Articles | Volume 17, issue 10
https://doi.org/10.5194/acp-17-6271-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-6271-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
22 May 2017
Research article |
| 22 May 2017
Depolarization ratios retrieved by AERONET sun–sky radiometer data and comparison to depolarization ratios measured with lidar
Youngmin Noh
International Environmental Research Center, Gwangju Institute of Science and Technology (GIST), Gwangju, South Korea
School of Physics, Astronomy and Mathematics, University of Hertfordshire, Hertfordshire, UK
Kyunghwa Lee
Gwangju Institute of Science and Technology (GIST), Gwangju, South Korea
Kwanchul Kim
Gwangju Institute of Science and Technology (GIST), Gwangju, South Korea
Kwonho Lee
Department of Atmospheric and Environmental Sciences, Gangneung-Wonju National University, Gangneung, South Korea
Atsushi Shimizu
National Institute for Environmental Studies, Tsukuba, Japan
Itaru Sano
Graduate School of Science and Engineering, Kindai University, Osaka, Japan
Chan Bong Park
Department of Electronic Engineering, Mokwon University, Daejeon, South Korea
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Juseon Shin, Gahyeong Kim, Dukhyeon Kim, Matthias Tesche, Gahyeon Park, and Youngmin Noh
Atmos. Meas. Tech., 17, 397–406, https://doi.org/10.5194/amt-17-397-2024, https://doi.org/10.5194/amt-17-397-2024, 2024
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We introduce the multi-section method, a novel approach for stable extinction coefficient retrievals in horizontally scanning aerosol lidar measurements, in this study. Our method effectively removes signal–noise-induced irregular peaks and derives a reference extinction coefficient, αref, from multiple scans, resulting in a strong correlation (>0.74) with PM2.5 mass concentrations. Case studies demonstrate its utility in retrieving spatio-temporal aerosol distributions and PM2.5 concentrations.
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We analyzed long-term AERONET sun/sky radiometer for 6 continentals to verify the trend of aerosol physical properties depending on sources (dust or pollution) and size (fine or coarse mode). We identified the trend of classified aerosol optical depth (AOD) and size change over 9 years. Especially, we find out aerosol properties causing AOD variations are different from regions and fine aerosol particle in most regions has become smaller using MK-test for trend analysis.
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This study proposes an aerosol-type classification based on parameters from the AErosol RObotic NETwork (AERONET) version 3 level 2.0 inversion product that describe light depolarization and absorption properties of atmospheric particles.
We compare our classification with an earlier method and find that the new approach allows for a refined classification of mineral dust that occurs as a mixture with other absorbing aerosols.
S.-K. Shin, D. Müller, C. Lee, K. H. Lee, D. Shin, Y. J. Kim, and Y. M. Noh
Atmos. Chem. Phys., 15, 6707–6720, https://doi.org/10.5194/acp-15-6707-2015, https://doi.org/10.5194/acp-15-6707-2015, 2015
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The measurements from 2009 to 2013 using a multiwavelength Raman lidar were conducted to identify the changes in optical properties of East Asian dust. We found that the optical properties of Asian dust change depending on the dust plume's vertical position and the change of vertical position during transport over China. We believe this paper provides a better understanding of the optical properties of mixed Asian dust plums and the effect of long-range transport on dust properties.
D. Shin, D. Müller, K. Lee, S. Shin, Y. J. Kim, C. K. Song, and Y. M. Noh
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-1171-2015, https://doi.org/10.5194/acpd-15-1171-2015, 2015
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We present for the first time results of Raman lidar observations of the temporal evolution of a stratospheric aerosol layer observed in the upper troposphere and lower stratosphere over Korea. We find what non-spherical particles may have been present in the lower stratosphere for at least six months after the eruption on the volcano. Our study adds to the limited information on volcanic aerosols over East Asia.
Y. M. Noh, H. Lee, D. Mueller, K. Lee, D. Shin, S. Shin, T. J. Choi, Y. J. Choi, and K. R. Kim
Atmos. Chem. Phys., 13, 7619–7629, https://doi.org/10.5194/acp-13-7619-2013, https://doi.org/10.5194/acp-13-7619-2013, 2013
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We introduce the multi-section method, a novel approach for stable extinction coefficient retrievals in horizontally scanning aerosol lidar measurements, in this study. Our method effectively removes signal–noise-induced irregular peaks and derives a reference extinction coefficient, αref, from multiple scans, resulting in a strong correlation (>0.74) with PM2.5 mass concentrations. Case studies demonstrate its utility in retrieving spatio-temporal aerosol distributions and PM2.5 concentrations.
Takuma Miyakawa, Akinori Ito, Chunmao Zhu, Atsushi Shimizu, Erika Matsumoto, Yusuke Mizuno, and Yugo Kanaya
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This study conducted semi-continuous measurements of PM2.5 aerosols and their elemental composition in western Japan, during spring 2018. It analyzed the emissions, transport, and wet removal of elements such as Pb, Cu, Fe, and Mn. It also assessed the accuracy of modeled concentrations and found overestimations of BC and underestimations of Cu and anthropogenic Fe in East Asia. Insights into emissions, removals, and source apportionment of trace metals in the East Asian outflow were provided.
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The evolution of aerosol in biomass burning smoke plumes that travel over marine clouds off the Atlantic coast of central Africa was studied using measurements made by a lidar deployed on a high-altitude aircraft. The main finding was that the physical properties of aerosol do not change appreciably once the plume has left land and travels over the ocean over a timescale of 1 to 2 d. Almost all particles in the plume are of radius less than 1 micrometer and spherical in shape.
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Today, few lidar are capable of triple-wavelength particle linear depolarization ratio (PLDR) measurements. This study is the first systematic investigation of the effect of different choices of PLDR input on the inversion of lidar measurements of mineral dust and dusty mixtures using light scattering by randomly oriented spheroids. We provide recommendations of the most suitable input parameters for use with the applied methodology, based on a relational assessment of the inversion output.
Sung-Kyun Shin, Matthias Tesche, Youngmin Noh, and Detlef Müller
Atmos. Meas. Tech., 12, 3789–3803, https://doi.org/10.5194/amt-12-3789-2019, https://doi.org/10.5194/amt-12-3789-2019, 2019
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This study proposes an aerosol-type classification based on parameters from the AErosol RObotic NETwork (AERONET) version 3 level 2.0 inversion product that describe light depolarization and absorption properties of atmospheric particles.
