liu, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Joe McNorton, Paul A. Miller, Joe R. Melton, Isamu Morino, Jurek Müller, Fabiola Murguia-Flores, Vaishali Naik, Yosuke Niwa, Sergio Noce, Simon O'Doherty, Robert J. Parker, Changhui Peng, Shushi Peng, Glen P. Peters, Catherine Prigent, Ronald Prinn, Michel Ramonet, Pierre Regnier, William J. Riley, Judith A. Rosentreter, Arjo Segers, Isobel J. Simpson, Hao Shi, Steven J. Smith, L. Paul Steele, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Francesco N. Tubiello, Aki Tsuruta, Nicolas Viovy, Apostolos Voulgarakis, Thomas S. Weber, Michiel van Weele, Guido R. van der Werf, Ray F. Weiss, Doug Worthy, Debra Wunch, Yi Yin, Yukio Yoshida, Wenxin Zhang, Zhen Zhang, Yuanhong Zhao, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data, 12, 1561–1623, https://doi.org/10.5194/essd-12-1561-2020, https://doi.org/10.5194/essd-12-1561-2020, 2020
Short summary
Short summary
Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. We have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate new research aimed at improving and regularly updating the global methane budget. This is the second version of the review dedicated to the decadal methane budget, integrating results of top-down and bottom-up estimates.
Gregory Duveiller, Federico Filipponi, Sophia Walther, Philipp Köhler, Christian Frankenberg, Luis Guanter, and Alessandro Cescatti
Earth Syst. Sci. Data, 12, 1101–1116, https://doi.org/10.5194/essd-12-1101-2020, https://doi.org/10.5194/essd-12-1101-2020, 2020
Short summary
Short summary
Sun-induced chlorophyll fluorescence is a valuable indicator of vegetation productivity, but our capacity to measure it from space using satellite remote techniques has been hampered by a lack of spatial detail. Based on prior knowledge of how ecosystems should respond to growing conditions in some modelling along with ancillary satellite observations, we provide here a new enhanced dataset with higher spatial resolution that better represents the spatial patterns of vegetation growth over land.
Robert L. Herman, John Worden, David Noone, Dean Henze, Kevin Bowman, Karen Cady-Pereira, Vivienne H. Payne, Susan S. Kulawik, and Dejian Fu
Atmos. Meas. Tech., 13, 1825–1834, https://doi.org/10.5194/amt-13-1825-2020, https://doi.org/10.5194/amt-13-1825-2020, 2020
Short summary
Short summary
This study is the first assessment and validation of AIRS HDO / H2O retrieved by optimal estimation. Initial comparisons with in situ measurements from NASA ORACLES are promising: the small bias and consistent rms of AIRS suggest that AIRS has well-characterized HDO / H2O. This analysis opens the possibility of a new 17-year long-term data record of global tropospheric HDO / H2O measured from space.
Wenfu Tang, Helen M. Worden, Merritt N. Deeter, David P. Edwards, Louisa K. Emmons, Sara Martínez-Alonso, Benjamin Gaubert, Rebecca R. Buchholz, Glenn S. Diskin, Russell R. Dickerson, Xinrong Ren, Hao He, and Yutaka Kondo
Atmos. Meas. Tech., 13, 1337–1356, https://doi.org/10.5194/amt-13-1337-2020, https://doi.org/10.5194/amt-13-1337-2020, 2020
Mark W. Shephard, Enrico Dammers, Karen E. Cady-Pereira, Shailesh K. Kharol, Jesse Thompson, Yonatan Gainariu-Matz, Junhua Zhang, Chris A. McLinden, Andrew Kovachik, Michael Moran, Shabtai Bittman, Christopher E. Sioris, Debora Griffin, Matthew J. Alvarado, Chantelle Lonsdale, Verica Savic-Jovcic, and Qiong Zheng
Atmos. Chem. Phys., 20, 2277–2302, https://doi.org/10.5194/acp-20-2277-2020, https://doi.org/10.5194/acp-20-2277-2020, 2020
Short summary
Short summary
Presented is a description and survey demonstrating the capabilities of the CrIS ammonia product for monitoring, air quality forecast model evaluation, dry deposition estimates, and emission estimates of an agricultural hotspot.
Alexander J. Turner, Philipp Köhler, Troy S. Magney, Christian Frankenberg, Inez Fung, and Ronald C. Cohen
Biogeosciences, 17, 405–422, https://doi.org/10.5194/bg-17-405-2020, https://doi.org/10.5194/bg-17-405-2020, 2020
Short summary
Short summary
We present the highest resolution solar-induced chlorophyll fluorescence (SIF) dataset from satellite measurements, providing previously unobservable phenomena related to plant photosynthesis. We find a strong correspondence between TROPOMI SIF and AmeriFlux GPP. We then observe a double peak in the seasonality of California's photosynthesis, not seen by traditional vegetation indices (e.g., MODIS). This is further corroborated by EOF/PC analysis.
Kazuyuki Miyazaki, Kevin W. Bowman, Keiya Yumimoto, Thomas Walker, and Kengo Sudo
Atmos. Chem. Phys., 20, 931–967, https://doi.org/10.5194/acp-20-931-2020, https://doi.org/10.5194/acp-20-931-2020, 2020
Short summary
Short summary
We introduce a multi-model, multi-constituent chemical data assimilation framework that directly accounts for model error in transport and chemistry by integrating a portfolio of forward chemical transport models. The assimilation was able to reduce ensemble forward model spread and bias relative to independent measurements. Diagnostic information readily available from the framework has the potential to improve chemical predictions through relationships such as emergent constraints.
Le Kuai, Kevin W. Bowman, Kazuyuki Miyazaki, Makoto Deushi, Laura Revell, Eugene Rozanov, Fabien Paulot, Sarah Strode, Andrew Conley, Jean-François Lamarque, Patrick Jöckel, David A. Plummer, Luke D. Oman, Helen Worden, Susan Kulawik, David Paynter, Andrea Stenke, and Markus Kunze
Atmos. Chem. Phys., 20, 281–301, https://doi.org/10.5194/acp-20-281-2020, https://doi.org/10.5194/acp-20-281-2020, 2020
Short summary
Short summary
The tropospheric ozone increase from pre-industrial to the present day leads to a radiative forcing. The top-of-atmosphere outgoing fluxes at the ozone band are controlled by ozone, water vapor, and temperature. We demonstrate a method to attribute the models’ flux biases to these key players using satellite-constrained instantaneous radiative kernels. The largest spread between models is found in the tropics, mainly driven by ozone and then water vapor.
Siraput Jongaramrungruang, Christian Frankenberg, Georgios Matheou, Andrew K. Thorpe, David R. Thompson, Le Kuai, and Riley M. Duren
Atmos. Meas. Tech., 12, 6667–6681, https://doi.org/10.5194/amt-12-6667-2019, https://doi.org/10.5194/amt-12-6667-2019, 2019
Short summary
Short summary
This paper demonstrates the use of high-resolution 2-D plume imagery from airborne remote sensing retrievals to quantify methane point-source emissions. It shows significant improvements on the flux estimates without the need for direct wind speed measurements. This paves the way for enhanced flux estimates in future field campaign and space-based observations to better understand the magnitude and distribution of various point sources of methane.
Elizabeth Asher, Rebecca S. Hornbrook, Britton B. Stephens, Doug Kinnison, Eric J. Morgan, Ralph F. Keeling, Elliot L. Atlas, Sue M. Schauffler, Simone Tilmes, Eric A. Kort, Martin S. Hoecker-Martínez, Matt C. Long, Jean-François Lamarque, Alfonso Saiz-Lopez, Kathryn McKain, Colm Sweeney, Alan J. Hills, and Eric C. Apel
Atmos. Chem. Phys., 19, 14071–14090, https://doi.org/10.5194/acp-19-14071-2019, https://doi.org/10.5194/acp-19-14071-2019, 2019
Short summary
Short summary
Halogenated organic trace gases, which are a source of reactive halogens to the atmosphere, exert a disproportionately large influence on atmospheric chemistry and climate. This paper reports novel aircraft observations of halogenated compounds over the Southern Ocean in summer and evaluates hypothesized regional sources and emissions of these trace gases through their relationships to additional aircraft observations.
Helen M. Worden, A. Anthony Bloom, John R. Worden, Zhe Jiang, Eloise A. Marais, Trissevgeni Stavrakou, Benjamin Gaubert, and Forrest Lacey
Atmos. Chem. Phys., 19, 13569–13579, https://doi.org/10.5194/acp-19-13569-2019, https://doi.org/10.5194/acp-19-13569-2019, 2019
Short summary
Short summary
Biogenic non-methane volatile organic compounds (NMVOCs) emitted from vegetation play a significant role in air quality and climate. However, there are large uncertainties in their role for climate. We present a Bayesian approach to estimate carbon monoxide fluxes that are chemically produced from biogenic sources. This provides independent constraints on models that predict biogenic emissions in order improve their capability for predicting air quality and future climate scenarios.
Susan S. Kulawik, Sean Crowell, David Baker, Junjie Liu, Kathryn McKain, Colm Sweeney, Sebastien C. Biraud, Steve Wofsy, Christopher W. O'Dell, Paul O. Wennberg, Debra Wunch, Coleen M. Roehl, Nicholas M. Deutscher, Matthäus Kiel, David W. T. Griffith, Voltaire A. Velazco, Justus Notholt, Thorsten Warneke, Christof Petri, Martine De Mazière, Mahesh K. Sha, Ralf Sussmann, Markus Rettinger, Dave F. Pollard, Isamu Morino, Osamu Uchino, Frank Hase, Dietrich G. Feist, Sébastien Roche, Kimberly Strong, Rigel Kivi, Laura Iraci, Kei Shiomi, Manvendra K. Dubey, Eliezer Sepulveda, Omaira Elena Garcia Rodriguez, Yao Té, Pascal Jeseck, Pauli Heikkinen, Edward J. Dlugokencky, Michael R. Gunson, Annmarie Eldering, David Crisp, Brendan Fisher, and Gregory B. Osterman
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-257, https://doi.org/10.5194/amt-2019-257, 2019
Publication in AMT not foreseen
Short summary
Short summary
This paper provides a benchmark of OCO-2 v8 and ACOS-GOSAT v7.3 XCO2 and lowermost tropospheric (LMT) errors. The paper focuses on the systematic errors and subtracts out validation, co-location, and random errors, looks at the correlation scale-length (spatially and temporally) of systematic errors, finding that the scale lengths are similar to bias correction scale-lengths. The assimilates of the bias correction term is used to place an error on fluxes estimates.
Daniel H. Cusworth, Daniel J. Jacob, Daniel J. Varon, Christopher Chan Miller, Xiong Liu, Kelly Chance, Andrew K. Thorpe, Riley M. Duren, Charles E. Miller, David R. Thompson, Christian Frankenberg, Luis Guanter, and Cynthia A. Randles
Atmos. Meas. Tech., 12, 5655–5668, https://doi.org/10.5194/amt-12-5655-2019, https://doi.org/10.5194/amt-12-5655-2019, 2019
Short summary
Short summary
We examine the potential for global detection of methane plumes from individual point sources with the new generation of spaceborne imaging spectrometers scheduled for launch in 2019–2025. We perform methane retrievals on simulated scenes with varying surfaces and atmospheric methane concentrations. Our results suggest that imaging spectrometers in space could play a transformative role in the future for quantifying methane emissions from point sources on a global scale.
Jacob K. Hedelius, Tai-Long He, Dylan B. A. Jones, Bianca C. Baier, Rebecca R. Buchholz, Martine De Mazière, Nicholas M. Deutscher, Manvendra K. Dubey, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Laura T. Iraci, Pascal Jeseck, Matthäus Kiel, Rigel Kivi, Cheng Liu, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Sébastien Roche, Coleen M. Roehl, Matthias Schneider, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Colm Sweeney, Yao Té, Osamu Uchino, Voltaire A. Velazco, Wei Wang, Thorsten Warneke, Paul O. Wennberg, Helen M. Worden, and Debra Wunch
Atmos. Meas. Tech., 12, 5547–5572, https://doi.org/10.5194/amt-12-5547-2019, https://doi.org/10.5194/amt-12-5547-2019, 2019
Short summary
Short summary
We seek ways to improve the accuracy of column measurements of carbon monoxide (CO) – an important tracer of pollution – made from the MOPITT satellite instrument. We devise a filtering scheme which reduces the scatter and also eliminates bias among the MOPITT detectors. Compared to ground-based observations, MOPITT measurements are about 6 %–8 % higher. When MOPITT data are implemented in a global assimilation model, they tend to reduce the model mismatch with aircraft measurements.
Susan S. Kulawik, Chris O'Dell, Robert R. Nelson, and Thomas E. Taylor
Atmos. Meas. Tech., 12, 5317–5334, https://doi.org/10.5194/amt-12-5317-2019, https://doi.org/10.5194/amt-12-5317-2019, 2019
Short summary
Short summary
This work investigates errors in CO2 near-infrared estimates retrieved from simulated radiances. We find that interferent errors are underpredicted and that nonlinearity causes significant errors.
Bo Zheng, Frederic Chevallier, Yi Yin, Philippe Ciais, Audrey Fortems-Cheiney, Merritt N. Deeter, Robert J. Parker, Yilong Wang, Helen M. Worden, and Yuanhong Zhao
Earth Syst. Sci. Data, 11, 1411–1436, https://doi.org/10.5194/essd-11-1411-2019, https://doi.org/10.5194/essd-11-1411-2019, 2019
Short summary
Short summary
We use a multi-species atmospheric Bayesian inversion approach to attribute satellite-observed atmospheric carbon monoxide (CO) variations to its sources and sinks in order to achieve a full closure of the global CO budget during 2000–2017. We identify a declining trend in the global CO budget since 2000, driven by reduced anthropogenic emissions in the US, Europe, and China, as well as by reduced biomass burning emissions globally, especially in equatorial Africa.
Merritt N. Deeter, David P. Edwards, Gene L. Francis, John C. Gille, Debbie Mao, Sara Martínez-Alonso, Helen M. Worden, Dan Ziskin, and Meinrat O. Andreae
Atmos. Meas. Tech., 12, 4561–4580, https://doi.org/10.5194/amt-12-4561-2019, https://doi.org/10.5194/amt-12-4561-2019, 2019
Short summary
Short summary
The MOPITT (Measurements of Pollution in the Troposphere) satellite instrument has been making nearly continuous observations of atmospheric carbon monoxide (CO) since 2000. MOPITT CO retrievals are routinely used to analyze emissions from fossil fuels and biomass burning, as well as the atmospheric transport of those emissions. This paper describes recent enhancements to the MOPITT retrieval algorithm. New validation results illustrate clear improvements in the fidelity of the MOPITT product.
Joannes D. Maasakkers, Daniel J. Jacob, Melissa P. Sulprizio, Tia R. Scarpelli, Hannah Nesser, Jian-Xiong Sheng, Yuzhong Zhang, Monica Hersher, A. Anthony Bloom, Kevin W. Bowman, John R. Worden, Greet Janssens-Maenhout, and Robert J. Parker
Atmos. Chem. Phys., 19, 7859–7881, https://doi.org/10.5194/acp-19-7859-2019, https://doi.org/10.5194/acp-19-7859-2019, 2019
Short summary
Short summary
We use 2010–2015 satellite observations of atmospheric methane to improve estimates of methane emissions and their trends, as well as the concentration and trend of tropospheric OH (hydroxyl radical, methane's main sink). We find overestimates of Chinese coal and Middle East oil/gas emissions in the prior estimate. The 2010–2015 growth in methane is attributed to an increase in emissions from India, China, and areas with large tropical wetlands. The contribution from OH is small in comparison.
Alexandra G. Konings, A. Anthony Bloom, Junjie Liu, Nicholas C. Parazoo, David S. Schimel, and Kevin W. Bowman
Biogeosciences, 16, 2269–2284, https://doi.org/10.5194/bg-16-2269-2019, https://doi.org/10.5194/bg-16-2269-2019, 2019
Short summary
Short summary
We estimate heterotrophic respiration (Rh) – the respiration from microbes in the soil – using satellite estimates of the net carbon flux and other quantities. Rh is an important carbon flux but is rarely studied by itself. Our method is the first to estimate how Rh varies in both space and time. The resulting new estimate of Rh is compared to the best currently available alternative, which is based on interpolating field measurements globally. The two estimates disagree and are both uncertain.
Emily Ramnarine, John K. Kodros, Anna L. Hodshire, Chantelle R. Lonsdale, Matthew J. Alvarado, and Jeffrey R. Pierce
Atmos. Chem. Phys., 19, 6561–6577, https://doi.org/10.5194/acp-19-6561-2019, https://doi.org/10.5194/acp-19-6561-2019, 2019
Short summary
Short summary
Biomass burning aerosols have important global radiative effects that depend on particle size. However, model estimates of these effects do not explicitly account for the coagulation of particles in biomass burning plumes. In this work, we present the first use of a sub-grid coagulation scheme in a global aerosol model to account for in-plume coagulation. We find that this in-plume coagulation leads to important changes in the biomass burning aerosol radiative effects.
John R. Worden, Susan S. Kulawik, Dejian Fu, Vivienne H. Payne, Alan E. Lipton, Igor Polonsky, Yuguang He, Karen Cady-Pereira, Jean-Luc Moncet, Robert L. Herman, Fredrick W. Irion, and Kevin W. Bowman
Atmos. Meas. Tech., 12, 2331–2339, https://doi.org/10.5194/amt-12-2331-2019, https://doi.org/10.5194/amt-12-2331-2019, 2019
Short summary
Short summary
In this paper we take the first steps towards generating a multi-decadal record of the deuterium content of water vapor, useful for evaluating the moisture sources and processes affecting water vapor, by estimating the deuterium content from thermal IR radiances from the AIRS instrument. We find the AIRS-based measurements are sensitive to the deuterium content of water vapor in the middle and lower troposphere with a single measurement uncertainty of ~ 3 % and an accuracy of ~ 0.7 %.
Wenfu Tang, Avelino F. Arellano, Benjamin Gaubert, Kazuyuki Miyazaki, and Helen M. Worden
Atmos. Chem. Phys., 19, 4269–4288, https://doi.org/10.5194/acp-19-4269-2019, https://doi.org/10.5194/acp-19-4269-2019, 2019
Martha P. Butler, Thomas Lauvaux, Sha Feng, Junjie Liu, Kevin W. Bowman, and Kenneth J. Davis
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2018-342, https://doi.org/10.5194/gmd-2018-342, 2019
Revised manuscript not accepted
Short summary
Short summary
This paper describes a mass-conserving framework for computing time-varying lateral boundary conditions from global model carbon dioxide concentrations for introduction into the WRF-Chem regional model. The goal is to create a laboratory environment in which carbon dioxide transport uncertainties may be explored separately from inversion-derived flux uncertainties. The software is currently available on GitHub at https://github.com/psu-inversion/WRF_Boundary_Coupling.
