Articles | Volume 22, issue 17
https://doi.org/10.5194/acp-22-11485-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-11485-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Sep 2022
Research article |
| 07 Sep 2022
| 07 Sep 2022
Comparison of middle- and low-latitude sodium layer from a ground-based lidar network, the Odin satellite, and WACCM–Na model
Deep Space Exploration Laboratory/School of Earth and Space Sciences, University of Science and Technology of China, Hefei, China
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
Department of Meteorology, University of Reading, Berkshire, UK
Anhui Mengcheng Geophysics National Observation and Research Station, University of Science and Technology of China, Hefei, China
Deep Space Exploration Laboratory/School of Earth and Space Sciences, University of Science and Technology of China, Hefei, China
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
Anhui Mengcheng Geophysics National Observation and Research Station, University of Science and Technology of China, Hefei, China
CAS Center for Excellence in Comparative Planetology, Hefei, China
Hefei National Laboratory for the Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, China
Frontiers Science Center for Planetary Exploration and Emerging Technologies, University of Science and Technology of China, Hefei, China
Christopher J. Scott
Department of Meteorology, University of Reading, Berkshire, UK
Mingjiao Jia
Shandong Guoyao Quantum Lidar Co., Ltd., Jinan, Shandong, China
Wuhu Feng
School of Chemistry, University of Leeds, Leeds, UK
National Center for Atmospheric Science, University of Leeds, Leeds, UK
John M. C. Plane
School of Chemistry, University of Leeds, Leeds, UK
Daniel R. Marsh
School of Chemistry, University of Leeds, Leeds, UK
National Center for Atmospheric Research, Boulder, CO, USA
Jonas Hedin
Department of Meteorology, Stockholm University, Stockholm, Sweden
Jörg Gumbel
Department of Meteorology, Stockholm University, Stockholm, Sweden
Xiankang Dou
Deep Space Exploration Laboratory/School of Earth and Space Sciences, University of Science and Technology of China, Hefei, China
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
Electronic Information School, Wuhan University, Wuhan, China
Related authors
Christopher John Scott, Matthew N. Wild, Luke Anthony Barnard, Bingkun Yu, Tatsuhiro Yokoyama, Michael Lockwood, Cathryn Mitchel, John Coxon, and Andrew Kavanagh
EGUsphere, https://doi.org/10.5194/egusphere-2023-2599, https://doi.org/10.5194/egusphere-2023-2599, 2023
Short summary
Short summary
Long-term change in the ionosphere are expected due to increase in greenhouse gases in the lower atmosphere. Empirical formulae are used to estimate height. Through comparison with independent data we show that there are seasonal and long-term biases introduced by the empirical model. We conclude that estimates of long-term changes in ionospheric height need to account for these biases.
Penghao Tian, Bingkun Yu, Hailun Ye, Xianghui Xue, Jianfei Wu, and Tingdi Chen
Atmos. Chem. Phys., 23, 13413–13431, https://doi.org/10.5194/acp-23-13413-2023, https://doi.org/10.5194/acp-23-13413-2023, 2023
Short summary
Short summary
Modeling and prediction of ionospheric irregularities is an important topic in upper-atmospheric and upper-ionospheric physics. We proposed an artificial intelligence model to reconstruct the E-region ionospheric irregularities and first developed an open-source application for the community. The model reveals complex relationships between ionospheric irregularities and external driving factors. The findings suggest that spatiotemporal information plays an important role in the reconstruction.
Bingkun Yu, Xianghui Xue, Christopher J. Scott, Jianfei Wu, Xinan Yue, Wuhu Feng, Yutian Chi, Daniel R. Marsh, Hanli Liu, Xiankang Dou, and John M. C. Plane
Atmos. Chem. Phys., 21, 4219–4230, https://doi.org/10.5194/acp-21-4219-2021, https://doi.org/10.5194/acp-21-4219-2021, 2021
Short summary
Short summary
A long-standing mystery of metal ions within Es layers in the Earth's upper atmosphere is the marked seasonal dependence, with a summer maximum and a winter minimum. We report a large-scale winter-to-summer transport of metal ions from 6-year multi-satellite observations and worldwide ground-based stations. A global atmospheric circulation is responsible for the phenomenon. Our results emphasise the effect of this atmospheric circulation on the transport of composition in the upper atmosphere.
Bingkun Yu, Xianghui Xue, Xin'an Yue, Chengyun Yang, Chao Yu, Xiankang Dou, Baiqi Ning, and Lianhuan Hu
Atmos. Chem. Phys., 19, 4139–4151, https://doi.org/10.5194/acp-19-4139-2019, https://doi.org/10.5194/acp-19-4139-2019, 2019
Short summary
Short summary
It reports the long-term climatology of the intensity of Es layers from COSMIC satellites. The global Es maps present high-resolution spatial distributions and seasonal dependence. It mainly occurs at mid-latitudes and polar regions. Based on wind shear theory, simulation results indicate the convergence of vertical ion velocity could partially explain the Es seasonal dependence and some disagreements between observations and simulations suggest other processes play roles in the Es variations.
Bingkun Yu, Xianghui Xue, Chengling Kuo, Gaopeng Lu, Xiankang Dou, Qi Gao, Jianfei Wu, Mingjiao Jia, Chao Yu, and Xiushu Qie
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-1025, https://doi.org/10.5194/acp-2018-1025, 2018
Preprint withdrawn
Short summary
Short summary
This paper explores the relationship between the intensifications of atomic sodium layer and Es layer in the Mesosphere/Lower Thermosphere (MLT) region (the earth's upper atmosphere at altitudes between 90 and 130 km above ground). The multi-instrument experiment of sodium lidar observations, ionospheric observations and sodium chemical simulations advances our understanding of the dynamical and chemical coupling processes in the mesosphere and ionosphere above thunderstorms.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
Short summary
Short summary
Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Connor J. Clayton, Daniel R. Marsh, Steven T. Turnock, Ailish M. Graham, Kirsty J. Pringle, Carly L. Reddington, Rajesh Kumar, and James B. McQuaid
EGUsphere, https://doi.org/10.5194/egusphere-2024-755, https://doi.org/10.5194/egusphere-2024-755, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We demonstrate that strong climate mitigation could lead to vastly improved air quality in Europe, however, only minimal benefits are seen following the current trajectory of climate mitigation. We use a model that allows us to see where the improvements are greatest (Central Europe) and analyse what sectors are most important for achieving these co-benefits (agriculture/power).
Peter Dalin, Urban Brändström, Johan Kero, Peter Voelger, Takanori Nishiyama, Trond Trondsen, Devin Wyatt, Craig Unick, Vladimir Perminov, Nikolay Pertsev, and Jonas Hedin
Atmos. Meas. Tech., 17, 1561–1576, https://doi.org/10.5194/amt-17-1561-2024, https://doi.org/10.5194/amt-17-1561-2024, 2024
Short summary
Short summary
A novel infrared imaging instrument (OH imager) was put into operation in November 2022 at the Swedish Institute of Space Physics in Kiruna (Sweden). The OH imager is dedicated to the study of nightglow emissions coming from the hydroxyl (OH) and molecular oxygen (O2) layers in the mesopause (80–100 km). Based on a brightness ratio of two OH emission lines, the neutral temperature is estimated at around 87 km. The average daily winter temperature for the period January–April 2023 is 203±10 K.
Ryan Hossaini, David Sherry, Zihao Wang, Martyn Chipperfield, Wuhu Feng, David Oram, Karina Adcock, Stephen Montzka, Isobel Simpson, Andrea Mazzeo, Amber Leeson, Elliot Atlas, and Charles C.-K. Chou
EGUsphere, https://doi.org/10.5194/egusphere-2024-560, https://doi.org/10.5194/egusphere-2024-560, 2024
Short summary
Short summary
Ethylene dichloride (EDC) is an industrial chemical used to produce polyvinyl chloride (PVC). We analysed EDC production data to estimate global EDC emissions (2002 to 2020). The emissions were included in an atmospheric model and evaluated by comparing simulated EDC to EDC measurements in the troposphere. We show EDC contributes ozone-depleting chlorine to the stratosphere and this has increased with increasing EDC emissions. EDC’s impact on stratospheric ozone is currently small, but non-zero.
Bernd Funke, Thierry Dudok de Wit, Ilaria Ermolli, Margit Haberreiter, Doug Kinnison, Daniel Marsh, Hilde Nesse, Annika Seppälä, Miriam Sinnhuber, and Ilya Usoskin
Geosci. Model Dev., 17, 1217–1227, https://doi.org/10.5194/gmd-17-1217-2024, https://doi.org/10.5194/gmd-17-1217-2024, 2024
Short summary
Short summary
We outline a road map for the preparation of a solar forcing dataset for the upcoming Phase 7 of the Coupled Model Intercomparison Project (CMIP7), considering the latest scientific advances made in the reconstruction of solar forcing and in the understanding of climate response while also addressing the issues that were raised during CMIP6.
Stefan Noll, John M. C. Plane, Wuhu Feng, Konstantinos S. Kalogerakis, Wolfgang Kausch, Carsten Schmidt, Michael Bittner, and Stefan Kimeswenger
Atmos. Chem. Phys., 24, 1143–1176, https://doi.org/10.5194/acp-24-1143-2024, https://doi.org/10.5194/acp-24-1143-2024, 2024
Short summary
Short summary
The Earth's nighttime radiation in the range from the near-UV to the near-IR mainly originates between 75 and 105 km and consists of lines of different species, which are important indicators of the chemistry and dynamics at these altitudes. Based on astronomical spectra, we have characterised the structure and variability of a pseudo-continuum of a high number of faint lines and discovered a new emission process in the near-IR. By means of simulations, we identified HO2 as the likely emitter.
Björn Linder, Peter Preusse, Qiuyu Chen, Ole Martin Christensen, Lukas Krasauskas, Linda Megner, Manfred Ern, and Jörg Gumbel
EGUsphere, https://doi.org/10.5194/egusphere-2024-136, https://doi.org/10.5194/egusphere-2024-136, 2024
Short summary
Short summary
The Swedish research satellite MATS (Mesospheric Airglow/Aerosol Tomography and Spectroscopy) is designed to study atmospheric waves in the Mesosphere and the lower Thermosphere. The waves perturb the temperature field and thus, by observing three-dimensional temperature fluctuations, their properties can be quantified. This pre-study uses synthetic MATS data generated from a general circulation model to investigate how well wave properties can be retrieved.
Ailish M. Graham, Richard J. Pope, Martyn P. Chipperfield, Sandip S. Dhomse, Matilda Pimlott, Wuhu Feng, Vikas Singh, Ying Chen, Oliver Wild, Ranjeet Sokhi, and Gufran Beig
Atmos. Chem. Phys., 24, 789–806, https://doi.org/10.5194/acp-24-789-2024, https://doi.org/10.5194/acp-24-789-2024, 2024
Short summary
Short summary
Our paper uses novel satellite datasets and high-resolution emissions datasets alongside a back-trajectory model to investigate the balance of local and external sources influencing NOx air pollution changes in Delhi. We find in the post-monsoon season that NOx from local and non-local transport emissions contributes most to poor air quality in Delhi. Therefore, air quality mitigation strategies in Delhi and surrounding regions are used to control this issue.
Richard J. Pope, Fiona M. O'Connor, Mohit Dalvi, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Brice Barret, Eric Le Flochmoen, Anne Boynard, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, Catherine Wespes, and Richard Rigby
EGUsphere, https://doi.org/10.5194/egusphere-2023-3109, https://doi.org/10.5194/egusphere-2023-3109, 2024
Short summary
Short summary
Ozone is a potent air pollutant in the lower troposphere with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in their long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that in North America, Europe and East Asia, the underlying trends are typically small with large uncertainties.
Andrea Pazmiño, Florence Goutail, Sophie Godin-Beekmann, Alain Hauchecorne, Jean-Pierre Pommereau, Martyn P. Chipperfield, Wuhu Feng, Franck Lefèvre, Audrey Lecouffe, Michel Van Roozendael, Nis Jepsen, Georg Hansen, Rigel Kivi, Kimberly Strong, and Kaley A. Walker
Atmos. Chem. Phys., 23, 15655–15670, https://doi.org/10.5194/acp-23-15655-2023, https://doi.org/10.5194/acp-23-15655-2023, 2023
Short summary
Short summary
The vortex-averaged ozone loss over the last 3 decades is evaluated for both polar regions using the passive ozone tracer of the chemical transport model TOMCAT/SLIMCAT and total ozone observations from the SAOZ network and MSR2 reanalysis. Three metrics were developed to compute ozone trends since 2000. The study confirms the ozone recovery in the Antarctic and shows a potential sign of quantitative detection of ozone recovery in the Arctic that needs to be robustly confirmed in the future.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
Short summary
Short summary
Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Chris Wilson, Brian J. Kerridge, Richard Siddans, David P. Moore, Lucy J. Ventress, Emily Dowd, Wuhu Feng, Martyn P. Chipperfield, and John J. Remedios
EGUsphere, https://doi.org/10.5194/egusphere-2023-1652, https://doi.org/10.5194/egusphere-2023-1652, 2023
Short summary
Short summary
The leaks from the Nord Stream gas pipelines in September 2022 released a large amount of methane (CH4) to the atmosphere. We provide observational data from a satellite instrument, IASI, that shows a large CH4 plume over the North Sea off the coast of Scandinavia. We use this, together with atmospheric models, to quantify the CH4 leaked into the atmosphere from the pipelines. We find that 215–390 Gg CH4 was emitted, making this the largest individual fossil fuel-related CH4 leak on record.
Christopher John Scott, Matthew N. Wild, Luke Anthony Barnard, Bingkun Yu, Tatsuhiro Yokoyama, Michael Lockwood, Cathryn Mitchel, John Coxon, and Andrew Kavanagh
EGUsphere, https://doi.org/10.5194/egusphere-2023-2599, https://doi.org/10.5194/egusphere-2023-2599, 2023
Short summary
Short summary
Long-term change in the ionosphere are expected due to increase in greenhouse gases in the lower atmosphere. Empirical formulae are used to estimate height. Through comparison with independent data we show that there are seasonal and long-term biases introduced by the empirical model. We conclude that estimates of long-term changes in ionospheric height need to account for these biases.
