Articles | Volume 16, issue 7
https://doi.org/10.5194/acp-16-4661-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-4661-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
14 Apr 2016
Research article |
| 14 Apr 2016
Effects of long-range aerosol transport on the microphysical properties of low-level liquid clouds in the Arctic
Quentin Coopman
CORRESPONDING AUTHOR
Department of Atmospheric Sciences, University of Utah, Salt Lake
City, UT, USA
Laboratoire d'Optique Atmosphérique, Université
de Lille/CNRS, Lille, France
Timothy J. Garrett
Department of Atmospheric Sciences, University of Utah, Salt Lake
City, UT, USA
Jérôme Riedi
Laboratoire d'Optique Atmosphérique, Université
de Lille/CNRS, Lille, France
Sabine Eckhardt
Norwegian Institute for Air Research,
Kjeller, Norway
Andreas Stohl
Norwegian Institute for Air Research,
Kjeller, Norway
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EGUsphere, https://doi.org/10.5194/egusphere-2024-1713, https://doi.org/10.5194/egusphere-2024-1713, 2024
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Computer models are essential for improving our understanding of how gases and particles move in the atmosphere. We present an update of the atmospheric transport model FLEXPART. FLEXPART 11 is more accurate due to a reduced number of interpolations and a new scheme for wet deposition. It can simulate non-spherical aerosols, and includes linear chemical reactions. It is parallelised using OpenMP and includes new user options. A new user manual details how to use FLEXPART 11.
Karlie N. Rees, Timothy J. Garrett, Thomas D. DeWitt, Corey Bois, Steven K. Krueger, and Jérôme C. Riedi
EGUsphere, https://doi.org/10.5194/egusphere-2024-552, https://doi.org/10.5194/egusphere-2024-552, 2024
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The shapes of clouds viewed from space reflect both vertical and horizontal motions in the atmosphere. The turbulence that shapes clouds is similarly described and related theoretically to the measured complexity of cloud perimeters from various satellites and a numerical model. We find agreement between theory and observations, and, remarkably, that the theory applies globally using only basic planetary physical parameters from the smallest scales of turbulence to the planetary scale.
Karl Espen Yttri, Are Bäcklund, Franz Conen, Sabine Eckhardt, Nikolaos Evangeliou, Markus Fiebig, Anne Kasper-Giebl, Avram Gold, Hans Gundersen, Cathrine Lund Myhre, Stephen Matthew Platt, David Simpson, Jason D. Surratt, Sönke Szidat, Martin Rauber, Kjetil Tørseth, Martin Album Ytre-Eide, Zhenfa Zhang, and Wenche Aas
Atmos. Chem. Phys., 24, 2731–2758, https://doi.org/10.5194/acp-24-2731-2024, https://doi.org/10.5194/acp-24-2731-2024, 2024
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We discuss carbonaceous aerosol (CA) observed at the high Arctic Zeppelin Observatory (2017 to 2020). We find that organic aerosol is a significant fraction of the Arctic aerosol, though less than sea salt aerosol and mineral dust, as well as non-sea-salt sulfate, originating mainly from anthropogenic sources in winter and from natural sources in summer, emphasizing the importance of wildfires for biogenic secondary organic aerosol and primary biological aerosol particles observed in the Arctic.
Thomas D. DeWitt and Timothy J. Garrett
EGUsphere, https://doi.org/10.5194/egusphere-2024-67, https://doi.org/10.5194/egusphere-2024-67, 2024
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There is considerable disagreement on mathematical parameters that describe the numbers of clouds of different sizes, as well as the size of the largest clouds. Both are key defining characteristics of the Earth's atmosphere. A previous study provided an incorrect explanation for the disagreement. Instead, the disagreements may be explained by prior studies not properly accounting for the size of their measurement domain. We offer recommendations for how the domain size can be accounted for.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Ondřej Tichý, Sabine Eckhardt, Yves Balkanski, Didier Hauglustaine, and Nikolaos Evangeliou
Atmos. Chem. Phys., 23, 15235–15252, https://doi.org/10.5194/acp-23-15235-2023, https://doi.org/10.5194/acp-23-15235-2023, 2023
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We show declining trends in NH3 emissions over Europe for 2013–2020 using advanced dispersion and inverse modelling and satellite measurements from CrIS. Emissions decreased by −26% since 2013, showing that the abatement strategies adopted by the European Union have been very efficient. Ammonia emissions are low in winter and peak in summer due to temperature-dependent soil volatilization. The largest decreases were observed in central and western Europe in countries with high emissions.
Jenny Oh, Chubashini Shunthirasingham, Ying Duan Lei, Faqiang Zhan, Yuening Li, Abigaëlle Dalpé Castilloux, Amina Ben Chaaben, Zhe Lu, Kelsey Lee, Frank A. P. C. Gobas, Sabine Eckhardt, Nick Alexandrou, Hayley Hung, and Frank Wania
Atmos. Chem. Phys., 23, 10191–10205, https://doi.org/10.5194/acp-23-10191-2023, https://doi.org/10.5194/acp-23-10191-2023, 2023
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An emerging brominated flame retardant (BFR) called TBECH (1,2-dibromo-4-(1,2-dibromoethyl)cyclohexane) has never been produced or imported for use in Canada yet is found to be one of the most abundant gaseous BFRs in the Canadian atmosphere. The recorded spatial and temporal variability of TBECH suggest that the release from imported consumer products containing TBECH is the most likely explanation for its environmental occurrence in Canada.
