Articles | Volume 17, issue 17
https://doi.org/10.5194/acp-17-10709-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-10709-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
12 Sep 2017
Research article |
| 12 Sep 2017
Atmospheric processes affecting the separation of volcanic ash and SO2 in volcanic eruptions: inferences from the May 2011 Grímsvötn eruption
Visiting scientist, Department of Atmospheric, Oceanic and
Planetary Physics, Clarendon Laboratory, University of Oxford, Oxford, UK
Mark Woodhouse
School of Mathematics, University of Bristol, Clifton, Bristol, UK
Herbert E. Huppert
Institute of Theoretical Geophysics, Department of Applied
Mathematics and Theoretical Physics, University of Cambridge, Cambridge, UK
Andrew Prata
Department of Meteorology, University of Reading, Earley Gate,
Reading, UK
Thor Thordarson
Faculty of Earth Sciences, University of Iceland,
Reykjavik, Iceland
Simon Carn
Department of Geological and Mining Engineering
and Sciences, Michigan Technological University, Houghton, MI, USA
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J. M. Balzani Lööv, B. Alfoldy, L. F. L. Gast, J. Hjorth, F. Lagler, J. Mellqvist, J. Beecken, N. Berg, J. Duyzer, H. Westrate, D. P. J. Swart, A. J. C. Berkhout, J.-P. Jalkanen, A. J. Prata, G. R. van der Hoff, and A. Borowiak
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Sulfur dioxide (SO2), a poisonous gas from human activities and volcanoes, causes air pollution, acid rain, and changes to climate and the ozone layer. Satellites have been used to monitor SO2 globally, including remote areas. Here we describe a new satellite SO2 dataset from the OMPS instrument that flies on the N20 satellite. Results show that the new dataset agrees well with the existing ones from other satellites and can help to continue the global monitoring of SO2 from space.
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Snow-covered terrain, with its high reflectance in the UV, typically enhances satellite sensitivity to boundary layer pollution. However, a significant fraction of high-quality cloud-free measurements over snow is currently excluded from analyses. In this study, we investigated how satellite SO2 measurements over snow-covered surfaces can be used to improve estimations of annual SO2 emissions.
Vitali E. Fioletov, Chris A. McLinden, Debora Griffin, Ihab Abboud, Nickolay Krotkov, Peter J. T. Leonard, Can Li, Joanna Joiner, Nicolas Theys, and Simon Carn
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Sulfur dioxide (SO2) measurements from three satellite instruments were used to update and extend the previously developed global catalogue of large SO2 emission sources. This version 2 of the global catalogue covers the period of 2005–2021 and includes a total of 759 continuously emitting point sources. The catalogue data show an approximate 50 % decline in global SO2 emissions between 2005 and 2021, although emissions were relatively stable during the last 3 years.
David Harning, Thor Thordarson, Áslaug Geirsdóttir, Gifford Miller, and Christopher Florian
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Preprint withdrawn
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Volcanic ash layers are a common tool to synchronize records of past climate, and their estimated age relies on external dating methods. Here, we show that the chemical composition of the well-known, 12000 year-old Vedde Ash is indistinguishable with several other ash layers in Iceland that are ~1000 years younger. Therefore, chemical composition alone cannot be used to identify the Vedde Ash in sedimentary records.
Julia Bruckert, Gholam Ali Hoshyaripour, Ákos Horváth, Lukas O. Muser, Fred J. Prata, Corinna Hoose, and Bernhard Vogel
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Nick Gorkavyi, Nickolay Krotkov, Can Li, Leslie Lait, Peter Colarco, Simon Carn, Matthew DeLand, Paul Newman, Mark Schoeberl, Ghassan Taha, Omar Torres, Alexander Vasilkov, and Joanna Joiner
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The 21 June 2019 eruption of the Raikoke volcano produced significant amounts of volcanic aerosols (sulfate and ash) and sulfur dioxide (SO2) gas that penetrated into the lower stratosphere. We showed that the amount of SO2 decreases with a characteristic period of 8–18 d and the peak of sulfate aerosol lags the initial peak of SO2 by 1.5 months. We also examined the dynamics of an unusual stratospheric coherent circular cloud of SO2 and aerosol observed from 18 July to 22 September 2019.
Lukas O. Muser, Gholam Ali Hoshyaripour, Julia Bruckert, Ákos Horváth, Elizaveta Malinina, Sandra Wallis, Fred J. Prata, Alexei Rozanov, Christian von Savigny, Heike Vogel, and Bernhard Vogel
Atmos. Chem. Phys., 20, 15015–15036, https://doi.org/10.5194/acp-20-15015-2020, https://doi.org/10.5194/acp-20-15015-2020, 2020
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Volcanic aerosols endanger aircraft and thus disrupt air travel globally. For aviation safety, it is vital to know the location and lifetime of such aerosols in the atmosphere. Here we show that the interaction of volcanic particles with each other eventually reduces their atmospheric lifetime. Moreover, we demonstrate that sunlight heats these particles, which lifts them several kilometers in the atmosphere. These findings support a more reliable forecast of volcanic aerosol dispersion.
Can Li, Nickolay A. Krotkov, Peter J. T. Leonard, Simon Carn, Joanna Joiner, Robert J. D. Spurr, and Alexander Vasilkov
Atmos. Meas. Tech., 13, 6175–6191, https://doi.org/10.5194/amt-13-6175-2020, https://doi.org/10.5194/amt-13-6175-2020, 2020
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Sulfur dioxide (SO2) is an important pollutant that causes haze and acid rain. The Ozone Monitoring Instrument (OMI) has been providing global observation of SO2 from space for over 15 years. In this paper, we introduce a new OMI SO2 dataset for global pollution monitoring. The dataset better accounts for the influences of different factors such as location and sun and satellite angles, leading to improved data quality. The new OMI SO2 dataset is publicly available through NASA's data center.
Bradford L. Fisher, Nickolay A. Krotkov, Pawan K. Bhartia, Can Li, Simon A. Carn, Eric Hughes, and Peter J. T. Leonard
Atmos. Meas. Tech., 12, 5137–5153, https://doi.org/10.5194/amt-12-5137-2019, https://doi.org/10.5194/amt-12-5137-2019, 2019
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This article describes a new discrete wavelength algorithm, MS_SO2, which has been used operationally to retrieve global daily volcanic SO2 vertical column densities and the UV volcanic ash index from the Total Ozone Mapping Spectrometer (TOMS) data collected by NASA’s Nimbus-7 satellite from 1978 to 1991. We examine the sensitivity of the algorithm to the detection of SO2, evaluate potential sources of error and compare results from MS_SO2 with the Principal Component Analysis (PCA) algorithm.
Áslaug Geirsdóttir, Gifford H. Miller, John T. Andrews, David J. Harning, Leif S. Anderson, Christopher Florian, Darren J. Larsen, and Thor Thordarson
Clim. Past, 15, 25–40, https://doi.org/10.5194/cp-15-25-2019, https://doi.org/10.5194/cp-15-25-2019, 2019
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Compositing climate proxies in sediment from seven Iceland lakes documents abrupt summer cooling between 4.5 and 4.0 ka, statistically indistinguishable from 4.2 ka. Although the decline in summer insolation was an important factor, a combination of superposed changes in ocean circulation and explosive Icelandic volcanism were likely responsible for the abrupt perturbation recorded by our proxies. Lake and catchment proxies recovered to a colder equilibrium state following the perturbation.
Claudia Timmreck, Graham W. Mann, Valentina Aquila, Rene Hommel, Lindsay A. Lee, Anja Schmidt, Christoph Brühl, Simon Carn, Mian Chin, Sandip S. Dhomse, Thomas Diehl, Jason M. English, Michael J. Mills, Ryan Neely, Jianxiong Sheng, Matthew Toohey, and Debra Weisenstein
Geosci. Model Dev., 11, 2581–2608, https://doi.org/10.5194/gmd-11-2581-2018, https://doi.org/10.5194/gmd-11-2581-2018, 2018
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The paper describes the experimental design of the Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP). ISA-MIP will improve understanding of stratospheric aerosol processes, chemistry, and dynamics and constrain climate impacts of background aerosol variability and small and large volcanic eruptions. It will help to asses the stratospheric aerosol contribution to the early 21st century global warming hiatus period and the effects from hypothetical geoengineering schemes.
Pieternel F. Levelt, Joanna Joiner, Johanna Tamminen, J. Pepijn Veefkind, Pawan K. Bhartia, Deborah C. Stein Zweers, Bryan N. Duncan, David G. Streets, Henk Eskes, Ronald van der A, Chris McLinden, Vitali Fioletov, Simon Carn, Jos de Laat, Matthew DeLand, Sergey Marchenko, Richard McPeters, Jerald Ziemke, Dejian Fu, Xiong Liu, Kenneth Pickering, Arnoud Apituley, Gonzalo González Abad, Antti Arola, Folkert Boersma, Christopher Chan Miller, Kelly Chance, Martin de Graaf, Janne Hakkarainen, Seppo Hassinen, Iolanda Ialongo, Quintus Kleipool, Nickolay Krotkov, Can Li, Lok Lamsal, Paul Newman, Caroline Nowlan, Raid Suleiman, Lieuwe Gijsbert Tilstra, Omar Torres, Huiqun Wang, and Krzysztof Wargan
Atmos. Chem. Phys., 18, 5699–5745, https://doi.org/10.5194/acp-18-5699-2018, https://doi.org/10.5194/acp-18-5699-2018, 2018
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The aim of this paper is to highlight the many successes of the Ozone Monitoring Instrument (OMI) spanning more than 13 years. Data from OMI have been used in a wide range of applications. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. OMI data continue to be used for new research and applications.
