Articles | Volume 21, issue 3
https://doi.org/10.5194/acp-21-1649-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-1649-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
09 Feb 2021
Research article |
| 09 Feb 2021
| 09 Feb 2021
Impacts of multi-layer overlap on contrail radiative forcing
Laboratory for Aviation and the Environment, Massachusetts Institute
of Technology, Cambridge, MA 02139, United States of America
Sebastian D. Eastham
Laboratory for Aviation and the Environment, Massachusetts Institute
of Technology, Cambridge, MA 02139, United States of America
Joint Program on the Science and Policy of Global Change, Massachusetts Institute of Technology, Cambridge, MA, United States of America
Florian Allroggen
Laboratory for Aviation and the Environment, Massachusetts Institute
of Technology, Cambridge, MA 02139, United States of America
Joint Program on the Science and Policy of Global Change, Massachusetts Institute of Technology, Cambridge, MA, United States of America
Raymond L. Speth
Laboratory for Aviation and the Environment, Massachusetts Institute
of Technology, Cambridge, MA 02139, United States of America
Joint Program on the Science and Policy of Global Change, Massachusetts Institute of Technology, Cambridge, MA, United States of America
Steven R. H. Barrett
Laboratory for Aviation and the Environment, Massachusetts Institute
of Technology, Cambridge, MA 02139, United States of America
Joint Program on the Science and Policy of Global Change, Massachusetts Institute of Technology, Cambridge, MA, United States of America
Related authors
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Caleb Akhtar Martínez, Sebastian D. Eastham, and Jerome P. Jarrett
EGUsphere, https://doi.org/10.5194/egusphere-2025-278, https://doi.org/10.5194/egusphere-2025-278, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Contrails are clouds that form behind aircraft and can warm the atmosphere as much as carbon dioxide emissions from those planes. This work compares two contrail models of different complexities to understand their lifecycle and impact. The models differ in how contrails evolve over time, implying that we may be significantly underestimating their climate impact. This highlights the need for model diversity and more evaluation against observations of long-lived contrails.
William J. Collins, Fiona M. O'Connor, Connor R. Barker, Rachael E. Byrom, Sebastian D. Eastham, Øivind Hodnebrog, Patrick Jöckel, Eloise A. Marais, Mariano Mertens, Gunnar Myhre, Matthias Nützel, Dirk Olivié, Ragnhild Bieltvedt Skeie, Laura Stecher, Larry W. Horowitz, Vaishali Naik, Gregory Faluvegi, Ulas Im, Lee T. Murray, Drew Shindell, Kostas Tsigaridis, Nathan Luke Abraham, and James Keeble
EGUsphere, https://doi.org/10.5194/egusphere-2024-3698, https://doi.org/10.5194/egusphere-2024-3698, 2024
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If reductions aren’t implemented to limit emissions of pollutants that produce ozone then we calculate that this will cause a warming of climate. We assess how the future warming from ozone is affected by changing meteorological variables such as clouds and atmospheric temperatures. We find that reductions in high cloud cover tend to slightly reduce the warming from ozone.
Vincent R. Meijer, Sebastian D. Eastham, Ian A. Waitz, and Steven R. H. Barrett
Atmos. Meas. Tech., 17, 6145–6162, https://doi.org/10.5194/amt-17-6145-2024, https://doi.org/10.5194/amt-17-6145-2024, 2024
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Aviation's climate impact is partly due to contrails: the clouds that form behind aircraft and which can linger for hours under certain atmospheric conditions. Accurately forecasting these conditions could allow aircraft to avoid forming these contrails and thus reduce their environmental footprint. Our research uses deep learning to identify three-dimensional contrail locations in two-dimensional satellite imagery, which can be used to assess and improve these forecasts.
Haipeng Lin, Louisa K. Emmons, Elizabeth W. Lundgren, Laura Hyesung Yang, Xu Feng, Ruijun Dang, Shixian Zhai, Yunxiao Tang, Makoto M. Kelp, Nadia K. Colombi, Sebastian D. Eastham, Thibaud M. Fritz, and Daniel J. Jacob
Atmos. Chem. Phys., 24, 8607–8624, https://doi.org/10.5194/acp-24-8607-2024, https://doi.org/10.5194/acp-24-8607-2024, 2024
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Tropospheric ozone is a major air pollutant, a greenhouse gas, and a major indicator of model skill. Global atmospheric chemistry models show large differences in simulations of tropospheric ozone, but isolating sources of differences is complicated by different model environments. By implementing the GEOS-Chem model side by side to CAM-chem within a common Earth system model, we identify and evaluate specific differences between the two models and their impacts on key chemical species.
Irene C. Dedoussi, Daven K. Henze, Sebastian D. Eastham, Raymond L. Speth, and Steven R. H. Barrett
Geosci. Model Dev., 17, 5689–5703, https://doi.org/10.5194/gmd-17-5689-2024, https://doi.org/10.5194/gmd-17-5689-2024, 2024
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Atmospheric model gradients provide a meaningful tool for better understanding the underlying atmospheric processes. Adjoint modeling enables computationally efficient gradient calculations. We present the adjoint of the GEOS-Chem unified chemistry extension (UCX). With this development, the GEOS-Chem adjoint model can capture stratospheric ozone and other processes jointly with tropospheric processes. We apply it to characterize the Antarctic ozone depletion potential of active halogen species.
Sebastian D. Eastham, Guillaume P. Chossière, Raymond L. Speth, Daniel J. Jacob, and Steven R. H. Barrett
Atmos. Chem. Phys., 24, 2687–2703, https://doi.org/10.5194/acp-24-2687-2024, https://doi.org/10.5194/acp-24-2687-2024, 2024
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Emissions from aircraft are known to cause air quality impacts worldwide, but the scale and mechanisms of this impact are not well understood. This work uses high-resolution computational modeling of the atmosphere to show that air pollution changes from aviation are mostly the result of emissions during cruise (high-altitude) operations, that these impacts are related to how much non-aviation pollution is present, and that prior regional assessments have underestimated these impacts.
Ruijun Dang, Daniel J. Jacob, Viral Shah, Sebastian D. Eastham, Thibaud M. Fritz, Loretta J. Mickley, Tianjia Liu, Yi Wang, and Jun Wang
Atmos. Chem. Phys., 23, 6271–6284, https://doi.org/10.5194/acp-23-6271-2023, https://doi.org/10.5194/acp-23-6271-2023, 2023
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We use the GEOS-Chem model to better understand the magnitude and trend in free tropospheric NO2 over the contiguous US. Model underestimate of background NO2 is largely corrected by considering aerosol nitrate photolysis. Increase in aircraft emissions affects satellite retrievals by altering the NO2 shape factor, and this effect is expected to increase in future. We show the importance of properly accounting for the free tropospheric background in interpreting NO2 observations from space.
Fangqun Yu, Gan Luo, Arshad Arjunan Nair, Sebastian Eastham, Christina J. Williamson, Agnieszka Kupc, and Charles A. Brock
Atmos. Chem. Phys., 23, 1863–1877, https://doi.org/10.5194/acp-23-1863-2023, https://doi.org/10.5194/acp-23-1863-2023, 2023
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Particle number concentrations and size distributions in the stratosphere are studied through model simulations and comparisons with measurements. The nucleation scheme used in most of the solar geoengineering modeling studies overpredicts the nucleation rates and particle number concentrations in the stratosphere. The model based on updated nucleation schemes captures reasonably well some aspects of particle size distributions but misses some features. The possible reasons are discussed.
Viral Shah, Daniel J. Jacob, Ruijun Dang, Lok N. Lamsal, Sarah A. Strode, Stephen D. Steenrod, K. Folkert Boersma, Sebastian D. Eastham, Thibaud M. Fritz, Chelsea Thompson, Jeff Peischl, Ilann Bourgeois, Ilana B. Pollack, Benjamin A. Nault, Ronald C. Cohen, Pedro Campuzano-Jost, Jose L. Jimenez, Simone T. Andersen, Lucy J. Carpenter, Tomás Sherwen, and Mat J. Evans
Atmos. Chem. Phys., 23, 1227–1257, https://doi.org/10.5194/acp-23-1227-2023, https://doi.org/10.5194/acp-23-1227-2023, 2023
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NOx in the free troposphere (above 2 km) affects global tropospheric chemistry and the retrieval and interpretation of satellite NO2 measurements. We evaluate free tropospheric NOx in global atmospheric chemistry models and find that recycling NOx from its reservoirs over the oceans is faster than that simulated in the models, resulting in increases in simulated tropospheric ozone and OH. Over the U.S., free tropospheric NO2 contributes the majority of the tropospheric NO2 column in summer.
Randall V. Martin, Sebastian D. Eastham, Liam Bindle, Elizabeth W. Lundgren, Thomas L. Clune, Christoph A. Keller, William Downs, Dandan Zhang, Robert A. Lucchesi, Melissa P. Sulprizio, Robert M. Yantosca, Yanshun Li, Lucas Estrada, William M. Putman, Benjamin M. Auer, Atanas L. Trayanov, Steven Pawson, and Daniel J. Jacob
Geosci. Model Dev., 15, 8731–8748, https://doi.org/10.5194/gmd-15-8731-2022, https://doi.org/10.5194/gmd-15-8731-2022, 2022
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Atmospheric chemistry models must be able to operate both online as components of Earth system models and offline as standalone models. The widely used GEOS-Chem model operates both online and offline, but the classic offline version is not suitable for massively parallel simulations. We describe a new generation of the offline high-performance GEOS-Chem (GCHP) that enables high-resolution simulations on thousands of cores, including on the cloud, with improved access, performance, and accuracy.
Thibaud M. Fritz, Sebastian D. Eastham, Louisa K. Emmons, Haipeng Lin, Elizabeth W. Lundgren, Steve Goldhaber, Steven R. H. Barrett, and Daniel J. Jacob
Geosci. Model Dev., 15, 8669–8704, https://doi.org/10.5194/gmd-15-8669-2022, https://doi.org/10.5194/gmd-15-8669-2022, 2022
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We bring the state-of-the-science chemistry module GEOS-Chem into the Community Earth System Model (CESM). We show that some known differences between results from GEOS-Chem and CESM's CAM-chem chemistry module may be due to the configuration of model meteorology rather than inherent differences in the model chemistry. This is a significant step towards a truly modular Earth system model and allows two strong but currently separate research communities to benefit from each other's advances.
William Atkinson, Sebastian D. Eastham, Y.-H. Henry Chen, Jennifer Morris, Sergey Paltsev, C. Adam Schlosser, and Noelle E. Selin
Geosci. Model Dev., 15, 7767–7789, https://doi.org/10.5194/gmd-15-7767-2022, https://doi.org/10.5194/gmd-15-7767-2022, 2022
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Understanding policy effects on human-caused air pollutant emissions is key for assessing related health impacts. We develop a flexible scenario tool that combines updated emissions data sets, long-term economic modeling, and comprehensive technology pathways to clarify the impacts of climate and air quality policies. Results show the importance of both policy levers in the future to prevent long-term emission increases from offsetting near-term air quality improvements from existing policies.