Manuel López-Puertas, Federico Fabiano, Victor Fomichev, Bernd Funke, and Daniel R. Marsh
EGUsphere, https://doi.org/10.5194/egusphere-2023-2424, https://doi.org/10.5194/egusphere-2023-2424, 2023
Short summary
Short summary
The radiative infrared cooling of CO2 in the middle atmosphere is crucial for computing its thermal structure. It requires however to include non-Local Thermodynamic Equilibrium processes which are computationally very expensive, so much that we cannot afford to include them in full in climate models. In this work, we present an updated, efficient and accurate parameterization of that cooling able to cope with CO2 abundances from half the preindustrial values to 10 times the current abundance.
Penghao Tian, Bingkun Yu, Hailun Ye, Xianghui Xue, Jianfei Wu, and Tingdi Chen
Atmos. Chem. Phys., 23, 13413–13431, https://doi.org/10.5194/acp-23-13413-2023, https://doi.org/10.5194/acp-23-13413-2023, 2023
Short summary
Short summary
Modeling and prediction of ionospheric irregularities is an important topic in upper-atmospheric and upper-ionospheric physics. We proposed an artificial intelligence model to reconstruct the E-region ionospheric irregularities and first developed an open-source application for the community. The model reveals complex relationships between ionospheric irregularities and external driving factors. The findings suggest that spatiotemporal information plays an important role in the reconstruction.
John M. C. Plane, Jörg Gumbel, Konstantinos S. Kalogerakis, Daniel R. Marsh, and Christian von Savigny
Atmos. Chem. Phys., 23, 13255–13282, https://doi.org/10.5194/acp-23-13255-2023, https://doi.org/10.5194/acp-23-13255-2023, 2023
Short summary
Short summary
The mesosphere or lower thermosphere region of the atmosphere borders the edge of space. It is subject to extreme ultraviolet photons and charged particles from the Sun and atmospheric gravity waves from below, which tend to break in this region. The pressure is very low, which facilitates chemistry involving species in excited states, and this is also the region where cosmic dust ablates and injects various metals. The result is a unique and exotic chemistry.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
Short summary
Short summary
In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Yajuan Li, Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Jianchun Bian, Yuan Xia, and Dong Guo
Atmos. Chem. Phys., 23, 13029–13047, https://doi.org/10.5194/acp-23-13029-2023, https://doi.org/10.5194/acp-23-13029-2023, 2023
Short summary
Short summary
For the first time a regularized multivariate regression model is used to estimate stratospheric ozone trends. Regularized regression avoids the over-fitting issue due to correlation among explanatory variables. We demonstrate that there are considerable differences in satellite-based and chemical-model-based ozone trends, highlighting large uncertainties in our understanding about ozone variability. We argue that caution is needed when interpreting results with different methods and datasets.
Tinna Lif Gunnarsdottir, Ingrid Mann, Wuhu Feng, Devin R. Huyghebaert, Ingemar Haeggstroem, Yasunobu Ogawa, Norihito Saito, Satonori Nozawa, and Takuya D. Kawahara
Ann. Geophys. Discuss., https://doi.org/10.5194/angeo-2023-29, https://doi.org/10.5194/angeo-2023-29, 2023
Revised manuscript accepted for ANGEO
Short summary
Short summary
Several tons of meteoric particles burn up in our atmosphere each day. This deposits a great deal of material that bids with other atmospheric particles and forms so-called Meteoric Smoke Particles. These particles are assumed to influence radar measurements. Here we have compared radar measurements with simulations of a radar spectrum with and without dust particles and found that dust influences the radar spectrum in the altitude range of 75–85 km.
Michael P. Cartwright, Richard J. Pope, Jeremy J. Harrison, Martyn P. Chipperfield, Chris Wilson, Wuhu Feng, David P. Moore, and Parvadha Suntharalingam
Atmos. Chem. Phys., 23, 10035–10056, https://doi.org/10.5194/acp-23-10035-2023, https://doi.org/10.5194/acp-23-10035-2023, 2023
Short summary
Short summary
A 3-D chemical transport model, TOMCAT, is used to simulate global atmospheric carbonyl sulfide (OCS) distribution. Modelled OCS compares well with satellite observations of OCS from limb-sounding satellite observations. Model simulations also compare adequately with surface and atmospheric observations and suitably capture the seasonality of OCS and background concentrations.
Yang Li, Wuhu Feng, Xin Zhou, Yajuan Li, and Martyn P. Chipperfield
EGUsphere, https://doi.org/10.5194/egusphere-2023-1452, https://doi.org/10.5194/egusphere-2023-1452, 2023
Short summary
Short summary
Tibetan Plateau (TP), the highest and largest plateau, experiences strong surface solar UV radiation, whose excess can cause harmful influences on the local biota. Hence, it is critical to study TP ozone. We find ENSO, the strongest interannual phenomenon, can induce tropospheric temperature change and thus cause tropopause movement, which in turn leads to ozone change. Our understanding implies that future more strong ENSO events will play a key role in ozone recovery and ecosystems of the TP.
Yanlin Li, Tai-Yin Huang, Julio Urbina, Fabio Vargas, and Wuhu Feng
Ann. Geophys. Discuss., https://doi.org/10.5194/angeo-2023-20, https://doi.org/10.5194/angeo-2023-20, 2023
Preprint under review for ANGEO
Short summary
Short summary
This work combines Lidar observation data and a new numerical sodium chemistry model, using data assimilation to study the relationship between the mesospheric sodium layer and the meteoric input function. The simulation captures the seasonal variability of sodium number density compared with lidar observations over Colorado State University lidar. The estimated global ablated meteoroid material inputs inferred from ALO and CSU observations are 116.85 t/day and 61.4 t/day, respectively.
Robert Wagner, Alexander D. James, Victoria L. Frankland, Ottmar Möhler, Benjamin J. Murray, John M. C. Plane, Harald Saathoff, Ralf Weigel, and Martin Schnaiter
Atmos. Chem. Phys., 23, 6789–6811, https://doi.org/10.5194/acp-23-6789-2023, https://doi.org/10.5194/acp-23-6789-2023, 2023
Short summary
Short summary
Polar stratospheric clouds (PSCs) play an important role in the depletion of stratospheric ozone. They can consist of different chemical species, including crystalline nitric acid hydrates. We found that mineral dust or meteoric ablation material can efficiently catalyse the formation of a specific phase of nitric acid dihydrate crystals. We determined predominant particle shapes and infrared optical properties of these crystals, which are important inputs for remote sensing detection of PSCs.
Alexander D. James, Finn Pace, Sebastien N. F. Sikora, Graham W. Mann, John M. C. Plane, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 2215–2233, https://doi.org/10.5194/acp-23-2215-2023, https://doi.org/10.5194/acp-23-2215-2023, 2023
Short summary
Short summary
Here, we examine whether several materials of meteoric origin can nucleate crystallisation in stratospheric cloud droplets which would affect ozone depletion. We find that material which could fragment on atmospheric entry without melting is unlikely to be present in high enough concentration in the stratosphere to contribute to observed crystalline clouds. Material which ablates completely then forms a new solid known as meteoric smoke can provide enough nucleation to explain observed clouds.
Wen Yi, Jie Zeng, Xianghui Xue, Iain Reid, Wei Zhong, Jianfei Wu, Tingdi Chen, and Xiankang Dou
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-254, https://doi.org/10.5194/amt-2022-254, 2022
Revised manuscript not accepted
Short summary
Short summary
In recent years, the concept of multistatic meteor radar systems has attracted the attention of the atmospheric radar community, focusing on the MLT region. In this study, we apply a multistatic meteor radar system consisting of a monostatic meteor radar in Mengcheng (33.36° N, 116.49° E) and a remote receiver in Changfeng (31.98° N, 117.22° E) to estimate the two-dimensional horizontal wind field, and the horizontal divergence and relative vorticity of the wind field.
Yajuan Li, Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Andreas Chrysanthou, Yuan Xia, and Dong Guo
Atmos. Chem. Phys., 22, 10635–10656, https://doi.org/10.5194/acp-22-10635-2022, https://doi.org/10.5194/acp-22-10635-2022, 2022
Short summary
Short summary
Chemical transport models forced with (re)analysis meteorological fields are ideally suited for interpreting the influence of important physical processes on the ozone variability. We use TOMCAT forced by ECMWF ERA-Interim and ERA5 reanalysis data sets to investigate the effects of reanalysis forcing fields on ozone changes. Our results show that models forced by ERA5 reanalyses may not yet be capable of reproducing observed changes in stratospheric ozone, particularly in the lower stratosphere.
Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Barry G. Latter, Diane S. Knappett, Dwayne E. Heard, Lucy J. Ventress, Richard Siddans, Wuhu Feng, and Martyn P. Chipperfield
Atmos. Chem. Phys., 22, 10467–10488, https://doi.org/10.5194/acp-22-10467-2022, https://doi.org/10.5194/acp-22-10467-2022, 2022
Short summary
Short summary
We present a new method to derive global information of the hydroxyl radical (OH), an important atmospheric oxidant. OH controls the lifetime of trace gases important to air quality and climate. We use satellite observations of ozone, carbon monoxide, methane and water vapour in a simple expression to derive OH around 3–4 km altitude. The derived OH compares well to model and aircraft OH data. We then apply the method to 10 years of satellite data to study the inter-annual variability of OH.
Shican Qiu, Mengxi Shi, Willie Soon, Mingjiao Jia, Xianghui Xue, Tao Li, Peng Ju, and Xiankang Dou
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1085, https://doi.org/10.5194/acp-2021-1085, 2022
Revised manuscript not accepted
Short summary
Short summary
The solitary wave theory is applied for the first time to study the sporadic sodium layers (NaS). We perform soliton fitting processes on the observed data from the Andes Lidar Observatory, and find out that 24/27 NaS events exhibit similar features to a soliton. Time series of the net anomaly reveal the same variation process to the solution of a five-order KdV equation. Our results suggest the NaS phenomenon would be an appropriate tracer for nonlinear wave studies in the atmosphere.
Davide Zanchettin, Claudia Timmreck, Myriam Khodri, Anja Schmidt, Matthew Toohey, Manabu Abe, Slimane Bekki, Jason Cole, Shih-Wei Fang, Wuhu Feng, Gabriele Hegerl, Ben Johnson, Nicolas Lebas, Allegra N. LeGrande, Graham W. Mann, Lauren Marshall, Landon Rieger, Alan Robock, Sara Rubinetti, Kostas Tsigaridis, and Helen Weierbach
Geosci. Model Dev., 15, 2265–2292, https://doi.org/10.5194/gmd-15-2265-2022, https://doi.org/10.5194/gmd-15-2265-2022, 2022
Short summary
Short summary
This paper provides metadata and first analyses of the volc-pinatubo-full experiment of CMIP6-VolMIP. Results from six Earth system models reveal significant differences in radiative flux anomalies that trace back to different implementations of volcanic forcing. Surface responses are in contrast overall consistent across models, reflecting the large spread due to internal variability. A second phase of VolMIP shall consider both aspects toward improved protocol for volc-pinatubo-full.
Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Ryan Hossaini, Graham W. Mann, Michelle L. Santee, and Mark Weber
Atmos. Chem. Phys., 22, 903–916, https://doi.org/10.5194/acp-22-903-2022, https://doi.org/10.5194/acp-22-903-2022, 2022
Short summary
Short summary
Solar flux variations associated with 11-year sunspot cycle is believed to exert important external climate forcing. As largest variations occur at shorter wavelengths such as ultra-violet part of the solar spectrum, associated changes in stratospheric ozone are thought to provide direct evidence for solar climate interaction. Until now, most of the studies reported double-peak structured solar cycle signal (SCS), but relatively new satellite data suggest only single-peak-structured SCS.
Ioannis A. Daglis, Loren C. Chang, Sergio Dasso, Nat Gopalswamy, Olga V. Khabarova, Emilia Kilpua, Ramon Lopez, Daniel Marsh, Katja Matthes, Dibyendu Nandy, Annika Seppälä, Kazuo Shiokawa, Rémi Thiéblemont, and Qiugang Zong
Ann. Geophys., 39, 1013–1035, https://doi.org/10.5194/angeo-39-1013-2021, https://doi.org/10.5194/angeo-39-1013-2021, 2021
Short summary
Short summary
We present a detailed account of the science programme PRESTO (PREdictability of the variable Solar–Terrestrial cOupling), covering the period 2020 to 2024. PRESTO was defined by a dedicated committee established by SCOSTEP (Scientific Committee on Solar-Terrestrial Physics). We review the current state of the art and discuss future studies required for the most effective development of solar–terrestrial physics.
Sandip S. Dhomse, Carlo Arosio, Wuhu Feng, Alexei Rozanov, Mark Weber, and Martyn P. Chipperfield
Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, https://doi.org/10.5194/essd-13-5711-2021, 2021
Short summary
Short summary
High-quality long-term ozone profile data sets are key to estimating short- and long-term ozone variability. Almost all the satellite (and chemical model) data sets show some kind of bias with respect to each other. This is because of differences in measurement methodologies as well as simplified processes in the models. We use satellite data sets and chemical model output to generate 42 years of ozone profile data sets using a random-forest machine-learning algorithm that is named ML-TOMCAT.
Jianfei Wu, Wuhu Feng, Han-Li Liu, Xianghui Xue, Daniel Robert Marsh, and John Maurice Campbell Plane
Atmos. Chem. Phys., 21, 15619–15630, https://doi.org/10.5194/acp-21-15619-2021, https://doi.org/10.5194/acp-21-15619-2021, 2021
Short summary
Short summary
Metal layers occur in the MLT region (80–120 km) from the ablation of cosmic dust. The latest lidar observations show these metals can reach a height approaching 200 km, which is challenging to explain. We have developed the first global simulation incorporating the full life cycle of metal atoms and ions. The model results compare well with lidar and satellite observations of the seasonal and diurnal variation of the metals and demonstrate the importance of ion mass and ion-neutral coupling.
Jayanarayanan Kuttippurath, Wuhu Feng, Rolf Müller, Pankaj Kumar, Sarath Raj, Gopalakrishna Pillai Gopikrishnan, and Raina Roy
Atmos. Chem. Phys., 21, 14019–14037, https://doi.org/10.5194/acp-21-14019-2021, https://doi.org/10.5194/acp-21-14019-2021, 2021
Short summary
Short summary
The Arctic winter/spring 2020 was one of the coldest with a strong and long-lasting vortex, high chlorine activation, severe denitrification, and unprecedented ozone loss. The loss was even equal to the levels of some of the warm Antarctic winters. Total column ozone values below 220 DU for several weeks and ozone loss saturation were observed during the period. These results show an unusual meteorology and warrant dedicated studies on the impact of climate change on ozone loss.
