Articles | Volume 23, issue 5
https://doi.org/10.5194/acp-23-3207-2023
https://doi.org/10.5194/acp-23-3207-2023
Research article
 | 
10 Mar 2023
Research article |  | 10 Mar 2023

Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations

Udo Frieß, Karin Kreher, Richard Querel, Holger Schmithüsen, Dan Smale, Rolf Weller, and Ulrich Platt

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Cited articles

Abbatt, J. P. D., Thomas, J. L., Abrahamsson, K., Boxe, C., Granfors, A., Jones, A. E., King, M. D., Saiz-Lopez, A., Shepson, P. B., Sodeau, J., Toohey, D. W., Toubin, C., von Glasow, R., Wren, S. N., and Yang, X.: Halogen activation via interactions with environmental ice and snow in the polar lower troposphere and other regions, Atmos. Chem. Phys., 12, 6237–6271, https://doi.org/10.5194/acp-12-6237-2012, 2012. a, b
Angot, H., Dastoor, A., De Simone, F., Gårdfeldt, K., Gencarelli, C. N., Hedgecock, I. M., Langer, S., Magand, O., Mastromonaco, M. N., Nordstrøm, C., Pfaffhuber, K. A., Pirrone, N., Ryjkov, A., Selin, N. E., Skov, H., Song, S., Sprovieri, F., Steffen, A., Toyota, K., Travnikov, O., Yang, X., and Dommergue, A.: Chemical cycling and deposition of atmospheric mercury in polar regions: review of recent measurements and comparison with models, Atmos. Chem. Phys., 16, 10735–10763, https://doi.org/10.5194/acp-16-10735-2016, 2016. a
Ariya, P. A., Khalizov, A., and Gidas, A.: Reactions of Gaseous Mercury with Atomic and Molecular Halogens: Kinetics, Product Studies, and Atmospheric Implications, J. Phys. Chem., 106, 7310–7320, https://doi.org/10.1021/jp020719o, 2002. a
Artiglia, L., Edebeli, J., Orlando, F., Chen, S., Lee, M.-T., Corral Arroyo, P., Gilgen, A., Bartels-Rausch, T., Kleibert, A., Vazdar, M., Andres Carignano, M., Francisco, J. S., Shepson, P. B., Gladich, I., and Ammann, M.: A surface-stabilized ozonide triggers bromide oxidation at the aqueous solution-vapour interface, Nat. Commun., 8, 700, https://doi.org/10.1038/s41467-017-00823-x, 2017. a
Barrie, L. and Platt, U.: Arctic tropospheric chemistry: and overview, Tellus B, 49, 449–454, https://doi.org/10.1034/j.1600-0889.49.issue5.2a.x, 1997. a
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Reactive bromine compounds, emitted by the sea ice during polar spring, play an important role in the atmospheric chemistry of the coastal regions of Antarctica. We investigate the sources and impacts of reactive bromine in detail using many years of measurements at two Antarctic sites located at opposite sides of the Antarctic continent. Using a multitude of meteorological observations, we were able to identify the main triggers and source regions for reactive bromine in Antarctica.
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