Articles | Volume 15, issue 12
https://doi.org/10.5194/acp-15-6775-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-6775-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
18 Jun 2015
Research article |
| 18 Jun 2015
Parameterization of convective transport in the boundary layer and its impact on the representation of the diurnal cycle of wind and dust emissions
Laboratoire de Météorologie Dynamique, CNRS/IPSL/UMPC, Paris, France
M. Gueye
LPAOSF, UCAD, Dakar, Sénégal
B. Diallo
Laboratoire de Météorologie Dynamique, CNRS/IPSL/UMPC, Paris, France
J.-L. Dufresne
Laboratoire de Météorologie Dynamique, CNRS/IPSL/UMPC, Paris, France
J. Escribano
Laboratoire de Météorologie Dynamique, CNRS/IPSL/UMPC, Paris, France
Laboratoire de Météorologie Dynamique, CNRS/IPSL/UMPC, Paris, France
B. Marticoréna
LISA, UMR CNRS 7583, UPEC, UPD, IPSL, Créteil, France
LISA, UMR CNRS 7583, UPEC, UPD, IPSL, Créteil, France
F. Guichard
CNRM-GAME, UMR CNRS 3589, Météo France, Toulouse, France
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Laurent Menut, Arineh Cholakian, Romain Pennel, Guillaume Siour, Sylvain Mailler, Myrto Valari, Lya Lugon, and Yann Meurdesoif
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Laurent Menut, Bertrand Bessagnet, Arineh Cholakian, Guillaume Siour, Sylvain Mailler, and Romain Pennel
Geosci. Model Dev., 17, 3645–3665, https://doi.org/10.5194/gmd-17-3645-2024, https://doi.org/10.5194/gmd-17-3645-2024, 2024
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This study is about the modelling of the atmospheric composition in Europe during the summer of 2022, when massive wildfires were observed. It is a sensitivity study dedicated to the relative impacts of two modelling processes that are able to modify the meteorology used for the calculation of the atmospheric chemistry and transport of pollutants.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
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Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
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This study explores the proportional relationships between carbonaceous aerosols (black and organic carbon) and trace gases using airborne measurements from two campaigns in Europe and East Asia. Differences between regions were found, but air quality models struggled to reproduce them accurately. We show that these proportional relationships can help to constrain models and can be used to infer aerosol concentrations from satellite observations of trace gases, especially in urban areas.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
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Sylvain Mailler, Romain Pennel, Laurent Menut, and Arineh Cholakian
Geosci. Model Dev., 16, 7509–7526, https://doi.org/10.5194/gmd-16-7509-2023, https://doi.org/10.5194/gmd-16-7509-2023, 2023
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We show that a new advection scheme named PPM + W (piecewise parabolic method + Walcek) offers geoscientific modellers an alternative, high-performance scheme designed for Cartesian-grid advection, with improved performance over the classical PPM scheme. The computational cost of PPM + W is not higher than that of PPM. With improved accuracy and controlled computational cost, this new scheme may find applications in chemistry-transport models, ocean models or atmospheric circulation models.
Gaëlle de Coëtlogon, Adrien Deroubaix, Cyrille Flamant, Laurent Menut, and Marco Gaetani
Atmos. Chem. Phys., 23, 15507–15521, https://doi.org/10.5194/acp-23-15507-2023, https://doi.org/10.5194/acp-23-15507-2023, 2023
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Using a numerical atmospheric model, we found that cooling sea surface temperatures along the southern coast of West Africa in July cause the “little dry season”. This effect reduces humidity and pollutant transport inland, potentially enhancing West Africa's synoptic and seasonal forecasting.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Laurent Menut
Geosci. Model Dev., 16, 4265–4281, https://doi.org/10.5194/gmd-16-4265-2023, https://doi.org/10.5194/gmd-16-4265-2023, 2023
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This study analyzes forecasts that were made in 2021 to help trigger measurements during the CADDIWA experiment. The WRF and CHIMERE models were run each day, and the first goal is to quantify the variability of the forecast as a function of forecast leads and forecast location. The possibility of using the different leads as an ensemble is also tested. For some locations, the correlation scores are better with this approach. This could be tested on operational forecast chains in the future.
Laurent Menut, Arineh Cholakian, Guillaume Siour, Rémy Lapere, Romain Pennel, Sylvain Mailler, and Bertrand Bessagnet
Atmos. Chem. Phys., 23, 7281–7296, https://doi.org/10.5194/acp-23-7281-2023, https://doi.org/10.5194/acp-23-7281-2023, 2023
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This study is about the wildfires occurring in France during the summer 2022. We study the forest fires that took place in the Landes during the summer of 2022. We show the direct impact of these fires on the air quality, especially downstream of the smoke plume towards the Paris region. We quantify the impact of these fires on the pollutants peak concentrations and the possible exceedance of thresholds.
Danny M. Leung, Jasper F. Kok, Longlei Li, Gregory S. Okin, Catherine Prigent, Martina Klose, Carlos Pérez García-Pando, Laurent Menut, Natalie M. Mahowald, David M. Lawrence, and Marcelo Chamecki
Atmos. Chem. Phys., 23, 6487–6523, https://doi.org/10.5194/acp-23-6487-2023, https://doi.org/10.5194/acp-23-6487-2023, 2023
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Desert dust modeling is important for understanding climate change, as dust regulates the atmosphere's greenhouse effect and radiation. This study formulates and proposes a more physical and realistic desert dust emission scheme for global and regional climate models. By considering more aeolian processes in our emission scheme, our simulations match better against dust observations than existing schemes. We believe this work is vital in improving dust representation in climate models.
Arineh Cholakian, Matthias Beekmann, Guillaume Siour, Isabelle Coll, Manuela Cirtog, Elena Ormeño, Pierre-Marie Flaud, Emilie Perraudin, and Eric Villenave
Atmos. Chem. Phys., 23, 3679–3706, https://doi.org/10.5194/acp-23-3679-2023, https://doi.org/10.5194/acp-23-3679-2023, 2023
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This article revolves around the simulation of biogenic secondary organic aerosols in the Landes forest (southwestern France). Several sensitivity cases involving biogenic emission factors, land cover data, anthropogenic emissions, and physical or meteorological parameters were performed and each compared to measurements both in the forest canopy and around the forest. The chemistry behind the formation of these aerosols and their production and transport in the forest canopy is discussed.
Sylvain Mailler, Laurent Menut, Arineh Cholakian, and Romain Pennel
Geosci. Model Dev., 16, 1119–1127, https://doi.org/10.5194/gmd-16-1119-2023, https://doi.org/10.5194/gmd-16-1119-2023, 2023
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Large or even
giantparticles of mineral dust exist in the atmosphere but, so far, solving an non-linear equation was needed to calculate the speed at which they fall in the atmosphere. The model we present, AerSett v1.0 (AERosol SETTling version 1.0), provides a new and simple way of calculating their free-fall velocity in the atmosphere, which will be useful to anyone trying to understand and represent adequately the transport of giant dust particles by the wind.
Rémy Lapere, Nicolás Huneeus, Sylvain Mailler, Laurent Menut, and Florian Couvidat
Atmos. Chem. Phys., 23, 1749–1768, https://doi.org/10.5194/acp-23-1749-2023, https://doi.org/10.5194/acp-23-1749-2023, 2023
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Glaciers in the Andes of central Chile are shrinking rapidly in response to global warming. This melting is accelerated by the deposition of opaque particles onto snow and ice. In this work, model simulations quantify typical deposition rates of soot on glaciers in summer and winter months and show that the contribution of emissions from Santiago is not as high as anticipated. Additionally, the combination of regional- and local-scale meteorology explains the seasonality in deposition.
Mathieu Lachatre, Sylvain Mailler, Laurent Menut, Arineh Cholakian, Pasquale Sellitto, Guillaume Siour, Henda Guermazi, Giuseppe Salerno, and Salvatore Giammanco
Atmos. Chem. Phys., 22, 13861–13879, https://doi.org/10.5194/acp-22-13861-2022, https://doi.org/10.5194/acp-22-13861-2022, 2022
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In this study, we have evaluated the predominance of various pathways of volcanic SO2 conversion to sulfates in the upper troposphere. We show that the main conversion pathway was gaseous oxidation by OH, although the liquid pathways were expected to be predominant. These results are interesting with respect to a better understanding of sulfate formation in the middle and upper troposphere and are an important component to help evaluate particulate matter radiative forcing.
Yoann Tellier, Cyril Crevoisier, Raymond Armante, Jean-Louis Dufresne, and Nicolas Meilhac
Geosci. Model Dev., 15, 5211–5231, https://doi.org/10.5194/gmd-15-5211-2022, https://doi.org/10.5194/gmd-15-5211-2022, 2022
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Accurate radiative transfer models (RTMs) are required to improve climate model simulations. We describe the module named 4A-Flux, which is implemented into 4A/OP RTM, aimed at calculating spectral longwave radiative fluxes given a description of the surface, atmosphere, and spectroscopy. In Pincus et al. (2020), 4A-Flux has shown good agreement with state-of-the-art RTMs. Here, it is applied to perform sensitivity studies and will be used to improve the understanding of radiative flux modeling.
Juan Cuesta, Lorenzo Costantino, Matthias Beekmann, Guillaume Siour, Laurent Menut, Bertrand Bessagnet, Tony C. Landi, Gaëlle Dufour, and Maxim Eremenko
Atmos. Chem. Phys., 22, 4471–4489, https://doi.org/10.5194/acp-22-4471-2022, https://doi.org/10.5194/acp-22-4471-2022, 2022
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We present the first comprehensive study integrating satellite observations of near-surface ozone pollution, surface in situ measurements, and a chemistry-transport model for quantifying the role of anthropogenic emission reductions during the COVID-19 lockdown in spring 2020. It confirms the occurrence of a net enhancement of ozone in central Europe and a reduction elsewhere, except for some hotspots, linked with the reduction of precursor emissions from Europe and the Northern Hemisphere.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Christophe Genthon, Dana Veron, Etienne Vignon, Delphine Six, Jean-Louis Dufresne, Jean-Baptiste Madeleine, Emmanuelle Sultan, and François Forget
Earth Syst. Sci. Data, 13, 5731–5746, https://doi.org/10.5194/essd-13-5731-2021, https://doi.org/10.5194/essd-13-5731-2021, 2021
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A 10-year dataset of observation in the atmospheric boundary layer at Dome C on the high Antarctic plateau is presented. This is obtained with sensors at six levels along a tower higher than 40 m. The temperature inversion can reach more than 25 °C along the tower in winter, while full mixing by convection can occur in summer. Different amplitudes of variability for wind and temperature at the different levels reflect different signatures of solar vs. synoptic forcing of the boundary layer.
Yangjunjie Xu-Yang, Rémi Losno, Fabrice Monna, Jean-Louis Rajot, Mohamed Labiadh, Gilles Bergametti, and Béatrice Marticorena
Atmos. Meas. Tech., 14, 7657–7680, https://doi.org/10.5194/amt-14-7657-2021, https://doi.org/10.5194/amt-14-7657-2021, 2021
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Suspended particles in air (aerosols) are sampled with a pump drawing ambient air through a filter. The air inlet must be carefully designed to control the size of sampled particles and to reject the largest ones (> 10 µm). A low-cost sampling head for determination of the finest fraction of aerosol (> 10 µm in diameter) is presented. Compositional data analysis (CoDA) tools are extensively used here to demonstrate similarity between the low-cost sampling head and other existing systems.
Laurent Menut, Bertrand Bessagnet, Régis Briant, Arineh Cholakian, Florian Couvidat, Sylvain Mailler, Romain Pennel, Guillaume Siour, Paolo Tuccella, Solène Turquety, and Myrto Valari
Geosci. Model Dev., 14, 6781–6811, https://doi.org/10.5194/gmd-14-6781-2021, https://doi.org/10.5194/gmd-14-6781-2021, 2021
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The CHIMERE chemistry-transport model is presented in its new version, V2020r1. Many changes are proposed compared to the previous version. These include online modeling, new parameterizations for aerosols, new emissions schemes, a new parameter file format, the subgrid-scale variability of urban concentrations and new transport schemes.
Gaëlle Dufour, Didier Hauglustaine, Yunjiang Zhang, Maxim Eremenko, Yann Cohen, Audrey Gaudel, Guillaume Siour, Mathieu Lachatre, Axel Bense, Bertrand Bessagnet, Juan Cuesta, Jerry Ziemke, Valérie Thouret, and Bo Zheng
Atmos. Chem. Phys., 21, 16001–16025, https://doi.org/10.5194/acp-21-16001-2021, https://doi.org/10.5194/acp-21-16001-2021, 2021
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The IASI observations and the LMDZ-OR-INCA model simulations show negative ozone trends in the Central East China region in the lower free (3–6 km column) and the upper free (6–9 km column) troposphere. Sensitivity studies from the model show that the Chinese anthropogenic emissions contribute to more than 50 % in the trend. The reduction in NOx emissions that has occurred since 2013 in China seems to lead to a decrease in ozone in the free troposphere, contrary to the increase at the surface.