Shican Qiu, Ning Wang, Willie Soon, Gaopeng Lu, Mingjiao Jia, Xingjin Wang, Xianghui Xue, Tao Li, and Xiankang Dou
Atmos. Chem. Phys., 21, 11927–11940, https://doi.org/10.5194/acp-21-11927-2021, https://doi.org/10.5194/acp-21-11927-2021, 2021
Short summary
Short summary
Our results suggest that lightning strokes would probably influence the ionosphere and thus give rise to the occurrence of a sporadic sodium layer (NaS), with the overturning of the electric field playing an important role. Model simulation results show that the calculated first-order rate coefficient could explain the efficient recombination of Na+→Na in this NaS case study. A conjunction between the lower and upper atmospheres could be established by these inter-connected phenomena.
Ville Maliniemi, Hilde Nesse Tyssøy, Christine Smith-Johnsen, Pavle Arsenovic, and Daniel R. Marsh
Atmos. Chem. Phys., 21, 11041–11052, https://doi.org/10.5194/acp-21-11041-2021, https://doi.org/10.5194/acp-21-11041-2021, 2021
Short summary
Short summary
We simulate ozone variability over the 21st century with different greenhouse gas scenarios. Our results highlight a novel mechanism of additional reactive nitrogen species descending to the Antarctic stratosphere from the thermosphere/upper mesosphere due to the accelerated residual circulation under climate change. This excess descending NOx can potentially prevent a super recovery of ozone in the Antarctic upper stratosphere.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Anne Kleinert, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, Daniel R. Marsh, and Gabriele P. Stiller
Atmos. Meas. Tech., 14, 4111–4138, https://doi.org/10.5194/amt-14-4111-2021, https://doi.org/10.5194/amt-14-4111-2021, 2021
Short summary
Short summary
An improved dataset of vertical temperature profiles of the Earth's atmosphere in the altitude range 5–70 km is presented. These profiles are derived from measurements of the MIPAS instrument onboard ESA's Envisat satellite. The overall improvements are based on upgrades in the input data and several improvements in the data processing approach. Both of these are discussed, and an extensive error discussion is included. Enhancements of the new dataset are demonstrated by means of examples.
Wei Zhong, Xianghui Xue, Wen Yi, Iain M. Reid, Tingdi Chen, and Xiankang Dou
Atmos. Meas. Tech., 14, 3973–3988, https://doi.org/10.5194/amt-14-3973-2021, https://doi.org/10.5194/amt-14-3973-2021, 2021
Christopher J. Scott, Shannon Jones, and Luke A. Barnard
Ann. Geophys., 39, 309–319, https://doi.org/10.5194/angeo-39-309-2021, https://doi.org/10.5194/angeo-39-309-2021, 2021
Short summary
Short summary
The composition of the upper atmosphere has been difficult to measure with localised observations relying on spacecraft, suborbital rockets or measurements of airglow from ground-based observatories. The height profile of ionisation within the neutral upper atmosphere is influenced by the composition of the neutral gas. We present a method for determining the neutral upper-atmosphere composition from measurements of the ionisation profile and compare these with spacecraft measurements.
Bingkun Yu, Xianghui Xue, Christopher J. Scott, Jianfei Wu, Xinan Yue, Wuhu Feng, Yutian Chi, Daniel R. Marsh, Hanli Liu, Xiankang Dou, and John M. C. Plane
Atmos. Chem. Phys., 21, 4219–4230, https://doi.org/10.5194/acp-21-4219-2021, https://doi.org/10.5194/acp-21-4219-2021, 2021
Short summary
Short summary
A long-standing mystery of metal ions within Es layers in the Earth's upper atmosphere is the marked seasonal dependence, with a summer maximum and a winter minimum. We report a large-scale winter-to-summer transport of metal ions from 6-year multi-satellite observations and worldwide ground-based stations. A global atmospheric circulation is responsible for the phenomenon. Our results emphasise the effect of this atmospheric circulation on the transport of composition in the upper atmosphere.
Jianyuan Wang, Wen Yi, Jianfei Wu, Tingdi Chen, Xianghui Xue, Robert A. Vincent, Iain M. Reid, Paulo P. Batista, Ricardo A. Buriti, Toshitaka Tsuda, and Xiankang Dou
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-33, https://doi.org/10.5194/acp-2021-33, 2021
Revised manuscript not accepted
Short summary
Short summary
In this study, we report the climatology of migrating and non-migrating tides in mesopause winds estimated using multiyear observations from three meteor radars in the southern equatorial region. The results reveal that the climatological patterns of tidal amplitudes by meteor radars is similar to the Climatological Tidal Model of the Thermosphere (CTMT) results and the differences are mainly due to the effect of the stratospheric sudden warming (SSW) event.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Ales Kuchar, William Ball, Pavle Arsenovic, Ellis Remsberg, Patrick Jöckel, Markus Kunze, David A. Plummer, Andrea Stenke, Daniel Marsh, Doug Kinnison, and Thomas Peter
Atmos. Chem. Phys., 21, 201–216, https://doi.org/10.5194/acp-21-201-2021, https://doi.org/10.5194/acp-21-201-2021, 2021
Short summary
Short summary
The solar signal in the mesospheric H2O and CO was extracted from the CCMI-1 model simulations and satellite observations using multiple linear regression (MLR) analysis. MLR analysis shows a pronounced and statistically robust solar signal in both H2O and CO. The model results show a general agreement with observations reproducing a negative/positive solar signal in H2O/CO. The pattern of the solar signal varies among the considered models, reflecting some differences in the model setup.
Benjamin Birner, Martyn P. Chipperfield, Eric J. Morgan, Britton B. Stephens, Marianna Linz, Wuhu Feng, Chris Wilson, Jonathan D. Bent, Steven C. Wofsy, Jeffrey Severinghaus, and Ralph F. Keeling
Atmos. Chem. Phys., 20, 12391–12408, https://doi.org/10.5194/acp-20-12391-2020, https://doi.org/10.5194/acp-20-12391-2020, 2020
Short summary
Short summary
With new high-precision observations from nine aircraft campaigns and 3-D chemical transport modeling, we show that the argon-to-nitrogen ratio (Ar / N2) in the lowermost stratosphere provides a useful constraint on the “age of air” (the time elapsed since entry of an air parcel into the stratosphere). Therefore, Ar / N2 in combination with traditional age-of-air indicators, such as CO2 and N2O, could provide new insights into atmospheric mixing and transport.
Thomas R. Lewis, Juan Carlos Gómez Martín, Mark A. Blitz, Carlos A. Cuevas, John M. C. Plane, and Alfonso Saiz-Lopez
Atmos. Chem. Phys., 20, 10865–10887, https://doi.org/10.5194/acp-20-10865-2020, https://doi.org/10.5194/acp-20-10865-2020, 2020
Short summary
Short summary
Iodine-bearing gasses emitted from the sea surface are chemically processed in the atmosphere, leading to iodine accumulation in aerosol and transport to continental ecosystems. Such processing involves light-induced break-up of large, particle-forming iodine oxides into smaller, ozone-depleting molecules. We combine experiments and theory to report the photolysis efficiency of iodine oxides required to assess the impact of iodine on ozone depletion and particle formation.
Niilo Kalakoski, Pekka T. Verronen, Annika Seppälä, Monika E. Szeląg, Antti Kero, and Daniel R. Marsh
Atmos. Chem. Phys., 20, 8923–8938, https://doi.org/10.5194/acp-20-8923-2020, https://doi.org/10.5194/acp-20-8923-2020, 2020
Short summary
Short summary
Effects of solar proton events (SPEs) on middle atmosphere chemistry were studied using the WACCM-D chemistry–climate model, including an improved representation of lower ionosphere ion chemistry. This study includes 66 events in the years 1989–2012 and uses a statistical approach to determine the impact of the improved chemistry scheme. The differences shown highlight the importance of ion chemistry in models used to study energetic particle precipitation.
Yajuan Li, Martyn P. Chipperfield, Wuhu Feng, Sandip S. Dhomse, Richard J. Pope, Faquan Li, and Dong Guo
Atmos. Chem. Phys., 20, 8627–8639, https://doi.org/10.5194/acp-20-8627-2020, https://doi.org/10.5194/acp-20-8627-2020, 2020
Short summary
Short summary
The Tibetan Plateau (TP) exerts important thermal and dynamical effects on atmospheric circulation, climate change as well as the ozone distribution. In this study, we use updated observations and model simulations to investigate the ozone trends and variations over the TP. Wintertime TP ozone variations are largely controlled by tropical to high-latitude transport processes, whereas summertime concentrations are a combined effect of photochemical decay and tropical processes.
Pekka T. Verronen, Daniel R. Marsh, Monika E. Szeląg, and Niilo Kalakoski
Ann. Geophys., 38, 833–844, https://doi.org/10.5194/angeo-38-833-2020, https://doi.org/10.5194/angeo-38-833-2020, 2020
Short summary
Short summary
This paper is the first to study how the representation of the magnetic-local-time (MLT) dependency of electron precipitation impacts middle-atmospheric-ozone response on monthly timescales. We use a state-of-the-art chemistry–climate model with detailed lower-ionospheric chemistry for an advanced representation of atmospheric impacts of electron forcing. We find that the use of daily zonal-mean electron forcing will provide an accurate ozone response in long-term climate simulations.
Clara Orbe, David A. Plummer, Darryn W. Waugh, Huang Yang, Patrick Jöckel, Douglas E. Kinnison, Beatrice Josse, Virginie Marecal, Makoto Deushi, Nathan Luke Abraham, Alexander T. Archibald, Martyn P. Chipperfield, Sandip Dhomse, Wuhu Feng, and Slimane Bekki
Atmos. Chem. Phys., 20, 3809–3840, https://doi.org/10.5194/acp-20-3809-2020, https://doi.org/10.5194/acp-20-3809-2020, 2020
Short summary
Short summary
Atmospheric composition is strongly influenced by global-scale winds that are not always properly simulated in computer models. A common approach to correct for this bias is to relax or
nudgeto the observed winds. Here we systematically evaluate how well this technique performs across a large suite of chemistry–climate models in terms of its ability to reproduce key aspects of both the tropospheric and stratospheric circulations.
Jörg Gumbel, Linda Megner, Ole Martin Christensen, Nickolay Ivchenko, Donal P. Murtagh, Seunghyuk Chang, Joachim Dillner, Terese Ekebrand, Gabriel Giono, Arvid Hammar, Jonas Hedin, Bodil Karlsson, Mikael Krus, Anqi Li, Steven McCallion, Georgi Olentšenko, Soojong Pak, Woojin Park, Jordan Rouse, Jacek Stegman, and Georg Witt
Atmos. Chem. Phys., 20, 431–455, https://doi.org/10.5194/acp-20-431-2020, https://doi.org/10.5194/acp-20-431-2020, 2020
Short summary
Short summary
Gravity waves can link together atmospheric conditions over large distances. MATS is a new Swedish satellite that will study gravity waves at altitudes around 80–110 km. MATS will take images of emissions from excited molecules, so-called airglow, and of the highest clouds in our atmosphere, so-called noctilucent clouds. These measurements will be analysed to provide three-dimensional wave structures and a comprehensive picture of wave interactions in the atmosphere.
Mingjiao Jia, Jinlong Yuan, Chong Wang, Haiyun Xia, Yunbin Wu, Lijie Zhao, Tianwen Wei, Jianfei Wu, Lu Wang, Sheng-Yang Gu, Liqun Liu, Dachun Lu, Rulong Chen, Xianghui Xue, and Xiankang Dou
Atmos. Chem. Phys., 19, 15431–15446, https://doi.org/10.5194/acp-19-15431-2019, https://doi.org/10.5194/acp-19-15431-2019, 2019
Short summary
Short summary
Gravitational waves (GWs) with periods ranging from 10 to 30 min over 10 h and 20 wave cycles are detected within a 2 km height in the atmospheric boundary layer (ABL) by a coherent Doppler wind lidar. Observations and computational fluid dynamics (CFD) simulations lead to a conclusion that the GWs are excited by the wind shear of a low-level jet under the condition of light horizontal wind. The GWs are trapped in the ABL due to a combination of thermal and Doppler ducts.
Ingo Wohltmann, Ralph Lehmann, Georg A. Gottwald, Karsten Peters, Alain Protat, Valentin Louf, Christopher Williams, Wuhu Feng, and Markus Rex
Geosci. Model Dev., 12, 4387–4407, https://doi.org/10.5194/gmd-12-4387-2019, https://doi.org/10.5194/gmd-12-4387-2019, 2019
Short summary
Short summary
We present a trajectory-based model for simulating the transport of air parcels by convection. Our model extends the approach of existing models by explicitly simulating vertical updraft velocities inside the clouds and the time that an air parcel spends inside the convective event.
Tasha Aylett, James S. A. Brooke, Alexander D. James, Mario Nachbar, Denis Duft, Thomas Leisner, and John M. C. Plane
Atmos. Chem. Phys., 19, 12767–12777, https://doi.org/10.5194/acp-19-12767-2019, https://doi.org/10.5194/acp-19-12767-2019, 2019
Short summary
Short summary
Interplanetary dust particles entering the Earth's atmosphere often melt and evaporate, injecting metals such as iron and magnesium into the atmosphere between 80 and 105 km. These metals become oxidized and then coagulate into small particles a few nanometres is size, known as meteoric smoke. In this study, iron oxide smoke particles were created in the laboratory, and their composition and optical properties were determined in order to understand satellite measurements.
Lina Broman, Susanne Benze, Jörg Gumbel, Ole Martin Christensen, and Cora E. Randall
Atmos. Chem. Phys., 19, 12455–12475, https://doi.org/10.5194/acp-19-12455-2019, https://doi.org/10.5194/acp-19-12455-2019, 2019
Short summary
Short summary
Combining satellite observations of polar mesospheric clouds are complicated due to satellite geometry and measurement technique. In this study, tomographic limb observations are compared to observations from a nadir-viewing satellite using a common volume approach. We present a technique that overcomes differences in scattering conditions and observation geometry. The satellites show excellent agreement, which lays the basis for future insights into horizontal and vertical cloud processes.