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Sung-Kyun Shin, Matthias Tesche, Detlef Müller, and Youngmin Noh
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Xiaole Pan, Baozhu Ge, Zhe Wang, Yu Tian, Hang Liu, Lianfang Wei, Siyao Yue, Itsushi Uno, Hiroshi Kobayashi, Tomoaki Nishizawa, Atsushi Shimizu, Pingqing Fu, and Zifa Wang
Atmos. Chem. Phys., 19, 219–232, https://doi.org/10.5194/acp-19-219-2019, https://doi.org/10.5194/acp-19-219-2019, 2019
Yu Tian, Xiaole Pan, Tomoaki Nishizawa, Hiroshi Kobayashi, Itsushi Uno, Xiquan Wang, Atsushi Shimizu, and Zifa Wang
Atmos. Chem. Phys., 18, 18203–18217, https://doi.org/10.5194/acp-18-18203-2018, https://doi.org/10.5194/acp-18-18203-2018, 2018
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East Asia is characterized by severe anthropogenic pollution and dust storms due to fuel consumption and the downwind location of dust sources. We studied the mixing states of dust and pollutants using an optical particle counter equipped with a polarization detection module, providing a deeper understanding of possible mechanisms of aerosols’ morphological change. In Beijing, the heterogeneous processes in the mixture of dust and emitted pollutants have a great influence on smog formation.
Sung-Kyun Shin, Matthias Tesche, Kwanchul Kim, Maria Kezoudi, Boyan Tatarov, Detlef Müller, and Youngmin Noh
Atmos. Chem. Phys., 18, 12735–12746, https://doi.org/10.5194/acp-18-12735-2018, https://doi.org/10.5194/acp-18-12735-2018, 2018
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We investigate lidar-specific parameters inferred from AERONET sun photometer measurements representative of mineral dust from different source regions. We compare our findings to the literature values on the lidar ratio and the particle linear depolarisation ratio. We find changing values for different source regions, which is in agreement with other observations. For longer wavelengths we find values that are in line with lidar observations.
Kai Tang, Zhongwei Huang, Jianping Huang, Teruya Maki, Shuang Zhang, Atsushi Shimizu, Xiaojun Ma, Jinsen Shi, Jianrong Bi, Tian Zhou, Guoyin Wang, and Lei Zhang
Atmos. Chem. Phys., 18, 7131–7148, https://doi.org/10.5194/acp-18-7131-2018, https://doi.org/10.5194/acp-18-7131-2018, 2018
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To our knowledge, this is the first simultaneous field measurement of bioaerosols in dust events at four sites along the transport pathway of Asian dust. The samples were analyzed by means of fluorescence microscopy, scanning electron microscopy, and MiSeq sequencing analysis. The results indicate that dust clouds can carry many bacteria of various types into downwind regions, the alpha and beta diversity of which were investigated.
Brent N. Holben, Jhoon Kim, Itaru Sano, Sonoyo Mukai, Thomas F. Eck, David M. Giles, Joel S. Schafer, Aliaksandr Sinyuk, Ilya Slutsker, Alexander Smirnov, Mikhail Sorokin, Bruce E. Anderson, Huizheng Che, Myungje Choi, James H. Crawford, Richard A. Ferrare, Michael J. Garay, Ukkyo Jeong, Mijin Kim, Woogyung Kim, Nichola Knox, Zhengqiang Li, Hwee S. Lim, Yang Liu, Hal Maring, Makiko Nakata, Kenneth E. Pickering, Stuart Piketh, Jens Redemann, Jeffrey S. Reid, Santo Salinas, Sora Seo, Fuyi Tan, Sachchida N. Tripathi, Owen B. Toon, and Qingyang Xiao
Atmos. Chem. Phys., 18, 655–671, https://doi.org/10.5194/acp-18-655-2018, https://doi.org/10.5194/acp-18-655-2018, 2018
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Aerosol particles, such as smoke, vary over space and time. This paper describes a series of very high-resolution ground-based aerosol measurement networks and associated studies that contributed new understanding of aerosol processes and detailed comparisons to satellite aerosol validation. Significantly, these networks also provide an opportunity to statistically relate grab samples of an aerosol parameter to companion satellite observations, a step toward air quality assessment from space.
Patricia Sawamura, Richard H. Moore, Sharon P. Burton, Eduard Chemyakin, Detlef Müller, Alexei Kolgotin, Richard A. Ferrare, Chris A. Hostetler, Luke D. Ziemba, Andreas J. Beyersdorf, and Bruce E. Anderson
Atmos. Chem. Phys., 17, 7229–7243, https://doi.org/10.5194/acp-17-7229-2017, https://doi.org/10.5194/acp-17-7229-2017, 2017
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We present a detailed evaluation of physical properties of aerosols, like aerosol number concentration and aerosol size, obtained from an advanced, airborne, multi-wavelength high-spectral-resolution lidar (HSRL-2) system. These lidar-retrieved physical properties were compared to airborne in situ measurements. Our findings highlight the advantages of advanced HSRL measurements and retrievals to help constrain the vertical distribution of aerosol volume or mass loading relevant for air quality.
Masatomo Fujiwara, Takuji Sugidachi, Toru Arai, Kensaku Shimizu, Mayumi Hayashi, Yasuhisa Noma, Hideaki Kawagita, Kazuo Sagara, Taro Nakagawa, Satoshi Okumura, Yoichi Inai, Takashi Shibata, Suginori Iwasaki, and Atsushi Shimizu
Atmos. Meas. Tech., 9, 5911–5931, https://doi.org/10.5194/amt-9-5911-2016, https://doi.org/10.5194/amt-9-5911-2016, 2016
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A meteorological balloon-borne cloud sensor called the cloud particle sensor (CPS) has been developed. The CPS can count the number of particles per second and can obtain the cloud phase information (i.e. liquid, ice, or mixed). Twenty-five test flights have been made between 2012 and 2015 at midlatitude and tropical sites. The results from the four flights are discussed.
Itaru Sano, Sonoyo Mukai, Makiko Nakata, and Brent N. Holben
Atmos. Chem. Phys., 16, 14795–14803, https://doi.org/10.5194/acp-16-14795-2016, https://doi.org/10.5194/acp-16-14795-2016, 2016
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We investigated the regional and local variation of aerosols based on large and small gridded sun photometer networks. The results show that long-range transboundary aerosols strongly affect aerosol condition over Japan even at a small island in the East China Sea. A dense instrument network (DRAGON) reveals the magnitude and variation of local aerosols.
Detlef Müller, Christine Böckmann, Alexei Kolgotin, Lars Schneidenbach, Eduard Chemyakin, Julia Rosemann, Pavel Znak, and Anton Romanov
Atmos. Meas. Tech., 9, 5007–5035, https://doi.org/10.5194/amt-9-5007-2016, https://doi.org/10.5194/amt-9-5007-2016, 2016
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We present a comparison study of two data inversion algorithms that are used to derive microphysical properties of atmospheric particle pollution. The algorithms have been developed for the analysis of data collected with advanced light detection and ranging (lidar) instruments from the European EARLINET network. The result of this study shows that two key parameters needed for climate change studies, i.e. particle size and light absorption capacity, can be derived with reasonable accuracy.