Liam Bindle, Randall V. Martin, Matthew J. Cooper, Elizabeth W. Lundgren, Sebastian D. Eastham, Benjamin M. Auer, Thomas L. Clune, Hongjian Weng, Jintai Lin, Lee T. Murray, Jun Meng, Christoph A. Keller, William M. Putman, Steven Pawson, and Daniel J. Jacob
Geosci. Model Dev., 14, 5977–5997, https://doi.org/10.5194/gmd-14-5977-2021, https://doi.org/10.5194/gmd-14-5977-2021, 2021
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Atmospheric chemistry models like GEOS-Chem are versatile tools widely used in air pollution and climate studies. The simulations used in such studies can be very computationally demanding, and thus it is useful if the model can simulate a specific geographic region at a higher resolution than the rest of the globe. Here, we implement, test, and demonstrate a new variable-resolution capability in GEOS-Chem that is suitable for simulations conducted on supercomputers.
Xuan Wang, Daniel J. Jacob, William Downs, Shuting Zhai, Lei Zhu, Viral Shah, Christopher D. Holmes, Tomás Sherwen, Becky Alexander, Mathew J. Evans, Sebastian D. Eastham, J. Andrew Neuman, Patrick R. Veres, Theodore K. Koenig, Rainer Volkamer, L. Gregory Huey, Thomas J. Bannan, Carl J. Percival, Ben H. Lee, and Joel A. Thornton
Atmos. Chem. Phys., 21, 13973–13996, https://doi.org/10.5194/acp-21-13973-2021, https://doi.org/10.5194/acp-21-13973-2021, 2021
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Halogen radicals have a broad range of implications for tropospheric chemistry, air quality, and climate. We present a new mechanistic description and comprehensive simulation of tropospheric halogens in a global 3-D model and compare the model results with surface and aircraft measurements. We find that halogen chemistry decreases the global tropospheric burden of ozone by 11 %, NOx by 6 %, and OH by 4 %.
Haipeng Lin, Daniel J. Jacob, Elizabeth W. Lundgren, Melissa P. Sulprizio, Christoph A. Keller, Thibaud M. Fritz, Sebastian D. Eastham, Louisa K. Emmons, Patrick C. Campbell, Barry Baker, Rick D. Saylor, and Raffaele Montuoro
Geosci. Model Dev., 14, 5487–5506, https://doi.org/10.5194/gmd-14-5487-2021, https://doi.org/10.5194/gmd-14-5487-2021, 2021
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Emissions are a central component of atmospheric chemistry models. The Harmonized Emissions Component (HEMCO) is a software component for computing emissions from a user-selected ensemble of emission inventories and algorithms. It allows users to select, add, and scale emissions from different sources through a configuration file with no change to the model source code. We demonstrate the implementation of HEMCO in several models, all sharing the same HEMCO core code and database library.
Xiao Lu, Lin Zhang, Tongwen Wu, Michael S. Long, Jun Wang, Daniel J. Jacob, Fang Zhang, Jie Zhang, Sebastian D. Eastham, Lu Hu, Lei Zhu, Xiong Liu, and Min Wei
Geosci. Model Dev., 13, 3817–3838, https://doi.org/10.5194/gmd-13-3817-2020, https://doi.org/10.5194/gmd-13-3817-2020, 2020
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This study presents the development and evaluation of a new climate chemistry model, BCC-GEOS-Chem v1.0, which couples the GEOS-Chem chemical transport model as an atmospheric chemistry component in the Beijing Climate Center atmospheric general circulation model. A 3-year (2012–2014) simulation of BCC-GEOS-Chem v1.0 shows that the model captures well the spatiotemporal distributions of tropospheric ozone, other gaseous pollutants, and aerosols.
Haipeng Lin, Xu Feng, Tzung-May Fu, Heng Tian, Yaping Ma, Lijuan Zhang, Daniel J. Jacob, Robert M. Yantosca, Melissa P. Sulprizio, Elizabeth W. Lundgren, Jiawei Zhuang, Qiang Zhang, Xiao Lu, Lin Zhang, Lu Shen, Jianping Guo, Sebastian D. Eastham, and Christoph A. Keller
Geosci. Model Dev., 13, 3241–3265, https://doi.org/10.5194/gmd-13-3241-2020, https://doi.org/10.5194/gmd-13-3241-2020, 2020
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Online coupling of meteorology and chemistry models often presents maintenance issues with hard-wired coding. We present WRF-GC, an one-way online coupling of the WRF meteorological model and GEOS-Chem atmospheric chemistry model for regional atmospheric chemistry and air quality modeling. Our coupling structure allows future versions of either parent model to be immediately integrated into WRF-GC. The WRF-GC model was able to well reproduce regional PM2.5 with greater computational efficiency.
Thibaud M. Fritz, Sebastian D. Eastham, Raymond L. Speth, and Steven R. H. Barrett
Atmos. Chem. Phys., 20, 5697–5727, https://doi.org/10.5194/acp-20-5697-2020, https://doi.org/10.5194/acp-20-5697-2020, 2020
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Aircraft exhaust drives formation of ozone and is a dominant anthropogenic influence in the upper troposphere. These impacts are mitigated by non-linear chemistry inside the aircraft plume, which cuts off part of the ozone production pathway and reduces the long-term impact of aircraft in a way which is not captured by current models. The ice clouds which form in aircraft exhaust ("contrails") also play a role, converting emitted nitrogen oxides into more stable forms such as nitric acid.
Lei Zhu, Daniel J. Jacob, Sebastian D. Eastham, Melissa P. Sulprizio, Xuan Wang, Tomás Sherwen, Mat J. Evans, Qianjie Chen, Becky Alexander, Theodore K. Koenig, Rainer Volkamer, L. Gregory Huey, Michael Le Breton, Thomas J. Bannan, and Carl J. Percival
Atmos. Chem. Phys., 19, 6497–6507, https://doi.org/10.5194/acp-19-6497-2019, https://doi.org/10.5194/acp-19-6497-2019, 2019
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We quantify the effect of sea salt aerosol on tropospheric bromine chemistry with a new mechanistic description of the halogen chemistry in a global atmospheric chemistry model. For the first time, we are able to reproduce the observed levels of bromide activation from the sea salt aerosol in a manner consistent with bromine oxide radical measured from various platforms. Sea salt aerosol plays a far more complex role in global tropospheric chemistry than previously recognized.
Xuan Wang, Daniel J. Jacob, Sebastian D. Eastham, Melissa P. Sulprizio, Lei Zhu, Qianjie Chen, Becky Alexander, Tomás Sherwen, Mathew J. Evans, Ben H. Lee, Jessica D. Haskins, Felipe D. Lopez-Hilfiker, Joel A. Thornton, Gregory L. Huey, and Hong Liao
Atmos. Chem. Phys., 19, 3981–4003, https://doi.org/10.5194/acp-19-3981-2019, https://doi.org/10.5194/acp-19-3981-2019, 2019
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Chlorine radicals have a broad range of implications for tropospheric chemistry, air quality, and climate. We present a comprehensive simulation of tropospheric chlorine in a global 3-D model, which includes explicit accounting of chloride mobilization from sea salt aerosol. We find the chlorine chemistry contributes 1.0 % of the global oxidation of methane and decreases global burdens of tropospheric ozone by 7 % and OH by 3 % through the associated bromine radical chemistry.
Sebastian D. Eastham, Michael S. Long, Christoph A. Keller, Elizabeth Lundgren, Robert M. Yantosca, Jiawei Zhuang, Chi Li, Colin J. Lee, Matthew Yannetti, Benjamin M. Auer, Thomas L. Clune, Jules Kouatchou, William M. Putman, Matthew A. Thompson, Atanas L. Trayanov, Andrea M. Molod, Randall V. Martin, and Daniel J. Jacob
Geosci. Model Dev., 11, 2941–2953, https://doi.org/10.5194/gmd-11-2941-2018, https://doi.org/10.5194/gmd-11-2941-2018, 2018
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Global atmospheric chemical transport models are crucial tools in atmospheric science, used to address problems ranging from climate change to acid rain. GEOS-Chem High Performance (GCHP) is a new implementation of the widely used GEOS-Chem model, designed for massively parallel architectures. GCHP v11-02c is shown to be highly scalable from 6 to over 500 cores, enabling the routine simulation of global atmospheric chemistry from the surface to the stratopause at resolutions of ~50 km or finer.
Jiawei Zhuang, Daniel J. Jacob, and Sebastian D. Eastham
Atmos. Chem. Phys., 18, 6039–6055, https://doi.org/10.5194/acp-18-6039-2018, https://doi.org/10.5194/acp-18-6039-2018, 2018
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Our work explains why current model simulations are unable to capture the intercontinental influences of pollution plumes that are often observed over some regions like California. Due to inadequate vertical grid resolution in these models, the plumes get diffused too rapidly during intercontinental transport. Increasing the vertical grid resolution greatly improves the simulation of plumes and considerably increases the estimate of local surface pollution influence.
Karen Yu, Christoph A. Keller, Daniel J. Jacob, Andrea M. Molod, Sebastian D. Eastham, and Michael S. Long
Geosci. Model Dev., 11, 305–319, https://doi.org/10.5194/gmd-11-305-2018, https://doi.org/10.5194/gmd-11-305-2018, 2018
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Global simulations of atmospheric chemistry are generally conducted with off-line chemical transport models (CTMs) driven by archived meteorological data from general circulation models (GCMs). The off-line approach has the advantages of simplicity and expediency, but it is unable to reproduce the GCM transport exactly. We investigate the cascade of errors associated with the off-line approach using the GEOS-5 GCM and GEOS-Chem CTM and discuss improvements in the use of archived meteorology.
Sebastian D. Eastham and Daniel J. Jacob
Atmos. Chem. Phys., 17, 2543–2553, https://doi.org/10.5194/acp-17-2543-2017, https://doi.org/10.5194/acp-17-2543-2017, 2017
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Intercontinental atmospheric transport can disrupt local chemistry and cause air quality issues thousands of kilometers from the source, complicating correct attribution of air quality exceedances. This transport occurs in long, thin plumes which current-generation models consistently fail to reproduce. Our study investigates the cause of this failure, finding that greater vertical resolution than is currently available is required to reliably resolve the plumes and their effects.
Tomás Sherwen, Johan A. Schmidt, Mat J. Evans, Lucy J. Carpenter, Katja Großmann, Sebastian D. Eastham, Daniel J. Jacob, Barbara Dix, Theodore K. Koenig, Roman Sinreich, Ivan Ortega, Rainer Volkamer, Alfonso Saiz-Lopez, Cristina Prados-Roman, Anoop S. Mahajan, and Carlos Ordóñez
Atmos. Chem. Phys., 16, 12239–12271, https://doi.org/10.5194/acp-16-12239-2016, https://doi.org/10.5194/acp-16-12239-2016, 2016
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We present a simulation of tropospheric Cl, Br, I chemistry within the GEOS-Chem CTM. We find a decrease in tropospheric ozone burden of 18.6 % and a 8.2 % decrease in global mean OH concentrations. Cl oxidation of some VOCs range from 15 to 27 % of the total loss. Bromine plays a small role in oxidising oVOCs. Surface ozone, ozone sondes, and methane lifetime are in general improved by the inclusion of halogens. We argue that simulated bromine and chlorine represent a lower limit.