Georgina M. Miles, Richard Siddans, Roy G. Grainger, Alfred J. Prata, Bradford Fisher, and Nickolay Krotkov
Atmos. Meas. Tech., 10, 2687–2702, https://doi.org/10.5194/amt-10-2687-2017, https://doi.org/10.5194/amt-10-2687-2017, 2017
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Volcanic eruptions are important in the way they perturb the climate and help us understand atmospheric processes. We show a new method to measure the SO2 released by explosive volcanic eruptions using the HIRS/2 satellite instrument, which measured atmospheric temperature and H2O. We apply the technique to the 1991 eruption of Cerro Hudson and show it is possible to detect SO2 with a good degree of accuracy. This method and instrument can potentially generate a climate-significant record.
Can Li, Nickolay A. Krotkov, Simon Carn, Yan Zhang, Robert J. D. Spurr, and Joanna Joiner
Atmos. Meas. Tech., 10, 445–458, https://doi.org/10.5194/amt-10-445-2017, https://doi.org/10.5194/amt-10-445-2017, 2017
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In this paper, we describe the new-generation OMI volcanic SO2 algorithm based on our principal component analysis (PCA) retrieval technique. We demonstrate significant improvement in the our new OMI volcanic SO2 data, with the retrieval noise reduced by a factor of 2 as compared with the previous dataset. The algorithm also improves the accuracy for large volcanic eruptions. It is also capable of producing consistent retrievals between different instruments.
Guangliang Fu, Fred Prata, Hai Xiang Lin, Arnold Heemink, Arjo Segers, and Sha Lu
Atmos. Chem. Phys., 17, 1187–1205, https://doi.org/10.5194/acp-17-1187-2017, https://doi.org/10.5194/acp-17-1187-2017, 2017
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A Satellite Observational Operator (SOO) is proposed to translates satellite-retrieved 2-D volcanic ash mass loadings to 3-D concentrations. The SOO makes the analysis step of assimilation comparable in the 3-D model space, and thus it avoids the artificial vertical correlations by not involving the integral operator in directly assimilating 2-D data. The results show that satellite data assimilation with SOO can efficiently improve the estimate of volcanic ash state and the forecast.
Verity J. B. Flower, Thomas Oommen, and Simon A. Carn
Atmos. Meas. Tech., 9, 5487–5498, https://doi.org/10.5194/amt-9-5487-2016, https://doi.org/10.5194/amt-9-5487-2016, 2016
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Volcanic eruptions pose a threat to human populations around the globe, but many active volcanoes are poorly monitored. This paper details the development of an automated volcanic plume detection method with focus on diffuse plumes, utilising daily, global observations of volcanic gases measured by satellites. The developed technique consistently distinguished volcanic plumes over 400 t, from control samples, indicating the potential for implementation within a volcanic alert system.
Vitali E. Fioletov, Chris A. McLinden, Nickolay Krotkov, Can Li, Joanna Joiner, Nicolas Theys, Simon Carn, and Mike D. Moran
Atmos. Chem. Phys., 16, 11497–11519, https://doi.org/10.5194/acp-16-11497-2016, https://doi.org/10.5194/acp-16-11497-2016, 2016
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We introduce the first space-based catalogue of SO2 emission sources seen by OMI. The inventory contains about 500 sources. They account for about a half of all SO2 emissions; the remaining half is likely related to sources emitting less than 30 kt yr−1 and not detected by OMI. The sources are grouped by type (volcanoes, power plants, oil- and gas-related sources, and smelters) and country. The catalogue presented herein can be used for verification of available SO2 emission inventories.
J. A. Stevenson, S. C. Millington, F. M. Beckett, G. T. Swindles, and T. Thordarson
Atmos. Meas. Tech., 8, 2069–2091, https://doi.org/10.5194/amt-8-2069-2015, https://doi.org/10.5194/amt-8-2069-2015, 2015
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We attempt to understand why volcanic ash grains found 100s of km from their source volcanoes (cryptotephra), which are typically 20–125 microns in length, are much larger than the size distributions measured by satellite remote sensing, which are centred at less than 10 microns. Our observations and models show that cryptotephra-sized grains are to be expected in distal plumes. Retrievals of effective radius made on simulated satellite images are shown to be biased toward smaller values.
J. M. Balzani Lööv, B. Alfoldy, L. F. L. Gast, J. Hjorth, F. Lagler, J. Mellqvist, J. Beecken, N. Berg, J. Duyzer, H. Westrate, D. P. J. Swart, A. J. C. Berkhout, J.-P. Jalkanen, A. J. Prata, G. R. van der Hoff, and A. Borowiak
Atmos. Meas. Tech., 7, 2597–2613, https://doi.org/10.5194/amt-7-2597-2014, https://doi.org/10.5194/amt-7-2597-2014, 2014
H. Brenot, N. Theys, L. Clarisse, J. van Geffen, J. van Gent, M. Van Roozendael, R. van der A, D. Hurtmans, P.-F. Coheur, C. Clerbaux, P. Valks, P. Hedelt, F. Prata, O. Rasson, K. Sievers, and C. Zehner
Nat. Hazards Earth Syst. Sci., 14, 1099–1123, https://doi.org/10.5194/nhess-14-1099-2014, https://doi.org/10.5194/nhess-14-1099-2014, 2014
J. Wang, S. Park, J. Zeng, C. Ge, K. Yang, S. Carn, N. Krotkov, and A. H. Omar
Atmos. Chem. Phys., 13, 1895–1912, https://doi.org/10.5194/acp-13-1895-2013, https://doi.org/10.5194/acp-13-1895-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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The emission, transport, and impacts of the extreme Saharan dust storm of 2015
California wildfire smoke contributes to a positive atmospheric temperature anomaly over the western United States
Dust storms from the Taklamakan Desert significantly darken snow surface on surrounding mountains
Opposite effects of aerosols and meteorological parameters on warm clouds in two contrasting regions over eastern China
Effect of wind speed on marine aerosol optical properties over remote oceans with use of spaceborne lidar observations
Assessment of smoke plume height products derived from multisource satellite observations using lidar-derived height metrics for wildfires in the western US
A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations
Opinion: Aerosol remote sensing over the next 20 years
Monitoring biomass burning aerosol transport using CALIOP observations and reanalysis models: a Canadian wildfire event in 2019
Thermal infrared observations of a western United States biomass burning aerosol plume
A new look into the impacts of dust radiative effects on the energetics of tropical easterly waves
Wind-driven emissions of coarse-mode particles in an urban environment
Measurement report: Dust and anthropogenic aerosols' vertical distributions over northern China dense aerosols gathered at the top of the mixing layer
Climatological assessment of the vertically resolved optical and microphysical aerosol properties by lidar measurements, sun photometer, and in situ observations over 17 years at Universitat Politècnica de Catalunya (UPC) Barcelona
Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments
Impact of assimilating NOAA VIIRS aerosol optical depth (AOD) observations on global AOD analysis from the Copernicus Atmosphere Monitoring Service (CAMS)
Spectral dependence of birch and pine pollen optical properties using a synergy of lidar instruments
Validation activities of Aeolus wind products on the southeastern Iberian Peninsula
Thermal infrared dust optical depth and coarse-mode effective diameter over oceans retrieved from collocated MODIS and CALIOP observations
A comprehensive reappraisal of long-term aerosol characteristics, trends, and variability in Asia
Satellite (GOSAT-2 CAI-2) retrieval and surface (ARFINET) observations of aerosol black carbon over India
Spatiotemporal variation characteristics of global fires and their emissions
The (mis)identification of high-latitude dust events using remote sensing methods in the Yukon, Canada: a sub-daily variability analysis
Comparison of dust optical depth from multi-sensor products and MONARCH (Multiscale Online Non-hydrostatic AtmospheRe CHemistry) dust reanalysis over North Africa, the Middle East, and Europe
Understanding day–night differences in dust aerosols over the dust belt of North Africa, the Middle East, and Asia
Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
Abdulamid A. Fakoya, Jens Redemann, Pablo E. Saide, Lan Gao, Logan T. Mitchell, Calvin Howes, Amie Dobracki, Ian Chang, Gonzalo A. Ferrada, Kristina Pistone, Samuel E. Leblanc, Michal Segal-Rozenhaimer, Arthur J. Sedlacek III, Thomas Eck, Brent Holben, Pawan Gupta, Elena Lind, Paquita Zuidema, Gregory Carmichael, and Connor J. Flynn
Atmos. Chem. Phys., 25, 7879–7902, https://doi.org/10.5194/acp-25-7879-2025, https://doi.org/10.5194/acp-25-7879-2025, 2025
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Tiny atmospheric particles from wildfire smoke impact the climate by interacting with sunlight and clouds, the extent of which is uncertain due to gaps in understanding how smoke changes over time. We developed a new method using remote sensing instruments to track how these particles evolve during atmospheric transport. Our results show that the ability of these particles to absorb sunlight increases as they travel. This discovery could help improve predictions of future climate scenarios.