Ramiro Checa-Garcia, Yves Balkanski, Samuel Albani, Tommi Bergman, Ken Carslaw, Anne Cozic, Chris Dearden, Beatrice Marticorena, Martine Michou, Twan van Noije, Pierre Nabat, Fiona M. O'Connor, Dirk Olivié, Joseph M. Prospero, Philippe Le Sager, Michael Schulz, and Catherine Scott
Atmos. Chem. Phys., 21, 10295–10335, https://doi.org/10.5194/acp-21-10295-2021, https://doi.org/10.5194/acp-21-10295-2021, 2021
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Thousands of tons of dust are emitted into the atmosphere every year, producing important impacts on the Earth system. However, current global climate models are not yet able to reproduce dust emissions, transport and depositions with the desirable accuracy. Our study analyses five different Earth system models to report aspects to be improved to reproduce better available observations, increase the consistency between models and therefore decrease the current uncertainties.
Audrey Fortems-Cheiney, Isabelle Pison, Grégoire Broquet, Gaëlle Dufour, Antoine Berchet, Elise Potier, Adriana Coman, Guillaume Siour, and Lorenzo Costantino
Geosci. Model Dev., 14, 2939–2957, https://doi.org/10.5194/gmd-14-2939-2021, https://doi.org/10.5194/gmd-14-2939-2021, 2021
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Up-to-date and accurate emission inventories for air pollutants are essential for understanding their role in the formation of tropospheric ozone and particulate matter, for anticipating pollution peaks and for identifying the key drivers that could help mitigate their emissions. Complementarily with bottom-up inventories, the system described here aims at updating and improving the knowledge on the high spatiotemporal variability of emissions of air pollutants.
Sanhita Ghosh, Shubha Verma, Jayanarayanan Kuttippurath, and Laurent Menut
Atmos. Chem. Phys., 21, 7671–7694, https://doi.org/10.5194/acp-21-7671-2021, https://doi.org/10.5194/acp-21-7671-2021, 2021
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Wintertime direct radiative perturbation due to black carbon (BC) aerosols was assessed over the Indo-Gangetic Plain with an efficiently modelled BC distribution. The atmospheric radiative warming due to BC was about 50–70 % larger than surface cooling. Compared to the atmosphere without BC, for which a net cooling at the top of the atmosphere was exhibited, enhanced atmospheric radiative warming by 2–3 times and a reduction in surface cooling by 10–20 % were found due to BC.
Sylvain Mailler, Romain Pennel, Laurent Menut, and Mathieu Lachâtre
Geosci. Model Dev., 14, 2221–2233, https://doi.org/10.5194/gmd-14-2221-2021, https://doi.org/10.5194/gmd-14-2221-2021, 2021
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Representing the advection of thin polluted plumes in numerical models is a challenging task since these models usually tend to excessively diffuse these plumes in the vertical direction. This numerical diffusion process is the cause of major difficulties in representing such dense and thin polluted plumes in numerical models. We propose here, and test in an academic framework, a novel method to solve this problem through the use of an antidiffusive advection scheme in the vertical direction.
Rémy Lapere, Laurent Menut, Sylvain Mailler, and Nicolás Huneeus
Atmos. Chem. Phys., 21, 6431–6454, https://doi.org/10.5194/acp-21-6431-2021, https://doi.org/10.5194/acp-21-6431-2021, 2021
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Based on modeling, the transport dynamics of ozone and fine particles in central Chile are investigated. Santiago emissions are found to influence air quality along a 1000 km plume as far as Argentina and northern Chile. In turn, emissions outside the metropolis contribute significantly to its recorded particles concentration. Emissions of precursors from Santiago are found to lead to the formation of a persistent ozone bubble in altitude, a phenomenon which is described for the first time.
Bertrand Bessagnet, Laurent Menut, and Maxime Beauchamp
Geosci. Model Dev., 14, 91–106, https://doi.org/10.5194/gmd-14-91-2021, https://doi.org/10.5194/gmd-14-91-2021, 2021
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This paper presents a new interpolator useful for geophysics applications. It can explore N-dimensional meshes, grids or look-up tables. The code accepts irregular but structured grids. Written in Fortran, it is easy to implement in existing codes and very fast and portable. We have compared it with a Python library. Python is convenient but suffers from portability and is sometimes not optimized enough. As an application case, this method is applied to atmospheric sciences.
Axel Fouqueau, Manuela Cirtog, Mathieu Cazaunau, Edouard Pangui, Pascal Zapf, Guillaume Siour, Xavier Landsheere, Guillaume Méjean, Daniele Romanini, and Bénédicte Picquet-Varrault
Atmos. Meas. Tech., 13, 6311–6323, https://doi.org/10.5194/amt-13-6311-2020, https://doi.org/10.5194/amt-13-6311-2020, 2020
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An incoherent broadband cavity-enhanced absorption spectroscopy (IBBCEAS) technique has been developed for the in situ monitoring of NO3 radicals in the CSA simulation chamber at LISA. The optical cavity allows a high sensitivity for NO3 detection up to 6 ppt for an integration time of 10 s. The technique is now fully operational and can be used to determine rate constants for fast reactions involving complex volatile organic compounds (with rate constants up to 10−10 cm3 molecule−1 s−1).
Mathieu Lachatre, Sylvain Mailler, Laurent Menut, Solène Turquety, Pasquale Sellitto, Henda Guermazi, Giuseppe Salerno, Tommaso Caltabiano, and Elisa Carboni
Geosci. Model Dev., 13, 5707–5723, https://doi.org/10.5194/gmd-13-5707-2020, https://doi.org/10.5194/gmd-13-5707-2020, 2020
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Excessive numerical diffusion is a major limitation in the representation of long-range transport in atmospheric models. In the present study, we focus on excessive diffusion in the vertical direction. We explore three possible ways of addressing this problem: increased vertical resolution, an advection scheme with anti-diffusive properties and more accurate representation of vertical wind. This study focused on a particular volcanic eruption event to improve atmospheric transport modeling.
Audrey Fortems-Cheiney, Gaëlle Dufour, Karine Dufossé, Florian Couvidat, Jean-Marc Gilliot, Guillaume Siour, Matthias Beekmann, Gilles Foret, Frederik Meleux, Lieven Clarisse, Pierre-François Coheur, Martin Van Damme, Cathy Clerbaux, and Sophie Génermont
Atmos. Chem. Phys., 20, 13481–13495, https://doi.org/10.5194/acp-20-13481-2020, https://doi.org/10.5194/acp-20-13481-2020, 2020
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Studies have suggested the importance of ammonia emissions on pollution particle formation over Europe, whose main atmospheric source is agriculture. In this study, we performed an inter-comparison of two alternative inventories, both with a reference inventory, that quantify the French ammonia emissions during spring 2011. Over regions with large mineral fertilizer use, like over northeastern France, NH3 emissions are probably considerably underestimated by the reference inventory.
Christopher J. Smith, Ryan J. Kramer, Gunnar Myhre, Kari Alterskjær, William Collins, Adriana Sima, Olivier Boucher, Jean-Louis Dufresne, Pierre Nabat, Martine Michou, Seiji Yukimoto, Jason Cole, David Paynter, Hideo Shiogama, Fiona M. O'Connor, Eddy Robertson, Andy Wiltshire, Timothy Andrews, Cécile Hannay, Ron Miller, Larissa Nazarenko, Alf Kirkevåg, Dirk Olivié, Stephanie Fiedler, Anna Lewinschal, Chloe Mackallah, Martin Dix, Robert Pincus, and Piers M. Forster
Atmos. Chem. Phys., 20, 9591–9618, https://doi.org/10.5194/acp-20-9591-2020, https://doi.org/10.5194/acp-20-9591-2020, 2020
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The spread in effective radiative forcing for both CO2 and aerosols is narrower in the latest CMIP6 (Coupled Model Intercomparison Project) generation than in CMIP5. For the case of CO2 it is likely that model radiation parameterisations have improved. Tropospheric and stratospheric radiative adjustments to the forcing behave differently for different forcing agents, and there is still significant diversity in how clouds respond to forcings, particularly for total anthropogenic forcing.
Solène Turquety, Laurent Menut, Guillaume Siour, Sylvain Mailler, Juliette Hadji-Lazaro, Maya George, Cathy Clerbaux, Daniel Hurtmans, and Pierre-François Coheur
Geosci. Model Dev., 13, 2981–3009, https://doi.org/10.5194/gmd-13-2981-2020, https://doi.org/10.5194/gmd-13-2981-2020, 2020
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Biomass burning emissions are a major source of trace gases and aerosols that need to be accounted for in air quality assessment and forecasting. The APIFLAME model presented in this paper allows the calculation of these emissions based on merged satellite observations at hourly time steps and kilometer scales. Implementing emissions in a chemistry transport model allows realistic simulations of fire plumes as illustrated for wildfires in Portugal in August 2016 using the CHIMERE model.
Pierre Sepulchre, Arnaud Caubel, Jean-Baptiste Ladant, Laurent Bopp, Olivier Boucher, Pascale Braconnot, Patrick Brockmann, Anne Cozic, Yannick Donnadieu, Jean-Louis Dufresne, Victor Estella-Perez, Christian Ethé, Frédéric Fluteau, Marie-Alice Foujols, Guillaume Gastineau, Josefine Ghattas, Didier Hauglustaine, Frédéric Hourdin, Masa Kageyama, Myriam Khodri, Olivier Marti, Yann Meurdesoif, Juliette Mignot, Anta-Clarisse Sarr, Jérôme Servonnat, Didier Swingedouw, Sophie Szopa, and Delphine Tardif
Geosci. Model Dev., 13, 3011–3053, https://doi.org/10.5194/gmd-13-3011-2020, https://doi.org/10.5194/gmd-13-3011-2020, 2020
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Our paper describes IPSL-CM5A2, an Earth system model that can be integrated for long (several thousands of years) climate simulations. We describe the technical aspects, assess the model computing performance and evaluate the strengths and weaknesses of the model, by comparing pre-industrial and historical runs to the previous-generation model simulations and to observations. We also present a Cretaceous simulation as a case study to show how the model simulates deep-time paleoclimates.
Antonio Tovar-Sánchez, Araceli Rodríguez-Romero, Anja Engel, Birthe Zäncker, Franck Fu, Emilio Marañón, María Pérez-Lorenzo, Matthieu Bressac, Thibaut Wagener, Sylvain Triquet, Guillaume Siour, Karine Desboeufs, and Cécile Guieu
Biogeosciences, 17, 2349–2364, https://doi.org/10.5194/bg-17-2349-2020, https://doi.org/10.5194/bg-17-2349-2020, 2020
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Residence times of particulate metals derived from aerosol deposition in the Sea Surface Microlayer of the Mediterranean Sea ranged from a couple of minutes (e.g., for Fe) to a few hours (e.g., for Cu). Microbial activity seems to play an important role in in this process and in the concentration and distribution of metals between diferent water layers.
Laurent Menut, Guillaume Siour, Bertrand Bessagnet, Florian Couvidat, Emilie Journet, Yves Balkanski, and Karine Desboeufs
Geosci. Model Dev., 13, 2051–2071, https://doi.org/10.5194/gmd-13-2051-2020, https://doi.org/10.5194/gmd-13-2051-2020, 2020
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Modelling of mineral dust is often done using one single mean species. In this study, differentiated mineral species with their chemical composition are implemented in the CHIMERE regional chemistry-transport model by using global databases. Simulations are carried out to quantify the realism and gain of such mineralogy.
Rémy Lapere, Laurent Menut, Sylvain Mailler, and Nicolás Huneeus
Atmos. Chem. Phys., 20, 4681–4694, https://doi.org/10.5194/acp-20-4681-2020, https://doi.org/10.5194/acp-20-4681-2020, 2020
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Based on measurements and modeling, this study shows that recent record-breaking peak events of fine particles in Santiago, Chile, can be traced back to massive barbecue cooking by its inhabitants during international soccer games. Decontamination plans in Santiago focus on decreasing emissions of pollutants from traffic, industry, and residential heating. This study implies that cultural habits such as barbecue cooking also need to be taken into account.
Bing Pu, Paul Ginoux, Huan Guo, N. Christina Hsu, John Kimball, Beatrice Marticorena, Sergey Malyshev, Vaishali Naik, Norman T. O'Neill, Carlos Pérez García-Pando, Juliette Paireau, Joseph M. Prospero, Elena Shevliakova, and Ming Zhao
Atmos. Chem. Phys., 20, 55–81, https://doi.org/10.5194/acp-20-55-2020, https://doi.org/10.5194/acp-20-55-2020, 2020
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Dust emission initiates when surface wind velocities exceed a threshold depending on soil and surface characteristics and varying spatially and temporally. Climate models widely use wind erosion thresholds. The climatological monthly global distribution of the wind erosion threshold, Vthreshold, is retrieved using satellite and reanalysis products and improves the simulation of dust frequency, magnitude, and the seasonal cycle in the Geophysical Fluid Dynamics Laboratory land–atmosphere model.
Laurent Menut, Paolo Tuccella, Cyrille Flamant, Adrien Deroubaix, and Marco Gaetani
Atmos. Chem. Phys., 19, 14657–14676, https://doi.org/10.5194/acp-19-14657-2019, https://doi.org/10.5194/acp-19-14657-2019, 2019
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Aerosol direct and indirect effects are studied over west Africa in the summer of 2016 using the coupled WRF-CHIMERE regional model including aerosol–cloud interaction parameterization. Sensitivity experiments are designed to gain insights into the impact of the aerosols dominating the atmospheric composition in southern west Africa. It is shown that the decrease of anthropogenic emissions along the coast has an impact on the mineral dust load over west Africa by increasing their emissions.