B. Quennehen, J.-C. Raut, K. S. Law, N. Daskalakis, G. Ancellet, C. Clerbaux, S.-W. Kim, M. T. Lund, G. Myhre, D. J. L. Olivié, S. Safieddine, R. B. Skeie, J. L. Thomas, S. Tsyro, A. Bazureau, N. Bellouin, M. Hu, M. Kanakidou, Z. Klimont, K. Kupiainen, S. Myriokefalitakis, J. Quaas, S. T. Rumbold, M. Schulz, R. Cherian, A. Shimizu, J. Wang, S.-C. Yoon, and T. Zhu
Atmos. Chem. Phys., 16, 10765–10792, https://doi.org/10.5194/acp-16-10765-2016, https://doi.org/10.5194/acp-16-10765-2016, 2016
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This paper evaluates the ability of six global models and one regional model in reproducing short-lived pollutants (defined here as ozone and its precursors, aerosols and black carbon) concentrations over Asia using satellite, ground-based and airborne observations.
Key findings are that models homogeneously reproduce the trace gas observations although nitrous oxides are underestimated, whereas the aerosol distributions are heterogeneously reproduced, implicating important uncertainties.
Elina Giannakaki, Pieter G. van Zyl, Detlef Müller, Dimitris Balis, and Mika Komppula
Atmos. Chem. Phys., 16, 8109–8123, https://doi.org/10.5194/acp-16-8109-2016, https://doi.org/10.5194/acp-16-8109-2016, 2016
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Optical and microphysical properties of different aerosol types over South Africa measured with a multi-wavelength polarization Raman lidar are presented. Aerosol characterization of elevated layers was performed. This study could assist in bridging existing gaps relating to aerosol properties over South Africa.
Makiko Nakata, Itaru Sano, Sonoyo Mukai, and Brent N. Holben
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-182, https://doi.org/10.5194/acp-2016-182, 2016
Revised manuscript not accepted
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We document the spatial and temporal variations of atmospheric aerosols in East Asia, specifically focusing on the NASA/AERONET-Osaka site in March 2012 during the AERONET “DRAGON-Japan” campaign. It has been shown that airborne pollutants can influence both the local atmosphere near to their source and relatively remote locations due to long-range transportation.
M. Mustafa Mamun and Detlef Müller
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2016-7, https://doi.org/10.5194/amt-2016-7, 2016
Revised manuscript has not been submitted
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For the first time we present an Artificial Neural Network (ANN) model which can estimate the intensive microphysical parameters of atmospheric pollution from Multiwavelength Raman/HSRL Lidar data. This feasibility study explores the potential of using ANN for future data analysis as an additional tool regarding established methods. We show that particle effective radius, real and imaginary part of complex refractive index can be retrieved from 3β+2α, 3β+1α, 2β+1α, and 3β optical lidar channels.
H. Irie, T. Nakayama, A. Shimizu, A. Yamazaki, T. Nagai, A. Uchiyama, Y. Zaizen, S. Kagamitani, and Y. Matsumi
Atmos. Meas. Tech., 8, 2775–2788, https://doi.org/10.5194/amt-8-2775-2015, https://doi.org/10.5194/amt-8-2775-2015, 2015
S.-K. Shin, D. Müller, C. Lee, K. H. Lee, D. Shin, Y. J. Kim, and Y. M. Noh
Atmos. Chem. Phys., 15, 6707–6720, https://doi.org/10.5194/acp-15-6707-2015, https://doi.org/10.5194/acp-15-6707-2015, 2015
Short summary
Short summary
The measurements from 2009 to 2013 using a multiwavelength Raman lidar were conducted to identify the changes in optical properties of East Asian dust. We found that the optical properties of Asian dust change depending on the dust plume's vertical position and the change of vertical position during transport over China. We believe this paper provides a better understanding of the optical properties of mixed Asian dust plums and the effect of long-range transport on dust properties.
D. Goto, T. Dai, M. Satoh, H. Tomita, J. Uchida, S. Misawa, T. Inoue, H. Tsuruta, K. Ueda, C. F. S. Ng, A. Takami, N. Sugimoto, A. Shimizu, T. Ohara, and T. Nakajima
Geosci. Model Dev., 8, 235–259, https://doi.org/10.5194/gmd-8-235-2015, https://doi.org/10.5194/gmd-8-235-2015, 2015
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An aerosol-coupled global non-hydrostatic model with a stretched-grid system has been developed to simulate aerosols on a region scale of 10 km grids. The regional simulation does require either a nesting technique or lateral boundary conditions, as opposed to general regional models. It generally reproduces monthly mean distributions of the observed sulfate and SO2 over East Asia as well as the diurnal and synoptic variations of the observed ones around the main target region, Tokyo/Japan.
D. Shin, D. Müller, K. Lee, S. Shin, Y. J. Kim, C. K. Song, and Y. M. Noh
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-1171-2015, https://doi.org/10.5194/acpd-15-1171-2015, 2015
Preprint withdrawn
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We present for the first time results of Raman lidar observations of the temporal evolution of a stratospheric aerosol layer observed in the upper troposphere and lower stratosphere over Korea. We find what non-spherical particles may have been present in the lower stratosphere for at least six months after the eruption on the volcano. Our study adds to the limited information on volcanic aerosols over East Asia.