Moritz Haarig, Ronny Engelmann, Holger Baars, Benedikt Gast, Dietrich Althausen, and Albert Ansmann
Atmos. Chem. Phys., 25, 7741–7763, https://doi.org/10.5194/acp-25-7741-2025, https://doi.org/10.5194/acp-25-7741-2025, 2025
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The lidar ratio is an important quantity in aerosol typing. Its spectral slope contains information about the source region or transport paths of the observed aerosol. The extension to 1064 nm is a recent development led by our institute. We gathered previous observations and added new ones to provide the spectral slope for the most important aerosol types such as marine and continental aerosol, dust, smoke, and sulfate. We compared it to assumptions used for spaceborne backscatter lidars.
Chanyoung Park, Brian J. Soden, Ryan J. Kramer, Tristan S. L'Ecuyer, and Haozhe He
Atmos. Chem. Phys., 25, 7299–7313, https://doi.org/10.5194/acp-25-7299-2025, https://doi.org/10.5194/acp-25-7299-2025, 2025
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This study addresses the long-standing challenge of quantifying the impact of aerosol–cloud interactions. Using satellite observations, reanalysis data, and a "perfect-model" cross-validation, we show that explicitly accounting for aerosol–cloud droplet activation rates is key to accurately estimating ERFaci (effective radiative forcing due to aerosol–cloud interactions). Our results indicate a smaller and less uncertain ERFaci than previously assessed, implying the reduced role of aerosol–cloud interactions in shaping climate sensitivity.
Xin Xi, Jun Wang, Zhendong Lu, Andrew M. Sayer, Jaehwa Lee, Robert C. Levy, Yujie Wang, Alexei Lyapustin, Hongqing Liu, Istvan Laszlo, Changwoo Ahn, Omar Torres, Sabur Abdullaev, James Limbacher, and Ralph A. Kahn
Atmos. Chem. Phys., 25, 7403–7429, https://doi.org/10.5194/acp-25-7403-2025, https://doi.org/10.5194/acp-25-7403-2025, 2025
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The Aralkum Desert is challenging for aerosol retrieval due to its bright, heterogeneous, and dynamic surfaces and the lack of in situ constraints on aerosol properties. The performance and consistency of satellite algorithms in observing Aralkum-generated saline dust remain unknown. This study compares multisensor UVAI (ultraviolet aerosol index), AOD (aerosol optical depth), and ALH (aerosol layer height) products and reveals inconsistencies and potential biases over the Aral Sea basin.
Yuyang Chang, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, Igor Veselovskii, Fabrice Ducos, Gaël Dubois, Masanori Saito, Anton Lopatin, Oleg Dubovik, and Cheng Chen
Atmos. Chem. Phys., 25, 6787–6821, https://doi.org/10.5194/acp-25-6787-2025, https://doi.org/10.5194/acp-25-6787-2025, 2025
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Our study retrieved dust aerosol microphysical properties from lidar measurements using different scattering models. Numeric simulations and real data applications revealed the importance of considering depolarization measurements and the superiority of the irregular–hexahedral model in the retrieval of dust aerosols from lidar measurements.
Jens Reichardt, Felix Lauermann, and Oliver Behrendt
Atmos. Chem. Phys., 25, 5857–5892, https://doi.org/10.5194/acp-25-5857-2025, https://doi.org/10.5194/acp-25-5857-2025, 2025
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Optical remote sensing systems, so-called lidars, are used to learn more about aerosols, which play an important role in atmospheric processes. The present study demonstrates that lidars, which measure the backscattering behavior of aerosols over the entire visible wavelength range, can increase our knowledge of the spatial and temporal occurrence of aerosol layers, the type of aerosol, and their interaction with clouds. The focus of the publication is on wildfire aerosol and Saharan dust.
Meloë S. F. Kacenelenbogen, Ralph Kuehn, Nandana Amarasinghe, Kerry Meyer, Edward Nowottnick, Mark Vaughan, Hong Chen, Sebastian Schmidt, Richard Ferrare, John Hair, Robert Levy, Hongbin Yu, Paquita Zuidema, Robert Holz, and Willem Marais
EGUsphere, https://doi.org/10.5194/egusphere-2025-1403, https://doi.org/10.5194/egusphere-2025-1403, 2025
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Aerosols perturb the radiation balance of the Earth-atmosphere system. To reduce the uncertainty in quantifying present-day climate change, we combine two satellite sensors and a model to assess the aerosol effects on radiation in all-sky conditions. Satellite-based and coincident aircraft measurements of aerosol radiative effects agree well over the Southeast Atlantic. This constitutes a crucial first evaluation before we apply our method to more years and regions of the world.
Benedikt Gast, Cristofer Jimenez, Albert Ansmann, Moritz Haarig, Ronny Engelmann, Felix Fritzsch, Athena A. Floutsi, Hannes Griesche, Kevin Ohneiser, Julian Hofer, Martin Radenz, Holger Baars, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 25, 3995–4011, https://doi.org/10.5194/acp-25-3995-2025, https://doi.org/10.5194/acp-25-3995-2025, 2025
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In this study, we discuss the enhanced detection capabilities of a fluorescence lidar in the case of optically thin aerosol layers in the upper troposphere and lower stratosphere (UTLS) region. Our results suggest that such thin aerosol layers are not so rare in the UTLS and can potentially trigger and impact cirrus cloud formation through heterogeneous ice nucleation. By altering the microphysical cloud properties, this could affect clouds' evolution and lifetime and thus their climate effect.
Qiaomin Pei, Chuanfeng Zhao, Yikun Yang, Annan Chen, Zhiyuan Cong, Xin Wan, Haotian Zhang, and Guangming Wu
EGUsphere, https://doi.org/10.5194/egusphere-2025-1172, https://doi.org/10.5194/egusphere-2025-1172, 2025
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This study investigates smoke's impact on atmospheric warming over the Himalayan and Tibetan Plateau (HTP) using MODIS fire data, ground-based and satellite aerosol observations, and model simulations. It finds that smoke aerosols – predominantly concentrated between 6 and 8 km in the mid-troposphere over southern HTP – likely alter regional atmospheric stability by modifying the vertical temperature profile, as indicated by a reduced lapse rate.
Marion Ranaivombola, Nelson Bègue, Lucas Vaz Peres, Farahnaz Fazel-Rastgar, Venkataraman Sivakumar, Gisèle Krysztofiak, Gwenaël Berthet, Fabrice Jegou, Stuart Piketh, and Hassan Bencherif
Atmos. Chem. Phys., 25, 3519–3540, https://doi.org/10.5194/acp-25-3519-2025, https://doi.org/10.5194/acp-25-3519-2025, 2025
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From September to October 2022, the Biomass Burning Aerosol Campaign (BiBAC) in Kruger National Park revealed a significant aerosol loading linked to biomass burning activity, with southeastward transport over southern Africa and the southwestern Indian Ocean (SWIO) basin. The study revealed a predominance of biomass burning aerosols and two distinct transport mechanisms of aerosol plumes and CO, underscoring the importance of east-coast observations in understanding atmospheric dynamics.
Zirui Zhang, Kaiming Huang, Fan Yi, Wei Cheng, Fuchao Liu, Jian Zhang, and Yue Jia
Atmos. Chem. Phys., 25, 3347–3361, https://doi.org/10.5194/acp-25-3347-2025, https://doi.org/10.5194/acp-25-3347-2025, 2025
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The height of the convective boundary layer (CBLH) is related to our health due to its crucial role in pollutant dispersion. The variance of vertical velocity from millimeter wave cloud radar (MMCR) can accurately capture the diurnal evolution of the CBLH, due to a small blind range and less impact by the residual layer. The CBLH is affected by radiation, humidity, cloud, and precipitation; thus, the MMCR is suitable for monitoring the CBLH, owing to its observation capability in various weather conditions.
Cheng Fan, Gerrit de Leeuw, Xiaoxi Yan, Jiantao Dong, Hanqing Kang, Chengwei Fang, Zhengqiang Li, and Ying Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2025-880, https://doi.org/10.5194/egusphere-2025-880, 2025
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This study describes the analysis of time series of the MODIS-derived Aerosol Optical Depth (AOD) over China between 2010 and 2024. Emission reduction policy has been effective in reducing the AOD until 2018. Thereafter the overall reduction until the end of the study was very small due to unfavorable meteorological factors cancelling favorable anthropogenic effects which resulted in AOD increase during extended periods. The variations over different areas in China are discussed.
