Articles | Volume 23, issue 9
https://doi.org/10.5194/acp-23-5517-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-5517-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report: Rapid decline of aerosol absorption coefficient and aerosol optical property effects on radiative forcing in an urban area of Beijing from 2018 to 2021
Xinyao Hu
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Junying Sun
CORRESPONDING AUTHOR
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
State Key Laboratory of Cryospheric Science, Northwest Institute of
Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000,
China
Can Xia
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
School of Atmospheric Physics, Nanjing University of Information Science and Technology, Nanjing 210044, China
Xiaojing Shen
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Yangmei Zhang
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Zhaodong Liu
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
School of Atmospheric Physics, Nanjing University of Information Science and Technology, Nanjing 210044, China
Sinan Zhang
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Jialing Wang
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Aoyuan Yu
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Jiayuan Lu
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Shuo Liu
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Xiaoye Zhang
State Key Laboratory of Severe Weather and Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
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Preprint archived
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Chupeng Zhang, Shangfei Hai, Yang Gao, Yuhang Wang, Shaoqing Zhang, Lifang Sheng, Bin Zhao, Shuxiao Wang, Jingkun Jiang, Xin Huang, Xiaojing Shen, Junying Sun, Aura Lupascu, Manish Shrivastava, Jerome D. Fast, Wenxuan Cheng, Xiuwen Guo, Ming Chu, Nan Ma, Juan Hong, Qiaoqiao Wang, Xiaohong Yao, and Huiwang Gao
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Xiaojing Shen, Junying Sun, Huizheng Che, Yangmei Zhang, Chunhong Zhou, Ke Gui, Wanyun Xu, Quan Liu, Junting Zhong, Can Xia, Xinyao Hu, Sinan Zhang, Jialing Wang, Shuo Liu, Jiayuan Lu, Aoyuan Yu, and Xiaoye Zhang
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Yifang Gu, Ru-Jin Huang, Jing Duan, Wei Xu, Chunshui Lin, Haobin Zhong, Ying Wang, Haiyan Ni, Quan Liu, Ruiguang Xu, Litao Wang, and Yong Jie Li
Atmos. Chem. Phys., 23, 5419–5433, https://doi.org/10.5194/acp-23-5419-2023, https://doi.org/10.5194/acp-23-5419-2023, 2023
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Yingfang Li, Zhili Wang, Yadong Lei, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 2499–2523, https://doi.org/10.5194/acp-23-2499-2023, https://doi.org/10.5194/acp-23-2499-2023, 2023
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Wenjie Zhang, Hong Wang, Xiaoye Zhang, Liping Huang, Yue Peng, Zhaodong Liu, Xiao Zhang, and Huizheng Che
Atmos. Chem. Phys., 22, 15207–15221, https://doi.org/10.5194/acp-22-15207-2022, https://doi.org/10.5194/acp-22-15207-2022, 2022
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Mengying Li, Shaocai Yu, Xue Chen, Zhen Li, Yibo Zhang, Zhe Song, Weiping Liu, Pengfei Li, Xiaoye Zhang, Meigen Zhang, Yele Sun, Zirui Liu, Caiping Sun, Jingkun Jiang, Shuxiao Wang, Benjamin N. Murphy, Kiran Alapaty, Rohit Mathur, Daniel Rosenfeld, and John H. Seinfeld
Atmos. Chem. Phys., 22, 11845–11866, https://doi.org/10.5194/acp-22-11845-2022, https://doi.org/10.5194/acp-22-11845-2022, 2022
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This study constructed an emission inventory of condensable particulate matter (CPM) in China with a focus on organic aerosols (OAs), based on collected CPM emission information. The results show that OA emissions are enhanced twofold for the years 2014 and 2017 after the inclusion of CPM in the new inventory. Sensitivity cases demonstrated the significant contributions of CPM emissions from stationary combustion and mobile sources to primary, secondary, and total OA concentrations.