Benjamin Gaubert, Britton B. Stephens, Sourish Basu, Frédéric Chevallier, Feng Deng, Eric A. Kort, Prabir K. Patra, Wouter Peters, Christian Rödenbeck, Tazu Saeki, David Schimel, Ingrid Van der Laan-Luijkx, Steven Wofsy, and Yi Yin
Biogeosciences, 16, 117–134, https://doi.org/10.5194/bg-16-117-2019, https://doi.org/10.5194/bg-16-117-2019, 2019
Short summary
Short summary
We have compared global carbon budgets calculated from numerical inverse models and CO2 observations, and evaluated how these systems reproduce vertical gradients in atmospheric CO2 from aircraft measurements. We found that available models have converged on near-neutral tropical total fluxes for several decades, implying consistent sinks in intact tropical forests, and that assumed fossil fuel emissions and predicted atmospheric growth rates are now the dominant axes of disagreement.
Debsunder Dutta, David S. Schimel, Ying Sun, Christiaan van der Tol, and Christian Frankenberg
Biogeosciences, 16, 77–103, https://doi.org/10.5194/bg-16-77-2019, https://doi.org/10.5194/bg-16-77-2019, 2019
Short summary
Short summary
Canopy structural and leaf photosynthesis parameterizations are often fixed over time in Earth system models and represent large sources of uncertainty in predictions of carbon and water fluxes. We develop a moving window nonlinear optimal parameter inversion framework using constraining flux and satellite reflectance observations. The results demonstrate the applicability of the approach for error reduction and capturing the seasonal variability of key ecosystem parameters.
Christopher W. O'Dell, Annmarie Eldering, Paul O. Wennberg, David Crisp, Michael R. Gunson, Brendan Fisher, Christian Frankenberg, Matthäus Kiel, Hannakaisa Lindqvist, Lukas Mandrake, Aronne Merrelli, Vijay Natraj, Robert R. Nelson, Gregory B. Osterman, Vivienne H. Payne, Thomas E. Taylor, Debra Wunch, Brian J. Drouin, Fabiano Oyafuso, Albert Chang, James McDuffie, Michael Smyth, David F. Baker, Sourish Basu, Frédéric Chevallier, Sean M. R. Crowell, Liang Feng, Paul I. Palmer, Mavendra Dubey, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, Coleen M. Roehl, Mahesh K. Sha, Kimberly Strong, Ralf Sussmann, Yao Te, Osamu Uchino, and Voltaire A. Velazco
Atmos. Meas. Tech., 11, 6539–6576, https://doi.org/10.5194/amt-11-6539-2018, https://doi.org/10.5194/amt-11-6539-2018, 2018
Dien Wu, John C. Lin, Benjamin Fasoli, Tomohiro Oda, Xinxin Ye, Thomas Lauvaux, Emily G. Yang, and Eric A. Kort
Geosci. Model Dev., 11, 4843–4871, https://doi.org/10.5194/gmd-11-4843-2018, https://doi.org/10.5194/gmd-11-4843-2018, 2018
Short summary
Short summary
Urban CO2 enhancement signals can be derived using satellite column CO2 concentrations and atmospheric transport models. However, uncertainties due to model configurations, atmospheric transport, and defined background values can potentially impact the derived urban signals. In this paper, we present a modified Lagrangian model framework that extracts urban CO2 signals from satellite observations and determines potential error impacts.
Alexander Gvakharia, Eric A. Kort, Mackenzie L. Smith, and Stephen Conley
Atmos. Meas. Tech., 11, 6059–6074, https://doi.org/10.5194/amt-11-6059-2018, https://doi.org/10.5194/amt-11-6059-2018, 2018
Short summary
Short summary
We present a new flight system to measure the atmospheric trace gases N2O, CO2, CO, and H2O. We use a novel calibration technique to correct altitude-dependent artifacts that have hindered similar instruments. In-flight null-tests and comparison with other flight-proven instruments provide validation. This high-precision, high-accuracy system provides opportunities for airborne studies to improve our understanding of N2O emission processes.
Dejian Fu, Susan S. Kulawik, Kazuyuki Miyazaki, Kevin W. Bowman, John R. Worden, Annmarie Eldering, Nathaniel J. Livesey, Joao Teixeira, Fredrick W. Irion, Robert L. Herman, Gregory B. Osterman, Xiong Liu, Pieternel F. Levelt, Anne M. Thompson, and Ming Luo
Atmos. Meas. Tech., 11, 5587–5605, https://doi.org/10.5194/amt-11-5587-2018, https://doi.org/10.5194/amt-11-5587-2018, 2018
Emily V. Fischer, Liye Zhu, Vivienne H. Payne, John R. Worden, Zhe Jiang, Susan S. Kulawik, Steven Brey, Arsineh Hecobian, Daniel Gombos, Karen Cady-Pereira, and Frank Flocke
Atmos. Chem. Phys., 18, 5639–5653, https://doi.org/10.5194/acp-18-5639-2018, https://doi.org/10.5194/acp-18-5639-2018, 2018
Short summary
Short summary
PAN is an atmospheric reservoir for nitrogen oxide radicals, and it plays a lead role in their redistribution in the troposphere. We analyze new Tropospheric Emission Spectrometer (TES) PAN observations over North America during July 2006 to 2009. We identify smoke-impacted TES PAN retrievals by co-location with NOAA Hazard Mapping System (HMS) smoke plumes. Depending on the year, 15–32 % of cases where elevated PAN is identified in TES observations overlap with smoke plumes.
David P. Edwards, Helen M. Worden, Doreen Neil, Gene Francis, Tim Valle, and Avelino F. Arellano Jr.
Atmos. Meas. Tech., 11, 1061–1085, https://doi.org/10.5194/amt-11-1061-2018, https://doi.org/10.5194/amt-11-1061-2018, 2018
Short summary
Short summary
The CHRONOS space mission would provide observations for emissions and transport studies of the highly uncertain air pollutants carbon monoxide and methane, with sub-hourly revisit at fine horizontal spatial resolution across North America. CHRONOS uses an imaging gas filter correlation radiometer hosted in geostationary orbit. CHRONOS' capability for monitoring evolving, or unanticipated, air pollution sources would find societal applications for air quality management and forecasting.
Jingqiu Mao, Annmarie Carlton, Ronald C. Cohen, William H. Brune, Steven S. Brown, Glenn M. Wolfe, Jose L. Jimenez, Havala O. T. Pye, Nga Lee Ng, Lu Xu, V. Faye McNeill, Kostas Tsigaridis, Brian C. McDonald, Carsten Warneke, Alex Guenther, Matthew J. Alvarado, Joost de Gouw, Loretta J. Mickley, Eric M. Leibensperger, Rohit Mathur, Christopher G. Nolte, Robert W. Portmann, Nadine Unger, Mika Tosca, and Larry W. Horowitz
Atmos. Chem. Phys., 18, 2615–2651, https://doi.org/10.5194/acp-18-2615-2018, https://doi.org/10.5194/acp-18-2615-2018, 2018
Short summary
Short summary
This paper is aimed at discussing progress in evaluating, diagnosing, and improving air quality and climate modeling using comparisons to SAS observations as a guide to thinking about improvements to mechanisms and parameterizations in models.
Xinxin Ye, Thomas Lauvaux, Eric A. Kort, Tomohiro Oda, Sha Feng, John C. Lin, Emily Yang, and Dien Wu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-1022, https://doi.org/10.5194/acp-2017-1022, 2017
Revised manuscript not accepted
Short summary
Short summary
Rapid global urbanization and significant fossil fuel consumption by cities emphasize the necessity of achieving independent and accurate quantification of the carbon emissions from urban areas. In this paper, we assess the potential of using total column CO2 concentration observed from satellite to quantify fossil-fuel carbon emissions from cities. This study could give insights into the capability of satellite observations on monitoring of the emissions on local scale.
Iris N. Dekker, Sander Houweling, Ilse Aben, Thomas Röckmann, Maarten Krol, Sara Martínez-Alonso, Merritt N. Deeter, and Helen M. Worden
Atmos. Chem. Phys., 17, 14675–14694, https://doi.org/10.5194/acp-17-14675-2017, https://doi.org/10.5194/acp-17-14675-2017, 2017
Short summary
Short summary
This study estimates carbon monoxide emissions from the city of Madrid using MOPITT satellite data. There are two methods used and reviewed in this paper: a method that can only estimate a trend in the emission and a newly developed method that also includes model data from WRF to quantify the emissions. We find Madrid CO emissions to be lower by 48 % for 2002 and by 17 % for 2006 compared with the EdgarV4.2 emission inventory, but uncertainty (20 to 50 %) remains.
Zachary R. Barkley, Thomas Lauvaux, Kenneth J. Davis, Aijun Deng, Natasha L. Miles, Scott J. Richardson, Yanni Cao, Colm Sweeney, Anna Karion, MacKenzie Smith, Eric A. Kort, Stefan Schwietzke, Thomas Murphy, Guido Cervone, Douglas Martins, and Joannes D. Maasakkers
Atmos. Chem. Phys., 17, 13941–13966, https://doi.org/10.5194/acp-17-13941-2017, https://doi.org/10.5194/acp-17-13941-2017, 2017
Short summary
Short summary
This study quantifies methane emissions from natural gas production in north-eastern Pennsylvania. Methane observations from 10 flights in spring 2015 are compared to model-projected values, and methane emissions from natural gas are adjusted within the model to create the best match between the two data sets. This study find methane emissions from natural gas production to be low and may be indicative of characteristics of the basin that make sources from north-eastern Pennsylvania unique.
Andrew K. Thorpe, Christian Frankenberg, David R. Thompson, Riley M. Duren, Andrew D. Aubrey, Brian D. Bue, Robert O. Green, Konstantin Gerilowski, Thomas Krings, Jakob Borchardt, Eric A. Kort, Colm Sweeney, Stephen Conley, Dar A. Roberts, and Philip E. Dennison
Atmos. Meas. Tech., 10, 3833–3850, https://doi.org/10.5194/amt-10-3833-2017, https://doi.org/10.5194/amt-10-3833-2017, 2017
Short summary
Short summary
At local scales emissions of methane (CH4) and carbon dioxide (CO2) are highly uncertain. The AVIRIS-NG imaging spectrometer maps large regions and generates high-spatial-resolution CH4 and CO2 concentration maps from anthropogenic and natural sources. Examples include CH4 from a processing plant, tank, pipeline leak, seep, mine vent shafts, and CO2 from power plants. This demonstrates a greenhouse gas monitoring capability that targets the two dominant anthropogenic climate-forcing agents.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Ray Weiss, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Atmos. Chem. Phys., 17, 11135–11161, https://doi.org/10.5194/acp-17-11135-2017, https://doi.org/10.5194/acp-17-11135-2017, 2017
Short summary
Short summary
Following the Global Methane Budget 2000–2012 published in Saunois et al. (2016), we use the same dataset of bottom-up and top-down approaches to discuss the variations in methane emissions over the period 2000–2012. The changes in emissions are discussed both in terms of trends and quasi-decadal changes. The ensemble gathered here allows us to synthesise the robust changes in terms of regional and sectorial contributions to the increasing methane emissions.
Stephen Conley, Ian Faloona, Shobhit Mehrotra, Maxime Suard, Donald H. Lenschow, Colm Sweeney, Scott Herndon, Stefan Schwietzke, Gabrielle Pétron, Justin Pifer, Eric A. Kort, and Russell Schnell
Atmos. Meas. Tech., 10, 3345–3358, https://doi.org/10.5194/amt-10-3345-2017, https://doi.org/10.5194/amt-10-3345-2017, 2017
Short summary
Short summary
This paper describes a new method of quantifying surface trace gas emissions (e.g. methane) from small aircraft (e.g. Mooney, Cessna) in about 30 min. This technique greatly enhances our ability to rapidly respond in the event of catastrophic failures such as Aliso Canyon and Deep Water Horizon.
Karen E. Cady-Pereira, Vivienne H. Payne, Jessica L. Neu, Kevin W. Bowman, Kazuyuki Miyazaki, Eloise A. Marais, Susan Kulawik, Zitely A. Tzompa-Sosa, and Jennifer D. Hegarty
Atmos. Chem. Phys., 17, 9379–9398, https://doi.org/10.5194/acp-17-9379-2017, https://doi.org/10.5194/acp-17-9379-2017, 2017
Short summary
Short summary
Air quality is a major issue for megacities. Our paper looks at satellite measurements over Mexico City and Lagos of several trace gases gases related to air quality to determine the temporal and spatial variability of these gases, and it relates this variability to local conditions, such as topography, winds and biomass burning events. We find that, while Mexico City is known for severe pollution events, the levels of of pollution in Lagos are much higher and more persistent.
John R. Worden, Gary Doran, Susan Kulawik, Annmarie Eldering, David Crisp, Christian Frankenberg, Chris O'Dell, and Kevin Bowman
Atmos. Meas. Tech., 10, 2759–2771, https://doi.org/10.5194/amt-10-2759-2017, https://doi.org/10.5194/amt-10-2759-2017, 2017
Short summary
Short summary
This paper evaluates the uncertainties of the total column carbon dioxide (XCO2) measurements from the NASA OCO-2 instrument by comparing observed variations in small geographical regions to the calculated uncertainties of the data within this region. In general we find that the reported XCO2 precision is related to that expected from the XCO2 radiance noise. However, the reported accuracy is at least smaller than the actual accuracy by a factor of 2–4.
Merritt N. Deeter, David P. Edwards, Gene L. Francis, John C. Gille, Sara Martínez-Alonso, Helen M. Worden, and Colm Sweeney
Atmos. Meas. Tech., 10, 2533–2555, https://doi.org/10.5194/amt-10-2533-2017, https://doi.org/10.5194/amt-10-2533-2017, 2017
Short summary
Short summary
This manuscript describes the methods used for deriving the latest version 7 product for atmospheric carbon monoxide (CO) from measurements made by the MOPITT (Measurements of Pollution in the Troposphere) satellite instrument. Comparisons of MOPITT-retrieved CO vertical profiles with in situ data measured from aircraft are also presented, and they demonstrate clear improvements relative to earlier MOPITT products. The new CO product is appropriate for a wide variety of applications.
Kazuyuki Miyazaki and Kevin Bowman
Atmos. Chem. Phys., 17, 8285–8312, https://doi.org/10.5194/acp-17-8285-2017, https://doi.org/10.5194/acp-17-8285-2017, 2017
Short summary
Short summary
The ACCMIP ensemble ozone simulations are evaluated by a state-of-the-art multi-constituent chemical reanalysis. The reanalysis product provides comprehensive and unique information on the weakness of the individual models and multi-model mean. The differences are less evident with the current sonde network, which is shown to provide biased regional and monthly ozone statistics. The evaluation results have implications for ozone radiative forcing and the response of chemistry to climate.
A. Anthony Bloom, Kevin W. Bowman, Meemong Lee, Alexander J. Turner, Ronny Schroeder, John R. Worden, Richard Weidner, Kyle C. McDonald, and Daniel J. Jacob
Geosci. Model Dev., 10, 2141–2156, https://doi.org/10.5194/gmd-10-2141-2017, https://doi.org/10.5194/gmd-10-2141-2017, 2017
Short summary
Short summary
Wetland emissions are a principal source of uncertainty in the global atmospheric methane budget due to poor knowledge of wetland processes. We construct a wetland methane emission and uncertainty dataset for use in global atmospheric methane models. Our wetland model ensemble is based on static wetland maps, satellite-derived inundation and carbon cycle models. The ensemble performs favourably against regional flux estimates and atmospheric methane measurements relative to previous studies.
Zhe Jiang, Helen Worden, John R. Worden, Daven K. Henze, Dylan B. A. Jones, Avelino F. Arellano, Emily V. Fischer, Liye Zhu, Kazuyuki Miyazaki, K. Folkert Boersma, and Vivienne H. Payne
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-382, https://doi.org/10.5194/acp-2017-382, 2017
Preprint withdrawn
Short summary
Short summary
We investigated the variation of US tropospheric NO2 in the past decade. We demonstrated significant divergence between the time variation in tropospheric NO2 columns from OMI retrievals and surface measurements. Our analysis suggests limited contributions from local effects such as fossil fuel emissions, lightning, or instrument artifacts, and indicates possible important contributions from long-range transport of Asian emissions that are modulated by ENSO.
Rebecca R. Buchholz, Merritt N. Deeter, Helen M. Worden, John Gille, David P. Edwards, James W. Hannigan, Nicholas B. Jones, Clare Paton-Walsh, David W. T. Griffith, Dan Smale, John Robinson, Kimberly Strong, Stephanie Conway, Ralf Sussmann, Frank Hase, Thomas Blumenstock, Emmanuel Mahieu, and Bavo Langerock
Atmos. Meas. Tech., 10, 1927–1956, https://doi.org/10.5194/amt-10-1927-2017, https://doi.org/10.5194/amt-10-1927-2017, 2017
Short summary
Short summary
The study presents the first systematic use of ground-based remote-sensing data from the Network for the Detection of Atmospheric Composition Change (NDACC) to validate satellite-based Measurements of Pollution in the Troposphere (MOPITT) total column carbon monoxide (CO). MOPITT generally shows low bias with respect to the ground-based instruments. The geographic and temporal dependence of validation results are determined. Our findings inform some recommendations for using MOPITT measurements.
Vivienne H. Payne, Emily V. Fischer, John R. Worden, Zhe Jiang, Liye Zhu, Thomas P. Kurosu, and Susan S. Kulawik
Atmos. Chem. Phys., 17, 6341–6351, https://doi.org/10.5194/acp-17-6341-2017, https://doi.org/10.5194/acp-17-6341-2017, 2017
Short summary
Short summary
Peroxyacetyl nitrate (PAN) plays a key role in atmospheric chemistry and long-range transport of pollution. In this paper, we present measurements of PAN from the Tropospheric Emission Spectrometer, an instrument on board the NASA Aura satellite since 2004. We focus on measurements of PAN in tropical regions, where data from ground-based and aircraft campaigns are particularly sparse. We observe temporal changes in PAN associated with changes in fires, convection and emissions.