C. L. Heald, D. A. Ridley, J. H. Kroll, S. R. H. Barrett, K. E. Cady-Pereira, M. J. Alvarado, and C. D. Holmes
Atmos. Chem. Phys., 14, 5513–5527, https://doi.org/10.5194/acp-14-5513-2014, https://doi.org/10.5194/acp-14-5513-2014, 2014
Related subject area
Subject: Radiation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Fine and coarse dust radiative impact during an intense Saharan dust outbreak over the Iberian Peninsula – short-wave direct radiative effect
Modeling actinic flux and photolysis frequencies in dense biomass burning plumes
Regional modeling of surface solar radiation, aerosol, and cloud cover spatial variability and projections over northern France and Benelux
A numerical sensitivity study on the snow-darkening effect by black carbon deposition over the Arctic in spring
Improved calculation of single-scattering properties of frozen droplets and frozen-droplet aggregates observed in deep convective clouds
Influence of cloudy and clear-sky partitions, aerosols, and geometry on the recent variability in surface solar irradiance components in northern France
Saharan dust impact on radiative heating rate errors inherent in reanalysis data in the African easterly wave development region
The Modulation of Synoptic Weather Patterns and Human Activities on the Diurnal Cycle of Summertime Canopy Urban Heat Island in Yangtze River Delta Urban Agglomeration, China
Combining observations and simulations to investigate the small-scale variability of surface solar irradiance under continental cumulus clouds
The impact of coupled 3D shortwave radiative transfer on surface radiation and cumulus clouds over land
Atmospheric cloud-radiative heating in CMIP6 and observations and its response to surface warming
Mechanisms of surface solar irradiance variability under broken clouds
Responses of polar energy budget to regional SST changes in extra-polar regions
Trends in observed surface solar radiation and their causes in Brazil in the first 2 decades of the 21st century
A sensitivity study on radiative effects due to the parameterization of dust optical properties in models
Uncertainties in cloud-radiative heating within an idealized extratropical cyclone
Evaluation of downward and upward solar irradiances simulated by the Integrated Forecasting System of ECMWF using airborne observations above Arctic low-level clouds
A colorful look at climate sensitivity
Sensitivity of cirrus and contrail radiative effect on cloud microphysical and environmental parameters
Evaluation of liquid cloud albedo susceptibility in E3SM using coupled eastern North Atlantic surface and satellite retrievals
Constraints on simulated past Arctic amplification and lapse rate feedback from observations
Comparison of methods to estimate aerosol effective radiative forcings in climate models
Montreal Protocol's impact on the ozone layer and climate
Opinion: The scientific and community-building roles of the Geoengineering Model Intercomparison Project (GeoMIP) – past, present, and future
Impacts of reductions in non-methane short-lived climate forcers on future climate extremes and the resulting population exposure risks in eastern and southern Asia
Investigating the radiative effect of Arctic cirrus measured in situ during the winter 2015–2016
Dependence of strategic solar climate intervention on background scenario and model physics
Combining short-range dispersion simulations with fine-scale meteorological ensembles: probabilistic indicators and evaluation during a 85Kr field campaign
Climate consequences of hydrogen emissions
Investigating the impact of Saharan dust aerosols on analyses and forecasts of African easterly waves by constraining aerosol effects in radiance data assimilation
Distinct surface response to black carbon aerosols
Estimating the potential cooling effect of cirrus thinning achieved via the seeding approach
Bias in CMIP6 models as compared to observed regional dimming and brightening
A test of the ability of current bulk optical models to represent the radiative properties of cirrus cloud across the mid- and far-infrared
The incorporation of the Tripleclouds concept into the δ-Eddington two-stream radiation scheme: solver characterization and its application to shallow cumulus clouds
Radiative heating rate profiles over the southeast Atlantic Ocean during the 2016 and 2017 biomass burning seasons
Effective radiative forcing and adjustments in CMIP6 models
Response of surface shortwave cloud radiative effect to greenhouse gases and aerosols and its impact on summer maximum temperature
Combining atmospheric and snow radiative transfer models to assess the solar radiative effects of black carbon in the Arctic
Accurate 3-D radiative transfer simulation of spectral solar irradiance during the total solar eclipse of 21 August 2017
Quantifying the bias of radiative heating rates in numerical weather prediction models for shallow cumulus clouds
The climate effects of increasing ocean albedo: an idealized representation of solar geoengineering
Changes in clouds and thermodynamics under solar geoengineering and implications for required solar reduction
Radiative impact of an extreme Arctic biomass-burning event
Contrails and their impact on shortwave radiation and photovoltaic power production – a regional model study
The influence of internal variability on Earth's energy balance framework and implications for estimating climate sensitivity
Insights into the diurnal cycle of global Earth outgoing radiation using a numerical weather prediction model
Determining the infrared radiative effects of Saharan dust: a radiative transfer modelling study based on vertically resolved measurements at Lampedusa
The early summertime Saharan heat low: sensitivity of the radiation budget and atmospheric heating to water vapour and dust aerosol
The role of 1-D and 3-D radiative heating in the organization of shallow cumulus convection and the formation of cloud streets
María-Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Michaël Sicard, Jesús Abril-Gago, Vanda Salgueiro, Adolfo Comerón, María José Granados-Muñoz, Maria João Costa, Constantino Muñoz-Porcar, Juan Antonio Bravo-Aranda, Daniele Bortoli, Alejandro Rodríguez-Gómez, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 25, 3213–3231, https://doi.org/10.5194/acp-25-3213-2025, https://doi.org/10.5194/acp-25-3213-2025, 2025
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Due to the significant radiative role of dust in climate change, vertical assessments of the short-wave dust direct radiative effect of both fine and coarse dust particles are performed separately. The study is focused on an intense Saharan dust outbreak crossing the Iberian Peninsula in springtime monitored by five Iberian lidar stations with southwest–northeast coverage. A comparative study to evaluate the differences found by considering the total dust (no separation) is also examined.
Jan-Lukas Tirpitz, Santo Fedele Colosimo, Nathaniel Brockway, Robert Spurr, Matt Christi, Samuel Hall, Kirk Ullmann, Johnathan Hair, Taylor Shingler, Rodney Weber, Jack Dibb, Richard Moore, Elizabeth Wiggins, Vijay Natraj, Nicolas Theys, and Jochen Stutz
Atmos. Chem. Phys., 25, 1989–2015, https://doi.org/10.5194/acp-25-1989-2025, https://doi.org/10.5194/acp-25-1989-2025, 2025
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We combine plume composition data from the 2019 NASA FIREX-AQ campaign with state-of-the-art radiative transfer modeling techniques to calculate distributions of actinic flux and photolysis frequencies in a wildfire plume. Excellent agreement of the model and observations demonstrates the applicability of this approach to constrain photochemistry in such plumes. We identify limiting factors for the modeling accuracy and discuss spatial and spectral features of the distributions.
Gabriel Chesnoiu, Isabelle Chiapello, Nicolas Ferlay, Pierre Nabat, Marc Mallet, and Véronique Riffault
Atmos. Chem. Phys., 25, 1307–1331, https://doi.org/10.5194/acp-25-1307-2025, https://doi.org/10.5194/acp-25-1307-2025, 2025
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The ALADIN regional climate model at 12.5 km resolution allows us to study the evolution of surface solar radiation (SSR) and key associated atmospheric parameters. Over northern France and Benelux, influenced by anthropogenic aerosols and cloudy conditions, regional evaluation of recent hindcast simulations shows satisfying results and high spatial variability. Future SSR evolution by the end of the century for two contrasting CMIP6 scenarios highlights large decreases in SSR for SSP3-7.0.
Zilu Zhang, Libo Zhou, and Meigen Zhang
Atmos. Chem. Phys., 25, 1–25, https://doi.org/10.5194/acp-25-1-2025, https://doi.org/10.5194/acp-25-1-2025, 2025
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By integrating the SNICAR model with Polar-WRF, we find that 50 ng g−1 black carbon (BC) deposition decreases snow albedo, increasing radiative forcing (RF) by 1–4 W m−2, especially in Greenland, Baffin Island, and eastern Siberia. The impact is strongly linked to BC mass, with deep snowpacks showing greater sensitivity. Snowmelt and land–atmosphere interactions are crucial. High-resolution modelling is necessary to better understand these effects on Arctic climate change.
Jeonggyu Kim, Sungmin Park, Greg M. McFarquhar, Anthony J. Baran, Joo Wan Cha, Kyoungmi Lee, Seoung Soo Lee, Chang Hoon Jung, Kyo-Sun Sunny Lim, and Junshik Um
Atmos. Chem. Phys., 24, 12707–12726, https://doi.org/10.5194/acp-24-12707-2024, https://doi.org/10.5194/acp-24-12707-2024, 2024
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We developed idealized models to represent the shapes of ice particles found in deep convective clouds and calculated their single-scattering properties. By comparing these results with in situ measurements, we discovered that a mixture of shape models matches in situ measurements more closely than single-form models or aggregate models. This finding has important implications for enhancing the simulation of single-scattering properties of ice crystals in deep convective clouds.
Gabriel Chesnoiu, Nicolas Ferlay, Isabelle Chiapello, Frédérique Auriol, Diane Catalfamo, Mathieu Compiègne, Thierry Elias, and Isabelle Jankowiak
Atmos. Chem. Phys., 24, 12375–12407, https://doi.org/10.5194/acp-24-12375-2024, https://doi.org/10.5194/acp-24-12375-2024, 2024
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The measured ground-based surface solar irradiance variability and its sensitivity to scene parameters are analysed with a filtering of sky conditions at a given site. Its multivariate analysis is applied to observed trends over 2010–2022. The recorded values show, in addition to the dominant effects of cloud occurrence, the variable effects of aerosol and geometry. Clear-sun-with-cloud situations are highlighted by SSI levels close to those of aerosol- and cloud-free situations.
Ruby W. Burgess and Mayra I. Oyola-Merced
Atmos. Chem. Phys., 24, 12183–12201, https://doi.org/10.5194/acp-24-12183-2024, https://doi.org/10.5194/acp-24-12183-2024, 2024
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This study explores how aerosols affect atmospheric heating over African easterly waves (AEWs). Using data from NASA's aircraft and outputs of reanalysis models, the research focuses on days with both Saharan dust and AEWs. Using a radiative transfer model, the study reveals significant differences in heating rates, emphasizing challenges in accurately representing aerosol effects in the atmosphere and underscoring the need for improved aerosol representation in weather models.
Tao Shi, Yuanjian Yang, Lian Zong, Min Guo, Ping Qi, and Simone Lolli
EGUsphere, https://doi.org/10.5194/egusphere-2024-3111, https://doi.org/10.5194/egusphere-2024-3111, 2024
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Our study explored the daily temperature patterns in urban areas of the Yangtze River Delta, focusing on how weather and human activities impact these patterns. We found that temperatures were higher at night, and weather patterns had a bigger impact during the day, while human activities mattered more at night. This helps us understand and address urban overheating.