Dhiraj Kumar Singh, Eric Pardyjak, and Timothy Garrett
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-148, https://doi.org/10.5194/amt-2023-148, 2023
Revised manuscript accepted for AMT
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Accurate measurements of the properties of snowflakes are challenging to make. We present a new technique for the real-time measurement of the density of freshly fallen individual snowflakes. A new thermal-imaging instrument, the Differential Emissivity Imaging Disdrometer (DEID), is shown to be capable of providing accurate estimates of individual snowflake and bulk-snow hydrometeor density. The method exploits the rate of heat transfer during the melting of a snowflake on a hotplate.
Xavier Ceamanos, Bruno Six, Suman Moparthy, Dominique Carrer, Adèle Georgeot, Josef Gasteiger, Jérôme Riedi, Jean-Luc Attié, Alexei Lyapustin, and Iosif Katsev
Atmos. Meas. Tech., 16, 2575–2599, https://doi.org/10.5194/amt-16-2575-2023, https://doi.org/10.5194/amt-16-2575-2023, 2023
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A new algorithm to retrieve the diurnal evolution of aerosol optical depth over land and ocean from geostationary meteorological satellites is proposed and successfully evaluated with reference ground-based and satellite data. The high-temporal-resolution aerosol observations that are obtained from the EUMETSAT Meteosat Second Generation mission are unprecedented and open the door to studies that cannot be conducted with the once-a-day observations available from low-Earth-orbit satellites.
Anja Eichler, Michel Legrand, Theo M. Jenk, Susanne Preunkert, Camilla Andersson, Sabine Eckhardt, Magnuz Engardt, Andreas Plach, and Margit Schwikowski
The Cryosphere, 17, 2119–2137, https://doi.org/10.5194/tc-17-2119-2023, https://doi.org/10.5194/tc-17-2119-2023, 2023
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We investigate how a 250-year history of the emission of air pollutants (major inorganic aerosol constituents, black carbon, and trace species) is preserved in ice cores from four sites in the European Alps. The observed uniform timing in species-dependent longer-term concentration changes reveals that the different ice-core records provide a consistent, spatially representative signal of the pollution history from western European countries.
Huazhe Shang, Souichiro Hioki, Guillaume Penide, Céline Cornet, Husi Letu, and Jérôme Riedi
Atmos. Chem. Phys., 23, 2729–2746, https://doi.org/10.5194/acp-23-2729-2023, https://doi.org/10.5194/acp-23-2729-2023, 2023
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We find that cloud profiles can be divided into four prominent patterns, and the frequency of these four patterns is related to intensities of cloud-top entrainment and precipitation. Based on these analyses, we further propose a cloud profile parameterization scheme allowing us to represent these patterns. Our results shed light on how to facilitate the representation of cloud profiles and how to link them to cloud entrainment or precipitating status in future remote-sensing applications.
Timothy J. Garrett, Matheus R. Grasselli, and Stephen Keen
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Current world economic production is rising relative to energy consumption. This increase in
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Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Christine D. Groot Zwaaftink, Wenche Aas, Sabine Eckhardt, Nikolaos Evangeliou, Paul Hamer, Mona Johnsrud, Arve Kylling, Stephen M. Platt, Kerstin Stebel, Hilde Uggerud, and Karl Espen Yttri
Atmos. Chem. Phys., 22, 3789–3810, https://doi.org/10.5194/acp-22-3789-2022, https://doi.org/10.5194/acp-22-3789-2022, 2022
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We investigate causes of a poor-air-quality episode in northern Europe in October 2020 during which EU health limits for air quality were vastly exceeded. Such episodes may trigger measures to improve air quality. Analysis based on satellite observations, transport simulations, and surface observations revealed two sources of pollution. Emissions of mineral dust in Central Asia and biomass burning in Ukraine arrived almost simultaneously in Norway, and transport continued into the Arctic.
Stephen M. Platt, Øystein Hov, Torunn Berg, Knut Breivik, Sabine Eckhardt, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Markus Fiebig, Rebecca Fisher, Georg Hansen, Hans-Christen Hansson, Jost Heintzenberg, Ove Hermansen, Dominic Heslin-Rees, Kim Holmén, Stephen Hudson, Roland Kallenborn, Radovan Krejci, Terje Krognes, Steinar Larssen, David Lowry, Cathrine Lund Myhre, Chris Lunder, Euan Nisbet, Pernilla B. Nizzetto, Ki-Tae Park, Christina A. Pedersen, Katrine Aspmo Pfaffhuber, Thomas Röckmann, Norbert Schmidbauer, Sverre Solberg, Andreas Stohl, Johan Ström, Tove Svendby, Peter Tunved, Kjersti Tørnkvist, Carina van der Veen, Stergios Vratolis, Young Jun Yoon, Karl Espen Yttri, Paul Zieger, Wenche Aas, and Kjetil Tørseth
Atmos. Chem. Phys., 22, 3321–3369, https://doi.org/10.5194/acp-22-3321-2022, https://doi.org/10.5194/acp-22-3321-2022, 2022
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Here we detail the history of the Zeppelin Observatory, a unique global background site and one of only a few in the high Arctic. We present long-term time series of up to 30 years of atmospheric components and atmospheric transport phenomena. Many of these time series are important to our understanding of Arctic and global atmospheric composition change. Finally, we discuss the future of the Zeppelin Observatory and emerging areas of future research on the Arctic atmosphere.