Michael Buchwitz, Oliver Schneising, Maximilian Reuter, Jens Heymann, Sven Krautwurst, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Christian Frankenberg, and Alexander J. Turner
Atmos. Chem. Phys., 17, 5751–5774, https://doi.org/10.5194/acp-17-5751-2017, https://doi.org/10.5194/acp-17-5751-2017, 2017
Short summary
Short summary
Methane is an important greenhouse gas and increasing atmospheric concentrations result in global warming. We present a simple method to derive annual methane emission estimates of methane hotspot areas from satellite data. We present results for four source areas. We found that our estimates are in good agreement with other studies/data sets for the Four Corners region in the USA and for Azerbaijan but we also found higher emissions for parts of California and Turkmenistan.
Min Huang, Gregory R. Carmichael, R. Bradley Pierce, Duseong S. Jo, Rokjin J. Park, Johannes Flemming, Louisa K. Emmons, Kevin W. Bowman, Daven K. Henze, Yanko Davila, Kengo Sudo, Jan Eiof Jonson, Marianne Tronstad Lund, Greet Janssens-Maenhout, Frank J. Dentener, Terry J. Keating, Hilke Oetjen, and Vivienne H. Payne
Atmos. Chem. Phys., 17, 5721–5750, https://doi.org/10.5194/acp-17-5721-2017, https://doi.org/10.5194/acp-17-5721-2017, 2017
Short summary
Short summary
In support of the HTAP phase 2 experiment, we conducted a number of regional-scale Sulfur Transport and dEposition Model base and sensitivity simulations over North America during May–June 2010. The STEM chemical boundary conditions were downscaled from three (GEOS-Chem, RAQMS, and ECMWF C-IFS) global chemical transport models' simulations. Analyses were performed on large spatial–temporal scales relative to HTAP1 and also on subcontinental and event scales including the use of satellite data.
Susan S. Kulawik, Chris O'Dell, Vivienne H. Payne, Le Kuai, Helen M. Worden, Sebastien C. Biraud, Colm Sweeney, Britton Stephens, Laura T. Iraci, Emma L. Yates, and Tomoaki Tanaka
Atmos. Chem. Phys., 17, 5407–5438, https://doi.org/10.5194/acp-17-5407-2017, https://doi.org/10.5194/acp-17-5407-2017, 2017
Short summary
Short summary
We introduce new vertically resolved GOSAT products that better separate locally and remotely influenced CO2. Current GOSAT column results for CO2 (XCO2) are sensitive to fluxes on continental scales, whereas flux estimates from surface and tower measurements are affected by sampling bias and model transport uncertainty. These new GOSAT measurements of boundary layer CO2 are validated against aircraft and surface observations of CO2 and are compared to vertically resolved MOPITT CO.
Zhe Jiang, John R. Worden, Helen Worden, Merritt Deeter, Dylan B. A. Jones, Avelino F. Arellano, and Daven K. Henze
Atmos. Chem. Phys., 17, 4565–4583, https://doi.org/10.5194/acp-17-4565-2017, https://doi.org/10.5194/acp-17-4565-2017, 2017
Short summary
Short summary
We constrain the long-term variation in global CO emissions for 2001–2015. Our results confirm that the decreasing trend of tropospheric CO in the Northern Hemisphere is due to decreasing CO emissions from anthropogenic and biomass burning sources. In particular, we find decreasing CO emissions from the United States and China in the past 15 years, unchanged anthropogenic CO emissions from Europe since 2008, and likely a positive trend from India and southeast Asia.
Kang Sun, Xiong Liu, Caroline R. Nowlan, Zhaonan Cai, Kelly Chance, Christian Frankenberg, Richard A. M. Lee, Randy Pollock, Robert Rosenberg, and David Crisp
Atmos. Meas. Tech., 10, 939–953, https://doi.org/10.5194/amt-10-939-2017, https://doi.org/10.5194/amt-10-939-2017, 2017
Short summary
Short summary
Accurately characterizing the instrument line shape (ILS) of the Orbiting Carbon Observatory-2 (OCO-2) is challenging and highly important due to its high spectral resolution and requirement for retrieval accuracy. Measured ILS during preflight experiments has been used in the OCO-2 CO2 retrieval. This study derives the on-orbit ILS of OCO-2 using its solar measurements and answers the questions whether on-orbit ILS has changed compared to preflight and whether it varies during the mission.
Chantelle R. Lonsdale, Jennifer D. Hegarty, Karen E. Cady-Pereira, Matthew J. Alvarado, Daven K. Henze, Matthew D. Turner, Shannon L. Capps, John B. Nowak, J. Andy Neuman, Ann M. Middlebrook, Roya Bahreini, Jennifer G. Murphy, Milos Z. Markovic, Trevor C. VandenBoer, Lynn M. Russell, and Amy Jo Scarino
Atmos. Chem. Phys., 17, 2721–2739, https://doi.org/10.5194/acp-17-2721-2017, https://doi.org/10.5194/acp-17-2721-2017, 2017
Short summary
Short summary
This study takes advantage of the high-resolution observations of NH3(g) made by the TES satellite instrument over Bakersfield during the CalNex campaign, along with campaign measurements, to compare CMAQ model results in the San Joaquin Valley, California. Additionally we evaluate the CMAQ bi-directional ammonia flux results using the CARB emissions inventory against these satellite and campaign measurements, not previously explored in combination.
Annmarie Eldering, Chris W. O'Dell, Paul O. Wennberg, David Crisp, Michael R. Gunson, Camille Viatte, Charles Avis, Amy Braverman, Rebecca Castano, Albert Chang, Lars Chapsky, Cecilia Cheng, Brian Connor, Lan Dang, Gary Doran, Brendan Fisher, Christian Frankenberg, Dejian Fu, Robert Granat, Jonathan Hobbs, Richard A. M. Lee, Lukas Mandrake, James McDuffie, Charles E. Miller, Vicky Myers, Vijay Natraj, Denis O'Brien, Gregory B. Osterman, Fabiano Oyafuso, Vivienne H. Payne, Harold R. Pollock, Igor Polonsky, Coleen M. Roehl, Robert Rosenberg, Florian Schwandner, Mike Smyth, Vivian Tang, Thomas E. Taylor, Cathy To, Debra Wunch, and Jan Yoshimizu
Atmos. Meas. Tech., 10, 549–563, https://doi.org/10.5194/amt-10-549-2017, https://doi.org/10.5194/amt-10-549-2017, 2017
Short summary
Short summary
This paper describes the measurements of atmospheric carbon dioxide collected in the first 18 months of the satellite mission known as the Orbiting Carbon Observatory-2 (OCO-2). The paper shows maps of the carbon dioxide data, data density, and other data fields that illustrate the data quality. This mission has collected a more precise, more dense dataset of carbon dioxide then we have ever had previously.
Kazuyuki Miyazaki, Henk Eskes, Kengo Sudo, K. Folkert Boersma, Kevin Bowman, and Yugo Kanaya
Atmos. Chem. Phys., 17, 807–837, https://doi.org/10.5194/acp-17-807-2017, https://doi.org/10.5194/acp-17-807-2017, 2017
Short summary
Short summary
Global surface emissions of nitrogen oxides (NOx) over a 10-year period (2005–2014) are estimated from assimilation of multiple satellite datasets. We present detailed distributions of the estimated NOx emission distributions for all major regions, the diurnal, seasonal, and decadal variability. The estimated emissions show a positive trend over India, China, and the Middle East, and a negative trend over the United States, southern Africa, and western Europe.
David Crisp, Harold R. Pollock, Robert Rosenberg, Lars Chapsky, Richard A. M. Lee, Fabiano A. Oyafuso, Christian Frankenberg, Christopher W. O'Dell, Carol J. Bruegge, Gary B. Doran, Annmarie Eldering, Brendan M. Fisher, Dejian Fu, Michael R. Gunson, Lukas Mandrake, Gregory B. Osterman, Florian M. Schwandner, Kang Sun, Tommy E. Taylor, Paul O. Wennberg, and Debra Wunch
Atmos. Meas. Tech., 10, 59–81, https://doi.org/10.5194/amt-10-59-2017, https://doi.org/10.5194/amt-10-59-2017, 2017
Short summary
Short summary
The Orbiting Carbon Observatory-2 carries and points a three-channel imaging grating spectrometer designed to collect high-resolution spectra of reflected sunlight within the molecular oxygen A-band at 0.765 microns and the carbon dioxide bands at 1.61 and 2.06 microns. Here, we describe the OCO-2 instrument, its data products, and its performance during its first 18 months in orbit.
Marielle Saunois, Philippe Bousquet, Ben Poulter, Anna Peregon, Philippe Ciais, Josep G. Canadell, Edward J. Dlugokencky, Giuseppe Etiope, David Bastviken, Sander Houweling, Greet Janssens-Maenhout, Francesco N. Tubiello, Simona Castaldi, Robert B. Jackson, Mihai Alexe, Vivek K. Arora, David J. Beerling, Peter Bergamaschi, Donald R. Blake, Gordon Brailsford, Victor Brovkin, Lori Bruhwiler, Cyril Crevoisier, Patrick Crill, Kristofer Covey, Charles Curry, Christian Frankenberg, Nicola Gedney, Lena Höglund-Isaksson, Misa Ishizawa, Akihiko Ito, Fortunat Joos, Heon-Sook Kim, Thomas Kleinen, Paul Krummel, Jean-François Lamarque, Ray Langenfelds, Robin Locatelli, Toshinobu Machida, Shamil Maksyutov, Kyle C. McDonald, Julia Marshall, Joe R. Melton, Isamu Morino, Vaishali Naik, Simon O'Doherty, Frans-Jan W. Parmentier, Prabir K. Patra, Changhui Peng, Shushi Peng, Glen P. Peters, Isabelle Pison, Catherine Prigent, Ronald Prinn, Michel Ramonet, William J. Riley, Makoto Saito, Monia Santini, Ronny Schroeder, Isobel J. Simpson, Renato Spahni, Paul Steele, Atsushi Takizawa, Brett F. Thornton, Hanqin Tian, Yasunori Tohjima, Nicolas Viovy, Apostolos Voulgarakis, Michiel van Weele, Guido R. van der Werf, Ray Weiss, Christine Wiedinmyer, David J. Wilton, Andy Wiltshire, Doug Worthy, Debra Wunch, Xiyan Xu, Yukio Yoshida, Bowen Zhang, Zhen Zhang, and Qiuan Zhu
Earth Syst. Sci. Data, 8, 697–751, https://doi.org/10.5194/essd-8-697-2016, https://doi.org/10.5194/essd-8-697-2016, 2016
Short summary
Short summary
An accurate assessment of the methane budget is important to understand the atmospheric methane concentrations and trends and to provide realistic pathways for climate change mitigation. The various and diffuse sources of methane as well and its oxidation by a very short lifetime radical challenge this assessment. We quantify the methane sources and sinks as well as their uncertainties based on both bottom-up and top-down approaches provided by a broad international scientific community.
Daniel J. Jacob, Alexander J. Turner, Joannes D. Maasakkers, Jianxiong Sheng, Kang Sun, Xiong Liu, Kelly Chance, Ilse Aben, Jason McKeever, and Christian Frankenberg
Atmos. Chem. Phys., 16, 14371–14396, https://doi.org/10.5194/acp-16-14371-2016, https://doi.org/10.5194/acp-16-14371-2016, 2016
Short summary
Short summary
Methane is a greenhouse gas emitted by a range of natural and anthropogenic sources. Atmospheric methane has been measured continuously from space since 2003, and new instruments are planned to launch in the near future that will greatly expand the capabilities of space-based observations. We review the value of current, future, and proposed satellite observations to better quantify methane emissions from the global scale down to the scale of point sources.
Brian Connor, Hartmut Bösch, James McDuffie, Tommy Taylor, Dejian Fu, Christian Frankenberg, Chris O'Dell, Vivienne H. Payne, Michael Gunson, Randy Pollock, Jonathan Hobbs, Fabiano Oyafuso, and Yibo Jiang
Atmos. Meas. Tech., 9, 5227–5238, https://doi.org/10.5194/amt-9-5227-2016, https://doi.org/10.5194/amt-9-5227-2016, 2016
Short summary
Short summary
We present an analysis of uncertainties in global measurements of the column-averaged dry-air mole fraction of CO2 (XCO2) by the satellite OCO-2. The analysis is based on our best estimates for uncertainties in the OCO-2 operational algorithm and its inputs. From these results we estimate the "variable error", which differs between soundings, to infer the error in the difference of XCO2 between any two soundings. Variable errors are usually < 1 ppm over ocean and ~ 0.5–2 ppm over land.
Zeli Tan, Qianlai Zhuang, Daven K. Henze, Christian Frankenberg, Ed Dlugokencky, Colm Sweeney, Alexander J. Turner, Motoki Sasakawa, and Toshinobu Machida
Atmos. Chem. Phys., 16, 12649–12666, https://doi.org/10.5194/acp-16-12649-2016, https://doi.org/10.5194/acp-16-12649-2016, 2016
Short summary
Short summary
Methane emissions from the pan-Arctic could be important in understanding the global carbon cycle but are still poorly constrained to date. This study demonstrated that satellite retrievals can be used to reduce the uncertainty of the estimates of these emissions. We also provided additional evidence for the existence of large methane emissions from pan-Arctic lakes in the Siberian yedoma permafrost region. We found that biogeochemical models should be improved for better estimates.
Remco A. Scheepmaker, Joost aan de Brugh, Haili Hu, Tobias Borsdorff, Christian Frankenberg, Camille Risi, Otto Hasekamp, Ilse Aben, and Jochen Landgraf
Atmos. Meas. Tech., 9, 3921–3937, https://doi.org/10.5194/amt-9-3921-2016, https://doi.org/10.5194/amt-9-3921-2016, 2016
Short summary
Short summary
We have developed an algorithm to measure HDO (heavy water) in the atmosphere using the TROPOMI satellite instrument, scheduled for launch in 2016. Giving an insight in the history of water vapour, these measurements will help to better understand the water cycle and its role in climate change. We use realistic measurement simulations to describe the performance of the algorithm, and show that TROPOMI will greatly improve and extend the HDO datasets from the previous SCIAMACHY and GOSAT missions.
Hilke Oetjen, Vivienne H. Payne, Jessica L. Neu, Susan S. Kulawik, David P. Edwards, Annmarie Eldering, Helen M. Worden, and John R. Worden
Atmos. Chem. Phys., 16, 10229–10239, https://doi.org/10.5194/acp-16-10229-2016, https://doi.org/10.5194/acp-16-10229-2016, 2016
Short summary
Short summary
We developed and tested a strategy for combining TES and IASI free-tropospheric ozone data. A time series of the merged ozone data is presented for regional monthly means over the western US, Europe, and eastern Asia. We show that free-tropospheric ozone over Europe and the western US has remained relatively constant over the past decade but that, contrary to expectations, ozone over Asia in recent years does not continue the rapid rate of increase observed from 2004–2010.
Makoto Inoue, Isamu Morino, Osamu Uchino, Takahiro Nakatsuru, Yukio Yoshida, Tatsuya Yokota, Debra Wunch, Paul O. Wennberg, Coleen M. Roehl, David W. T. Griffith, Voltaire A. Velazco, Nicholas M. Deutscher, Thorsten Warneke, Justus Notholt, John Robinson, Vanessa Sherlock, Frank Hase, Thomas Blumenstock, Markus Rettinger, Ralf Sussmann, Esko Kyrö, Rigel Kivi, Kei Shiomi, Shuji Kawakami, Martine De Mazière, Sabrina G. Arnold, Dietrich G. Feist, Erica A. Barrow, James Barney, Manvendra Dubey, Matthias Schneider, Laura T. Iraci, James R. Podolske, Patrick W. Hillyard, Toshinobu Machida, Yousuke Sawa, Kazuhiro Tsuboi, Hidekazu Matsueda, Colm Sweeney, Pieter P. Tans, Arlyn E. Andrews, Sebastien C. Biraud, Yukio Fukuyama, Jasna V. Pittman, Eric A. Kort, and Tomoaki Tanaka
Atmos. Meas. Tech., 9, 3491–3512, https://doi.org/10.5194/amt-9-3491-2016, https://doi.org/10.5194/amt-9-3491-2016, 2016
Short summary
Short summary
In this study, we correct the biases of GOSAT XCO2 and XCH4 using TCCON data. To evaluate the effectiveness of our correction method, uncorrected/corrected GOSAT data are compared to independent XCO2 and XCH4 data derived from aircraft measurements. Consequently, we suggest that this method is effective for reducing the biases of the GOSAT data. We consider that our work provides GOSAT data users with valuable information and contributes to the further development of studies on greenhouse gases.
Matthew J. Alvarado, Chantelle R. Lonsdale, Helen L. Macintyre, Huisheng Bian, Mian Chin, David A. Ridley, Colette L. Heald, Kenneth L. Thornhill, Bruce E. Anderson, Michael J. Cubison, Jose L. Jimenez, Yutaka Kondo, Lokesh K. Sahu, Jack E. Dibb, and Chien Wang
Atmos. Chem. Phys., 16, 9435–9455, https://doi.org/10.5194/acp-16-9435-2016, https://doi.org/10.5194/acp-16-9435-2016, 2016
Short summary
Short summary
Understanding the scattering and absorption of light by aerosols is necessary for understanding air quality and climate change. We used data from the 2008 ARCTAS campaign to evaluate aerosol optical property models using a closure methodology that separates errors in these models from other errors in aerosol emissions, chemistry, or transport. We find that the models on average perform reasonably well, and make suggestions for how remaining biases could be reduced.
Christian Frankenberg, Susan S. Kulawik, Steven C. Wofsy, Frédéric Chevallier, Bruce Daube, Eric A. Kort, Christopher O'Dell, Edward T. Olsen, and Gregory Osterman
Atmos. Chem. Phys., 16, 7867–7878, https://doi.org/10.5194/acp-16-7867-2016, https://doi.org/10.5194/acp-16-7867-2016, 2016
Short summary
Short summary
We use observations from the HIAPER Pole-to-Pole Observations (HIPPO) flights from January 2009 through September 2011 to validate CO2 measurements from satellites (GOSAT, TES, AIRS) and atmospheric inversion models (CarbonTracker CT2013B, MACC v13r1).
