Articles | Volume 18, issue 13
https://doi.org/10.5194/acp-18-9823-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-9823-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Technical note: Updated parameterization of the reactive uptake of glyoxal and methylglyoxal by atmospheric aerosols and cloud droplets
Leah A. Curry
Department of Chemical Engineering, Columbia University, New York, NY 10027, USA
William G. Tsui
Department of Chemical Engineering, Columbia University, New York, NY 10027, USA
Department of Chemical Engineering, Columbia University, New York, NY 10027, USA
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Cited
26 citations as recorded by crossref.
- Advanced modeling of gas chemistry and aerosol dynamics with SSH-aerosol v2.0 K. Sartelet et al.
- On the sources and sinks of atmospheric VOCs: an integrated analysis of recent aircraft campaigns over North America X. Chen et al.
- Field observational constraints on the controllers in glyoxal (CHOCHO) reactive uptake to aerosol D. Kim et al.
- Modeling the molecular composition of secondary organic aerosol under highly polluted conditions: A case study in the Yangtze River Delta Region in China Q. Huang et al.
- Revisiting the global budget of atmospheric glyoxal: updates on terrestrial and marine precursor emissions, chemistry, and impacts on atmospheric oxidation capacity A. Zhang et al.
- Positive Feedback between Partitioning of Carbonyl Compounds and Particulate Sulfur Formation during Haze Episodes H. Shen et al.
- Regional modeling of secondary organic aerosol formation over eastern China: The impact of uptake coefficients of dicarbonyls and semivolatile process of primary organic aerosol X. Chen et al.
- Electrospray surface-enhanced Raman spectroscopy (ES-SERS) for studying organic coatings of atmospheric aerosol particles M. Gen et al.
- Assessment of dicarbonyl contributions to secondary organic aerosols over China using RAMS-CMAQ J. Li et al.
- Heterogeneous formation and light absorption of secondary organic aerosols from acetone photochemical reactions: remarkably enhancing effects of seeds and ammonia S. Zhang et al.
- Development of SOA modules in the WRF-Chem model and evaluation of the key formation pathways of SOA and associated health risk over mainland China L. Wu et al.
- Synergistic Uptake by Acidic Sulfate Particles of Gaseous Mixtures of Glyoxal and Pinanediol Y. Qin et al.
- Kinetics and Mechanisms of Reactive Uptake of Methylglyoxal on Deliquesced Ammonium Salts: Acid Catalysis and Sulfate Inhibition H. Liu et al.
- Formation and composition of organic aerosols from the uptake of glyoxal on natural mineral dust aerosols: a laboratory study F. Battaglia et al.
- The application and uncertainty of the observation-based model in ozone and secondary aerosols simulation: A review J. Wei et al.
- Hygroscopicity of isoprene-derived secondary organic aerosol mixture proxies: importance of diffusion and salting-in effects N. Ferdousi-Rokib et al.
- Multi-Oxygenated Organic Compounds in Fine Particulate Matter Collected in the Western Mediterranean Area E. Borrás et al.
- Carbonyl compounds in the atmosphere: A review of abundance, source and their contributions to O3 and SOA formation Q. Liu et al.
- Comparison of Gas–Particle Partitioning of Glyoxal and Methylglyoxal in the Summertime Atmosphere at the Foot and Top of Mount Hua W. Qi et al.
- Global VOC emissions quantified from inversion of TROPOMI spaceborne formaldehyde and glyoxal data Y. Sfendla et al.
- Glyoxal as a Potential Source of Highly Viscous Aerosol Particles J. Peters et al.
- Molecular Characterization and Source Identification of Atmospheric Particulate Organosulfates Using Ultrahigh Resolution Mass Spectrometry K. Wang et al.
- Single-particle experiments measuring humidity and inorganic salt effects on gas-particle partitioning of butenedial A. Birdsall et al.
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al.
- Observations of glyoxal and methylglyoxal in a suburban area of the Yangtze River Delta, China J. Liu et al.
- Reversible and irreversible gas–particle partitioning of dicarbonyl compounds observed in the real atmosphere J. Hu et al.