Henda Guermazi, Pasquale Sellitto, Juan Cuesta, Maxim Eremenko, Mathieu Lachatre, Sylvain Mailler, Elisa Carboni, Giuseppe Salerno, Tommaso Caltabiano, Laurent Menut, Mohamed Moncef Serbaji, Farhat Rekhiss, and Bernard Legras
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-341, https://doi.org/10.5194/amt-2019-341, 2019
Revised manuscript not accepted
Samuel Nahmani, Olivier Bock, and Françoise Guichard
Atmos. Chem. Phys., 19, 9541–9561, https://doi.org/10.5194/acp-19-9541-2019, https://doi.org/10.5194/acp-19-9541-2019, 2019
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A mesoscale convective system (MCS) is a cloud system that occurs in connection with an ensemble of thunderstorms and produces a contiguous precipitation area of the order of 100 km or more. Numerous questions related to MCSs remain poorly answered (e.g., their life cycle, and interactions between physical processes and atmospheric circulations). This work shows how a GPS technique can provide relevant and complementary information on MCSs passing over or in the vicinity of observation stations.
Mathieu Lachatre, Audrey Fortems-Cheiney, Gilles Foret, Guillaume Siour, Gaëlle Dufour, Lieven Clarisse, Cathy Clerbaux, Pierre-François Coheur, Martin Van Damme, and Matthias Beekmann
Atmos. Chem. Phys., 19, 6701–6716, https://doi.org/10.5194/acp-19-6701-2019, https://doi.org/10.5194/acp-19-6701-2019, 2019
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It has been observed from satellite-based instruments that ammonia levels strongly increased between 2011 and 2015. We have used the CHIMERE CTM to understand what could explain such an increase. We first focused on meteorological condition variations, and it has been concluded that meteorology did not explain ammonia evolution. Then, we focused on SO2 and NOx emission evolution rates to evaluate their influences on ammonia. It appears that theses decreases were the main explanation.
Marwa Majdi, Solene Turquety, Karine Sartelet, Carole Legorgeu, Laurent Menut, and Youngseob Kim
Atmos. Chem. Phys., 19, 785–812, https://doi.org/10.5194/acp-19-785-2019, https://doi.org/10.5194/acp-19-785-2019, 2019
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Joel Brito, Cyrielle Denjean, Volker Dreiling, Andreas Fink, Corinne Jambert, Norbert Kalthoff, Peter Knippertz, Russ Ladkin, Sylvain Mailler, Marlon Maranan, Federica Pacifico, Bruno Piguet, Guillaume Siour, and Solène Turquety
Atmos. Chem. Phys., 19, 473–497, https://doi.org/10.5194/acp-19-473-2019, https://doi.org/10.5194/acp-19-473-2019, 2019
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This article presents a detailed analysis of anthropogenic and biomass burning pollutants over the Gulf of Guinea coastal region, using observations from the DACCIWA field campaign and modeling. The novelty is that we focus on how these two pollution sources are mixed and transported further inland. We show that during the day pollutants are accumulated along the coastline and transported northward as soon as the daytime convection in the atmospheric boundary layer ceases (16:00 UTC).
Paola Formenti, Stuart John Piketh, Andreas Namwoonde, Danitza Klopper, Roelof Burger, Mathieu Cazaunau, Anaïs Feron, Cécile Gaimoz, Stephen Broccardo, Nicola Walton, Karine Desboeufs, Guillaume Siour, Mattheus Hanghome, Samuel Mafwila, Edosa Omoregie, Wolfgang Junkermann, and Willy Maenhaut
Atmos. Chem. Phys., 18, 17003–17016, https://doi.org/10.5194/acp-18-17003-2018, https://doi.org/10.5194/acp-18-17003-2018, 2018
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Three-years of continuous measurements at the Henties Bay Aerosol Observatory (HBAO; 22°S, 14°05’E), Namibia, show that during the austral wintertime, long- and medium-range transport of pollution from biomass and fossil fuel burning give rise to peaks of light-absorbing black carbon aerosols into the marine boundary layer ahead of the main biomass burning season. This could affect the cloud properties.
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Angela Benedetti, Jeffrey S. Reid, Peter Knippertz, John H. Marsham, Francesca Di Giuseppe, Samuel Rémy, Sara Basart, Olivier Boucher, Ian M. Brooks, Laurent Menut, Lucia Mona, Paolo Laj, Gelsomina Pappalardo, Alfred Wiedensohler, Alexander Baklanov, Malcolm Brooks, Peter R. Colarco, Emilio Cuevas, Arlindo da Silva, Jeronimo Escribano, Johannes Flemming, Nicolas Huneeus, Oriol Jorba, Stelios Kazadzis, Stefan Kinne, Thomas Popp, Patricia K. Quinn, Thomas T. Sekiyama, Taichu Tanaka, and Enric Terradellas
Atmos. Chem. Phys., 18, 10615–10643, https://doi.org/10.5194/acp-18-10615-2018, https://doi.org/10.5194/acp-18-10615-2018, 2018
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Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centers. This development is due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation authorities, solar energy plant managers, climate service providers, and health professionals. This paper describes the advances in the field and sets out requirements for observations for the sustainability of these activities.
Arineh Cholakian, Matthias Beekmann, Augustin Colette, Isabelle Coll, Guillaume Siour, Jean Sciare, Nicolas Marchand, Florian Couvidat, Jorge Pey, Valerie Gros, Stéphane Sauvage, Vincent Michoud, Karine Sellegri, Aurélie Colomb, Karine Sartelet, Helen Langley DeWitt, Miriam Elser, André S. H. Prévot, Sonke Szidat, and François Dulac
Atmos. Chem. Phys., 18, 7287–7312, https://doi.org/10.5194/acp-18-7287-2018, https://doi.org/10.5194/acp-18-7287-2018, 2018
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In this work, four schemes for the simulation of organic aerosols in the western Mediterranean basin are added to the CHIMERE chemistry–transport model; the resulting simulations are then compared to measurements obtained from ChArMEx. It is concluded that the scheme taking into account the fragmentation and the formation of nonvolatile organic aerosols corresponds better to measurements; the major source of this aerosol in the western Mediterranean is found to be of biogenic origin.
Alessandro Anav, Chiara Proietti, Laurent Menut, Stefano Carnicelli, Alessandra De Marco, and Elena Paoletti
Atmos. Chem. Phys., 18, 5747–5763, https://doi.org/10.5194/acp-18-5747-2018, https://doi.org/10.5194/acp-18-5747-2018, 2018
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Soil moisture and water stress play a pivotal role in regulating stomatal behaviour of plants; however, the role of water availability is often neglected in atmospheric chemistry modelling studies.
We show how dry deposition significantly declines when soil moisture is used to regulate the stomatal opening, mainly in semi-arid environments. Despite the fact that dry deposition occurs from the top of canopy to ground level, it affects the concentration of gases remaining in the lower atmosphere.
Laurent Menut, Cyrille Flamant, Solène Turquety, Adrien Deroubaix, Patrick Chazette, and Rémi Meynadier
Atmos. Chem. Phys., 18, 2687–2707, https://doi.org/10.5194/acp-18-2687-2018, https://doi.org/10.5194/acp-18-2687-2018, 2018
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During the DACCIWA project, the tropospheric chemical composition in large cities along the Gulf of Guinea is modelled using WRF and CHIMERE, with and without biomass burning emissions. The difference shows the net impact of fires on air quality in Lagos and Abidjan.
Roland Séférian, Sunghye Baek, Olivier Boucher, Jean-Louis Dufresne, Bertrand Decharme, David Saint-Martin, and Romain Roehrig
Geosci. Model Dev., 11, 321–338, https://doi.org/10.5194/gmd-11-321-2018, https://doi.org/10.5194/gmd-11-321-2018, 2018
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This paper presents a new interactive scheme for ocean surface albedo suited for the current generation of Earth system models. This scheme computes the ocean surface albedo accounting for the spectral dependence (across a range of wavelengths between 200 and 4000 nm), the characteristics of incident solar radiation (direct of diffuse), the effects of surface winds, chlorophyll content and whitecaps in addition to the canonical solar zenith angle dependence.
Adrien Deroubaix, Cyrille Flamant, Laurent Menut, Guillaume Siour, Sylvain Mailler, Solène Turquety, Régis Briant, Dmitry Khvorostyanov, and Suzanne Crumeyrolle
Atmos. Chem. Phys., 18, 445–465, https://doi.org/10.5194/acp-18-445-2018, https://doi.org/10.5194/acp-18-445-2018, 2018
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CO and PM2.5 are analyzed over the Guinean Gulf coastal region during the beginning of the 2006 West African monsoon. A biomass burning plume from Central Africa is observed since June at the Guinean coast. In June, the modeled anthropogenic PM2.5 concentrations are higher than in May or July. An important part of the pollution emitted along the coastline is transported to the north at night within the surface layer and within the nocturnal low-level jet.
Florian Couvidat, Bertrand Bessagnet, Marta Garcia-Vivanco, Elsa Real, Laurent Menut, and Augustin Colette
Geosci. Model Dev., 11, 165–194, https://doi.org/10.5194/gmd-11-165-2018, https://doi.org/10.5194/gmd-11-165-2018, 2018
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This paper includes the development of a new aerosol module in the air quality model CHIMERE to improve particulate matter (PM) simulation. The results of the model are compared to numerous measurements over Europe to evaluate the strengths and weaknesses of the model.
Habib Senghor, Éric Machu, Frédéric Hourdin, and Amadou Thierno Gaye
Atmos. Chem. Phys., 17, 8395–8410, https://doi.org/10.5194/acp-17-8395-2017, https://doi.org/10.5194/acp-17-8395-2017, 2017
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This work focus on the distribution of dust particles emitted in western Africa and having consequences on human health and marine ecosystems. The understanding of their fate requires a better understanding of the processes governing their variability. Using satellite observations and ground measurements, we present the seasonality of their distribution and explain the processes responsible for this distribution as well as their transition from the African continent towards the Atlantic Ocean.
Sylvain Mailler, Laurent Menut, Dmitry Khvorostyanov, Myrto Valari, Florian Couvidat, Guillaume Siour, Solène Turquety, Régis Briant, Paolo Tuccella, Bertrand Bessagnet, Augustin Colette, Laurent Létinois, Kostantinos Markakis, and Frédérik Meleux
Geosci. Model Dev., 10, 2397–2423, https://doi.org/10.5194/gmd-10-2397-2017, https://doi.org/10.5194/gmd-10-2397-2017, 2017
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CHIMERE is a chemistry-transport model initially designed for box-modelling of the regional atmospheric composition. In the recent years, CHIMERE has been extended to be able to model atmospheric composition at all scales from urban to hemispheric scale, which implied major changes on the coordinate systems as well as on physical processes. This study describes how and why these changes have been brought to the model, largely increasing the range of its possible use.
Pavlos Kalabokas, Jens Hjorth, Gilles Foret, Gaëlle Dufour, Maxim Eremenko, Guillaume Siour, Juan Cuesta, and Matthias Beekmann
Atmos. Chem. Phys., 17, 3905–3928, https://doi.org/10.5194/acp-17-3905-2017, https://doi.org/10.5194/acp-17-3905-2017, 2017
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The main atmospheric mechanisms linked with spring surface ozone episodes over the western Mediterranean are examined. It comes out that high surface midday ozone values are usually linked with regional ozone episodes, which are strongly influenced by some specific meteorological conditions. The better understanding of the ozone variability in the lower troposphere and the boundary layer over the examined regions will help in the formulation of more effective policies in environment and climate.
Laurent Menut, Sylvain Mailler, Bertrand Bessagnet, Guillaume Siour, Augustin Colette, Florian Couvidat, and Frédérik Meleux
Geosci. Model Dev., 10, 1199–1208, https://doi.org/10.5194/gmd-10-1199-2017, https://doi.org/10.5194/gmd-10-1199-2017, 2017
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A simple and complementary model evaluation technique for regional chemistry transport is discussed. The methodology is based on the concept that we can learn about model performance by comparing the simulation results with observational data available for time periods other than the period originally targeted.
Molly B. Smith, Natalie M. Mahowald, Samuel Albani, Aaron Perry, Remi Losno, Zihan Qu, Beatrice Marticorena, David A. Ridley, and Colette L. Heald
Atmos. Chem. Phys., 17, 3253–3278, https://doi.org/10.5194/acp-17-3253-2017, https://doi.org/10.5194/acp-17-3253-2017, 2017
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Using different meteorology reanalyses to drive dust in climate modeling can produce dissimilar global dust distributions, especially in the Southern Hemisphere (SH). It may therefore not be advisable for SH dust studies to base results on simulations driven by one reanalysis. Northern Hemisphere dust varies mostly on seasonal timescales, while SH dust varies on interannual timescales. Dust is an important part of climate modeling, and we hope this contributes to understanding these simulations.
Régis Briant, Paolo Tuccella, Adrien Deroubaix, Dmitry Khvorostyanov, Laurent Menut, Sylvain Mailler, and Solène Turquety
Geosci. Model Dev., 10, 927–944, https://doi.org/10.5194/gmd-10-927-2017, https://doi.org/10.5194/gmd-10-927-2017, 2017
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This paper presents the coupling of the CHIMERE chemistry-transport model with the WRF meteorological model, using the OASIS3-MCT coupler. WRF meteorological fields along with CHIMERE aerosol optical properties are exchanged through the coupler at a high frequency in order to model the aerosol direct and semi-direct effects.