Dejian Fu, Kevin W. Bowman, Helen M. Worden, Vijay Natraj, John R. Worden, Shanshan Yu, Pepijn Veefkind, Ilse Aben, Jochen Landgraf, Larrabee Strow, and Yong Han
Atmos. Meas. Tech., 9, 2567–2579, https://doi.org/10.5194/amt-9-2567-2016, https://doi.org/10.5194/amt-9-2567-2016, 2016
Sarah A. Strode, Helen M. Worden, Megan Damon, Anne R. Douglass, Bryan N. Duncan, Louisa K. Emmons, Jean-Francois Lamarque, Michael Manyin, Luke D. Oman, Jose M. Rodriguez, Susan E. Strahan, and Simone Tilmes
Atmos. Chem. Phys., 16, 7285–7294, https://doi.org/10.5194/acp-16-7285-2016, https://doi.org/10.5194/acp-16-7285-2016, 2016
Short summary
Short summary
We use global models to interpret trends in MOPITT observations of CO. Simulations with time-dependent emissions reproduce the observed trends over the eastern USA and Europe, suggesting that the emissions are reasonable for these regions. The simulations produce a positive trend over eastern China, contrary to the observed negative trend. This may indicate that the assumed emission trend over China is too positive. However, large variability in the overhead ozone column also contributes.
Glynn C. Hulley, Riley M. Duren, Francesca M. Hopkins, Simon J. Hook, Nick Vance, Pierre Guillevic, William R. Johnson, Bjorn T. Eng, Jonathan M. Mihaly, Veljko M. Jovanovic, Seth L. Chazanoff, Zak K. Staniszewski, Le Kuai, John Worden, Christian Frankenberg, Gerardo Rivera, Andrew D. Aubrey, Charles E. Miller, Nabin K. Malakar, Juan M. Sánchez Tomás, and Kendall T. Holmes
Atmos. Meas. Tech., 9, 2393–2408, https://doi.org/10.5194/amt-9-2393-2016, https://doi.org/10.5194/amt-9-2393-2016, 2016
Short summary
Short summary
Using data from a new airborne Hyperspectral Thermal Emission Spectrometer (HyTES) instrument, we present a technique for the detection and wide-area mapping of emission plumes of methane and other atmospheric trace gas species over challenging and diverse environmental conditions with high spatial resolution, that permits direct attribution to sources in complex environments.
Hélène Brogniez, Stephen English, Jean-François Mahfouf, Andreas Behrendt, Wesley Berg, Sid Boukabara, Stefan Alexander Buehler, Philippe Chambon, Antonia Gambacorta, Alan Geer, William Ingram, E. Robert Kursinski, Marco Matricardi, Tatyana A. Odintsova, Vivienne H. Payne, Peter W. Thorne, Mikhail Yu. Tretyakov, and Junhong Wang
Atmos. Meas. Tech., 9, 2207–2221, https://doi.org/10.5194/amt-9-2207-2016, https://doi.org/10.5194/amt-9-2207-2016, 2016
Short summary
Short summary
Because a systematic difference between measurements of water vapor performed by space-borne observing instruments in the microwave spectral domain and their numerical modeling was recently highlighted, this work discusses and gives an overview of the various errors and uncertainties associated with each element in the comparison process. Indeed, the knowledge of absolute errors in any observation of the climate system is key, more specifically because we need to detect small changes.
Thomas E. Taylor, Christopher W. O'Dell, Christian Frankenberg, Philip T. Partain, Heather Q. Cronk, Andrey Savtchenko, Robert R. Nelson, Emily J. Rosenthal, Albert Y. Chang, Brenden Fisher, Gregory B. Osterman, Randy H. Pollock, David Crisp, Annmarie Eldering, and Michael R. Gunson
Atmos. Meas. Tech., 9, 973–989, https://doi.org/10.5194/amt-9-973-2016, https://doi.org/10.5194/amt-9-973-2016, 2016
Short summary
Short summary
NASA's Orbiting Carbon Observatory-2 (OCO-2) is providing approximately 1 million soundings per day of the total column of carbon dioxide (XCO2). The retrieval of XCO2 can only be performed for soundings sufficiently free of cloud and aerosol. This work highlights comparisons of OCO-2 cloud screening algorithms to the MODIS cloud mask product. We find agreement approximately 85 % of the time with some significant spatial and small seasonal dependencies.
Susan Kulawik, Debra Wunch, Christopher O'Dell, Christian Frankenberg, Maximilian Reuter, Tomohiro Oda, Frederic Chevallier, Vanessa Sherlock, Michael Buchwitz, Greg Osterman, Charles E. Miller, Paul O. Wennberg, David Griffith, Isamu Morino, Manvendra K. Dubey, Nicholas M. Deutscher, Justus Notholt, Frank Hase, Thorsten Warneke, Ralf Sussmann, John Robinson, Kimberly Strong, Matthias Schneider, Martine De Mazière, Kei Shiomi, Dietrich G. Feist, Laura T. Iraci, and Joyce Wolf
Atmos. Meas. Tech., 9, 683–709, https://doi.org/10.5194/amt-9-683-2016, https://doi.org/10.5194/amt-9-683-2016, 2016
Short summary
Short summary
To accurately estimate source and sink locations of carbon dioxide, systematic errors in satellite measurements and models must be characterized. This paper examines two satellite data sets (GOSAT, launched 2009, and SCIAMACHY, launched 2002), and two models (CarbonTracker and MACC) vs. the TCCON CO2 validation data set. We assess biases and errors by season and latitude, satellite performance under averaging, and diurnal variability. Our findings are useful for assimilation of satellite data.
S. Doniki, D. Hurtmans, L. Clarisse, C. Clerbaux, H. M. Worden, K. W. Bowman, and P.-F. Coheur
Atmos. Chem. Phys., 15, 12971–12987, https://doi.org/10.5194/acp-15-12971-2015, https://doi.org/10.5194/acp-15-12971-2015, 2015
F. Deng, D. B. A. Jones, T. W. Walker, M. Keller, K. W. Bowman, D. K. Henze, R. Nassar, E. A. Kort, S. C. Wofsy, K. A. Walker, A. E. Bourassa, and D. A. Degenstein
Atmos. Chem. Phys., 15, 11773–11788, https://doi.org/10.5194/acp-15-11773-2015, https://doi.org/10.5194/acp-15-11773-2015, 2015
Short summary
Short summary
The upper troposphere and lower stratosphere (UTLS) is characterized by strong gradients in the distribution of long-lived tracers, which are sensitive to discrepancies in transport in models. We found that our model overestimates CO2 in the polar UTLS through comparison of modeled CO2 with aircraft observations. We then corrected the modeled CO2 and quantified the impact of the correction on the flux estimates using an atmospheric model together with atmospheric CO2 measured from a satellite.
D. R. Thompson, I. Leifer, H. Bovensmann, M. Eastwood, M. Fladeland, C. Frankenberg, K. Gerilowski, R. O. Green, S. Kratwurst, T. Krings, B. Luna, and A. K. Thorpe
Atmos. Meas. Tech., 8, 4383–4397, https://doi.org/10.5194/amt-8-4383-2015, https://doi.org/10.5194/amt-8-4383-2015, 2015
Short summary
Short summary
We discuss principles for real-time infrared spectral signature detection and measurement, and report performance onboard the NASA Airborne Visible Infrared Spectrometer - Next Generation (AVIRIS-NG). We describe a case study of the NASA/ESA CO2 and MEthane eXperiment (COMEX), a multi-platform campaign to measure CH4 plumes released from anthropogenic sources including oil and gas infrastructure. AVIRIS-NG successfully detected CH4 plumes in concert with other in situ and remote instruments.
M. George, C. Clerbaux, I. Bouarar, P.-F. Coheur, M. N. Deeter, D. P. Edwards, G. Francis, J. C. Gille, J. Hadji-Lazaro, D. Hurtmans, A. Inness, D. Mao, and H. M. Worden
Atmos. Meas. Tech., 8, 4313–4328, https://doi.org/10.5194/amt-8-4313-2015, https://doi.org/10.5194/amt-8-4313-2015, 2015
K. C. Wells, D. B. Millet, N. Bousserez, D. K. Henze, S. Chaliyakunnel, T. J. Griffis, Y. Luan, E. J. Dlugokencky, R. G. Prinn, S. O'Doherty, R. F. Weiss, G. S. Dutton, J. W. Elkins, P. B. Krummel, R. Langenfelds, L. P. Steele, E. A. Kort, S. C. Wofsy, and T. Umezawa
Geosci. Model Dev., 8, 3179–3198, https://doi.org/10.5194/gmd-8-3179-2015, https://doi.org/10.5194/gmd-8-3179-2015, 2015
Short summary
Short summary
This paper introduces a new inversion framework for N2O using GEOS-Chem and its adjoint, which we employed in a series of observing system simulation experiments to evaluate the source and sink constraints provided by surface and aircraft-based N2O measurements. We also applied a new approach for estimating a posteriori uncertainty for high-dimensional inversions, and used it to quantify the spatial and temporal resolution of N2O emission constraints achieved with the current observing network.
P. D. Hamer, K. W. Bowman, D. K. Henze, J.-L. Attié, and V. Marécal
Atmos. Chem. Phys., 15, 10645–10667, https://doi.org/10.5194/acp-15-10645-2015, https://doi.org/10.5194/acp-15-10645-2015, 2015
Short summary
Short summary
Using a simplified air quality forecasting model, we explore how characteristics of air quality observations affect our ability to understand and predict ozone air pollution. We show that the photochemical conditions can strongly influence the observing priorities for ozone prediction, such as which species are observed and how well, when, and how frequently. High-freqency observations of ozone, NOx and HCHO in combination during the morning and afternoon are particularly advantageous.
J. R. Worden, A. J. Turner, A. Bloom, S. S. Kulawik, J. Liu, M. Lee, R. Weidner, K. Bowman, C. Frankenberg, R. Parker, and V. H. Payne
Atmos. Meas. Tech., 8, 3433–3445, https://doi.org/10.5194/amt-8-3433-2015, https://doi.org/10.5194/amt-8-3433-2015, 2015
Short summary
Short summary
Here we demonstrate the potential for estimating lower tropospheric CH4 concentrations through the combination of free-tropospheric methane measurements from the Aura Tropospheric Emission Spectrometer (TES) and XCH4 (dry-mole air fraction of methane) from the Greenhouse Gases Observing Satellite - Thermal And Near-infrared for carbon Observation (GOSAT TANSO).
E. N. Koffi, P. J. Rayner, A. J. Norton, C. Frankenberg, and M. Scholze
Biogeosciences, 12, 4067–4084, https://doi.org/10.5194/bg-12-4067-2015, https://doi.org/10.5194/bg-12-4067-2015, 2015
Short summary
Short summary
We investigate the utility of satellite measurements of solar-induced chlorophyll fluorescence (SIF) in constraining gross primary productivity (GPP). We simulate SIF with the biosphere model BETHY coupled with the fluorescence model SCOPE. The model simulates well the patterns of SIF. SIF is sensitive to leaf chlorophyll and incoming radiation but not to the key physiological parameter Vcmax controlling GPP. Thus, further model development is necessary before SIF can be used to constrain GPP.
A. J. Turner, D. J. Jacob, K. J. Wecht, J. D. Maasakkers, E. Lundgren, A. E. Andrews, S. C. Biraud, H. Boesch, K. W. Bowman, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, A. Kuze, J. Notholt, H. Ohyama, R. Parker, V. H. Payne, R. Sussmann, C. Sweeney, V. A. Velazco, T. Warneke, P. O. Wennberg, and D. Wunch
Atmos. Chem. Phys., 15, 7049–7069, https://doi.org/10.5194/acp-15-7049-2015, https://doi.org/10.5194/acp-15-7049-2015, 2015
Z. Jiang, D. B. A. Jones, J. Worden, H. M. Worden, D. K. Henze, and Y. X. Wang
Atmos. Chem. Phys., 15, 6801–6814, https://doi.org/10.5194/acp-15-6801-2015, https://doi.org/10.5194/acp-15-6801-2015, 2015
Short summary
Short summary
We present a high-resolution (0.5 x 0.667) regional CO inversion over North America in the period of June 2004–May 2005, using a combination of GEOS-Chem model and MOPITT CO observations. With optimized lateral boundary conditions, we show that regional inversion analyses can reduce the sensitivity of the CO source estimates to errors in long-range transport and in the distributions of the hydroxyl radical (OH), and consequently, provide better quantification on regional CO source estimates.
M. J. Alvarado, C. R. Lonsdale, R. J. Yokelson, S. K. Akagi, H. Coe, J. S. Craven, E. V. Fischer, G. R. McMeeking, J. H. Seinfeld, T. Soni, J. W. Taylor, D. R. Weise, and C. E. Wold
Atmos. Chem. Phys., 15, 6667–6688, https://doi.org/10.5194/acp-15-6667-2015, https://doi.org/10.5194/acp-15-6667-2015, 2015
Short summary
Short summary
Being able to understand and simulate the chemical evolution of biomass burning smoke plumes under a wide variety of conditions is a critical part of forecasting the impact of these fires on air quality, atmospheric composition, and climate. Here we use an improved model of this chemistry to simulate the evolution of ozone and secondary organic aerosol within a young biomass burning smoke plume from the Williams prescribed burn in chaparral, which was sampled over California in November 2009.
R. A. Scheepmaker, C. Frankenberg, N. M. Deutscher, M. Schneider, S. Barthlott, T. Blumenstock, O. E. Garcia, F. Hase, N. Jones, E. Mahieu, J. Notholt, V. Velazco, J. Landgraf, and I. Aben
Atmos. Meas. Tech., 8, 1799–1818, https://doi.org/10.5194/amt-8-1799-2015, https://doi.org/10.5194/amt-8-1799-2015, 2015
L. Guanter, I. Aben, P. Tol, J. M. Krijger, A. Hollstein, P. Köhler, A. Damm, J. Joiner, C. Frankenberg, and J. Landgraf
Atmos. Meas. Tech., 8, 1337–1352, https://doi.org/10.5194/amt-8-1337-2015, https://doi.org/10.5194/amt-8-1337-2015, 2015
Short summary
Short summary
This paper investigates the potential of the upcoming TROPOspheric Monitoring Instrument (TROPOMI) instrument for the retrieval of the chlorophyll fluorescence signal emitted in the 650–850nm spectral range by the photosynthetic machinery of green plants. We find that TROPOMI will allow substantial improvements in the space monitoring of fluorescence with respect to current spaceborne instruments such as GOME-2 and SCIAMACHY.
M. J. Alvarado, V. H. Payne, K. E. Cady-Pereira, J. D. Hegarty, S. S. Kulawik, K. J. Wecht, J. R. Worden, J. V. Pittman, and S. C. Wofsy
Atmos. Meas. Tech., 8, 965–985, https://doi.org/10.5194/amt-8-965-2015, https://doi.org/10.5194/amt-8-965-2015, 2015
Z. Jiang, D. B. A. Jones, H. M. Worden, and D. K. Henze
Atmos. Chem. Phys., 15, 1521–1537, https://doi.org/10.5194/acp-15-1521-2015, https://doi.org/10.5194/acp-15-1521-2015, 2015
Short summary
Short summary
Using MOPITT (version 5) tropospheric profile and surface layer retrievals, we constrain global CO emissions in the period of June 2004 – May 2005. The inversions suggest a reduction in CO emission in the tropics and an increase in emissions at middle and high latitudes. The results demonstrate that the use of the surface layer retrievals from MOPITT can significantly mitigate the potential impacts of model bias in OH and long-range transport on CO emission estimates.
C. Frankenberg, R. Pollock, R. A. M. Lee, R. Rosenberg, J.-F. Blavier, D. Crisp, C. W. O'Dell, G. B. Osterman, C. Roehl, P. O. Wennberg, and D. Wunch
Atmos. Meas. Tech., 8, 301–313, https://doi.org/10.5194/amt-8-301-2015, https://doi.org/10.5194/amt-8-301-2015, 2015
K. W. Wong, D. Fu, T. J. Pongetti, S. Newman, E. A. Kort, R. Duren, Y.-K. Hsu, C. E. Miller, Y. L. Yung, and S. P. Sander
Atmos. Chem. Phys., 15, 241–252, https://doi.org/10.5194/acp-15-241-2015, https://doi.org/10.5194/acp-15-241-2015, 2015
M. Alexe, P. Bergamaschi, A. Segers, R. Detmers, A. Butz, O. Hasekamp, S. Guerlet, R. Parker, H. Boesch, C. Frankenberg, R. A. Scheepmaker, E. Dlugokencky, C. Sweeney, S. C. Wofsy, and E. A. Kort
Atmos. Chem. Phys., 15, 113–133, https://doi.org/10.5194/acp-15-113-2015, https://doi.org/10.5194/acp-15-113-2015, 2015
H. Oetjen, V. H. Payne, S. S. Kulawik, A. Eldering, J. Worden, D. P. Edwards, G. L. Francis, H. M. Worden, C. Clerbaux, J. Hadji-Lazaro, and D. Hurtmans
Atmos. Meas. Tech., 7, 4223–4236, https://doi.org/10.5194/amt-7-4223-2014, https://doi.org/10.5194/amt-7-4223-2014, 2014
Short summary
Short summary
We apply the TES ozone retrieval algorithm to IASI radiances and characterise the uncertainties and information content of the retrieved ozone profiles. We find that our biases with respect to sondes and our degrees of freedom for signal for ozone are comparable to previously published results from other IASI ozone algorithms. We find that predicted and empirical errors are consistent. In general, the precision of the IASI ozone profiles is better than 20%.
V. H. Payne, M. J. Alvarado, K. E. Cady-Pereira, J. R. Worden, S. S. Kulawik, and E. V. Fischer
Atmos. Meas. Tech., 7, 3737–3749, https://doi.org/10.5194/amt-7-3737-2014, https://doi.org/10.5194/amt-7-3737-2014, 2014
Short summary
Short summary
Peroxyacetyl nitrate (PAN) plays an important role in the distribution of lower-atmospheric ozone. PAN can be transported far from the original pollution source, leading to ozone formation and degraded air quality in remote areas. Satellite observations from the Tropospheric Emission Spectrometer (TES) are sensitive to PAN at lower altitude than previous global data sets. We describe characteristics of the data and show elevated PAN associated with boreal fires and outflow of Asian pollution.