Boris Strelnikov, Martin Eberhart, Martin Friedrich, Jonas Hedin, Mikhail Khaplanov, Gerd Baumgarten, Bifford P. Williams, Tristan Staszak, Heiner Asmus, Irina Strelnikova, Ralph Latteck, Mykhaylo Grygalashvyly, Franz-Josef Lübken, Josef Höffner, Raimund Wörl, Jörg Gumbel, Stefan Löhle, Stefanos Fasoulas, Markus Rapp, Aroh Barjatya, Michael J. Taylor, and Pierre-Dominique Pautet
Atmos. Chem. Phys., 19, 11443–11460, https://doi.org/10.5194/acp-19-11443-2019, https://doi.org/10.5194/acp-19-11443-2019, 2019
Short summary
Short summary
Sounding rockets are the only means of measuring small-scale structures (i.e., spatial scales of kilometers to centimeters) in the Earth's middle atmosphere (50–120 km). We present and analyze brand-new high-resolution measurements of atomic oxygen (O) concentration together with high-resolution measurements of ionospheric plasma and neutral air parameters. We found a new behavior of the O inside turbulent layers, which might be essential to adequately model weather and climate.
Matthew J. Rowlinson, Alexandru Rap, Stephen R. Arnold, Richard J. Pope, Martyn P. Chipperfield, Joe McNorton, Piers Forster, Hamish Gordon, Kirsty J. Pringle, Wuhu Feng, Brian J. Kerridge, Barry L. Latter, and Richard Siddans
Atmos. Chem. Phys., 19, 8669–8686, https://doi.org/10.5194/acp-19-8669-2019, https://doi.org/10.5194/acp-19-8669-2019, 2019
Short summary
Short summary
Wildfires and meteorology have a substantial effect on atmospheric concentrations of greenhouse gases such as methane and ozone. During the 1997 El Niño event, unusually large fire emissions indirectly increased global methane through carbon monoxide emission, which decreased the oxidation capacity of the atmosphere. There were also large regional changes to tropospheric ozone concentrations, but contrasting effects of fire and meteorology resulted in a small change to global radiative forcing.
Chong Wang, Mingjiao Jia, Haiyun Xia, Yunbin Wu, Tianwen Wei, Xiang Shang, Chengyun Yang, Xianghui Xue, and Xiankang Dou
Atmos. Meas. Tech., 12, 3303–3315, https://doi.org/10.5194/amt-12-3303-2019, https://doi.org/10.5194/amt-12-3303-2019, 2019
Short summary
Short summary
To investigate the relationship between BLH and air pollution under different conditions, a compact micro-pulse lidar integrating both direct-detection lidar and coherent Doppler wind lidar is built. Evolution of atmospheric boundary layer height (BLH), aerosol layer and fine structure in cloud base are well retrieved. Negative correlation exists between BLH and PM2.5. Different trends show that the relationship between PM2.5 and BLH should be considered in different boundary layer categories.
Wen Yi, Xianghui Xue, Iain M. Reid, Damian J. Murphy, Chris M. Hall, Masaki Tsutsumi, Baiqi Ning, Guozhu Li, Robert A. Vincent, Jinsong Chen, Jianfei Wu, Tingdi Chen, and Xiankang Dou
Atmos. Chem. Phys., 19, 7567–7581, https://doi.org/10.5194/acp-19-7567-2019, https://doi.org/10.5194/acp-19-7567-2019, 2019
Short summary
Short summary
The seasonal variations in the mesopause densities, especially with regard to its global structure, are still unclear. In this study, we report the climatology of the mesopause density estimated using multiyear observations from nine meteor radars from Arctic to Antarctic latitudes. The results reveal a significant AO and SAO in mesopause density, an asymmetry between the two polar regions and evidence of intraseasonal oscillations (ISOs), perhaps associated with the ISOs of the troposphere.
Martin Eberhart, Stefan Löhle, Boris Strelnikov, Jonas Hedin, Mikhail Khaplanov, Stefanos Fasoulas, Jörg Gumbel, Franz-Josef Lübken, and Markus Rapp
Atmos. Meas. Tech., 12, 2445–2461, https://doi.org/10.5194/amt-12-2445-2019, https://doi.org/10.5194/amt-12-2445-2019, 2019
Short summary
Short summary
This paper describes the measurement of atomic oxygen in the upper atmosphere onboard sounding rockets using solid electrolyte sensors. Calibration of the sensors in the laboratory is explained in detail. Results from the WADIS-2 rocket campaign show profiles of atomic oxygen density with a high spatial resolution.
Mario Nachbar, Henrike Wilms, Denis Duft, Tasha Aylett, Kensei Kitajima, Takuya Majima, John M. C. Plane, Markus Rapp, and Thomas Leisner
Atmos. Chem. Phys., 19, 4311–4322, https://doi.org/10.5194/acp-19-4311-2019, https://doi.org/10.5194/acp-19-4311-2019, 2019
Short summary
Short summary
Polar mesospheric clouds (PMC) are water ice clouds forming on nanoparticles in the polar summer mesopause. We investigate the impact of solar radiation on PMC formation in the laboratory. We show that Mie theory calculations combined with an equilibrium temperature model presented in this work predict the warming of the particles very well. Using this model we demonstrate that the impact of solar radiation on ice particle formation is significantly lower than previously assumed.
Bingkun Yu, Xianghui Xue, Xin'an Yue, Chengyun Yang, Chao Yu, Xiankang Dou, Baiqi Ning, and Lianhuan Hu
Atmos. Chem. Phys., 19, 4139–4151, https://doi.org/10.5194/acp-19-4139-2019, https://doi.org/10.5194/acp-19-4139-2019, 2019
Short summary
Short summary
It reports the long-term climatology of the intensity of Es layers from COSMIC satellites. The global Es maps present high-resolution spatial distributions and seasonal dependence. It mainly occurs at mid-latitudes and polar regions. Based on wind shear theory, simulation results indicate the convergence of vertical ion velocity could partially explain the Es seasonal dependence and some disagreements between observations and simulations suggest other processes play roles in the Es variations.
Tao Yuan, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Chem. Phys., 19, 3769–3777, https://doi.org/10.5194/acp-19-3769-2019, https://doi.org/10.5194/acp-19-3769-2019, 2019
Short summary
Short summary
The Na layer in the upper atmosphere is very sensitive to solar radiation and varies considerably during sunrise and sunset. In this paper, we use the lidar observations and an advanced model to investigate this process. We found that the variation is mostly due to the changes in several photochemical reactions involving Na compounds, especially NaHCO3. We also reveal that the Fe layer in the same region changes more quickly than the Na layer due to a faster reaction rate of FeOH to sunlight.
Ove Havnes, Tarjei Antonsen, Gerd Baumgarten, Thomas W. Hartquist, Alexander Biebricher, Åshild Fredriksen, Martin Friedrich, and Jonas Hedin
Atmos. Meas. Tech., 12, 1673–1683, https://doi.org/10.5194/amt-12-1673-2019, https://doi.org/10.5194/amt-12-1673-2019, 2019
Short summary
Short summary
We present a new method of analyzing data from rocket-borne aerosol detectors of the Faraday cup type (DUSTY). By using models for how aerosols are charged in the mesosphere and how they interact in a collision with the probes, fundamental parameters like aerosol radius, charge, and number density can be derived. The resolution can be down to ~ 10 cm, which is much lower than other available methods. The theory is furthermore used to analyze DUSTY data from the 2016 rocket campaign MAXIDUSTY.
Mykhaylo Grygalashvyly, Martin Eberhart, Jonas Hedin, Boris Strelnikov, Franz-Josef Lübken, Markus Rapp, Stefan Löhle, Stefanos Fasoulas, Mikhail Khaplanov, Jörg Gumbel, and Ekaterina Vorobeva
Atmos. Chem. Phys., 19, 1207–1220, https://doi.org/10.5194/acp-19-1207-2019, https://doi.org/10.5194/acp-19-1207-2019, 2019
Short summary
Short summary
Based on rocket-borne true common volume observations of atomic oxygen, atmospheric band emission (762 nm), and background atmosphere density and temperature, one-step, two-step, and combined mechanisms of
O2(b1Σg+) formation were analyzed. We found new coefficients for the fit function based on self-consistent temperature, atomic oxygen, and volume emission observations. This can be used for atmospheric band volume emission modeling or the estimation of atomic oxygen by known volume emission.
David E. Siskind, McArthur Jones Jr., Douglas P. Drob, John P. McCormack, Mark E. Hervig, Daniel R. Marsh, Martin G. Mlynczak, Scott M. Bailey, Astrid Maute, and Nicholas J. Mitchell
Ann. Geophys., 37, 37–48, https://doi.org/10.5194/angeo-37-37-2019, https://doi.org/10.5194/angeo-37-37-2019, 2019
Short summary
Short summary
We use data from two NASA satellites and a general circulation model of the upper atmosphere to elucidate the key factors governing the abundance and diurnal variation of nitric oxide (NO) at near-solar minimum conditions and low latitudes. This has been difficult to do previously, because NO data are typically taken from satellites in sun-synchronous orbits, meaning that they only acquire data in fixed local times. We overcome this limitation through model simulations of the NO diurnal cycle.
Evgenia Galytska, Alexey Rozanov, Martyn P. Chipperfield, Sandip. S. Dhomse, Mark Weber, Carlo Arosio, Wuhu Feng, and John P. Burrows
Atmos. Chem. Phys., 19, 767–783, https://doi.org/10.5194/acp-19-767-2019, https://doi.org/10.5194/acp-19-767-2019, 2019
Short summary
Short summary
In this study we analysed ozone changes in the tropical mid-stratosphere as observed by the SCIAMACHY instrument during 2004–2012. We used simulations from TOMCAT model with different chemical and dynamical forcings to reveal primary causes of ozone changes. We also considered measured NO2 and modelled NOx, NOx, and N2O data. With modelled AoA data we identified seasonal changes in the upwelling speed and explained how those changes affect N2O chemistry which leads to observed ozone changes.
Debora Griffin, Kaley A. Walker, Ingo Wohltmann, Sandip S. Dhomse, Markus Rex, Martyn P. Chipperfield, Wuhu Feng, Gloria L. Manney, Jane Liu, and David Tarasick
Atmos. Chem. Phys., 19, 577–601, https://doi.org/10.5194/acp-19-577-2019, https://doi.org/10.5194/acp-19-577-2019, 2019
Short summary
Short summary
Ozone in the stratosphere is important to protect the Earth from UV radiation. Using measurements taken by the Atmospheric Chemistry Experiment satellite between 2005 and 2013, we examine different methods to calculate the ozone loss in the high Arctic and establish the altitude at which most of the ozone is destroyed. Our results show that the different methods agree within the uncertainties. Recommendations are made on which methods are most appropriate to use.
Joe McNorton, Chris Wilson, Manuel Gloor, Rob J. Parker, Hartmut Boesch, Wuhu Feng, Ryan Hossaini, and Martyn P. Chipperfield
Atmos. Chem. Phys., 18, 18149–18168, https://doi.org/10.5194/acp-18-18149-2018, https://doi.org/10.5194/acp-18-18149-2018, 2018
Short summary
Short summary
Since 2007 atmospheric methane (CH4) has been unexpectedly increasing following a 6-year hiatus. We have used an atmospheric model to attribute regional sources and global sinks of CH4 using observations for the 2003–2015 period. Model results show the renewed growth is best explained by decreased atmospheric removal, decreased biomass burning emissions, and an increased energy sector (mainly from Africa–Middle East and Southern Asia–Oceania) and wetland emissions (mainly from northern Eurasia).
Bingkun Yu, Xianghui Xue, Chengling Kuo, Gaopeng Lu, Xiankang Dou, Qi Gao, Jianfei Wu, Mingjiao Jia, Chao Yu, and Xiushu Qie
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-1025, https://doi.org/10.5194/acp-2018-1025, 2018
Preprint withdrawn
Short summary
Short summary
This paper explores the relationship between the intensifications of atomic sodium layer and Es layer in the Mesosphere/Lower Thermosphere (MLT) region (the earth's upper atmosphere at altitudes between 90 and 130 km above ground). The multi-instrument experiment of sodium lidar observations, ionospheric observations and sodium chemical simulations advances our understanding of the dynamical and chemical coupling processes in the mesosphere and ionosphere above thunderstorms.
John M. C. Plane, Wuhu Feng, Juan Carlos Gómez Martín, Michael Gerding, and Shikha Raizada
Atmos. Chem. Phys., 18, 14799–14811, https://doi.org/10.5194/acp-18-14799-2018, https://doi.org/10.5194/acp-18-14799-2018, 2018
Short summary
Short summary
Meteoric ablation creates layers of metal atoms in the atmosphere around 90 km. Although Ca and Na have similar elemental abundances in most minerals found in the solar system, surprisingly the Ca abundance in the atmosphere is less than 1 % that of Na. This study uses a detailed chemistry model of Ca, largely based on laboratory kinetics measurements, in a whole-atmosphere model to show that the depletion is caused by inefficient ablation of Ca and the formation of stable molecular reservoirs.
Christopher J. Scott and Patrick Major
Ann. Geophys., 36, 1243–1254, https://doi.org/10.5194/angeo-36-1243-2018, https://doi.org/10.5194/angeo-36-1243-2018, 2018
Short summary
Short summary
The variability of the Earth's ionosphere (the electrified region of the Earth's upper atmosphere) results from external forcing from above (through solar activity and space weather effects) and from below (via natural sources such as lightning storms and tectonics). Bombing raids over Europe during World War II were used to determine the quantitative impact of explosions on the ionosphere. It was found that raids using more than 300 tonnes of explosives weakened the ionosphere for up to 5 h.
Tao Li, Chao Ban, Xin Fang, Jing Li, Zhaopeng Wu, Wuhu Feng, John M. C. Plane, Jiangang Xiong, Daniel R. Marsh, Michael J. Mills, and Xiankang Dou
Atmos. Chem. Phys., 18, 11683–11695, https://doi.org/10.5194/acp-18-11683-2018, https://doi.org/10.5194/acp-18-11683-2018, 2018
Short summary
Short summary
A total of 154 nights of observations by the USTC Na temperature and wind lidar (32° N, 117° E) suggest significant seasonal variability in the mesopause. Chemistry plays an important role in Na atom formation. More than half of the observed gravity wave (GW) momentum flux (MF), whose divergence determines the GW forcing, is induced by short-period (10 min–2 h) waves. The anticorrelation between MF and zonal wind (U) suggests strong filtering of short-period GWs by semiannual oscillation U.