Peter Good, Timothy Andrews, Robin Chadwick, Jean-Louis Dufresne, Jonathan M. Gregory, Jason A. Lowe, Nathalie Schaller, and Hideo Shiogama
Geosci. Model Dev., 9, 4019–4028, https://doi.org/10.5194/gmd-9-4019-2016, https://doi.org/10.5194/gmd-9-4019-2016, 2016
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The nonlinMIP model intercomparison project is described. nonlinMIP provides experiments that account for state-dependent regional and global climate responses. The experiments have two main applications: 1) to focus understanding of responses to CO2 forcing on states relevant to specific policy or scientific questions (e.g.
change under low-forcing scenarios, the benefits of mitigation, or from past cold climates to
the present day), or 2) to understand state dependence of climate responses.
Laurent Menut, Guillaume Siour, Sylvain Mailler, Florian Couvidat, and Bertrand Bessagnet
Atmos. Chem. Phys., 16, 12961–12982, https://doi.org/10.5194/acp-16-12961-2016, https://doi.org/10.5194/acp-16-12961-2016, 2016
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The aerosol is modelled during the summer 2013 with the WRF and CHIMERE models and over a large area encompassing Africa, Mediterranean sea and west Europe. The modelled aerosol is compared to available measurements such as the AERONET and EMEP networks. The model ability to estimate the aerosol speciation and size distribution is quantified.
Bertrand Bessagnet, Guido Pirovano, Mihaela Mircea, Cornelius Cuvelier, Armin Aulinger, Giuseppe Calori, Giancarlo Ciarelli, Astrid Manders, Rainer Stern, Svetlana Tsyro, Marta García Vivanco, Philippe Thunis, Maria-Teresa Pay, Augustin Colette, Florian Couvidat, Frédérik Meleux, Laurence Rouïl, Anthony Ung, Sebnem Aksoyoglu, José María Baldasano, Johannes Bieser, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, Sandro Finardi, Richard Kranenburg, Camillo Silibello, Claudio Carnevale, Wenche Aas, Jean-Charles Dupont, Hilde Fagerli, Lucia Gonzalez, Laurent Menut, André S. H. Prévôt, Pete Roberts, and Les White
Atmos. Chem. Phys., 16, 12667–12701, https://doi.org/10.5194/acp-16-12667-2016, https://doi.org/10.5194/acp-16-12667-2016, 2016
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The EURODELTA III exercise allows a very comprehensive intercomparison and evaluation of air quality models' performance. On average, the models provide a rather good picture of the particulate matter (PM) concentrations over Europe even if the highest concentrations are underestimated. The meteorology is responsible for model discrepancies, while the lack of emissions, particularly in winter, is mentioned as the main reason for the underestimations of PM.
Fleur Couvreux, Eric Bazile, Guylaine Canut, Yann Seity, Marie Lothon, Fabienne Lohou, Françoise Guichard, and Erik Nilsson
Atmos. Chem. Phys., 16, 8983–9002, https://doi.org/10.5194/acp-16-8983-2016, https://doi.org/10.5194/acp-16-8983-2016, 2016
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This study evaluates the ability of operational models to predict the boundary-layer turbulent processes and mesoscale variability observed during the Boundary Layer Late-Afternoon and Sunset Turbulence field campaign. The models succeed in reproducing the variability from one day to another in terms of cloud cover, temperature and boundary-layer depth. However, they exhibit some systematic biases. The high-resolution model reproduces the vertical structures better.
Vincent Lemaire, Isabelle Coll, Florian Couvidat, Camille Mouchel-Vallon, Christian Seigneur, and Guillaume Siour
Geosci. Model Dev., 9, 1361–1382, https://doi.org/10.5194/gmd-9-1361-2016, https://doi.org/10.5194/gmd-9-1361-2016, 2016
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Oligomerization is one of the most important identified processes of secondary organic aerosol evolution. We have simulated the formation of oligomers from biogenic precursors, using two different parameterizations implemented in the air quality model CHIMERE. This study shows that oligomer concentration fields are quite sensitive to the way the competition between local formation, evaporation and transport is restituted. The benefits and disadvantages of each approach are discussed in details.
Vincent E. P. Lemaire, Augustin Colette, and Laurent Menut
Atmos. Chem. Phys., 16, 2559–2574, https://doi.org/10.5194/acp-16-2559-2016, https://doi.org/10.5194/acp-16-2559-2016, 2016
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Because of its sensitivity to unfavorable weather patterns, air pollution is sensitive to climate change. Its impact is typically assessed using deterministic chemistry-transport models forced by an ensemble of climate projection. Because of the high computational cost of such initiative, elaborated techniques are required to optimize the exploration of ensemble of future projections. We develop such a technique, which also allows quantifying uncertainties in climate and air quality projections.
S. Mailler, L. Menut, A. G. di Sarra, S. Becagli, T. Di Iorio, B. Bessagnet, R. Briant, P. Formenti, J.-F. Doussin, J. L. Gómez-Amo, M. Mallet, G. Rea, G. Siour, D. M. Sferlazzo, R. Traversi, R. Udisti, and S. Turquety
Atmos. Chem. Phys., 16, 1219–1244, https://doi.org/10.5194/acp-16-1219-2016, https://doi.org/10.5194/acp-16-1219-2016, 2016
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We studied the impact of aerosols on tropospheric photolysis rates at Lampedusa during the CharMEx/ADRIMED campaign in June 2013. It is shown by using the CHIMERE chemistry-transport model (CTM) as well as in situ and remote-sensing measurements that taking into account the radiative effect of the tropospheric aerosols improves the ability of the model to reproduce the observed photolysis rates. It is hence important for CTMs to include the radiative effect of aerosols on photochemistry.
F. Wang, F. Cheruy, and J.-L. Dufresne
Geosci. Model Dev., 9, 363–381, https://doi.org/10.5194/gmd-9-363-2016, https://doi.org/10.5194/gmd-9-363-2016, 2016
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The soil thermodynamics in the IPSL climate model is improved by adopting a common vertical discretization for soil moisture and temperature, by coupling soil heat convection-conduction process, and by computing the thermal properties as a function of soil moisture and texture. The dependence of the soil thermal properties on moisture and texture lead to the most significant changes in the surface temperature, with the strongest effects taking place over dry areas and during the night.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
T. Dubos, S. Dubey, M. Tort, R. Mittal, Y. Meurdesoif, and F. Hourdin
Geosci. Model Dev., 8, 3131–3150, https://doi.org/10.5194/gmd-8-3131-2015, https://doi.org/10.5194/gmd-8-3131-2015, 2015
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The design of the icosahedral atmospheric dynamical core DYNAMICO is presented. The key contribution is to combine a strict separatation of kinematics from dynamics to a Hamiltonian formulation of the equations of motion in a non-Eulerian vertical coordinate to achieve energetic consistency. This approach allows for a unified treatment of various equations of motion: multi-layer shallow-water equations and hydrostatic primitive equations.
V. Marécal, V.-H. Peuch, C. Andersson, S. Andersson, J. Arteta, M. Beekmann, A. Benedictow, R. Bergström, B. Bessagnet, A. Cansado, F. Chéroux, A. Colette, A. Coman, R. L. Curier, H. A. C. Denier van der Gon, A. Drouin, H. Elbern, E. Emili, R. J. Engelen, H. J. Eskes, G. Foret, E. Friese, M. Gauss, C. Giannaros, J. Guth, M. Joly, E. Jaumouillé, B. Josse, N. Kadygrov, J. W. Kaiser, K. Krajsek, J. Kuenen, U. Kumar, N. Liora, E. Lopez, L. Malherbe, I. Martinez, D. Melas, F. Meleux, L. Menut, P. Moinat, T. Morales, J. Parmentier, A. Piacentini, M. Plu, A. Poupkou, S. Queguiner, L. Robertson, L. Rouïl, M. Schaap, A. Segers, M. Sofiev, L. Tarasson, M. Thomas, R. Timmermans, Á. Valdebenito, P. van Velthoven, R. van Versendaal, J. Vira, and A. Ung
Geosci. Model Dev., 8, 2777–2813, https://doi.org/10.5194/gmd-8-2777-2015, https://doi.org/10.5194/gmd-8-2777-2015, 2015
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This paper describes the air quality forecasting system over Europe put in place in the Monitoring Atmospheric Composition and Climate projects. It provides daily and 4-day forecasts and analyses for the previous day for major gas and particulate pollutants and their main precursors. These products are based on a multi-model approach using seven state-of-the-art models developed in Europe. An evaluation of the performance of the system is discussed in the paper.
M. Sofiev, U. Berger, M. Prank, J. Vira, J. Arteta, J. Belmonte, K.-C. Bergmann, F. Chéroux, H. Elbern, E. Friese, C. Galan, R. Gehrig, D. Khvorostyanov, R. Kranenburg, U. Kumar, V. Marécal, F. Meleux, L. Menut, A.-M. Pessi, L. Robertson, O. Ritenberga, V. Rodinkova, A. Saarto, A. Segers, E. Severova, I. Sauliene, P. Siljamo, B. M. Steensen, E. Teinemaa, M. Thibaudon, and V.-H. Peuch
Atmos. Chem. Phys., 15, 8115–8130, https://doi.org/10.5194/acp-15-8115-2015, https://doi.org/10.5194/acp-15-8115-2015, 2015
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The paper presents the first ensemble modelling experiment for forecasting the atmospheric dispersion of birch pollen in Europe. The study included 7 models of MACC-ENS tested over the season of 2010 and applied for 2013 in forecasting and reanalysis modes. The results were compared with observations in 11 countries, members of European Aeroallergen Network. The models successfully reproduced the timing of the unusually late season of 2013 but had more difficulties with absolute concentration.
G. Rea, S. Turquety, L. Menut, R. Briant, S. Mailler, and G. Siour
Atmos. Chem. Phys., 15, 8013–8036, https://doi.org/10.5194/acp-15-8013-2015, https://doi.org/10.5194/acp-15-8013-2015, 2015
L. Menut, G. Rea, S. Mailler, D. Khvorostyanov, and S. Turquety
Atmos. Chem. Phys., 15, 7897–7911, https://doi.org/10.5194/acp-15-7897-2015, https://doi.org/10.5194/acp-15-7897-2015, 2015
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The atmospheric composition was extensively studied in the European Mediterranean region and during summer 2013 within the framework of the ADRIMED project. During the campaign experiment, the WRF and CHIMERE models were used in forecast mode in order to help scientists to decide whether intensive observation periods should be triggered or not. This study quantifies the origin of the forecast error by comparing several forecast leads to the corresponding measurements.
C. Leauthaud, J. Demarty, B. Cappelaere, M. Grippa, L. Kergoat, C. Velluet, F. Guichard, E. Mougin, S. Chelbi, and B. Sultan
Proc. IAHS, 371, 195–201, https://doi.org/10.5194/piahs-371-195-2015, https://doi.org/10.5194/piahs-371-195-2015, 2015
L. Menut, S. Mailler, G. Siour, B. Bessagnet, S. Turquety, G. Rea, R. Briant, M. Mallet, J. Sciare, P. Formenti, and F. Meleux
Atmos. Chem. Phys., 15, 6159–6182, https://doi.org/10.5194/acp-15-6159-2015, https://doi.org/10.5194/acp-15-6159-2015, 2015
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The ozone and aerosol concentration variability is studied over the Euro-Mediterranean area during the months of June and July 2013 and in the framework of the ADRIMED project. A first analysis is performed using meteorological variables, ozone and aerosol concentrations using routine network station, satellite and specific ADRIMED project airborne measurements. This analysis is complemented by modeling using the WRF and CHIMERE regional models.
E. Cuevas, C. Camino, A. Benedetti, S. Basart, E. Terradellas, J. M. Baldasano, J. J. Morcrette, B. Marticorena, P. Goloub, A. Mortier, A. Berjón, Y. Hernández, M. Gil-Ojeda, and M. Schulz
Atmos. Chem. Phys., 15, 3991–4024, https://doi.org/10.5194/acp-15-3991-2015, https://doi.org/10.5194/acp-15-3991-2015, 2015
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Atmospheric mineral dust from a MACC-II short reanalysis (2007-2008) has been evaluated over northern Africa and the Middle East using satellite aerosol products, AERONET data, in situ PM10 concentrations, and extinction vertical profiles. The MACC-II AOD spatial and temporal variability shows good agreement with satellite sensors and AERONET. We find a good agreement in averaged extinction vertical profiles between MACC-II and lidars. MACC correctly reproduces daily to interannual PM10.
K. Haustein, R. Washington, J. King, G. Wiggs, D. S. G. Thomas, F. D. Eckardt, R. G. Bryant, and L. Menut
Geosci. Model Dev., 8, 341–362, https://doi.org/10.5194/gmd-8-341-2015, https://doi.org/10.5194/gmd-8-341-2015, 2015
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In this paper, the performance of three commonly used dust emissions schemes is investigated using a box model environment and observational data obtained in Botswana (Sua Pan). The results suggest that all schemes fail to reproduce the observed horizontal dust flux properly. They overestimate its magnitude by several orders of magnitude. The key parameter for this mismatch is the surface crusting which limits the availability of erosive material, even at higher wind speeds.
