Articles | Volume 24, issue 10
https://doi.org/10.5194/acp-24-6047-2024
https://doi.org/10.5194/acp-24-6047-2024
Research article
 | 
27 May 2024
Research article |  | 27 May 2024

Combined assimilation of NOAA surface and MIPAS satellite observations to constrain the global budget of carbonyl sulfide

Jin Ma, Linda M. J. Kooijmans, Norbert Glatthor, Stephen A. Montzka, Marc von Hobe, Thomas Röckmann, and Maarten C. Krol

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Subject: Gases | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Cited articles

Abadie, C., Maignan, F., Remaud, M., Ogée, J., Campbell, J. E., Whelan, M. E., Kitz, F., Spielmann, F. M., Wohlfahrt, G., Wehr, R., Sun, W., Raoult, N., Seibt, U., Hauglustaine, D., Lennartz, S. T., Belviso, S., Montagne, D., and Peylin, P.: Global modelling of soil carbonyl sulfide exchanges, Biogeosciences, 19, 2427–2463, https://doi.org/10.5194/bg-19-2427-2022, 2022. a, b
Baartman, S. L., Krol, M. C., Röckmann, T., Hattori, S., Kamezaki, K., Yoshida, N., and Popa, M. E.: A GC-IRMS method for measuring sulfur isotope ratios of carbonyl sulfide from small air samples, Open Research Europe, 1, 105, https://doi.org/10.12688/openreseurope.13875.2, 2021. a
Barkley, M. P., Palmer, P. I., Boone, C. D., Bernath, P. F., and Suntharalingam, P.: Global distributions of carbonyl sulfide in the upper troposphere and stratosphere, Geophys. Res. Lett., 35, L14810, https://doi.org/10.1029/2008GL034270, 2008. a
Barnes, I., Becker, K. H., and Patroescu, I.: The tropospheric oxidation of DMS: A new source of OCS, Geophys. Res. Lett., 21, 2389–2392, https://doi.org/10.1029/94GL02499, 1994. a, b
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The global budget of atmospheric COS can be optimised by inverse modelling using TM5-4DVAR, with the co-constraints of NOAA surface observations and MIPAS satellite data. We found reduced COS biosphere uptake from inversions and improved land and ocean separation using MIPAS satellite data assimilation. Further improvements are expected from better quantification of COS ocean and biosphere fluxes.
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