D. Müller, C. A. Hostetler, R. A. Ferrare, S. P. Burton, E. Chemyakin, A. Kolgotin, J. W. Hair, A. L. Cook, D. B. Harper, R. R. Rogers, R. W. Hare, C. S. Cleckner, M. D. Obland, J. Tomlinson, L. K. Berg, and B. Schmid
Atmos. Meas. Tech., 7, 3487–3496, https://doi.org/10.5194/amt-7-3487-2014, https://doi.org/10.5194/amt-7-3487-2014, 2014
P. Sawamura, D. Müller, R. M. Hoff, C. A. Hostetler, R. A. Ferrare, J. W. Hair, R. R. Rogers, B. E. Anderson, L. D. Ziemba, A. J. Beyersdorf, K. L. Thornhill, E. L. Winstead, and B. N. Holben
Atmos. Meas. Tech., 7, 3095–3112, https://doi.org/10.5194/amt-7-3095-2014, https://doi.org/10.5194/amt-7-3095-2014, 2014
K. Osada, S. Ura, M. Kagawa, M. Mikami, T. Y. Tanaka, S. Matoba, K. Aoki, M. Shinoda, Y. Kurosaki, M. Hayashi, A. Shimizu, and M. Uematsu
Atmos. Chem. Phys., 14, 1107–1121, https://doi.org/10.5194/acp-14-1107-2014, https://doi.org/10.5194/acp-14-1107-2014, 2014
Y. M. Noh, H. Lee, D. Mueller, K. Lee, D. Shin, S. Shin, T. J. Choi, Y. J. Choi, and K. R. Kim
Atmos. Chem. Phys., 13, 7619–7629, https://doi.org/10.5194/acp-13-7619-2013, https://doi.org/10.5194/acp-13-7619-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations
Opinion: Aerosol remote sensing over the next 20 years
Monitoring biomass burning aerosol transport using CALIOP observations and reanalysis models: a Canadian wildfire event in 2019
Thermal infrared observations of a western United States biomass burning aerosol plume
A new look into the impacts of dust radiative effects on the energetics of tropical easterly waves
Wind-driven emissions of coarse-mode particles in an urban environment
The Emission, Transport, and Impacts of the Extreme Saharan Dust Storm in 2015
Measurement report: Dust and anthropogenic aerosols' vertical distributions over northern China dense aerosols gathered at the top of the mixing layer
Climatological assessment of the vertically resolved optical and microphysical aerosol properties by lidar measurements, sun photometer, and in situ observations over 17 years at Universitat Politècnica de Catalunya (UPC) Barcelona
Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments
Impact of assimilating NOAA VIIRS aerosol optical depth (AOD) observations on global AOD analysis from the Copernicus Atmosphere Monitoring Service (CAMS)
Spectral dependence of birch and pine pollen optical properties using a synergy of lidar instruments
Validation activities of Aeolus wind products on the southeastern Iberian Peninsula
Thermal infrared dust optical depth and coarse-mode effective diameter over oceans retrieved from collocated MODIS and CALIOP observations
A comprehensive reappraisal of long-term aerosol characteristics, trends, and variability in Asia
Satellite (GOSAT-2 CAI-2) retrieval and surface (ARFINET) observations of aerosol black carbon over India
Spatiotemporal variation characteristics of global fires and their emissions
The (mis)identification of high-latitude dust events using remote sensing methods in the Yukon, Canada: a sub-daily variability analysis
Comparison of dust optical depth from multi-sensor products and MONARCH (Multiscale Online Non-hydrostatic AtmospheRe CHemistry) dust reanalysis over North Africa, the Middle East, and Europe
Understanding day–night differences in dust aerosols over the dust belt of North Africa, the Middle East, and Asia
Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions
Validation of the TROPOMI/S5P aerosol layer height using EARLINET lidars
Vertical characterization of fine and coarse dust particles during an intense Saharan dust outbreak over the Iberian Peninsula in springtime 2021
Aerosol optical depth regime over megacities of the world
South American 2020 regional smoke plume: intercomparison with previous years, impact on solar radiation, and the role of Pantanal biomass burning season
Circular polarization in atmospheric aerosols
Spatiotemporal continuous estimates of daily 1 km PM2.5 from 2000 to present under the Tracking Air Pollution in China (TAP) framework
Robust evidence for reversal of the trend in aerosol effective climate forcing
Simultaneous retrievals of biomass burning aerosols and trace gases from the ultraviolet to near-infrared over northern Thailand during the 2019 pre-monsoon season
A decadal assessment of the climatology of aerosol and cloud properties over South Africa
Aerosol characterisation in the subtropical eastern North Atlantic region using long-term AERONET measurements
Long-range transport of Asian dust to the Arctic: identification of transport pathways, evolution of aerosol optical properties, and impact assessment on surface albedo changes
Canadian and Alaskan wildfire smoke particle properties, their evolution, and controlling factors, from satellite observations
Evaluation of aerosol optical depths and clear-sky radiative fluxes of the CERES Edition 4.1 SYN1deg data product
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 1: Climatology and trend
Vertical structure of biomass burning aerosol transported over the southeast Atlantic Ocean
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 2: Statistics of extreme AOD events, and implications for the impact of regional biomass burning processes
Aerosol atmospheric rivers: climatology, event characteristics, and detection algorithm sensitivities
Dust transport and advection measurement with spaceborne lidars ALADIN and CALIOP and model reanalysis data
Record-breaking dust loading during two mega dust storm events over northern China in March 2021: aerosol optical and radiative properties and meteorological drivers
Wintertime Saharan dust transport towards the Caribbean: an airborne lidar case study during EUREC4A
Evaluation of aerosol number concentrations from CALIPSO with ATom airborne in situ measurements
Zonal variations in the vertical distribution of atmospheric aerosols over the Indian region and the consequent radiative effects
Global maps of aerosol single scattering albedo using combined CERES-MODIS retrieval
James L. Gomez, Robert J. Allen, and King-Fai Li
Atmos. Chem. Phys., 24, 6937–6963, https://doi.org/10.5194/acp-24-6937-2024, https://doi.org/10.5194/acp-24-6937-2024, 2024
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Wildfires in California (CA) have grown very large during the past 20 years. These fires emit sunlight-absorbing aerosols. Analyzing observational data, our study finds that aerosols emitted from large fires in northern CA spread throughout CA and Nevada and heat the atmosphere. This heating is consistent with larger-than-normal temperatures and dry conditions. Further study is needed to determine how much the aerosols heat the atmosphere and whether they are drying the atmosphere as well.
Yuxuan Xing, Yang Chen, Shirui Yan, Xiaoyi Cao, Yong Zhou, Xueying Zhang, Tenglong Shi, Xiaoying Niu, Dongyou Wu, Jiecan Cui, Yue Zhou, Xin Wang, and Wei Pu
Atmos. Chem. Phys., 24, 5199–5219, https://doi.org/10.5194/acp-24-5199-2024, https://doi.org/10.5194/acp-24-5199-2024, 2024
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This study investigated the impact of dust storms from the Taklamakan Desert on surrounding high mountains and regional radiation balance. Using satellite data and simulations, researchers found that dust storms significantly darken the snow surface in the Tien Shan, Kunlun, and Qilian mountains, reaching mountains up to 1000 km away. This darkening occurs not only in spring but also during summer and autumn, leading to increased absorption of solar radiation.
Yuqin Liu, Tao Lin, Jiahua Zhang, Fu Wang, Yiyi Huang, Xian Wu, Hong Ye, Guoqin Zhang, Xin Cao, and Gerrit de Leeuw
Atmos. Chem. Phys., 24, 4651–4673, https://doi.org/10.5194/acp-24-4651-2024, https://doi.org/10.5194/acp-24-4651-2024, 2024
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A new method, the geographical detector method (GDM), has been applied to satellite data, in addition to commonly used statistical methods, to study the sensitivity of cloud properties to aerosol over China. Different constraints for aerosol and cloud liquid water path apply over polluted and clean areas. The GDM shows that cloud parameters are more sensitive to combinations of parameters than to individual parameters, but confounding effects due to co-variation of parameters cannot be excluded.
Kangwen Sun, Guangyao Dai, Songhua Wu, Oliver Reitebuch, Holger Baars, Jiqiao Liu, and Suping Zhang
Atmos. Chem. Phys., 24, 4389–4409, https://doi.org/10.5194/acp-24-4389-2024, https://doi.org/10.5194/acp-24-4389-2024, 2024
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This paper investigates the correlation between marine aerosol optical properties and wind speeds over remote oceans using the spaceborne lidars ALADIN and CALIOP. Three remote ocean areas are selected. Pure marine aerosol optical properties at 355 nm are derived from ALADIN. The relationships between marine aerosol optical properties and wind speeds are analyzed within and above the marine atmospheric boundary layer, revealing the effect of wind speed on marine aerosols over remote oceans.