M. N. Deeter, S. Martínez-Alonso, D. P. Edwards, L. K. Emmons, J. C. Gille, H. M. Worden, C. Sweeney, J. V. Pittman, B. C. Daube, and S. C. Wofsy
Atmos. Meas. Tech., 7, 3623–3632, https://doi.org/10.5194/amt-7-3623-2014, https://doi.org/10.5194/amt-7-3623-2014, 2014
Short summary
Short summary
The MOPITT Version 6 product for carbon monoxide (CO) incorporates several enhancements. First, a geolocation bias has been eliminated. Second, the new variable a priori for CO concentrations is based on simulations performed with the CAM-Chem chemical transport model for the years 2000-2009. Third, required meteorological fields are extracted from the MERRA reanalysis. Finally, a retrieval bias in the upper troposphere was substantially reduced. Validation results are presented.
R. L. Herman, J. E. Cherry, J. Young, J. M. Welker, D. Noone, S. S. Kulawik, and J. Worden
Atmos. Meas. Tech., 7, 3127–3138, https://doi.org/10.5194/amt-7-3127-2014, https://doi.org/10.5194/amt-7-3127-2014, 2014
V. Gryazin, C. Risi, J. Jouzel, N. Kurita, J. Worden, C. Frankenberg, V. Bastrikov, K. Gribanov, and O. Stukova
Atmos. Chem. Phys., 14, 9807–9830, https://doi.org/10.5194/acp-14-9807-2014, https://doi.org/10.5194/acp-14-9807-2014, 2014
M. Inoue, I. Morino, O. Uchino, Y. Miyamoto, T. Saeki, Y. Yoshida, T. Yokota, C. Sweeney, P. P. Tans, S. C. Biraud, T. Machida, J. V. Pittman, E. A. Kort, T. Tanaka, S. Kawakami, Y. Sawa, K. Tsuboi, and H. Matsueda
Atmos. Meas. Tech., 7, 2987–3005, https://doi.org/10.5194/amt-7-2987-2014, https://doi.org/10.5194/amt-7-2987-2014, 2014
Q. Zhu, Q. Zhuang, D. Henze, K. Bowman, M. Chen, Y. Liu, Y. He, H. Matsueda, T. Machida, Y. Sawa, and W. Oechel
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-22587-2014, https://doi.org/10.5194/acpd-14-22587-2014, 2014
Revised manuscript not accepted
K. J. Wecht, D. J. Jacob, M. P. Sulprizio, G. W. Santoni, S. C. Wofsy, R. Parker, H. Bösch, and J. Worden
Atmos. Chem. Phys., 14, 8173–8184, https://doi.org/10.5194/acp-14-8173-2014, https://doi.org/10.5194/acp-14-8173-2014, 2014
E. Hache, J.-L. Attié, C. Tourneur, P. Ricaud, L. Coret, W. A. Lahoz, L. El Amraoui, B. Josse, P. Hamer, J. Warner, X. Liu, K. Chance, M. Höpfner, R. Spurr, V. Natraj, S. Kulawik, A. Eldering, and J. Orphal
Atmos. Meas. Tech., 7, 2185–2201, https://doi.org/10.5194/amt-7-2185-2014, https://doi.org/10.5194/amt-7-2185-2014, 2014
S. Massart, A. Agusti-Panareda, I. Aben, A. Butz, F. Chevallier, C. Crevoisier, R. Engelen, C. Frankenberg, and O. Hasekamp
Atmos. Chem. Phys., 14, 6139–6158, https://doi.org/10.5194/acp-14-6139-2014, https://doi.org/10.5194/acp-14-6139-2014, 2014
B. Dils, M. Buchwitz, M. Reuter, O. Schneising, H. Boesch, R. Parker, S. Guerlet, I. Aben, T. Blumenstock, J. P. Burrows, A. Butz, N. M. Deutscher, C. Frankenberg, F. Hase, O. P. Hasekamp, J. Heymann, M. De Mazière, J. Notholt, R. Sussmann, T. Warneke, D. Griffith, V. Sherlock, and D. Wunch
Atmos. Meas. Tech., 7, 1723–1744, https://doi.org/10.5194/amt-7-1723-2014, https://doi.org/10.5194/amt-7-1723-2014, 2014
C. L. Heald, D. A. Ridley, J. H. Kroll, S. R. H. Barrett, K. E. Cady-Pereira, M. J. Alvarado, and C. D. Holmes
Atmos. Chem. Phys., 14, 5513–5527, https://doi.org/10.5194/acp-14-5513-2014, https://doi.org/10.5194/acp-14-5513-2014, 2014
S. Houweling, M. Krol, P. Bergamaschi, C. Frankenberg, E. J. Dlugokencky, I. Morino, J. Notholt, V. Sherlock, D. Wunch, V. Beck, C. Gerbig, H. Chen, E. A. Kort, T. Röckmann, and I. Aben
Atmos. Chem. Phys., 14, 3991–4012, https://doi.org/10.5194/acp-14-3991-2014, https://doi.org/10.5194/acp-14-3991-2014, 2014
F. Deng, D. B. A. Jones, D. K. Henze, N. Bousserez, K. W. Bowman, J. B. Fisher, R. Nassar, C. O'Dell, D. Wunch, P. O. Wennberg, E. A. Kort, S. C. Wofsy, T. Blumenstock, N. M. Deutscher, D. W. T. Griffith, F. Hase, P. Heikkinen, V. Sherlock, K. Strong, R. Sussmann, and T. Warneke
Atmos. Chem. Phys., 14, 3703–3727, https://doi.org/10.5194/acp-14-3703-2014, https://doi.org/10.5194/acp-14-3703-2014, 2014
C. Liu, S. Beirle, T. Butler, P. Hoor, C. Frankenberg, P. Jöckel, M. Penning de Vries, U. Platt, A. Pozzer, M. G. Lawrence, J. Lelieveld, H. Tost, and T. Wagner
Atmos. Chem. Phys., 14, 1717–1732, https://doi.org/10.5194/acp-14-1717-2014, https://doi.org/10.5194/acp-14-1717-2014, 2014
A. K. Thorpe, C. Frankenberg, and D. A. Roberts
Atmos. Meas. Tech., 7, 491–506, https://doi.org/10.5194/amt-7-491-2014, https://doi.org/10.5194/amt-7-491-2014, 2014
L. Kuai, J. Worden, S. S. Kulawik, S. A. Montzka, and J. Liu
Atmos. Meas. Tech., 7, 163–172, https://doi.org/10.5194/amt-7-163-2014, https://doi.org/10.5194/amt-7-163-2014, 2014
B. H. Kahn, F. W. Irion, V. T. Dang, E. M. Manning, S. L. Nasiri, C. M. Naud, J. M. Blaisdell, M. M. Schreier, Q. Yue, K. W. Bowman, E. J. Fetzer, G. C. Hulley, K. N. Liou, D. Lubin, S. C. Ou, J. Susskind, Y. Takano, B. Tian, and J. R. Worden
Atmos. Chem. Phys., 14, 399–426, https://doi.org/10.5194/acp-14-399-2014, https://doi.org/10.5194/acp-14-399-2014, 2014
J. Yoon, A. Pozzer, P. Hoor, D. Y. Chang, S. Beirle, T. Wagner, S. Schloegl, J. Lelieveld, and H. M. Worden
Atmos. Chem. Phys., 13, 11307–11316, https://doi.org/10.5194/acp-13-11307-2013, https://doi.org/10.5194/acp-13-11307-2013, 2013
J. Joiner, L. Guanter, R. Lindstrot, M. Voigt, A. P. Vasilkov, E. M. Middleton, K. F. Huemmrich, Y. Yoshida, and C. Frankenberg
Atmos. Meas. Tech., 6, 2803–2823, https://doi.org/10.5194/amt-6-2803-2013, https://doi.org/10.5194/amt-6-2803-2013, 2013
L. Mandrake, C. Frankenberg, C. W. O'Dell, G. Osterman, P. Wennberg, and D. Wunch
Atmos. Meas. Tech., 6, 2851–2864, https://doi.org/10.5194/amt-6-2851-2013, https://doi.org/10.5194/amt-6-2851-2013, 2013
H. He, J. W. Stehr, J. C. Hains, D. J. Krask, B. G. Doddridge, K. Y. Vinnikov, T. P. Canty, K. M. Hosley, R. J. Salawitch, H. M. Worden, and R. R. Dickerson
Atmos. Chem. Phys., 13, 7859–7874, https://doi.org/10.5194/acp-13-7859-2013, https://doi.org/10.5194/acp-13-7859-2013, 2013
M. J. Alvarado, V. H. Payne, E. J. Mlawer, G. Uymin, M. W. Shephard, K. E. Cady-Pereira, J. S. Delamere, and J.-L. Moncet
Atmos. Chem. Phys., 13, 6687–6711, https://doi.org/10.5194/acp-13-6687-2013, https://doi.org/10.5194/acp-13-6687-2013, 2013
H. M. Worden, D. P. Edwards, M. N. Deeter, D. Fu, S. S. Kulawik, J. R. Worden, and A. Arellano
Atmos. Meas. Tech., 6, 1633–1646, https://doi.org/10.5194/amt-6-1633-2013, https://doi.org/10.5194/amt-6-1633-2013, 2013
W. W. Verstraeten, K. F. Boersma, J. Zörner, M. A. F. Allaart, K. W. Bowman, and J. R. Worden
Atmos. Meas. Tech., 6, 1413–1423, https://doi.org/10.5194/amt-6-1413-2013, https://doi.org/10.5194/amt-6-1413-2013, 2013
K. W. Bowman, D. T. Shindell, H. M. Worden, J.F. Lamarque, P. J. Young, D. S. Stevenson, Z. Qu, M. de la Torre, D. Bergmann, P. J. Cameron-Smith, W. J. Collins, R. Doherty, S. B. Dalsøren, G. Faluvegi, G. Folberth, L. W. Horowitz, B. M. Josse, Y. H. Lee, I. A. MacKenzie, G. Myhre, T. Nagashima, V. Naik, D. A. Plummer, S. T. Rumbold, R. B. Skeie, S. A. Strode, K. Sudo, S. Szopa, A. Voulgarakis, G. Zeng, S. S. Kulawik, A. M. Aghedo, and J. R. Worden
Atmos. Chem. Phys., 13, 4057–4072, https://doi.org/10.5194/acp-13-4057-2013, https://doi.org/10.5194/acp-13-4057-2013, 2013
R. A. Scheepmaker, C. Frankenberg, A. Galli, A. Butz, H. Schrijver, N. M. Deutscher, D. Wunch, T. Warneke, S. Fally, and I. Aben
Atmos. Meas. Tech., 6, 879–894, https://doi.org/10.5194/amt-6-879-2013, https://doi.org/10.5194/amt-6-879-2013, 2013
D. Fu, J. R. Worden, X. Liu, S. S. Kulawik, K. W. Bowman, and V. Natraj
Atmos. Chem. Phys., 13, 3445–3462, https://doi.org/10.5194/acp-13-3445-2013, https://doi.org/10.5194/acp-13-3445-2013, 2013
D. S. Stevenson, P. J. Young, V. Naik, J.-F. Lamarque, D. T. Shindell, A. Voulgarakis, R. B. Skeie, S. B. Dalsoren, G. Myhre, T. K. Berntsen, G. A. Folberth, S. T. Rumbold, W. J. Collins, I. A. MacKenzie, R. M. Doherty, G. Zeng, T. P. C. van Noije, A. Strunk, D. Bergmann, P. Cameron-Smith, D. A. Plummer, S. A. Strode, L. Horowitz, Y. H. Lee, S. Szopa, K. Sudo, T. Nagashima, B. Josse, I. Cionni, M. Righi, V. Eyring, A. Conley, K. W. Bowman, O. Wild, and A. Archibald
Atmos. Chem. Phys., 13, 3063–3085, https://doi.org/10.5194/acp-13-3063-2013, https://doi.org/10.5194/acp-13-3063-2013, 2013
D. T. Shindell, O. Pechony, A. Voulgarakis, G. Faluvegi, L. Nazarenko, J.-F. Lamarque, K. Bowman, G. Milly, B. Kovari, R. Ruedy, and G. A. Schmidt
Atmos. Chem. Phys., 13, 2653–2689, https://doi.org/10.5194/acp-13-2653-2013, https://doi.org/10.5194/acp-13-2653-2013, 2013
P. J. Young, A. T. Archibald, K. W. Bowman, J.-F. Lamarque, V. Naik, D. S. Stevenson, S. Tilmes, A. Voulgarakis, O. Wild, D. Bergmann, P. Cameron-Smith, I. Cionni, W. J. Collins, S. B. Dalsøren, R. M. Doherty, V. Eyring, G. Faluvegi, L. W. Horowitz, B. Josse, Y. H. Lee, I. A. MacKenzie, T. Nagashima, D. A. Plummer, M. Righi, S. T. Rumbold, R. B. Skeie, D. T. Shindell, S. A. Strode, K. Sudo, S. Szopa, and G. Zeng
Atmos. Chem. Phys., 13, 2063–2090, https://doi.org/10.5194/acp-13-2063-2013, https://doi.org/10.5194/acp-13-2063-2013, 2013
C. Frankenberg, D. Wunch, G. Toon, C. Risi, R. Scheepmaker, J.-E. Lee, P. Wennberg, and J. Worden
Atmos. Meas. Tech., 6, 263–274, https://doi.org/10.5194/amt-6-263-2013, https://doi.org/10.5194/amt-6-263-2013, 2013
H. M. Worden, M. N. Deeter, C. Frankenberg, M. George, F. Nichitiu, J. Worden, I. Aben, K. W. Bowman, C. Clerbaux, P. F. Coheur, A. T. J. de Laat, R. Detweiler, J. R. Drummond, D. P. Edwards, J. C. Gille, D. Hurtmans, M. Luo, S. Martínez-Alonso, S. Massie, G. Pfister, and J. X. Warner
Atmos. Chem. Phys., 13, 837–850, https://doi.org/10.5194/acp-13-837-2013, https://doi.org/10.5194/acp-13-837-2013, 2013
M. Huang, G. R. Carmichael, T. Chai, R. B. Pierce, S. J. Oltmans, D. A. Jaffe, K. W. Bowman, A. Kaduwela, C. Cai, S. N. Spak, A. J. Weinheimer, L. G. Huey, and G. S. Diskin
Atmos. Chem. Phys., 13, 359–391, https://doi.org/10.5194/acp-13-359-2013, https://doi.org/10.5194/acp-13-359-2013, 2013
Related subject area
Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Biosphere–atmosphere related processes influence trace-gas and aerosol satellite–model biases
Estimation of diurnal emissions of CO2 from thermal power plants using spaceborne integrated path differential absorption (IPDA) lidar
Increase in carbon monoxide (CO) and aerosol optical depth (AOD) observed by satellites in the Northern Hemisphere over the summers of 2008–2023, linked to an increase in wildfires
Monitoring of total and off-road NOx emissions from Canadian oil sands surface mining using the Ozone Monitoring Instrument
Large reductions in satellite-derived and modelled European lower-tropospheric ozone during and after the COVID-19 pandemic (2020–2022)
Air quality trends and regimes in South Korea inferred from 2015–2023 surface and satellite observations
What can we learn about tropospheric OH from satellite observations of methane?
Identifying missing sources and reducing NOx emissions uncertainty over China using daily satellite data and a mass-conserving method
Feasibility of robust estimates of ozone production rates using a synergy of satellite observations, ground-based remote sensing, and models
Satellite Detection of NO2 Distributions and Comparison with Ground-Based Concentrations
Global Patterns and Trends in Ground-Level Ozone Chemical Formation Regimes from 1996 to 2022
Upper-tropospheric pollutants observed by MIPAS: geographic and seasonal variations
Comparing space-based to reported carbon monoxide emission estimates for Europe's iron and steel plants
Unleashing the potential of geostationary satellite observations in air quality forecasting through artificial intelligence techniques
Tropical upper-tropospheric trends in ozone and carbon monoxide (2005–2020): observational and model results
Global seasonal urban, industrial, and background NO2 estimated from TROPOMI satellite observations
Ground-based Tropospheric Ozone Measurements: Regional tropospheric ozone column trends from the TOAR-II/ HEGIFTOM homogenized datasets
Opposing trends in the peak and low ozone concentrations in eastern China: anthropogenic and meteorological influences
Quantifying biases in TROPESS AIRS, CrIS, and joint AIRS+OMI tropospheric ozone products using ozonesondes
Vertical profiles of global tropospheric nitrogen dioxide (NO2) obtained by cloud slicing the TROPOspheric Monitoring Instrument (TROPOMI)
Opinion: Beyond global means – novel space-based approaches to indirectly constrain the concentrations of and trends and variations in the tropospheric hydroxyl radical (OH)
Satellite-observed relationships between land cover, burned area, and atmospheric composition over the southern Amazon
Ammonia emission estimates using CrIS satellite observations over Europe
Insights into the long-term (2005–2021) spatiotemporal evolution of summer ozone production sensitivity in the Northern Hemisphere derived with the Ozone Monitoring Instrument (OMI)
Tropical tropospheric ozone distribution and trends from in situ and satellite data
Estimation of ground-level NO2 and its spatiotemporal variations in China using GEMS measurements and a nested machine learning model
Measurement Report: Diurnal Variability of NO2 and HCHO Lower Tropospheric Vertical Profiles in Southeastern Los Angeles
Investigation of the impact of satellite vertical sensitivity on long-term retrieved lower-tropospheric ozone trends
Quantifying the diurnal variation in atmospheric NO2 from Geostationary Environment Monitoring Spectrometer (GEMS) observations
State-wide California 2020 Carbon Dioxide Budget Estimated with OCO-2 and OCO-3 satellite data
Ammonia in the upper troposphere–lower stratosphere (UTLS): GLORIA airborne measurements for CAMS model evaluation in the Asian monsoon and in biomass burning plumes above the South Atlantic
A lightweight NO2-to-NOx conversion model for quantifying NOx emissions of point sources from NO2 satellite observations
Towards a sector-specific CO∕CO2 emission ratio: satellite-based observations of CO release from steel production in Germany
Monitoring European anthropogenic NOx emissions from space
Global carbon emission accounting: national-level assessment of wildfire CO2 emission – a case study of China
Pyrogenic HONO seen from space: insights from global IASI observations
First evaluation of the GEMS formaldehyde product against TROPOMI and ground-based column measurements during the in-orbit test period
High-resolution mapping of nitrogen oxide emissions in large US cities from TROPOMI retrievals of tropospheric nitrogen dioxide columns
Quantifying the tropospheric ozone radiative effect and its temporal evolution in the satellite era
A satellite chronology of plumes from the April 2021 eruption of La Soufrière, St Vincent
Investigation of spatial and temporal variability in lower tropospheric ozone from RAL Space UV–Vis satellite products
Two years of satellite-based carbon dioxide emission quantification at the world's largest coal-fired power plants
Tropical tropospheric ozone and carbon monoxide distributions: characteristics, origins, and control factors, as seen by IAGOS and IASI
Investigation of the summer 2018 European ozone air pollution episodes using novel satellite data and modelling
Bridging the spatial gaps of the Ammonia Monitoring Network using satellite ammonia measurements
A roadmap to estimating agricultural ammonia volatilization over Europe using satellite observations and simulation data
Investigation of meteorological conditions and BrO during ozone depletion events in Ny-Ålesund between 2010 and 2021
Quantification of carbon monoxide emissions from African cities using TROPOMI
Nitrogen oxides emissions from selected cities in North America, Europe, and East Asia observed by the TROPOspheric Monitoring Instrument (TROPOMI) before and after the COVID-19 pandemic
Remotely sensed and surface measurement- derived mass-conserving inversion of daily NOx emissions and inferred combustion technologies in energy-rich northern China
Emma Sands, Ruth M. Doherty, Fiona M. O'Connor, Richard J. Pope, James Weber, and Daniel P. Grosvenor
Atmos. Chem. Phys., 25, 7269–7297, https://doi.org/10.5194/acp-25-7269-2025, https://doi.org/10.5194/acp-25-7269-2025, 2025
Short summary
Short summary
We perform a detailed satellite–model comparison for isoprene, formaldehyde and aerosol optical depth in an Earth system model. We quantify the impacts of several processes that affect how biosphere–atmosphere interactions influence atmospheric chemistry and aerosols. Our findings highlight that the aerosol direct effect is sensitive to the processes studied. These results can inform future investigations of how the biosphere can affect atmospheric composition and climate.