Amanda C. Maycock, Katja Matthes, Susann Tegtmeier, Hauke Schmidt, Rémi Thiéblemont, Lon Hood, Hideharu Akiyoshi, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Oliver Kirner, Markus Kunze, Marion Marchand, Daniel R. Marsh, Martine Michou, David Plummer, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Yousuke Yamashita, and Kohei Yoshida
Atmos. Chem. Phys., 18, 11323–11343, https://doi.org/10.5194/acp-18-11323-2018, https://doi.org/10.5194/acp-18-11323-2018, 2018
Short summary
Short summary
The 11-year solar cycle is an important driver of climate variability. Changes in incoming solar ultraviolet radiation affect atmospheric ozone, which in turn influences atmospheric temperatures. Constraining the impact of the solar cycle on ozone is therefore important for understanding climate variability. This study examines the representation of the solar influence on ozone in numerical models used to simulate past and future climate. We highlight important differences among model datasets.
Maarten Krol, Marco de Bruine, Lars Killaars, Huug Ouwersloot, Andrea Pozzer, Yi Yin, Frederic Chevallier, Philippe Bousquet, Prabir Patra, Dmitry Belikov, Shamil Maksyutov, Sandip Dhomse, Wuhu Feng, and Martyn P. Chipperfield
Geosci. Model Dev., 11, 3109–3130, https://doi.org/10.5194/gmd-11-3109-2018, https://doi.org/10.5194/gmd-11-3109-2018, 2018
Short summary
Short summary
The TransCom inter-comparison project regularly carries out studies to quantify errors in simulated atmospheric transport. This paper presents the first results of an age of air (AoA) inter-comparison of six global transport models. Following a protocol, six models simulated five tracers from which atmospheric transport times can easily be deduced. Results highlight that inter-model differences associated with atmospheric transport are still large and require further analysis.
Koen Hendrickx, Linda Megner, Daniel R. Marsh, and Christine Smith-Johnsen
Atmos. Chem. Phys., 18, 9075–9089, https://doi.org/10.5194/acp-18-9075-2018, https://doi.org/10.5194/acp-18-9075-2018, 2018
Short summary
Short summary
The mechanisms that produce, destroy and transport nitric oxide (NO) in the Antarctic mesosphere and lower thermosphere are investigated in AIM-SOFIE satellite observations and compared to SD-WACCM simulations. During winter, NO concentrations are most similar while the altitude of maximum NO number densities is most separated. Even though the rate of descent is similar in both datasets, the simulated descending NO flux is too low in concentration, which reflects a missing source of NO.
Jens-Uwe Grooß, Rolf Müller, Reinhold Spang, Ines Tritscher, Tobias Wegner, Martyn P. Chipperfield, Wuhu Feng, Douglas E. Kinnison, and Sasha Madronich
Atmos. Chem. Phys., 18, 8647–8666, https://doi.org/10.5194/acp-18-8647-2018, https://doi.org/10.5194/acp-18-8647-2018, 2018
Short summary
Short summary
We investigate a discrepancy between model simulations and observations of HCl in the dark polar stratosphere. In early winter, the less-well-studied period of the onset of chlorine activation, observations show a much faster depletion of HCl than simulations of three models. This points to some unknown process that is currently not represented in the models. Various hypotheses for potential causes are investigated that partly reduce the discrepancy. The impact on polar ozone depletion is low.
Richard J. Pope, Martyn P. Chipperfield, Stephen R. Arnold, Norbert Glatthor, Wuhu Feng, Sandip S. Dhomse, Brian J. Kerridge, Barry G. Latter, and Richard Siddans
Atmos. Chem. Phys., 18, 8389–8408, https://doi.org/10.5194/acp-18-8389-2018, https://doi.org/10.5194/acp-18-8389-2018, 2018
Erkki Kyrölä, Monika E. Andersson, Pekka T. Verronen, Marko Laine, Simo Tukiainen, and Daniel R. Marsh
Atmos. Chem. Phys., 18, 5001–5019, https://doi.org/10.5194/acp-18-5001-2018, https://doi.org/10.5194/acp-18-5001-2018, 2018
Short summary
Short summary
In this work we compare three key constituents of the middle atmosphere (ozone, NO2, and NO3) from the GOMOS satellite instrument with the WACCM model. We find that in the stratosphere (below 50 km) ozone differences are very small, but in the mesosphere large deviations are found. GOMOS and WACCM NO2 agree reasonably well except in the polar areas. These differences can be connected to the solar particle storms. For NO3, WACCM results agree with GOMOS with a very high correlation.
Alexander D. James, James S. A. Brooke, Thomas P. Mangan, Thomas F. Whale, John M. C. Plane, and Benjamin J. Murray
Atmos. Chem. Phys., 18, 4519–4531, https://doi.org/10.5194/acp-18-4519-2018, https://doi.org/10.5194/acp-18-4519-2018, 2018
Short summary
Short summary
Crystal nucleation in polar stratospheric clouds (PSCs) has a direct impact on stratospheric chemistry and ozone. However, the mechanism of nucleation has been unclear for decades, limiting prediction of the response of ozone to atmospheric changes. We experimentally demonstrate that meteoric material can trigger nucleation heterogeneously and this can produce observed crystal concentrations in PSCs. This discovery paves the way to robust modelling of past and future trends in PSCs and ozone.
Martin P. Langowski, Christian von Savigny, John P. Burrows, Didier Fussen, Erin C. M. Dawkins, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Meas. Tech., 10, 2989–3006, https://doi.org/10.5194/amt-10-2989-2017, https://doi.org/10.5194/amt-10-2989-2017, 2017
Short summary
Short summary
Meteoric metals form metal layers in the upper atmosphere anandplay a role in the formation of middle-atmospheric clouds and aerosols. However, the total metal influx rate is not well known. Global Na datasets from measurements and a model are available, which had not been compared yet on a global scale until this paper. Overall the agreement is good, and many differences between measurements are also found in the model simulations. However, the modeled layer altitude is too low.
Sarah A. Monks, Stephen R. Arnold, Michael J. Hollaway, Richard J. Pope, Chris Wilson, Wuhu Feng, Kathryn M. Emmerson, Brian J. Kerridge, Barry L. Latter, Georgina M. Miles, Richard Siddans, and Martyn P. Chipperfield
Geosci. Model Dev., 10, 3025–3057, https://doi.org/10.5194/gmd-10-3025-2017, https://doi.org/10.5194/gmd-10-3025-2017, 2017
Short summary
Short summary
The TOMCAT chemical transport model has been updated with the chemical degradation of ethene, propene, toluene, butane and monoterpenes. The tropospheric chemical mechanism is documented and the model is evaluated against surface, balloon, aircraft and satellite data. The model is generally able to capture the main spatial and seasonal features of carbon monoxide, ozone, volatile organic compounds and reactive nitrogen. However,
some model biases are found that require further investigation.
Katja Matthes, Bernd Funke, Monika E. Andersson, Luke Barnard, Jürg Beer, Paul Charbonneau, Mark A. Clilverd, Thierry Dudok de Wit, Margit Haberreiter, Aaron Hendry, Charles H. Jackman, Matthieu Kretzschmar, Tim Kruschke, Markus Kunze, Ulrike Langematz, Daniel R. Marsh, Amanda C. Maycock, Stergios Misios, Craig J. Rodger, Adam A. Scaife, Annika Seppälä, Ming Shangguan, Miriam Sinnhuber, Kleareti Tourpali, Ilya Usoskin, Max van de Kamp, Pekka T. Verronen, and Stefan Versick
Geosci. Model Dev., 10, 2247–2302, https://doi.org/10.5194/gmd-10-2247-2017, https://doi.org/10.5194/gmd-10-2247-2017, 2017
Short summary
Short summary
The solar forcing dataset for climate model experiments performed for the upcoming IPCC report is described. This dataset provides the radiative and particle input of solar variability on a daily basis from 1850 through to 2300. With this dataset a better representation of natural climate variability with respect to the output of the Sun is provided which provides the most sophisticated and comprehensive respresentation of solar variability that has been used in climate model simulations so far.
Wenshou Tian, Yuanpu Li, Fei Xie, Jiankai Zhang, Martyn P. Chipperfield, Wuhu Feng, Yongyun Hu, Sen Zhao, Xin Zhou, Yun Yang, and Xuan Ma
Atmos. Chem. Phys., 17, 6705–6722, https://doi.org/10.5194/acp-17-6705-2017, https://doi.org/10.5194/acp-17-6705-2017, 2017
Short summary
Short summary
Although the principal mechanisms responsible for the formation of the Antarctic ozone hole are well understood, the factors or processes that generate interannual variations in ozone levels in the southern high-latitude stratosphere remain under debate. This study finds that the SST variations across the East Asian marginal seas (5° S–35° N, 100–140° E) could modulate the southern high-latitude stratospheric ozone interannual changes.
Yunxia Yuan, Nickolay Ivchenko, Gunnar Tibert, Marin Stanev, Jonas Hedin, and Jörg Gumbel
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-91, https://doi.org/10.5194/amt-2017-91, 2017
Revised manuscript has not been submitted
Short summary
Short summary
The paper presents a method to determine altitude profile of atmospheric density, temperature and wind by means of analysing the reconstructed trajectory of a rigid falling sphere released from a sounding rocket. The trajectory reconstruction is achieved by post-flight analysis of GPS raw data gathered in the sphere. A comparison of the results with independent measurements is presented, with good agreement of the falling sphere results with other sources in the stratosphere.
Boris Strelnikov, Artur Szewczyk, Irina Strelnikova, Ralph Latteck, Gerd Baumgarten, Franz-Josef Lübken, Markus Rapp, Stefanos Fasoulas, Stefan Löhle, Martin Eberhart, Ulf-Peter Hoppe, Tim Dunker, Martin Friedrich, Jonas Hedin, Mikhail Khaplanov, Jörg Gumbel, and Aroh Barjatya
Ann. Geophys., 35, 547–565, https://doi.org/10.5194/angeo-35-547-2017, https://doi.org/10.5194/angeo-35-547-2017, 2017
Short summary
Short summary
The WADIS sounding rocket mission utilized multi-point turbulence measurements in the mesosphere by different techniques, i.e., with ionization gauges carried by rockets and ground-based MAARSY and EISCAT radars. Results show that turbulence energy dissipation rates oscillate in space and time with amplitude of up to 2 orders of magnitude. Spatial oscillations show the same wavelengths as atmospheric gravity waves. Temporal variability reveals periods of atmospheric tides and gravity waves.
Stefanie Unterguggenberger, Stefan Noll, Wuhu Feng, John M. C. Plane, Wolfgang Kausch, Stefan Kimeswenger, Amy Jones, and Sabine Moehler
Atmos. Chem. Phys., 17, 4177–4187, https://doi.org/10.5194/acp-17-4177-2017, https://doi.org/10.5194/acp-17-4177-2017, 2017
Short summary
Short summary
This study focuses on the analysis of astronomical medium-resolution spectra from the VLT in Chile to measure airglow pseudo-continuum emission of FeO in the optical regime. Compared to OH or Na emissions, this emission is difficult to measure. Using 3.5 years of spectroscopic data, we found annual and semi-annual variations of the FeO emission. Furthermore, we used WACCM to determine the quantum yield of the FeO-producing Fe + O3 reaction in the atmosphere, which has not been done before.
Jochen Stutz, Bodo Werner, Max Spolaor, Lisa Scalone, James Festa, Catalina Tsai, Ross Cheung, Santo F. Colosimo, Ugo Tricoli, Rasmus Raecke, Ryan Hossaini, Martyn P. Chipperfield, Wuhu Feng, Ru-Shan Gao, Eric J. Hintsa, James W. Elkins, Fred L. Moore, Bruce Daube, Jasna Pittman, Steven Wofsy, and Klaus Pfeilsticker
Atmos. Meas. Tech., 10, 1017–1042, https://doi.org/10.5194/amt-10-1017-2017, https://doi.org/10.5194/amt-10-1017-2017, 2017
Short summary
Short summary
A new limb-scanning Differential Optical Absorption Spectroscopy (DOAS) instrument was developed for NASA’s Global Hawk unmanned aerial system during the Airborne Tropical TRopopause EXperiment to study trace gases in the tropical tropopause layer. A new technique that uses in situ and DOAS O3 observations together with radiative transfer calculations allows the retrieval of mixing ratios from the slant column densities of BrO and NO2 at high accuracies of 0.5 ppt and 15 ppt, respectively.
Bernd Funke, William Ball, Stefan Bender, Angela Gardini, V. Lynn Harvey, Alyn Lambert, Manuel López-Puertas, Daniel R. Marsh, Katharina Meraner, Holger Nieder, Sanna-Mari Päivärinta, Kristell Pérot, Cora E. Randall, Thomas Reddmann, Eugene Rozanov, Hauke Schmidt, Annika Seppälä, Miriam Sinnhuber, Timofei Sukhodolov, Gabriele P. Stiller, Natalia D. Tsvetkova, Pekka T. Verronen, Stefan Versick, Thomas von Clarmann, Kaley A. Walker, and Vladimir Yushkov
Atmos. Chem. Phys., 17, 3573–3604, https://doi.org/10.5194/acp-17-3573-2017, https://doi.org/10.5194/acp-17-3573-2017, 2017
Short summary
Short summary
Simulations from eight atmospheric models have been compared to tracer and temperature observations from seven satellite instruments in order to evaluate the energetic particle indirect effect (EPP IE) during the perturbed northern hemispheric (NH) winter 2008/2009. Models are capable to reproduce the EPP IE in dynamically and geomagnetically quiescent NH winter conditions. The results emphasize the need for model improvements in the dynamical representation of elevated stratopause events.