Agnieszka Czerwińska, Janusz Krzyścin, Janusz Jarosławski, Piotr S. Sobolewski, and Aleksander Pietruczuk
EGUsphere, https://doi.org/10.5194/egusphere-2025-1129, https://doi.org/10.5194/egusphere-2025-1129, 2025
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Excessive levels of ultraviolet solar radiation at the Earth's surface have been linked to several types of skin cancer. The world's longest record of solar radiation intensities causing harmful skin redness comes from observations at Belsk, Poland, between 1976 and 2023. In this century, the intensity of such radiation is stable, but 15 % higher than in the 1970s. This trend is due to the combined effects of a decrease in stratospheric ozone and an increase in cloud transparency before 2000.
Igor Veselovskii, Mikhail Korenskiy, Nikita Kasianik, Boris Barchunov, Qiaoyun Hu, Philippe Goloub, and Thierry Podvin
Atmos. Chem. Phys., 25, 1603–1615, https://doi.org/10.5194/acp-25-1603-2025, https://doi.org/10.5194/acp-25-1603-2025, 2025
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A fluorescence lidar was used to study transported Canadian smoke in May–September 2023. The fluorescence measurements were taken at five wavelengths. The results revealed that fluorescence capacity increases with altitude, suggesting a higher concentration of organic compounds in the upper troposphere and lower stratosphere than in the lower troposphere. The fluorescence spectra peaked in the 513 and 560 nm channels in smoke layers but decreased with wavelength in urban aerosols.
Maria Filioglou, Petri Tiitta, Xiaoxia Shang, Ari Leskinen, Pasi Ahola, Sanna Pätsi, Annika Saarto, Ville Vakkari, Uula Isopahkala, and Mika Komppula
Atmos. Chem. Phys., 25, 1639–1657, https://doi.org/10.5194/acp-25-1639-2025, https://doi.org/10.5194/acp-25-1639-2025, 2025
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Every year a vast number of people experience allergic reactions due to exposure to airborne pollen. These symptoms are concentration dependent; thus accurate information about the pollen load in the atmosphere is essential. Moreover, pollen grains and fragments of it are likely to contribute to cloud processes and suppress precipitation. Here, we estimate the concentration and cloud-relevant parameters of birch pollen in the atmosphere using observations from a PollyXT and a CL61 ceilometer.
Blake T. Sorenson, Jianglong Zhang, Jeffrey S. Reid, and Peng Xian
EGUsphere, https://doi.org/10.5194/egusphere-2025-80, https://doi.org/10.5194/egusphere-2025-80, 2025
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Plumes of wildfire smoke in the Arctic affect the Arctic radiative budget. Using a neural network and observations from satellite-based sensors, we analyzed the direct radiative forcing of smoke particles on the Arctic climate and estimated long-term forcing trends. Strong negative trends in aerosol direct radiative forcing were found in northern Russia and Canada, with positive trends found over parts of the Arctic Ocean. Overall, smoke plumes may act to counter future Arctic warming.
Fengjiao Chen, Yuanjian Yang, Lu Yu, Yang Li, Weiguang Liu, Yan Liu, and Simone Lolli
Atmos. Chem. Phys., 25, 1587–1601, https://doi.org/10.5194/acp-25-1587-2025, https://doi.org/10.5194/acp-25-1587-2025, 2025
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The microphysical mechanisms of precipitation responsible for the varied impacts of aerosol particles on shallow precipitation remain unclear. This study reveals that coarse aerosol particles invigorate shallow rainfall through enhanced coalescence processes, whereas fine aerosol particles suppress shallow rainfall through intensified microphysical breaks. These impacts are independent of thermodynamic environments but are more significant in low-humidity conditions.
Sohee Joo, Juseon Shin, Matthias Tesche, Naghmeh Dehkhoda, Taegyeong Kim, and Youngmin Noh
Atmos. Chem. Phys., 25, 1023–1036, https://doi.org/10.5194/acp-25-1023-2025, https://doi.org/10.5194/acp-25-1023-2025, 2025
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In our study, we investigated why, in northeast Asia, visibility has not improved even though air pollution levels have decreased. By examining trends in Seoul and Ulsan, we found that the particles in the air are getting smaller, which scatters light more effectively and reduces how far we can see. Our findings suggest that changes in particle properties adversely affected public perception of air quality improvement even though the PM2.5 mass concentration is continuously decreasing.
Norman T. O'Neill, Keyvan Ranjbar, Liviu Ivănescu, Yann Blanchard, Seyed Ali Sayedain, and Yasmin AboEl-Fetouh
Atmos. Chem. Phys., 25, 27–44, https://doi.org/10.5194/acp-25-27-2025, https://doi.org/10.5194/acp-25-27-2025, 2025
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Dust from mid-latitude deserts or from local drainage basins is a weak component of atmospheric aerosols in the Arctic. Satellite-based dust estimates are often overestimated because dust and cloud measurements can be confused. Illustrations are given with an emphasis on the flawed claim that a classic indicator of dust (negative brightness temperature differences) is proof of the presence of airborne Arctic dust. Low-altitude warm-water plumes are the likely source of such negative values.
Saleem Ali, Chandan Sarangi, and Sanjay Kumar Mehta
EGUsphere, https://doi.org/10.5194/egusphere-2024-3093, https://doi.org/10.5194/egusphere-2024-3093, 2024
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The pollutants over Northern India are transported towards South India under the influence of the prevalent wind system, especially during winter. This long-range transport induces a widespread haziness over southern India, lasting for days. We evaluated the occurrence of such transport episodes over south India using observational methods and found that it suppresses the boundary layer height by ~38 % compared to the clear days while exacerbating the surface pollution by ~30–35 %.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Julian Hofer, Moritz Haarig, Ulla Wandinger, Bernd Heinold, Ina Tegen, Matthias Faust, Holger Baars, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
EGUsphere, https://doi.org/10.5194/egusphere-2024-3159, https://doi.org/10.5194/egusphere-2024-3159, 2024
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This study investigates how hematite (an iron oxide mineral) in the Saharan Desert dust affects how dust particles interact with radiation. Using lidar data from Cabo Verde (2021–2022) and hematite content from atmospheric model simulations, the results show that higher hematite fraction leads to stronger particle backscattering at specific wavelengths. These findings can improve the representaiton of mineral dust in climate models, particularly regarding their radiative effect.
Perla Alalam, Fabrice Ducos, and Hervé Herbin
Atmos. Chem. Phys., 24, 12277–12294, https://doi.org/10.5194/acp-24-12277-2024, https://doi.org/10.5194/acp-24-12277-2024, 2024
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This study dives into the impact of mineral dust laboratory complex refractive indices (CRIs) on quantifying the dust microphysical properties using satellite infrared remote sensing. Results show that using CRIs obtained by advanced realistic techniques can improve the accuracy of these measurements, emphasizing the importance of choosing the suitable CRI in atmospheric models. This improvement is crucial for better predicting the dust radiative effect and impact on the climate.
Nabia Gulistan, Khan Alam, and Yangang Liu
Atmos. Chem. Phys., 24, 11333–11349, https://doi.org/10.5194/acp-24-11333-2024, https://doi.org/10.5194/acp-24-11333-2024, 2024
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This study looks at the influence of aerosol and meteorology on precipitating and non-precipitating clouds over the Indo-Gangetic Plain (IGP). A major finding of this study was that the high loading of aerosols led to a high occurrence of precipitating clouds under unstable conditions in summer. The study has the potential to open a new avenue for the scientific community to further explore and understand the complications of aerosol–cloud–precipitation over the complex topography of the IGP.
Myungje Choi, Alexei Lyapustin, Gregory L. Schuster, Sujung Go, Yujie Wang, Sergey Korkin, Ralph Kahn, Jeffrey S. Reid, Edward J. Hyer, Thomas F. Eck, Mian Chin, David J. Diner, Olga Kalashnikova, Oleg Dubovik, Jhoon Kim, and Hans Moosmüller
Atmos. Chem. Phys., 24, 10543–10565, https://doi.org/10.5194/acp-24-10543-2024, https://doi.org/10.5194/acp-24-10543-2024, 2024
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This paper introduces a retrieval algorithm to estimate two key absorbing components in smoke (black carbon and brown carbon) using DSCOVR EPIC measurements. Our analysis reveals distinct smoke properties, including spectral absorption, layer height, and black carbon and brown carbon, over North America and central Africa. The retrieved smoke properties offer valuable observational constraints for modeling radiative forcing and informing health-related studies.
Brian Harr, Bing Pu, and Qinjian Jin
Atmos. Chem. Phys., 24, 8625–8651, https://doi.org/10.5194/acp-24-8625-2024, https://doi.org/10.5194/acp-24-8625-2024, 2024
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We found that the formation of the extreme trans-Atlantic African dust event in June 2015 was associated with a brief surge in dust emissions over western North Africa and extreme circulation patterns, including intensified easterly jets, which facilitated the westward transport of dust. The dust plume modified radiative flux along its transport pathway but had minor impacts on air quality in the US due to the record-high Caribbean low-level jet advecting part of the plume to the Pacific.
