Articles | Volume 25, issue 1
https://doi.org/10.5194/acp-25-1-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-1-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
A numerical sensitivity study on the snow-darkening effect by black carbon deposition over the Arctic in spring
Zilu Zhang
Department of Lower Atmosphere Observation Research (LAOR), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
College of Earth and Planetary Science, University of Chinese Academy of Sciences, Beijing, China
Libo Zhou
CORRESPONDING AUTHOR
Department of Lower Atmosphere Observation Research (LAOR), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
College of Earth and Planetary Science, University of Chinese Academy of Sciences, Beijing, China
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
College of Earth and Planetary Science, University of Chinese Academy of Sciences, Beijing, China
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
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A CMAQ EnSRF-based regional inversion system was extended to resolve satellite retrievals into biogenic source–sink changes. The size of the assimilated biosphere sink in China inferred from GOSAT was −0.47 Pg C yr−1. The biosphere flux at the provincial scale was re-estimated following the refined description in the regional inversion.
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This study constructed an emission inventory of condensable particulate matter (CPM) in China with a focus on organic aerosols (OAs), based on collected CPM emission information. The results show that OA emissions are enhanced twofold for the years 2014 and 2017 after the inclusion of CPM in the new inventory. Sensitivity cases demonstrated the significant contributions of CPM emissions from stationary combustion and mobile sources to primary, secondary, and total OA concentrations.
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Short summary
By integrating the SNICAR model with Polar-WRF, we find that 50 ng g−1 black carbon (BC) deposition decreases snow albedo, increasing radiative forcing (RF) by 1–4 W m−2, especially in Greenland, Baffin Island, and eastern Siberia. The impact is strongly linked to BC mass, with deep snowpacks showing greater sensitivity. Snowmelt and land–atmosphere interactions are crucial. High-resolution modelling is necessary to better understand these effects on Arctic climate change.
By integrating the SNICAR model with Polar-WRF, we find that 50 ng g−1 black carbon (BC)...
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