Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-14979-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-14979-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
11 Dec 2019
Research article |
| 11 Dec 2019
| 11 Dec 2019
Evidence of the complexity of aerosol transport in the lower troposphere on the Namibian coast during AEROCLO-sA
Patrick Chazette
CORRESPONDING AUTHOR
Laboratoire des Sciences du Climat et de l'Environnement (LSCE),
Laboratoire mixte CEA-CNRS-UVSQ, UMR
CNRS 1572, CEA Saclay, 91191 Gif-sur-Yvette, France
Cyrille Flamant
LATMOS/IPSL, Sorbonne Université, CNRS, UVSQ, Paris, France
Julien Totems
Laboratoire des Sciences du Climat et de l'Environnement (LSCE),
Laboratoire mixte CEA-CNRS-UVSQ, UMR
CNRS 1572, CEA Saclay, 91191 Gif-sur-Yvette, France
Marco Gaetani
LATMOS/IPSL, Sorbonne Université, CNRS, UVSQ, Paris, France
Laboratoire Interuniversitaire des Systèmes Atmosphériques
(LISA) UMR CNRS 7583, Université Paris-Est-Créteil, Université
de Paris, Institut Pierre Simon Laplace, Créteil, France
Gwendoline Smith
Laboratoire des Sciences du Climat et de l'Environnement (LSCE),
Laboratoire mixte CEA-CNRS-UVSQ, UMR
CNRS 1572, CEA Saclay, 91191 Gif-sur-Yvette, France
Laboratoire Interuniversitaire des Systèmes Atmosphériques
(LISA) UMR CNRS 7583, Université Paris-Est-Créteil, Université
de Paris, Institut Pierre Simon Laplace, Créteil, France
Alexandre Baron
Laboratoire des Sciences du Climat et de l'Environnement (LSCE),
Laboratoire mixte CEA-CNRS-UVSQ, UMR
CNRS 1572, CEA Saclay, 91191 Gif-sur-Yvette, France
Xavier Landsheere
Laboratoire Interuniversitaire des Systèmes Atmosphériques
(LISA) UMR CNRS 7583, Université Paris-Est-Créteil, Université
de Paris, Institut Pierre Simon Laplace, Créteil, France
Karine Desboeufs
Laboratoire Interuniversitaire des Systèmes Atmosphériques
(LISA) UMR CNRS 7583, Université Paris-Est-Créteil, Université
de Paris, Institut Pierre Simon Laplace, Créteil, France
Jean-François Doussin
Laboratoire Interuniversitaire des Systèmes Atmosphériques
(LISA) UMR CNRS 7583, Université Paris-Est-Créteil, Université
de Paris, Institut Pierre Simon Laplace, Créteil, France
Paola Formenti
Laboratoire Interuniversitaire des Systèmes Atmosphériques
(LISA) UMR CNRS 7583, Université Paris-Est-Créteil, Université
de Paris, Institut Pierre Simon Laplace, Créteil, France
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Hendrik Fuchs, Niklas Illmann, Amalia Muñoz, Mila Ródenas, Bénédicte Picquet-Varrault, M. Rami Alfarra, Cecilia Arsene, Iustinian G. Bejan, David M. Bell, Merete Bilde, Alexander Böhmländer, Mixtli Campos-Pineda, Mathieu Cazaunau, Patrice Coll, Véronique Daële, Claudia Di Biagio, Michael Flynn, Paola Formenti, Hartmut Herrmann, Kristina Höhler, Thorsten Hohaus, Matthew S. Johnson, Eija Juurola, Niku Kivekäs, Jan Kaiser, Christos Kaltsonoudis, Paolo Laj, Dario Massabò, Federico Mazzei, Gordon McFiggans, Max R. McGillen, Abdelwahid Mellouki, Peter Mettke, Ottmar Möhler, Falk Mothes, Dennis Niedermeier, Anna Novelli, Romeo I. Olariu, Spyros N. Pandis, Iulia Patroescu-Klotz, Rosa Maria Petracca Altieri, Paolo Prati, Claudiu Roman, Albert A. Ruth, Harald Saathoff, Silvio Schmalfuß, Frank Stratmann, Virginia Vernocchi, Aristeidis Voliotis, Jens Voigtländer, Annele Virtanen, Andreas Wahner, Robert Wagner, John Wenger, Sören Zorn, Peter Wiesen, and Jean-Francois Doussin
Atmos. Meas. Tech., 19, 4165–4199, https://doi.org/10.5194/amt-19-4165-2026, https://doi.org/10.5194/amt-19-4165-2026, 2026
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Aerosol Research Discuss., https://doi.org/10.5194/ar-2026-20, https://doi.org/10.5194/ar-2026-20, 2026
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This study improves the accuracy of optical particle counters (OPCs), instruments used to measure airborne particles important for air quality and climate research. Because OPC measurements depend not only on particle size but also on composition and shape, results can be uncertain. The paper provides a standardized database of correction factors for five commercial OPCs, helping researchers produce more reliable and consistent aerosol measurements across a wide range of atmospheric conditions.
Elie Al Marj, Ambre Delater, Aline Gratien, Marie Line Torrijos, Juan Camilo Macias Rodriguez, Mathieu Cazaunau, Edouard Pangui, Antonin Bergé, Cécile Gaimoz, Thomas Bertin, Emmanuelle Mebold, Bénédicte Picquet-Varrault, Jean-François Doussin, Clément Buissot, Sophie Lanone, and Patrice Coll
EGUsphere, https://doi.org/10.5194/egusphere-2026-1743, https://doi.org/10.5194/egusphere-2026-1743, 2026
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The "PolluRisk" platform simulated two urban scenarios: standard traffic and biomass burning. Using a smog chamber, the study showed that wood heating significantly modified aerosol chemistry, with organic fractions reaching 40 % of PM1 mass. Advanced mass spectrometry identified specific tracers of oxidation and combustion. These findings improve air quality models and help investigate health effects linked to real-world pollution exposure in moderately polluted cities.
Paola Formenti, Danitza Klopper, Anais Feron, Mathieu Cazaunau, Servanne Chevaillier, Karine Desboeufs, Claudia Di Biagio, Clarissa Baldo, Cécile Gaimoz, Vincent Michoud, Cécile Mirande-Bret, Sylvain Triquet, François Hemeret, Richard Valorso, Stephen Broccardo, Andreas Namwoonde, Mattheus Hanghome, Chiara Giorio, and Stuart J. Piketh
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2026-95, https://doi.org/10.5194/essd-2026-95, 2026
Revised manuscript under review for ESSD
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The southern African west coast is highly impacted by climate change and aerosols from natural and human sources, yet observations are scarce. We present measurements (2014–2019) from the Henties Bay Aerosol Observatory in Namibia, including aerosol properties, ozone and meteorology. This unique dataset will support process studies and improve regional climate modelling.
Johannes Heuser, Claudia Di Biagio, Jérôme Yon, Mathieu Cazaunau, Antonin Bergé, Edouard Pangui, Marco Zanatta, Laura Renzi, Angela Marinoni, Chenjie Yu, Servanne Chevaillier, Daniel Ferry, Paolo Laj, Michel Maillé, Paola Formenti, Benedicte Picquet-Varrault, and Jean-Francois Doussin
EGUsphere, https://doi.org/10.5194/egusphere-2026-1867, https://doi.org/10.5194/egusphere-2026-1867, 2026
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Large simulation chamber experiments were performed to investigate the impact of non-absorbing coating on the absorption of fractal BC-containing soot. Results show the strong and combined effect of morphological modifications and mixing state heterogeneity on BC absorption, both depending on the reaction dynamics of coating formation and ageing of the coated soot. The range of measured absorption cannot be captured by common model approximations, highlighting the need for new formalisms.
Pasquale Sellitto, Maxim Eremenko, Paola Formenti, Perla Alalam, Michael Höpfner, and Claudia Di Biagio
Atmos. Meas. Tech., 19, 2751–2762, https://doi.org/10.5194/amt-19-2751-2026, https://doi.org/10.5194/amt-19-2751-2026, 2026
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The Far-infrared Outgoing Radiation Understanding and Monitoring (FORUM) mission will bring the first satellite instrument capable of observing the Earth's far infrared (FIR) spectra with a high spectral resolution. FORUM will crucially contribute to water vapour, clouds and surface observations. We found that FORUM will provide also a significant sensitivity to dust aerosol, especially in cases of large burdens of mid-to-long-range transported plumes of dust in the free and upper troposphere.
Chenjie Yu, Paola Formenti, Joel F. de Brito, Astrid Bauville, Antonin Bergé, Hichem Bouzidi, Mathieu Cazaunau, Manuela Cirtog, Claudia Di Biagio, Ludovico Di Antonio, Cécile Gaimoz, Franck Maisonneuve, Pascal Zapf, Tobias Seubert, Simone T. Andersen, Patrick Dewald, Gunther N. T. E. Türk, John N. Crowley, Alexandre Kukui, Chaoyang Xue, Cyrielle Denjean, Olivier Garrouste, Jean-Claude Etienne, Huihui Wu, James D. Allan, Dantong Liu, Yangzhou Wu, Christopher Cantrell, and Vincent Michoud
Atmos. Chem. Phys., 26, 5313–5332, https://doi.org/10.5194/acp-26-5313-2026, https://doi.org/10.5194/acp-26-5313-2026, 2026
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We presented a field measurement in a Paris suburban forest region to characterise the impacts of photochemical aging process on aerosol physical chemical properties. Photochemical production of organic aerosols increased forest fine particle mass and significantly enhanced absorption of short-wavelength sunlight. This study highlights the critical need to incorporate light absorbing carbonaceous particles formation mechanisms into models to accurately simulate their direct radiative impacts.
Zhen Yang, Bärbel Vogel, Felix Plöger, Zhixuan Bai, Dan Li, Sabine Griessbach, Lars Hoffmann, Frank G. Wienhold, Elizabeth Asher, Alexandre A. Baron, Katie R. Smith, Troy Thornberry, Jianchun Bian, and Michaela I. Hegglin
Atmos. Chem. Phys., 26, 4749–4769, https://doi.org/10.5194/acp-26-4749-2026, https://doi.org/10.5194/acp-26-4749-2026, 2026
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Balloon measurements over Lhasa, China, combined with satellite guided modelling, tracked aerosol from the 2019 Raikoke eruption through the Asian summer monsoon anticyclone. We find two altitude dependent routes into the anticyclone. It partly blocks transport but also allows entry and mixing, explaining the gradual weakening of the layers. Balloon measurements over Boulder, United States, outside the anticyclone, provide an independent check outside the region.