Tamás Kovács, Wuhu Feng, Anna Totterdill, John M. C. Plane, Sandip Dhomse, Juan Carlos Gómez-Martín, Gabriele P. Stiller, Florian J. Haenel, Christopher Smith, Piers M. Forster, Rolando R. García, Daniel R. Marsh, and Martyn P. Chipperfield
Atmos. Chem. Phys., 17, 883–898, https://doi.org/10.5194/acp-17-883-2017, https://doi.org/10.5194/acp-17-883-2017, 2017
Short summary
Short summary
Sulfur hexafluoride (SF6) is a very potent greenhouse gas, which is present in the atmosphere only through its industrial use, for example as an electrical insulator. To estimate accurately the impact of SF6 emissions on climate we need to know how long it persists in the atmosphere before being removed. Previous estimates of the SF6 lifetime indicate a large degree of uncertainty. Here we use a detailed atmospheric model to calculate a current best estimate of the SF6 lifetime.
Martyn P. Chipperfield, Qing Liang, Matthew Rigby, Ryan Hossaini, Stephen A. Montzka, Sandip Dhomse, Wuhu Feng, Ronald G. Prinn, Ray F. Weiss, Christina M. Harth, Peter K. Salameh, Jens Mühle, Simon O'Doherty, Dickon Young, Peter G. Simmonds, Paul B. Krummel, Paul J. Fraser, L. Paul Steele, James D. Happell, Robert C. Rhew, James Butler, Shari A. Yvon-Lewis, Bradley Hall, David Nance, Fred Moore, Ben R. Miller, James W. Elkins, Jeremy J. Harrison, Chris D. Boone, Elliot L. Atlas, and Emmanuel Mahieu
Atmos. Chem. Phys., 16, 15741–15754, https://doi.org/10.5194/acp-16-15741-2016, https://doi.org/10.5194/acp-16-15741-2016, 2016
Short summary
Short summary
Carbon tetrachloride (CCl4) is a compound which, when released into the atmosphere, can cause depletion of the stratospheric ozone layer. Its emissions are controlled under the Montreal Protocol, and its atmospheric abundance is slowly decreasing. However, this decrease is not as fast as expected based on estimates of its emissions and its atmospheric lifetime. We have used an atmospheric model to look at the uncertainties in the CCl4 lifetime and to examine the impact on its atmospheric decay.
Alfonso Saiz-Lopez, John M. C. Plane, Carlos A. Cuevas, Anoop S. Mahajan, Jean-François Lamarque, and Douglas E. Kinnison
Atmos. Chem. Phys., 16, 15593–15604, https://doi.org/10.5194/acp-16-15593-2016, https://doi.org/10.5194/acp-16-15593-2016, 2016
Short summary
Short summary
Electronic structure calculations are used to survey possible reactions that HOI and I2 could undergo at night in the lower troposphere, and hence reconcile measurements and models. The reactions NO3 + HOI and I2 + NO3 are included in two models to explore a new nocturnal iodine radical activation mechanism, leading to a reduction of nighttime HOI and I2. This chemistry can have a large impact on NO3 levels in the MBL, and hence upon the nocturnal oxidizing capacity of the marine atmosphere.
Wayne K. Hocking, Reynold E. Silber, John M. C. Plane, Wuhu Feng, and Marcial Garbanzo-Salas
Ann. Geophys., 34, 1119–1144, https://doi.org/10.5194/angeo-34-1119-2016, https://doi.org/10.5194/angeo-34-1119-2016, 2016
Short summary
Short summary
Meteoroids entering the atmosphere produce trails of ionized particles which can be detected with radar. The weakest ones are called underdense (the most common), the strongest are called overdense, and intermediate ones are transitional. Meteor radar signatures are used to determine atmospheric parameters like temperature and winds. We present new results which show the effect of ozone on the transitional trail lifetimes, which may eventually allow radar to measure mesospheric ozone.
Richard J. Pope, Nigel A. D. Richards, Martyn P. Chipperfield, David P. Moore, Sarah A. Monks, Stephen R. Arnold, Norbert Glatthor, Michael Kiefer, Tom J. Breider, Jeremy J. Harrison, John J. Remedios, Carsten Warneke, James M. Roberts, Glenn S. Diskin, Lewis G. Huey, Armin Wisthaler, Eric C. Apel, Peter F. Bernath, and Wuhu Feng
Atmos. Chem. Phys., 16, 13541–13559, https://doi.org/10.5194/acp-16-13541-2016, https://doi.org/10.5194/acp-16-13541-2016, 2016
Anna Totterdill, Tamás Kovács, Wuhu Feng, Sandip Dhomse, Christopher J. Smith, Juan Carlos Gómez-Martín, Martyn P. Chipperfield, Piers M. Forster, and John M. C. Plane
Atmos. Chem. Phys., 16, 11451–11463, https://doi.org/10.5194/acp-16-11451-2016, https://doi.org/10.5194/acp-16-11451-2016, 2016
Short summary
Short summary
In this study we have experimentally determined the infrared absorption cross sections of NF3 and CFC-115, calculated the radiative forcing and efficiency using two radiative transfer models and identified the effect of clouds and stratospheric adjustment. We have also determined their atmospheric lifetimes using the Whole Atmosphere Community Climate Model.
Tamás Kovács, John M. C. Plane, Wuhu Feng, Tibor Nagy, Martyn P. Chipperfield, Pekka T. Verronen, Monika E. Andersson, David A. Newnham, Mark A. Clilverd, and Daniel R. Marsh
Geosci. Model Dev., 9, 3123–3136, https://doi.org/10.5194/gmd-9-3123-2016, https://doi.org/10.5194/gmd-9-3123-2016, 2016
Short summary
Short summary
This study was completed on D-region atmospheric model development. The sophisticated 3-D Whole Atmosphere Community Climate Model (WACCM) and the 1-D Sodynkalä Ion and Neutral Chemistry Model (SIC) were combined in order to provide a detailed, accurate model (WACCM-SIC) that considers the processes taking place in solar proton events. The original SIC model was reduced by mechanism reduction, which provided an accurate sub-mechanism (rSIC, WACCM-rSIC) of the original model.
Simone Tilmes, Jean-Francois Lamarque, Louisa K. Emmons, Doug E. Kinnison, Dan Marsh, Rolando R. Garcia, Anne K. Smith, Ryan R. Neely, Andrew Conley, Francis Vitt, Maria Val Martin, Hiroshi Tanimoto, Isobel Simpson, Don R. Blake, and Nicola Blake
Geosci. Model Dev., 9, 1853–1890, https://doi.org/10.5194/gmd-9-1853-2016, https://doi.org/10.5194/gmd-9-1853-2016, 2016
Short summary
Short summary
The state of the art Community Earth System Model, CESM1 CAM4-chem has been used to perform reference and sensitivity simulations as part of the Chemistry Climate Model Initiative (CCMI). Specifics of the model and details regarding the setup of the simulations are described. In additions, the main behavior of the model, including selected chemical species have been evaluated with climatological datasets. This paper is therefore a references for studies that use the provided model results.
Charles H. Jackman, Daniel R. Marsh, Douglas E. Kinnison, Christopher J. Mertens, and Eric L. Fleming
Atmos. Chem. Phys., 16, 5853–5866, https://doi.org/10.5194/acp-16-5853-2016, https://doi.org/10.5194/acp-16-5853-2016, 2016
Short summary
Short summary
Two global models were used to investigate the impact of galactic cosmic ray (GCRs) on the atmosphere over the 1960-2010 time period. The primary impact of the naturally occurring GCRs on ozone was found to be due to their production of NOx and this impact varies with the atmospheric chlorine loading, sulfate aerosol loading, and solar cycle variation. GCR-caused decreases of annual average global total ozone were computed to be 0.2 % or less.
N. S. Umo, B. J. Murray, M. T. Baeza-Romero, J. M. Jones, A. R. Lea-Langton, T. L. Malkin, D. O'Sullivan, L. Neve, J. M. C. Plane, and A. Williams
Atmos. Chem. Phys., 15, 5195–5210, https://doi.org/10.5194/acp-15-5195-2015, https://doi.org/10.5194/acp-15-5195-2015, 2015
Short summary
Short summary
Combustion ash particles nucleate ice in the immersion mode at conditions relevant to mixed-phase clouds. Hence, combustion ashes could play an important role in primary ice formation in mixed-phase clouds, especially in clouds that are formed near the emission source of these aerosol particles. From this study, there is a need to quantify the atmospheric abundance of combustion ashes in order to quantitatively assess the impact of combustion ashes on mixed-phase clouds.
O. M. Christensen, P. Eriksson, J. Urban, D. Murtagh, K. Hultgren, and J. Gumbel
Atmos. Meas. Tech., 8, 1981–1999, https://doi.org/10.5194/amt-8-1981-2015, https://doi.org/10.5194/amt-8-1981-2015, 2015
Short summary
Short summary
Polar mesospheric clouds are clouds that form in the summer polar mesopause, 80km above the surface. In this study we present new measurements by the Odin satellite, which are able to determine water vapour, temperature and cloud coverage with a high resolution and a large geographical coverage. Using these data we can see structures in the clouds and background atmosphere that have not been detectable by previous measurements.
C. J. Scott and R. Stamper
Ann. Geophys., 33, 449–455, https://doi.org/10.5194/angeo-33-449-2015, https://doi.org/10.5194/angeo-33-449-2015, 2015
Short summary
Short summary
We use a novel technique to infer long-term compositional changes to the thermosphere from the annual variation of the ionospheric F2 region. A global analysis of these data reveal that long-term changes differ between geographic locations in a way that is very similar to the observed variation in the ionospheric response to increased atmospheric CO2 levels. In the absence of long-term measurements of thermospheric composition, further, detailed, modelling work is required.
M. P. Langowski, C. von Savigny, J. P. Burrows, W. Feng, J. M. C. Plane, D. R. Marsh, D. Janches, M. Sinnhuber, A. C. Aikin, and P. Liebing
Atmos. Chem. Phys., 15, 273–295, https://doi.org/10.5194/acp-15-273-2015, https://doi.org/10.5194/acp-15-273-2015, 2015
Short summary
Short summary
Global concentration fields of Mg and Mg+ in the Earth's upper mesosphere and lower thermosphere (70-150km) are presented. These are retrieved from SCIAMACHY/Envisat satellite grating spectrometer measurements in limb viewing geometry between 2008 and 2012.
These were compared with WACCM-Mg model results and a large fraction of the available measurement results for these species, and an interpretation of the results is done. The variation of these species during NLC presence is discussed.
X. Yue, W. S. Schreiner, Z. Zeng, Y.-H. Kuo, and X. Xue
Atmos. Meas. Tech., 8, 225–236, https://doi.org/10.5194/amt-8-225-2015, https://doi.org/10.5194/amt-8-225-2015, 2015
Short summary
Short summary
The occurrence of sporadic E (Es) layers has been a hot scientific topic for a long time. GNSS (global navigation satellite system)-based radio occultation (RO) has proven to be a powerful technique for detecting the global Es layers. In this paper, we show some examples of multiple Es layers occurring in one RO event and the occurrence of Es in a broad region during a certain time interval. The results are then evaluated by independent observations such as lidar and ionosondes.
H. Berresheim, M. Adam, C. Monahan, C. O'Dowd, J. M. C. Plane, B. Bohn, and F. Rohrer
Atmos. Chem. Phys., 14, 12209–12223, https://doi.org/10.5194/acp-14-12209-2014, https://doi.org/10.5194/acp-14-12209-2014, 2014
Short summary
Short summary
Sulfuric acid plays a major role in the formation of aerosol particles and clouds. Measurements at the west coast of Ireland reveal that oxidation of SO2 by OH explains only 20%, on average, of H2SO4 formation in coastal marine air. Additional sources may be (a) oxidation by Criegee intermediates produced photolytically and/or (b) formation from SO3 instead of SO2 in the oxidation of dimethyl sulfide, suggesting an important role of marine emissions in the self-cleaning power of the atmosphere.