Jingting Huang, S. Marcela Loría-Salazar, Min Deng, Jaehwa Lee, and Heather A. Holmes
Atmos. Chem. Phys., 24, 3673–3698, https://doi.org/10.5194/acp-24-3673-2024, https://doi.org/10.5194/acp-24-3673-2024, 2024
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Increased wildfire intensity has resulted in taller wildfire smoke plumes. We investigate the vertical structure of wildfire smoke plumes using aircraft lidar data and establish two effective smoke plume height metrics. Four novel satellite-based plume height products are evaluated for wildfires in the western US. Our results provide guidance on the strengths and limitations of these satellite products and set the stage for improved plume rise estimates by leveraging satellite products.
Piyushkumar N. Patel, Jonathan H. Jiang, Ritesh Gautam, Harish Gadhavi, Olga Kalashnikova, Michael J. Garay, Lan Gao, Feng Xu, and Ali Omar
Atmos. Chem. Phys., 24, 2861–2883, https://doi.org/10.5194/acp-24-2861-2024, https://doi.org/10.5194/acp-24-2861-2024, 2024
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Global measurements of cloud condensation nuclei (CCN) are essential for understanding aerosol–cloud interactions and predicting climate change. To address this gap, we introduced a remote sensing algorithm that retrieves vertically resolved CCN number concentrations from airborne and spaceborne lidar systems. This innovation offers a global distribution of CCN concentrations from space, facilitating model evaluation and precise quantification of aerosol climate forcing.
Lorraine A. Remer, Robert C. Levy, and J. Vanderlei Martins
Atmos. Chem. Phys., 24, 2113–2127, https://doi.org/10.5194/acp-24-2113-2024, https://doi.org/10.5194/acp-24-2113-2024, 2024
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Aerosols are small liquid or solid particles suspended in the atmosphere, including smoke, particulate pollution, dust, and sea salt. Today, we rely on satellites viewing Earth's atmosphere to learn about these particles. Here, we speculate on the future to imagine how satellite viewing of aerosols will change. We expect more public and private satellites with greater capabilities, better ways to infer information from satellites, and merging of data with models.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Blake T. Sorenson, Jeffrey S. Reid, Jianglong Zhang, Robert E. Holz, William L. Smith Sr., and Amanda Gumber
Atmos. Chem. Phys., 24, 1231–1248, https://doi.org/10.5194/acp-24-1231-2024, https://doi.org/10.5194/acp-24-1231-2024, 2024
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Smoke particles are typically submicron in size and assumed to have negligible impacts at the thermal infrared spectrum. However, we show that infrared signatures can be observed over dense smoke plumes from satellites. We found that giant particles are unlikely to be the dominant cause. Rather, co-transported water vapor injected to the middle to upper troposphere and surface cooling beneath the plume due to shadowing are significant, with the surface cooling effect being the most dominant.
Farnaz Hosseinpour and Eric M. Wilcox
Atmos. Chem. Phys., 24, 707–724, https://doi.org/10.5194/acp-24-707-2024, https://doi.org/10.5194/acp-24-707-2024, 2024
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This study shows mechanistic relationships between the radiative effect of dust aerosols in the Saharan air layer and the kinetic energy of the African easterly waves across the tropical Atlantic Ocean using 22 years of daily satellite observations and reanalysis data based on satellite assimilation. Our findings suggest that dust aerosols not merely are transported by these waves but also contribute to the growth of waves through the enhancement of diabatic heating induced by dust.
Markus D. Petters, Tyas Pujiastuti, Ajmal Rasheeda Satheesh, Sabin Kasparoglu, Bethany Sutherland, and Nicholas Meskhidze
Atmos. Chem. Phys., 24, 745–762, https://doi.org/10.5194/acp-24-745-2024, https://doi.org/10.5194/acp-24-745-2024, 2024
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This work introduces a new method that uses remote sensing techniques to obtain surface number emissions of particles with a diameter greater than 500 nm. The technique was applied to study particle emissions at an urban site near Houston, TX, USA. The emissions followed a diurnal pattern and peaked near noon local time. The daily averaged emissions correlated with wind speed. The source is likely due to wind-driven erosion of material situated on asphalted and other hard surfaces.
Brian Harr, Bing Pu, and Qinjian Jin
EGUsphere, https://doi.org/10.5194/egusphere-2023-2896, https://doi.org/10.5194/egusphere-2023-2896, 2024
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We found that the formation of the extreme trans-Atlantic African dust event in June 2015 is associated with a brief surge in dust emissions over western North Africa and extreme circulation patterns, such as the greatly intensified easterly jets, that facilitated the westward transport of dust. The dust plume modified radiative flux along its transport pathway but had minor air quality impacts on the U.S. as the record-high Caribbean low-level jet advected part of the plume to the Pacific.
Zhuang Wang, Chune Shi, Hao Zhang, Yujia Chen, Xiyuan Chi, Congzi Xia, Suyao Wang, Yizhi Zhu, Kaidi Zhang, Xintong Chen, Chengzhi Xing, and Cheng Liu
Atmos. Chem. Phys., 23, 14271–14292, https://doi.org/10.5194/acp-23-14271-2023, https://doi.org/10.5194/acp-23-14271-2023, 2023
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The annual cycle of dust and anthropogenic aerosols' vertical distributions was revealed by polarization Raman lidar in Beijing. Anthropogenic aerosols typically accumulate at the top of the mixing layer (ML) due to the hygroscopic growth of atmospheric particles, and this is most significant in summer. There is no significant relationship between bottom dust mass concentration and ML height, while the dust in the upper air tends to be distributed near the mixing layer.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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We evaluated the long-term trends and seasonal variability of the vertically resolved aerosol properties over the past 17 years in Barcelona. Results shows that air quality is improved, with a consistent drop in PM concentrations at the surface, as well as the column aerosol optical depth. The results also show that natural dust outbreaks are more likely in summer, with aerosols reaching an altitude of 5 km, while in winter, aerosols decay as an exponential with a scale height of 600 m.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Jesús Abril-Gago, Pablo Ortiz-Amezcua, Diego Bermejo-Pantaleón, Juana Andújar-Maqueda, Juan Antonio Bravo-Aranda, María José Granados-Muñoz, Francisco Navas-Guzmán, Lucas Alados-Arboledas, Inmaculada Foyo-Moreno, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 8453–8471, https://doi.org/10.5194/acp-23-8453-2023, https://doi.org/10.5194/acp-23-8453-2023, 2023
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Validation activities of Aeolus wind products were performed in Granada with different upward-probing instrumentation (Doppler lidar system and radiosondes) and spatiotemporal collocation criteria. Specific advantages and disadvantages of each instrument were identified, and an optimal comparison criterion is proposed. Aeolus was proven to provide reliable wind products, and the upward-probing instruments were proven to be useful for Aeolus wind product validation activities.