Laura Renzi, Claudia Di Biagio, Johannes Heuser, Marco Zanatta, Mathieu Cazaunau, Antonin Bergé, Edouard Pangui, Jérôme Yon, Tommaso Isolabella, Dario Massabò, Virginia Vernocchi, Martina Mazzini, Franziska Vogel, Chenjie Yu, Paola Formenti, Benedicte Picquet-Varrault, Jean-Francois Doussin, and Angela Marinoni
Atmos. Meas. Tech., 19, 1365–1383, https://doi.org/10.5194/amt-19-1365-2026, https://doi.org/10.5194/amt-19-1365-2026, 2026
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This study investigates how particle properties affect the accuracy of a common air pollution instrument, the dual-spot aethalometer. By combining lab experiments with real-world data from a mountain site in Italy, we found that the correction factor for this instrument varies mainly due to particle size and measurement conditions. Understanding these influences helps improve air quality monitoring, which is important for assessing pollution impacts on health and climate.
Claudia Di Biagio, Elisa Bru, Avila Orta, Servanne Chevaillier, Clarissa Baldo, Antonin Bergé, Mathieu Cazaunau, Sandra Lafon, Sophie Nowak, Edouard Pangui, Meinrat O. Andreae, Pavla Dagsson-Waldhauserova, Kebonyethata Dintwe, Konrad Kandler, James S. King, Amelie Chaput, Gregory S. Okin, Stuart Piketh, Thuraya Saeed, David Seibert, Zongbo Shi, Earle Williams, Pasquale Sellitto, and Paola Formenti
Atmos. Chem. Phys., 26, 1079–1091, https://doi.org/10.5194/acp-26-1079-2026, https://doi.org/10.5194/acp-26-1079-2026, 2026
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Spectroscopy measurements show that the absorbance of dust in the far-infrared up to 25 µm is comparable in intensity to that in the mid-infrared (3–15 µm) suggesting possible relevance for its direct radiative effect. Absorption signatures differ between Icelandic and low/mid-latitude dust due to differences in mineralogical composition. Spectral differences could be used to characterise the mineralogy and trace the origin of airborne dust based on infrared remote sensing observations.
Diana L. Pereira, Aline Gratien, Chiara Giorio, Emmanuelle Mebold, Thomas Bertin, Cécile Gaimoz, Jean-François Doussin, and Paola Formenti
Atmos. Meas. Tech., 19, 1–19, https://doi.org/10.5194/amt-19-1-2026, https://doi.org/10.5194/amt-19-1-2026, 2026
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This study provides two methods for the quantification of molecular markers to improve the description of secondary organic aerosols using chromatographic techniques coupled with mass spectrometry. Compounds from various chemical functionalities (alcohols, acids, aldehydes), from biogenic and anthropogenic origin, were identified. Improved method performance was observed for nitro compounds, which have been associated with anthropogenic activities.
Frédéric Laly, Patrick Chazette, Julien Totems, Vincent Crenn, David Ledur, and Alexandre Marpillat
Atmos. Meas. Tech., 18, 7629–7649, https://doi.org/10.5194/amt-18-7629-2025, https://doi.org/10.5194/amt-18-7629-2025, 2025
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This article presents the evolution of aerosol optical properties as derived from a Raman lidar in relation to relative humidity over the Paris area. It examines the influence of aerosol chemical compounds linked to air mass origins, as well as their relationship with the efficiency of aerosol growth. Such a study provides a better understanding of the interactions between aerosols and water vapour, which is important for reducing the uncertainties surrounding the Earth's radiative balance.
Luis Valero, Konrad Kandler, Sina Jost, Holger Tost, Luca Katarina Eichhorn, Christian von Glahn, Harald Rott, Marilena Flory, Alexandre Baron, Kathie Smith, Troy Thornberry, and Ralf Weigel
EGUsphere, https://doi.org/10.5194/egusphere-2025-5568, https://doi.org/10.5194/egusphere-2025-5568, 2025
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We developed a low-cost, balloon-lifted platform with lightweight instruments to measure particles and collect samples. We tested this platform during two field campaigns in Germany. A case study showed its ability to observe the vertical distribution of particles and how they form cloud droplets. Electronic microscope analysis of the samples identified their chemical composition. This work shows the platform is a capable tool for studying atmospheric processes.
Sandrine Bony, Basile Poujol, Brett McKim, Nicolas Rochetin, Marie Lothon, Julia Windmiller, Nicolas Maury, Clarisse Dufaux, Louis Jaffeux, Patrick Chazette, and Julien Delanoë
Atmos. Chem. Phys., 25, 17331–17362, https://doi.org/10.5194/acp-25-17331-2025, https://doi.org/10.5194/acp-25-17331-2025, 2025
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Space photographs of the Earth show that clouds form diverse, common but poorly understood cloud patterns. The analysis of observations gathered from research aircraft over the tropical ocean shows that the merging of thermals and clouds in the first kilometer of the atmosphere plays a key role in controlling the size, depth and spacing of clouds. This reveals a fundamental process through which clouds interact with each other and with their environment.
Paola Formenti, Chiara Giorio, Karine Desboeufs, Alexander Zherebker, Marco Gaetani, Clarissa Baldo, Gautier Landrot, Simona Montebello, Servanne Chevaillier, Sylvain Triquet, Guillaume Siour, Claudia Di Biagio, Francesco Battaglia, Jean-François Doussin, Anais Feron, Andreas Namwoonde, and Stuart John Piketh
Atmos. Chem. Phys., 25, 16127–16145, https://doi.org/10.5194/acp-25-16127-2025, https://doi.org/10.5194/acp-25-16127-2025, 2025
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The elemental composition and solubility of several metals, including iron, at a coastal site in Namibia in August–September 2017, indicate that natural and anthropogenic dust had different solubility depending on mineralogy but mostly on the processing by fluoride ions from marine emissions, pointing to the complexity of atmospheric--oceanic interactions in this region of the world influenced by the Benguela current and significant aerosol load.
Chiara Giorio, Anne Monod, Valerio Di Marco, Pierre Herckes, Denise Napolitano, Amy Sullivan, Gautier Landrot, Daniel Warnes, Marika Nasti, Sara D'Aronco, Agathe Gérardin, Nicolas Brun, Karine Desboeufs, Sylvain Triquet, Servanne Chevaillier, Claudia Di Biagio, Francesco Battaglia, Frédéric Burnet, Stuart J. Piketh, Andreas Namwoonde, Jean-François Doussin, and Paola Formenti
Atmos. Chem. Phys., 25, 16107–16125, https://doi.org/10.5194/acp-25-16107-2025, https://doi.org/10.5194/acp-25-16107-2025, 2025
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We present a comparison between concentrations of dissolved trace metals in pairs of total suspended particulate (TSP) and fog samples collected in Henties Bay, Namibia, during the AErosols, Radiation and CLOuds in southern Africa (AEROCLO-sA) field campaign. We found enhanced concentrations of dissolved metals in fog samples, which we attributed to metal–ligand complex formation in the early stages of particle activation into droplets that can then remain in a kinetically stable form in fog or lead to the formation of colloidal nanoparticles.
Natalia Castillo Bautista, Marco Gaetani, Leonard F. Borchert, Benjamin Poschlod, Lukas Brunner, Jana Sillmann, and Mario L. V. Martina
EGUsphere, https://doi.org/10.5194/egusphere-2025-5073, https://doi.org/10.5194/egusphere-2025-5073, 2025
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When hot temperatures and drought occur together (compound events), they can cause harmful impacts on crops and society. Using six decades of climate data, we show that such compound events repeatedly occurred in three breadbaskets of the Northern Hemisphere. These events are linked to atmospheric circulation patterns that favor heat and dryness, which in turn interact to amplify the impact. Our study contributes to understand the drivers of these events to support climate impact assessment.
Francesco Battaglia, Paola Formenti, Chiara Giorio, Mathieu Cazaunau, Edouard Pangui, Antonin Bergé, Aline Gratien, Diana L. Pereira, Thomas Bertin, Joel F. de Brito, Manolis N. Romanias, Vincent Michoud, Clarissa Baldo, Servanne Chevaillier, Gael Noyalet, Philippe Decorse, Bénédicte Picquet-Varrault, and Jean-François Doussin
Atmos. Chem. Phys., 25, 12409–12431, https://doi.org/10.5194/acp-25-12409-2025, https://doi.org/10.5194/acp-25-12409-2025, 2025
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This paper presents an experimental investigation of the interactions between glyoxal, an important volatile organic compound, and mineral dust particles of size and composition typical of natural conditions. We show that their interactions modify, in a definitive way, the concentrations of the gas phase and the surface properties of the dust, which could have important implications for the atmospheric composition and the Earth's climate.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Cathy Clerbaux, Pierre-François Coheur, Andrea Pazmiño, Michaël Sicard, Anne Boynard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
Atmos. Chem. Phys., 25, 10887–10905, https://doi.org/10.5194/acp-25-10887-2025, https://doi.org/10.5194/acp-25-10887-2025, 2025
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On 15 January 2022, the Hunga volcano erupted, releasing sulfur dioxide and water vapor into the stratosphere, impacting ozone levels over the Indian Ocean. Satellite data show the presence of a transient ozone depletion event related to the water vapor anomalies and sulfate aerosol clouds. Ozone reduction was confined to two distinct layers. On 21 January, the fifth percentile of total and stratospheric column ozone anomalies reached −18.6 and −14.5 DU, respectively.
Tanguy Jonville, Maurus Borne, Cyrille Flamant, Juan Cuesta, Olivier Bock, Pierre Bosser, Christophe Lavaysse, Andreas Fink, and Peter Knippertz
Atmos. Chem. Phys., 25, 9765–9786, https://doi.org/10.5194/acp-25-9765-2025, https://doi.org/10.5194/acp-25-9765-2025, 2025
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Tropical waves structure the atmosphere. Four types of tropical waves (equatorial Rossby – ER, Kelvin, MRG-TD1, and MRG-TD2 – mixed Rossby gravity–tropical depressions) are studied using filters, satellite measurements, and in situ data from the Clouds–Atmosphere Dynamics–Dust Interaction in West Africa (CADDIWA) campaign held in September 2021 in Cabo Verde. ER waves impact temperature and humidity above 2500 m, MRG-TD1 around 3500 m, and MRG-TD2 around 2000 m. Interactions between these waves favor tropical cyclone formation.
Daniele Zannoni, Hans Christian Steen-Larsen, Harald Sodemann, Iris Thurnherr, Cyrille Flamant, Patrick Chazette, Julien Totems, Martin Werner, and Myriam Raybaut
Atmos. Chem. Phys., 25, 9471–9495, https://doi.org/10.5194/acp-25-9471-2025, https://doi.org/10.5194/acp-25-9471-2025, 2025
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High-resolution airborne observations reveal that mixing between the free troposphere and surface evapotranspiration flux primarily modulates the water vapor isotopic composition in the lower troposphere. Water vapor isotope structure variations occur on the scale of hundreds of meters, underlining the utility of stable isotopes for studying microscale atmospheric dynamics. This study also provides the basis for better validation of water vapor isotope remote sensing retrievals with surface observations.