R. Locatelli, P. Bousquet, F. Hourdin, M. Saunois, A. Cozic, F. Couvreux, J.-Y. Grandpeix, M.-P. Lefebvre, C. Rio, P. Bergamaschi, S. D. Chambers, U. Karstens, V. Kazan, S. van der Laan, H. A. J. Meijer, J. Moncrieff, M. Ramonet, H. A. Scheeren, C. Schlosser, M. Schmidt, A. Vermeulen, and A. G. Williams
Geosci. Model Dev., 8, 129–150, https://doi.org/10.5194/gmd-8-129-2015, https://doi.org/10.5194/gmd-8-129-2015, 2015
E. Terrenoire, B. Bessagnet, L. Rouïl, F. Tognet, G. Pirovano, L. Létinois, M. Beauchamp, A. Colette, P. Thunis, M. Amann, and L. Menut
Geosci. Model Dev., 8, 21–42, https://doi.org/10.5194/gmd-8-21-2015, https://doi.org/10.5194/gmd-8-21-2015, 2015
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The model reproduces the temporal variability of NO2, O3, PM10, PM2.5 better at rural than urban background stations.
The fractional biases show that the model performs slightly better at RB sites than at UB sites for NO2, O3 and PM10.
At UB sites, CHIMERE reproduces PM2.5 better than PM10.
This is primarily the result of an underestimation of coarse particulate matter (PM) associated with uncertainties on SOA chemistry and their precursor emissions, dust and sea salt.
M. Lothon, F. Lohou, D. Pino, F. Couvreux, E. R. Pardyjak, J. Reuder, J. Vilà-Guerau de Arellano, P Durand, O. Hartogensis, D. Legain, P. Augustin, B. Gioli, D. H. Lenschow, I. Faloona, C. Yagüe, D. C. Alexander, W. M. Angevine, E Bargain, J. Barrié, E. Bazile, Y. Bezombes, E. Blay-Carreras, A. van de Boer, J. L. Boichard, A. Bourdon, A. Butet, B. Campistron, O. de Coster, J. Cuxart, A. Dabas, C. Darbieu, K. Deboudt, H. Delbarre, S. Derrien, P. Flament, M. Fourmentin, A. Garai, F. Gibert, A. Graf, J. Groebner, F. Guichard, M. A. Jiménez, M. Jonassen, A. van den Kroonenberg, V. Magliulo, S. Martin, D. Martinez, L. Mastrorillo, A. F. Moene, F. Molinos, E. Moulin, H. P. Pietersen, B. Piguet, E. Pique, C. Román-Cascón, C. Rufin-Soler, F. Saïd, M. Sastre-Marugán, Y. Seity, G. J. Steeneveld, P. Toscano, O. Traullé, D. Tzanos, S. Wacker, N. Wildmann, and A. Zaldei
Atmos. Chem. Phys., 14, 10931–10960, https://doi.org/10.5194/acp-14-10931-2014, https://doi.org/10.5194/acp-14-10931-2014, 2014
L. Menut, S. Mailler, G. Siour, B. Bessagnet, S. Turquety, G. Rea, R. Briant, M. Mallet, J. Sciare, and P. Formenti
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-23075-2014, https://doi.org/10.5194/acpd-14-23075-2014, 2014
Revised manuscript not accepted
R. Briant, L. Menut, G. Siour, and C. Prigent
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmdd-7-3441-2014, https://doi.org/10.5194/gmdd-7-3441-2014, 2014
Revised manuscript not accepted
L. Menut, R. Vautard, A. Colette, D. Khvorostyanov, A. Potier, L. Hamaoui-Laguel, N. Viovy, and M. Thibaudon
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-10891-2014, https://doi.org/10.5194/acpd-14-10891-2014, 2014
Revised manuscript not accepted
P. Yiou, M. Boichu, R. Vautard, M. Vrac, S. Jourdain, E. Garnier, F. Fluteau, and L. Menut
Clim. Past, 10, 797–809, https://doi.org/10.5194/cp-10-797-2014, https://doi.org/10.5194/cp-10-797-2014, 2014
F. Lohou, L. Kergoat, F. Guichard, A. Boone, B. Cappelaere, J.-M. Cohard, J. Demarty, S. Galle, M. Grippa, C. Peugeot, D. Ramier, C. M. Taylor, and F. Timouk
Atmos. Chem. Phys., 14, 3883–3898, https://doi.org/10.5194/acp-14-3883-2014, https://doi.org/10.5194/acp-14-3883-2014, 2014
S. Turquety, L. Menut, B. Bessagnet, A. Anav, N. Viovy, F. Maignan, and M. Wooster
Geosci. Model Dev., 7, 587–612, https://doi.org/10.5194/gmd-7-587-2014, https://doi.org/10.5194/gmd-7-587-2014, 2014
J. C. Péré, B. Bessagnet, M. Mallet, F. Waquet, I. Chiapello, F. Minvielle, V. Pont, and L. Menut
Atmos. Chem. Phys., 14, 1999–2013, https://doi.org/10.5194/acp-14-1999-2014, https://doi.org/10.5194/acp-14-1999-2014, 2014
M. Boichu, L. Menut, D. Khvorostyanov, L. Clarisse, C. Clerbaux, S. Turquety, and P.-F. Coheur
Atmos. Chem. Phys., 13, 8569–8584, https://doi.org/10.5194/acp-13-8569-2013, https://doi.org/10.5194/acp-13-8569-2013, 2013
A. Colette, B. Bessagnet, R. Vautard, S. Szopa, S. Rao, S. Schucht, Z. Klimont, L. Menut, G. Clain, F. Meleux, G. Curci, and L. Rouïl
Atmos. Chem. Phys., 13, 7451–7471, https://doi.org/10.5194/acp-13-7451-2013, https://doi.org/10.5194/acp-13-7451-2013, 2013
L. Menut, B. Bessagnet, D. Khvorostyanov, M. Beekmann, N. Blond, A. Colette, I. Coll, G. Curci, G. Foret, A. Hodzic, S. Mailler, F. Meleux, J.-L. Monge, I. Pison, G. Siour, S. Turquety, M. Valari, R. Vautard, and M. G. Vivanco
Geosci. Model Dev., 6, 981–1028, https://doi.org/10.5194/gmd-6-981-2013, https://doi.org/10.5194/gmd-6-981-2013, 2013
S. Mailler, D. Khvorostyanov, and L. Menut
Atmos. Chem. Phys., 13, 5987–5998, https://doi.org/10.5194/acp-13-5987-2013, https://doi.org/10.5194/acp-13-5987-2013, 2013
V. Michoud, A. Kukui, M. Camredon, A. Colomb, A. Borbon, K. Miet, B. Aumont, M. Beekmann, R. Durand-Jolibois, S. Perrier, P. Zapf, G. Siour, W. Ait-Helal, N. Locoge, S. Sauvage, C. Afif, V. Gros, M. Furger, G. Ancellet, and J. F. Doussin
Atmos. Chem. Phys., 12, 11951–11974, https://doi.org/10.5194/acp-12-11951-2012, https://doi.org/10.5194/acp-12-11951-2012, 2012
S. Stromatas, S. Turquety, L. Menut, H. Chepfer, J. C. Péré, G. Cesana, and B. Bessagnet
Geosci. Model Dev., 5, 1543–1564, https://doi.org/10.5194/gmd-5-1543-2012, https://doi.org/10.5194/gmd-5-1543-2012, 2012
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Exploring the aerosol activation properties in coastal shallow convection using cloud- and particle-resolving models
Machine-learning-assisted inference of the particle charge fraction and the ion-induced nucleation rates during new particle formation events
Modeling CMAQ dry deposition treatment over the western Pacific: a distinct characteristic of mineral dust and anthropogenic aerosols
Impact of post-monsoon crop residue burning on PM2.5 over northern India: optimizing emissions using a high-density in situ surface observation network
Modeling simulation of aerosol light absorption over the Beijing–Tianjin–Hebei region: the impact of mixing state and aging processes
An investigation of the impact of Canadian wildfires on US air quality using model, satellite, and ground measurements
How to trace the origins of short-lived atmospheric species: an Arctic example
Dust-producing weather patterns of the North American Great Plains
High-resolution air quality maps for Bucharest using a mixed-effects modeling framework
Interdecadal shift in the impact of winter land-sea thermal contrasts on following spring transcontinental dust transport pathways in North Africa
Anthropogenic and Natural Causes for the Interannual Variation of PM2.5 in East Asia During Summer Monsoon Periods From 2008 to 2018
Construction and application of a pollen emissions model based on phenology and random forests
An uncertain future for the climate and health impacts of anthropogenic aerosols in Africa
The impact of uncertainty in black carbon's refractive index on simulated optical depth and radiative forcing
Gas-phase collision rate enhancement factors for acid-base clusters up to 2 nm in diameter from atomistic simulation and the interacting hard sphere model
Characterization of brown carbon absorption in different European environments through source contribution analysis
Accounting for the black carbon aging process in a two-way coupled meteorology–air quality model
The effectiveness of solar radiation management using fine sea spray across multiple climatic regions
A global dust emission dataset for estimating dust radiative forcings in climate models
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution
Spatial and temporal evolution of future atmospheric reactive nitrogen deposition in China under different climate change mitigation strategies
Steady-state mixing state of black carbon aerosols from a particle-resolved model
Direct radiative forcing of light-absorbing carbonaceous aerosol and the influencing factors over China
Distinctive dust weather intensities in North China resulted from two types of atmospheric circulation anomalies
Biomass burning emission analysis based on MODIS aerosol optical depth and AeroCom multi-model simulations: implications for model constraints and emission inventories
Quasi-weekly oscillation of regional PM2.5 transport over China driven by the synoptic-scale disturbance of the East Asian winter monsoon circulation
Solar radiation estimation in West Africa: impact of dust conditions during the 2021 dry season
Modeling urban pollutant transport at multi-resolutions: Impacts of turbulent mixing
Homogeneous ice nucleation in adsorbed water films: A theoretical approach
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK Earth System Model
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Impact of Topographic Wind Conditions on Dust Particle Size Distribution: Insights from a Regional Dust Reanalysis Dataset
Uncovering the Impact of Urban Functional Zones on Air Quality in China
Seasonal differences in observed versus modeled new particle formation over boreal regions
Warming effects of reduced sulfur emissions from shipping
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
Multi-model effective radiative forcing of the 2020 sulfur cap for shipping
Representation of iron aerosol size distributions of anthropogenic emissions is critical in evaluating atmospheric soluble iron input to the ocean
Radiative and climate effects of aerosol scattering in long-wave radiation based on global climate modeling
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
A Novel Method to Quantify the Uncertainty Contribution of Aerosol-Radiative Interaction Factors
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
Impact of biomass burning aerosols (BBA) on the tropical African climate in an ocean–atmosphere–aerosol coupled climate model
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Strong inter-model differences and biases in CMIP6 simulations of PM2.5, aerosol optical depth, and precipitation over Africa
Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm
Dust aerosol from the Aralkum Desert influences the radiation budget and atmospheric dynamics of Central Asia
Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Synergistic effects of the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) on dust activities in North China during the following spring
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Ge Yu, Yueya Wang, Zhe Wang, and Xiaoming Shi
Atmos. Chem. Phys., 25, 7527–7542, https://doi.org/10.5194/acp-25-7527-2025, https://doi.org/10.5194/acp-25-7527-2025, 2025
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Studying the cloud-forming capacity of aerosols is crucial in climate research. The PartMC model can provide detailed particle information and help these studies. This model is integrated with the ideal meteorological Cloud Model 1 (CM1) to simulate the aerosols at cloud-forming locations. Significant changes are revealed in the hygroscopicity distribution of aerosols within ascending air parcels. Additionally, different ascent times also affect aerosol aging processes.
Pan Wang, Yue Zhao, Jiandong Wang, Veli-Matti Kerminen, Jingkun Jiang, and Chenxi Li
Atmos. Chem. Phys., 25, 7431–7446, https://doi.org/10.5194/acp-25-7431-2025, https://doi.org/10.5194/acp-25-7431-2025, 2025
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We developed a numerical model to investigate the evolution of the charge state of newly formed atmospheric particles. Based on the simulation results, we successfully employed neural networks to predict particle charge states and estimate ion-induced nucleation rates. This study provides new insights into the dynamics of particle charging and introduces advanced methods for evaluating ion-induced nucleation in atmospheric research.
Steven Soon-Kai Kong, Joshua S. Fu, Neng-Huei Lin, Guey-Rong Sheu, and Wei-Syun Huang
Atmos. Chem. Phys., 25, 7245–7268, https://doi.org/10.5194/acp-25-7245-2025, https://doi.org/10.5194/acp-25-7245-2025, 2025
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The accuracy of the chemical transport model, a key focus of our research, is strongly dependent on the dry deposition parameterization. Our findings show that the refined CMAQ dust model correlated well with ground-based and high-altitude in situ measurements by implementing the suggested dry deposition schemes. Furthermore, we reveal the mixing state of two types of aerosols at the upper level, a finding supported by both the optimized model and measurements.