Jianyu Zheng, Zhibo Zhang, Hongbin Yu, Anne Garnier, Qianqian Song, Chenxi Wang, Claudia Di Biagio, Jasper F. Kok, Yevgeny Derimian, and Claire Ryder
Atmos. Chem. Phys., 23, 8271–8304, https://doi.org/10.5194/acp-23-8271-2023, https://doi.org/10.5194/acp-23-8271-2023, 2023
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We developed a multi-year satellite-based retrieval of dust optical depth at 10 µm and the coarse-mode dust effective diameter over global oceans. It reveals climatological coarse-mode dust transport patterns and regional differences over the North Atlantic, the Indian Ocean and the North Pacific.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Mukunda M. Gogoi, S. Suresh Babu, Ryoichi Imasu, and Makiko Hashimoto
Atmos. Chem. Phys., 23, 8059–8079, https://doi.org/10.5194/acp-23-8059-2023, https://doi.org/10.5194/acp-23-8059-2023, 2023
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Considering the climate warming potential of atmospheric black carbon (BC), satellite-based retrieval is a novel idea. This study highlights the regional distribution of BC based on observations by the Cloud and Aerosol Imager-2 on board the GOSAT-2 satellite and near-surface measurements of BC in ARFINET. The satellite retrieval fairly depicts the regional and seasonal features of BC over the Indian region, which are similar to those recorded by surface observations.
Hao Fan, Xingchuan Yang, Chuanfeng Zhao, Yikun Yang, and Zhenyao Shen
Atmos. Chem. Phys., 23, 7781–7798, https://doi.org/10.5194/acp-23-7781-2023, https://doi.org/10.5194/acp-23-7781-2023, 2023
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Using 20-year multi-source data, this study shows pronounced regional and seasonal variations in fire activities and emissions. Seasonal variability of fires is larger with increasing latitude. The increase in temperature in the Northern Hemisphere's middle- and high-latitude forest regions was primarily responsible for the increase in fires and emissions, while the changes in fire occurrence in tropical regions were more influenced by the decrease in precipitation and relative humidity.
Rosemary Huck, Robert G. Bryant, and James King
Atmos. Chem. Phys., 23, 6299–6318, https://doi.org/10.5194/acp-23-6299-2023, https://doi.org/10.5194/acp-23-6299-2023, 2023
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This study shows that mineral aerosol (dust) emission events in high-latitude areas are under-represented in both ground- and space-based detecting methods. This is done through a suite of ground-based data to prove that dust emissions from the proglacial area, Lhù’ààn Mân, occur almost daily but are not always recorded at different timescales. Dust has multiple effects on atmospheric processes; therefore, accurate quantification is important in the calibration and validation of climate models.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
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We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Ross Herbert and Philip Stier
Atmos. Chem. Phys., 23, 4595–4616, https://doi.org/10.5194/acp-23-4595-2023, https://doi.org/10.5194/acp-23-4595-2023, 2023
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We provide robust evidence from multiple sources showing that smoke from fires in the Amazon rainforest significantly modifies the diurnal cycle of convection and cools the climate. Low to moderate amounts of smoke increase deep convective clouds and rain, whilst beyond a threshold amount, the smoke starts to suppress the convection and rain. We are currently at this threshold, suggesting increases in fires from agricultural practices or droughts will reduce cloudiness and rain over the region.
Yue Huang, Jasper F. Kok, Masanori Saito, and Olga Muñoz
Atmos. Chem. Phys., 23, 2557–2577, https://doi.org/10.5194/acp-23-2557-2023, https://doi.org/10.5194/acp-23-2557-2023, 2023
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Global aerosol models and remote sensing retrievals use dust optical models with inconsistent and inaccurate dust shape approximations. Here, we present a new dust optical model constrained by measured dust shape distributions. This new dust optical model is an improvement on the current dust optical models used in models and retrieval algorithms, as quantified by comparisons against laboratory and field observations of dust optics.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
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Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
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An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
Kyriakoula Papachristopoulou, Ioannis-Panagiotis Raptis, Antonis Gkikas, Ilias Fountoulakis, Akriti Masoom, and Stelios Kazadzis
Atmos. Chem. Phys., 22, 15703–15727, https://doi.org/10.5194/acp-22-15703-2022, https://doi.org/10.5194/acp-22-15703-2022, 2022
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Megacities' air quality is determined by atmospheric aerosols. We focus on changes over the last two decades in the 81 largest cities, using satellite data. European and American cities have lower aerosol compared to African and Asian cities. For European, North American and East Asian cities, aerosols are decreasing over time, especially in China and the US. In the remaining cities, aerosol loads are increasing, particularly in India.
Nilton Évora do Rosário, Elisa Thomé Sena, and Marcia Akemi Yamasoe
Atmos. Chem. Phys., 22, 15021–15033, https://doi.org/10.5194/acp-22-15021-2022, https://doi.org/10.5194/acp-22-15021-2022, 2022
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The 2020 burning season in Brazil was marked by an atypically high number of fire spots across Pantanal, leading to high amounts of smoke within the biome. This study shows that smoke over Pantanal, usually a fraction of that over Amazonia, was higher and resulted mainly from fires in conservation and indigenous areas. It also contributes to highlighting Pantanal's 2020 burning season as the worst combination of a climate extreme scenario and inadequately enforced environmental regulations.
Santiago Gassó and Kirk D. Knobelspiesse
Atmos. Chem. Phys., 22, 13581–13605, https://doi.org/10.5194/acp-22-13581-2022, https://doi.org/10.5194/acp-22-13581-2022, 2022
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Atmospheric particles interact with light resulting in observable optical polarization. Thus, we can learn about their composition from space. New satellite sensor technology measures full polarization of reflected sunlight. This paper considers circular polarization, an overlooked category of polarization with distinctive features that could bring new insights. We review existing literature and make novel computations to consider this previously underappreciated category of polarization.
Qingyang Xiao, Guannan Geng, Shigan Liu, Jiajun Liu, Xia Meng, and Qiang Zhang
Atmos. Chem. Phys., 22, 13229–13242, https://doi.org/10.5194/acp-22-13229-2022, https://doi.org/10.5194/acp-22-13229-2022, 2022
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We provided complete coverage PM2.5 concentrations at a 1-km resolution from 2000 to the present, carefully considering the significant changes in land use characteristics in China. This high-resolution PM2.5 data successfully revealed the local-scale PM2.5 variations. We noticed changes in PM2.5 spatial patterns in association with the clean air policies, with the pollution hotspots having transferred from urban centers to rural regions with limited air quality monitoring.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Ukkyo Jeong, Si-Chee Tsay, N. Christina Hsu, David M. Giles, John W. Cooper, Jaehwa Lee, Robert J. Swap, Brent N. Holben, James J. Butler, Sheng-Hsiang Wang, Somporn Chantara, Hyunkee Hong, Donghee Kim, and Jhoon Kim
Atmos. Chem. Phys., 22, 11957–11986, https://doi.org/10.5194/acp-22-11957-2022, https://doi.org/10.5194/acp-22-11957-2022, 2022
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Ultraviolet (UV) measurements from satellite and ground are important for deriving information on several atmospheric trace and aerosol characteristics. Simultaneous retrievals of aerosol and trace gases in this study suggest that water uptake by aerosols is one of the important phenomena affecting aerosol properties over northern Thailand, which is important for regional air quality and climate. Obtained aerosol properties covering the UV are also important for various satellite algorithms.