Mégane Ventura, Fabien Waquet, Isabelle Chiapello, Gérard Brogniez, Frédéric Parol, Frédérique Auriol, Rodrigue Loisil, Cyril Delegove, Luc Blarel, Oleg Dubovik, Marc Mallet, Cyrille Flamant, and Paola Formenti
Atmos. Meas. Tech., 18, 4005–4024, https://doi.org/10.5194/amt-18-4005-2025, https://doi.org/10.5194/amt-18-4005-2025, 2025
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Biomass-burning aerosols (BBAs) from Central Africa are transported above stratocumulus clouds. The absorption of solar energy by aerosols induces warming, altering the cloud dynamics. We developed an approach that combines polarimeter and lidar to quantify this. This methodology is assessed during the AEROCLO-sA (AErosol RadiatiOn and CLOud in Southern Africa) campaign. To validate it, we used irradiance measurements acquired during aircraft spiral descents. A major perspective is the generalization of this method to the global level.
Abdulaziz T. Yakubu, Danitza Klopper, Henno Havenga, Roelof Burger, Paola Formenti, and Stuart J. Piketh
EGUsphere, https://doi.org/10.5194/egusphere-2025-1827, https://doi.org/10.5194/egusphere-2025-1827, 2025
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Low-level inversions experienced along the Namibia coast and adjacent ocean have implications for air pollutant dispersion and low clouds. These affect air quality, human health, radiative forcing and climate change. We used reanalysis and satellite datasets to understand inversion properties over the region. The result shows inversion prominence at night and in winter, seasonally influences pollutant trapping and initiates stratocumulus clouds formation, but is not liable for their extent.
Johannes Heuser, Claudia Di Biagio, Jérôme Yon, Mathieu Cazaunau, Antonin Bergé, Edouard Pangui, Marco Zanatta, Laura Renzi, Angela Marinoni, Satoshi Inomata, Chenjie Yu, Vera Bernardoni, Servanne Chevaillier, Daniel Ferry, Paolo Laj, Michel Maillé, Dario Massabò, Federico Mazzei, Gael Noyalet, Hiroshi Tanimoto, Brice Temime-Roussel, Roberta Vecchi, Virginia Vernocchi, Paola Formenti, Bénédicte Picquet-Varrault, and Jean-François Doussin
Atmos. Chem. Phys., 25, 6407–6428, https://doi.org/10.5194/acp-25-6407-2025, https://doi.org/10.5194/acp-25-6407-2025, 2025
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The spectral optical properties of combustion soot aerosols with varying black (BC) and brown carbon (BrC) content were studied in an atmospheric simulation chamber. Measurements of the mass spectral absorption cross section (MAC), supplemented by literature data, allowed us to establish a generalised exponential relationship between the spectral absorption and the elemental-to-total-carbon ratio (EC / TC) in soot. This relationship can provide a useful tool for modelling the properties of soot.
Patrick Chazette, Julien Totems, and Frédéric Laly
Atmos. Meas. Tech., 18, 2681–2699, https://doi.org/10.5194/amt-18-2681-2025, https://doi.org/10.5194/amt-18-2681-2025, 2025
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The use of active remote sensing instruments to sample the atmospheric environment requires accurate calibration that is stable over time so that measurements are reproducible. This is the case for measurements of atmospheric water vapour using Raman lidar, which are of growing interest in the context of climate risks such as extreme precipitation. This study addresses this issue. It is based on six campaigns spread over a period of 7 years between 2016 and 2022.
Simone T. Andersen, Rolf Sander, Patrick Dewald, Laura Wüst, Tobias Seubert, Gunther N. T. E. Türk, Jan Schuladen, Max R. McGillen, Chaoyang Xue, Abdelwahid Mellouki, Alexandre Kukui, Vincent Michoud, Manuela Cirtog, Mathieu Cazaunau, Astrid Bauville, Hichem Bouzidi, Paola Formenti, Cyrielle Denjean, Jean-Claude Etienne, Olivier Garrouste, Christopher Cantrell, Jos Lelieveld, and John N. Crowley
Atmos. Chem. Phys., 25, 5893–5909, https://doi.org/10.5194/acp-25-5893-2025, https://doi.org/10.5194/acp-25-5893-2025, 2025
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Measurements and modelling of reactive nitrogen gases observed in a suburban temperate forest in Rambouillet, France, circa 50 km southwest of Paris in 2022 indicate that the biosphere rapidly scavenges organic nitrates of mixed biogenic and anthropogenic origin, resulting in short lifetimes for, for example, alkyl nitrates and peroxy nitrates.
Diana L. Pereira, Chiara Giorio, Aline Gratien, Alexander Zherebker, Gael Noyalet, Servanne Chevaillier, Stéphanie Alage, Elie Almarj, Antonin Bergé, Thomas Bertin, Mathieu Cazaunau, Patrice Coll, Ludovico Di Antonio, Sergio Harb, Johannes Heuser, Cécile Gaimoz, Oscar Guillemant, Brigitte Language, Olivier Lauret, Camilo Macias, Franck Maisonneuve, Bénédicte Picquet-Varrault, Raquel Torres, Sylvain Triquet, Pascal Zapf, Lelia Hawkins, Drew Pronovost, Sydney Riley, Pierre-Marie Flaud, Emilie Perraudin, Pauline Pouyes, Eric Villenave, Alexandre Albinet, Olivier Favez, Robin Aujay-Plouzeau, Vincent Michoud, Christopher Cantrell, Manuela Cirtog, Claudia Di Biagio, Jean-François Doussin, and Paola Formenti
Atmos. Chem. Phys., 25, 4885–4905, https://doi.org/10.5194/acp-25-4885-2025, https://doi.org/10.5194/acp-25-4885-2025, 2025
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In order to study aerosols in environments influenced by anthropogenic and biogenic emissions, we performed analyses of samples collected during the ACROSS (Atmospheric Chemistry Of the Suburban Forest) campaign in summer 2022 in the greater Paris area. After analysis of the chemical composition by means of total carbon determination and high-resolution mass spectrometry, this work highlights the influence of anthropogenic inputs on the chemical composition of both urban and forested areas.
Ludovico Di Antonio, Matthias Beekmann, Guillaume Siour, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Joel F. de Brito, Paola Formenti, Cecile Gaimoz, Olivier Garret, Aline Gratien, Valérie Gros, Martial Haeffelin, Lelia N. Hawkins, Simone Kotthaus, Gael Noyalet, Diana L. Pereira, Jean-Eudes Petit, Eva Drew Pronovost, Véronique Riffault, Chenjie Yu, Gilles Foret, Jean-François Doussin, and Claudia Di Biagio
Atmos. Chem. Phys., 25, 4803–4831, https://doi.org/10.5194/acp-25-4803-2025, https://doi.org/10.5194/acp-25-4803-2025, 2025
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The summer of 2022 has been considered a proxy for future climate scenarios due to its hot and dry conditions. In this paper, we use the measurements from the Atmospheric Chemistry of the Suburban Forest (ACROSS) campaign, conducted in the Paris area in June–July 2022, along with observations from existing networks, to evaluate a 3D chemistry transport model (WRF–CHIMERE) simulation. Results are shown to be satisfactory, allowing us to explain the gas and aerosol variability at the campaign sites.
Ludovico Di Antonio, Claudia Di Biagio, Paola Formenti, Aline Gratien, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Patrice Coll, Barbara D'Anna, Joel F. de Brito, David O. De Haan, Juliette R. Dignum, Shravan Deshmukh, Olivier Favez, Pierre-Marie Flaud, Cecile Gaimoz, Lelia N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Emilie Perraudin, Jean-Eudes Petit, Prodip Acharja, Laurent Poulain, Pauline Pouyes, Eva Drew Pronovost, Véronique Riffault, Kanuri I. Roundtree, Marwa Shahin, Guillaume Siour, Eric Villenave, Pascal Zapf, Gilles Foret, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 25, 3161–3189, https://doi.org/10.5194/acp-25-3161-2025, https://doi.org/10.5194/acp-25-3161-2025, 2025
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The spectral complex refractive index (CRI) and single scattering albedo were retrieved from submicron aerosol measurements at three sites within the greater Paris area during the ACROSS field campaign (June–July 2022). Measurements revealed urban emission impact on surrounding areas. CRI full period averages at 520 nm were 1.41 – 0.037i (urban), 1.52 – 0.038i (peri-urban), and 1.50 – 0.025i (rural). Organic aerosols dominated the aerosol mass and contributed up to 22 % of absorption at 370 nm.
Alexandre Mass, Hendrik Andersen, Jan Cermak, Paola Formenti, Eva Pauli, and Julian Quinting
Atmos. Chem. Phys., 25, 491–510, https://doi.org/10.5194/acp-25-491-2025, https://doi.org/10.5194/acp-25-491-2025, 2025
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This study investigates the interaction between smoke aerosols and fog and low clouds (FLCs) in the Namib Desert between June and October. Here, a satellite-based dataset of FLCs, reanalysis data and machine learning are used to systematically analyze FLC persistence under different aerosol loadings. Aerosol plumes are shown to modify local thermodynamics, which increase FLC persistence. But fully disentangling aerosol effects from meteorological ones remains a challenge.
Michaël Sicard, Alexandre Baron, Marion Ranaivombola, Dominique Gantois, Tristan Millet, Pasquale Sellitto, Nelson Bègue, Hassan Bencherif, Guillaume Payen, Nicolas Marquestaut, and Valentin Duflot
Atmos. Chem. Phys., 25, 367–381, https://doi.org/10.5194/acp-25-367-2025, https://doi.org/10.5194/acp-25-367-2025, 2025
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This study quantifies the radiative impact over Réunion Island (21° S, 55° E) of the aerosols and water vapor injected into the stratosphere by the Hunga volcano in the South Pacific. The overall aerosol and water vapor impact on the Earth’s radiation budget for the whole period is negative (cooling, -0.82 ± 0.35 W m-2) and dominated by the aerosols. At the Earth’s surface, aerosols are the main drivers and produce a negative (cooling, -1.04 ± 0.36 W m-2) radiative impact.