Karlie N. Rees and Timothy J. Garrett
Atmos. Meas. Tech., 14, 7681–7691, https://doi.org/10.5194/amt-14-7681-2021, https://doi.org/10.5194/amt-14-7681-2021, 2021
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Monte Carlo simulations are used to establish baseline precipitation measurement uncertainties according to World Meteorological Organization standards. Measurement accuracy depends on instrument sampling area, time interval, and precipitation rate. Simulations are compared with field measurements taken by an emerging hotplate precipitation sensor. We find that the current collection area is sufficient for light rain, but a larger collection area is required to detect moderate to heavy rain.
Dhiraj K. Singh, Spencer Donovan, Eric R. Pardyjak, and Timothy J. Garrett
Atmos. Meas. Tech., 14, 6973–6990, https://doi.org/10.5194/amt-14-6973-2021, https://doi.org/10.5194/amt-14-6973-2021, 2021
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This paper describes a new instrument for quantifying the physical characteristics of hydrometeors such as snow and rain. The device can measure the mass, size, density and type of individual hydrometeors as well as their bulk properties. The instrument is called the Differential Emissivity Imaging Disdrometer (DEID) and is composed of a thermal camera and hotplate. The DEID measures hydrometeors at sampling frequencies up to 1 Hz with masses and effective diameters greater than 1 µg and 200 µm.
Karlie N. Rees, Dhiraj K. Singh, Eric R. Pardyjak, and Timothy J. Garrett
Atmos. Chem. Phys., 21, 14235–14250, https://doi.org/10.5194/acp-21-14235-2021, https://doi.org/10.5194/acp-21-14235-2021, 2021
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Accurate predictions of weather and climate require descriptions of the mass and density of snowflakes as a function of their size. Few measurements have been obtained to date because snowflakes are so small and fragile. This article describes results from a new instrument that automatically measures individual snowflake size, mass, and density. Key findings are that small snowflakes have much lower densities than is often assumed and that snowflake density increases with temperature.
Jessica L. McCarty, Juha Aalto, Ville-Veikko Paunu, Steve R. Arnold, Sabine Eckhardt, Zbigniew Klimont, Justin J. Fain, Nikolaos Evangeliou, Ari Venäläinen, Nadezhda M. Tchebakova, Elena I. Parfenova, Kaarle Kupiainen, Amber J. Soja, Lin Huang, and Simon Wilson
Biogeosciences, 18, 5053–5083, https://doi.org/10.5194/bg-18-5053-2021, https://doi.org/10.5194/bg-18-5053-2021, 2021
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Fires, including extreme fire seasons, and fire emissions are more common in the Arctic. A review and synthesis of current scientific literature find climate change and human activity in the north are fuelling an emerging Arctic fire regime, causing more black carbon and methane emissions within the Arctic. Uncertainties persist in characterizing future fire landscapes, and thus emissions, as well as policy-relevant challenges in understanding, monitoring, and managing Arctic fire regimes.
Karl Espen Yttri, Francesco Canonaco, Sabine Eckhardt, Nikolaos Evangeliou, Markus Fiebig, Hans Gundersen, Anne-Gunn Hjellbrekke, Cathrine Lund Myhre, Stephen Matthew Platt, André S. H. Prévôt, David Simpson, Sverre Solberg, Jason Surratt, Kjetil Tørseth, Hilde Uggerud, Marit Vadset, Xin Wan, and Wenche Aas
Atmos. Chem. Phys., 21, 7149–7170, https://doi.org/10.5194/acp-21-7149-2021, https://doi.org/10.5194/acp-21-7149-2021, 2021
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Carbonaceous aerosol sources and trends were studied at the Birkenes Observatory. A large decrease in elemental carbon (EC; 2001–2018) and a smaller decline in levoglucosan (2008–2018) suggest that organic carbon (OC)/EC from traffic/industry is decreasing, whereas the abatement of OC/EC from biomass burning has been less successful. Positive matrix factorization apportioned 72 % of EC to fossil fuel sources and 53 % (PM2.5) and 78 % (PM10–2.5) of OC to biogenic sources.
Nikolaos Evangeliou, Yves Balkanski, Sabine Eckhardt, Anne Cozic, Martin Van Damme, Pierre-François Coheur, Lieven Clarisse, Mark W. Shephard, Karen E. Cady-Pereira, and Didier Hauglustaine
Atmos. Chem. Phys., 21, 4431–4451, https://doi.org/10.5194/acp-21-4431-2021, https://doi.org/10.5194/acp-21-4431-2021, 2021
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Ammonia, a substance that has played a key role in sustaining life, has been increasing in the atmosphere, affecting climate and humans. Understanding the reasons for this increase is important for the beneficial use of ammonia. The evolution of satellite products gives us the opportunity to calculate ammonia emissions easier. We calculated global ammonia emissions over the last 10 years, incorporated them into a chemistry model and recorded notable improvement in reproducing observations.