Zili He, Quentin Libois, Najda Villefranque, Hartwig Deneke, Jonas Witthuhn, and Fleur Couvreux
Atmos. Chem. Phys., 24, 11391–11408, https://doi.org/10.5194/acp-24-11391-2024, https://doi.org/10.5194/acp-24-11391-2024, 2024
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This study uses observations and simulations to analyze how cumulus clouds affect spacial solar radiation variability on the ground. Results show that the simulations reproduce the observations well and improve understanding of cloud impacts on radiation. The research also indicates that a few strategically placed sensors, capitalizing on measurement timing, can effectively measure these variations, aiding in the development of detailed weather prediction models.
Mirjam Tijhuis, Bart J. H. van Stratum, and Chiel C. van Heerwaarden
Atmos. Chem. Phys., 24, 10567–10582, https://doi.org/10.5194/acp-24-10567-2024, https://doi.org/10.5194/acp-24-10567-2024, 2024
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Radiative transfer in the atmosphere is a 3D processes, which is often modelled in 1D for computational efficiency. We studied the differences between using 1D and 3D radiative transfer. With 3D radiation, larger clouds that contain more liquid water develop. However, they cover roughly the same part of the sky, and the average total radiation at the surface is nearly unchanged. The increase in cloud size might be important for weather models, as it can impact the formation of rain, for example.
Aiko Voigt, Stefanie North, Blaž Gasparini, and Seung-Hee Ham
Atmos. Chem. Phys., 24, 9749–9775, https://doi.org/10.5194/acp-24-9749-2024, https://doi.org/10.5194/acp-24-9749-2024, 2024
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Clouds shape weather and climate by interacting with photons, which changes temperatures within the atmosphere. We assess how well CMIP6 climate models capture this radiative heating by clouds within the atmosphere. While we find large differences among models, especially in cold regions of the atmosphere with abundant ice clouds, we also demonstrate that physical understanding allows us to predict the response of clouds and their radiative heating near the tropopause to climate change.
Wouter Mol and Chiel van Heerwaarden
EGUsphere, https://doi.org/10.5194/egusphere-2024-2396, https://doi.org/10.5194/egusphere-2024-2396, 2024
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Sunlight varies often and quickly under broken cloud cover, and every cloud field creates a unique pattern of sunlight on the surface below. These variations affect many processes in the Earth system, from photosynthesis and chemistry, to cloud formation itself. The exact way in which cloud particles interact with sunlight is complex and expensive to calculate. We demonstrate a simplified framework which explains how sunlight changes for potentially any cloud field.
Qingmin Wang, Yincheng Liu, Lujun Zhang, and Chen Zhou
EGUsphere, https://doi.org/10.5194/egusphere-2024-2379, https://doi.org/10.5194/egusphere-2024-2379, 2024
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Our research explores how SST changes in non-polar regions impact the polar energy budget. Through idealized SST experiments, we found that warming in tropical and midlatitude oceans raises polar temperatures via enhanced atmospheric energy transport, leading to surface warming and top-of-atmosphere cooling in polar areas. This study highlights the distinct impacts of tropical Pacific and Indian Ocean SST changes on Arctic and Antarctic climates.
Lucas Ferreira Correa, Doris Folini, Boriana Chtirkova, and Martin Wild
Atmos. Chem. Phys., 24, 8797–8819, https://doi.org/10.5194/acp-24-8797-2024, https://doi.org/10.5194/acp-24-8797-2024, 2024
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We investigated the causes of the decadal trends of solar radiation measured at 34 stations in Brazil in the first 2 decades of the 21st century. We observed strong negative trends in north and northeast Brazil associated with changes in both atmospheric absorption (anthropogenic) and cloud cover (natural). In other parts of the country no strong trends were observed as a result of competing effects. This provides a better understanding of the energy balance in the region.
Ilias Fountoulakis, Alexandra Tsekeri, Stelios Kazadzis, Vassilis Amiridis, Angelos Nersesian, Maria Tsichla, Emmanouil Proestakis, Antonis Gkikas, Kyriakoula Papachristopoulou, Vasileios Barlakas, Claudia Emde, and Bernhard Mayer
Atmos. Chem. Phys., 24, 4915–4948, https://doi.org/10.5194/acp-24-4915-2024, https://doi.org/10.5194/acp-24-4915-2024, 2024
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In our study we provide an assessment, through a sensitivity study, of the limitations of models to calculate the dust direct radiative effect (DRE) due to the underrepresentation of its size, refractive index (RI), and shape. Our results indicate the necessity of including more realistic sizes and RIs for dust particles in dust models, in order to derive better estimations of the dust direct radiative effects.
Behrooz Keshtgar, Aiko Voigt, Bernhard Mayer, and Corinna Hoose
Atmos. Chem. Phys., 24, 4751–4769, https://doi.org/10.5194/acp-24-4751-2024, https://doi.org/10.5194/acp-24-4751-2024, 2024
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Cloud-radiative heating (CRH) affects extratropical cyclones but is uncertain in weather and climate models. We provide a framework to quantify uncertainties in CRH within an extratropical cyclone due to four factors and show that the parameterization of ice optical properties contributes significantly to uncertainty in CRH. We also argue that ice optical properties, by affecting CRH on spatial scales of 100 km, are relevant for the large-scale dynamics of extratropical cyclones.
Hanno Müller, André Ehrlich, Evelyn Jäkel, Johannes Röttenbacher, Benjamin Kirbus, Michael Schäfer, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 4157–4175, https://doi.org/10.5194/acp-24-4157-2024, https://doi.org/10.5194/acp-24-4157-2024, 2024
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A weather model is used to compare solar radiation with measurements from an aircraft campaign in the Arctic. Model and observations agree on the downward radiation but show differences in the radiation reflected by the surface and the clouds, which in the model is too low above sea ice and too high above open ocean. The model–observation bias is reduced above open ocean by a realistic fraction of clouds and less cloud liquid water and above sea ice by less dark sea ice and more cloud droplets.
Bjorn Stevens and Lukas Kluft
Atmos. Chem. Phys., 23, 14673–14689, https://doi.org/10.5194/acp-23-14673-2023, https://doi.org/10.5194/acp-23-14673-2023, 2023
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A simple model is introduced to account for the spectral diversity of radiant energy transfer. It provides an improved basis for assessing the different ways in which clouds influence Earth’s climate sensitivity, demonstrating how many cloud effects depend on the existing cloud climatology. Given existing assessments of changes in cloud albedo with warming, it is determined that clouds reduce Earth's climate sensitivity as compared to what it would be in a counterfactual world without clouds.
Kevin Wolf, Nicolas Bellouin, and Olivier Boucher
Atmos. Chem. Phys., 23, 14003–14037, https://doi.org/10.5194/acp-23-14003-2023, https://doi.org/10.5194/acp-23-14003-2023, 2023
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Cirrus and contrails considerably impact Earth's energy budget. Such ice clouds can have a positive (warming) or negative (cooling) net radiative effect (RE), which depends on cloud and ambient properties. The effect of eight parameters on the cloud RE is estimated. In total, 283 500 radiative transfer simulations have been performed, spanning the typical parameter ranges associated with cirrus and contrails. Specific cases are selected and discussed. The data set is publicly available.
Adam C. Varble, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Shuaiqi Tang, and Jerome Fast
Atmos. Chem. Phys., 23, 13523–13553, https://doi.org/10.5194/acp-23-13523-2023, https://doi.org/10.5194/acp-23-13523-2023, 2023
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We evaluate how clouds change in response to changing atmospheric particle (aerosol) concentrations in a climate model and find that the model-predicted cloud brightness increases too much as aerosols increase because the cloud drop number increases too much. Excessive drizzle in the model mutes this difference. Many differences between observational and model estimates are explained by varying assumptions of how much liquid has been lost in clouds, which impacts the estimated cloud drop number.
Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
Atmos. Chem. Phys., 23, 9963–9992, https://doi.org/10.5194/acp-23-9963-2023, https://doi.org/10.5194/acp-23-9963-2023, 2023
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Lapse rate feedback (LRF) is a major driver of the Arctic amplification (AA) of climate change. It arises because the warming is stronger at the surface than aloft. Several processes can affect the LRF in the Arctic, such as the omnipresent temperature inversion. Here, we compare multimodel climate simulations to Arctic-based observations from a large research consortium to broaden our understanding of these processes, find synergy among them, and constrain the Arctic LRF and AA.
Mark D. Zelinka, Christopher J. Smith, Yi Qin, and Karl E. Taylor
Atmos. Chem. Phys., 23, 8879–8898, https://doi.org/10.5194/acp-23-8879-2023, https://doi.org/10.5194/acp-23-8879-2023, 2023
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The primary uncertainty in how strongly Earth's climate has been perturbed by human activities comes from the unknown radiative impact of aerosol changes. Accurately quantifying these forcings – and their sub-components – in climate models is crucial for understanding the past and future simulated climate. In this study we describe biases in previously published estimates of aerosol radiative forcing in climate models and provide corrected estimates along with code for users to compute them.
Tatiana Egorova, Jan Sedlacek, Timofei Sukhodolov, Arseniy Karagodin-Doyennel, Franziska Zilker, and Eugene Rozanov
Atmos. Chem. Phys., 23, 5135–5147, https://doi.org/10.5194/acp-23-5135-2023, https://doi.org/10.5194/acp-23-5135-2023, 2023
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This paper describes the climate and atmosphere benefits of the Montreal Protocol, simulated with the state-of-the-art Earth system model SOCOLv4.0. We have added to and confirmed the previous studies by showing that without the Montreal Protocol by the end of the 21st century there would be a dramatic reduction in the ozone layer as well as substantial perturbation of the essential climate variables in the troposphere caused by the warming from increasing ozone-depleting substances.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Yingfang Li, Zhili Wang, Yadong Lei, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 2499–2523, https://doi.org/10.5194/acp-23-2499-2023, https://doi.org/10.5194/acp-23-2499-2023, 2023
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Since few studies have assessed the impacts of future combined reductions in aerosols, ozone, and their precursors on future climate change, we use models with an interactive representation of tropospheric aerosols and atmospheric chemistry schemes to quantify the impact of their reductions on the Asian climate. Our results suggest that their reductions will exacerbate the warming effect caused by greenhouse gases, increasing future climate extremes and associated population exposure risk.
Andreas Marsing, Ralf Meerkötter, Romy Heller, Stefan Kaufmann, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, and Christiane Voigt
Atmos. Chem. Phys., 23, 587–609, https://doi.org/10.5194/acp-23-587-2023, https://doi.org/10.5194/acp-23-587-2023, 2023
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We employ highly resolved aircraft measurements of profiles of the ice water content (IWC) in Arctic cirrus clouds in winter and spring, when solar irradiation is low. Using radiation transfer calculations, we assess the cloud radiative effect over different surfaces like snow or ocean. The variability in the IWC of the clouds affects their overall radiative effect and drives internal processes. This helps understand the role of cirrus in a rapidly changing Arctic environment.
