Articles | Volume 18, issue 13
Atmos. Chem. Phys., 18, 9823–9830, 2018
https://doi.org/10.5194/acp-18-9823-2018
Atmos. Chem. Phys., 18, 9823–9830, 2018
https://doi.org/10.5194/acp-18-9823-2018

Technical note 12 Jul 2018

Technical note | 12 Jul 2018

Technical note: Updated parameterization of the reactive uptake of glyoxal and methylglyoxal by atmospheric aerosols and cloud droplets

Leah A. Curry et al.

Related authors

Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds
Andreas Tilgner, Thomas Schaefer, Becky Alexander, Mary Barth, Jeffrey L. Collett Jr., Kathleen M. Fahey, Athanasios Nenes, Havala O. T. Pye, Hartmut Herrmann, and V. Faye McNeill
Atmos. Chem. Phys., 21, 13483–13536, https://doi.org/10.5194/acp-21-13483-2021,https://doi.org/10.5194/acp-21-13483-2021, 2021
Short summary
Opinion: The germicidal effect of ambient air (open-air factor) revisited
R. Anthony Cox, Markus Ammann, John N. Crowley, Paul T. Griffiths, Hartmut Herrmann, Erik H. Hoffmann, Michael E. Jenkin, V. Faye McNeill, Abdelwahid Mellouki, Christopher J. Penkett, Andreas Tilgner, and Timothy J. Wallington
Atmos. Chem. Phys., 21, 13011–13018, https://doi.org/10.5194/acp-21-13011-2021,https://doi.org/10.5194/acp-21-13011-2021, 2021
Short summary
Evaluated kinetic and photochemical data for atmospheric chemistry: volume VIII – gas-phase reactions of organic species with four, or more, carbon atoms ( ≥  C4)
Abdelwahid Mellouki, Markus Ammann, R. Anthony Cox, John N. Crowley, Hartmut Herrmann, Michael E. Jenkin, V. Faye McNeill, Jürgen Troe, and Timothy J. Wallington
Atmos. Chem. Phys., 21, 4797–4808, https://doi.org/10.5194/acp-21-4797-2021,https://doi.org/10.5194/acp-21-4797-2021, 2021
Short summary
Evaluated kinetic and photochemical data for atmospheric chemistry: Volume VII – Criegee intermediates
R. Anthony Cox, Markus Ammann, John N. Crowley, Hartmut Herrmann, Michael E. Jenkin, V. Faye McNeill, Abdelwahid Mellouki, Jürgen Troe, and Timothy J. Wallington
Atmos. Chem. Phys., 20, 13497–13519, https://doi.org/10.5194/acp-20-13497-2020,https://doi.org/10.5194/acp-20-13497-2020, 2020
Short summary
Concept for an electrostatic focusing device for continuous ambient pressure aerosol concentration
Joseph L. Woo, Neha Sareen, Allison N. Schwier, and V. Faye McNeill
Atmos. Meas. Tech., 12, 3395–3402, https://doi.org/10.5194/amt-12-3395-2019,https://doi.org/10.5194/amt-12-3395-2019, 2019
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Predicting gas–particle partitioning coefficients of atmospheric molecules with machine learning
Emma Lumiaro, Milica Todorović, Theo Kurten, Hanna Vehkamäki, and Patrick Rinke
Atmos. Chem. Phys., 21, 13227–13246, https://doi.org/10.5194/acp-21-13227-2021,https://doi.org/10.5194/acp-21-13227-2021, 2021
Short summary
Development of a new emission reallocation method for industrial sources in China
Yun Fat Lam, Chi Chiu Cheung, Xuguo Zhang, Joshua S. Fu, and Jimmy Chi Hung Fung
Atmos. Chem. Phys., 21, 12895–12908, https://doi.org/10.5194/acp-21-12895-2021,https://doi.org/10.5194/acp-21-12895-2021, 2021
Short summary
Projections of shipping emissions and the related impact on air pollution and human health in the Nordic region
Camilla Geels, Morten Winther, Camilla Andersson, Jukka-Pekka Jalkanen, Jørgen Brandt, Lise M. Frohn, Ulas Im, Wing Leung, and Jesper H. Christensen
Atmos. Chem. Phys., 21, 12495–12519, https://doi.org/10.5194/acp-21-12495-2021,https://doi.org/10.5194/acp-21-12495-2021, 2021
Short summary
A predictive model for salt nanoparticle formation using heterodimer stability calculations
Sabrina Chee, Kelley Barsanti, James N. Smith, and Nanna Myllys
Atmos. Chem. Phys., 21, 11637–11654, https://doi.org/10.5194/acp-21-11637-2021,https://doi.org/10.5194/acp-21-11637-2021, 2021
Short summary
Using GECKO-A to derive mechanistic understanding of secondary organic aerosol formation from the ubiquitous but understudied camphene
Isaac Kwadjo Afreh, Bernard Aumont, Marie Camredon, and Kelley Claire Barsanti
Atmos. Chem. Phys., 21, 11467–11487, https://doi.org/10.5194/acp-21-11467-2021,https://doi.org/10.5194/acp-21-11467-2021, 2021
Short summary

Cited articles

Aster, R. C., Thurber, C. H., and Borchers, B.: Parameter estimation and inverse problems, Elsevier Academic Press, 15–26, 2005.
Betterton, E. A. and Hoffmann, M. R.: Henry's Law Constants of Some Environmentally Important Aldehydes, Environ. Sci. Technol., 22, 1415–1418, 1988.
Bird, R. B., Stewart, W. E., and Lightfoot, E. N.: Transport Phenomena, Revised 2nd Edition, John Wiley & Sons, Inc., 528–530, 2006.
Carlton, A. G., Turpin, B. J., Altieri, K. E., Seitzinger, S., Reff, A., Lim, H.-J., and Ervens, B.: Atmospheric oxalic acid and SOA production from glyoxal: Results of aqueous photooxidation experiments, Atmos. Environ., 41, 7588–7602, https://doi.org/10.1016/j.atmosenv.2007.05.035, 2007.
Carlton, A. G., Turpin, B. J., Altieri, K. E., Seitzinger, S. P., Mathur, R., Roselle, S. J. and Weber, R. J.: CMAQ Model Performance Enhanced When In-Cloud Secondary Organic Aerosol is Included: Comparisons of Organic Carbon Predictions with Measurements, Environ. Sci. Technol., 42, 8798–8802, https://doi.org/10.1021/es801192n, 2008.
Download
Short summary
We have developed a new parameterization of the reactive uptake of glyoxal and methylglyoxal by atmospheric aerosols and cloud droplets. Our calculations take into account newly available information regarding the gas–particle partitioning of these species and their chemical processing in the aerosol phase. We expect application of these parameterizations will result in improved representation of aqueous secondary organic aerosol formation in atmospheric chemistry models.
Altmetrics
Final-revised paper
Preprint