Xuanye Zhang, Hailong Yang, Lingbing Bu, Zengchang Fan, Wei Xiao, Binglong Chen, Lu Zhang, Sihan Liu, Zhongting Wang, Jiqiao Liu, Weibiao Chen, and Xuhui Lee
Atmos. Chem. Phys., 25, 6725–6740, https://doi.org/10.5194/acp-25-6725-2025, https://doi.org/10.5194/acp-25-6725-2025, 2025
Short summary
Short summary
This study utilized the IPDA (integrated path differential absorption) lidar on board the DQ-1 satellite to monitor emissions from localized strong point sources and, for the first time, observed the diurnal variation in CO2 emissions from a high-latitude power plant. Overall, power plant CO2 emissions were largely consistent with local electricity consumption patterns, with most plants emitting less at night than during the day and with higher emissions in winter compared to spring and autumn.
Antoine Ehret, Solène Turquety, Maya George, Juliette Hadji-Lazaro, and Cathy Clerbaux
Atmos. Chem. Phys., 25, 6365–6394, https://doi.org/10.5194/acp-25-6365-2025, https://doi.org/10.5194/acp-25-6365-2025, 2025
Short summary
Short summary
Biomass burning has a considerable effect on the chemical composition of the atmosphere and climate, due to the emission of trace gases and aerosols. We examine the relationship between fire variability and the values of carbon monoxide and aerosol optical depth observed by satellites. The observed increase in wildfires has led to a corresponding rise in the mean and extreme values of carbon monoxide and aerosol optical depth during the summer and early autumn across the Northern Hemisphere.
Chris A. McLinden, Debora Griffin, Vitali Fioletov, Junhua Zhang, Enrico Dammers, Cristen Adams, Mallory Loria, Nickolay Krotkov, and Lok N. Lamsal
Atmos. Chem. Phys., 25, 6093–6120, https://doi.org/10.5194/acp-25-6093-2025, https://doi.org/10.5194/acp-25-6093-2025, 2025
Short summary
Short summary
The Ozone Monitoring Instrument (OMI) was used to understand the evolution of NOx emissions from the Canadian oil sands. OMI NO2 combined with winds and reported stack emissions found emissions from the heavy-hauler mine fleet have remained flat since 2005, whereas the total oil sands mined have more than doubled. This difference is a result of emissions standards that limit NOx emissions becoming more stringent over this period, confirming the efficacy of the policy enacting these standards.
Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Wuhu Feng, and Martyn P. Chipperfield
Atmos. Chem. Phys., 25, 4391–4401, https://doi.org/10.5194/acp-25-4391-2025, https://doi.org/10.5194/acp-25-4391-2025, 2025
Short summary
Short summary
Globally, lockdowns were implemented to limit the spread of COVID-19, leading to a decrease in emissions of key air pollutants. Here, we use novel satellite data and a chemistry model to investigate the impact of the pandemic on tropospheric ozone (O3), a key pollutant, in 2020. Overall, we found substantial decreases of up to 20 %, two-thirds of which came from emission reductions, while one-third was due to a decrease in the stratospheric O3 flux into the troposphere.
Yujin J. Oak, Daniel J. Jacob, Drew C. Pendergrass, Ruijun Dang, Nadia K. Colombi, Heesung Chong, Seoyoung Lee, Su Keun Kuk, and Jhoon Kim
Atmos. Chem. Phys., 25, 3233–3252, https://doi.org/10.5194/acp-25-3233-2025, https://doi.org/10.5194/acp-25-3233-2025, 2025
Short summary
Short summary
We analyze 2015–2023 air quality trends in South Korea using surface and satellite observations. Primary pollutants have decreased, consistent with emissions reductions. Surface O3 continues to increase and PM2.5 has decreased overall, but the nitrate component has not. O3 and PM2.5 nitrate depend on nonlinear responses from precursor emissions. Satellite data indicate a recent shift to NOx-sensitive O3 and nitrate formation, where further NOx reductions will benefit both O3 and PM2.5 pollution.
Elise Penn, Daniel J. Jacob, Zichong Chen, James D. East, Melissa P. Sulprizio, Lori Bruhwiler, Joannes D. Maasakkers, Hannah Nesser, Zhen Qu, Yuzhong Zhang, and John Worden
Atmos. Chem. Phys., 25, 2947–2965, https://doi.org/10.5194/acp-25-2947-2025, https://doi.org/10.5194/acp-25-2947-2025, 2025
Short summary
Short summary
The hydroxyl radical (OH) destroys many air pollutants, including methane. Global-mean OH cannot be directly measured, and thus it is inferred with the methyl chloroform (MCF) proxy. MCF is decreasing, and a replacement is needed. We use satellite observations of methane in two spectral ranges as a proxy for OH. We find shortwave infrared observations can characterize yearly OH and its seasonality but not the latitudinal distribution. Thermal infrared observations add little information.
Lingxiao Lu, Jason Blake Cohen, Kai Qin, Xiaolu Li, and Qin He
Atmos. Chem. Phys., 25, 2291–2309, https://doi.org/10.5194/acp-25-2291-2025, https://doi.org/10.5194/acp-25-2291-2025, 2025
Short summary
Short summary
This study applies an approach that assimilates NO2 vertical column densities from TROPOMI in a mass-conserving manner and inverts daily NOx emissions, presented over rapidly changing regions in China. Source attribution is quantified by the local thermodynamics of the combustion temperature (NOx/NO2). Emission results identify sources which do not exist in the a priori datasets, especially medium industrial sources located next to the Yangtze River.
Amir H. Souri, Gonzalo González Abad, Glenn M. Wolfe, Tijl Verhoelst, Corinne Vigouroux, Gaia Pinardi, Steven Compernolle, Bavo Langerock, Bryan N. Duncan, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2061–2086, https://doi.org/10.5194/acp-25-2061-2025, https://doi.org/10.5194/acp-25-2061-2025, 2025
Short summary
Short summary
We establish a simple yet robust relationship between ozone production rates and geophysical parameters obtained from several intensive atmospheric composition campaigns. We show that satellite remote sensing data can effectively constrain these parameters, enabling us to produce the first global maps of ozone production rates with unprecedented resolution.
Summer Joy Acker, Tracey Holloway, and Monica K. Harkey
EGUsphere, https://doi.org/10.5194/egusphere-2025-226, https://doi.org/10.5194/egusphere-2025-226, 2025
Short summary
Short summary
Nitrogen dioxide (NO2) is a harmful air pollutant linked to heart and lung diseases, regulated in the U.S. through annual and 1-hour standards. Most areas lack ground monitors, so satellites can help fill this gap. While past studies showed satellites capture annual NO2 patterns well, we assess their ability to reflect 1-hour pollution levels. We find satellites perform best farther from roads and in winter. TEMPO, a new satellite taking hourly measurements, improves the detection of higher NO2.
Yu Tian, Siyi Wang, and Xiaomeng Jin
EGUsphere, https://doi.org/10.5194/egusphere-2025-368, https://doi.org/10.5194/egusphere-2025-368, 2025
Short summary
Short summary
We leverage over two-decade ground-based ozone observations alongside space-based observations of ozone precursors (NO2 and formaldehyde) to study the long-term evolution in ozone chemical regimes across global source regions. We find a global trend towards NOx-limited regimes, supported by increasing satellite-based HCHO/NO2 and a diminishing ozone weekend effect.
Norbert Glatthor, Gabriele P. Stiller, Thomas von Clarmann, Bernd Funke, Sylvia Kellmann, and Andrea Linden
Atmos. Chem. Phys., 25, 1175–1208, https://doi.org/10.5194/acp-25-1175-2025, https://doi.org/10.5194/acp-25-1175-2025, 2025
Short summary
Short summary
We present global upper-tropospheric distributions of the pollutants HCN, CO, C2H2, C2H6, PAN, and HCOOH, observed between 2002 and 2012 by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on the Environmental Satellite (Envisat). By comparing the spatial distributions of their volume mixing ratios and by global correlation and regression analyses, we draw conclusions on their sources, such as biomass burning, anthropogenic sources, and biogenic release.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, Ivar R. van der Velde, and Ilse Aben
Atmos. Chem. Phys., 25, 555–574, https://doi.org/10.5194/acp-25-555-2025, https://doi.org/10.5194/acp-25-555-2025, 2025
Short summary
Short summary
The production of steel coincides with large emissions of greenhouse gases and air pollutants including carbon monoxide. European facilities are required to report their emissions, which are estimated using a variety of methods. We evaluate these estimates using carbon monoxide concentrations measured via satellite. We find generally good agreement between our values and those reported but also identify some uncertainties, showing that satellites can provide insights into these emissions.
Chengxin Zhang, Xinhan Niu, Hongyu Wu, Zhipeng Ding, Ka Lok Chan, Jhoon Kim, Thomas Wagner, and Cheng Liu
Atmos. Chem. Phys., 25, 759–770, https://doi.org/10.5194/acp-25-759-2025, https://doi.org/10.5194/acp-25-759-2025, 2025
Short summary
Short summary
This research utilizes hourly air pollution observations from the world’s first geostationary satellite to develop a spatiotemporal neural network model for full-coverage surface NO2 pollution prediction over the next 24 hours, achieving outstanding forecasting performance and efficacy. These results highlight the profound impact of geostationary satellite observations in advancing air quality forecasting models, thereby contributing to future models for health exposure to air pollution.
Lucien Froidevaux, Douglas E. Kinnison, Benjamin Gaubert, Michael J. Schwartz, Nathaniel J. Livesey, William G. Read, Charles G. Bardeen, Jerry R. Ziemke, and Ryan A. Fuller
Atmos. Chem. Phys., 25, 597–624, https://doi.org/10.5194/acp-25-597-2025, https://doi.org/10.5194/acp-25-597-2025, 2025
Short summary
Short summary
We compare observed changes in ozone (O3) and carbon monoxide (CO) in the tropical upper troposphere (10–15 km altitude) for 2005–2020 to predictions from model simulations that track the evolution of natural and industrial emissions transported to this region. An increasing trend in measured upper-tropospheric O3 is well matched by model trends. We find that changes in modeled industrial CO surface emissions lead to better model agreement with observed slight decreases in upper-tropospheric CO.
Vitali Fioletov, Chris A. McLinden, Debora Griffin, Xiaoyi Zhao, and Henk Eskes
Atmos. Chem. Phys., 25, 575–596, https://doi.org/10.5194/acp-25-575-2025, https://doi.org/10.5194/acp-25-575-2025, 2025
Short summary
Short summary
Satellite data were used to estimate urban per capita emissions for 261 major cities worldwide. Three components in tropospheric NO2 data (background NO2, NO2 from urban sources, and NO2 from industrial point sources) were isolated, and then each of these components was analyzed separately. The largest per capita emissions were found in the Middle East and the smallest in India and southern Africa. Urban weekend emissions are 20 %–50 % less than workday emissions for all regions except China.
Roeland Van Malderen, Zhou Zang, Kai-Lan Chang, Robin Björklund, Owen R. Cooper, Jane Liu, Eliane Maillard Barras, Corinne Vigouroux, Irina Petropavlovskikh, Thierry Leblanc, Valérie Thouret, Pawel Wolff, Peter Effertz, Audrey Gaudel, David W. Tarasick, Herman G. J. Smit, Anne M. Thompson, Ryan M. Stauffer, Debra E. Kollonige, Deniz Poyraz, Gérard Ancellet, Marie-Renée De Backer, Matthias M. Frey, James W. Hannigan, José L. Hernandez, Bryan J. Johnson, Nicholas Jones, Rigel Kivi, Emmanuel Mahieu, Isamu Morino, Glen McConville, Katrin Müller, Isao Murata, Justus Notholt, Ankie Piters, Maxime Prignon, Richard Querel, Vincenzo Rizi, Dan Smale, Wolfgang Steinbrecht, Kimberly Strong, and Ralf Sussmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-3745, https://doi.org/10.5194/egusphere-2024-3745, 2025
Short summary
Short summary
Tropospheric ozone is an important greenhouse gas and an air pollutant, whose distribution and time variability is mainly governed by anthropogenic emissions and dynamics. In this paper, we assess regional trends of tropospheric ozone column amounts, based on two different approaches of merging or synthesizing ground-based observations and their trends within specific regions. Our findings clearly demonstrate regional trend differences, but also consistently higher pre- than post-COVID trends.
Zhuang Wang, Chune Shi, Hao Zhang, Xianguang Ji, Yizhi Zhu, Congzi Xia, Xiaoyun Sun, Xinfeng Lin, Shaowei Yan, Suyao Wang, Yuan Zhou, Chengzhi Xing, Yujia Chen, and Cheng Liu
Atmos. Chem. Phys., 25, 347–366, https://doi.org/10.5194/acp-25-347-2025, https://doi.org/10.5194/acp-25-347-2025, 2025
Short summary
Short summary
This study attempts to explain the surface ozone background and typical and peak trends in eastern China by combining a large number of ground-based and satellite observations. We found diametrically opposed trends in peak (decreasing) and low (increasing) ozone concentrations. Anthropogenic emissions primarily drive trends in low and peak ozone concentrations in eastern China, though meteorological effects also play a role.
Elyse A. Pennington, Gregory B. Osterman, Vivienne H. Payne, Kazuyuki Miyazaki, Kevin W. Bowman, and Jessica L. Neu
EGUsphere, https://doi.org/10.5194/egusphere-2024-3701, https://doi.org/10.5194/egusphere-2024-3701, 2024
Short summary
Short summary
Tropospheric ozone is a harmful pollutant & powerful greenhouse gas. For satellite products to accurately quantify trends in tropospheric ozone, they must have low bias compared to a reliable source of data. This study compares 3 TROPESS satellite products – CrIS, AIRS, & AIRSOMI – to ozonesonde data. They have low global measurement bias & thus can be used to detect global tropospheric ozone trends, but the measurement bias should be considered in certain regions & time periods.
Rebekah P. Horner, Eloise A. Marais, Nana Wei, Robert G. Ryan, and Viral Shah
Atmos. Chem. Phys., 24, 13047–13064, https://doi.org/10.5194/acp-24-13047-2024, https://doi.org/10.5194/acp-24-13047-2024, 2024
Short summary
Short summary
Nitrogen oxides (NOx ≡ NO + NO2) affect tropospheric ozone and the hydroxyl radical, influencing climate and atmospheric oxidation. To address the lack of routine observations of NOx, we cloud slice satellite observations of NO2 to derive a new dataset of global vertical profiles of NO2. We evaluate our data against in situ aircraft observations and use these data to critique the contemporary understanding of tropospheric NOx, as simulated by the GEOS-Chem model.
Bryan N. Duncan, Daniel C. Anderson, Arlene M. Fiore, Joanna Joiner, Nickolay A. Krotkov, Can Li, Dylan B. Millet, Julie M. Nicely, Luke D. Oman, Jason M. St. Clair, Joshua D. Shutter, Amir H. Souri, Sarah A. Strode, Brad Weir, Glenn M. Wolfe, Helen M. Worden, and Qindan Zhu
Atmos. Chem. Phys., 24, 13001–13023, https://doi.org/10.5194/acp-24-13001-2024, https://doi.org/10.5194/acp-24-13001-2024, 2024
Short summary
Short summary
Trace gases emitted to or formed within the atmosphere may be chemically or physically removed from the atmosphere. One trace gas, the hydroxyl radical (OH), is responsible for initiating the chemical removal of many trace gases, including some greenhouse gases. Despite its importance, scientists have not been able to adequately measure OH. In this opinion piece, we discuss promising new methods to indirectly constrain OH using satellite data of trace gases that control the abundance of OH.
Emma Sands, Richard J. Pope, Ruth M. Doherty, Fiona M. O'Connor, Chris Wilson, and Hugh Pumphrey
Atmos. Chem. Phys., 24, 11081–11102, https://doi.org/10.5194/acp-24-11081-2024, https://doi.org/10.5194/acp-24-11081-2024, 2024
Short summary
Short summary
Changes in vegetation alongside biomass burning impact regional atmospheric composition and air quality. Using satellite remote sensing, we find a clear linear relationship between forest cover and isoprene and a pronounced non-linear relationship between burned area and nitrogen dioxide in the southern Amazon, a region of substantial deforestation. These quantified relationships can be used for model evaluation and further exploration of biosphere-atmosphere interactions in Earth System Models.
Jieying Ding, Ronald van der A, Henk Eskes, Enrico Dammers, Mark Shephard, Roy Wichink Kruit, Marc Guevara, and Leonor Tarrason
Atmos. Chem. Phys., 24, 10583–10599, https://doi.org/10.5194/acp-24-10583-2024, https://doi.org/10.5194/acp-24-10583-2024, 2024
Short summary
Short summary
Here we applied the existing Daily Emissions Constrained by Satellite Observations (DECSO) inversion algorithm to NH3 observations from the CrIS satellite instrument to estimate NH3 emissions. As NH3 in the atmosphere is influenced by NOx, we implemented DECSO to estimate NOx and NH3 emissions simultaneously. The emissions are derived over Europe for 2020 at a spatial resolution of 0.2° using daily observations from CrIS and TROPOMI. Results are compared to bottom-up emission inventories.