John T. Fasullo and Jadwiga H. Richter
Atmos. Chem. Phys., 23, 163–182, https://doi.org/10.5194/acp-23-163-2023, https://doi.org/10.5194/acp-23-163-2023, 2023
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The continued high levels of anthropogenic greenhouse gas emissions increase the likelihood that key climate warming thresholds will be exceeded in the coming decades. Here we examine a recently proposed geoengineering approach using two recently produced climate model experiments. We find the associated latitudinal distribution of aerosol mass to exhibit substantial uncertainty, suggesting the need for significant flexibility in the location and amount of aerosol delivery, if implemented.
Youness El-Ouartassy, Irène Korsakissok, Matthieu Plu, Olivier Connan, Laurent Descamps, and Laure Raynaud
Atmos. Chem. Phys., 22, 15793–15816, https://doi.org/10.5194/acp-22-15793-2022, https://doi.org/10.5194/acp-22-15793-2022, 2022
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This work investigates the potential value of using fine-scale meteorological ensembles to represent the inherent meteorological uncertainties in atmospheric dispersion model outputs. Probabilistic scores were used to evaluate the probabilistic performance of dispersion ensembles, using an original dataset of new continuous 85Kr air concentration measurements and a well-known source term. The results show that the ensemble dispersion simulations perform better than deterministic ones.
Ilissa B. Ocko and Steven P. Hamburg
Atmos. Chem. Phys., 22, 9349–9368, https://doi.org/10.5194/acp-22-9349-2022, https://doi.org/10.5194/acp-22-9349-2022, 2022
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Hydrogen is considered a key strategy to decarbonize the global economy. However, hydrogen is also a short-lived indirect greenhouse gas that can easily leak into the atmosphere. Given that the climate impacts from hydrogen emissions are not well understood, especially in the near term, we assess impacts over all timescales for plausible emissions rates. We find that hydrogen leakage can cause more warming than widely perceived; thus, attention is needed to minimize emissions.
Dustin Francis Phillip Grogan, Cheng-Hsuan Lu, Shih-Wei Wei, and Sheng-Po Chen
Atmos. Chem. Phys., 22, 2385–2398, https://doi.org/10.5194/acp-22-2385-2022, https://doi.org/10.5194/acp-22-2385-2022, 2022
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This study shows that incorporating aerosols into satellite radiance calculations affects the representation of African easterly waves (AEWs), and their environment, over North Africa and the eastern Atlantic in a numerical weather model. These changes are driven by radiative effects of Saharan dust captured by the aerosol-affected radiances, which modify the initial fields and can improve the forecasting of AEWs.
Tao Tang, Drew Shindell, Yuqiang Zhang, Apostolos Voulgarakis, Jean-Francois Lamarque, Gunnar Myhre, Gregory Faluvegi, Bjørn H. Samset, Timothy Andrews, Dirk Olivié, Toshihiko Takemura, and Xuhui Lee
Atmos. Chem. Phys., 21, 13797–13809, https://doi.org/10.5194/acp-21-13797-2021, https://doi.org/10.5194/acp-21-13797-2021, 2021
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Previous studies showed that black carbon (BC) could warm the surface with decreased incoming radiation. With climate models, we found that the surface energy redistribution plays a more crucial role in surface temperature compared with other forcing agents. Though BC could reduce the surface heating, the energy dissipates less efficiently, which is manifested by reduced convective and evaporative cooling, thereby warming the surface.
Jiaojiao Liu and Xiangjun Shi
Atmos. Chem. Phys., 21, 10609–10624, https://doi.org/10.5194/acp-21-10609-2021, https://doi.org/10.5194/acp-21-10609-2021, 2021
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Cirrus thinning, which reduces the warming effect of cirrus clouds, has been investigated as a new geoengineering approach. In this study, a flexible seeding method is used to exploit the potential cooling effect of cirrus thinning. Simulation results show that the seeding method is essential for estimating the cooling effect. Cirrus thinning with the flexible seeding method could produce a considerable cooling effect, which is much stronger than the fixed seeding method.
Kine Onsum Moseid, Michael Schulz, Trude Storelvmo, Ingeborg Rian Julsrud, Dirk Olivié, Pierre Nabat, Martin Wild, Jason N. S. Cole, Toshihiko Takemura, Naga Oshima, Susanne E. Bauer, and Guillaume Gastineau
Atmos. Chem. Phys., 20, 16023–16040, https://doi.org/10.5194/acp-20-16023-2020, https://doi.org/10.5194/acp-20-16023-2020, 2020
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In this study we compare solar radiation at the surface from observations and Earth system models from 1961 to 2014. We find that the models do not reproduce the so-called
global dimmingas found in observations. Only model experiments with anthropogenic aerosol emissions display any dimming at all. The discrepancies between observations and models are largest in China, which we suggest is in part due to erroneous aerosol precursor emission inventories in the emission dataset used for CMIP6.
Richard J. Bantges, Helen E. Brindley, Jonathan E. Murray, Alan E. Last, Jacqueline E. Russell, Cathryn Fox, Stuart Fox, Chawn Harlow, Sebastian J. O'Shea, Keith N. Bower, Bryan A. Baum, Ping Yang, Hilke Oetjen, and Juliet C. Pickering
Atmos. Chem. Phys., 20, 12889–12903, https://doi.org/10.5194/acp-20-12889-2020, https://doi.org/10.5194/acp-20-12889-2020, 2020
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Understanding how ice clouds influence the Earth's energy balance remains a key challenge for predicting the future climate. These clouds are ubiquitous and are composed of ice crystals that have complex shapes that are incredibly difficult to model. This work exploits new measurements of the Earth's emitted thermal energy made from instruments flown on board an aircraft to test how well the latest ice cloud models can represent these clouds. Results indicate further developments are required.
Nina Črnivec and Bernhard Mayer
Atmos. Chem. Phys., 20, 10733–10755, https://doi.org/10.5194/acp-20-10733-2020, https://doi.org/10.5194/acp-20-10733-2020, 2020
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Unresolved interaction between clouds and atmospheric radiation is a source of uncertainty in weather and climate models. The present study highlights the potential of the state-of-the-art Tripleclouds radiative solver for shallow cumulus clouds, exposing the significance of properly representing subgrid cloud horizontal heterogeneity. The Tripleclouds concept was thereby incorporated in the widely employed δ-Eddington two-stream radiation scheme within the comprehensive libRadtran library.
Allison B. Marquardt Collow, Mark A. Miller, Lynne C. Trabachino, Michael P. Jensen, and Meng Wang
Atmos. Chem. Phys., 20, 10073–10090, https://doi.org/10.5194/acp-20-10073-2020, https://doi.org/10.5194/acp-20-10073-2020, 2020
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Uncertainties in marine boundary layer clouds arise in the presence of biomass burning aerosol, as is the case over the southeast Atlantic Ocean. Heating due to this aerosol has the potential to alter the thermodynamic profile as the aerosol is transported across the Atlantic Ocean. Radiation transfer experiments indicate local shortwave aerosol heating is ~2–8 K d−1; however uncertainties in this quantity exist due to the single-scattering albedo and back trajectories of the aerosol plume.
Christopher J. Smith, Ryan J. Kramer, Gunnar Myhre, Kari Alterskjær, William Collins, Adriana Sima, Olivier Boucher, Jean-Louis Dufresne, Pierre Nabat, Martine Michou, Seiji Yukimoto, Jason Cole, David Paynter, Hideo Shiogama, Fiona M. O'Connor, Eddy Robertson, Andy Wiltshire, Timothy Andrews, Cécile Hannay, Ron Miller, Larissa Nazarenko, Alf Kirkevåg, Dirk Olivié, Stephanie Fiedler, Anna Lewinschal, Chloe Mackallah, Martin Dix, Robert Pincus, and Piers M. Forster
Atmos. Chem. Phys., 20, 9591–9618, https://doi.org/10.5194/acp-20-9591-2020, https://doi.org/10.5194/acp-20-9591-2020, 2020
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The spread in effective radiative forcing for both CO2 and aerosols is narrower in the latest CMIP6 (Coupled Model Intercomparison Project) generation than in CMIP5. For the case of CO2 it is likely that model radiation parameterisations have improved. Tropospheric and stratospheric radiative adjustments to the forcing behave differently for different forcing agents, and there is still significant diversity in how clouds respond to forcings, particularly for total anthropogenic forcing.
Tao Tang, Drew Shindell, Yuqiang Zhang, Apostolos Voulgarakis, Jean-Francois Lamarque, Gunnar Myhre, Camilla W. Stjern, Gregory Faluvegi, and Bjørn H. Samset
Atmos. Chem. Phys., 20, 8251–8266, https://doi.org/10.5194/acp-20-8251-2020, https://doi.org/10.5194/acp-20-8251-2020, 2020
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By using climate simulations, we found that both CO2 and black carbon aerosols could reduce low-level cloud cover, which is mainly due to changes in relative humidity, cloud water, dynamics, and stability. Because the impact of cloud on solar radiation is in effect only during daytime, such cloud reduction could enhance solar heating, thereby raising the daily maximum temperature by 10–50 %, varying by region, which has great implications for extreme climate events and socioeconomic activity.
Tobias Donth, Evelyn Jäkel, André Ehrlich, Bernd Heinold, Jacob Schacht, Andreas Herber, Marco Zanatta, and Manfred Wendisch
Atmos. Chem. Phys., 20, 8139–8156, https://doi.org/10.5194/acp-20-8139-2020, https://doi.org/10.5194/acp-20-8139-2020, 2020
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Solar radiative effects of Arctic black carbon (BC) particles (suspended in the atmosphere and in the surface snowpack) were quantified under cloudless and cloudy conditions. An atmospheric and a snow radiative transfer model were coupled to account for radiative interactions between both compartments. It was found that (i) the warming effect of BC in the snowpack overcompensates for the atmospheric BC cooling effect, and (ii) clouds tend to reduce the atmospheric BC cooling and snow BC warming.
Paul Ockenfuß, Claudia Emde, Bernhard Mayer, and Germar Bernhard
Atmos. Chem. Phys., 20, 1961–1976, https://doi.org/10.5194/acp-20-1961-2020, https://doi.org/10.5194/acp-20-1961-2020, 2020
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We model solar radiation as it would be measured on the Earth's surface in the core shadow of a total solar eclipse. Subsequently, we compare our results to observations during the total eclipse 2017 for ultraviolet, visible and near-infrared wavelengths. Moreover, we analyze the effect of the surface reflectance, the ozone profile, aerosol and the topography and give a visualization of the prevailing photons paths in the atmosphere during the eclipse.
Nina Črnivec and Bernhard Mayer
Atmos. Chem. Phys., 19, 8083–8100, https://doi.org/10.5194/acp-19-8083-2019, https://doi.org/10.5194/acp-19-8083-2019, 2019
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The interaction between radiation and clouds represents a source of uncertainty in numerical weather prediction (NWP), due to both intrinsic problems of one-dimensional radiation schemes and poor representation of clouds. The underlying question addressed in this study is how large the bias is of radiative heating rates in NWP models for shallow cumulus clouds and how it scales with various parameters, such as solar zenith angle, surface albedo, cloud cover and liquid water path.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Rick D. Russotto and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 11905–11925, https://doi.org/10.5194/acp-18-11905-2018, https://doi.org/10.5194/acp-18-11905-2018, 2018
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In simulations with different climate models in which the strength of the Sun is reduced to cancel the surface warming from a quadrupling of atmospheric carbon dioxide, low cloud cover decreases, high cloud cover increases, the upper troposphere and stratosphere cool, and water vapor concentration decreases. The stratospheric cooling and low cloud reduction result in more sunlight reduction being needed than originally thought.