Cedric G. Ngoungue Langue, Christophe Lavaysse, and Cyrille Flamant
Nat. Hazards Earth Syst. Sci., 25, 147–168, https://doi.org/10.5194/nhess-25-147-2025, https://doi.org/10.5194/nhess-25-147-2025, 2025
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The present study addresses the predictability of heat waves at subseasonal timescales in West African cities over the period 2001–2020. Two models, the European Centre for Medium-Range Weather Forecasts (ECMWF) and the UK Met Office models, were evaluated using two reanalyses: ERA5 and MERRA. The results suggest that at subseasonal timescales, the forecast models provide a better forecast than climatology, but the hit rate and false alarm rate are sub-optimal.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven G. Howell
Atmos. Chem. Phys., 24, 13849–13864, https://doi.org/10.5194/acp-24-13849-2024, https://doi.org/10.5194/acp-24-13849-2024, 2024
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Using airborne measurements over the southeast Atlantic Ocean, we examined how much moisture aerosols take up during Africa’s biomass burning season. Our study revealed the important role of organic aerosols and introduced a predictive model for moisture uptake, accounting for organics, sulfate, and black carbon, summarizing results from various campaigns. These findings improve our understanding of aerosol–moisture interactions and their radiative effects in this climatically critical region.
Frédéric Laly, Patrick Chazette, Julien Totems, Jérémy Lagarrigue, Laurent Forges, and Cyrille Flamant
Earth Syst. Sci. Data, 16, 5579–5602, https://doi.org/10.5194/essd-16-5579-2024, https://doi.org/10.5194/essd-16-5579-2024, 2024
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We present a dataset of water vapor mixing ratio profiles acquired during the Water Vapor Lidar Network Assimilation campaign in fall and winter 2022 and summer 2023, using three lidar systems deployed on the western Mediterranean coastline. This innovative campaign provides access to lower-tropospheric water vapor variability to constrain meteorological forecasting models. The scientific objective is to improve forecasting of heavy-precipation events that lead to flash floods and landslides.
Laura T. Massano, Giorgia Fosser, Marco Gaetani, and Cécile Caillaud
Nat. Hazards Earth Syst. Sci., 24, 4293–4315, https://doi.org/10.5194/nhess-24-4293-2024, https://doi.org/10.5194/nhess-24-4293-2024, 2024
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Traditional wine-growing regions are threatened by expected climate change. Climate models and observations are used to calculate bioclimatic indices based on both temperature and precipitation. These indices are correlated with grape productivity in two wine-growing regions in Italy. This analysis paves the way for using climate models to study how climate change will affect wine production in the future.
Paola Formenti and Claudia Di Biagio
Earth Syst. Sci. Data, 16, 4995–5007, https://doi.org/10.5194/essd-16-4995-2024, https://doi.org/10.5194/essd-16-4995-2024, 2024
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Particles from deserts and semi-vegetated areas (mineral dust) are important for Earth's climate and human health, notably depending on their size. In this paper we collect and make a synthesis of a body of these observations since 1972 in order to provide researchers modeling Earth's climate and developing satellite observations from space with a simple way of confronting their results and understanding their validity.
Marco Gaetani, Gabriele Messori, Francesco S. R. Pausata, Shivangi Tiwari, M. Carmen Alvarez Castro, and Qiong Zhang
Clim. Past, 20, 1735–1759, https://doi.org/10.5194/cp-20-1735-2024, https://doi.org/10.5194/cp-20-1735-2024, 2024
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Palaeoclimate reconstructions suggest that, around 6000 years ago, a greening of the Sahara took place, accompanied by climate changes in the Northern Hemisphere at middle to high latitudes. In this study, a climate model is used to investigate how this drastic environmental change in the Sahara impacted remote regions. Specifically, climate simulations reveal significant modifications in atmospheric circulation over the North Atlantic, affecting North American and European climates.
Maëlie Chazette, Patrick Chazette, Ilja M. Reiter, Xiaoxia Shang, Julien Totems, Jean-Philippe Orts, Irène Xueref-Remy, and Nicolas Montes
Biogeosciences, 21, 3289–3303, https://doi.org/10.5194/bg-21-3289-2024, https://doi.org/10.5194/bg-21-3289-2024, 2024
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The approach presented is original in its coupling between field observations and airborne lidar observations. It has been applied to an instrumented reference forest site in the south of France, which is heavily impacted by climate change. It leads to the evaluation of tree heights and ends with assessments of aerial and root carbon stocks. A detailed assessment of uncertainties is presented to add a level of reliability to the scientific products delivered.
Nelson Bègue, Alexandre Baron, Gisèle Krysztofiak, Gwenaël Berthet, Corinna Kloss, Fabrice Jégou, Sergey Khaykin, Marion Ranaivombola, Tristan Millet, Thierry Portafaix, Valentin Duflot, Philippe Keckhut, Hélène Vérèmes, Guillaume Payen, Mahesh Kumar Sha, Pierre-François Coheur, Cathy Clerbaux, Michaël Sicard, Tetsu Sakai, Richard Querel, Ben Liley, Dan Smale, Isamu Morino, Osamu Uchino, Tomohiro Nagai, Penny Smale, John Robinson, and Hassan Bencherif
Atmos. Chem. Phys., 24, 8031–8048, https://doi.org/10.5194/acp-24-8031-2024, https://doi.org/10.5194/acp-24-8031-2024, 2024
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During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean basin experienced significant perturbations. Numerical models indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers.
Chenjie Yu, Edouard Pangui, Kevin Tu, Mathieu Cazaunau, Maxime Feingesicht, Landsheere Xavier, Thierry Bourrianne, Vincent Michoud, Christopher Cantrell, Timothy B. Onasch, Andrew Freedman, and Paola Formenti
Atmos. Meas. Tech., 17, 3419–3437, https://doi.org/10.5194/amt-17-3419-2024, https://doi.org/10.5194/amt-17-3419-2024, 2024
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To meet the requirements for measuring aerosol optical properties on airborne platforms and conducting dual-wavelength measurements, we introduced A2S2, an airborne dual-wavelength cavity-attenuated phase-shift single monitor. This study reports the results in the laboratory and an aircraft campaign over Paris and its surrounding regions. The results demonstrate A2S2's reliability in measuring aerosol optical properties at both wavelengths and its suitability for future aircraft campaigns.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Cyrille Flamant, Jean-Pierre Chaboureau, Marco Gaetani, Kerstin Schepanski, and Paola Formenti
Atmos. Chem. Phys., 24, 4265–4288, https://doi.org/10.5194/acp-24-4265-2024, https://doi.org/10.5194/acp-24-4265-2024, 2024
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In the austral dry season, the atmospheric composition over southern Africa is dominated by biomass burning aerosols and terrigenous aerosols (so-called mineral dust). This study suggests that the radiative effect of biomass burning aerosols needs to be taken into account to properly forecast dust emissions in Namibia.
Anil Kumar Mandariya, Junteng Wu, Anne Monod, Paola Formenti, Bénédicte Picquet-Varrault, Mathieu Cazaunau, Stephan Mertes, Laurent Poulain, Antonin Berge, Edouard Pangui, Andreas Tilgner, Thomas Schaefer, Liang Wen, Hartmut Herrmann, and Jean-François Doussin
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-206, https://doi.org/10.5194/amt-2023-206, 2024
Publication in AMT not foreseen
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An optimized and controlled protocol for generating quasi-adiabatic expansion clouds under simulated dark and light conditions was presented. The irradiated clouds clearly showed a gradual activation of seed particles into droplets. In contrast, non-irradiated clouds faced a flash activation. This paper will lay the foundation for multiphase photochemical studies implying water-soluble volatile organic compounds and particulate matter formation during cloud formation-evaporation cycles.
Karine Desboeufs, Paola Formenti, Raquel Torres-Sánchez, Kerstin Schepanski, Jean-Pierre Chaboureau, Hendrik Andersen, Jan Cermak, Stefanie Feuerstein, Benoit Laurent, Danitza Klopper, Andreas Namwoonde, Mathieu Cazaunau, Servanne Chevaillier, Anaïs Feron, Cécile Mirande-Bret, Sylvain Triquet, and Stuart J. Piketh
Atmos. Chem. Phys., 24, 1525–1541, https://doi.org/10.5194/acp-24-1525-2024, https://doi.org/10.5194/acp-24-1525-2024, 2024
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This study investigates the fractional solubility of iron (Fe) in dust particles along the coast of Namibia, a critical region for the atmospheric Fe supply of the South Atlantic Ocean. Our results suggest a possible two-way interplay whereby marine biogenic emissions from the coastal marine ecosystems into the atmosphere would increase the solubility of Fe-bearing dust by photo-reduction processes. The subsequent deposition of soluble Fe could act to further enhance marine biogenic emissions.
Maurus Borne, Peter Knippertz, Martin Weissmann, Benjamin Witschas, Cyrille Flamant, Rosimar Rios-Berrios, and Peter Veals
Atmos. Meas. Tech., 17, 561–581, https://doi.org/10.5194/amt-17-561-2024, https://doi.org/10.5194/amt-17-561-2024, 2024
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This study assesses the quality of Aeolus wind measurements over the tropical Atlantic. The results identified the accuracy and precision of the Aeolus wind measurements and the potential source of errors. For instance, the study revealed atmospheric conditions that can deteriorate the measurement quality, such as weaker laser signal in cloudy or dusty conditions, and confirmed the presence of an orbital-dependant bias. These results can help to improve the Aeolus wind measurement algorithm.
Gaëlle de Coëtlogon, Adrien Deroubaix, Cyrille Flamant, Laurent Menut, and Marco Gaetani
Atmos. Chem. Phys., 23, 15507–15521, https://doi.org/10.5194/acp-23-15507-2023, https://doi.org/10.5194/acp-23-15507-2023, 2023
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Using a numerical atmospheric model, we found that cooling sea surface temperatures along the southern coast of West Africa in July cause the “little dry season”. This effect reduces humidity and pollutant transport inland, potentially enhancing West Africa's synoptic and seasonal forecasting.
Patrick Chazette and Jean-Christophe Raut
Atmos. Meas. Tech., 16, 5847–5861, https://doi.org/10.5194/amt-16-5847-2023, https://doi.org/10.5194/amt-16-5847-2023, 2023
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The vertical profiles of the effective radii of ice crystals and ice water content in Arctic semi-transparent stratiform clouds were assessed using quantitative ground-based lidar measurements. The field campaign was part of the Pollution in the ARCtic System (PARCS) project which took place from 13 to 26 May 2016 in Hammerfest (70° 39′ 48″ N, 23° 41′ 00″ E). We show that under certain cloud conditions, lidar measurement combined with a dedicated algorithmic approach is an efficient tool.