Mizuo Kajino, Kentaro Ishijima, Joseph Ching, Kazuyo Yamaji, Rio Ishikawa, Tomoki Kajikawa, Tanbir Singh, Tomoki Nakayama, Yutaka Matsumi, Koyo Kojima, Taisei Machida, Takashi Maki, Prabir K. Patra, and Sachiko Hayashida
Atmos. Chem. Phys., 25, 7137–7160, https://doi.org/10.5194/acp-25-7137-2025, https://doi.org/10.5194/acp-25-7137-2025, 2025
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Air pollution in Delhi during the post-monsoon period is severe, and association with intensive crop residue burning (CRB) over Punjab state has attracted attention. However, the relationship has been unclear as the CRB emissions conventionally derived from satellites were underestimated due to clouds or thick smoke/haze over the region. We evaluated the impact of CRB on PM2.5 to be about 50 %, based on a combination of numerical modeling and an observation network using low-cost sensors we installed.
Huiyun Du, Jie Li, Xueshun Chen, Gabriele Curci, Fangqun Yu, Yele Sun, Xu Dao, Song Guo, Zhe Wang, Wenyi Yang, Lianfang Wei, and Zifa Wang
Atmos. Chem. Phys., 25, 5665–5681, https://doi.org/10.5194/acp-25-5665-2025, https://doi.org/10.5194/acp-25-5665-2025, 2025
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Inadequate consideration of mixing states and coatings on black carbon (BC) hinders aerosol radiation forcing quantification. Core–shell mixing aligns well with observations, but partial internal mixing is a more realistic representation. We used a microphysics module to determine the fraction of embedded BC and coating aerosols, constraining the mixing state. This reduced absorption enhancement by 30 %–43 % in northern China, offering insights into BC's radiative effects.
Zhixin Xue, Nair Udaysankar, and Sundar A. Christopher
Atmos. Chem. Phys., 25, 5497–5517, https://doi.org/10.5194/acp-25-5497-2025, https://doi.org/10.5194/acp-25-5497-2025, 2025
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Canadian wildfires in August 2018 significantly increased surface air pollution across the United States (US) – by up to 69 % in some areas. Using model, satellite, and ground measurements, the study highlights how weather patterns and long-range smoke transport drive pollution. The northwestern US was most affected by Canadian wildfire smoke, while the northeastern US experienced the least impact. These findings indicate the growing concern that wildfire smoke poses to air quality across the US.
Anderson Da Silva, Louis Marelle, Jean-Christophe Raut, Yvette Gramlich, Karolina Siegel, Sophie L. Haslett, Claudia Mohr, and Jennie L. Thomas
Atmos. Chem. Phys., 25, 5331–5354, https://doi.org/10.5194/acp-25-5331-2025, https://doi.org/10.5194/acp-25-5331-2025, 2025
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Particle sources in polar climates are unclear, affecting climate representation in models. This study introduces an evaluated method for tracking particles with backward modeling. Tests on simulated particles allowed us to show that traditional detection methods often misidentify sources. An improved method that accurately traces the origins of aerosol particles in the Arctic is presented. The study recommends using this enhanced method for better source identification of atmospheric species.
Stuart Evans
Atmos. Chem. Phys., 25, 4833–4845, https://doi.org/10.5194/acp-25-4833-2025, https://doi.org/10.5194/acp-25-4833-2025, 2025
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This study of the North American Great Plains identifies the various weather patterns responsible for blowing dust in all parts of the region using a weather pattern classification. In the southwestern plains passing cold fronts are the primary cause of dust; in the understudied northern plains, summertime patterns and southerly pre-frontal winds are most important in the west and east, respectively. These results are valuable to understanding and forecasting dust in this complex source region.
Camelia Talianu, Jeni Vasilescu, Doina Nicolae, Alexandru Ilie, Andrei Dandocsi, Anca Nemuc, and Livio Belegante
Atmos. Chem. Phys., 25, 4639–4654, https://doi.org/10.5194/acp-25-4639-2025, https://doi.org/10.5194/acp-25-4639-2025, 2025
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For Bucharest, Romania's capital, mobile measurements during two intensive campaigns and mixed-effect LUR (land-use regression) models to derive seasonal maps of near-surface PM10, NO2 and UFPs (ultrafine particles) have successfully been used. The model's performance was evaluated, demonstrating its potential for high-resolution mapping in other cities with well-characterized urban structures and diverse in situ monitoring stations.
Qi Wen, Yan Li, Mengying Du, Wenjun Song, Linbo Wei, Zhilan Wang, and Xu Li
EGUsphere, https://doi.org/10.5194/egusphere-2025-826, https://doi.org/10.5194/egusphere-2025-826, 2025
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We find that, through an interdecadal phase-locking effect of sea-land thermal forcing-North Atlantic Oscillation-Westerly Jet coupling, springtime dust from North Africa is more likely to be transported eastwards (extending into North America) after the late 1990s, whereas before that time westward transport paths for dust were more frequent. Subject to thermal forcing, wind speed and drought contribute to dust emissions in the two periods, respectively.
Danyang Ma, Min Xie, Huan He, Tijian Wang, Mengzhu Xi, Lingyun Feng, Shuxian Zhang, and Shitong Chen
EGUsphere, https://doi.org/10.5194/egusphere-2025-10, https://doi.org/10.5194/egusphere-2025-10, 2025
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The PM2.5 concentration in China underwent significant changes in 2013. We examined the underlying causes from three perspectives: anthropogenic pollutant emissions, meteorological conditions, and CO2 concentration variations. Our study highlighted the importance of considering the role of CO2 on vegetation when predicting PM2.5 concentrations and developing corresponding control strategies.
Jiangtao Li, Xingqin An, Zhaobin Sun, Caihua Ye, Qing Hou, Yuxin Zhao, and Zhe Liu
Atmos. Chem. Phys., 25, 3583–3602, https://doi.org/10.5194/acp-25-3583-2025, https://doi.org/10.5194/acp-25-3583-2025, 2025
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Climate change and pollution have intensified pollen allergies. We developed a pollen emissions model using phenology and random forests. Key factors affecting annual pollen emissions include temperature, relative humidity and sunshine hours. Pollen dispersal starts around 10 August, peaks around 30 August and ends by 25 September, lasting about 45 d. Over time, annual pollen emissions exhibit significant fluctuations and a downward trend.
Joe Adabouk Amooli, Marianne T. Lund, Sourangsu Chowdhury, Gunnar Myhre, Ane N. Johansen, Bjørn H. Samset, and Daniel M. Westervelt
EGUsphere, https://doi.org/10.5194/egusphere-2025-948, https://doi.org/10.5194/egusphere-2025-948, 2025
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We analyze various projections of African aerosol emissions and their potential impacts on climate and public health. We find that future emissions vary widely across emission projections, with differences in sectoral emission distributions. Using the Oslo chemical transport model, we show that air pollution exposure in some regions of Africa could increase significantly by 2050, increasing pollution-related deaths, with most scenarios projecting aerosol-induced warming over sub-Saharan Africa.
Ruth A. R. Digby, Knut von Salzen, Adam H. Monahan, Nathan P. Gillett, and Jiangnan Li
Atmos. Chem. Phys., 25, 3109–3130, https://doi.org/10.5194/acp-25-3109-2025, https://doi.org/10.5194/acp-25-3109-2025, 2025
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The refractive index of black carbon (BCRI), which determines how much energy black carbon absorbs and scatters, is difficult to measure, and different climate models use different values. We show that varying the BCRI across commonly used values can increase absorbing aerosol optical depth by 42 % and the warming effect from interactions between black carbon and radiation by 47 %, an appreciable fraction of the overall spread between models reported in recent literature assessments.
Valtteri Tikkanen, Huan Yang, Hanna Vehkamäki, and Bernhard Reischl
EGUsphere, https://doi.org/10.5194/egusphere-2025-507, https://doi.org/10.5194/egusphere-2025-507, 2025
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Collisions of neutral molecules and clusters is the prevalent pathway in atmospheric new particle formation. In heavily polluted urban areas, where clusters are formed rapidly and in large number, cluster-cluster collisions also become relevant. We calculate cluster-cluster collision rates from atomistic molecular dynamics simulations and an interacting hard sphere model. Not accounting for long-range attractive interactions underestimates collision and particle formation rates significantly.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre S. H. Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurélien Chauvigné, Sébastien Conil, Marco Pandolfi, and Oriol Jorba
Atmos. Chem. Phys., 25, 2667–2694, https://doi.org/10.5194/acp-25-2667-2025, https://doi.org/10.5194/acp-25-2667-2025, 2025
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Brown carbon (BrC) absorbs ultraviolet (UV) and visible light, influencing climate. This study explores BrC's imaginary refractive index (k) using data from 12 European sites. Residential emissions are a major organic aerosol (OA) source in winter, while secondary organic aerosol (SOA) dominates in summer. Source-specific k values were derived, improving model accuracy. The findings highlight BrC's climate impact and emphasize source-specific constraints in atmospheric models.
Yuzhi Jin, Jiandong Wang, Chao Liu, David C. Wong, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
Atmos. Chem. Phys., 25, 2613–2630, https://doi.org/10.5194/acp-25-2613-2025, https://doi.org/10.5194/acp-25-2613-2025, 2025
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Black carbon (BC) affects climate and the environment, and its aging process alters its properties. Current models, like WRF-CMAQ, lack full accounting for it. We developed the WRF-CMAQ-BCG model to better represent BC aging by introducing bare and coated BC species and their conversion. The WRF-CMAQ-BCG model introduces the capability to simulate BC mixing states and bare and coated BC wet deposition, and it improves the accuracy of BC mass concentration and aerosol optics.
Zhe Song, Shaocai Yu, Pengfei Li, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, and Daniel Rosenfeld
Atmos. Chem. Phys., 25, 2473–2494, https://doi.org/10.5194/acp-25-2473-2025, https://doi.org/10.5194/acp-25-2473-2025, 2025
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Our results with injected sea salt aerosols for five open oceans show that sea salt aerosols with low injection amounts dominate shortwave radiation, mainly through indirect effects. As indirect aerosol effects saturate with increasing injection rates, direct effects exceed indirect effects. This implies that marine cloud brightening is best implemented in areas with extensive cloud cover, while aerosol direct scattering effects remain dominant when clouds are scarce.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
Atmos. Chem. Phys., 25, 2311–2331, https://doi.org/10.5194/acp-25-2311-2025, https://doi.org/10.5194/acp-25-2311-2025, 2025
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This study derives a gridded dust emission dataset for 1841–2000 by employing a combination of observed dust from core records and reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to better match observations than other mechanistic models.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2087–2121, https://doi.org/10.5194/acp-25-2087-2025, https://doi.org/10.5194/acp-25-2087-2025, 2025
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We use the GEOS-Chem model to simulate aerosol distributions and properties over the western North Atlantic Ocean (WNAO) during the winter and summer deployments in 2020 of the NASA ACTIVATE mission. Model results are evaluated against aircraft, ground-based, and satellite observations. The improved understanding of life cycle, composition, transport pathways, and distribution of aerosols has important implications for characterizing aerosol–cloud–meteorology interactions over WNAO.
Mingrui Ma, Jiachen Cao, Dan Tong, Bo Zheng, and Yu Zhao
Atmos. Chem. Phys., 25, 2147–2166, https://doi.org/10.5194/acp-25-2147-2025, https://doi.org/10.5194/acp-25-2147-2025, 2025
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We combined two global climate change pathways and three national emission control scenarios to analyze the future evolution of reactive nitrogen (Nr) deposition till the 2060s in China with air quality modeling. We show China’s clean air and carbon neutrality policies would overcome the adverse effects of climate change and efficiently reduce Nr deposition. The outflow of Nr fluxes from mainland China to the west Pacific would also be clearly reduced from continuous stringent emission controls.