B. Ehard, P. Achtert, and J. Gumbel
Ann. Geophys., 32, 1395–1405, https://doi.org/10.5194/angeo-32-1395-2014, https://doi.org/10.5194/angeo-32-1395-2014, 2014
Y. J. Liu, J. M. C. Plane, B. R. Clemesha, J. H. Wang, and X. W. Cheng
Ann. Geophys., 32, 1321–1332, https://doi.org/10.5194/angeo-32-1321-2014, https://doi.org/10.5194/angeo-32-1321-2014, 2014
A. Spolaor, P. Vallelonga, J. Gabrieli, T. Martma, M. P. Björkman, E. Isaksson, G. Cozzi, C. Turetta, H. A. Kjær, M. A. J. Curran, A. D. Moy, A. Schönhardt, A.-M. Blechschmidt, J. P. Burrows, J. M. C. Plane, and C. Barbante
Atmos. Chem. Phys., 14, 9613–9622, https://doi.org/10.5194/acp-14-9613-2014, https://doi.org/10.5194/acp-14-9613-2014, 2014
S. M. MacDonald, J. C. Gómez Martín, R. Chance, S. Warriner, A. Saiz-Lopez, L. J. Carpenter, and J. M. C. Plane
Atmos. Chem. Phys., 14, 5841–5852, https://doi.org/10.5194/acp-14-5841-2014, https://doi.org/10.5194/acp-14-5841-2014, 2014
G. Chiodo, D. R. Marsh, R. Garcia-Herrera, N. Calvo, and J. A. García
Atmos. Chem. Phys., 14, 5251–5269, https://doi.org/10.5194/acp-14-5251-2014, https://doi.org/10.5194/acp-14-5251-2014, 2014
A. C. Kren, D. R. Marsh, A. K. Smith, and P. Pilewskie
Atmos. Chem. Phys., 14, 4843–4856, https://doi.org/10.5194/acp-14-4843-2014, https://doi.org/10.5194/acp-14-4843-2014, 2014
M. Lockwood, H. Nevanlinna, M. Vokhmyanin, D. Ponyavin, S. Sokolov, L. Barnard, M. J. Owens, R. G. Harrison, A. P. Rouillard, and C. J. Scott
Ann. Geophys., 32, 367–381, https://doi.org/10.5194/angeo-32-367-2014, https://doi.org/10.5194/angeo-32-367-2014, 2014
M. Lockwood, H. Nevanlinna, L. Barnard, M. J. Owens, R. G. Harrison, A. P. Rouillard, and C. J. Scott
Ann. Geophys., 32, 383–399, https://doi.org/10.5194/angeo-32-383-2014, https://doi.org/10.5194/angeo-32-383-2014, 2014
C. J. Scott, R. Stamper, and H. Rishbeth
Ann. Geophys., 32, 113–119, https://doi.org/10.5194/angeo-32-113-2014, https://doi.org/10.5194/angeo-32-113-2014, 2014
M. Lockwood, L. Barnard, H. Nevanlinna, M. J. Owens, R. G. Harrison, A. P. Rouillard, and C. J. Davis
Ann. Geophys., 31, 1957–1977, https://doi.org/10.5194/angeo-31-1957-2013, https://doi.org/10.5194/angeo-31-1957-2013, 2013
M. Lockwood, L. Barnard, H. Nevanlinna, M. J. Owens, R. G. Harrison, A. P. Rouillard, and C. J. Davis
Ann. Geophys., 31, 1979–1992, https://doi.org/10.5194/angeo-31-1979-2013, https://doi.org/10.5194/angeo-31-1979-2013, 2013
A. Spolaor, J. Gabrieli, T. Martma, J. Kohler, M. B. Björkman, E. Isaksson, C. Varin, P. Vallelonga, J. M. C. Plane, and C. Barbante
The Cryosphere, 7, 1645–1658, https://doi.org/10.5194/tc-7-1645-2013, https://doi.org/10.5194/tc-7-1645-2013, 2013
A. Spolaor, P. Vallelonga, J. M. C. Plane, N. Kehrwald, J. Gabrieli, C. Varin, C. Turetta, G. Cozzi, R. Kumar, C. Boutron, and C. Barbante
Atmos. Chem. Phys., 13, 6623–6635, https://doi.org/10.5194/acp-13-6623-2013, https://doi.org/10.5194/acp-13-6623-2013, 2013
P. Achtert, M. Khaplanov, F. Khosrawi, and J. Gumbel
Atmos. Meas. Tech., 6, 91–98, https://doi.org/10.5194/amt-6-91-2013, https://doi.org/10.5194/amt-6-91-2013, 2013
M. Rapp, J. M. C. Plane, B. Strelnikov, G. Stober, S. Ernst, J. Hedin, M. Friedrich, and U.-P. Hoppe
Ann. Geophys., 30, 1661–1673, https://doi.org/10.5194/angeo-30-1661-2012, https://doi.org/10.5194/angeo-30-1661-2012, 2012
A. S. Mahajan, J. C. Gómez Martín, T. D. Hay, S.-J. Royer, S. Yvon-Lewis, Y. Liu, L. Hu, C. Prados-Roman, C. Ordóñez, J. M. C. Plane, and A. Saiz-Lopez
Atmos. Chem. Phys., 12, 11609–11617, https://doi.org/10.5194/acp-12-11609-2012, https://doi.org/10.5194/acp-12-11609-2012, 2012
Related subject area
Subject: Dynamics | Research Activity: Remote Sensing | Altitude Range: Mesosphere | Science Focus: Chemistry (chemical composition and reactions)
Significant enhancements of the mesospheric Na layer bottom below 75 km observed by a full-diurnal-cycle lidar at Beijing (40.41° N, 116.01° E), China
Signatures of the 2-day wave and sudden stratospheric warmings in Arctic water vapour observed by ground-based microwave radiometry
Mesosphere-to-stratosphere descent of odd nitrogen in February–March 2009 after sudden stratospheric warming
Yuan Xia, Jing Jiao, Satonori Nozawa, Xuewu Cheng, Jihong Wang, Chunhua Shi, Lifang Du, Yajuan Li, Haoran Zheng, Faquan Li, and Guotao Yang
Atmos. Chem. Phys., 22, 13817–13831, https://doi.org/10.5194/acp-22-13817-2022, https://doi.org/10.5194/acp-22-13817-2022, 2022
Short summary
Short summary
The layer of sodium atoms is generally located above 80 km. This study reports the significant enhancements of the sodium layer below 75 km where sodium atoms are short-lived. The neutral chemical reactions were suggested as making a critical contribution. The reported results provide clear observational evidence for the role of planetary waves in the variation of metal layers, and have implications for the response of the metal layers to perturbations in the lower atmosphere.
B. Tschanz and N. Kämpfer
Atmos. Chem. Phys., 15, 5099–5108, https://doi.org/10.5194/acp-15-5099-2015, https://doi.org/10.5194/acp-15-5099-2015, 2015
S.-M. Salmi, P. T. Verronen, L. Thölix, E. Kyrölä, L. Backman, A. Yu. Karpechko, and A. Seppälä
Atmos. Chem. Phys., 11, 4645–4655, https://doi.org/10.5194/acp-11-4645-2011, https://doi.org/10.5194/acp-11-4645-2011, 2011
Cited articles
Andrioli, V., Xu, J., Batista, P., Pimenta, A., Resende, L., Savio, S.,
Fagundes, P., Yang, G., Jiao, J., Cheng, X., Wang, C., and Liu Z.: Nocturnal and seasonal
variation of Na and K layers simultaneously observed in the MLT Region at
23∘ S, J. Geophys. Res.-Space, 125, e2019JA027164, https://doi.org/10.1029/2019JA027164,
2020. a, b, c
Cai, X., Yuan, T., and Eccles, J. V.: A numerical investigation on tidal and
gravity wave contributions to the summer time Na variations in the
midlatitude E region, J. Geophys. Res.-Space, 122,
10–577, 2017. a
CDAAC: COSMIC RO data, CDAAC [data set], https://data.cosmic.ucar.edu/gnss-ro/, last access: 1 September 2022. a
Chu, Y.-H., Wang, C., Wu, K., Chen, K., Tzeng, K., Su, C.-L., Feng, W., and
Plane, J. M. C.: Morphology of sporadic E layer retrieved from COSMIC GPS radio
occultation measurements: Wind shear theory examination, J.
Geophys. Res.-Space, 119, 2117–2136, 2014. a
Clemesha, B.: Sporadic neutral metal layers in the mesosphere and lower
thermosphere, J. Atmos. Terr. Phys., 57, 725–736,
1995. a
Clemesha, B., Kirchhoff, V., Simonich, D., and Takahashi, H.: Evidence of an
extra-terrestrial source for the mesospheric sodium layer, Geophys.
Res. Lett., 5, 873–876, 1978. a
Daly, S. M., Feng, W., Mangan, T. P., Gerding, M., and Plane, J. M. C.: The
meteoric Ni layer in the upper atmosphere, J. Geophys. Res.-Space, 125, e2020JA028083, https://doi.org/10.1029/2020JA028083, 2020. a
Davis, C. J. and Johnson, C.: Lightning-induced intensification of the
ionospheric sporadic E layer, Nature, 435, 799–801, 2005. a
Dou, X.-K., Xue, X.-H., Chen, T.-D., Wan, W.-X., Cheng, X.-W., Li, T., Chen, C., Qiu, S., and Chen, Z.-Y.: A statistical study of sporadic sodium layer observed by Sodium lidar at Hefei (31.8∘ N, 117.3∘ E), Ann. Geophys., 27, 2247–2257, https://doi.org/10.5194/angeo-27-2247-2009, 2009. a, b
Dou, X.-K., Xue, X.-H., Li, T., Chen, T.-D., Chen, C., and Qiu, S.-C.: Possible
relations between meteors, enhanced electron density layers, and sporadic
sodium layers, J. Geophys. Res.-Space, 115, A06311, https://doi.org/10.1029/2009JA014575, 2010. a, b
Fan, Z., Plane, J. M. C., and Gumbel, J.: On the global distribution of sporadic
sodium layers, Geophys. Res. Lett., 34, L15808, https://doi.org/10.1029/2007GL030542, 2007a. a
Fan, Z. Y., Plane, J. M. C., Gumbel, J., Stegman, J., and Llewellyn, E. J.: Satellite measurements of the global mesospheric sodium layer, Atmos. Chem. Phys., 7, 4107–4115, https://doi.org/10.5194/acp-7-4107-2007, 2007b. a, b
Feng, W., Höffner, J., Marsh, D., Chipperfield, M., Dawkins, E., Viehl, T.,
and Plane, J. M. C.: Diurnal variation of the potassium layer in the upper
atmosphere, Geophys. Res. Lett., 42, 3619–3626, 2015. a
Fussen, D., Vanhellemont, F., Bingen, C., Kyrölä, E., Tamminen, J.,
Sofieva, V., Hassinen, S., Seppälä, A., Verronen, P., Bertaux, J.-L.,
Hauchecorne, A., Dalaudier, F., Renard, J.-B., Fraisse, R., Fanton d'Andon, O., Barrot, G., Mangin, A., The'odore, B., Guirlet, M., Koopman, R., Snoeij, P., and Saavedra, L.: Global measurement of the mesospheric sodium layer by the star
occultation instrument GOMOS, Geophys. Res. Lett., 31, L24110, https://doi.org/10.1029/2004GL021618, 2004. a
Fussen, D., Vanhellemont, F., Tétard, C., Mateshvili, N., Dekemper, E., Loodts, N., Bingen, C., Kyrölä, E., Tamminen, J., Sofieva, V., Hauchecorne, A., Dalaudier, F., Bertaux, J.-L., Barrot, G., Blanot, L., Fanton d'Andon, O., Fehr, T., Saavedra, L., Yuan, T., and She, C.-Y.: A global climatology of the mesospheric sodium layer from GOMOS data during the 2002–2008 period, Atmos. Chem. Phys., 10, 9225–9236, https://doi.org/10.5194/acp-10-9225-2010, 2010. a, b
Gardner, C. S. and Liu, A. Z.: Measuring eddy heat, constituent, and momentum
fluxes with high-resolution Na and Fe Doppler lidars, J. Geophys.
Res.-Atmos., 119, 10583–10603, 2014. a
Gardner, C. S., Plane, J. M. C., Pan, W., Vondrak, T., Murray, B. J., and Chu, X.:
Seasonal variations of the Na and Fe layers at the South Pole and their
implications for the chemistry and general circulation of the polar
mesosphere, J. Geophys. Res.-Atmos., 110, D10302, https://doi.org/10.1029/2004JD005670, 2005. a, b, c
Gumbel, J., Fan, Z., Waldemarsson, T., Stegman, J., Witt, G., Llewellyn, E.,
She, C.-Y., and Plane, J. M. C.: Retrieval of global mesospheric sodium densities
from the Odin satellite, Geophys. Res. Lett., 34, L04813, https://doi.org/10.1029/2006GL028687, 2007. a, b, c, d
Hocke, K., Lainer, M., Moreira, L., Hagen, J., Fernandez Vidal, S., and Schranz, F.: Atmospheric inertia-gravity waves retrieved from level-2 data of the satellite microwave limb sounder Aura/MLS, Ann. Geophys., 34, 781–788, https://doi.org/10.5194/angeo-34-781-2016, 2016. a
Hunten, D. M.: Spectroscopic studies of the twilight airglow, Space Sci.
Rev., 6, 493–573, 1967. a
Kane, T., Grime, B., Franke, S., Kudeki, E., Urbina, J., Kelley, M., and
Collins, S.: Joint observations of sodium enhancements and field-aligned
ionospheric irregularities, Geophys. Res. Lett., 28, 1375–1378,
2001. a
Koch, J., Bourassa, A., Lloyd, N., Roth, C., and von Savigny, C.: Comparison of mesospheric sodium profile retrievals from OSIRIS and SCIAMACHY nightglow measurements, Atmos. Chem. Phys., 22, 3191–3202, https://doi.org/10.5194/acp-22-3191-2022, 2022. a
Krueger, D. A., She, C.-Y., and Yuan, T.: Retrieving mesopause temperature and
line-of-sight wind from full-diurnal-cycle Na lidar observations, Appl.
Optics, 54, 9469–9489, 2015. a
Langowski, M. P., von Savigny, C., Burrows, J. P., Feng, W., Plane, J. M. C., Marsh, D. R., Janches, D., Sinnhuber, M., Aikin, A. C., and Liebing, P.: Global investigation of the Mg atom and ion layers using SCIAMACHY/Envisat observations between 70 and 150 km altitude and WACCM-Mg model results, Atmos. Chem. Phys., 15, 273–295, https://doi.org/10.5194/acp-15-273-2015, 2015. a
Langowski, M. P., von Savigny, C., Burrows, J. P., Fussen, D., Dawkins, E. C. M., Feng, W., Plane, J. M. C., and Marsh, D. R.: Comparison of global datasets of sodium densities in the mesosphere and lower thermosphere from GOMOS, SCIAMACHY and OSIRIS measurements and WACCM model simulations from 2008 to 2012, Atmos. Meas. Tech., 10, 2989–3006, https://doi.org/10.5194/amt-10-2989-2017, 2017. a, b
Li, T., Ban, C., Fang, X., Li, J., Wu, Z., Feng, W., Plane, J. M. C., Xiong, J., Marsh, D. R., Mills, M. J., and Dou, X.: Climatology of mesopause region nocturnal temperature, zonal wind and sodium density observed by sodium lidar over Hefei, China (32∘ N, 117∘ E), Atmos. Chem. Phys., 18, 11683–11695, https://doi.org/10.5194/acp-18-11683-2018, 2018. a, b, c
Liu, A. Z., Lu, X., and Franke, S. J.: Diurnal variation of gravity wave
momentum flux and its forcing on the diurnal tide, J. Geophys.
Res.-Atmos., 118, 1668–1678, 2013. a
Liu, A. Z., Guo, Y., Vargas, F., and Swenson, G. R.: First measurement of
horizontal wind and temperature in the lower thermosphere (105–140 km) with
a Na Lidar at Andes Lidar Observatory, Geophys. Res. Lett., 43,
2374–2380, 2016. a
Llewellyn, E., Lloyd, N., Degenstein, D., Gattinger, R., Petelina, S.,
Bourassa, A., Wiensz, J., Ivanov, E., McDade, I., Solheim, B., McConnell, J., Haley, C., Savigny, C., Sioris, C., McLinden, C., Griffioen, E., Kaminski, J., Evans, W., Puckrin, E., Strong, K., Wehrle, V., Hum, R., Kendall, D., Matsushita, J., Murtagh, D., Brohede, S., Stegman, J., Witt, G., Barnes, G., Payne, W., Piché, L., Smith, K., Warshaw, G., Deslauniers, D., Marchand, P., Richardson, E., King, R., Wevers, I., McCreath, W., Kyrölä, E., Oikarinen, L., Leppelmeier, G., Auvinen, H., Mégie, G., Hauchecorne, A., Lefèvre, F., de La Nöe, J., Ricaud, P., Frisk, U., Sjoberg, F., von Schéele, F., and Nordh L.: The
OSIRIS instrument on the Odin spacecraft, Can. J. Phys., 82,
411–422, 2004. a
Marsh, D. R., Garcia, R. R., Kinnison, D., Boville, B., Sassi, F., Solomon, S.,
and Matthes, K.: Modeling the whole atmosphere response to solar cycle
changes in radiative and geomagnetic forcing, J. Geophys.