Leonie Villiger, Marina Dütsch, Sandrine Bony, Marie Lothon, Stephan Pfahl, Heini Wernli, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Cyrille Flamant, Alfons Schwarzenboeck, Martin Werner, and Franziska Aemisegger
Atmos. Chem. Phys., 23, 14643–14672, https://doi.org/10.5194/acp-23-14643-2023, https://doi.org/10.5194/acp-23-14643-2023, 2023
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This study evaluates three numerical simulations performed with an isotope-enabled weather forecast model and investigates the coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. We show that the simulations reproduce key characteristics of shallow trade-wind clouds as observed during the field experiment EUREC4A and that the spatial distribution of stable-water-vapour isotopes is shaped by the overturning circulation associated with these clouds.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
EGUsphere, https://doi.org/10.5194/egusphere-2023-2645, https://doi.org/10.5194/egusphere-2023-2645, 2023
Preprint withdrawn
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The eruption of the Hunga Tonga volcano in January 2022 released substantial amounts of aerosols, sulfur dioxide, and water vapor into the stratosphere. Satellite and ground instruments followed the displacement of the volcanic aerosol plume and its impact on ozone levels over the Indian Ocean. Ozone data reveal the presence of a persistent ozone mini-hole structure from 17 January to 22 January, with most ozone depletion occurring within the ozone layer at the location of the aerosol plume.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, and Paola Formenti
EGUsphere, https://doi.org/10.5194/egusphere-2023-2319, https://doi.org/10.5194/egusphere-2023-2319, 2023
Preprint archived
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Our study examined the interaction between atmospheric particles and moisture over the south-eastern Atlantic Ocean during the biomass burning seasons in Africa. We found that organic components of these particles play a more important role in aerosol-moisture interactions than previously expected. This discovery is important as such interactions impact radiation and climate. Current climate models might need better representations of the moisture-absorbing properties of organic aerosols.
Thomas Audoux, Benoit Laurent, Karine Desboeufs, Gael Noyalet, Franck Maisonneuve, Olivier Lauret, and Servanne Chevaillier
Atmos. Chem. Phys., 23, 13485–13503, https://doi.org/10.5194/acp-23-13485-2023, https://doi.org/10.5194/acp-23-13485-2023, 2023
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In the Paris region, a campaign was conducted to study wet deposition of aerosol particles during rainfall events. Simultaneous measurements of aerosol and wet deposition allowed us to discuss their transfer from the atmosphere to rain. Chemical evolution within events revealed meteorology, atmospheric conditions and local vs. long range sources as key factors. This study highlights the variability of wet deposition and the need to consider event-specific factors to understand its mechanisms.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Clarissa Baldo, Paola Formenti, Claudia Di Biagio, Gongda Lu, Congbo Song, Mathieu Cazaunau, Edouard Pangui, Jean-Francois Doussin, Pavla Dagsson-Waldhauserova, Olafur Arnalds, David Beddows, A. Robert MacKenzie, and Zongbo Shi
Atmos. Chem. Phys., 23, 7975–8000, https://doi.org/10.5194/acp-23-7975-2023, https://doi.org/10.5194/acp-23-7975-2023, 2023
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This paper presents new shortwave spectral complex refractive index and single scattering albedo data for Icelandic dust. Our results show that the imaginary part of the complex refractive index of Icelandic dust is at the upper end of the range of low-latitude dust. Furthermore, we observed that Icelandic dust is more absorbing towards the near-infrared, which we attribute to its high magnetite content. These findings are important for modeling dust aerosol radiative effects in the Arctic.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Cedric Gacial Ngoungue Langue, Christophe Lavaysse, Mathieu Vrac, and Cyrille Flamant
Nat. Hazards Earth Syst. Sci., 23, 1313–1333, https://doi.org/10.5194/nhess-23-1313-2023, https://doi.org/10.5194/nhess-23-1313-2023, 2023
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Heat waves (HWs) are climatic hazards that affect the planet. We assess here uncertainties encountered in the process of HW detection and analyse their recent trends in West Africa using reanalysis data. Three types of uncertainty have been investigated. We identified 6 years with higher frequency of HWs, possibly due to higher sea surface temperatures in the equatorial Atlantic. We noticed an increase in HW characteristics during the last decade, which could be a consequence of climate change.
Michael John Weston, Stuart John Piketh, Frédéric Burnet, Stephen Broccardo, Cyrielle Denjean, Thierry Bourrianne, and Paola Formenti
Atmos. Chem. Phys., 22, 10221–10245, https://doi.org/10.5194/acp-22-10221-2022, https://doi.org/10.5194/acp-22-10221-2022, 2022
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An aerosol-aware microphysics scheme is evaluated for fog cases in Namibia. AEROCLO-sA campaign observations are used to access and parameterise the model. The model cloud condensation nuclei activation is lower than the observations. The scheme is designed for clouds with updrafts, while fog typically forms in stable conditions. A pseudo updraft speed assigned to the lowest model levels helps achieve more realistic cloud droplet number concentration and size distribution in the model.
Caroline Dang, Michal Segal-Rozenhaimer, Haochi Che, Lu Zhang, Paola Formenti, Jonathan Taylor, Amie Dobracki, Sara Purdue, Pui-Shan Wong, Athanasios Nenes, Arthur Sedlacek III, Hugh Coe, Jens Redemann, Paquita Zuidema, Steven Howell, and James Haywood
Atmos. Chem. Phys., 22, 9389–9412, https://doi.org/10.5194/acp-22-9389-2022, https://doi.org/10.5194/acp-22-9389-2022, 2022
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Transmission electron microscopy was used to analyze aged African smoke particles and how the smoke interacts with the marine atmosphere. We found that the volatility of organic aerosol increases with biomass burning plume age, that black carbon is often mixed with potassium salts and that the marine atmosphere can incorporate Na and Cl into smoke particles. Marine salts are more processed when mixed with smoke plumes, and there are interesting Cl-rich yet Na-absent marine particles.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Arthur J. Sedlacek III, Ernie R. Lewis, Amie Dobracki, Jenny P. S. Wong, Paola Formenti, Steven G. Howell, and Athanasios Nenes
Atmos. Chem. Phys., 22, 9199–9213, https://doi.org/10.5194/acp-22-9199-2022, https://doi.org/10.5194/acp-22-9199-2022, 2022
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Widespread biomass burning (BB) events occur annually in Africa and contribute ~ 1 / 3 of global BB emissions, which contain a large family of light-absorbing organics, known as brown carbon (BrC), whose absorption of incident radiation is difficult to estimate, leading to large uncertainties in the global radiative forcing estimation. This study quantifies the BrC absorption of aged BB particles and highlights the potential presence of absorbing iron oxides in this climatically important region.
Jean-Pierre Chaboureau, Laurent Labbouz, Cyrille Flamant, and Alma Hodzic
Atmos. Chem. Phys., 22, 8639–8658, https://doi.org/10.5194/acp-22-8639-2022, https://doi.org/10.5194/acp-22-8639-2022, 2022
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Ground-based, spaceborne and rare airborne observations of biomass burning aerosols (BBAs) during the AEROCLO-sA field campaign in 2017 are complemented with convection-permitting simulations with online trajectories. The results show that the radiative effect of the BBA accelerates the southern African easterly jet and generates upward motions that transport the BBAs to higher altitudes and farther southwest.
Enza Di Tomaso, Jerónimo Escribano, Sara Basart, Paul Ginoux, Francesca Macchia, Francesca Barnaba, Francesco Benincasa, Pierre-Antoine Bretonnière, Arnau Buñuel, Miguel Castrillo, Emilio Cuevas, Paola Formenti, María Gonçalves, Oriol Jorba, Martina Klose, Lucia Mona, Gilbert Montané Pinto, Michail Mytilinaios, Vincenzo Obiso, Miriam Olid, Nick Schutgens, Athanasios Votsis, Ernest Werner, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2785–2816, https://doi.org/10.5194/essd-14-2785-2022, https://doi.org/10.5194/essd-14-2785-2022, 2022
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MONARCH reanalysis of desert dust aerosols extends the existing observation-based information for mineral dust monitoring by providing 3-hourly upper-air, surface and total column key geophysical variables of the dust cycle over Northern Africa, the Middle East and Europe, at a 0.1° horizontal resolution in a rotated grid, from 2007 to 2016. This work provides evidence of the high accuracy of this data set and its suitability for air quality and health and climate service applications.
Axel Fouqueau, Manuela Cirtog, Mathieu Cazaunau, Edouard Pangui, Jean-François Doussin, and Bénédicte Picquet-Varrault
Atmos. Chem. Phys., 22, 6411–6434, https://doi.org/10.5194/acp-22-6411-2022, https://doi.org/10.5194/acp-22-6411-2022, 2022
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Biogenic volatile organic compounds are intensely emitted by forests and crops and react with the nitrate radical during the nighttime to form functionalized products. The purpose of this study is to furnish kinetic and mechanistic data for terpinolene and β-caryophyllene, using simulation chamber experiments. Rate constants have been measured using both relative and absolute methods, and mechanistic studies have been conducted in order to identify and quantify the main reaction products.
Cyrille Flamant, Marco Gaetani, Jean-Pierre Chaboureau, Patrick Chazette, Juan Cuesta, Stuart John Piketh, and Paola Formenti
Atmos. Chem. Phys., 22, 5701–5724, https://doi.org/10.5194/acp-22-5701-2022, https://doi.org/10.5194/acp-22-5701-2022, 2022
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Rivers of smoke extend from tropical southern Africa towards the Indian Ocean during the winter fire season, controlled by the interaction of tropical easterly waves, and westerly waves at mid latitudes. During the AEROCLO-sA field campaign in 2017, a river of smoke was directly observed over Namibia. In this paper, the evolution and atmospheric drivers of the river of smoke are described, and the role of a mid-latitude cut-off low in lifting the smoke to the upper troposphere is highlighted.
Sandrine Bony, Marie Lothon, Julien Delanoë, Pierre Coutris, Jean-Claude Etienne, Franziska Aemisegger, Anna Lea Albright, Thierry André, Hubert Bellec, Alexandre Baron, Jean-François Bourdinot, Pierre-Etienne Brilouet, Aurélien Bourdon, Jean-Christophe Canonici, Christophe Caudoux, Patrick Chazette, Michel Cluzeau, Céline Cornet, Jean-Philippe Desbios, Dominique Duchanoy, Cyrille Flamant, Benjamin Fildier, Christophe Gourbeyre, Laurent Guiraud, Tetyana Jiang, Claude Lainard, Christophe Le Gac, Christian Lendroit, Julien Lernould, Thierry Perrin, Frédéric Pouvesle, Pascal Richard, Nicolas Rochetin, Kevin Salaün, Alfons Schwarzenboeck, Guillaume Seurat, Bjorn Stevens, Julien Totems, Ludovic Touzé-Peiffer, Gilles Vergez, Jessica Vial, Leonie Villiger, and Raphaela Vogel
Earth Syst. Sci. Data, 14, 2021–2064, https://doi.org/10.5194/essd-14-2021-2022, https://doi.org/10.5194/essd-14-2021-2022, 2022
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The French ATR42 research aircraft participated in the EUREC4A international field campaign that took place in 2020 over the tropical Atlantic, east of Barbados. We present the extensive instrumentation of the aircraft, the research flights and the different measurements. We show that the ATR measurements of humidity, wind, aerosols and cloudiness in the lower atmosphere are robust and consistent with each other. They will make it possible to advance understanding of cloud–climate interactions.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Karine Desboeufs, Franck Fu, Matthieu Bressac, Antonio Tovar-Sánchez, Sylvain Triquet, Jean-François Doussin, Chiara Giorio, Patrick Chazette, Julie Disnaquet, Anaïs Feron, Paola Formenti, Franck Maisonneuve, Araceli Rodríguez-Romero, Pascal Zapf, François Dulac, and Cécile Guieu
Atmos. Chem. Phys., 22, 2309–2332, https://doi.org/10.5194/acp-22-2309-2022, https://doi.org/10.5194/acp-22-2309-2022, 2022
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This article reports the first concurrent sampling of wet deposition samples and surface seawater and was performed during the PEACETIME cruise in the remote Mediterranean (May–June 2017). Through the chemical composition of trace metals (TMs) in these samples, it emphasizes the decrease of atmospheric metal pollution in this area during the last few decades and the critical role of wet deposition as source of TMs for Mediterranean surface seawater, especially for intense dust deposition events.
