Articles | Volume 19, issue 2
https://doi.org/10.5194/acp-19-1343-2019
https://doi.org/10.5194/acp-19-1343-2019
Research article
 | 
01 Feb 2019
Research article |  | 01 Feb 2019

Nitrogen-containing secondary organic aerosol formation by acrolein reaction with ammonia/ammonium

Zhijian Li, Sergey A. Nizkorodov, Hong Chen, Xiaohui Lu, Xin Yang, and Jianmin Chen

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Cited articles

Aiona, P. K., Lee, H. J., Lin, P., Heller, F., Laskin, A., Laskin, J., and Nizkorodov, S. A.: A Role for 2-Methyl Pyrrole in the Browning of 4-Oxopentanal and Limonene Secondary Organic Aerosol, Environ. Sci. Technol., 51, 11048–11056, https://doi.org/10.1021/acs.est.7b02293, 2017. 
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Bauer, R., du Toit, M., and Kossmann, J.: Influence of environmental parameters on production of the acrolein precursor 3-hydroxypropionaldehyde by Lactobacillus reuteri DSMZ 20016 and its accumulation by wine lactobacilli, Int. J. Food Microbiol., 137, 28–31, https://doi.org/10.1016/j.ijfoodmicro.2009.10.012, 2010. 
Bauer, R., Hiten, F., Crouch, A. M., Kossmann, J., and Burger, B. V.: Acrolein Dimer as a Marker for Direct Detection of Acrolein in Wine, South African J. Enol. Viticul., 33, 72–79, 2012. 
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Short summary
In this work, we found that acrolein, the smallest α,β-unsaturated aldehyde, has the potential to form light-absorbing heterocyclic secondary organic aerosol. In the gaseous phase, acrolein can react with gaseous ammonia, forming 3-picoline. In the liquid phase, the dissolved acrolein can react with ammonium to form higher molecular-weight pyridinium compounds. All the pyridinium compounds can increase the light absorptivity of aerosol particles.
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