James L. Gomez, Robert J. Allen, and King-Fai Li
Atmos. Chem. Phys., 24, 6937–6963, https://doi.org/10.5194/acp-24-6937-2024, https://doi.org/10.5194/acp-24-6937-2024, 2024
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Wildfires in California (CA) have grown very large during the past 20 years. These fires emit sunlight-absorbing aerosols. Analyzing observational data, our study finds that aerosols emitted from large fires in northern CA spread throughout CA and Nevada and heat the atmosphere. This heating is consistent with larger-than-normal temperatures and dry conditions. Further study is needed to determine how much the aerosols heat the atmosphere and whether they are drying the atmosphere as well.
Yuxuan Xing, Yang Chen, Shirui Yan, Xiaoyi Cao, Yong Zhou, Xueying Zhang, Tenglong Shi, Xiaoying Niu, Dongyou Wu, Jiecan Cui, Yue Zhou, Xin Wang, and Wei Pu
Atmos. Chem. Phys., 24, 5199–5219, https://doi.org/10.5194/acp-24-5199-2024, https://doi.org/10.5194/acp-24-5199-2024, 2024
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This study investigated the impact of dust storms from the Taklamakan Desert on surrounding high mountains and regional radiation balance. Using satellite data and simulations, researchers found that dust storms significantly darken the snow surface in the Tien Shan, Kunlun, and Qilian mountains, reaching mountains up to 1000 km away. This darkening occurs not only in spring but also during summer and autumn, leading to increased absorption of solar radiation.
Yuqin Liu, Tao Lin, Jiahua Zhang, Fu Wang, Yiyi Huang, Xian Wu, Hong Ye, Guoqin Zhang, Xin Cao, and Gerrit de Leeuw
Atmos. Chem. Phys., 24, 4651–4673, https://doi.org/10.5194/acp-24-4651-2024, https://doi.org/10.5194/acp-24-4651-2024, 2024
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A new method, the geographical detector method (GDM), has been applied to satellite data, in addition to commonly used statistical methods, to study the sensitivity of cloud properties to aerosol over China. Different constraints for aerosol and cloud liquid water path apply over polluted and clean areas. The GDM shows that cloud parameters are more sensitive to combinations of parameters than to individual parameters, but confounding effects due to co-variation of parameters cannot be excluded.
Kangwen Sun, Guangyao Dai, Songhua Wu, Oliver Reitebuch, Holger Baars, Jiqiao Liu, and Suping Zhang
Atmos. Chem. Phys., 24, 4389–4409, https://doi.org/10.5194/acp-24-4389-2024, https://doi.org/10.5194/acp-24-4389-2024, 2024
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This paper investigates the correlation between marine aerosol optical properties and wind speeds over remote oceans using the spaceborne lidars ALADIN and CALIOP. Three remote ocean areas are selected. Pure marine aerosol optical properties at 355 nm are derived from ALADIN. The relationships between marine aerosol optical properties and wind speeds are analyzed within and above the marine atmospheric boundary layer, revealing the effect of wind speed on marine aerosols over remote oceans.
Jingting Huang, S. Marcela Loría-Salazar, Min Deng, Jaehwa Lee, and Heather A. Holmes
Atmos. Chem. Phys., 24, 3673–3698, https://doi.org/10.5194/acp-24-3673-2024, https://doi.org/10.5194/acp-24-3673-2024, 2024
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Increased wildfire intensity has resulted in taller wildfire smoke plumes. We investigate the vertical structure of wildfire smoke plumes using aircraft lidar data and establish two effective smoke plume height metrics. Four novel satellite-based plume height products are evaluated for wildfires in the western US. Our results provide guidance on the strengths and limitations of these satellite products and set the stage for improved plume rise estimates by leveraging satellite products.
Piyushkumar N. Patel, Jonathan H. Jiang, Ritesh Gautam, Harish Gadhavi, Olga Kalashnikova, Michael J. Garay, Lan Gao, Feng Xu, and Ali Omar
Atmos. Chem. Phys., 24, 2861–2883, https://doi.org/10.5194/acp-24-2861-2024, https://doi.org/10.5194/acp-24-2861-2024, 2024
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Global measurements of cloud condensation nuclei (CCN) are essential for understanding aerosol–cloud interactions and predicting climate change. To address this gap, we introduced a remote sensing algorithm that retrieves vertically resolved CCN number concentrations from airborne and spaceborne lidar systems. This innovation offers a global distribution of CCN concentrations from space, facilitating model evaluation and precise quantification of aerosol climate forcing.
Lorraine A. Remer, Robert C. Levy, and J. Vanderlei Martins
Atmos. Chem. Phys., 24, 2113–2127, https://doi.org/10.5194/acp-24-2113-2024, https://doi.org/10.5194/acp-24-2113-2024, 2024
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Aerosols are small liquid or solid particles suspended in the atmosphere, including smoke, particulate pollution, dust, and sea salt. Today, we rely on satellites viewing Earth's atmosphere to learn about these particles. Here, we speculate on the future to imagine how satellite viewing of aerosols will change. We expect more public and private satellites with greater capabilities, better ways to infer information from satellites, and merging of data with models.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Blake T. Sorenson, Jeffrey S. Reid, Jianglong Zhang, Robert E. Holz, William L. Smith Sr., and Amanda Gumber
Atmos. Chem. Phys., 24, 1231–1248, https://doi.org/10.5194/acp-24-1231-2024, https://doi.org/10.5194/acp-24-1231-2024, 2024
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Smoke particles are typically submicron in size and assumed to have negligible impacts at the thermal infrared spectrum. However, we show that infrared signatures can be observed over dense smoke plumes from satellites. We found that giant particles are unlikely to be the dominant cause. Rather, co-transported water vapor injected to the middle to upper troposphere and surface cooling beneath the plume due to shadowing are significant, with the surface cooling effect being the most dominant.
Farnaz Hosseinpour and Eric M. Wilcox
Atmos. Chem. Phys., 24, 707–724, https://doi.org/10.5194/acp-24-707-2024, https://doi.org/10.5194/acp-24-707-2024, 2024
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This study shows mechanistic relationships between the radiative effect of dust aerosols in the Saharan air layer and the kinetic energy of the African easterly waves across the tropical Atlantic Ocean using 22 years of daily satellite observations and reanalysis data based on satellite assimilation. Our findings suggest that dust aerosols not merely are transported by these waves but also contribute to the growth of waves through the enhancement of diabatic heating induced by dust.
Markus D. Petters, Tyas Pujiastuti, Ajmal Rasheeda Satheesh, Sabin Kasparoglu, Bethany Sutherland, and Nicholas Meskhidze
Atmos. Chem. Phys., 24, 745–762, https://doi.org/10.5194/acp-24-745-2024, https://doi.org/10.5194/acp-24-745-2024, 2024
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This work introduces a new method that uses remote sensing techniques to obtain surface number emissions of particles with a diameter greater than 500 nm. The technique was applied to study particle emissions at an urban site near Houston, TX, USA. The emissions followed a diurnal pattern and peaked near noon local time. The daily averaged emissions correlated with wind speed. The source is likely due to wind-driven erosion of material situated on asphalted and other hard surfaces.
Zhuang Wang, Chune Shi, Hao Zhang, Yujia Chen, Xiyuan Chi, Congzi Xia, Suyao Wang, Yizhi Zhu, Kaidi Zhang, Xintong Chen, Chengzhi Xing, and Cheng Liu
Atmos. Chem. Phys., 23, 14271–14292, https://doi.org/10.5194/acp-23-14271-2023, https://doi.org/10.5194/acp-23-14271-2023, 2023
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The annual cycle of dust and anthropogenic aerosols' vertical distributions was revealed by polarization Raman lidar in Beijing. Anthropogenic aerosols typically accumulate at the top of the mixing layer (ML) due to the hygroscopic growth of atmospheric particles, and this is most significant in summer. There is no significant relationship between bottom dust mass concentration and ML height, while the dust in the upper air tends to be distributed near the mixing layer.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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We evaluated the long-term trends and seasonal variability of the vertically resolved aerosol properties over the past 17 years in Barcelona. Results shows that air quality is improved, with a consistent drop in PM concentrations at the surface, as well as the column aerosol optical depth. The results also show that natural dust outbreaks are more likely in summer, with aerosols reaching an altitude of 5 km, while in winter, aerosols decay as an exponential with a scale height of 600 m.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Jesús Abril-Gago, Pablo Ortiz-Amezcua, Diego Bermejo-Pantaleón, Juana Andújar-Maqueda, Juan Antonio Bravo-Aranda, María José Granados-Muñoz, Francisco Navas-Guzmán, Lucas Alados-Arboledas, Inmaculada Foyo-Moreno, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 8453–8471, https://doi.org/10.5194/acp-23-8453-2023, https://doi.org/10.5194/acp-23-8453-2023, 2023
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Validation activities of Aeolus wind products were performed in Granada with different upward-probing instrumentation (Doppler lidar system and radiosondes) and spatiotemporal collocation criteria. Specific advantages and disadvantages of each instrument were identified, and an optimal comparison criterion is proposed. Aeolus was proven to provide reliable wind products, and the upward-probing instruments were proven to be useful for Aeolus wind product validation activities.