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025, https://doi.org/10.5194/acp-25-1869-2025, 2025
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Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of the BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with a characteristic time of less than 1 d. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Shuangqin Yang, Yusi Liu, Li Chen, Nan Cao, Jing Wang, and Shuang Gao
EGUsphere, https://doi.org/10.5194/egusphere-2024-3705, https://doi.org/10.5194/egusphere-2024-3705, 2025
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Black carbon, primary brown carbon, and secondary brown carbon are the leading light-absorbing carbonaceous aerosols (LACs) that contribute significantly to climate change. We modified the GEOS-Chem model to simulate the climate change by LACs based on local emission inventory, and explored the impacts of LACs properties and atmospheric variables on the corresponding DRFs in seven regions of China. The study confirms the warming effect of LACs and deepens our knowledge of their climatic effects.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
Atmos. Chem. Phys., 25, 1711–1724, https://doi.org/10.5194/acp-25-1711-2025, https://doi.org/10.5194/acp-25-1711-2025, 2025
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Dust days during the spring seasons of 2015–2023 in North China were classified into Mongolian cyclone and cold high types depending on the presence of the Mongolian cyclone. The Mongolian cyclone type led to more frequent and severe dust weather, indicated by PM10 concentrations. To comprehensively forecast the two types of dust weather, a common predictor was established based on 500 hPa anomalous circulation systems, offering insights for dust weather forecasting and climate prediction.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Yongqing Bai, Tianliang Zhao, Kai Meng, Yue Zhou, Jie Xiong, Xiaoyun Sun, Lijuan Shen, Yanyu Yue, Yan Zhu, Weiyang Hu, and Jingyan Yao
Atmos. Chem. Phys., 25, 1273–1287, https://doi.org/10.5194/acp-25-1273-2025, https://doi.org/10.5194/acp-25-1273-2025, 2025
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We proposed a composite statistical method to identify the quasi-weekly oscillation (QWO) of regional PM2.5 transport over China in winter from 2015 to 2019. The QWO of regional PM2.5 transport is constrained by synoptic-scale disturbances of the East Asian winter monsoon circulation with the periodic activities of the Siberian high, providing a new insight into the understanding of regional pollutant transport with meteorological drivers in atmospheric environment changes.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
Atmos. Chem. Phys., 25, 997–1021, https://doi.org/10.5194/acp-25-997-2025, https://doi.org/10.5194/acp-25-997-2025, 2025
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Solar energy production in West Africa is set to rise and needs accurate solar radiation estimates which are affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cuts errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Zining Yang, Qiuyan Du, Qike Yang, Chun Zhao, Gudongze Li, Zihan Xia, Mingyue Xu, Renmin Yuan, Yubin Li, Kaihui Xia, Jun Gu, and Jiawang Feng
EGUsphere, https://doi.org/10.5194/egusphere-2024-3890, https://doi.org/10.5194/egusphere-2024-3890, 2025
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This study investigates the impact of turbulent mixing on black carbon (BC) concentrations in urban areas using WRF-Chem at 25, 5, and 1 km resolutions. Significant variations in BC and turbulent mixing occur mainly at night. Higher resolutions reduce BC overestimation due to enhanced PBL mixing coefficients and vertical wind fluxes. Small-scale eddies at higher resolutions increase BC lifetime and column concentrations. Land use and terrain variations across multi-resolutions affect PBL mixing.
Ari Laaksonen, Golnaz Roudsari, Ana A. Piedehierro, and André Welti
EGUsphere, https://doi.org/10.5194/egusphere-2024-4095, https://doi.org/10.5194/egusphere-2024-4095, 2025
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The mechanisms of ice nucleation at temperatures below 235 K have remained unclear for the past century. We suggest that ice nucleation is caused by the freezing of water adsorbed on aerosol surfaces. To test this hypothesis, we derived theoretical equations to predict the exact atmospheric conditions under which ice nucleation occurs. Our predictions agree well with experiments. The new theory thus provides a basis for an improved description of ice nucleation in the atmosphere.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025, https://doi.org/10.5194/acp-25-327-2025, 2025
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Xinyue Huang, Wenyu Gao, and Hosein Foroutan
EGUsphere, https://doi.org/10.5194/egusphere-2024-3076, https://doi.org/10.5194/egusphere-2024-3076, 2024
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This study investigates the relationship between wind-blown dust aerosols size distribution and wind conditions over topography at a regional scale, utilizing 10 years of dust reanalysis data. Linear regression models suggest that higher wind speeds and steeper land slopes, particularly under uphill winds, are associated with increased fractions of coarser dust particles. Moreover, these positive correlations weaken during summer and afternoon events, likely related to the haboob storms.
Lulu Yuan, Wenchao Han, Jiachen Meng, Yang Wang, Haojie Yu, and Wenze Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-3350, https://doi.org/10.5194/egusphere-2024-3350, 2024
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This study utilizes multi-source data to reveal the impact of various urban functional zones in China on the spatial distribution of pollutants. The findings indicate that the residential and commercial zones see notable air quality gains, but the improvement of air quality in the transportation zone is the least considerable. Moreover, the industrial zone has the most seasonal air quality variation. Therefore, air pollution prevention policies should consider differences in functional zones.
Carl Svenhag, Pontus Roldin, Tinja Olenius, Robin Wollesen de Jonge, Sara Blichner, Daniel Yazgi, and Moa Sporre
EGUsphere, https://doi.org/10.5194/egusphere-2024-3626, https://doi.org/10.5194/egusphere-2024-3626, 2024
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This study investigates the model representation of how particles are formed and grow in the atmosphere. Using modeled and observed data from two boreal forest stations in 2018, we identify key factors for NPF to improve particle-climate predictions in the global EC-Earth3 model. Comparisons with the detailed ADCHEM model show that adding ammonia improves particle growth predictions, though EC-Earth3 still highly underestimates the number of particles during warmer months.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
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A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
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Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
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In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
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Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Thomas Drugé, Pierre Nabat, Martine Michou, and Marc Mallet
EGUsphere, https://doi.org/10.5194/egusphere-2024-3659, https://doi.org/10.5194/egusphere-2024-3659, 2024
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Aerosol scattering in long-wave radiation is often neglected in climate models. In this study, we analyze its impact through a physical modeling of this process in the CNRM ARPEGE-Climat model. It mainly leads to surface LW radiation increases across Sahara, Sahel and Arabian Peninsula, resulting in daily minimum near-surface temperature rises. Other changes in atmospheric fields are also simulated.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Bishuo He and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-3441, https://doi.org/10.5194/egusphere-2024-3441, 2024
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Factor-uncertainty analysis helps us understand their impacts on complex systems. Traditional methods have many limitations. This study introduces a new method to measure how each factor contributes to uncertainty. It gains insights into the role of each variable and works for all multi-factor systems. As an application, we analyzed how aerosols affect solar radiation and identified the key factors. These analyses can improve our understanding of the role of aerosols in climate change.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Catherine Anne Toolan, Joe Adabouk Amooli, Laura J. Wilcox, Bjørn H. Samset, Andrew G. Turner, and Daniel M. Westervelt
EGUsphere, https://doi.org/10.5194/egusphere-2024-3057, https://doi.org/10.5194/egusphere-2024-3057, 2024
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Our research explores how well air pollution and rainfall patterns in Africa are represented in current climate models, by comparing model data to observations from 1981 to 2023. While most models capture seasonal air quality changes well, they struggle to replicate the distribution of non-dust pollutants and certain rainfall patterns, especially over east Africa. Improving these models is crucial for better climate predictions and preparing for future risks.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Cited articles
Alfaro, S. C. and Gomes, L.: Modeling mineral aerosol production by wind erosion: emission intensities and aerosol size distribution in source areas, J. Geophys. Res., 106, 18075–18084, 2001.
Angevine, W. M., Jiang, H., and Mauritsen, T.: Performance of an eddy diffusivity-mass flux scheme for shallow cumulus boundary layers, Mon. Weather Rev., 138, 2895–2912, 2010.
Ayotte, K. W., Sullivan, P. P., Andrén, A., Doney, S. C., Holtslag, A. A., Large, W. G., McWilliams, J. C., Moeng, C.-N., Otte, M. J., Tribbia, J. J., and Wyngaard, J. C.: An evaluation of neutral and convective planetary boundary-layer parameterizations relative to large eddy simulations, Bound.-Lay. Meteorol., 79, 131–175, 1996.
Bain, C. L., Parker, D. J., Taylor, C. M., Kergoat, L., and Guichard, F.: Observations of the Nocturnal Boundary Layer Associated with the West African Monsoon, Mon. Weather Rev., 138, 3142–3156, https://doi.org/10.1175/2010MWR3287.1, 2010.
Beljaars, A. C. M. and Viterbo, P.: The sensitivity of winter evaporation to the formulation of aerodynamic resistance in the ECMWF model, Bound.-Lay. Meteorol., 71, 135–149, https://doi.org/10.1007/BF00709223, 1994.
Cakmur, R. V., Miller, R. L., and Torres, O.: Incorporating the effect of small-scale circulations upon dust emission in an atmospheric general circulation model, J. Geophys. Res., 109, D07201, https://doi.org/10.1029/2003JD004067, 2004.
Callot, Y., Marticorena, B., and Bergametti, G.: Geomorphologic approach for modelling the surface features of arid environments in a model of dust emissions: application to the Sahara desert, Geodin. Acta., 13, 245–270, https://doi.org/10.1016/S0985-3111(00)01044-5, 2000.
Chatfield, R. B. and Brost, R. A.: A two-stream model of the vertical transport of trace species in the convective boundary layer, J. Geophys. Res., 92, 13263–13276, 1987.
Coindreau, O., Hourdin, F., Haeffelin, M., Mathieu, A., and Rio, C.: A global climate model with strechable grid and nudging: a tool for assesment of physical parametrizations, Mon. Weather Rev., 135, 1474–1489, 2007.
Cuesta, J., Marsham, J. H., Parker, D. J., and Flamant, C.: Dynamical mechanisms controlling the vertical redistribution of dust and the thermodynamic structure of the West Saharan atmospheric boundary layer during summer, Atmos. Sci. Lett., 10, 34–42, https://doi.org/10.1002/asl.207, 2009.
Deardorff, J. W.: Preliminary results from numerical integrations of the unstable planetary boundary layer, J. Atmos. Sci., 27, 1209–1211, 1970.
Deardorff, J. W.: Theoretical expression for the countergradient vertical heat flux, J. Geophys. Res., 77, 5900–5904, 1972.
Dufresne, J.-L., Foujols, M.-A., Denvil, S., Caubel, A., Marti, O., Aumont, O., Balkanski, Y., Bekki, S., Bellenger, H., Benshila, R., Bony, S., Bopp, L., Braconnot, P., Brockmann, P., Cadule, P., Cheruy, F., Codron, F., Cozic, A., Cugnet, D., de Noblet, N., Duvel, J.-P., Ethé, C., Fairhead, L., Fichefet, T., Flavoni, S., Friedlingstein, P., Grandpeix, J.-Y., Guez, L., Guilyardi, E., Hauglustaine, D., Hourdin, F., Idelkadi, A., Ghattas, J., Joussaume, S., Kageyama, M., Krinner, G., Labetoulle, S., Lahellec, A., Lefebvre, M.-P., Lefevre, F., Levy, C., Li, Z. X., Lloyd, J., Lott, F., Madec, G., Mancip, M., Marchand, M., Masson, S., Meurdesoif, Y., Mignot, J., Musat, I., Parouty, S., Polcher, J., Rio, C., Schulz, M., Swingedouw, D., Szopa, S., Talandier, C., Terray, P., Viovy, N., and Vuichard, N.: Climate change projections using the IPSL-CM5 Earth System Model: from CMIP3 to CMIP5, Clim. Dynam., 40, 2123–2165, https://doi.org/10.1007/s00382-012-1636-1, 2013.
Engelstaedter, S., Tegen, I., and Washington, R.: North African dust emissions and transport, Earth-Sci. Rev., 79, 73–100, https://doi.org/10.1016/j.earscirev.2006.06.004, 2006.
Fiedler, S., Schepanski, K., Heinold, B., Knippertz, P., and Tegen, I.: Climatology of nocturnal low-level jets over North Africa and implications for modeling mineral dust emission, J. Geophys. Res., 118, 6100–6121, https://doi.org/10.1002/jgrd.50394, 2013.
Forêt, G., Bergametti, G., Dulac, F., and Menut, L.: An optimized particle size bin scheme for modeling mineral dust aerosol, J. Geophys. Res., 111, D17310, https://doi.org/10.1029/2005JD006797, 2006.
Gillette, D. A.: Fine Particulate emissions due to wind erosion, Trans. Am. Soc. Agric. Engrs., 20, 890–987, 2003.
Gounou, A., Guichard, F., and Couvreux, F.: Observations of diurnal cycles over a West African meridional transect: pre-monsoon and full-monsoon seasons, Bound.-Lay. Meteorol., 144, 329–357, https://doi.org/10.1007/s10546-012-9723-8, 2012.
Gomes, L., Rajot, J. L., Alfaro, S. C., and Gaudichet, A.: Validation of a dust production model from measurements performed in semi-arid agricultural areas of Spain and Niger, Catena, 52, 257–271, https://doi.org/10.1016/S0341-8162(03)00017-1, 2003.
Grandpeix, J. and Lafore, J.: A density current parameterization coupled with Emanuel's convection scheme, Part I: The models, J. Atmos. Sci., 67, 881–897, https://doi.org/10.1175/2009JAS3044.1, 2010.
Guichard, F., Kergoat, L., Mougin, E., Timouk, F., Baup, F., Hiernaux, P., and Lavenu, F.: Surface thermodynamics and radiative budget in the Sahelian Gourma: Seasonal and diurnal cycles, J. Hydrol., 375, 161–177, https://doi.org/10.1016/j.jhydrol.2008.09.007, 2009.
Holben, B. N., Tanre, D., Smirnov, A., Eck, T. F., Slutsker, I., Abuhassan, N., Newcomb, W. W., Schafer, J., Chatenet, B., Lavenu, F., Kaufman, Y., Van de Castle, J., Setzer, A., Markham, B., Clark, D., Frouin, R., Halthore, R., Karnieli, A., O'Neill, N. T., Pietras, C., Pinker, R. T., Voss, K., and Zibordi, G.: An emerging ground-based aerosol climatology: Aerosol Optical Depth from AERONET, J. Geophys. Res., 106, 12067–12098, 2001.
Holtslag, A. A. M. and Boville, B. A.: Local versus non-local boundary-layer diffusion in a global climate model, J. Climate, 6, 1825–1842, 1993.
Hourdin, F., Couvreux, F., and Menut, L.: Parameterisation of the dry convective boundary layer based on a mass flux representation of thermals, J. Atmos. Sci., 59, 1105–1123, 2002.