Patrick Chazette, Alexandre Baron, and Cyrille Flamant
Atmos. Chem. Phys., 22, 1271–1292, https://doi.org/10.5194/acp-22-1271-2022, https://doi.org/10.5194/acp-22-1271-2022, 2022
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Within the framework of the international EUREC4A project, horizontal lidar measurements were carried out over Barbados from the French research aircraft ATR-42. These measurements highlighted the strong heterogeneity of the aerosol field (mainly dust and biomass burning aerosols) and therefore of the associated optical properties. This heterogeneity varies according to meteorological conditions and could significantly modulate the climatic impact of aerosols trapped over the tropical Atlantic.
Paola Formenti, Claudia Di Biagio, Yue Huang, Jasper Kok, Marc Daniel Mallet, Damien Boulanger, and Mathieu Cazaunau
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-403, https://doi.org/10.5194/amt-2021-403, 2021
Publication in AMT not foreseen
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This paper provides with standardized correction factors for the measurements of the most common instruments used in the atmosphere to measure the concentration per size of aerosol particles. These correction factors are provided to users with supplementary information for their use.
Matthieu Bressac, Thibaut Wagener, Nathalie Leblond, Antonio Tovar-Sánchez, Céline Ridame, Vincent Taillandier, Samuel Albani, Sophie Guasco, Aurélie Dufour, Stéphanie H. M. Jacquet, François Dulac, Karine Desboeufs, and Cécile Guieu
Biogeosciences, 18, 6435–6453, https://doi.org/10.5194/bg-18-6435-2021, https://doi.org/10.5194/bg-18-6435-2021, 2021
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Phytoplankton growth is limited by the availability of iron in about 50 % of the ocean. Atmospheric deposition of desert dust represents a key source of iron. Here, we present direct observations of dust deposition in the Mediterranean Sea. A key finding is that the input of iron from dust primarily occurred in the deep ocean, while previous studies mainly focused on the ocean surface. This new insight will enable us to better represent controls on global marine productivity in models.
Julien Totems, Patrick Chazette, and Alexandre Baron
Atmos. Meas. Tech., 14, 7525–7544, https://doi.org/10.5194/amt-14-7525-2021, https://doi.org/10.5194/amt-14-7525-2021, 2021
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We describe in detail the design and calibration of the new Raman channels for the WALI system, going over the important sources of bias and uncertainty on retrieved temperature profiles. For the first time, their impact is investigated using horizontal shots in a homogenous atmosphere: the magnitude of the highlighted biases can be much larger than the targeted absolute accuracy of 1° C. Actual measurement errors are quantified using radiosoundings launched close to the lidar site.
Marco Gaetani, Benjamin Pohl, Maria del Carmen Alvarez Castro, Cyrille Flamant, and Paola Formenti
Atmos. Chem. Phys., 21, 16575–16591, https://doi.org/10.5194/acp-21-16575-2021, https://doi.org/10.5194/acp-21-16575-2021, 2021
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During the dry austral winter, biomass fires in tropical Africa emit large amounts of smoke in the atmosphere, with large impacts on climate and air quality. The study of the relationship between atmospheric circulation and smoke transport shows that midlatitude atmospheric disturbances may deflect the smoke from tropical Africa towards southern Africa. Understanding the distribution of the smoke in the region is crucial for climate modelling and air quality monitoring.
Elvira Pulido-Villena, Karine Desboeufs, Kahina Djaoudi, France Van Wambeke, Stéphanie Barrillon, Andrea Doglioli, Anne Petrenko, Vincent Taillandier, Franck Fu, Tiphanie Gaillard, Sophie Guasco, Sandra Nunige, Sylvain Triquet, and Cécile Guieu
Biogeosciences, 18, 5871–5889, https://doi.org/10.5194/bg-18-5871-2021, https://doi.org/10.5194/bg-18-5871-2021, 2021
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We report on phosphorus dynamics in the surface layer of the Mediterranean Sea. Highly sensitive phosphate measurements revealed vertical gradients above the phosphacline. The relative contribution of diapycnal fluxes to total external supply of phosphate to the mixed layer decreased towards the east, where atmospheric deposition dominated. Taken together, external sources of phosphate contributed little to total supply, which was mainly sustained by enzymatic hydrolysis of organic phosphorus.
France Van Wambeke, Vincent Taillandier, Karine Desboeufs, Elvira Pulido-Villena, Julie Dinasquet, Anja Engel, Emilio Marañón, Céline Ridame, and Cécile Guieu
Biogeosciences, 18, 5699–5717, https://doi.org/10.5194/bg-18-5699-2021, https://doi.org/10.5194/bg-18-5699-2021, 2021
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Simultaneous in situ measurements of (dry and wet) atmospheric deposition and biogeochemical stocks and fluxes in the sunlit waters of the open Mediterranean Sea revealed complex physical and biological processes occurring within the mixed layer. Nitrogen (N) budgets were computed to compare the sources and sinks of N in the mixed layer. The transitory effect observed after a wet dust deposition impacted the microbial food web down to the deep chlorophyll maximum.
Jonas Hamperl, Clément Capitaine, Jean-Baptiste Dherbecourt, Myriam Raybaut, Patrick Chazette, Julien Totems, Bruno Grouiez, Laurence Régalia, Rosa Santagata, Corinne Evesque, Jean-Michel Melkonian, Antoine Godard, Andrew Seidl, Harald Sodemann, and Cyrille Flamant
Atmos. Meas. Tech., 14, 6675–6693, https://doi.org/10.5194/amt-14-6675-2021, https://doi.org/10.5194/amt-14-6675-2021, 2021
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Laser active remote sensing of tropospheric water vapor is a promising technology for enhancing our understanding of processes governing the global hydrological cycle. We investigate the potential of a ground-based lidar to monitor the main water vapor isotopes at high spatio-temporal resolutions in the lower troposphere. Using a realistic end-to-end simulator, we show that high-precision measurements can be achieved within a range of 1.5 km, in mid-latitude or tropical environments.
Cedric G. Ngoungue Langue, Christophe Lavaysse, Mathieu Vrac, Philippe Peyrillé, and Cyrille Flamant
Weather Clim. Dynam., 2, 893–912, https://doi.org/10.5194/wcd-2-893-2021, https://doi.org/10.5194/wcd-2-893-2021, 2021
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This work assesses the forecast of the temperature over the Sahara, a key driver of the West African Monsoon, at a seasonal timescale. The seasonal models are able to reproduce the climatological state and some characteristics of the temperature during the rainy season in the Sahel. But, because of errors in the timing, the forecast skill scores are significant only for the first 4 weeks.
Cited articles
Ackerman, A. S., Toon, O. B., Stevens, D. E., Heymsfield, A. J., Ramanathan,
V., and Welton, E. J.: Reduction of tropical cloudiness by soot, Science,
288, 1042–1047, https://doi.org/10.1126/SCIENCE.288.5468.1042, 2000.
Adebiyi, A. A. and Zuidema, P.: The role of the southern African easterly
jet in modifying the southeast Atlantic aerosol and cloud environments, Q.
J. Roy. Meteorol. Soc., 142, 1574–1589, https://doi.org/10.1002/qj.2765, 2016.
Adebiyi, A. A., Zuidema, P., and Abel, S. J.: The convolution of dynamics and
moisture with the presence of shortwave absorbing aerosols over the
southeast Atlantic, J. Climate, 28, 1997–2024,
https://doi.org/10.1175/JCLI-D-14-00352.1, 2015.
Andreae, M. O., Elbert, W., and de Mora, S. J.: Biogenic sulfur emissions and
aerosols over the tropical South Atlantic: 3. Atmospheric dimethylsulfide,
aerosols and cloud condensation nuclei, J. Geophys. Res., 100, 11335,
https://doi.org/10.1029/94jd02828, 2004.
Ångström, A.: The parameters of atmospheric turbidity, Tellus A, 16,
64–75, https://doi.org/10.3402/tellusa.v16i1.8885, 1964.
Bates, T. S., Quinn, P. K., Coffman, D. J., Johnson, J. E., Miller, T. L.,
Covert, D. S., Wiedensohler, A., Leinert, S., Nowak, A., and Neusüss, C.:
Regional physical and chemical properties of the marine boundary layer
aerosol across the Atlantic during Aerosols99: An overview, J. Geophys. Res.-Atmos., 106, 20767–20782, https://doi.org/10.1029/2000JD900578, 2001.
Bruneau, D., Pelon, J., Blouzon, F., Spatazza, J., Genau, P., Buchholtz, G.,
Amarouche, N., Abchiche, A. and Aouji, O.: 355-nm high spectral resolution
airborne lidar LNG: system description and first results, Appl. Opt.,
54, 8776, https://doi.org/10.1364/AO.54.008776, 2015.
Burton, S. P., Ferrare, R. A., Hostetler, C. A., Hair, J. W., Rogers, R. R., Obland, M. D., Butler, C. F., Cook, A. L., Harper, D. B., and Froyd, K. D.: Aerosol classification using airborne High Spectral Resolution Lidar measurements – methodology and examples, Atmos. Meas. Tech., 5, 73–98, https://doi.org/10.5194/amt-5-73-2012, 2012.
Chazette, P.: The monsoon aerosol extinction properties at Goa during INDOEX
as measured with lidar, J. Geophys. Res., 108, 4187,
https://doi.org/10.1029/2002JD002074, 2003.