26 citations as recorded by crossref.
- Advanced modeling of gas chemistry and aerosol dynamics with SSH-aerosol v2.0 K. Sartelet et al.
- On the sources and sinks of atmospheric VOCs: an integrated analysis of recent aircraft campaigns over North America X. Chen et al.
- Field observational constraints on the controllers in glyoxal (CHOCHO) reactive uptake to aerosol D. Kim et al.
- Modeling the molecular composition of secondary organic aerosol under highly polluted conditions: A case study in the Yangtze River Delta Region in China Q. Huang et al.
- Revisiting the global budget of atmospheric glyoxal: updates on terrestrial and marine precursor emissions, chemistry, and impacts on atmospheric oxidation capacity A. Zhang et al.
- Positive Feedback between Partitioning of Carbonyl Compounds and Particulate Sulfur Formation during Haze Episodes H. Shen et al.
- Regional modeling of secondary organic aerosol formation over eastern China: The impact of uptake coefficients of dicarbonyls and semivolatile process of primary organic aerosol X. Chen et al.
- Electrospray surface-enhanced Raman spectroscopy (ES-SERS) for studying organic coatings of atmospheric aerosol particles M. Gen et al.
- Assessment of dicarbonyl contributions to secondary organic aerosols over China using RAMS-CMAQ J. Li et al.
- Heterogeneous formation and light absorption of secondary organic aerosols from acetone photochemical reactions: remarkably enhancing effects of seeds and ammonia S. Zhang et al.
- Development of SOA modules in the WRF-Chem model and evaluation of the key formation pathways of SOA and associated health risk over mainland China L. Wu et al.
- Synergistic Uptake by Acidic Sulfate Particles of Gaseous Mixtures of Glyoxal and Pinanediol Y. Qin et al.
- Kinetics and Mechanisms of Reactive Uptake of Methylglyoxal on Deliquesced Ammonium Salts: Acid Catalysis and Sulfate Inhibition H. Liu et al.
- Formation and composition of organic aerosols from the uptake of glyoxal on natural mineral dust aerosols: a laboratory study F. Battaglia et al.
- The application and uncertainty of the observation-based model in ozone and secondary aerosols simulation: A review J. Wei et al.
- Hygroscopicity of isoprene-derived secondary organic aerosol mixture proxies: importance of diffusion and salting-in effects N. Ferdousi-Rokib et al.
- Multi-Oxygenated Organic Compounds in Fine Particulate Matter Collected in the Western Mediterranean Area E. Borrás et al.
- Carbonyl compounds in the atmosphere: A review of abundance, source and their contributions to O3 and SOA formation Q. Liu et al.
- Comparison of Gas–Particle Partitioning of Glyoxal and Methylglyoxal in the Summertime Atmosphere at the Foot and Top of Mount Hua W. Qi et al.
- Global VOC emissions quantified from inversion of TROPOMI spaceborne formaldehyde and glyoxal data Y. Sfendla et al.
- Glyoxal as a Potential Source of Highly Viscous Aerosol Particles J. Peters et al.
- Molecular Characterization and Source Identification of Atmospheric Particulate Organosulfates Using Ultrahigh Resolution Mass Spectrometry K. Wang et al.
- Single-particle experiments measuring humidity and inorganic salt effects on gas-particle partitioning of butenedial A. Birdsall et al.
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al.
- Observations of glyoxal and methylglyoxal in a suburban area of the Yangtze River Delta, China J. Liu et al.
- Reversible and irreversible gas–particle partitioning of dicarbonyl compounds observed in the real atmosphere J. Hu et al.
Saved (final revised paper)
Latest update: 18 May 2026
Short summary
We have developed a new parameterization of the reactive uptake of glyoxal and methylglyoxal by atmospheric aerosols and cloud droplets. Our calculations take into account newly available information regarding the gas–particle partitioning of these species and their chemical processing in the aerosol phase. We expect application of these parameterizations will result in improved representation of aqueous secondary organic aerosol formation in atmospheric chemistry models.
We have developed a new parameterization of the reactive uptake of glyoxal and methylglyoxal by...
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