Hourdin, F., Foujols, M.-A., Codron, F., Guemas, V., Dufresne, J.-L., Bony, S., Denvil, S., Guez, L., Lott, F., Ghattas, J., Braconnot, P., Marti, O., Meurdesoif, Y., and Bopp, L.: Impact of the LMDZ atmospheric grid configuration on the climate and sensitivity of the IPSL-CM5A coupled model, Clim. Dynam., 40, 2167–2192, https://doi.org/10.1007/s00382-012-1411-3, 2013a.
Hourdin, F., Grandpeix, J.-Y., Rio, C., Bony, S., Jam, A., Cheruy, F., Rochetin, N., Fairhead, L., Idelkadi, A., Musat, I., Dufresne, J.-L., Lahellec, A., Lefebvre, M.-P., and Roehrig, R.: LMDZ5B: the atmospheric component of the IPSL climate model with revisited parameterizations for clouds and convection, Clim. Dynam., 40, 2193–2222, https://doi.org/10.1007/s00382-012-1343-y, 2013b.
Jam, A., Hourdin, F., Rio, C., and Couvreux, F.: Resolved versus parametrized boundary-layer plumes, Part III: Derivation of a statistical scheme for cumulus clouds, Bound.-Lay. Meteorol., 147, 421–441, https://doi.org/10.1007/s10546-012-9789-3, 2013.
Knippertz, P. and Todd, M. C.: Mineral dust aerosols over the Sahara: meteorological controls on emission and transport and implications for modeling, Rev. Geophys., 50, RG1007, https://doi.org/10.1029/2011RG000362, 2012.
Laurent, B., Marticorena, B., Bergametti, G., Léon, J. F., and Mahowald, N. M.: Modeling mineral dust emissions from the Sahara desert using new surface properties and soil database, J. Geophys. Res., 113, D14218, https://doi.org/10.1029/2007JD009484, 2008.
Largeron, Y., Guichard, F., Bouniol, D., Couvreux, F., Kergoat, L., and Marticorena, B.: Can we use surface wind fields from meteorological reanalyses for Sahelian dust emission simulations?, Geophys. Res. Lett., 42, 2490–2499, https://doi.org/10.1002/2014GL062938, 2015.
Lothon, M., Saïd, F., Lohou, F., and Campistron, B.: Observation of the diurnal cycle in the low troposphere of West Africa, Mon. Weather Rev., 136, 3477, https://doi.org/10.1175/2008MWR2427.1, 2008.
Marticorena, B. and Bergametti, G.: Modeling the atmospheric dust cycle: 1 Design of a soil derived dust production scheme, J. Geophys. Res., 100, 16415–16430, 1995a.
Marticorena, B. and Bergametti, G.: Modeling the atmospheric dust cycle: design of a soil-derived emission scheme, J. Geophys. Res., 102, 16415–16430, 1995b.
Marticorena, B., Bergametti, G., Aumont, B., Callot, Y., N'doumé, C., and Legrand, M.: Modeling the atmospheric dust cycle: 2. Simulation of Saharan dust sources, J. Geophys. Res., 102, 4387–4404, https://doi.org/10.1029/96JD02964, 1997.
Marticorena, B., Chatenet, B., Rajot, J. L., Traoré, S., Coulibaly, M., Diallo, A., Koné, I., Maman, A., NDiaye, T., and Zakou, A.: Temporal variability of mineral dust concentrations over West Africa: analyses of a pluriannual monitoring from the AMMA Sahelian Dust Transect, Atmos. Chem. Phys., 10, 8899–8915, https://doi.org/10.5194/acp-10-8899-2010, 2010.
Menut, L., Schmechtig, C., and Marticorena, B.: Sensitivity of the sandblasting fluxes calculations to the soil size distribution accuracy, J. Atmos. Ocean. Tech., 22, 1875–1884, 2005.
Menut, L., Foret, G., and Bergametti, G.: Sensitivity of mineral dust concentrations to the model size distribution accuracy, J. Geophys. Res.-Atmos., 112, D10210, https://doi.org/10.1029/2006JD007766, 2007.
Menut, L., Chiapello, I., and Moulin, C.: Previsibility of mineral dust concentrations: the CHIMERE-DUST forecast during the first AMMA experiment dry season, J. Geophys. Res., 114, D07202, https://doi.org/10.1029/2008JD010523, 2009.
Menut, L., Bessagnet, B., Khvorostyanov, D., Beekmann, M., Blond, N., Colette, A., Coll, I., Curci, G., Foret, G., Hodzic, A., Mailler, S., Meleux, F., Monge, J.-L., Pison, I., Siour, G., Turquety, S., Valari, M., Vautard, R., and Vivanco, M. G.: CHIMERE 2013: a model for regional atmospheric composition modelling, Geosci. Model Dev., 6, 981–1028, https://doi.org/10.5194/gmd-6-981-2013, 2013.
Moulin, C., Gordon, H. R., Banzon, V. F., and Evans, R. H.: Assessment of Saharan dust absorption in the visible from SeaWiFS imagery, J. Geophys. Res., 106, 18239, https://doi.org/10.1029/2000JD900812, 2001.
Neggers, R. A. J.: A dual mass flux framework for boundary layer convection, Part II: Clouds, J. Atmos. Sci., 66, 1489–1506, 2009.
Neggers, R. A. J., Köhler, M., and Beljaars, A. C. M.: A dual mass flux framework for boundary layer convection. Part I: Transport, J. Atmos. Sci., 66, 1465, https://doi.org/10.1175/2008JAS2635.1, 2009.
Nickling, W. G. and Gillies, J. A.: Emission of fine-grained particulates from desert soils, in Paleoclimatology and Paleometeorology: Modern and Past Patterns of Global Atmospheric Transport, edited by: Leinen, M. and Sarnthein, M., Kluwer Academic Publ., Dordrecht, 133–165, 1989.
Nickling, W. G. and Gillies, J. A.: Dust emission and transport in Mali, West Africa, Sedimentology, 40, 859–868, 1993.
Parker, D. J., Burton, R. R., Diongue-Niang, A., Ellis, R. J., Felton, M., Taylor, C. M., Thorncroft, C. D., Bessemoulin, P., and Tompkins, A. M.: The diurnal cycle of the West African monsoon circulation, Q. J. Roy. Meteor. Soc., 131, 2839–2860, https://doi.org/10.1256/qj.04.52, 2005.
Pergaud, J., Masson, V., Malardel, S., and Couvreux, F.: A parameterization of dry thermals and shallow cumuli for mesoscale numerical weather prediction, Bound.-Lay. Meteorol., 132, 83–106, https://doi.org/10.1007/s10546-009-9388-0, 2009.
Rajot, J. L., Alfaro, S. C., Gomes, L., and Gaudichet, A.: Soil crusting on sandy soils and its influence on wind erosion, Catena, 53, 1–16, 2003.
Redelsperger, J.-L., Thorncroft, C. D., Diedhiou, A., Lebel, T., Parker, D. J., and Polcher, J.: African monsoon multidisciplinary analysis: an international research project and field campaign, B. Am. Meteorol. Soc., 87, 1739–1746, https://doi.org/10.1175/BAMS-87-12-1739, 2006.
Rio, C. and Hourdin, F.: A thermal plume model for the convective boundary layer: representation of cumulus clouds, J. Atmos. Sci., 65, 407–425, 2008.
Rio, C., Hourdin, F., Grandpeix, J., and Lafore, J.: Shifting the diurnal cycle of parameterized deep convection over land, Geophys. Res. Lett., 36, L07809, https://doi.org/10.1029/2008GL036779, 2009.
Rio, C., Hourdin, F., Couvreux, F., and Jam, A.: Resolved versus parametrized boundary-layer plumes, Part II: Continuous formulations of mixing rates for mass-flux schemes, Bound.-Lay. Meteorol., 135, 469–483, https://doi.org/10.1007/s10546-010-9478-z, 2010.
Schepanski, K., Tegen, I., Todd, M. C., Heinold, B., BöNisch, G., Laurent, B., and Macke, A.: Meteorological processes forcing Saharan dust emission inferred from MSG-SEVIRI observations of subdaily dust source activation and numerical models, J. Geophys. Res.-Atmos., 114, D10201, https://doi.org/10.1029/2008JD010325, 2009.
Schmechtig, C., Marticorena, B., Chatenet, B., Bergametti, G., Rajot, J. L., and Coman, A.: Simulation of the mineral dust content over Western Africa from the event to the annual scale with the CHIMERE-DUST model, Atmos. Chem. Phys., 11, 7185–7207, https://doi.org/10.5194/acp-11-7185-2011, 2011.
Seinfeld, J. H. and Pandis, S. N. (Eds.): Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, in: Atmospheric chemistry and physics: from air pollution to climate change, New York, NY: Wiley, 1998 Physical description: xxvii, 1326 pp., Wiley-Interscience Publication, ISBN: 0471178152, 1998.
Shao, Y. and Lu, I.: A simple expression for wind erosion threshold friction velocity, J. Geophys. Res., 105, 22437–22443, 2000.
Shao, Y., Ishizuka, M., Mikami, M., and Leys, J. F.: Parameterization of size-resolved dust emission and validation with measurements, J. Geophys. Res., 116, D08203, https://doi.org/10.1029/2010JD014527, 2011.
Siebesma, A. P., Soares, P. M. M., and Teixeira, J.: A combined eddy-diffusivity mass-flux approach for the convective boundary layer, J. Atmos. Sci., 64, 1230, https://doi.org/10.1175/JAS3888.1, 2007.
Slingo, A., Ackerman, T. P., Allan, R. P., Kassianov, E. I., McFarlane, S. A., Robinson, G. J., Barnard, J. C., Miller, M. A., Harries, J. E., Russell, J. E., and Dewitte, S.: Observations of the impact of a major Saharan dust storm on the atmospheric radiation balance, Geophys. Res. Lett., 33, L24817, https://doi.org/10.1029/2006GL027869, 2006.
Soares, P. M. M., Miranda, P. M. A., Siebesma, A. P., and Teixeira, J.: An eddy-diffusivity/mass-flux parametrization for dry and shallow cumulus convection, Q. J. Roy. Meteor. Soc., 130, 3365–3383, 2004.
Solmon, F., Mallet, M., Elguindi, N., Giorgi, F., Zakey, A., and Konaré, A.: Dust aerosol impact on regional precipitation over western Africa, mechanisms and sensitivity to absorption properties, Geophys. Res. Lett., 35, L24705, https://doi.org/10.1029/2008GL035900, 2008.
Sow, M., Alfaro, S. C., Rajot, J. L., and Marticorena, B.: Size resolved dust emission fluxes measured in Niger during 3 dust storms of the AMMA experiment, Atmos. Chem. Phys., 9, 3881–3891, https://doi.org/10.5194/acp-9-3881-2009, 2009.
Spyrou, C., Kallos, G., Mitsakou, C., Athanasiadis, P., Kalogeri, C., and Iacono, M. J.: Modeling the radiative effects of desert dust on weather and regional climate, Atmos. Chem. Phys., 13, 5489–5504, https://doi.org/10.5194/acp-13-5489-2013, 2013.
Stull, R. B.: Transilient turbulence theory, Part I: The concept of eddy-mixing across finite distances, J. Atmos. Sci., 41, 3351–3367, 1984.
Taylor, K. E., Stouffer, R. J., and Meehl, G. A.: An overview of CMIP5 and the experiment design, B. Am. Meteorol. Soc., 93, 485–498, https://doi.org/10.1175/BAMS-D-11-00094.1, 2012.
Tegen, I., Schepanski, K., and Heinold, B.: Comparing two years of Saharan dust source activation obtained by regional modelling and satellite observations, Atmos. Chem. Phys., 13, 2381–2390, https://doi.org/10.5194/acp-13-2381-2013, 2013.
Tiedtke, M.: A comprehensive mass flux scheme for cumulus parameterization in large-scale models, Mon. Weather Rev., 117, 1179–1800, 1989.
Todd, M. C., Bou Karam, D., Cavazos, C., Bouet, C., Heinold, B., Baldasano, J. M., Cautenet, G., Koren, I., Perez, C., Solmon, F., Tegen, I., Tulet, P., Washington, R., and Zakey, A.: Quantifying uncertainty in estimates of mineral dust flux: an intercomparison of model performance over the Bodélé Depression, northern Chad, J. Geophys. Res.-Atmos., 113, D24107, https://doi.org/10.1029/2008JD010476, 2008.
Troen, I. and Mahrt, L.: A simple model of the atmospheric boundary layer: sensitivity to surface evaporation, Bound.-Lay. Meteorol., 37, 129–148, 1986.
Yamada, T.: Simulations of nocturnal drainage flows by a q2l turbulence closure model, J. Atmos. Sci., 40, 91–106, 1983.
Yoshioka, M., Mahowald, N. M., Conley, A. J., Collins, W. D., Fillmore, D. W., Zender, C. S., and Coleman, D. B.: Impact of desert dust radiative forcing on sahel precipitation: relative importance of dust compared to sea surface temperature variations, vegetation changes, and greenhouse gas warming, J. Climate, 20, 1445, https://doi.org/10.1175/JCLI4056.1, 2007.
Short summary
New parameterizations of the convective boundary layer are used to better represent the diurnal cycle of near-surface wind over Sahara and Sahel in a climate model and the associated emission of dust.
New parameterizations of the convective boundary layer are used to better represent the diurnal...
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