Jianyu Zheng, Zhibo Zhang, Hongbin Yu, Anne Garnier, Qianqian Song, Chenxi Wang, Claudia Di Biagio, Jasper F. Kok, Yevgeny Derimian, and Claire Ryder
Atmos. Chem. Phys., 23, 8271–8304, https://doi.org/10.5194/acp-23-8271-2023, https://doi.org/10.5194/acp-23-8271-2023, 2023
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We developed a multi-year satellite-based retrieval of dust optical depth at 10 µm and the coarse-mode dust effective diameter over global oceans. It reveals climatological coarse-mode dust transport patterns and regional differences over the North Atlantic, the Indian Ocean and the North Pacific.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Mukunda M. Gogoi, S. Suresh Babu, Ryoichi Imasu, and Makiko Hashimoto
Atmos. Chem. Phys., 23, 8059–8079, https://doi.org/10.5194/acp-23-8059-2023, https://doi.org/10.5194/acp-23-8059-2023, 2023
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Considering the climate warming potential of atmospheric black carbon (BC), satellite-based retrieval is a novel idea. This study highlights the regional distribution of BC based on observations by the Cloud and Aerosol Imager-2 on board the GOSAT-2 satellite and near-surface measurements of BC in ARFINET. The satellite retrieval fairly depicts the regional and seasonal features of BC over the Indian region, which are similar to those recorded by surface observations.
Hao Fan, Xingchuan Yang, Chuanfeng Zhao, Yikun Yang, and Zhenyao Shen
Atmos. Chem. Phys., 23, 7781–7798, https://doi.org/10.5194/acp-23-7781-2023, https://doi.org/10.5194/acp-23-7781-2023, 2023
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Using 20-year multi-source data, this study shows pronounced regional and seasonal variations in fire activities and emissions. Seasonal variability of fires is larger with increasing latitude. The increase in temperature in the Northern Hemisphere's middle- and high-latitude forest regions was primarily responsible for the increase in fires and emissions, while the changes in fire occurrence in tropical regions were more influenced by the decrease in precipitation and relative humidity.
Rosemary Huck, Robert G. Bryant, and James King
Atmos. Chem. Phys., 23, 6299–6318, https://doi.org/10.5194/acp-23-6299-2023, https://doi.org/10.5194/acp-23-6299-2023, 2023
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This study shows that mineral aerosol (dust) emission events in high-latitude areas are under-represented in both ground- and space-based detecting methods. This is done through a suite of ground-based data to prove that dust emissions from the proglacial area, Lhù’ààn Mân, occur almost daily but are not always recorded at different timescales. Dust has multiple effects on atmospheric processes; therefore, accurate quantification is important in the calibration and validation of climate models.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
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We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Ross Herbert and Philip Stier
Atmos. Chem. Phys., 23, 4595–4616, https://doi.org/10.5194/acp-23-4595-2023, https://doi.org/10.5194/acp-23-4595-2023, 2023
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We provide robust evidence from multiple sources showing that smoke from fires in the Amazon rainforest significantly modifies the diurnal cycle of convection and cools the climate. Low to moderate amounts of smoke increase deep convective clouds and rain, whilst beyond a threshold amount, the smoke starts to suppress the convection and rain. We are currently at this threshold, suggesting increases in fires from agricultural practices or droughts will reduce cloudiness and rain over the region.
Cited articles
Ansmann, A., Seifert, P., Tesche, M., and Wandinger, U.: Profiling of fine and coarse particle mass: case studies of Saharan dust and Eyjafjallajökull/Grimsvötn volcanic plumes, Atmos. Chem. Phys., 12, 9399–9415, https://doi.org/10.5194/acp-12-9399-2012, 2012.
Arason, P., Petersen, G. N., and Bjornsson, H.: Observations of the altitude of the volcanic plume during the eruption of Eyjafjallajökull, April–May 2010, Earth Syst. Sci. Data, 3, 9–17, https://doi.org/10.5194/essd-3-9-2011, 2011.
Bourassa, A. E., Robock, A., Randel, W. J., Deshler, T., Rieger, L. A., Lloyd, N. D., Llewellyn, E. T., and Degenstein, D. A.: Large volcanic aerosol load in the stratosphere linked to Asian monsoon transport, Science, 337, 78–81, 2012.
Brown, R., Bonadonna, C., and Durant, A.: A review of volcanic ash aggregation, Phys. Chem. Earth, 45–46, 65–78, https://doi.org/10.1016/j.pce.2011.11.001, 2012.
Bursik, M.: Tephra dispersal, Geological Society, London, Special Publications, 145, 115–144, https://doi.org/10.1144/GSL.SP.1996.145.01.07, 1998.
Bursik, M.: Effect of wind on the rise height of volcanic plumes, Geophys. Res. Lett., 28, 3621–3624, 2001.
Carey, S. and Bursik, M.: Volcanic plumes, Encyclopedia of volcanoes. Academic Press, San Diego, 572–585, 2015.
Carn, S., Strow, L., de Souza-Machado, S., Edmonds, Y., and Hannon, S.: Quantifying tropospheric volcanic emissions with AIRS: The 2002 eruption of Mt. Etna (Italy), Geophys. Res. Lett., 32, 2 https://doi.org/10.1029/2004GL021034, 2005.
Carn, S., Clarisse, L., and Prata, A.: Multi-decadal satellite measurements of global volcanic degassing, J. Volcanol. Geoth. Res., 311, 99–134, 2016.
Clarisse, L. and Prata, F.: Infrared sounding of volcanic ash, in: Volcanic Ash, edited by: Mackie, S., Elsevier, 2016.
Clarisse, L., Coheur, P. F., Prata, A. J., Hurtmans, D., Razavi, A., Phulpin, T., Hadji-Lazaro, J., and Clerbaux, C.: Tracking and quantifying volcanic SO2 with IASI, the September 2007 eruption at Jebel at Tair, Atmos. Chem. Phys., 8, 7723–7734, https://doi.org/10.5194/acp-8-7723-2008, 2008.
Clarisse, L., Prata, F., Lacour, J.-L., Hurtmans, D., Clerbaux, C., and Coheur, P.-F.: A correlation method for volcanic ash detection using hyperspectral infrared measurements, Geophys. Res. Lett., 37, 19, https://doi.org/10.1029/2010GL044828, 2010.
Costa, A., Folch, A., and Macedonio, G.: A model for wet aggregation of ash particles in volcanic plumes and clouds: 1. Theoretical formulation, J. Geophys. Res.-Sol. Ea., 115, https://doi.org/10.1016/j.epsl.2005.11.019, 2010.
Degruyter, W. and Bonadonna, C.: Improving on mass flow rate estimates of volcanic eruptions, Geophys. Res. Lett., 39, 16, https://doi.org/10.1029/2012GL052566, 2012.
Draxler, R. and Rolph, G.: HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) model access via NOAA ARL READY website, available at: http://www.arl.noaa.gov/ready/hysplit4.html (last access: 1 September 2017), NOAA Air Resources Laboratory, Silver Spring, 2003.
Durant, A., Rose, W., Sarna-Wojcicki, A., Carey, S., and Volentik, A.: Hydrometeor-enhanced tephra sedimentation: Constraints from the 18 May 1980 eruption of Mount St. Helens, J. Geophys. Res., 114, B03204, https://doi.org/10.1029/2008JB005756, 2009.
Eckhardt, S., Prata, A. J., Seibert, P., Stebel, K., and Stohl, A.: Estimation of the vertical profile of sulfur dioxide injection into the atmosphere by a volcanic eruption using satellite column measurements and inverse transport modeling, Atmos. Chem. Phys., 8, 3881–3897, https://doi.org/10.5194/acp-8-3881-2008, 2008.
Folch, A., Costa, A., and Macedonio, G.: FALL3D: A computational model for transport and deposition of volcanic ash, Comput. Geosci., 35, 1334–1342, 2009.
Folch, A., Costa, A., and Macedonio, G.: FPLUME-1.0: An integral volcanic plume model accounting for ash aggregation, Geosci. Model Dev., 9, 431–450, https://doi.org/10.5194/gmd-9-431-2016, 2016.
Fromm, M., Kablick, G., Nedoluha, G., Carboni, E., Grainger, R., Campbell, J., and Lewis, J.: Correcting the record of volcanic stratospheric aerosol impact: Nabro and Sarychev Peak, J. Geophys. Res.-Atmos., 119, 17, https://doi.org/10.1002/2014JD021507, 2014.
Fu, G., Prata, F., Lin, H. X., Heemink, A., Segers, A., and Lu, S.: Data assimilation for volcanic ash plumes using a satellite observational operator: a case study on the 2010 Eyjafjallajökull volcanic eruption, Atmos. Chem. Phys., 17, 1187–1205, https://doi.org/10.5194/acp-17-1187-2017, 2017.