Matthew S. Johnson, Sajeev Philip, Scott Meech, Rajesh Kumar, Meytar Sorek-Hamer, Yoichi P. Shiga, and Jia Jung
Atmos. Chem. Phys., 24, 10363–10384, https://doi.org/10.5194/acp-24-10363-2024, https://doi.org/10.5194/acp-24-10363-2024, 2024
Short summary
Short summary
Satellites, like the Ozone Monitoring Instrument (OMI), retrieve proxy species of ozone (O3) formation (formaldehyde and nitrogen dioxide) and the ratios (FNRs) which can define O3 production sensitivity regimes. Here we investigate trends of OMI FNRs from 2005 to 2021, and they have increased in major cities, suggesting a transition from radical- to NOx-limited regimes. OMI also observed the impact of reduced emissions during the 2020 COVID-19 lockdown that resulted in increased FNRs.
Audrey Gaudel, Ilann Bourgeois, Meng Li, Kai-Lan Chang, Jerald Ziemke, Bastien Sauvage, Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Nadia Smith, Daan Hubert, Arno Keppens, Juan Cuesta, Klaus-Peter Heue, Pepijn Veefkind, Kenneth Aikin, Jeff Peischl, Chelsea R. Thompson, Thomas B. Ryerson, Gregory J. Frost, Brian C. McDonald, and Owen R. Cooper
Atmos. Chem. Phys., 24, 9975–10000, https://doi.org/10.5194/acp-24-9975-2024, https://doi.org/10.5194/acp-24-9975-2024, 2024
Short summary
Short summary
The study examines tropical tropospheric ozone changes. In situ data from 1994–2019 display increased ozone, notably over India, Southeast Asia, and Malaysia and Indonesia. Sparse in situ data limit trend detection for the 15-year period. In situ and satellite data, with limited sampling, struggle to consistently detect trends. Continuous observations are vital over the tropical Pacific Ocean, Indian Ocean, western Africa, and South Asia for accurate ozone trend estimation in these regions.
Naveed Ahmad, Changqing Lin, Alexis K. H. Lau, Jhoon Kim, Tianshu Zhang, Fangqun Yu, Chengcai Li, Ying Li, Jimmy C. H. Fung, and Xiang Qian Lao
Atmos. Chem. Phys., 24, 9645–9665, https://doi.org/10.5194/acp-24-9645-2024, https://doi.org/10.5194/acp-24-9645-2024, 2024
Short summary
Short summary
This study developed a nested machine learning model to convert the GEMS NO2 column measurements into ground-level concentrations across China. The model directly incorporates the NO2 mixing height (NMH) into the methodological framework. The study underscores the importance of considering NMH when estimating ground-level NO2 from satellite column measurements and highlights the significant advantages of new-generation geostationary satellites in air quality monitoring.
Peter Peterson, Lisa Hernandez, Leslie Tanaka, and Alejandro Dunnick
EGUsphere, https://doi.org/10.5194/egusphere-2024-1460, https://doi.org/10.5194/egusphere-2024-1460, 2024
Short summary
Short summary
This work uses spectroscopy to examine the vertical distribution of nitrogen dioxide and formaldehyde in southeastern Los Angeles, USA, a region heavily impacted by ozone pollution. We examine how both the amount and vertical profile of the two species varies throughout the day, finding that differences between the two species impact the utilization of satellite-based measurements to diagnose ozone production chemistry and these impacts are variable depending on the time of day.
Richard J. Pope, Fiona M. O'Connor, Mohit Dalvi, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Brice Barret, Eric Le Flochmoen, Anne Boynard, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, Catherine Wespes, and Richard Rigby
Atmos. Chem. Phys., 24, 9177–9195, https://doi.org/10.5194/acp-24-9177-2024, https://doi.org/10.5194/acp-24-9177-2024, 2024
Short summary
Short summary
Ozone is a potent air pollutant in the lower troposphere, with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that, in North America, Europe, and East Asia, the underlying trends are typically small with large uncertainties.
David P. Edwards, Sara Martínez-Alonso, Duseong S. Jo, Ivan Ortega, Louisa K. Emmons, John J. Orlando, Helen M. Worden, Jhoon Kim, Hanlim Lee, Junsung Park, and Hyunkee Hong
Atmos. Chem. Phys., 24, 8943–8961, https://doi.org/10.5194/acp-24-8943-2024, https://doi.org/10.5194/acp-24-8943-2024, 2024
Short summary
Short summary
Until recently, satellite observations of atmospheric pollutants at any location could only be obtained once a day. New geostationary satellites stare at a region of the Earth to make hourly measurements, and the Geostationary Environment Monitoring Spectrometer is the first looking at Asia. These data and model simulations show how the change seen for one important pollutant that determines air quality depends on a combination of pollution emissions, atmospheric chemistry, and meteorology.
Matthew S. Johnson, Sofia D. Hamilton, Seongeun Jeong, Yuyan Cui, Dien Wu, Alex Turner, and Marc Fischer
EGUsphere, https://doi.org/10.5194/egusphere-2024-2152, https://doi.org/10.5194/egusphere-2024-2152, 2024
Short summary
Short summary
Satellites, such as NASA’s Orbiting Carbon Observatory-2 and -3 (OCO-2/3), retrieve carbon dioxide (CO2) concentrations which provide vital information for estimating surface CO2 emissions. Here we investigate the ability of OCO-2/3 retrievals to constrain CO2 emissions for the state of California for the major emission sectors (i.e., fossil fuels, net ecosystem exchange, wildfire).
Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Vincent Huijnen, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Martin Riese, Björn-Martin Sinnhuber, Jörn Ungermann, Gerald Wetzel, and Wolfgang Woiwode
Atmos. Chem. Phys., 24, 8125–8138, https://doi.org/10.5194/acp-24-8125-2024, https://doi.org/10.5194/acp-24-8125-2024, 2024
Short summary
Short summary
We present airborne infrared limb sounding GLORIA measurements of ammonia (NH3) in the upper troposphere of air masses within the Asian monsoon and of those connected with biomass burning. Comparing CAMS (Copernicus Atmosphere Monitoring Service) model data, we find that the model reproduces the measured enhanced NH3 within the Asian monsoon well but not that within biomass burning plumes, where no enhanced NH3 is measured in the upper troposphere but considerable amounts are simulated by CAMS.
Sandro Meier, Erik F. M. Koene, Maarten Krol, Dominik Brunner, Alexander Damm, and Gerrit Kuhlmann
Atmos. Chem. Phys., 24, 7667–7686, https://doi.org/10.5194/acp-24-7667-2024, https://doi.org/10.5194/acp-24-7667-2024, 2024
Short summary
Short summary
Nitrogen oxides (NOx = NO + NO2) are important air pollutants. This study addresses the challenge of accurately estimating NOx emissions from NO2 satellite observations. We develop a realistic model to convert NO2 to NOx by using simulated plumes from various power plants. We apply the model to satellite NO2 observations, significantly reducing biases in estimated NOx emissions. The study highlights the potential for a consistent, high-resolution estimation of NOx emissions using satellite data.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Chem. Phys., 24, 7609–7621, https://doi.org/10.5194/acp-24-7609-2024, https://doi.org/10.5194/acp-24-7609-2024, 2024
Short summary
Short summary
Large quantities of CO and CO2 are emitted during conventional steel production. As satellite-based estimates of CO2 emissions at the facility level are challenging, co-emitted CO can indicate the carbon footprint of steel plants. We estimate CO emissions for German steelworks and use CO2 emissions from emissions trading data to derive a sector-specific CO/CO2 emission ratio for the steel industry; it is a prerequisite to use CO as a proxy for CO2 emissions from similar steel production sites.
Ronald J. van der A, Jieying Ding, and Henk Eskes
Atmos. Chem. Phys., 24, 7523–7534, https://doi.org/10.5194/acp-24-7523-2024, https://doi.org/10.5194/acp-24-7523-2024, 2024
Short summary
Short summary
Using observations of the Sentinel-5P satellite and the latest version of the inversion algorithm DECSO, anthropogenic NOx emissions are derived for Europe for the years 2019–2022 with a spatial resolution of 0.2°. The results are compared with European emissions of the Copernicus Atmosphere Monitoring Service.
Xuehong Gong, Zeyu Liu, Jie Tian, Qiyuan Wang, Guohui Li, Zhisheng An, and Yongming Han
EGUsphere, https://doi.org/10.5194/egusphere-2024-1684, https://doi.org/10.5194/egusphere-2024-1684, 2024
Short summary
Short summary
Our study analyzed CO2 emissions from wildfires in China from 2001 to 2022. Cropland and forest fires contributed the most, while grassland fires were the least. Emissions from forest and shrub fires decreased significantly, while cropland fires increased. The highest emissions were in Heilongjiang and Inner Mongolia. China's effective policy management has reduced wildfire-related CO2 emissions, aiding global climate change efforts.
Bruno Franco, Lieven Clarisse, Nicolas Theys, Juliette Hadji-Lazaro, Cathy Clerbaux, and Pierre Coheur
Atmos. Chem. Phys., 24, 4973–5007, https://doi.org/10.5194/acp-24-4973-2024, https://doi.org/10.5194/acp-24-4973-2024, 2024
Short summary
Short summary
Using IASI global infrared measurements, we retrieve nitrous acid (HONO) in fire plumes from space. We detect large enhancements of pyrogenic HONO worldwide, especially from intense wildfires at Northern Hemisphere mid- and high latitudes. Predominance of IASI nighttime over daytime measurements sheds light on HONO's extended lifetime and secondary formation during long-range transport in smoke plumes. Our findings deepen the understanding of atmospheric HONO, crucial for air quality assessment.
Gitaek T. Lee, Rokjin J. Park, Hyeong-Ahn Kwon, Eunjo S. Ha, Sieun D. Lee, Seunga Shin, Myoung-Hwan Ahn, Mina Kang, Yong-Sang Choi, Gyuyeon Kim, Dong-Won Lee, Deok-Rae Kim, Hyunkee Hong, Bavo Langerock, Corinne Vigouroux, Christophe Lerot, Francois Hendrick, Gaia Pinardi, Isabelle De Smedt, Michel Van Roozendael, Pucai Wang, Heesung Chong, Yeseul Cho, and Jhoon Kim
Atmos. Chem. Phys., 24, 4733–4749, https://doi.org/10.5194/acp-24-4733-2024, https://doi.org/10.5194/acp-24-4733-2024, 2024
Short summary
Short summary
This study evaluates the Geostationary Environment Monitoring Spectrometer (GEMS) HCHO product by comparing its vertical column densities (VCDs) with those of TROPOMI and ground-based observations. Based on some sensitivity tests, obtaining radiance references under clear-sky conditions significantly improves HCHO retrieval quality. GEMS HCHO VCDs captured seasonal and diurnal variations well during the first year of observation, showing consistency with TROPOMI and ground-based observations.
Fei Liu, Steffen Beirle, Joanna Joiner, Sungyeon Choi, Zhining Tao, K. Emma Knowland, Steven J. Smith, Daniel Q. Tong, Siqi Ma, Zachary T. Fasnacht, and Thomas Wagner
Atmos. Chem. Phys., 24, 3717–3728, https://doi.org/10.5194/acp-24-3717-2024, https://doi.org/10.5194/acp-24-3717-2024, 2024
Short summary
Short summary
Using satellite data, we developed a coupled method independent of the chemical transport model to map NOx emissions across US cities. After validating our technique with synthetic data, we charted NOx emissions from 2018–2021 in 39 cities. Our results closely matched EPA estimates but also highlighted some inconsistencies in both magnitude and spatial distribution. This research can help refine strategies for monitoring and managing air quality.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
Short summary
Short summary
Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Isabelle A. Taylor, Roy G. Grainger, Andrew T. Prata, Simon R. Proud, Tamsin A. Mather, and David M. Pyle
Atmos. Chem. Phys., 23, 15209–15234, https://doi.org/10.5194/acp-23-15209-2023, https://doi.org/10.5194/acp-23-15209-2023, 2023
Short summary
Short summary
This study looks at sulfur dioxide (SO2) and ash emissions from the April 2021 eruption of La Soufrière on St Vincent. Using satellite data, 35 eruptive events were identified. Satellite data were used to track SO2 as it was transported around the globe. The majority of SO2 was emitted into the upper troposphere and lower stratosphere. Similarities with the 1979 eruption of La Soufrière highlight the value of studying these eruptions to be better prepared for future eruptions.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
Short summary
Short summary
Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Daniel H. Cusworth, Andrew K. Thorpe, Charles E. Miller, Alana K. Ayasse, Ralph Jiorle, Riley M. Duren, Ray Nassar, Jon-Paul Mastrogiacomo, and Robert R. Nelson
Atmos. Chem. Phys., 23, 14577–14591, https://doi.org/10.5194/acp-23-14577-2023, https://doi.org/10.5194/acp-23-14577-2023, 2023
Short summary
Short summary
Carbon dioxide (CO2) emissions from combustion sources are uncertain in many places across the globe. Satellites have the ability to detect and quantify emissions from large CO2 point sources, including coal-fired power plants. In this study, we tasked two satellites to routinely observe CO2 emissions at 30 coal-fired power plants between 2021 and 2022. These results present the largest dataset of space-based CO2 emission estimates to date.
Maria Tsivlidou, Bastien Sauvage, Yasmine Bennouna, Romain Blot, Damien Boulanger, Hannah Clark, Eric Le Flochmoën, Philippe Nédélec, Valérie Thouret, Pawel Wolff, and Brice Barret
Atmos. Chem. Phys., 23, 14039–14063, https://doi.org/10.5194/acp-23-14039-2023, https://doi.org/10.5194/acp-23-14039-2023, 2023
Short summary
Short summary
The tropics are a region where the ozone increase has been most apparent since 1980 and where observations are sparse. Using aircraft, satellite, and model data, we document the characteristics of tropospheric ozone and CO over the whole tropics for the last 2 decades. We explore the origin of the observed CO anomalies and investigate transport processes driving the tropical CO and O3 distribution. Our study highlights the importance of anthropogenic emissions, mostly over the northern tropics.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
Short summary
Short summary
In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Rui Wang, Da Pan, Xuehui Guo, Kang Sun, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, Cathy Clerbaux, Melissa Puchalski, and Mark A. Zondlo
Atmos. Chem. Phys., 23, 13217–13234, https://doi.org/10.5194/acp-23-13217-2023, https://doi.org/10.5194/acp-23-13217-2023, 2023
Short summary
Short summary
Ammonia (NH3) is a key precursor for fine particulate matter (PM2.5) and a primary form of reactive nitrogen, yet it has sparse ground measurements. We perform the first comprehensive comparison between ground observations and satellite retrievals in the US, demonstrating that satellite NH3 data can help fill spatial gaps in the current ground monitoring networks. Trend analyses using both datasets highlight increasing NH3 trends across the US, including the NH3 hotspots and urban areas.
Rimal Abeed, Camille Viatte, William C. Porter, Nikolaos Evangeliou, Cathy Clerbaux, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, and Sarah Safieddine
Atmos. Chem. Phys., 23, 12505–12523, https://doi.org/10.5194/acp-23-12505-2023, https://doi.org/10.5194/acp-23-12505-2023, 2023
Short summary
Short summary
Ammonia emissions from agricultural activities will inevitably increase with the rise in population. We use a variety of datasets (satellite, reanalysis, and model simulation) to calculate the first regional map of ammonia emission potential during the start of the growing season in Europe. We then apply our developed method using a climate model to show the effect of the temperature increase on future ammonia columns under two possible climate scenarios.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
Short summary
Short summary
During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, and Ilse Aben
Atmos. Chem. Phys., 23, 8899–8919, https://doi.org/10.5194/acp-23-8899-2023, https://doi.org/10.5194/acp-23-8899-2023, 2023
Short summary
Short summary
We present a fast method to evaluate carbon monoxide emissions from cities in Africa. Carbon monoxide is important for climate change in an indirect way, as it is linked to ozone, methane, and carbon dioxide. Our measurements are made with a satellite that sees the entire globe every single day. This means that we can check from space whether the current knowledge of emission rates is up to date. We make the comparison and show that the emission rates in northern Africa are underestimated.
Chantelle R. Lonsdale and Kang Sun
Atmos. Chem. Phys., 23, 8727–8748, https://doi.org/10.5194/acp-23-8727-2023, https://doi.org/10.5194/acp-23-8727-2023, 2023
Short summary
Short summary
The COVID-19 pandemic, which was caused by the SARS-CoV-2 virus, emerged in 2019, and its still evolving variants have resulted in unprecedented shifts in human activities and anthropogenic emissions into the Earth's atmosphere. We present monthly nitrogen oxide emissions over three major continents from May 2018 to January 2023 to capture variations before and after the COVID-19 pandemic. We focus on a diverse collection of 54 cities to quantify the post-COVID-19 perturbations.
Xiaolu Li, Jason Blake Cohen, Kai Qin, Hong Geng, Xiaohui Wu, Liling Wu, Chengli Yang, Rui Zhang, and Liqin Zhang
Atmos. Chem. Phys., 23, 8001–8019, https://doi.org/10.5194/acp-23-8001-2023, https://doi.org/10.5194/acp-23-8001-2023, 2023
Short summary
Short summary
Remotely sensed NO2 and surface NOx are combined with a mathematical method to estimate daily NOx emissions. The results identify new sources and improve existing estimates. The estimation is driven by three flexible factors: thermodynamics of combustion, chemical loss, and atmospheric transport. The thermodynamic term separates power, iron, and cement from coking, boilers, and aluminum. This work finds three causes for the extremes: emissions, UV radiation, and transport.
Cited articles
Andreae, M. O. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Global Biogeochem. Cycles, 15, 955–966, 2001.
Beer, R., Glavich, T. A. and Rider, D. M.: Tropospheric emission spectrometer for the Earth Observing System's Aura satellite, Appl. Optics, 40, 2356–2367, 2001.
Bey, I., Jacob, D., Yantosca, R., Logan, J., Field, B., Fiore, A., Li, Q., Liu, H. Y., Mickley, L., and Schultz, M. G.: Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation, J. Geophys. Res.-Atmos., 106, 23073–23095, 2001.