Chazette, P. and Totems, J.: Mini N2-Raman Lidar onboard ultra-light
aircraft for aerosol measurements: Demonstration and extrapolation, Remote
Sens., 2016, 9, https://doi.org/10.3390/rs9121226, 2017.
Chazette, P., Bocquet, M., Royer, P., Winiarek, V., Raut, J. C., Labazuy,
P., Gouhier, M., Lardier, M., and Cariou, J. P.: Eyjafjallajökull ash
concentrations derived from both lidar and modeling, J. Geophys. Res.-Atmos., 117, D00U14, https://doi.org/10.1029/2011JD015755, 2012a.
Chazette, P., Dabas, A., Sanak, J., Lardier, M., and Royer, P.: French airborne lidar measurements for Eyjafjallajökull ash plume survey, Atmos. Chem. Phys., 12, 7059–7072, https://doi.org/10.5194/acp-12-7059-2012, 2012b.
Chazette, P., Totems, J., Ancellet, G., Pelon, J., and Sicard, M.: Temporal consistency of lidar observations during aerosol transport events in the framework of the ChArMEx/ADRIMED campaign at Minorca in June 2013, Atmos. Chem. Phys., 16, 2863–2875, https://doi.org/10.5194/acp-16-2863-2016, 2016.
Chew, B. N., Campbell, J. R., Reid, J. S., Giles, D. M., Welton, E. J.,
Salinas, S. V., and Liew, S. C.: Tropical cirrus cloud contamination in sun
photometer data, Atmos. Environ., 45, 6724–6731,
https://doi.org/10.1016/j.atmosenv.2011.08.017, 2011.
Clements, C. B., Potter, B. E., and Zhong, S.: In situ measurements of water
vapor, heat, and CO2 fluxes within a prescribed grass fire, Int. J. Wildl.
Fire, 15, 299–306, https://doi.org/10.1071/WF05101, 2006.
Deaconu, L. T., Ferlay, N., Waquet, F., Peers, F., Thieuleux, F., and Goloub, P.: Satellite inference of water vapour and above-cloud aerosol combined effect on radiative budget and cloud-top processes in the southeastern Atlantic Ocean, Atmos. Chem. Phys., 19, 11613–11634, https://doi.org/10.5194/acp-19-11613-2019, 2019.
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P.,
Kobayashi, S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P.,
Bechtold, P., Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N.,
Delsol, C., Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S.
B., Hersbach, H., Hólm, E. V, Isaksen, L., Kållberg, P., Köhler,
M., Matricardi, M., Mcnally, A. P., Monge-Sanz, B. M., Morcrette, J. J.,
Park, B. K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J. N., and
Vitart, F.: The ERA-Interim reanalysis: Configuration and performance of the
data assimilation system, Q. J. Roy. Meteorol. Soc., 137, 553–597, 2011.
Diamond, M. S., Dobracki, A., Freitag, S., Small Griswold, J. D., Heikkila, A., Howell, S. G., Kacarab, M. E., Podolske, J. R., Saide, P. E., and Wood, R.: Time-dependent entrainment of smoke presents an observational challenge for assessing aerosol–cloud interactions over the southeast Atlantic Ocean, Atmos. Chem. Phys., 18, 14623–14636, https://doi.org/10.5194/acp-18-14623-2018, 2018.
Dieudonné, E., Chazette, P., Marnas, F., Totems, J., and Shang, X.: Raman
Lidar Observations of Aerosol Optical Properties in 11 Cities from France to
Siberia, Remote Sens., 9, 978, https://doi.org/10.3390/rs9100978, 2017.
Draxler, R. R. R. and Rolph, G. D. D.: HYSPLIT (HYbrid Single-Particle
Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website
(http://www.arl.noaa.gov/HYSPLIT.php, last access: 23 November 2019), NOAA Air Resources Laboratory,
College Park, MD., NOAA Air Resour. Lab. available at:
http://ready.arl.noaa.gov/HYSPLIT_ash.php (last access: 23 November 2019), 2014.
Dubovik, O., Smirnov, A., Holben, B. N., King, M. D., Kaufman, Y. J., Eck,
T. F., and Slutsker, I.: Accuracy assessments of aerosol optical properties
retrieved from Aerosol Robotic Network (AERONET) Sun and sky radiance
measurements, J. Geophys. Res.-Atmos., 105, 9791–9806,
https://doi.org/10.1029/2000JD900040, 2000.
Flamant, C., Pelon, J., Chazette, P., Trouillet, V., Quinn, P. K., Frouin, R., Bruneau, D., Leon, J.-F., Bates, T. S., Johnson, J., and Livingston, J.: Airborne lidar measurements of aerosol spatial distribution and optical properties over the Atlantic Ocean during a European pollution outbreak of ACE-2, Tellus B, 52, 662–677, doi:10.1034/j.1600-0889.2000.00083.x, 2000.
Formenti, P., Piketh, S. J., Namwoonde, A., Klopper, D., Burger, R., Cazaunau, M., Feron, A., Gaimoz, C., Broccardo, S., Walton, N., Desboeufs, K., Siour, G., Hanghome, M., Mafwila, S., Omoregie, E., Junkermann, W., and Maenhaut, W.: Three years of measurements of light-absorbing aerosols over coastal Namibia: seasonality, origin, and transport, Atmos. Chem. Phys., 18, 17003–17016, https://doi.org/10.5194/acp-18-17003-2018, 2018.
Formenti, P., D'Anna, B., Flamant, C., Mallet, M. D., Piketh, S. J.,
Schepanski, K., Waquet, F., Auriol, F., Brogniez, G., Burnet, F.,
Chaboureau, J.-P., Chauvigné, A., Chazette, P., Denjean, C., Desboeufs,
K., Doussin, J.-F., Elguindi, N., Feuerstein, S., Gaetani, M., Giorio, C.,
Klopper, D., Mallet, M. D., Nabat, P., Monod, A., Solmon, F., Namwoonde, A.,
Chikwililwa, C., Mushi, R., Welton, E. J., Holben, B., Formenti, P., D'Anna,
B., Flamant, C., Mallet, M. D., Piketh, S. J., Schepanski, K., Waquet, F.,
Auriol, F., Brogniez, G., Burnet, F., Chaboureau, J.-P., Chauvigné, A.,
Chazette, P., Denjean, C., Desboeufs, K., Doussin, J.-F., Elguindi, N.,
Feuerstein, S., Gaetani, M., Giorio, C., Klopper, D., Mallet, M. D., Nabat,
P., Monod, A., Solmon, F., Namwoonde, A., Chikwililwa, C., Mushi, R.,
Welton, E. J. and Holben, B.: The Aerosols, Radiation and Clouds in southern
Africa (AEROCLO-sA) field campaign in Namibia: overview, illustrative
observations and way forward, B. Am. Meteor. Soc., 100, 1277–1298,
https://doi.org/10.1175/BAMS-D-17-0278.1, 2019.
Fuchs, J., Cermak, J., Andersen, H., Hollmann, R., and Schwarz, K.: On the
Influence of Air Mass Origin on Low-Cloud Properties in the Southeast
Atlantic, J. Geophys. Res.-Atmos., 122, 11076–11091,
https://doi.org/10.1002/2017JD027184, 2017.
Ginoux, P., Prospero, J. M., Gill, T. E., Hsu, N. C., and Zhao, M.:
Global-scale attribution of anthropogenic and natural dust sources and their
emission rates based on MODIS Deep Blue aerosol products, Rev. Geophys.,
50, 1–36, https://doi.org/10.1029/2012RG000388, 2012.
Gordon, H., Field, P. R., Abel, S. J., Dalvi, M., Grosvenor, D. P., Hill, A. A., Johnson, B. T., Miltenberger, A. K., Yoshioka, M., and Carslaw, K. S.: Large simulated radiative effects of smoke in the south-east Atlantic, Atmos. Chem. Phys., 18, 15261–15289, https://doi.org/10.5194/acp-18-15261-2018, 2018.
Hamonou, E., Chazette, P., Balis, D., Dulac, F., Schneider, X., Galani, E.,
Ancellet, G., and Papayannis, A.: Characterization of the vertical structure
of Saharan dust export to the Mediterranean basin, J. Geophys. Res.,
104, 22257, https://doi.org/10.1029/1999JD900257, 1999.
Hoffmann, L., Günther, G., Li, D., Stein, O., Wu, X., Griessbach, S., Heng, Y., Konopka, P., Müller, R., Vogel, B., and Wright, J. S.: From ERA-Interim to ERA5: the considerable impact of ECMWF's next-generation reanalysis on Lagrangian transport simulations, Atmos. Chem. Phys., 19, 3097–3124, https://doi.org/10.5194/acp-19-3097-2019, 2019.
Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer,
A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F.,
Jankowiak, I., and Smirnov, A.: AERONET – A Federated Instrument Network and
Data Archive for Aerosol Characterization, Remote Sens. Environ., 66,
1–16, https://doi.org/10.1016/S0034-4257(98)00031-5, 1998.
Holz, A., Paritsis, J., Mundo, I. A., Veblen, T. T., Kitzberger, T.,
Williamson, G. J., Aráoz, E., Bustos-Schindler, C., González, M. E.,
Grau, H. R., and Quezada, J. M.: Southern Annular Mode drives multicentury
wildfire activity in southern South America., P. Natl. Acad. Sci. USA, 114, 9552–9557, https://doi.org/10.1073/pnas.1705168114, 2017.
Ichoku, C., Giglio, L., Wooster, M. J., and Remer, L. A.: Global
characterization of biomass-burning patterns using satellite measurements of
fire radiative energy, Remote Sens. Environ., 112, 2950–2962,
https://doi.org/10.1016/j.rse.2008.02.009, 2008.
Johansson, L., Jalkanen, J. P., and Kukkonen, J.: Global assessment of
shipping emissions in 2015 on a high spatial and temporal resolution, Atmos.
Environ., 167, 403–415, https://doi.org/10.1016/j.atmosenv.2017.08.042, 2017.
Jones, A. and Haywood, J. M.: Sea-spray geoengineering in the HadGEM2-ES earth-system model: radiative impact and climate response, Atmos. Chem. Phys., 12, 10887–10898, https://doi.org/10.5194/acp-12-10887-2012, 2012.
Jones, A., Haywood, J., and Boucher, O.: Climate impacts of geoengineering
marine stratocumulus clouds, J. Geophys. Res.-Atmos., 114, D10106,
https://doi.org/10.1029/2008JD011450, 2009.
Keil, A. and Haywood, J. M.: Solar radiative forcing by biomass burning
aerosol particles during SAFARI 2000: A case study based on measured aerosol
and cloud properties, J. Geophys. Res.-Atmos., 108, 8467–8476,
https://doi.org/10.1029/2002jd002315, 2003.