Souichiro Hioki, Jérôme Riedi, and Mohamed S. Djellali
Atmos. Meas. Tech., 14, 1801–1816, https://doi.org/10.5194/amt-14-1801-2021, https://doi.org/10.5194/amt-14-1801-2021, 2021
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This research estimates the magnitude of a motion-induced error in the measurement of polarimetric state of light by a planned instrument on a future satellite. We discovered that the motion-induced error can not be cancelled out by spatiotemporal averaging, but it can be predicted from the along-track change of the intensity of light. With the estimated statistics and the simulation model, this research paves a way to provide pixel-level quality information in the future satellite products.
Nikolaos Evangeliou, Stephen M. Platt, Sabine Eckhardt, Cathrine Lund Myhre, Paolo Laj, Lucas Alados-Arboledas, John Backman, Benjamin T. Brem, Markus Fiebig, Harald Flentje, Angela Marinoni, Marco Pandolfi, Jesus Yus-Dìez, Natalia Prats, Jean P. Putaud, Karine Sellegri, Mar Sorribas, Konstantinos Eleftheriadis, Stergios Vratolis, Alfred Wiedensohler, and Andreas Stohl
Atmos. Chem. Phys., 21, 2675–2692, https://doi.org/10.5194/acp-21-2675-2021, https://doi.org/10.5194/acp-21-2675-2021, 2021
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Following the transmission of SARS-CoV-2 to Europe, social distancing rules were introduced to prevent further spread. We investigate the impacts of the European lockdowns on black carbon (BC) emissions by means of in situ observations and inverse modelling. BC emissions declined by 23 kt in Europe during the lockdowns as compared with previous years and by 11 % as compared to the period prior to lockdowns. Residential combustion prevailed in Eastern Europe, as confirmed by remote sensing data.
Kyle E. Fitch, Chaoxun Hang, Ahmad Talaei, and Timothy J. Garrett
Atmos. Meas. Tech., 14, 1127–1142, https://doi.org/10.5194/amt-14-1127-2021, https://doi.org/10.5194/amt-14-1127-2021, 2021
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Snow measurements are very sensitive to wind. Here, we compare airflow and snowfall simulations to Arctic observations for a Multi-Angle Snowflake Camera to show that measurements of fall speed, orientation, and size are accurate only with a double wind fence and winds below 5 m s−1. In this case, snowflakes tend to fall with a nearly horizontal orientation; the largest flakes are as much as 5 times more likely to be observed. Adjustments are needed for snow falling in naturally turbulent air.
Ignacio Pisso, Espen Sollum, Henrik Grythe, Nina I. Kristiansen, Massimo Cassiani, Sabine Eckhardt, Delia Arnold, Don Morton, Rona L. Thompson, Christine D. Groot Zwaaftink, Nikolaos Evangeliou, Harald Sodemann, Leopold Haimberger, Stephan Henne, Dominik Brunner, John F. Burkhart, Anne Fouilloux, Jerome Brioude, Anne Philipp, Petra Seibert, and Andreas Stohl
Geosci. Model Dev., 12, 4955–4997, https://doi.org/10.5194/gmd-12-4955-2019, https://doi.org/10.5194/gmd-12-4955-2019, 2019
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We present the latest release of the Lagrangian transport model FLEXPART, which simulates the transport, diffusion, dry and wet deposition, radioactive decay, and 1st-order chemical reactions of atmospheric tracers. The model has been recently updated both technically and in the representation of physicochemical processes. We describe the changes, document the most recent input and output files, provide working examples, and introduce testing capabilities.
Karl Espen Yttri, David Simpson, Robert Bergström, Gyula Kiss, Sönke Szidat, Darius Ceburnis, Sabine Eckhardt, Christoph Hueglin, Jacob Klenø Nøjgaard, Cinzia Perrino, Ignazio Pisso, Andre Stephan Henry Prevot, Jean-Philippe Putaud, Gerald Spindler, Milan Vana, Yan-Lin Zhang, and Wenche Aas
Atmos. Chem. Phys., 19, 4211–4233, https://doi.org/10.5194/acp-19-4211-2019, https://doi.org/10.5194/acp-19-4211-2019, 2019
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Carbonaceous aerosols from natural sources were abundant regardless of season. Residential wood burning (RWB) emissions were occasionally equally as large as or larger than of fossil-fuel sources, depending on season and region. RWB emissions are poorly constrained; thus emissions inventories need improvement. Harmonizing emission factors between countries is likely the most important step to improve model calculations for biomass burning emissions and European PM2.5 concentrations in general.
Nikolaos Evangeliou, Arve Kylling, Sabine Eckhardt, Viktor Myroniuk, Kerstin Stebel, Ronan Paugam, Sergiy Zibtsev, and Andreas Stohl
Atmos. Chem. Phys., 19, 1393–1411, https://doi.org/10.5194/acp-19-1393-2019, https://doi.org/10.5194/acp-19-1393-2019, 2019
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We simulated the peatland fires that burned in Greenland in summer 2017. Using satellite data, we estimated that the total burned area was 2345 ha, the fuel amount consumed 117 kt C and the emissions of BC, OC and BrC 23.5, 731 and 141 t, respectively. About 30 % of the emissions were deposited on snow or ice surfaces. This caused a maximum albedo change of 0.007 and a surface radiative forcing of 0.03–0.04 W m−2, with local maxima of up to 0.63–0.77 W m−2. Overall, the fires had a small impact.