Res.-Atmos., 112, D23306, https://doi.org/10.1029/2006JD008306, 2007. a
Meridian Space Weather Monitoring Project: Na lidar data, CMP [data set], https://data.meridianproject.ac.cn/data-directory/, last access: 1 September 2022. a
Molod, A., Takacs, L., Suarez, M., and Bacmeister, J.: Development of the GEOS-5 atmospheric general circulation model: evolution from MERRA to MERRA2, Geosci. Model Dev., 8, 1339–1356, https://doi.org/10.5194/gmd-8-1339-2015, 2015. a
Murtagh, D., Frisk, U., Merino, F., Ridal, M., Jonsson, A., Stegman, J., Witt,
G., Eriksson, P., Jiménez, C., Megie, G., de la Noë, J., Ricaud, P., Baron, P., Pardo, J., Hauchcorne, A., Llewellyn, E., Degenstein, D., Gattinger, R., Lloyd, N., Evans, W., McDade, I., Haley, C., Sioris, C., Savigny, C., Solheim, B., McConnell, J., Strong, K., Richardson, E., Leppelmeier, G., Kyrölä, E., Auvinen, H., and Oikarinen, L.: An overview of the Odin
atmospheric mission, Can. J. Phys., 80, 309–319, 2002. a
NSSDC: Na lidar data, NSSDC [data set], http://www.nssdc.ac.cn, last access: 1 September 2022. a
Pfrommer, T., Hickson, P., and She, C.-Y.: A large-aperture sodium fluorescence
lidar with very high resolution for mesopause dynamics and adaptive optics
studies, Geophys. Res. Lett., 36, L15831, https://doi.org/10.1029/2009GL038802, 2009. a
Plane, J. M. C., Murray, B. J., Chu, X., and Gardner, C. S.: Removal of meteoric
iron on polar mesospheric clouds, Science, 304, 426–428, 2004. a
Plane, J. M. C., Feng, W., Dawkins, E., Chipperfield, M., Höffner, J.,
Janches, D., and Marsh, D.: Resolving the strange behavior of
extraterrestrial potassium in the upper atmosphere, Geophys. Res.
Lett., 41, 4753–4760, 2014. a
Plane, J. M. C., Gómez-Martín, J. C., Feng, W., and Janches, D.: Silicon
chemistry in the mesosphere and lower thermosphere, J. Geophys.
Res.-Atmos., 121, 3718–3728, 2016. a
Plane, J. M. C., Feng, W., Gómez Martín, J. C., Gerding, M., and Raizada, S.: A new model of meteoric calcium in the mesosphere and lower thermosphere, Atmos. Chem. Phys., 18, 14799–14811, https://doi.org/10.5194/acp-18-14799-2018, 2018. a, b
Plane, J. M. C., Daly, S. M., Feng, W., Gerding, M., and Gómez Martín,
J. C.: Meteor-Ablated Aluminum in the Mesosphere-Lower Thermosphere, J. Geophys. Res.-Space, 126, e2020JA028792, https://doi.org/10.1029/2020JA028792, 2021. a
Qiu, L., Yu, T., Yan, X., Sun, Y.-Y., Zuo, X., Yang, N., Wang, J., and Qi, Y.:
Altitudinal and Latitudinal Variations in Ionospheric Sporadic-E Layer
Obtained From FORMOSAT-3/COSMIC Radio Occultation, J. Geophys.
Res.-Space, 126, e2021JA029454, https://doi.org/10.1029/2021JA029454,
2021a. a, b
Qiu, S., Soon, W., Xue, X., Li, T., Wang, W., Jia, M., Ban, C., Fang, X., Tang,
Y., and Dou, X.: Sudden sodium layers: Their appearance and disappearance,
J. Geophys. Res.-Space, 123, 5102–5118, 2018. a
Qiu, S., Wang, N., Soon, W., Lu, G., Jia, M., Wang, X., Xue, X., Li, T., and Dou, X.: The sporadic sodium layer: a possible tracer for the conjunction between the upper and lower atmospheres, Atmos. Chem. Phys., 21, 11927–11940, https://doi.org/10.5194/acp-21-11927-2021, 2021. a
Raizada, S., Rapp, M., Lübken, F.-J., Höffner, J., Zecha, M., and
Plane, J. M. C.: Effect of ice particles on the mesospheric potassium layer at
Spitsbergen (78∘ N), J. Geophys. Res.-Atmos., 112, D08307, https://doi.org/10.1029/2005JD006938, 2007. a
Rodgers, C. D.: Inverse methods for atmospheric sounding: theory and practice,
Vol. 2, World scientific, River Edge, USA, 2000. a
Sandford, M. and Gibson, A.: Laser radar measurements of the atmospheric sodium
layer, J. Atmos. Terr. Phys., 32, 1423–1430, 1970. a
Sarkhel, S., Raizada, S., Mathews, J. D., Smith, S., Tepley, C. A., Rivera,
F. J., and Gonzalez, S. A.: Identification of large-scale billow-like
structure in the neutral sodium layer over Arecibo, J. Geophys.
Res.-Space, 117, A10301, https://doi.org/10.1029/2012JA017891, 2012. a
She, C.-Y., Liu, A. Z., Yuan, T., Yue, J., Li, T., Ban, C., and Friedman,
J. S.: MLT science enabled by atmospheric lidars, Upper Atmosphere Dynamics
and Energetics, 395–450, 2021. a
Suzuki, S., Nakamura, T., Ejiri, M. K., Tsutsumi, M., Shiokawa, K., and
Kawahara, T. D.: Simultaneous airglow, lidar, and radar measurements of
mesospheric gravity waves over Japan, J. Geophys. Res.-Atmos., 115, D24113, https://doi.org/10.1029/2010JD014674, 2010. a
Tsai, L.-C., Su, S.-Y., Liu, C.-H., Schuh, H., Wickert, J., and Alizadeh,
M. M.: Global morphology of ionospheric sporadic E layer from the
FormoSat-3/COSMIC GPS radio occultation experiment, GPS Solutions, 22, 1–12,
2018. a
University of Saskatchewan: OSIRIS data, University of Saskatchewan [data set], https://research-groups.usask.ca/osiris/data-products.php, last access: 1 September 2022. a
Vishnu Prasanth, P., Sivakumar, V., Sridharan, S., Bhavani Kumar, Y., Bencherif, H., and Narayana Rao, D.: Lidar observations of sodium layer over low latitude, Gadanki (13.5∘ N, 79.2∘ E): seasonal and nocturnal variations, Ann. Geophys., 27, 3811–3823, https://doi.org/10.5194/angeo-27-3811-2009, 2009. a
Wang, C.: New chains of space weather monitoring stations in China, Space
Weather, 8, S08001, https://doi.org/10.1029/2010SW000603, 2010. a
Whitehead, J.: Formation of the sporadic E layer in the temperate zones,
Nature, 188, 567–567, 1960. a
Whitehead, J.: Production and prediction of sporadic E, Rev. Geophys.,
8, 65–144, 1970. a
Whitehead, J.: Recent work on mid-latitude and equatorial sporadic-E, J. Atmos. Terr. Phys., 51, 401–424, 1989. a
Williams, B. P., Berkey, F. T., Sherman, J., and She, C. Y.: Coincident extremely large sporadic sodium and sporadic E layers observed in the lower thermosphere over Colorado and Utah, Ann. Geophys., 25, 3–8, https://doi.org/10.5194/angeo-25-3-2007, 2007. a
Wu, J., Feng, W., Xue, X., Marsh, D., Plane, J. M. C., and Dou, X.: The 27-Day Solar
Rotational Cycle Response in the Mesospheric Metal Layers at Low Latitudes,
Geophys. Res. Lett., 46, 7199–7206, 2019. a
Wu, J., Feng, W., Liu, H.-L., Xue, X., Marsh, D. R., and Plane, J. M. C.: Self-consistent global transport of metallic ions with WACCM-X, Atmos. Chem. Phys., 21, 15619–15630, https://doi.org/10.5194/acp-21-15619-2021, 2021. a, b, c, d
Xia, Y., Cheng, X., Li, F., Yang, Y., Jiao, J., Xun, Y., Li, Y., Du, L., Wang,
J., and Yang, G.: Diurnal variation of atmospheric metal Na layer and
nighttime top extension detected by a Na lidar with narrowband spectral
filters at Beijing, China, J. Quant. Spectrosc. Ra., 255, 107256, https://doi.org/10.1016/j.jqsrt.2020.107256, 2020. a, b
Xia, Y., Nozawa, S., Jiao, J., Wang, J., Li, F., Cheng, X., Yang, Y., Du, L.,
and Yang, G.: Statistical study on sporadic sodium layers (SSLs) based on
diurnal sodium lidar observations at Beijing, China (40.5∘ N, 116∘ E),
J. Atmos. Sol.-Terr. Phy., 212, 105512, https://doi.org/10.1016/j.jastp.2020.105512, 2021. a
Xue, X., Li, G., Dou, X., Yue, X., Yang, G., Chen, J., Chen, T., Ning, B.,
Wang, J., Wang, G., and Wan, W.: An overturning-like thermospheric Na layer and
its relevance to Ionospheric field aligned irregularity and sporadic E,
J. Atmos. Sol.-Terr. Phy., 162, 151–161, 2017. a
Yu, B., Xue, X., Kuo, C., Lu, G., Scott, C. J., Wu, J., Ma, J., Dou, X., Gao,
Q., Ning, B., , Hu, L., Wang, G., Jia, M., Yu, C., and Qie, X.: The intensification of metallic layered phenomena above
thunderstorms through the modulation of atmospheric tides, Scientific
reports, 9, 1–13, 2019a. a
Yu, B., Xue, X., Yue, X., Yang, C., Yu, C., Dou, X., Ning, B., and Hu, L.: The global climatology of the intensity of the ionospheric sporadic E layer, Atmos. Chem. Phys., 19, 4139–4151, https://doi.org/10.5194/acp-19-4139-2019, 2019b. a, b, c, d
Yu, B., Scott, C. J., Xue, X., Yue, X., and Dou, X.: Derivation of global
ionospheric Sporadic E critical frequency (foEs) data from the amplitude
variations in GPS/GNSS radio occultations, Roy. Soc. Open Sci., 7,
200320, https://doi.org/10.1098/rsos.200320, 2020. a
Yu, B., Scott, C., Xue, X., Yue, X., Chi, Y., Dou, X., and Lockwood, M.: A
signature of 27-day solar rotation in the concentration of metallic ions
within the terrestrial ionosphere, Astrophys. J., 916, 106, https://doi.org/10.3847/1538-4357/ac0886, 2021a. a
Yu, B., Xue, X., Scott, C. J., Wu, J., Yue, X., Feng, W., Chi, Y., Marsh, D. R., Liu, H., Dou, X., and Plane, J. M. C.: Interhemispheric transport of metallic ions within ionospheric sporadic E layers by the lower thermospheric meridional circulation, Atmos. Chem. Phys., 21, 4219–4230, https://doi.org/10.5194/acp-21-4219-2021, 2021c. a, b
Yuan, T., She, C.-Y., Kawahara, T. D., and Krueger, D.: Seasonal variations of
midlatitude mesospheric Na layer and their tidal period perturbations based
on full diurnal cycle Na lidar observations of 2002–2008, J.
Geophys. Res.-Atmos., 117, D11304, https://doi.org/10.1029/2011JD017031, 2012. a, b, c
Yuan, T., Fish, C., Sojka, J., Rice, D., Taylor, M., and Mitchell, N.:
Coordinated investigation of summer time mid-latitude descending E layer (Es)
perturbations using Na lidar, ionosonde, and meteor wind radar observations
over Logan, Utah (41.7∘ N, 111.8∘ W), J. Geophys. Res.-Atmos., 118, 1734–1746, 2013. a
Yuan, T., She, C., Oberheide, J., and Krueger, D. A.: Vertical tidal wind
climatology from full-diurnal-cycle temperature and Na density lidar
observations at Ft. Collins, CO (41∘ N, 105∘ W), J. Geophys.
Res.-Atmos., 119, 4600–4615, 2014a. a
Yuan, T., Wang, J., Cai, X., Sojka, J., Rice, D., Oberheide, J., and Criddle,
N.: Investigation of the seasonal and local time variations of the
high-altitude sporadic Na layer (Nas) formation and the associated
midlatitude descending E layer (Es) in lower E region, J. Geophys.
Res.-Space, 119, 5985–5999, 2014b. a, b
Yuan, T., Feng, W., Plane, J. M. C., and Marsh, D. R.: Photochemistry on the bottom side of the mesospheric Na layer, Atmos. Chem. Phys., 19, 3769–3777, https://doi.org/10.5194/acp-19-3769-2019, 2019. a, b
Yue, X., Schreiner, W. S., Zeng, Z., Kuo, Y.-H., and Xue, X.: Case study on complex sporadic E layers observed by GPS radio occultations, Atmos. Meas. Tech., 8, 225–236, https://doi.org/10.5194/amt-8-225-2015, 2015. a, b
Yue, X., Schreiner, W. S., Pedatella, N. M., and Kuo, Y.-H.: Characterizing GPS
radio occultation loss of lock due to ionospheric weather, Space Weather, 14,
285–299, 2016. a
Zeng, X., Xue, X., Dou, X., Liang, C., and Jia, M.: COSMIC GPS observations of
topographic gravity waves in the stratosphere around the Tibetan Plateau,
Sci. China Earth Sci., 60, 188–197, 2017. a
Short summary
We present a study on the climatology of the metal sodium layer in the upper atmosphere from the ground-based measurements obtained from a lidar network, the Odin satellite measurements, and a global model of meteoric sodium in the atmosphere. Comprehensively, comparisons show good agreement and some discrepancies between ground-based observations, satellite measurements, and global model simulations.
We present a study on the climatology of the metal sodium layer in the upper atmosphere from the...
Altmetrics
Final-revised paper
Preprint