Glaze, L. and Baloga, S.: Sensitivity of buoyant plume heights to ambient atmospheric conditions: Implications for volcanic eruption columns, J. Geophys. Res., 101, 1529–1540, https://doi.org/10.1029/95JD03071, 1996.
Gudmundsson, M., Höskuldsson, Á., Larsen, G., Thordarson, T., Oladottir, B., Oddsson, B., Gudnason, J., Högnadottir, T., Stevenson, J., Houghton, B., and McGarvie, D.: The May 2011 eruption of Grímsvötn, Geophys. Res. Abstr., vol. 14, p. 12119, EGU General Assembly 2012, Vienna, Austria, 2012a.
Gudmundsson, M. T., Thordarson, T., Höskuldsson, Á., Larsen, G., Björnsson, H., Prata, F. J., Oddsson, B., Magnússon, E., Högnadóttir, T., Petersen, G. N., and Hayward, C. L.: Ash generation and distribution from the April-May 2010 eruption of Eyjafjallajökull, Iceland, Scientific reports, 2, 2012b.
Guo, S., Bluth, G. J., Rose, W. I., Watson, I. M., and Prata, A.: Re-evaluation of SO2 release of the 15 June 1991 Pinatubo eruption using ultraviolet and infrared satellite sensors, Geochem. Geophy. Geosys., 5, 572, https://doi.org/10.1038/srep00572, 2004.
Hoffmann, L., Grießbach, S., and Meyer, C. I.: Volcanic emissions from AIRS observations: detection methods, case study, and statistical analysis, in: Proceedings of the SPIE, p. 924214, Forschungszentrum Jülich GmbH (Germany), 2014.
Holasek, R. E., Woods, A. W., and Self, S.: Experiments on gas-ash separation processes in volcanic umbrella plumes, J. Volcanol. Geoth. Res., 70, 169–181, 1996.
Hunt, W. H., Winker, D. M., Vaughan, M. A., Powell, K. A., Lucker, P. L., and Weimer, C.: CALIPSO Lidar Description and Performance Assessment, J. Atmos. Ocean. Tech., 26, 1214–1228, 2009.
James, M., Gilbert, J., and Lane, S.: Experimental investigation of volcanic particle aggregation in the absence of liquid phase, J. Geophys. Res., 107, 2191, https://doi.org/10.1029/2001JB000950, 2002.
James, M., Lane, S., and Gilbert, J.: Density, construction, and drag coefficient of electrostatic volcanic ash aggregates, J. Geophys. Res., 108, 2435, https://doi.org/10.1029/2002JB002011, 2003.
Johnson, C., Hogg, A., Huppert, H., Sparks, R., Phillips, J., Slim, A., and Woodhouse, M.: Modelling Intrusions through quiescent and moving ambients, J. Fluid Mech., 771, 370–406, https://doi.org/10.1017/jfm.2015.180, 2015.
Jones, A., Thomson, D., Hort, M., and Devenish, B.: The UK Met Office's next-generation atmospheric dispersion model, NAME III, in: Air Pollution Modeling and its Application XVII, Springer, 580–589, 2007.
Jude-Eton, T., Thordarson, T., Gudmundsson, M., and Oddsson, B.: Dynamics, stratigraphy and proximal dispersal of supraglacial tephra during the ice-confined 2004 eruption at Grímsvötn Volcano, Iceland, B. Volcanol., 74, 1057–1082, 2012.
Kristiansen, N., Stohl, A., Prata, A., Richter, A., Eckhardt, S., Seibert, P., Hoffmann, A., Ritter, C., Bitar, L., Duck, T., Bitar, L., Duck, T. J., and Stebel, K.: Remote sensing and inverse transport modeling of the Kasatochi eruption sulfur dioxide cloud, J. Geophys. Res.-Atmos., 115, https://doi.org/10.1029/2009JD013286, 2010.
Kylling, A., Kahnert, M., Lindqvist, H., and Nousiainen, T.: Volcanic ash infrared signature: porous non-spherical ash particle shapes compared to homogeneous spherical ash particles, Atmos. Meas. Tech., 7, 919–929, https://doi.org/10.5194/amt-7-919-2014, 2014.
Mastin, L.: A user-friendly one-dimensional model for wet volcanic plumes, Geochem. Geophy. Geosys., 8, Q03014, https://doi.org/10.1029/2006GC001455, 2007.
Mastin, L., Guffanti, M., Servranckx, R., Webley, P., Barsotti, S., Dean, K., Durant, A., Ewert, J., Neri, A., Rose, W., and Schneider, D.: A multidisciplinary effort to assign realistic source parameters to models of volcanic ash-cloud transport and dispersion during eruptions, J. Volcanol. Geoth. Res., 186, 10–21, 2009.
Morton, B., Taylor, G., and Turner, J.: Turbulent Gravitational Convection from Maintained and Instantaneous Sources, Philos. T. R. Soc. Lond. A, 234, 1–23, https://doi.org/10.1098/rspa.1956.0011, 1956.
Moxnes, E. D., Kristiansen, N. I., Stohl, A., Clarisse, L., Durant, A., Weber, K., and Vogel, A.: Separation of ash and sulfur dioxide during the 2011 Grímsvötn eruption, J. Geophys. Res.-Atmos., 119, 7477–7501, 2014.
Papanicolaou, P. and List, E.: Investigations of round vertical turbulent buoyant jets, J. Fluid Mech., 195, 341–391, https://doi.org/10.1017/S0022112088002447, 1988.
Petersen, G. N., Bjornsson, H., Arason, P., and von Löwis, S.: Two weather radar time series of the altitude of the volcanic plume during the May 2011 eruption of Grímsvötn, Iceland, Earth Syst. Sci. Data, 4, 121–127, https://doi.org/10.5194/essd-4-121-2012, 2012.
Prata, A.: Satellite detection of hazardous volcanic clouds and the risk to global air traffic, Nat. Hazards, 51, 303–324, 2009.
Prata, A. and Bernardo, C.: Retrieval of volcanic SO2 column abundance from Atmospheric Infrared Sounder data, J. Geophys. Res.-Atmos., 112, https://doi.org/10.1029/2006JD007955, 2007.
Prata, A. and Grant, I.: Retrieval of microphysical and morphological properties of volcanic ash plumes from satellite data: Application to Mt Ruapehu, New Zealand, Q. J. Roy. Meteorl Soc., 127, 2153–2179, 2001.
Prata, A. and Prata, A.: Eyjafjallajökull volcanic ash concentrations determined using Spin Enhanced Visible and Infrared Imager measurements, J. Geophys. Res.-Atmos., 117, https://doi.org/10.1029/2011JD016800, 2012.
Prata, A. and Rose, W.: Volcanic ash hazards to aviation, in: Encyclopedia of Volcanoes, chap. 52, 2015.
Prata, A. J., Gangale, G., Clarisse, L., and Karagulian, F.: Ash and sulfur dioxide in the 2008 eruptions of Okmok and Kasatochi: Insights from high spectral resolution satellite measurements, J. Geophys. Res.-Atmos., 115, D2, https://doi.org/10.1029/2009JD013556, 2010.
Prata, A. T., Siems, S. T., and Manton, M. J.: Quantification of volcanic cloud top heights and thicknesses using A-train observations for the 2008 Chaitén eruption, J. Geophys. Res.-Atmos., 120, 2928–2950, 2015.
Prata, A. T., Young, S. A., Siems, S. T., and Manton, M. J.: Lidar ratios of stratospheric volcanic ash and sulfate aerosols retrieved from CALIOP measurements, Atmos. Chem. Phys., 17, 8599–8618, https://doi.org/10.5194/acp-17-8599-2017, 2017.
Rienecker, M. M., Suarez, M. J., Todling, R., Bacmeister, J., Takacs, L., Liu, H. C., Gu, W., Sienkiewicz, M., Koster, R. D., Gelaro, R., Stajner, I., and Nielsen, J. E.: The GEOS-5 Data Assimilation System–Documentation of Versions 5.0.1, 5.1.0, and 5.2.0, Technical Report Series on Global Modeling and Data Assimilation, 27, NASA/TM-2008-104606, 1–118, 2008.
Robock, A.: Volcanic eruptions and climate, Rev. Geophys., 38, 191–219, 2000.
Self, S. and Rampino, M. R.: The 1883 eruption of Krakatau, Nature, 294, 699–704, 1981.
Sigmarsson, O., Haddadi, B., Carn, S., Moune, S., Gudnason, J., Yang, K., and Clarisse, L.: The sulfur budget of the 2011 Grímsvötn eruption, Iceland, Geophys. Res. Lett., 40, 6095–6100, 2013.
Sparks, R.: The dimensions and dynamics of volcanic eruption columns, Bull. Volcanol., 48, 3–15, https://doi.org/10.1007/BF01073509, 1986.