Jing Duan, Ru-Jin Huang, Yifang Gu, Chunshui Lin, Haobin Zhong, Wei Xu, Quan Liu, Yan You, Jurgita Ovadnevaite, Darius Ceburnis, Thorsten Hoffmann, and Colin O'Dowd
Atmos. Chem. Phys., 22, 10139–10153, https://doi.org/10.5194/acp-22-10139-2022, https://doi.org/10.5194/acp-22-10139-2022, 2022
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Lei Li, Yevgeny Derimian, Cheng Chen, Xindan Zhang, Huizheng Che, Gregory L. Schuster, David Fuertes, Pavel Litvinov, Tatyana Lapyonok, Anton Lopatin, Christian Matar, Fabrice Ducos, Yana Karol, Benjamin Torres, Ke Gui, Yu Zheng, Yuanxin Liang, Yadong Lei, Jibiao Zhu, Lei Zhang, Junting Zhong, Xiaoye Zhang, and Oleg Dubovik
Earth Syst. Sci. Data, 14, 3439–3469, https://doi.org/10.5194/essd-14-3439-2022, https://doi.org/10.5194/essd-14-3439-2022, 2022
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A climatology of aerosol composition concentration derived from POLDER-3 observations using GRASP/Component is presented. The conceptual specifics of the GRASP/Component approach are in the direct retrieval of aerosol speciation without intermediate retrievals of aerosol optical characteristics. The dataset of satellite-derived components represents scarce but imperative information for validation and potential adjustment of chemical transport models.
Junting Zhong, Xiaoye Zhang, Ke Gui, Jie Liao, Ye Fei, Lipeng Jiang, Lifeng Guo, Liangke Liu, Huizheng Che, Yaqiang Wang, Deying Wang, and Zijiang Zhou
Earth Syst. Sci. Data, 14, 3197–3211, https://doi.org/10.5194/essd-14-3197-2022, https://doi.org/10.5194/essd-14-3197-2022, 2022
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Historical long-term PM2.5 records with high temporal resolution are essential but lacking for research and environmental management. Here, we reconstruct site-based and gridded PM2.5 datasets at 6-hour intervals from 1960 to 2020 that combine visibility, meteorological data, and emissions based on a machine learning model with extracted spatial features. These two PM2.5 datasets will lay the foundation of research studies associated with air pollution, climate change, and aerosol reanalysis.
Haochi Che, Michal Segal-Rozenhaimer, Lu Zhang, Caroline Dang, Paquita Zuidema, Arthur J. Sedlacek III, Xiaoye Zhang, and Connor Flynn
Atmos. Chem. Phys., 22, 8767–8785, https://doi.org/10.5194/acp-22-8767-2022, https://doi.org/10.5194/acp-22-8767-2022, 2022
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A 17-month in situ study on Ascension Island found low single-scattering albedo and strong absorption enhancement of the marine boundary layer aerosols during biomass burnings on the African continent, along with apparent patterns of regular monthly variability. We further discuss the characteristics and drivers behind these changes and find that biomass burning conditions in Africa may be the main factor influencing the optical properties of marine boundary aerosols.
Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhong, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, Shichang Kang, and Jianzhong Xu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-211, https://doi.org/10.5194/essd-2022-211, 2022
Manuscript not accepted for further review
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A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple short-term intensive field observations. The real-time online high-time-resolution (hourly) data of aerosol properties in the different TP region are integrated in a new dataset and can provide supporting for related studies in in the TP.
Ke Gui, Wenrui Yao, Huizheng Che, Linchang An, Yu Zheng, Lei Li, Hujia Zhao, Lei Zhang, Junting Zhong, Yaqiang Wang, and Xiaoye Zhang
Atmos. Chem. Phys., 22, 7905–7932, https://doi.org/10.5194/acp-22-7905-2022, https://doi.org/10.5194/acp-22-7905-2022, 2022
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This study investigates the aerosol optical and radiative properties and meteorological drivers during two mega SDS events over Northern China in March 2021. The MODIS-retrieved DOD data registered these two events as the most intense episode in the same period in history over the past 20 years. These two extreme SDS events were associated with both atmospheric circulation extremes and local meteorological anomalies that favor enhanced dust emissions in the Gobi Desert.
Siyuan Li, Dantong Liu, Shaofei Kong, Yangzhou Wu, Kang Hu, Huang Zheng, Yi Cheng, Shurui Zheng, Xiaotong Jiang, Shuo Ding, Dawei Hu, Quan Liu, Ping Tian, Delong Zhao, and Jiujiang Sheng
Atmos. Chem. Phys., 22, 6937–6951, https://doi.org/10.5194/acp-22-6937-2022, https://doi.org/10.5194/acp-22-6937-2022, 2022
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The understanding of secondary organic aerosols is hindered by the aerosol–gas evolution by different oxidation mechanisms. By concurrently measuring detailed mass spectra of aerosol and gas phases in a megacity online, we identified the primary and secondary source sectors and investigated the transformation between gas and aerosol phases influenced by photooxidation and moisture. The results will help us to understand the respective evolution of major sources in a typical urban environment.