Justyna Lisok, Anna Rozwadowska, Jesper G. Pedersen, Krzysztof M. Markowicz, Christoph Ritter, Jacek W. Kaminski, Joanna Struzewska, Mauro Mazzola, Roberto Udisti, Silvia Becagli, and Izabela Gorecka
Atmos. Chem. Phys., 18, 8829–8848, https://doi.org/10.5194/acp-18-8829-2018, https://doi.org/10.5194/acp-18-8829-2018, 2018
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The aim of the presented study was to investigate the impact on the radiation budget and atmospheric dynamics of a biomass-burning plume, transported from Alaska to the High Arctic region of Ny-Ålesund, Svalbard, in early July 2015. We found that the smoke plume may significantly alter radiative properties of the atmosphere. Furthermore, the simulations of atmospheric dynamics indicated a vertical positive displacement and broadening of the plume with time.
Simon Gruber, Simon Unterstrasser, Jan Bechtold, Heike Vogel, Martin Jung, Henry Pak, and Bernhard Vogel
Atmos. Chem. Phys., 18, 6393–6411, https://doi.org/10.5194/acp-18-6393-2018, https://doi.org/10.5194/acp-18-6393-2018, 2018
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A numerical model also used for operational weather forecast was applied to investigate the impact of contrails and contrail cirrus on the radiative fluxes at the earth's surface. Accounting for contrails produced by aircraft enables the model to simulate high clouds that are otherwise missing. In a case study, we find that the effect of these extra clouds is to reduce the incoming shortwave radiation at the surface as well as the production of photovoltaic power by up to 10 %.
Andrew E. Dessler, Thorsten Mauritsen, and Bjorn Stevens
Atmos. Chem. Phys., 18, 5147–5155, https://doi.org/10.5194/acp-18-5147-2018, https://doi.org/10.5194/acp-18-5147-2018, 2018
Short summary
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One of the most important parameters in climate science is the equilibrium climate sensitivity (ECS). Estimates of this quantity based on 20th-century observations suggest low values of ECS (below 2 °C). We show that these calculations may be significantly in error. Together with other recent work on this problem, it seems probable that the ECS is larger than suggested by the 20th-century observations.
Jake J. Gristey, J. Christine Chiu, Robert J. Gurney, Cyril J. Morcrette, Peter G. Hill, Jacqueline E. Russell, and Helen E. Brindley
Atmos. Chem. Phys., 18, 5129–5145, https://doi.org/10.5194/acp-18-5129-2018, https://doi.org/10.5194/acp-18-5129-2018, 2018
Daniela Meloni, Alcide di Sarra, Gérard Brogniez, Cyrielle Denjean, Lorenzo De Silvestri, Tatiana Di Iorio, Paola Formenti, José L. Gómez-Amo, Julian Gröbner, Natalia Kouremeti, Giuliano Liuzzi, Marc Mallet, Giandomenico Pace, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 18, 4377–4401, https://doi.org/10.5194/acp-18-4377-2018, https://doi.org/10.5194/acp-18-4377-2018, 2018
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This study examines how different aerosol optical properties determine the dust longwave radiative effects at the surface, in the atmosphere and at the top of the atmosphere, based on the combination of remote sensing and in situ observations from the ground, from airborne sensors, and from space, by means of radiative transfer modelling. The closure experiment is based on longwave irradiances and spectral brightness temperatures measured during the 2013 ChArMEx–ADRIMED campaign at Lampedusa.
Netsanet K. Alamirew, Martin C. Todd, Claire L. Ryder, John H. Marsham, and Yi Wang
Atmos. Chem. Phys., 18, 1241–1262, https://doi.org/10.5194/acp-18-1241-2018, https://doi.org/10.5194/acp-18-1241-2018, 2018
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This paper quantifies the radiative effects of dust and water vapour in the Saharan heat low. Dust has a warming effect at the top of the atmosphere while cooling the surface. Water vapour has a warming effect both at the top of atmosphere and the surface. We find dust and water vapour have similar effects in driving the variability in the top-of-atmosphere radiative budget, while dust has a stronger effect than water vapour in controlling day-to-day variability of the surface radiative budget.
Fabian Jakub and Bernhard Mayer
Atmos. Chem. Phys., 17, 13317–13327, https://doi.org/10.5194/acp-17-13317-2017, https://doi.org/10.5194/acp-17-13317-2017, 2017
Short summary
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The formation of shallow cumulus cloud streets was historically attributed primarily to dynamics. Here, we focus on the interaction between radiatively induced surface heterogeneities and the resulting patterns in the flow. Our results suggest that solar radiative heating has the potential to organize clouds perpendicular to the sun's incidence angle.
Cited articles
Baran, A. J.: From the single-scattering properties of ice crystals to
climate prediction: A way forward, Atmos. Res., 112, 45–69,
https://doi.org/10.1016/J.ATMOSRES.2012.04.010, 2012.
Barker, H. W., Kato, S., and Wehr, T.: Computation of Solar Radiative Fluxes by 1D and 3D Methods Using Cloudy Atmospheres Inferred from A-train Satellite Data, Surv. Geophys., 33, 657–676,
https://doi.org/10.1007/s10712-011-9164-9, 2012.
Barker, H. W.: Representing cloud overlap with an effective decorrelation length: An assessment using CloudSat and CALIPSO data, J. Geophys. Res., 113, D24205, https://doi.org/10.1029/2008JD010391, 2008.
Bedka, S. T., Minnis, P., Duda, D. P., Chee, T. L., and Palikonda, R.: Properties of linear contrails in the Northern Hemisphere derived from 2006 Aqua MODIS observations, Geophys. Res. Lett., 40, 772–777, https://doi.org/10.1029/2012GL054363, 2013.
Bickel, M., Ponater, M., Bock, L., Burkhardt, U., and Reineke, S.: Estimating the effective radiative forcing of contrail cirrus, J. Climate, 33, 1991–2005, https://doi.org/10.1175/JCLI-D-19-0467.1, 2020.
Bock, L., and Burkhardt, U.: Reassessing properties and radiative forcing of contrail cirrus using a climate model, J. Geophys. Res.-Atmos., 121, 9717–9736, https://doi.org/10.1002/2016JD025112, 2016.
Bock, L. and Burkhardt, U.: Contrail cirrus radiative forcing for future air traffic, Atmos. Chem. Phys., 19, 8163–8174, https://doi.org/10.5194/acp-19-8163-2019, 2019.
Boeing: Boeing Commercial Market Outlook (2020–2039), available at: https://www.boeing.com/resources/boeingdotcom/market/assets/downloads/2020_CMO_PDF_Download.pdf, last access: 11 October 2020.
Burkhardt, U. and Kärcher, B.: Process-based simulation of contrail cirrus in a global climate model. J. Geophys. Res., 114, D16201, https://doi.org/10.1029/2008JD011491, 2009.
Burkhardt, U. and Kärcher, B.: Global radiative forcing from contrail cirrus, Nat. Clim. Change, 1, 54–58, https://doi.org/10.1038/nclimate1068, 2011.
Burkhardt, U., Bock, L., and Bier, A.: Mitigating the contrail cirrus climate impact by reducing aircraft soot number emissions, NPJ Clim. Atmos. Sci., 1, 37, https://doi.org/10.1038/s41612-018-0046-4, 2018.
Byrnes, S. J.: Multilayer optical calculations, arXiv [preprint], arXiv:1603.02720v2, 28 August 2016.
Caiazzo, F., Agarwal, A., Speth, R. L., and Barrett, S. R. H.: Impact of biofuels on contrail warming, Environ. Res. Lett., 12, 114013,
https://doi.org/10.1088/1748-9326/aa893b, 2017.
Chen, C.-C. and Gettelman, A.: Simulated radiative forcing from contrails and contrail cirrus, Atmos. Chem. Phys., 13, 12525–12536, https://doi.org/10.5194/acp-13-12525-2013, 2013.
Chen, C.-C. and Gettelman, A.: Simulated 2050 aviation radiative forcing from contrails and aerosols, Atmos. Chem. Phys., 16, 7317–7333, https://doi.org/10.5194/acp-16-7317-2016, 2016.
Chou, M., Lee, K., Tsay, S., and Fu, Q.: Parameterization for Cloud Longwave Scattering for Use in Atmospheric Models, J. Climate, 12,
159–169, https://doi.org/10.1175/1520-0442-12.1.159, 1999.
Coakley, J. A. and Chylek, P.: The two-stream approximation in radiative transfer: Including the angle of the incident radiation, J. Atmos. Sci., 32, 409–418, 1975.
Corti, T. and Peter, T.: A simple model for cloud radiative forcing, Atmos. Chem. Phys., 9, 5751–5758, https://doi.org/10.5194/acp-9-5751-2009, 2009.
Costa, S. M. S. and Shine, K. P.: An estimate of the global impact of multiple scattering by clouds on outgoing long-wave radiation, Q. J. Roy. Meteor. Soc., 132, 885–895, https://doi.org/10.1256/qj.05.169, 2006
Davis, A. B. and Marshak, A.: Solar radiation transport in the cloudy atmosphere: a 3D perspective on observations and climate impacts, Reports Prog. Phys., 73, 026801, https://doi.org/10.1088/0034-4885/73/2/026801, 2010.
Davis, S. M., Hegglin, M. I., Fujiwara, M., Dragani, R., Harada, Y., Kobayashi, C., Long, C., Manney, G. L., Nash, E. R., Potter, G. L., Tegtmeier, S., Wang, T., Wargan, K., and Wright, J. S.: Assessment of upper tropospheric and stratospheric water vapor and ozone in reanalyses as part of S-RIP, Atmos. Chem. Phys., 17, 12743–12778, https://doi.org/10.5194/acp-17-12743-2017, 2017.
Dessler, A. E. and Yang, P.: The Distribution of Tropical Thin Cirrus Clouds Inferred from Terra MODIS Data, J. Climate, 16, 1241–1247,
https://doi.org/10.1175/1520-0442(2003)16<1241:TDOTTC>2.0.CO;2, 2003.
Febvre, G., Gayet, J.-F., Minikin, A., Schlager, H., Shcherbakov, V., Jourdan, O., Busen, R., Fiebig, M., Kärcher, B., and Schumann, U.: On optical and microphysical characteristics of contrails and cirrus, J.
Geophys. Res.-Atmos., 114, D02204, https://doi.org/10.1029/2008JD010184, 2009.
Frömming, C., Ponater, M., Burkhardt, U., Stenke, A., Pechtl, S., and Sausen, R.: Sensitivity of contrail coverage and contrail radiative forcing to selected key parameters, Atmos. Environ., 45, 1483–1490, https://doi.org/10.1016/J.ATMOSENV.2010.11.033, 2011.