Abdulaziz Tunde Yakubu and Naven Chetty
Atmos. Chem. Phys., 22, 11065–11087, https://doi.org/10.5194/acp-22-11065-2022, https://doi.org/10.5194/acp-22-11065-2022, 2022
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This study examined the source of atmospheric aerosols and their role in forming clouds and rainfall over South Africa. The research provided answers to the cause of low precipitation, mainly linked to drought and water shortages experienced over the region. Further insight into the cause of occasional flooding that occurs in other parts of the area is provided. Finally, the study described the relationship between aerosol–cloud precipitation based on observation over the region.
África Barreto, Rosa D. García, Carmen Guirado-Fuentes, Emilio Cuevas, A. Fernando Almansa, Celia Milford, Carlos Toledano, Francisco J. Expósito, Juan P. Díaz, and Sergio F. León-Luis
Atmos. Chem. Phys., 22, 11105–11124, https://doi.org/10.5194/acp-22-11105-2022, https://doi.org/10.5194/acp-22-11105-2022, 2022
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A comprehensive characterization of atmospheric aerosols in the subtropical eastern North Atlantic has been carried out in this paper using long-term ground AERONET photometric observations over the period 2005–2020 from a unique network made up of four stations strategically located from sea level to 3555 m height on the island of Tenerife. This is a region that can be considered a key location to study the seasonal dependence of dust transport from the Sahel-Sahara.
Xiaoxi Zhao, Kan Huang, Joshua S. Fu, and Sabur F. Abdullaev
Atmos. Chem. Phys., 22, 10389–10407, https://doi.org/10.5194/acp-22-10389-2022, https://doi.org/10.5194/acp-22-10389-2022, 2022
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Long-range transport of Asian dust to the Arctic was considered an important source of Arctic air pollution. Different transport routes to the Arctic had divergent effects on the evolution of aerosol properties. Depositions of long-range-transported dust particles can reduce the Arctic surface albedo considerably. This study implied that the ubiquitous long-transport dust from China exerted considerable aerosol indirect effects on the Arctic and may have potential biogeochemical significance.
Katherine T. Junghenn Noyes, Ralph A. Kahn, James A. Limbacher, and Zhanqing Li
Atmos. Chem. Phys., 22, 10267–10290, https://doi.org/10.5194/acp-22-10267-2022, https://doi.org/10.5194/acp-22-10267-2022, 2022
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We compare retrievals of wildfire smoke particle size, shape, and light absorption from the MISR satellite instrument to modeling and other satellite data on land cover type, drought conditions, meteorology, and estimates of fire intensity (fire radiative power – FRP). We find statistically significant differences in the particle properties based on burning conditions and land cover type, and we interpret how changes in these properties point to specific aerosol aging mechanisms.
David W. Fillmore, David A. Rutan, Seiji Kato, Fred G. Rose, and Thomas E. Caldwell
Atmos. Chem. Phys., 22, 10115–10137, https://doi.org/10.5194/acp-22-10115-2022, https://doi.org/10.5194/acp-22-10115-2022, 2022
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This paper presents an evaluation of the aerosol analysis incorporated into the Clouds and the Earth's Radiant Energy System (CERES) data products as well as the aerosols' impact on solar radiation reaching the surface. CERES is a NASA Earth observation mission with instruments flying on various polar-orbiting satellites. Its primary objective is the study of the radiative energy balance of the climate system as well as examination of the influence of clouds and aerosols on this balance.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Harshvardhan Harshvardhan, Richard Ferrare, Sharon Burton, Johnathan Hair, Chris Hostetler, David Harper, Anthony Cook, Marta Fenn, Amy Jo Scarino, Eduard Chemyakin, and Detlef Müller
Atmos. Chem. Phys., 22, 9859–9876, https://doi.org/10.5194/acp-22-9859-2022, https://doi.org/10.5194/acp-22-9859-2022, 2022
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The evolution of aerosol in biomass burning smoke plumes that travel over marine clouds off the Atlantic coast of central Africa was studied using measurements made by a lidar deployed on a high-altitude aircraft. The main finding was that the physical properties of aerosol do not change appreciably once the plume has left land and travels over the ocean over a timescale of 1 to 2 d. Almost all particles in the plume are of radius less than 1 micrometer and spherical in shape.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Sudip Chakraborty, Bin Guan, Duane E. Waliser, and Arlindo M. da Silva
Atmos. Chem. Phys., 22, 8175–8195, https://doi.org/10.5194/acp-22-8175-2022, https://doi.org/10.5194/acp-22-8175-2022, 2022
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This study explores extreme aerosol transport events by aerosol atmospheric rivers (AARs) and shows the characteristics of individual AARs such as length, width, length-to-width ratio, transport strength, and dominant transport direction, the seasonal variations, the relationship to the spatial distribution of surface emissions, the vertical profiles of wind, aerosol mixing ratio, and aerosol mass fluxes, and the major planetary-scale aerosol transport pathways.
Guangyao Dai, Kangwen Sun, Xiaoye Wang, Songhua Wu, Xiangying E, Qi Liu, and Bingyi Liu
Atmos. Chem. Phys., 22, 7975–7993, https://doi.org/10.5194/acp-22-7975-2022, https://doi.org/10.5194/acp-22-7975-2022, 2022
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In this paper, a Sahara dust event is tracked with the spaceborne lidars ALADIN and CALIOP and the models ECMWF and HYSPLIT. The performance of ALADIN and CALIOP on tracking the dust event and on the observations of dust optical properties and wind fields during the dust transport is evaluated. The dust mass advection is defined, which is calculated with the combination of data from ALADIN and CALIOP coupled with the products from models to describe the dust transport quantitatively.
Ke Gui, Wenrui Yao, Huizheng Che, Linchang An, Yu Zheng, Lei Li, Hujia Zhao, Lei Zhang, Junting Zhong, Yaqiang Wang, and Xiaoye Zhang
Atmos. Chem. Phys., 22, 7905–7932, https://doi.org/10.5194/acp-22-7905-2022, https://doi.org/10.5194/acp-22-7905-2022, 2022
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This study investigates the aerosol optical and radiative properties and meteorological drivers during two mega SDS events over Northern China in March 2021. The MODIS-retrieved DOD data registered these two events as the most intense episode in the same period in history over the past 20 years. These two extreme SDS events were associated with both atmospheric circulation extremes and local meteorological anomalies that favor enhanced dust emissions in the Gobi Desert.