Kim, M.-H., Omar, A. H., Tackett, J. L., Vaughan, M. A., Winker, D. M., Trepte, C. R., Hu, Y., Liu, Z., Poole, L. R., Pitts, M. C., Kar, J., and Magill, B. E.: The CALIPSO version 4 automated aerosol classification and lidar ratio selection algorithm, Atmos. Meas. Tech., 11, 6107–6135, https://doi.org/10.5194/amt-11-6107-2018, 2018.
Kim, S.-W., Chazette, P., Dulac, F., Sanak, J., Johnson, B., and Yoon, S.-C.: Vertical structure of aerosols and water vapor over West Africa during the African monsoon dry season, Atmos. Chem. Phys., 9, 8017–8038, https://doi.org/10.5194/acp-9-8017-2009, 2009.
King, M. D., Kaufman, Y. J., Menzel, W. P., and Tanré, D.: Remote Sensing
of Cloud, Aerosol, and Water Vapor Properties from the Moderate Resolution
Imaging Spectrometer (MODIS), IEEE T. Geosci. Remote, 30,
2–27, https://doi.org/10.1109/36.124212, 1992.
Léon, J.-F., Chazette, P., Pelon, J., Dulac, F., Randriamiarisoa, H.,
patrick Chazette, Pelon, J., Dulac, F., and Randriamiarisoa, H.: Aerosol
direct radiative impact over the INDOEX area based on passive and active
remote sensing, J. Geophys. Res., 107, 8006, https://doi.org/10.1029/2000JD000116,
2002.
Lim, E.-P., Hendon, H. H., Arblaster, J. M., Delage, F., Nguyen, H., Min,
S.-K., and Wheeler, M. C.: The impact of the Southern Annular Mode on future
changes in Southern Hemisphere rainfall, Geophys. Res. Lett., 43,
7160–7167, https://doi.org/10.1002/2016GL069453, 2016.
McFarquhar, G. M. and Wang, H.: Effects of aerosols on trade wind cumuli
over the Indian Ocean: Model simulations, Q. J. Roy. Meteorol. Soc., 132,
821–843, https://doi.org/10.1256/qj.04.179, 2006.
Müller, D., Ansmann, A., Mattis, I., Tesche, M., Wandinger, U.,
Althausen, D., and Pisani, G.: Aerosol-type-dependent lidar ratios observed
with Raman lidar, J. Geophys. Res., 112, D16202,
https://doi.org/10.1029/2006JD008292, 2007.
Myhre, G., Samset, B. H., Schulz, M., Balkanski, Y., Bauer, S., Berntsen, T. K., Bian, H., Bellouin, N., Chin, M., Diehl, T., Easter, R. C., Feichter, J., Ghan, S. J., Hauglustaine, D., Iversen, T., Kinne, S., Kirkevåg, A., Lamarque, J.-F., Lin, G., Liu, X., Lund, M. T., Luo, G., Ma, X., van Noije, T., Penner, J. E., Rasch, P. J., Ruiz, A., Seland, Ø., Skeie, R. B., Stier, P., Takemura, T., Tsigaridis, K., Wang, P., Wang, Z., Xu, L., Yu, H., Yu, F., Yoon, J.-H., Zhang, K., Zhang, H., and Zhou, C.: Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations, Atmos. Chem. Phys., 13, 1853–1877, https://doi.org/10.5194/acp-13-1853-2013, 2013.
Nicolet, M.: On the molecular scattering in the terrestrial atmosphere?: An
empirical formula for its calculation in the homosphere, Planet. Space Sci.,
32, 1467–1468, https://doi.org/10.1016/0032-0633(84)90089-8, 1984.
Oreopoulos, L. and Platnick, S.: Radiative susceptibility of cloudy
atmospheres to droplet number perturbations: 2. Global analysis from MODIS,
J. Geophys. Res., 113, D14S21, https://doi.org/10.1029/2007JD009655, 2008.
Parmar, R. S., Welling, M., Andreae, M. O., and Helas, G.: Water vapor release from biomass combustion, Atmos. Chem. Phys., 8, 6147–6153, https://doi.org/10.5194/acp-8-6147-2008, 2008.
Ramanathan, V., Li, F., Ramana, M. V, Praveen, P. S., Kim, D., Corrigan, C.
E., Nguyen, H., Stone, E. A., Schauer, J. J., Carmichael, G. R., Adhikary,
B., and Yoon, S. C.: Atmospheric brown clouds: Hemispherical and regional
variations in long-range transport, absorption, and radiative forcing, J.
Geophys. Res, 112, 22–21, https://doi.org/10.1029/2006JD008124, 2007.
Raut, J.-C. and Chazette, P.: Radiative budget in the presence of multi-layered aerosol structures in the framework of AMMA SOP-0, Atmos. Chem. Phys., 8, 6839–6864, https://doi.org/10.5194/acp-8-6839-2008, 2008.
Raut, J.-C. and Chazette, P.: Assessment of vertically-resolved PM10 from mobile lidar observations, Atmos. Chem. Phys., 9, 8617–8638, https://doi.org/10.5194/acp-9-8617-2009, 2009.
Remer, L. A., Kaufman, Y. J., Tanré, D., Mattoo, S., Chu, D. A.,
Martins, J. V., Li, R.-R., Ichoku, C., Levy, R. C., Kleidman, R. G., Eck, T.
F., Vermote, E., and Holben, B. N.: The MODIS Aerosol Algorithm, Products,
and Validation, J. Atmos. Sci., 62, 947–973, https://doi.org/10.1175/JAS3385.1,
2005.
Royer, P., Raut, J.-C., Ajello, G., Berthier, S., and Chazette, P.: Synergy between CALIOP and MODIS instruments for aerosol monitoring: application to the Po Valley, Atmos. Meas. Tech., 3, 893–907, https://doi.org/10.5194/amt-3-893-2010, 2010.
Royer, P., Chazette, P., Lardier, M. and Sauvage, L.: Aerosol content survey
by mini
Royer, P., Chazette, P., Lardier, M. and Sauvage, L.: Aerosol content survey
by mini N2-Raman lidar: Application to local and long-range transport
aerosols, Atmos. Environ., 45, 7487–7495,
https://doi.org/10.1016/j.atmosenv.2010.11.001, 2011b.
Salmonson, V. V., Barnes, W. L., Maymon, P. W., Montgomery,
H. E., and Ostrow, H.: MODIS: Advanced Facility Instrument for Studies
of the Earth as a System, IEEE T. Geosci. Remote, 27, 145–153,
https://doi.org/10.1109/36.20292, 1989.
Stein, A. F., Draxler, R. R., Rolph, G. D., Stunder, B. J. B., Cohen, M. D.,
Ngan, F., Stein, A. F., Draxler, R. R., Rolph, G. D., Stunder, B. J. B.,
Cohen, M. D., and Ngan, F.: NOAA's HYSPLIT Atmospheric Transport and
Dispersion Modeling System, B. Am. Meteor. Soc., 96, 2059–2077,
https://doi.org/10.1175/BAMS-D-14-00110.1, 2015.
Stier, P., Schutgens, N. A. J., Bellouin, N., Bian, H., Boucher, O., Chin, M., Ghan, S., Huneeus, N., Kinne, S., Lin, G., Ma, X., Myhre, G., Penner, J. E., Randles, C. A., Samset, B., Schulz, M., Takemura, T., Yu, F., Yu, H., and Zhou, C.: Host model uncertainties in aerosol radiative forcing estimates: results from the AeroCom Prescribed intercomparison study, Atmos. Chem. Phys., 13, 3245–3270, https://doi.org/10.5194/acp-13-3245-2013, 2013.
Stohl, A.: Computation, accuracy and applications of trajectories – A review
and bibliography, Atmos. Environ., 32, 947–966,
https://doi.org/10.1016/S1352-2310(97)00457-3, 1998.
Swap, R. J., Annegarn, H. J., Suttles, J. T., King, M. D., Platnick, S.,
Privette, J. L., and Scholes, R. J.: Africa burning: A thematic analysis of
the Southern African Regional Science Initiative (SAFARI 2000), J. Geophys.
Res.-Atmos., 108, 8465–8479, https://doi.org/10.1029/2003JD003747, 2003.
Trenberth, K. E.: Interannual Variability of the 500 mb Zonal Mean Flow in
the Southern Hemisphere, Mon. Weather Rev., 107, 1515–1524,
https://doi.org/10.1175/1520-0493(1979)107<1515:ivotmz>2.0.co;2,
2002.
Tyson, P. D. and Preston-White, R. A.: The weather and climate of southern
Africa, Oxford University Press, available at:
https://global.oup.com/academic/product/the-weather-and-climate-of-southern-africa-9780195718065?lang=en&cc=in
(last access: 29 April 2019), 2000.
Vickery, K. J., Eckardt, F. D., and Bryant, R. G.: A sub-basin scale dust
plume source frequency inventory for southern Africa, 2005–2008, Geophys.
Res. Lett., 40, 5274–5279, https://doi.org/10.1002/grl.50968, 2013.
Winker, D. M., Hunt, W. H., and McGill, M. J.: Initial performance assessment
of CALIOP, Geophys. Res. Lett., 34, L19803, https://doi.org/10.1029/2007GL030135,
2007.
Yorks, J. E., McGill, M. J., Palm, S. P., Hlavka, D. L., Selmer, P. A.,
Nowottnick, E. P., Vaughan, M. A., Rodier, S. D., and Hart, W. D.: An
overview of the CATS level 1 processing algorithms and data products,
Geophys. Res. Lett., 43, 4632–4639, https://doi.org/10.1002/2016GL068006, 2016.
Zuidema, P., Redemann, J., Haywood, J., Wood, R., Piketh, S., Hipondoka, M.,
and Formenti, P.: Smoke and clouds above the southeast Atlantic: Upcoming
field campaigns probe absorbing aerosol's impact on climate, B. Am.
Meteor. Soc., 97, 1131–1135, https://doi.org/10.1175/BAMS-D-15-00082.1, 2016.
Zuidema, P., Sedlacek, A. J., Flynn, C., Springston, S., Delgadillo, R.,
Zhang, J., Aiken, A. C., Koontz, A., and Muradyan, P.: The Ascension Island
Boundary Layer in the Remote Southeast Atlantic is Often Smoky, Geophys.
Res. Lett., 45, 4456–4465, https://doi.org/10.1002/2017GL076926, 2018.
Short summary
Evolution of the vertical distribution and optical properties of aerosols in the free troposphere is analysed for the first time over the Namibian coast, a region where uncertainties on aerosol–cloud coupling in climate simulations are significant. The high variability of atmospheric aerosol composition is highlighted using a combination of ground-based, airborne and space-borne lidar. Aerosols are mainly transported from Angola, but part of the highest aerosol layer may come from South America.
Evolution of the vertical distribution and optical properties of aerosols in the free...
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