Yu Zheng, Huizheng Che, Yupeng Wang, Xiangao Xia, Xiuqing Hu, Xiaochun Zhang, Jun Zhu, Jibiao Zhu, Hujia Zhao, Lei Li, Ke Gui, and Xiaoye Zhang
Atmos. Meas. Tech., 15, 2139–2158, https://doi.org/10.5194/amt-15-2139-2022, https://doi.org/10.5194/amt-15-2139-2022, 2022
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Ground-based observations of aerosols and aerosol data verification is important for satellite and climate model modification. Here we present an evaluation of aerosol microphysical, optical and radiative properties measured using a multiwavelength photometer with a highly integrated design and smart control performance. The validation of this product is discussed in detail using AERONET as a reference. This work contributes to reducing AOD uncertainties in China and combating climate change.
Clémence Rose, Martine Collaud Coen, Elisabeth Andrews, Yong Lin, Isaline Bossert, Cathrine Lund Myhre, Thomas Tuch, Alfred Wiedensohler, Markus Fiebig, Pasi Aalto, Andrés Alastuey, Elisabeth Alonso-Blanco, Marcos Andrade, Begoña Artíñano, Todor Arsov, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Juan Andrés Casquero-Vera, Sébastien Conil, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Maria I. Gini, Francisco Javier Gómez-Moreno, Martin Gysel-Beer, Anna Gannet Hallar, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Adam Kristensson, Markku Kulmala, Heikki Lihavainen, Neng-Huei Lin, Hassan Lyamani, Angela Marinoni, Sebastiao Martins Dos Santos, Olga L. Mayol-Bracero, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Jakub Ondracek, Marco Pandolfi, Noemi Pérez, Tuukka Petäjä, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Jean-Philippe Putaud, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Junying Sun, Pierre Tulet, Ville Vakkari, Pieter Gideon van Zyl, Fernando Velarde, Paolo Villani, Stergios Vratolis, Zdenek Wagner, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Vladimir Zdimal, and Paolo Laj
Atmos. Chem. Phys., 21, 17185–17223, https://doi.org/10.5194/acp-21-17185-2021, https://doi.org/10.5194/acp-21-17185-2021, 2021
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Aerosol particles are a complex component of the atmospheric system the effects of which are among the most uncertain in climate change projections. Using data collected at 62 stations, this study provides the most up-to-date picture of the spatial distribution of particle number concentration and size distribution worldwide, with the aim of contributing to better representation of aerosols and their interactions with clouds in models and, therefore, better evaluation of their impact on climate.
Wenxing Jia and Xiaoye Zhang
Atmos. Chem. Phys., 21, 16827–16841, https://doi.org/10.5194/acp-21-16827-2021, https://doi.org/10.5194/acp-21-16827-2021, 2021
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Heavy aerosol pollution incidents have attracted much attention since 2013, but the temporal and spatial limitations of observations and the inaccuracy of simulation are a stumbling block to assessing pollution mechanisms. The correct simulation of boundary layer mixing process of pollutant is a challenge for mesoscale numerical models. We add the turbulent diffusion term of aerosol to the WRF-Chem model to prove the impact of turbulent diffusion on pollutant concentration.
Ke Gui, Huizheng Che, Yu Zheng, Hujia Zhao, Wenrui Yao, Lei Li, Lei Zhang, Hong Wang, Yaqiang Wang, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 15309–15336, https://doi.org/10.5194/acp-21-15309-2021, https://doi.org/10.5194/acp-21-15309-2021, 2021
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This study utilized the globally gridded aerosol extinction data from CALIOP during 2007–2019 to investigate the 3D climatology, trends, and meteorological drivers of tropospheric type-dependent aerosols. Results revealed that the planetary boundary layer (PBL) and the free troposphere contribute 62.08 % and 37.92 %, respectively, of the global tropospheric TAOD. Trends in
CALIOP-derived aerosol loading, in particular those partitioned in the PBL, can be explained to a large extent by meteorology.
Quan Liu, Dantong Liu, Yangzhou Wu, Kai Bi, Wenkang Gao, Ping Tian, Delong Zhao, Siyuan Li, Chenjie Yu, Guiqian Tang, Yunfei Wu, Kang Hu, Shuo Ding, Qian Gao, Fei Wang, Shaofei Kong, Hui He, Mengyu Huang, and Deping Ding
Atmos. Chem. Phys., 21, 14749–14760, https://doi.org/10.5194/acp-21-14749-2021, https://doi.org/10.5194/acp-21-14749-2021, 2021
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Through simultaneous online measurements of detailed aerosol compositions at both surface and surface-influenced mountain sites, the evolution of aerosol composition during daytime vertical transport was investigated. The results show that, from surface to the top of the planetary boundary layer, the oxidation state of organic aerosol had been significantly enhanced due to evaporation and further oxidation of these evaporated gases.