Stephen M. Platt, Sabine Eckhardt, Benedicte Ferré, Rebecca E. Fisher, Ove Hermansen, Pär Jansson, David Lowry, Euan G. Nisbet, Ignacio Pisso, Norbert Schmidbauer, Anna Silyakova, Andreas Stohl, Tove M. Svendby, Sunil Vadakkepuliyambatta, Jürgen Mienert, and Cathrine Lund Myhre
Atmos. Chem. Phys., 18, 17207–17224, https://doi.org/10.5194/acp-18-17207-2018, https://doi.org/10.5194/acp-18-17207-2018, 2018
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We measured atmospheric mixing ratios of methane over the Arctic Ocean around Svalbard and compared observed variations to inventories for anthropogenic, wetland, and biomass burning methane emissions and an atmospheric transport model. With knowledge of where variations were expected due to the aforementioned land-based emissions, we were able to identify and quantify a methane source from the ocean north of Svalbard, likely from sub-sea hydrocarbon seeps and/or gas hydrate decomposition.
Nikolaos Evangeliou, Rona L. Thompson, Sabine Eckhardt, and Andreas Stohl
Atmos. Chem. Phys., 18, 15307–15327, https://doi.org/10.5194/acp-18-15307-2018, https://doi.org/10.5194/acp-18-15307-2018, 2018
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We present BC inversions at high northern latitudes in 2013–2015. The emissions were high close to the gas flaring regions in Russia and in western Canada. The posterior emissions of BC at latitudes > 50° N were estimated as 560 ± 171 kt yr-1, smaller than in bottom-up inventories. Posterior concentrations over the Arctic compared with independent observations from flight and ship campaigns showed small biases. Seasonal maxima were estimated in summer months due to biomass burning, mainly in Europe.
Lauren M. Zamora, Ralph A. Kahn, Klaus B. Huebert, Andreas Stohl, and Sabine Eckhardt
Atmos. Chem. Phys., 18, 14949–14964, https://doi.org/10.5194/acp-18-14949-2018, https://doi.org/10.5194/acp-18-14949-2018, 2018
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We use satellite data and model output to estimate how airborne particles (aerosols) affect cloud ice particles and droplets over the Arctic Ocean. Aerosols from sources like smoke and pollution can change cloud cover, precipitation frequency, and the portion of liquid- vs. ice-containing clouds, which in turn can impact the surface energy budget. By improving our understanding these aerosol–cloud interactions, this work can help climate predictions for the rapidly changing Arctic.
Céline Cornet, Laurent C.-Labonnote, Fabien Waquet, Frédéric Szczap, Lucia Deaconu, Frédéric Parol, Claudine Vanbauce, François Thieuleux, and Jérôme Riédi
Atmos. Meas. Tech., 11, 3627–3643, https://doi.org/10.5194/amt-11-3627-2018, https://doi.org/10.5194/amt-11-3627-2018, 2018
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Simulations of total and polarized cloud reflectance angular signatures such as the ones measured by the multi-angular and polarized radiometer POLDER3/PARASOL are used to evaluate cloud heterogeneity effects on cloud parameter retrievals. Effects on optical thickness, albedo of the cloudy scenes, effective radius and variance of the cloud droplet size distribution, cloud top pressure and aerosol above cloud are analyzed.
Nikolaos Evangeliou, Vladimir P. Shevchenko, Karl Espen Yttri, Sabine Eckhardt, Espen Sollum, Oleg S. Pokrovsky, Vasily O. Kobelev, Vladimir B. Korobov, Andrey A. Lobanov, Dina P. Starodymova, Sergey N. Vorobiev, Rona L. Thompson, and Andreas Stohl
Atmos. Chem. Phys., 18, 963–977, https://doi.org/10.5194/acp-18-963-2018, https://doi.org/10.5194/acp-18-963-2018, 2018
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We present EC measurements from an uncertain region in terms of emissions (Russia). Its origin is quantified with a Lagrangian model that uses a recently developed feature that allows backward estimation of the specific source locations that contribute to the deposited mass. In NW European Russia transportation and domestic combustion from Finland was important. A systematic underestimation was found in W Siberia at places where gas flaring was important, implying miscalculation or sources.
Bastien Sauvage, Alain Fontaine, Sabine Eckhardt, Antoine Auby, Damien Boulanger, Hervé Petetin, Ronan Paugam, Gilles Athier, Jean-Marc Cousin, Sabine Darras, Philippe Nédélec, Andreas Stohl, Solène Turquety, Jean-Pierre Cammas, and Valérie Thouret
Atmos. Chem. Phys., 17, 15271–15292, https://doi.org/10.5194/acp-17-15271-2017, https://doi.org/10.5194/acp-17-15271-2017, 2017
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We provide the scientific community with a SOFT-IO tool based on the coupling of Lagrangian modeling with emission inventories and aircraft CO measurements, which is able to calculate the contribution of the sources and geographical origins of CO measurements, with good performances. Calculated CO added-value products will help scientists in interpreting large IAGOS CO data set. SOFT-IO could further be applied to other CO data sets or used to help validate emission inventories.