Manuel Gutleben, Silke Groß, Christian Heske, and Martin Wirth
Atmos. Chem. Phys., 22, 7319–7330, https://doi.org/10.5194/acp-22-7319-2022, https://doi.org/10.5194/acp-22-7319-2022, 2022
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The main transportation route of Saharan mineral dust particles leads over the subtropical Atlantic Ocean and is subject to a seasonal variation. This study investigates the characteristics of wintertime transatlantic dust transport towards the Caribbean by means of airborne lidar measurements. It is found that dust particles are transported at low atmospheric altitudes (<3.5 km) embedded in a relatively moist mixture with two other particle types, namely marine and biomass-burning particles.
Goutam Choudhury, Albert Ansmann, and Matthias Tesche
Atmos. Chem. Phys., 22, 7143–7161, https://doi.org/10.5194/acp-22-7143-2022, https://doi.org/10.5194/acp-22-7143-2022, 2022
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Lidars provide height-resolved type-specific aerosol properties and are key in studying vertically collocated aerosols and clouds. In this study, we compare the aerosol number concentrations derived from spaceborne lidar with the in situ flight measurements. Our results show a reasonable agreement between both datasets. Such an agreement has not been achieved yet. It shows the potential of spaceborne lidar in studying aerosol–cloud interactions, which is needed to improve our climate forecasts.
Nair K. Kala, Narayana Sarma Anand, Mohanan R. Manoj, Harshavardhana S. Pathak, Krishnaswamy K. Moorthy, and Sreedharan K. Satheesh
Atmos. Chem. Phys., 22, 6067–6085, https://doi.org/10.5194/acp-22-6067-2022, https://doi.org/10.5194/acp-22-6067-2022, 2022
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We present the 3-D distribution of atmospheric aerosols and highlight its variation with respect to longitudes over the Indian mainland and the surrounding oceans using long-term satellite observations and realistic synthesised data. The atmospheric heating due to the 3-D distribution of aerosols is estimated using radiative transfer calculations. We believe that our findings will have strong implications for aerosol–radiation interactions in regional climate simulations.
Archana Devi and Sreedharan K. Satheesh
Atmos. Chem. Phys., 22, 5365–5376, https://doi.org/10.5194/acp-22-5365-2022, https://doi.org/10.5194/acp-22-5365-2022, 2022
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Global maps of aerosol absorption were generated using a multi-satellite retrieval algorithm. The retrieved values were validated with available aircraft-based measurements and compared with other global datasets. Seasonal and spatial distributions of aerosol absorption over various regions are also presented. The global maps of single scattering albedo with improved accuracy provide important input to climate models for assessing the climatic impact of aerosols on regional and global scales.
Cited articles
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Freudenthaler, V., Esselborn, M., Wiegner, M., Heese, B., Tesche, M., Ansmann, A., Müller, D., Althausen, D., Wirth, M., Fix, A., Ehret, G., Knippertz, P., Toledano, C., Gasteiger, J., Garhammer, M., and Seefeldner, M.: Depolarization ratio profiling at several wavelengths in pure Saharan dust during SAMUM 2006, Tellus B, 61, 165–179, https://doi.org/10.1111/j.1600-0889.2008.00396.x, 2009.
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Haywood, J. M., Allan, R. P., Culverwell, I., Slingo, T., Milton, S., Edwards, J., and Clerbaux, N.: Can desert dust explain the outgoing longwave radiation anomaly over the Sahara during July 2003?, J. Geophys. Res., 110, D05105, https://doi.org/10.1029/2004JD005232, 2005.
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Iwasaka, Y., Shibata, T., Nagatani, T., Shi, G.-Y., Kim, Y. S., Matsuki, A., Trochkine, D., Zhang, D., Yamada, M., Nagatani, M., Nakata, H., Shen, Z., Li, G., Chen, B., and Kawahira, K.: Large depolarization ratio of free tropospheric aerosols over the Taklamakan Desert revealed by lidar measurements: Possible diffusion and transport of dust particles, J. Geophys. Res., 108, 8652, https://doi.org/10.1029/2002JD003267, 2003.
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Kim, D., Chin, M., Yu, H., Eck, T. F., Sinyuk, A., Smirnov, A., and Holben, B. N.: Dust optical properties over North Africa and Arabian Peninsula derived from the AERONET dataset, Atmos. Chem. Phys., 11, 10733–10741, https://doi.org/10.5194/acp-11-10733-2011, 2011.
Kinne, S., Schulz, M., Textor, C., Guibert, S., Balkanski, Y., Bauer, S. E., Berntsen, T., Berglen, T. F., Boucher, O., Chin, M., Collins, W., Dentener, F., Diehl, T., Easter, R., Feichter, J., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Herzog, M., Horowitz, L., Isaksen, I., Iversen, T., Kirkevåg, A., Kloster, S., Koch, D., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Lesins, G., Liu, X., Lohmann, U., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, O., Stier, P., Takemura, T., and Tie, X.: An AeroCom initial assessment – optical properties in aerosol component modules of global models, Atmos. Chem. Phys., 6, 1815–1834, https://doi.org/10.5194/acp-6-1815-2006, 2006.
Lafon, S., Rajot, J.-L., Alfaro, S. C., and Gaudichet, A.: Quantification of iron oxides in desert aerosol, Atmos. Environ., 38, 1211–1218, https://doi.org/10.1016/j.atmosenv.2003.11.006, 2004.
Lafon, S., Sokolik, I. N., Rajot, J. L., Caquineau, S., and Gaudichet, A.: Characterization of iron oxides in mineral dust aerosols: Implications for light absorption, J. Geophys. Res., 111, D21207, https://doi.org/10.1029/2005JD007016, 2006.
Lee, J., Kim, J., Song, C. H., Ryu, J.-H., Ahn, Y.-H., and Song, C. K.: Algorithm for retrieval of aerosol optical properties over the ocean from the Geostationary Ocean Color Imager, Remote Sens. Environ., 114, 1077–1088, https://doi.org/10.1016/j.rse.2009.12.021, 2010a.
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Mamouri, R.-E. and Ansmann, A.: Potential of polarization/Raman lidar to separate fine dust, coarse dust, maritime, and anthropogenic aerosol profiles, Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-131, in review, 2017.
Maring, H., Savoie, D. L., Izaguirre, M. A., Custals, L., and Reid, J. S.: Mineral dust aerosol size distribution change during atmospheric transport, J. Geophys. Res., 108, 8592, https://doi.org/10.1029/2002JD002536, 2003.
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This paper compares the particle linear depolarization ratio retrieved by AERONET with respect to the one measured by lidar. We can confirm that AERONET derived linear particle depolarization ratio can be used to retrieve the dust ratio in mixed dust plumes. We expect that our results can increase availability of AERONET sun–sky radiometer data in the atmospheric aerosol research and aerosol type classification.
This paper compares the particle linear depolarization ratio retrieved by AERONET with respect...
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