Qingyang Xiao, Yixuan Zheng, Guannan Geng, Cuihong Chen, Xiaomeng Huang, Huizheng Che, Xiaoye Zhang, Kebin He, and Qiang Zhang
Atmos. Chem. Phys., 21, 9475–9496, https://doi.org/10.5194/acp-21-9475-2021, https://doi.org/10.5194/acp-21-9475-2021, 2021
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We used both statistical methods and a chemical transport model to assess the contribution of meteorology and emissions to PM2.5 during 2000–2018. Both methods revealed that emissions dominated the long-term PM2.5 trend with notable meteorological effects ranged up to 37.9 % of regional annual average PM2.5. The meteorological contribution became more beneficial to PM2.5 control in southern China but more unfavorable in northern China during the studied period.
Xiaojing Shen, Junying Sun, Fangqun Yu, Ying Wang, Junting Zhong, Yangmei Zhang, Xinyao Hu, Can Xia, Sinan Zhang, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 7039–7052, https://doi.org/10.5194/acp-21-7039-2021, https://doi.org/10.5194/acp-21-7039-2021, 2021
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In this work, we revealed the changes of PNSD and NPF events during the COVID-19 lockdown period in Beijing, China, to illustrate the impact of reduced primary emission and elavated atmospheric oxidized capicity on the nucleation and growth processes. The subsequent growth of nucleated particles and their contribution to the aerosol pollution formation were also explored, to highlight the necessity of controlling the nanoparticles in the future air quality management.
Linlin Liang, Guenter Engling, Chang Liu, Wanyun Xu, Xuyan Liu, Yuan Cheng, Zhenyu Du, Gen Zhang, Junying Sun, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 3181–3192, https://doi.org/10.5194/acp-21-3181-2021, https://doi.org/10.5194/acp-21-3181-2021, 2021
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A unique episode with extreme biomass burning (BB) impact, with daily concentration of levoglucosan as high as 4.37 µg m-3, was captured at an area upwind of Beijing. How this extreme BB pollution event was generated and what were the chemical properties of PM2.5 under this kind severe BB pollution level in the real atmospheric environment were both presented in this measurement report. Moreover, the variation of the ratios of BB tracers during different BB pollution periods was also exhibited.
Lei Zhang, Sunling Gong, Tianliang Zhao, Chunhong Zhou, Yuesi Wang, Jiawei Li, Dongsheng Ji, Jianjun He, Hongli Liu, Ke Gui, Xiaomei Guo, Jinhui Gao, Yunpeng Shan, Hong Wang, Yaqiang Wang, Huizheng Che, and Xiaoye Zhang
Geosci. Model Dev., 14, 703–718, https://doi.org/10.5194/gmd-14-703-2021, https://doi.org/10.5194/gmd-14-703-2021, 2021
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Development of chemical transport models with advanced physics and chemical schemes is important for improving air-quality forecasts. This study develops the chemical module CUACE by updating with a new particle dry deposition scheme and adding heterogenous chemical reactions and couples it with the WRF model. The coupled model (WRF/CUACE) was able to capture well the variations of PM2.5, O3, NO2, and secondary inorganic aerosols in eastern China.
María A. Burgos, Elisabeth Andrews, Gloria Titos, Angela Benedetti, Huisheng Bian, Virginie Buchard, Gabriele Curci, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Anton Laakso, Julie Letertre-Danczak, Marianne T. Lund, Hitoshi Matsui, Gunnar Myhre, Cynthia Randles, Michael Schulz, Twan van Noije, Kai Zhang, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Junying Sun, Ernest Weingartner, and Paul Zieger
Atmos. Chem. Phys., 20, 10231–10258, https://doi.org/10.5194/acp-20-10231-2020, https://doi.org/10.5194/acp-20-10231-2020, 2020
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We investigate how well models represent the enhancement in scattering coefficients due to particle water uptake, and perform an evaluation of several implementation schemes used in ten Earth system models. Our results show the importance of the parameterization of hygroscopicity and model chemistry as drivers of some of the observed diversity amongst model estimates. The definition of dry conditions and the phenomena taking place in this relative humidity range also impact the model evaluation.
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Short summary
The simultaneous measurements under dry conditions of aerosol optical properties were conducted at three wavelengths for PM1 and PM10 in urban Beijing from 2018 to 2021. Considerable reductions in aerosol absorption coefficient and increased single scattering albedo demonstrated that absorbing aerosols were more effectively controlled than scattering aerosols due to pollution control measures. The aerosol radiative effect and the transport's impact on aerosol optical properties were analysed.
The simultaneous measurements under dry conditions of aerosol optical properties were conducted...
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