Sabine Eckhardt, Massimo Cassiani, Nikolaos Evangeliou, Espen Sollum, Ignacio Pisso, and Andreas Stohl
Geosci. Model Dev., 10, 4605–4618, https://doi.org/10.5194/gmd-10-4605-2017, https://doi.org/10.5194/gmd-10-4605-2017, 2017
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We extend the backward modelling technique in the existing model FLEXPART to substances deposited at the Earth’s surface by wet scavenging and dry deposition. This means that for existing measurements of a substance in snow, ice cores or rain samples the source regions can be determined. This will help the interpretation of the measurement as well as gaining information of emission strength at the source of the deposited substance.
Mathias Gergely, Steven J. Cooper, and Timothy J. Garrett
Atmos. Chem. Phys., 17, 12011–12030, https://doi.org/10.5194/acp-17-12011-2017, https://doi.org/10.5194/acp-17-12011-2017, 2017
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This study investigates the importance of snowflake surface-area-to-volume ratio (SAV) for the interpretation of snowfall triple-frequency radar signatures. The results indicate that snowflake SAV has a strong impact on modeled snowfall radar signatures and therefore may be used to further constrain (the large variety and high natural variability of) snowflake shape for snowfall remote sensing, e.g., to distinguish graupel snow from snowfall characterized by large aggregate snowflakes.
Franz Conen, Sabine Eckhardt, Hans Gundersen, Andreas Stohl, and Karl Espen Yttri
Atmos. Chem. Phys., 17, 11065–11073, https://doi.org/10.5194/acp-17-11065-2017, https://doi.org/10.5194/acp-17-11065-2017, 2017
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Observation of ice nuclei active at −8 °C show that rainfall drives their abundance throughout all seasons and that they are equally distributed amongst coarse and fine fraction of PM10. Concurrent measurements of fungal spore markers suggest that some fraction of INP-8 may consist of fungal spores during the warm part of the year. Snow cover suppresses the aerosolisation of ice nuclei. Changes in snow cover and rainfall may affect atmospheric concentrations of ice nuclei in future.
Christine D. Groot Zwaaftink, Ólafur Arnalds, Pavla Dagsson-Waldhauserova, Sabine Eckhardt, Joseph M. Prospero, and Andreas Stohl
Atmos. Chem. Phys., 17, 10865–10878, https://doi.org/10.5194/acp-17-10865-2017, https://doi.org/10.5194/acp-17-10865-2017, 2017
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How much dust do Icelandic sources emit and where is this dust deposited? We modelled dust emission and transport from Icelandic sources over 27 years with FLEXPART. Results show that Icelandic dust sources can have emission rates similar to parts of the Sahara and considerable amounts of dust are deposited in the ocean and on glaciers.
Lauren M. Zamora, Ralph A. Kahn, Sabine Eckhardt, Allison McComiskey, Patricia Sawamura, Richard Moore, and Andreas Stohl
Atmos. Chem. Phys., 17, 7311–7332, https://doi.org/10.5194/acp-17-7311-2017, https://doi.org/10.5194/acp-17-7311-2017, 2017
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Clouds have a major but uncertain effect on Arctic surface temperatures. Here, we used remote sensing observations to better understand aerosol effects on one type of Arctic cloud. By modifying a variety of cloud properties, aerosols in this type of cloud indirectly reduced the net warming effect of these clouds on the surface by ~ 10 % of the clean-background cloud effect, not including changes in cloud fraction. This work will improve our ability to predict future Arctic surface temperatures.
Henrik Grythe, Nina I. Kristiansen, Christine D. Groot Zwaaftink, Sabine Eckhardt, Johan Ström, Peter Tunved, Radovan Krejci, and Andreas Stohl
Geosci. Model Dev., 10, 1447–1466, https://doi.org/10.5194/gmd-10-1447-2017, https://doi.org/10.5194/gmd-10-1447-2017, 2017
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A new and more physically based treatment of how removal by precipitation is calculated by FLEXPART is introduced to take into account more aspects of aerosol diversity. Also new is the definition of clouds and cloud properties. Results from simulations show good agreement with observed atmospheric concentrations for distinctly different aerosols. Atmospheric lifetimes were found to vary from a few hours (large aerosol particles) up to a month (small non-soluble particles)
Guillaume Merlin, Jérôme Riedi, Laurent C. Labonnote, Céline Cornet, Anthony B. Davis, Phillipe Dubuisson, Marine Desmons, Nicolas Ferlay, and Frédéric Parol
Atmos. Meas. Tech., 9, 4977–4995, https://doi.org/10.5194/amt-9-4977-2016, https://doi.org/10.5194/amt-9-4977-2016, 2016
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The vertical distribution of cloud cover has a significant impact on a large number of meteorological and climatic processes. Cloud top altitude (CTOP) and cloud geometrical thickness (CGT) are essential for understanding these processes. Previous studies established the possibility of retrieving those parameters from multi-angular oxygen A-band measurements. Here we perform a study and comparison of the performance of future instruments.