Bloom, A. A., Palmer, P. I., Fraser, A., Reay, D. S. and Frankenberg, C.: Large-Scale Controls of Methanogenesis Inferred from Methane and Gravity Spaceborne Data, Science, 327, 322–325, https://doi.org/10.1126/science.1175176, 2010.
Bousquet, P., Ciais, P., Miller, J. B., Dlugokencky, E. J., Hauglustaine, D. A., Prigent, C., Van Der Werf, G. R., Peylin, P., Brunke, E.-G., Carouge, C., Langenfelds, R. L., Lathière, J., Papa, F., Ramonet, M., Schmidt, M., Steele, L. P., Tyler, S. C., and White, J.: Contribution of anthropogenic and natural sources to atmospheric methane variability, Nature, 443, 439–443, https://doi.org/10.1038/nature05132, 2006.
Bousquet, P., Ringeval, B., Pison, I., Dlugokencky, E. J., Brunke, E.-G., Carouge, C., Chevallier, F., Fortems-Cheiney, A., Frankenberg, C., Hauglustaine, D. A., Krummel, P. B., Langenfelds, R. L., Ramonet, M., Schmidt, M., Steele, L. P., Szopa, S., Yver, C., Viovy, N., and Ciais, P.: Source attribution of the changes in atmospheric methane for 2006–2008, Atmos. Chem. Phys., 11, 3689–3700, https://doi.org/10.5194/acp-11-3689-2011, 2011.
Bowman, K. W., Rodgers, C. D., Kulawik, S. S., Worden, J., Sarkissian, E., Osterman, G., Steck, T., Lou, M., Eldering, A., Shephard, M., Worden, H., Lampel, M., Clough, S., Brown, P., Rinsland, C., Gunson, M., and Beer, R.: Tropospheric Emission Spectrometer: Retrieval Method and Error Analysis, IEEE T. Geosci. Remote Sens., 44, 1297–1307, https://doi.org/10.1109/TGRS.2006.871234, 2006.
Christian, T. J.: Comprehensive laboratory measurements of biomass-burning emissions: 1. Emissions from Indonesian, African, and other fuels, J. Geophys. Res., 108, 4719, https://doi.org/10.1029/2003JD003704, 2003.
Clough, S. A., Shephard, M. W., Worden, J., Brown, P. D., Worden, H. M., Luo, M., Rodgers, C. D., Rinsland, C. P., Goldman, A. and Brown, L.: Forward model and Jacobians for tropospheric emission spectrometer retrievals, IEEE T. Geosci. Remote Sens., 44, 1308–1323, 2006.
Crevoisier, C., Nobileau, D., Fiore, A. M., Armante, R., Chédin, A., and Scott, N. A.: Tropospheric methane in the tropics – first year from IASI hyperspectral infrared observations, Atmos. Chem. Phys., 9, 6337–6350, https://doi.org/10.5194/acp-9-6337-2009, 2009
Deeter, M. N., Worden, H. M., Gille, J. C., Edwards, D. P., Mao, D., and Drummond, J. R.: MOPITT multispectral CO retrievals: Origins and effects of geophysical radiance errors, J. Geophys. Res., 116, D15303, https://doi.org/10.1029/2011JD015703, 2011.
Deeter, M. N., Worden, H. M., Edwards, D. P., Gille, J. C., and Andrews, A. E.: Evaluation of MOPITT retrievals of lower-tropospheric carbon monoxide over the United States, J. Geophys. Res., 117, D13306, https://doi.org/10.1029/2012JD017553, 2012.
Denman, K. L., Brasseur, G., Chidthaisong, A., Ciais, P., Cox, P. M., Dickinson, R. E., Hauglustaine, D., Heinze, C., Holland, E., Jacob, D.,, Lohmann, U., Ramachandran, S., da Silva Dias, P. L., Wofsy, S. C., and Zhang X.: Couplings Between Changes in the Climate System and Biogeochemistry, in: Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 2007.
Dlugokencky, E. J., Bruhwiler, L., White, J. W. C., Emmons, L. K., Novelli, P. C., Montzka, S. A., Masarie, K. A., Lang, P. M., Crotwell, A. M., Miller, J. B., and Gatti, L. V.: Observational constraints on recent increases in the atmospheric CH 4burden, Geophys. Res. Lett., 36, L18803, https://doi.org/10.1029/2009GL039780, 2009.
Dlugokencky, E. J., Nisbet, E. G., Fisher, R., and Lowry, D.: Global atmospheric methane: budget, changes and dangers, Philos. T. Roy. Soc. A, 369, 2058–2072, https://doi.org/10.1098/rsta.2010.0341, 2011.
Edwards, D. P., Pétron, G., Novelli, P. C., Emmons, L. K., Gille, J. C., and Drummond, J. R.: Southern Hemisphere carbon monoxide interannual variability observed by Terra/Measurement of Pollution in the Troposphere (MOPITT), J. Geophys. Res., 111, D16303, https://doi.org/10.1029/2006JD007079, 2006.
Eldering, A., Kulawik, S. S., Worden, J., Bowman, K., and Osterman, G.: Implementation of cloud retrievals for TES atmospheric retrievals: 2. Characterization of cloud top pressure and effective optical depth retrievals, J. Geophys. Res., 113, D16S37, https://doi.org/10.1029/2007JD008858, 2008.
Forster, P., Ramaswamy, V., Artaxo, P., Berntsen, T., Betts, R., Fahey, D. W., Haywood, J., Lean, J., Lowe, D. C., Myhre, G., Nganga, J., Prinn, R., Raga, G., Schulz, M., and Van Dorland, R.: Changes in Atmospheric Constituents and in Radiative Forcing, in: Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 2007
Frankenberg, C., Meirink, J., Van Weele, M., Platt, U., and Wagner, T.: Assessing methane emissions from global space-borne observations, Science, 308, 1010–1014, https://doi.org/10.1126/science.1106644, 2005.
Frankenberg, C., Aben, I., Bergamaschi, P., Dlugokencky, E. J., van Hees, R., Houweling, S., van der Meer, P., Snel, R., and Tol, P.: Global column-averaged methane mixing ratios from 2003 to 2009 as derived from SCIAMACHY: Trends and variability, J. Geophys. Res., 116, D04302, https://doi.org/10.1029/2010JD014849, 2011.
Fung, I., Prather, M., John, J., Lerner, J., and Matthews, E.: Three-dimensional model synthesis of the global methane cycle, J. Geophys. Res., 96, 13033–13065, 1991.
Gonzi, S. and Palmer, P. I.: Vertical transport of surface fire emissions observed from space, J. Geophys. Res., 115, D02306, https://doi.org/10.1029/2009JD012053, 2010.
Ho, S.-P., Edwards, D. P., Gille, J. C., Luo, M., Osterman, G. B., Kulawik, S. S., and Worden, H.: A global comparison of carbon monoxide profiles and column amounts from Tropospheric Emission Spectrometer (TES) and Measurements of Pollution in the Troposphere (MOPITT), J. Geophys. Res., 114, D21307, https://doi.org/10.1029/2009JD012242, 2009.
Kaplan, J. O.: Wetlands at the Last Glacial Maximum: Distribution and methane emissions, Geophys. Res. Lett., 29, 1079, https://doi.org/10.1029/2001GL013366, 2002.
Keppel-Aleks, G., Wennberg, P. O., and Schneider, T.: Sources of variations in total column carbon dioxide, Atmos. Chem. Phys., 11, 3581–3593, https://doi.org/10.5194/acp-11-3581-2011, 2011.
Keppel-Aleks, G., Wennberg, P. O., Washenfelder, R. A., Wunch, D., Schneider, T., Toon, G. C., Andres, R. J., Blavier, J.-F., Connor, B., Davis, K. J., Desai, A. R., Messerschmidt, J., Notholt, J., Roehl, C. M., Sherlock, V., Stephens, B. B., Vay, S. A., and Wofsy, S. C.: The imprint of surface fluxes and transport on variations in total column carbon dioxide, Biogeosciences, 9, 875–891, https://doi.org/10.5194/bg-9-875-2012, 2012.
Kirchstetter, T. W., Novakov, T., and Hobbs, P. V.: Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon, J. Geophys. Res., 109, D21208, https://doi.org/10.1029/2004JD004999, 2004.
Kulawik, S. S., Worden, J., Eldering, A., Bowman, K., Gunson, M., Osterman, G. B., Zhang, L., Clough, S. A., Shephard, M. W., and Beer, R.: Implementation of cloud retrievals for Tropospheric Emission Spectrometer (TES) atmospheric retrievals: part 1. Description and characterization of errors on trace gas retrievals, J. Geophys. Res., 111, D24204, https://doi.org/10.1029/2005JD006733, 2006.
Lelieveld, J., Crutzen, P. J., and Dentener, F. J.: Changing concentration, lifetime and climate forcing of atmospheric methane, Tellus, 50, 128–150, 1998.
Logan, J. A., Megretskaia, I., Nassar, R., Murray, L. T., Zhang, L., Bowman, K. W., Worden, H. M., and Luo, M.: Effects of the 2006 El Niño on tropospheric composition as revealed by data from the Tropospheric Emission Spectrometer (TES), Geophys. Res. Lett., 35, L03816, https://doi.org/10.1029/2007GL031698, 2008.
Luo, M., rinsland, C., Fisher, B., Sachse, G., Diskin, G., Logan, J., Worden, H., Kulawik, S., Osterman, G., Eldering, A., Herman, R., Shephard, M. :TES carbon monoxide validation with DACOM aircraft measurements during INTEX-B 2006, J. Geophys. Res., 112, D24S48, https://doi.org/10.1029/2007JD008803, 2007.
Luo, M., Boxe, C., Jiang, J., Nassar, R., and Livesey, N.: Interpretation of Aura satellite observations of CO and aerosol index related to the December 2006 Australia fires, Remote Sens. Environ., 114, 2853–2862, https://doi.org/10.1016/j.rse.2010.07.003, 2010.
Nassar, R., Logan, J. A., Megretskaia, I. A., Murray, L. T., Zhang, L., and Jones, D. B. A.: Analysis of tropical tropospheric ozone, carbon monoxide, and water vapor during the 2006 El Niño using TES observations and the GEOS-Chem model, J. Geophys. Res., 114, D17304, https://doi.org/10.1029/2009JD011760, 2009.
O'Connor, F. M., Boucher, O., Gedney, N., Jones, C. D., Folberth, G. A., Coppell, R., Friedlingstein, P., Collins, W. J., Chappellaz, J., Ridley, J. and Johnson, C. E.: Possible role of wetlands, permafrost, and methane hydrates in the methane cycle under future climate change: A review, Rev. Geophys., 48, RG4005, https://doi.org/10.1029/2010RG000326, 2010.
Palmer, P. I., Suntharalingam, P., Jones, D. B. A., Jacob, D. J., Streets, D. G., Fu, Q., Vay, S. A., and Sachse, G. W.: Using CO2: CO correlations to improve inverse analyses of carbon fluxes, J. Geophys. Res., 111, D12318, https://doi.org/10.1029/2005JD006697, 2006.
Page, S. E., Siegert, F., Rieley, J. O., Boehm, H. D. V., Jaya, A., and Limin, S.: The amount of carbon released from peat and forest fires in Indonesia during 1997, Nature, 420, 61–65, 2002.
Park, R. J.: Natural and transboundary pollution influences on sulfate-nitrate-ammonium aerosols in the United States: Implications for policy, J. Geophys. Res., 109, D15204, https://doi.org/10.1029/2003JD004473, 2004.
Pétron, G., Frost, G., Miller, B. R., Hirsch, A. I., Montzka, S. A., Karion, A., Trainer, M., Sweeney, C., Andrews, A. E., Miller, L., Kofler, J., Bar-Ilan, A., Dlugokencky, E. J., Patrick, L., Moore, C. T., Jr., Ryerson, T. B., Siso, C., Kolodzey, W., Lang, P. M., Conway, T., Novelli, P., Masarie, K., Hall, B., Guenther, D., Kitzis, D., Miller, J., Welsh, D., Wolfe, D., Neff, W., and Tans, P.: Hydrocarbon emissions characterization in the Colorado Front Range: A pilot study, J. Geophys. Res., 117, D04304, https://doi.org/10.1029/2011JD016360, 2012.
Pickett-Heaps, C. A., Jacob, D. J., Wecht, K. J., Kort, E. A., Wofsy, S. C., Diskin, G. S., Worthy, D. E. J., Kaplan, J. O., Bey, I., and Drevet, J.: Magnitude and seasonality of wetland methane emissions from the Hudson Bay Lowlands (Canada), Atmos. Chem. Phys., 11, 3773–3779, https://doi.org/10.5194/acp-11-3773-2011, 2011.
Prinn, R. G., Huang, J., Weiss, R. F., Cunnold, D. M., Fraser, P. J., Simmonds, P. G., McCulloch, A., Harth, C., Reimann, S., and Salameh, P.: Evidence for variability of atmospheric hydroxyl radicals over the past quarter century, Geophys. Res. Lett., 32, L07809, https://doi.org/10.1029/2004GL022228, 2005.
Rigby, M., Prinn, R. G., Fraser, P. J., Simmonds, P. G., Langenfelds, R. L., Huang, J., Cunnold, D. M., Steele, L. P., Krummel, P. B., Weiss, R. F., O'doherty, S., Salameh, P. K., Wang, H. J., Harth, C. M., Mühle, J., and Porter, L. W.: Renewed growth of atmospheric methane, Geophys. Res. Lett., 35, L22805, https://doi.org/10.1029/2008GL036037, 2008.
Rodgers, C. D.: Inverse Methods for Atmospheric Sounding: Theory and Practice, World Scientific Publishing Co., Singapore, 2000.
Rodgers, C. D. and Connor, B. J.: Intercomparison of remote sounding instruments, J. Geophys. Res.-Atmos., 108, 4116, https://doi.org/10.1029/2002JD002299, 2003.
Schuck, T. J., Ishijima, K., Patra, P. K., Baker, A. K., Machida, T., Matsueda, H., Sawa, Y., Umezawa, T., Brenninkmeijer, C. A. M., and Lelieveld, J.: Distribution of methane in the tropical upper troposphere measured by CARIBIC and CONTRAIL aircraft, J. Geophys. Res., 117, D19304, https://doi.org/10.1029/2012JD018199, 2012.
Shindell, D., Kuylenstierna, J. C. I., Vignati, E., Van Dingenen, R., Amann, M., Klimont, Z., Anenberg, S. C., Muller, N., Janssens-Maenhout, G., Raes, F., Schwartz, J., Faluvegi, G., Pozzoli, L., Kupiainen, K., Hoglund-Isaksson, L., Emberson, L., Streets, D., Ramanathan, V., Hicks, K., Oanh, N. T. K., Milly, G., Williams, M., Demkine, V., and Fowler, D.: Simultaneously Mitigating Near-Term Climate Change and Improving Human Health and Food Security, Science, 335, 183–189, https://doi.org/10.1126/science.1210026, 2012.
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Kasibhatla, P. S., and Arellano Jr., A. F.: Interannual variability in global biomass burning emissions from 1997 to 2004, Atmos. Chem. Phys., 6, 3423–3441, https://doi.org/10.5194/acp-6-3423-2006, 2006.
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Mu, M., Kasibhatla, P. S., Morton, D. C., DeFries, R. S., Jin, Y., and van Leeuwen, T. T.: Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009), Atmos. Chem. Phys., 10, 11707–11735, https://doi.org/10.5194/acp-10-11707-2010, 2010.
Verma, S., Worden, J., Pierce, B., Jones, D. B. A., Al-Saadi, J., Boersma, F., Bowman, K., Eldering, A., Fisher, B., Jourdain, L., Kulawik, S., Worden, H..: Ozone production in boreal fire smoke plumes using observations from the Tropospheric Emission Spectrometer and the Ozone Monitoring Instrument, J. Geophys. Res., 114, D02303, https://doi.org/10.1029/2008JD010108, 2009.
Wang, H., Jacob, D. J., Kopacz, M., Jones, D. B. A., Suntharalingam, P., Fisher, J. A., Nassar, R., Pawson, S., and Nielsen, J. E.: Error correlation between CO2 and CO as constraint for CO2 flux inversions using satellite data, Atmos. Chem. Phys., 9, 7313–7323, https://doi.org/10.5194/acp-9-7313-2009, 2009.
Wang, J. S., Logan, J. A., McElroy, M. B., Duncan, B. N., Megretskaia, I. A., and Yantosca, R. M.: A 3-D model analysis of the slowdown and interannual variability in the methane growth rate from 1988 to 1997, Global Biogeochem. Cy., 18, GB3011, https://doi.org/10.1029/2003GB002180, 2004.
Wecht, K. J., Jacob, D. J., Wofsy, S. C., Kort, E. A., Worden, J. R., Kulawik, S. S., Henze, D. K., Kopacz, M., and Payne, V. H.: Validation of TES methane with HIPPO aircraft observations: implications for inverse modeling of methane sources, Atmos. Chem. Phys., 12, 1823–1832, https://doi.org/10.5194/acp-12-1823-2012, 2012.
Worden, J., Kulawik, S., Shepard, M., Clough, S., Worden, H., Bowman, K., and Goldman, A.: Predicted errors of tropospheric emission spectrometer nadir retrievals from spectral window selection, J. Geophys. Res., 109, D09308, https://doi.org/10.1029/2004JD004522, 2004.
Worden, H. M., Deeter, M. N., Edwards, D. P., Gille, J. C., Drummond, J. R., and Nedelec, P.: Observations of near-surface carbon monoxide from space using MOPITT multispectral retrievals, J. Geophys. Res., 115, D18314, https://doi.org/10.1029/2010JD014242, 2010.
Worden, J., Kulawik, S., Frankenberg, C., Payne, V., Bowman, K., Cady-Peirara, K., Wecht, K., Lee, J.-E., and Noone, D.: Profiles of CH4, HDO, H$-2$O, and N2O with improved lower tropospheric vertical resolution from Aura TES radiances, Atmos. Meas. Tech., 5, 397–411, https://doi.org/10.5194/amt-5-397-2012, 2012.
Xiong, X., Houweling, S., Wei, J., Maddy, E., Sun, F., and Barnet, C.: Methane plume over south Asia during the monsoon season: satellite observation and model simulation, Atmos. Chem. Phys., 9, 783–794, https://doi.org/10.5194/acp-9-783-2009, 2009.
Altmetrics
Final-revised paper
Preprint