Sparks, R., Bursik, M., Carey, S., Gilbert, J., Glaze, L., Sigurdsson, H., and Woods, A.: Volcanic Plumes, John Wileys & Sons, 1997a.
Sparks, R. S. J., Bursik, M., Carey, S., Gilbert, J., Glaze, L., Sigurdsson, H., and Woods, A.: Volcanic plumes, Wiley, 1997b.
Stevenson, J. A., Loughlin, S., Rae, C., Thordarson, T., Milodowski, A. E., Gilbert, J. S., Harangi, S., Lukács, R., Höjgaard, B., Árting, U., Pyne-O'Donnell, S., MacLeod, A., Whitney, B., and Cassidy, M.: Distal deposition of tephra from the Eyjafjallajökull 2010 summit eruption, J. Geophys. Res.-Sol. Ea., 117, B9, https://doi.org/10.1029/2011JB008904, 2012.
Stevenson, J. A., Loughlin, S. C., Font, A., Fuller, G. W., MacLeod, A., Oliver, I. W., Jackson, B., Horwell, C. J., Thordarson, T., and Dawson, I.: UK monitoring and deposition of tephra from the May 2011 eruption of Grímsvötn, Iceland, J. Appl. Volcanol., 2, 3, https://doi.org/10.1186/2191-5040-2-3, 2013.
Stevenson, J. A., Millington, S. C., Beckett, F. M., Swindles, G. T., and Thordarson, T.: Big grains go far: understanding the discrepancy between tephrochronology and satellite infrared measurements of volcanic ash, Atmos. Meas. Tech., 8, 2069–2091, https://doi.org/10.5194/amt-8-2069-2015, 2015.
Stohl, A., Prata, A. J., Eckhardt, S., Clarisse, L., Durant, A., Henne, S., Kristiansen, N. I., Minikin, A., Schumann, U., Seibert, P., Stebel, K., Thomas, H. E., Thorsteinsson, T., Tørseth, K., and Weinzierl, B.: Determination of time- and height-resolved volcanic ash emissions and their use for quantitative ash dispersion modeling: the 2010 Eyjafjallajökull eruption, Atmos. Chem. Phys., 11, 4333–4351, https://doi.org/10.5194/acp-11-4333-2011, 2011.
Telling, J. and Dufek, J.: An experimental evaluation of ash aggregation in explosive volcanic eruptions, J. Volcanol. Geoth. Res.h, 209–210, 1–8, https://doi.org/10.1016/j.jvolgeores.2011.09.008, 2012.
Telling, J., Dufek, J., and Shaikh, A.: Ash aggregation in explosive volcanic eruptions, Geophys. Res. Lett., 40, 2355–2360, https://doi.org/10.1002/grl.50376, 2013a.
Telling, J., Dufek, J., and Shaikh, A.: Ash aggregation in explosive volcanic eruptions, Geophys. Res. Lett., 40, 2355–2360, 2013b.
Tesche, M., Glantz, P., Johansson, C., Norman, M., Hiebsch, A., Ansmann, A., Althausen, D., Engelmann, R., and Seifert, P.: Volcanic ash over Scandinavia originating from the Grímsvötn eruptions in May 2011, J. Geophys. Res.-Atmos., 117, https://doi.org/10.1029/2011JD017090, 2012.
Textor, C., Graf, H.-F., Herzog, M., Oberhuber, J. M., Rose, W. I., and Ernst, G. G.: Volcanic particle aggregation in explosive eruption columns. Part I: Parameterization of the microphysics of hydrometeors and ash, J. Volcanol. Geoth. Res., 150, 359–377, 2006.
Thomas, H. E. and Prata, A. J.: Sulphur dioxide as a volcanic ash proxy during the April–May 2010 eruption of Eyjafjallajökull Volcano, Iceland, Atmos. Chem. Phys., 11, 6871–6880, https://doi.org/10.5194/acp-11-6871-2011, 2011.
Thordarson, T. and Larsen, G.: Volcanism in Iceland in historical time: Volcano types, eruption styles and eruptive history, J. Geodyn., 43, 118–152, 2007.
Thordarson, T. and Self, S.: Atmospheric and environmental effects of the 1783–1784 Laki eruption: a review and reassessment, J. Geophys. Res., 108, 4011, https://doi.org/10.1029/2001JD002042, 2003.
Tupper, A., Textor, C., Herzog, M., Graf, H.-F., and Richards, M. S.: Tall clouds from small eruptions: the sensitivity of eruption height and fine ash content to tropospheric instability, Nat.Hazards, 51, 375–401, https://doi.org/10.1007/s11069-009-9433-9, 2009.
Van Eaton, A., Muirhead, J., Wilson, C., and Cimarelli, C.: Growth of volcanic ash aggregates in the presence of liquid water and ice: an experimental approach, Bull. Volcanol., 74, 1963–1984, https://doi.org/10.1007/s00445-012-0634-9, 2012.
Van Eaton, A., Mastin, L., Herzog, M., Schwaiger, H., Schneider, D., Wallace, K., and Clarke, A.: Hail formation triggers rapid ash aggregation in volcanic plumes, Nature Communications, 6, 1–7, https://doi.org/10.1038/ncomms8860, 2015.
Vaughan, M. A., Powell, K. A., Kuehn, R. E., Young, S. A., Winker, D. M., Hostetler, C. A., Hunt, W. H., Liu, Z., McGill, M. J., and Getzewich, B. J.: Fully Automated Detection of Cloud and Aerosol Layers in the CALIPSO Lidar Measurements, J. Atmos. Ocean. Tech., 26, 2034–2050, 2009.
Veitch, G. and Woods, A.: Particle aggregation in volcanic eruption columns, J. Geophys. Rese.-Sol. Ea., 106, 26425–26441, https://doi.org/10.1029/2000JB900343, 2001.
Wen, S. and Rose, W. I.: Retrieval of sizes and total masses of particles in volcanic clouds using AVHRR bands 4 and 5, J. Geophys. Res.-Atmos., 99, 5421–5431, 1994.
Wilson, L. and Huang, T.: The influence of shape on the atmospheric settling velocity of volcanic ash particles, Earth Planet. Sc. Lett., 44, 311–324, https://doi.org/10.1016/0012-821X(79)90179-1, 1979.
Wilson, L., Sparks, R., Huang, T., and Watkins, N.: The Control of Volcanic Column Heights by Eruption Energetics and Dynamics, J. Geophys. Res., 83, 1829–1836, 1978.
Winker, D. M., Liu, Z., Omar, A., Tackett, J., and Fairlie, D.: CALIOP observations of the transport of ash from the Eyjafjallajökull volcano in April 2010, J. Geophys. Res.-Atmos., 117, D00U15, https://doi.org/10.1029/2011JD016499, 2012.
Woodhouse, M. and Behnke, S.: Charge structure in volcanic plumes: a comparison of plume properties predicted by an integral plume model to observations of volcanic lightning during the 2010 eruption of Eyjafjallajökull, Iceland, Bull. Volcanol., 76, 828, https://doi.org/10.1007/s00445-014-0828-4, 2014.
Woodhouse, M., Hogg, A., Phillips, J., and Sparks, R.: Interaction between volcanic plumes and wind during the 2010 Eyjafjallajökull eruption, Iceland, J. Geophys. Res., 118, 92–109, https://doi.org/10.1029/2012JB009592., 2013.
Woods, A.: The fluid dynamics and thermodynamics of eruption columns, Bull. Volcanol., 50, 169–193, 1988.
Woods, A.: Moist Convection and the Injection of Volcanic Ash Into the Atmosphere, J. Geophys. Res., 98, 17627–17636, https://doi.org/10.1029/93JB00718, 1993.
Woods, A. W., Holasek, R. E., and Self, S.: Wind-driven dispersal of volcanic ash plumes and its control on the thermal structure of the plume-top, Bull. Volcanol., 57, 283–292, 1995.
Yang, K., Krotkov, N. A., Krueger, A. J., Carn, S. A., Bhartia, P. K., and Levelt, P. F.: Retrieval of large volcanic SO2 columns from the Aura Ozone Monitoring Instrument: Comparison and limitations, J. Geophys. Res.-Atmos., 112, https://doi.org/10.1029/2007JD008825. 2007a.
Yang, P., Feng, Q., Hong, G., Kattawar, G. W., Wiscombe, W. J., Mishchenko, M. I., Dubovik, O., Laszlo, I., and Sokolik, I. N.: Modeling of the scattering and radiative properties of nonspherical dust-like aerosols, J. Aerosol Sci., 38, 995–1014, https://doi.org/10.1016/j.jaerosci.2007.07.001, 2007b.
Short summary
This paper investigates the separation of gases and particles that frequently occurs during violent volcanic eruptions. This problem is important because atmospheric winds spread volcanic aerosols at great distances from the source, and wind shear then causes the aerosols to spread in different directions at different altitudes. This has important repercussions for accurately forecasting the movement of hazardous volcanic clouds. The May 2011 Grímsvötn eruption is analysed in great detail.
This paper investigates the separation of gases and particles that frequently occurs during...
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