Fu, Q. and Liou, K. N.: On the correlated k-distribution method for radiative transfer in nonhomogeneous atmospheres, J. Atmos. Sci., 49, 2139–2156, https://doi.org/10.1175/1520-0469(1992)049<2139:OTCDMF>2.0.CO;2, 1992.
Fu, Q. and Liou, K. N.: Parameterization of the Radiative Properties of Cirrus Clouds, J. Atmos. Sci., 50, 2008–2025,
https://doi.org/10.1175/1520-0469(1993)050<2008:POTRPO>2.0.CO;2, 1993.
Fu, Q. A.: An accurate parameterization of the solar radiative properties of cirrus clouds for climate models, J. Climate, 9, 2058–2082, 1996.
Fu, Q., Liou, K. N., Cribb, M., Charlock, T. P., and Grossman, A.: Multiple scattering parameterization in thermal infrared radiative transfer, J. Atmos. Sci., 54, 2799–2812,
https://doi.org/10.1175/1520-0469(1997)054<2799:MSPITI>2.0.CO;2, 1997.
Gayet, J.-F., Shcherbakov, V., Voigt, C., Schumann, U., Schäuble, D., Jessberger, P., Petzold, A., Minikin, A., Schlager, H., Dubovik, O., and Lapyonok, T.: The evolution of microphysical and optical properties of an A380 contrail in the vortex phase, Atmos. Chem. Phys., 12, 6629–6643, https://doi.org/10.5194/acp-12-6629-2012, 2012.
Geleyn, J. F. and Hollingsworth, A.: An economical analytical method for the computation of the interaction between scattering and line absorption of radiation, Beitr. Phys. Atmos., 52, 1–16, 1978.
Gerber, H., Takano, Y., Garrett, T. J., and Hobbs, P. V.:
Nephelometermeasurements of the asymmetry parameter, volume extinction
coefficient, and backscatter ratio in Arctic clouds, J. Atmos. Sci., 57,
3021–3034, 2000.
Gounou, A. and Hogan, R. J.: A sensitivity study of the effect of horizontal photon transport on the radiative forcing of contrails, J. Atmos. Sci., 64, 1706–1716, 2007.
Gu, B.: Evaluations and Improvements of the RRTMG and Fu-Liou Radiative Transfer Model Simulations of Clouds, PhD thesis, Texas A and M University, available at: https://hdl.handle.net/1969.1/189047 (last access:15 November 2020), 2019.
Hanrahan, P. and Krüger, W.: Reflection from layered surfaces due to subsurface scattering. In Proceedings of the 20th annual conference on Computer graphics and interactive techniques (SIGGRAPH '93). Association for Computing Machinery, New York, NY, USA, 165–174, https://doi.org/10.1145/166117.166139, 1993.
Heymsfield, A. J. and Platt, C. M. R.: A Parameterization of
theParticle-Size Spectrum of Ice Clouds in Terms of the Ambient-Temperature
and the Ice Water-Content, J. Atmos. Sci., 41, 846–855, 1984.
Heymsfield, A. J., Lawson, R. P., and Sachse, G. W.: Growth of ice crystals in a precipitating contrail, Geophys. Res. Lett., 25, 1335–1338, https://doi.org/10.1029/98GL00189, 1998.
Heymsfield, A., Winker, D., Avery, M., Vaughan, M., Diskin, G., Deng, M., Mitev, V., and Matthey, R.: Relationsips between ice water content andvolume extinction coefficient from in situ observations for temperatures
from 0∘ to -86∘C: Implications for spaceborne lidar retrievals, J. Appl. Meteorol. Clim., 53, 479–505, 2014.
Hogan, R. J. and Illingworth, A. J.: Deriving cloud overlap statistics from radar, Q. J. Roy. Meteor. Soc., 126, 2903–2909, https://doi.org/10.1002/qj.49712656914, 2000.
Hogan, R. J. and Shonk, J. K. P.: Incorporating the Effects of 3D Radiative Transfer in the Presence of Clouds into Two-Stream Multilayer Radiation Schemes, J. Atmos. Sci., 70, 708–724, https://doi.org/10.1175/JAS-D-12-041.1, 2013.
IPCC 2013 Climate Change: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge and New York, 2013.
Iwabuchi, H., Yang, P., Liou, K. N., and Minnis, P.: Physical and optical properties of persistent contrails: Climatology and interpretation, J. Geophys. Res., 117, D06215, https://doi.org/10.1029/2011JD017020, 2012.
Jiang, J. H., Su, H., Zhai, C., Wu, L., Minschwaner, K., Molod, A. M., and Tompkins, A. M.: An assessment of upper troposphere and lower
stratosphere water vapor in MERRA, MERRA2, and ECMWF reanalyses using Aura
MLS observations, J. Geophys. Res.-Atmos., 120, 11468–11485,
https://doi.org/10.1002/2015JD023752, 2015.
Jourdan, O., Oshchepkov, S., Shcherbakov, V., Gayet, J.-F., and Isaka, H. Assessment of cloud optical parameters in the solar region: Retrievals from airborne measurements of scattering phase functions, J. Geophys. Res., 108, 4572, https://doi.org/10.1029/2003JD003493, 2003.
Kalogirou, S. A.: Solar energy engineering: processes and systems, Elsevier, Academic Press, Burlington, MA, San Diego, CA, London, UK, 2014.
Kärcher, B.: Properties of subvisible cirrus clouds formed by homogeneous freezing, Atmos. Chem. Phys., 2, 161–170, https://doi.org/10.5194/acp-2-161-2002, 2002.
Kärcher, B., Burkhardt, U., Unterstrasser, S., and Minnis, P.: Factors controlling contrail cirrus optical depth, Atmos. Chem. Phys., 9, 6229–6254, https://doi.org/10.5194/acp-9-6229-2009, 2009.
Kärcher, B. and Burkhardt, U.: Effects of optical depth variability on contrail radiative forcing, Q. J. Roy. Meteor. Soc., 139, 1658–1664, https://doi.org/10.1002/qj.2053, 2013.
Kärcher, B.: Formation and radiative forcing of contrail cirrus, Nat. Commun., 9, 1824, https://doi.org/10.1038/s41467-018-04068-0, 2018.
Kato, S., Rose, F. G., and Charlock, T. P.: Computation of Domain-Averaged Irradiance Using Satellite-Derived Cloud Properties, J. Atmos. Ocean. Tech., 22b, 146–164, 2005.
Key, J. R., Yang, P., Baum, B. A., and Nasiri,' S. L.: Parameterization of shortwave ice cloud optical properties for various particle habits, J. Geophys. Res.-Atmos., 107, https://doi.org/10.1029/2001JD000742, 2002.
Kim, Y.-H., Min, S.-K.,Son, S.-W., and Choi, J.: Attribution of the local Hadley cell widening in the Southern Hemisphere, Geophys. Res. Lett., 44, 1015–1024, https://doi.org/10.1002/2016GL072353, 2017.
Kokhanovsky, A.: Optical properties of terrestrial clouds, Earth-Sci. Rev., 64, 189–241, https://doi.org/10.1016/S0012-8252(03)00042-4, 2004.
Lee, D. S., Fahey, D. W., Skowron, A., Allen, M. R., Burkhardt, U., Chen, Q., Doherty, S. J., Freeman, S., Forster, P. M., Fuglestvedt, J., Gettelman, A., De León, R. R., Lim, L. L., Lund, M. T., Millar, R. J., Owen, B., Penner, J. E., Pitari, G., Prather, M. J., Sausen, R., and Wilcox, L. J.: The contribution of global aviation to anthropogenic climate forcing for 2000 to 2018, Atmos. Environ., 244, 117834,
https://doi.org/10.1016/j.atmosenv.2020.117834, 2020.
Liou, K.-N.: Influence of Cirrus Clouds on Weather and Climate Processes: A Global Perspective, Mon. Weather Rev., 114, 1167–1199,
https://doi.org/10.1175/1520-0493(1986)114<1167:IOCCOW>2.0.CO;2, 1986.
Liou, K. N., Yang, P., Takano, Y., Sassen, K., Charlock, T., and Arnott, W.: On the radiative properties of contrail cirrus, Geophys. Res. Lett., 25, 1161–1164, https://doi.org/10.1029/97GL03508, 1998.
Loeb, N. G., Doelling, D. R., Wang, H., Su, W., Nguyen, C., Corbett, J. G., Liang, L., Mitrescu, C., Rose, F. G., and Kato, S.: Clouds and the Earth's Radiant Energy System (CERES) Energy Balanced and Filled (EBAF) Top-of-Atmosphere (TOA) Edition-4.0 Data Product, J. Climate, 31, 895–918, https://doi.org/10.1175/JCLI-D-17-0208.1, 2018.
Lolli, S., Campbell, J. R., Lewis, J. R., Gu, Y., and Welton, E. J.: Technical note: Fu–Liou–Gu and Corti–Peter model performance evaluation for radiative retrievals from cirrus clouds, Atmos. Chem. Phys., 17, 7025–7034, https://doi.org/10.5194/acp-17-7025-2017, 2017.
Marchand, R., Ackerman, T., Smyth, M., and Rossow, W. B.: A review of cloud top height and optical depth histograms from MISR, ISCCP, and MODIS, J. Geophys. Res., 115, D16206, https://doi.org/10.1029/2009JD013422, 2010.
Markowicz, K. M. and Witek, M. L.: Simulations of Contrail Optical
Properties and Radiative Forcing for Various Crystal Shapes, J. Appl. Meteorol. Clim., 50, 1740–1755, https://doi.org/10.1175/2011JAMC2618.1, 2011a.
Markowicz, K. M. and Witek, M.: Sensitivity study of global contrail radiative forcing due to particle shape, J. Geophys. Res., 116, D23203, https://doi.org/10.1029/2011JD016345, 2011b.
Marquart, S., and Mayer, B.: Towards a reliable GCM estimation of contrail radiative forcing, Geophys. Res. Lett., 29, 8, https://doi.org/10.1029/2001GL014075, 2002.
Marquart, S., Ponater, M., Mager, F., and Sausen, R.: Future Development of Contrail Cover, Optical Depth, and Radiative Forcing: Impacts of Increasing Air Traffic and Climate Change, J. Climate, 16, 2890–2904, https://doi.org/10.1175/1520-0442(2003)016<2890:FDOCCO>2.0.CO;2,
2003.
Mayer, B. and Kylling, A.: Technical note: The libRadtran software package for radiative transfer calculations – description and examples of use, Atmos. Chem. Phys., 5, 1855–1877, https://doi.org/10.5194/acp-5-1855-2005, 2005.
Meerkötter, R., Schumann, U., Doelling, D. R., Minnis, P., Nakajima, T., and Tsushima, Y.: Radiative forcing by contrails, Ann. Geophys., 17, 1080–1094, https://doi.org/10.1007/s00585-999-1080-7, 1999.
Minnis, P., Schumann, U., Doelling, D. R., Gierens, K. M., and Fahey, D. W.: Global distribution of contrail radiative forcing, Geophys. Res. Lett., 26, 1853–1856, https://doi.org/10.1029/1999GL900358, 1999.