Husi Letu, Hiroshi Ishimoto, Jerome Riedi, Takashi Y. Nakajima, Laurent C.-Labonnote, Anthony J. Baran, Takashi M. Nagao, and Miho Sekiguchi
Atmos. Chem. Phys., 16, 12287–12303, https://doi.org/10.5194/acp-16-12287-2016, https://doi.org/10.5194/acp-16-12287-2016, 2016
Souichiro Hioki, Ping Yang, Bryan A. Baum, Steven Platnick, Kerry G. Meyer, Michael D. King, and Jerome Riedi
Atmos. Chem. Phys., 16, 7545–7558, https://doi.org/10.5194/acp-16-7545-2016, https://doi.org/10.5194/acp-16-7545-2016, 2016
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The degree of surface roughness of ice particles within thick, cold ice clouds is inferred from multi-directional, multi-spectral satellite polarimetric observations over oceans, assuming a column-aggregate particle habit. An improved roughness inference scheme is employed, which provides a more noise-resilient roughness estimate than the conventional approach. A global one-month data sample shows the use and the limit of a severely roughened ice habit to simulate the polarized reflectivity.
N. Evangeliou, Y. Balkanski, W. M. Hao, A. Petkov, R. P. Silverstein, R. Corley, B. L. Nordgren, S. P. Urbanski, S. Eckhardt, A. Stohl, P. Tunved, S. Crepinsek, A. Jefferson, S. Sharma, J. K. Nøjgaard, and H. Skov
Atmos. Chem. Phys., 16, 7587–7604, https://doi.org/10.5194/acp-16-7587-2016, https://doi.org/10.5194/acp-16-7587-2016, 2016
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In this study, we focused on how vegetation fires that occurred in northern Eurasia during the period 2002–2013 influenced the budget of BC in the Arctic. An average area of 250 000 km2 yr−1 was burned in northern Eurasia and the global emissions of BC ranged between 8.0 and 9.5 Tg yr−1, while 102 ± 29 kt yr−1 BC from biomass burning was deposited on the Arctic. About 46 % of the Arctic BC from vegetation fires originated from Siberia, 6 % from Kazakhstan, 5 % from Europe, and about 1 % from Mon
Benjamin Marchant, Steven Platnick, Kerry Meyer, G. Thomas Arnold, and Jérôme Riedi
Atmos. Meas. Tech., 9, 1587–1599, https://doi.org/10.5194/amt-9-1587-2016, https://doi.org/10.5194/amt-9-1587-2016, 2016
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The current paper presents the new MODIS Collection 6 (C6) cloud thermodynamic phase classification algorithm. To evaluate the performance of the C6 cloud phase algorithm, extensive granule-level and global comparisons have been conducted against the heritage C5 algorithm and CALIOP. A wholesale improvement is seen for C6 compared to C5.
T. J. Garrett
Earth Syst. Dynam., 6, 673–688, https://doi.org/10.5194/esd-6-673-2015, https://doi.org/10.5194/esd-6-673-2015, 2015
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GCMs and economic models are often coupled for climate scenarios. Here, what is examined is how well a simple non-equilibrium thermodynamic model can represent the multi-decadal growth of global civilization. Initialized with growth trends from the 1950s, the model attains high skill at hindcasting how fast the GDP and energy consumption grew during the 2000s. This opens treating the coupled economy and climate as a physically deterministic response to available flows of energy and matter.
A. Stohl, B. Aamaas, M. Amann, L. H. Baker, N. Bellouin, T. K. Berntsen, O. Boucher, R. Cherian, W. Collins, N. Daskalakis, M. Dusinska, S. Eckhardt, J. S. Fuglestvedt, M. Harju, C. Heyes, Ø. Hodnebrog, J. Hao, U. Im, M. Kanakidou, Z. Klimont, K. Kupiainen, K. S. Law, M. T. Lund, R. Maas, C. R. MacIntosh, G. Myhre, S. Myriokefalitakis, D. Olivié, J. Quaas, B. Quennehen, J.-C. Raut, S. T. Rumbold, B. H. Samset, M. Schulz, Ø. Seland, K. P. Shine, R. B. Skeie, S. Wang, K. E. Yttri, and T. Zhu
Atmos. Chem. Phys., 15, 10529–10566, https://doi.org/10.5194/acp-15-10529-2015, https://doi.org/10.5194/acp-15-10529-2015, 2015
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This paper presents a summary of the findings of the ECLIPSE EU project. The project has investigated the climate and air quality impacts of short-lived climate pollutants (especially methane, ozone, aerosols) and has designed a global mitigation strategy that maximizes co-benefits between air quality and climate policy. Transient climate model simulations allowed quantifying the impacts on temperature (e.g., reduction in global warming by 0.22K for the decade 2041-2050) and precipitation.
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
S. Eckhardt, B. Quennehen, D. J. L. Olivié, T. K. Berntsen, R. Cherian, J. H. Christensen, W. Collins, S. Crepinsek, N. Daskalakis, M. Flanner, A. Herber, C. Heyes, Ø. Hodnebrog, L. Huang, M. Kanakidou, Z. Klimont, J. Langner, K. S. Law, M. T. Lund, R. Mahmood, A. Massling, S. Myriokefalitakis, I. E. Nielsen, J. K. Nøjgaard, J. Quaas, P. K. Quinn, J.-C. Raut, S. T. Rumbold, M. Schulz, S. Sharma, R. B. Skeie, H. Skov, T. Uttal, K. von Salzen, and A. Stohl
Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, https://doi.org/10.5194/acp-15-9413-2015, 2015
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The concentrations of sulfate, black carbon and other aerosols in the Arctic are characterized by high values in late winter and spring (so-called Arctic Haze) and low values in summer. Models have long been struggling to capture this seasonality. In this study, we evaluate sulfate and BC concentrations from different updated models and emissions against a comprehensive pan-Arctic measurement data set. We find that the models improved but still struggle to get the maximum concentrations.