Minnis, P., Trepte, Q., Sun-Mack, S., Chen, Y., Doelling, D., Young, D., Spangenberg, D., Miller, W., Wielicki, B., Brown, R., Gibson, S., and Geier, E.: Cloud detection in nonpolar regions for CERES using TRMM VIRS and terra and aqua MODIS data, IEEE T. Geosci. Remote, 46, 3857–3884, https://doi.org/10.1109/TGRS.2008.2001351, 2008.
Minnis, P., Bedka, S. T., Duda, D. P., Bedka, K. M., Chee, T., Ayers, J. K., Palikonda, R., Spangenberg, D. A., Khlopenkov, K. V., and Boeke, R.: Linear contrail and contrail cirrus properties determined from satellite data, Geophys. Res. Lett., 40, 3220–3226, https://doi.org/10.1002/grl.50569, 2013.
Myhre, G. and Stordal, F.: On the tradeoff of the solar and thermal infrared radiative impact of contrails, Geophys. Res. Lett., 28, 3119–3122, https://doi.org/10.1029/2001GL013193, 2001.
Myhre, G., Kvalevåg, M., Rädel, G., Cook, J., Shine, K. P., Clark, H., Kärcher, F., Markowicz, K., Kardas, A., Wolkenberg, P., Balkanski, Y., Ponater, M., Forster, P., Rap, A., Leon, R., and Rodriguez: Intercomparison of radiative forcing calculations of stratospheric water vapour and contrails, Meteorol. Z., 18, 585–596,
https://doi.org/10.1127/0941-2948/2009/0411, 2009.
NASA Langley Research Center Atmospheric Science Data Center 2015: CERES SYN1deg Observed Radiative Fluxes and Clouds with Computed Profile Fluxes, dataset, available at: https://ceres.larc.nasa.gov/data/, last access: 5 May 2020.
NASA: Langley Fu and Liou Radiative Transfer Code: model, available at: https://cloudsgate2.larc.nasa.gov/cgi-bin/fuliou/lflcode/accesslfl.cgi,
last access: 15 January 2020.
Nousiainen, T. and McFarquhar, G. M.: Light Scattering by Quasi-Spherical Ice Crystals, J. Atmos. Sci., 61, 2229–2248,
https://doi.org/10.1175/1520-0469(2004)061<2229:LSBQIC>2.0.CO;2, 2004.
Norris, J. R., Allen, R. J., Evan, A. T., Zelinka, M. D., O'Dell, C. W., and Klein, S. A.: Evidence for climate change in the satellite cloud record, Nature, 536, p. 72, https://doi.org/10.1038/nature18273, 2016.
Olsen, S. C., Wuebbles, D. J., and Owen, B.: Comparison of global 3-D aviation emissions datasets, Atmos. Chem. Phys., 13, 429–441, https://doi.org/10.5194/acp-13-429-2013, 2013.
Penner, J. E., Lister, D. H., Griggs, D. J., Dokken, D. J., and McFarland, M.: Aviation and the Global Atmosphere – A Special Report of IPCC Working Groups I and III, Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, 365 pp., 1999.
Ponater, M., Marquart, S., and Sausen, R.: Contrails in a comprehensive global climate model: Parameterization and radiative forcing results, J. Geophys. Res.-Atmos., 107, ACL 2-1–ACL 2-15, https://doi.org/10.1029/2001JD000429, 2002.
Rädel, G. and Shine, K. P.: Radiative forcing by persistent contrails and its dependence on cruise altitudes, J. Geophys. Res.-Atmos., 113, D07105, https://doi.org/10.1029/2007JD009117, 2008.
Rap, A., Forster, P. M., Jones, A., Boucher, O., Haywood, J. M., Bellouin, N., and De Leon, R. R.: Parameterization of contrails in the UK Met Office Climate Model, J. Geophys. Res., 115, D10205, https://doi.org/10.1029/2009JD012443, 2010.
Ritter, B. and Geleyn, J.-F.: A comprehensive radiation scheme for numerical weather prediction models with potential applications in climate simulations, Mon. Weather Rev., 120, 303–325, 1992.
Rose F. G., Charlock, T. P., Fu, Q., Kato, S., Rutan, D. A., and Jin, Z.: CERES Proto-Edition 3 Radiative Transfer: Model Tests
and Radiative Closure Over Surface Validation Sites, Proceedings
12th Conf. on Atmos. Radiation (AMS), P2.4, 10–14 July 2006, Madison, WI, 2006.
Sanz-Morère, I., Eastham, S. D., Speth, R. L., and Barrett, S. R. H.: Reducing Uncertainty in Contrail Radiative Forcing Resulting from
Uncertainty in Ice Crystal Properties, Environ. Sci. Tech. Let., 7, 371–375, https://doi.org/10.1021/acs.estlett.0c00150, 2020.
Sassen, K., Wang, Z., and Liu, D.: Global distribution of cirrus clouds from CloudSat/Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) measurements, J. Geophys. Res., 113, D00A12, https://doi.org/10.1029/2008JD009972, 2008.
Schumann, U.: Influence of propulsion efficiency on contrail formation, Aerosp. Sci. Technol., 4, 391–401, https://doi.org/10.1016/S1270-9638(00)01062-2, 2000.
Schumann, U.: A contrail cirrus prediction model, Geosci. Model Dev., 5, 543–580, https://doi.org/10.5194/gmd-5-543-2012, 2012.
Schumann, U., Mayer, B., Graf, K., and Mannstein, H.: A Parametric Radiative Forcing Model for Contrail Cirrus, J. Appl. Meteorol. Clim., 51, 1391–1406, https://doi.org/10.1175/JAMC-D-11-0242.1, 2012.
Schumann, U. and Graf, K.: Aviation-induced cirrus and radiation changes at diurnal timescales, J. Geophys. Res., 118, 2404–2421,
https://doi.org/10.1002/jgrd.50184, 2013.
Schumann, U., Penner, J. E., Chen, Y., Zhou, C., and Graf, K.: Dehydration effects from contrails in a coupled contrail–climate model, Atmos. Chem. Phys., 15, 11179–11199, https://doi.org/10.5194/acp-15-11179-2015, 2015.
Schumann, U., Baumann, R., Baumgardner, D., Bedka, S. T., Duda, D. P., Freudenthaler, V., Gayet, J.-F., Heymsfield, A. J., Minnis, P., Quante, M., Raschke, E., Schlager, H., Vázquez-Navarro, M., Voigt, C., and Wang, Z.: Properties of individual contrails: a compilation of observations and some comparisons, Atmos. Chem. Phys., 17, 403–438, https://doi.org/10.5194/acp-17-403-2017, 2017.
Schumann, U. and Heymsfield, A. J.: On the Life Cycle of Individual Contrails and Contrail Cirrus, Meteorol. Monogr., 58, 3.1–3.24, https://doi.org/10.1175/AMSMONOGRAPHS-D-16-0005.1, 2017.
Schwarz, M., Folini, D., Yang, S., Allan, R. P., and Wild, M.: Changes in atmospheric shortwave absorption as important driver of dimming and brightening, Nat. Geosci. 13, 110–115, https://doi.org/10.1038/s41561-019-0528-y, 2020.
Simone, N. W., Stettler, M. E. J., and Barrett, S. R. H.: Rapid estimation of global civil aviation emissions with uncertainty quantification, Transp. Res. Pt. D, 25, 33–41, https://doi.org/10.1016/j.trd.2013.07.00, 2013.
Spangenberg, D. A., Minnis, P., Bedka, S. T., Palikonda, R., Duda, D. P., and Rose, F. G.: Contrail radiative forcing over the Northern Hemisphere from 2006 Aqua MODIS data, Geophys. Res. Lett., 40, 595–600, https://doi.org/10.1002/grl.50168, 2013.
Stephens, G. L., Tsay, S. C., Stackhouse, P. W., and Flatau, P. J.: The Relevance of the Microphysical and Radiative Properties of Cirrus Clouds to Climate and Climatic Feedback, J. Atmos. Sci., 47, 1742–1753, 1990.
Stephens, G. L., Gabriel, P. M., and Partain, P. T.: Parameterization of Atmospheric Radiative Transfer. Part I: Validity of Simple Models, J. Atmos. Sci., 58, 3391–3409, https://doi.org/10.1175/1520-0469(2001)058<3391:POARTP>2.0.CO;2, 2001.
Stuber, N. and Forster, P.: The impact of diurnal variations of air traffic on contrail radiative forcing, Atmos. Chem. Phys., 7, 3153–3162, https://doi.org/10.5194/acp-7-3153-2007, 2007.
Tang, G., Yang, P., Kattawar, G. W., Huang, X., Mlawer, E. J., Baum, B. A., and King, M. D.: Improvement of the Simulation of Cloud Longwave Scattering in Broadband Radiative Transfer Models, J. Atmos. Sci., 75, 2217–2233, https://doi.org/10.1175/JAS-D-18-0014.1, 2018.
Tesche, M., Achtert, P., Glantz, P., and Noone, K. J.: Aviation effects on
already-existing cirrus clouds, Nat. Commun., 7, 12016,
https://doi.org/10.1038/ncomms12016, 2016.
Teoh, R., Schumann, U., Majumdar, A., and Stettler, M. E. J.: Mitigating the Climate Forcing of Aircraft Contrails by Small-Scale Diversions and
Technology Adoption, Environ. Sci. Technol., 54, 2941–2950, https://doi.org/10.1021/acs.est.9b05608, 2020.
Voigt, C., Schumann, U., Jessberger, P., Jurkat, T., Petzold, A., Gayet, J.-F., Krämer, M., Thornberry, T., and Fahey, D. W.: Extinction and optical depth of contrails, Geophys. Res. Lett., 38, L11806, https://doi.org/10.1029/2011GL047189, 2011.
Warren, S. G., Hahn, C. H., London, J., Chervin, R. M., and Jenne, R. L.: Global Distribution of Total Cloud Cover and Cloud Type Amounts Over the Ocean, NCAR Technical Note NCAR/TN-317+STR, https://doi.org/10.5065/D6QC01D1, 1988.
Yang, P., Baum, B. A., Heymsfield, A. J., Hu, Y. X., Huang, H.-L., Tsay, S.-C., and Ackerman, S.: Single-scattering properties of droxtals, J. Quant. Spectrosc. Ra., 79–80, 1159–1169,
https://doi.org/10.1016/S0022-4073(02)00347-3, 2003.
Yi, B., Yang, P., Liou, K.‐N., Minnis, P., and Penner, J. E.: Simulation of the global contrail radiative forcing: A sensitivity analysis, Geophys. Res. Lett., 39, L00F03, https://doi.org/10.1029/2012GL054042, 2012.
Short summary
Contrails cause ~50 % of aviation climate impacts, but this is highly uncertain. This is partly due to the effect of overlap between contrails and other cloud layers. We developed a model to quantify this effect, finding that overlap with natural clouds increased contrails' radiative forcing in 2015. This suggests that cloud avoidance may help in reducing aviation's climate impacts. We also find that contrail–contrail overlap reduces impacts by ~3 %, increasing non-linearly with optical depth.
Contrails cause ~50 % of aviation climate impacts, but this is highly uncertain. This is partly...
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