A. Kylling, N. Kristiansen, A. Stohl, R. Buras-Schnell, C. Emde, and J. Gasteiger
Atmos. Meas. Tech., 8, 1935–1949, https://doi.org/10.5194/amt-8-1935-2015, https://doi.org/10.5194/amt-8-1935-2015, 2015
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Water and ice clouds affect detection and retrieval of volcanic ash clouds by satellite instruments. Synthetic infrared satellite images were generated for the Eyjafjallajokull 2010 and Grimsvotn 2011 eruptions by combining weather forecast, ash transport and radiative transfer modelling. Clouds decreased the number of pixels identified as ash and generally increased the retrieved ash-mass loading compared to the cloudless case; however, large differences were seen between scenes.
H. S. Gadhavi, K. Renuka, V. Ravi Kiran, A. Jayaraman, A. Stohl, Z. Klimont, and G. Beig
Atmos. Chem. Phys., 15, 1447–1461, https://doi.org/10.5194/acp-15-1447-2015, https://doi.org/10.5194/acp-15-1447-2015, 2015
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Emission inventories are a key component of simulating past, present and future climate. In this article we have evaluated three black carbon emission inventories for emissions of India using observations made from a strategic location. Annual average simulated black carbon concentration is found to be 35% to 60% lower than observed concentration because of underestimation of emissions of southern India in the inventories.
R. L. Thompson and A. Stohl
Geosci. Model Dev., 7, 2223–2242, https://doi.org/10.5194/gmd-7-2223-2014, https://doi.org/10.5194/gmd-7-2223-2014, 2014
W. C. Keene, J. L. Moody, J. N. Galloway, J. M. Prospero, O. R. Cooper, S. Eckhardt, and J. R. Maben
Atmos. Chem. Phys., 14, 8119–8135, https://doi.org/10.5194/acp-14-8119-2014, https://doi.org/10.5194/acp-14-8119-2014, 2014
S. Zeng, J. Riedi, C. R. Trepte, D. M. Winker, and Y.-X. Hu
Atmos. Chem. Phys., 14, 7125–7134, https://doi.org/10.5194/acp-14-7125-2014, https://doi.org/10.5194/acp-14-7125-2014, 2014
K. E. Yttri, C. Lund Myhre, S. Eckhardt, M. Fiebig, C. Dye, D. Hirdman, J. Ström, Z. Klimont, and A. Stohl
Atmos. Chem. Phys., 14, 6427–6442, https://doi.org/10.5194/acp-14-6427-2014, https://doi.org/10.5194/acp-14-6427-2014, 2014
X. Fang, R. L. Thompson, T. Saito, Y. Yokouchi, J. Kim, S. Li, K. R. Kim, S. Park, F. Graziosi, and A. Stohl
Atmos. Chem. Phys., 14, 4779–4791, https://doi.org/10.5194/acp-14-4779-2014, https://doi.org/10.5194/acp-14-4779-2014, 2014
B. H. Cole, P. Yang, B. A. Baum, J. Riedi, and L. C.-Labonnote
Atmos. Chem. Phys., 14, 3739–3750, https://doi.org/10.5194/acp-14-3739-2014, https://doi.org/10.5194/acp-14-3739-2014, 2014
M. Fiebig, D. Hirdman, C. R. Lunder, J. A. Ogren, S. Solberg, A. Stohl, and R. L. Thompson
Atmos. Chem. Phys., 14, 3083–3093, https://doi.org/10.5194/acp-14-3083-2014, https://doi.org/10.5194/acp-14-3083-2014, 2014
F. Waquet, F. Peers, P. Goloub, F. Ducos, F. Thieuleux, Y. Derimian, J. Riedi, M. Chami, and D. Tanré
Atmos. Chem. Phys., 14, 1755–1768, https://doi.org/10.5194/acp-14-1755-2014, https://doi.org/10.5194/acp-14-1755-2014, 2014
J. L. Moody, W. C. Keene, O. R. Cooper, K. J. Voss, R. Aryal, S. Eckhardt, B. Holben, J. R. Maben, M. A. Izaguirre, and J. N. Galloway
Atmos. Chem. Phys., 14, 691–717, https://doi.org/10.5194/acp-14-691-2014, https://doi.org/10.5194/acp-14-691-2014, 2014
M. Cassiani, A. Stohl, and S. Eckhardt
Atmos. Chem. Phys., 13, 9975–9996, https://doi.org/10.5194/acp-13-9975-2013, https://doi.org/10.5194/acp-13-9975-2013, 2013
P. Kokkalis, A. Papayannis, V. Amiridis, R. E. Mamouri, I. Veselovskii, A. Kolgotin, G. Tsaknakis, N. I. Kristiansen, A. Stohl, and L. Mona
Atmos. Chem. Phys., 13, 9303–9320, https://doi.org/10.5194/acp-13-9303-2013, https://doi.org/10.5194/acp-13-9303-2013, 2013
S. Zeng, J. Riedi, F. Parol, C. Cornet, and F. Thieuleux
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-6-8371-2013, https://doi.org/10.5194/amtd-6-8371-2013, 2013
Revised manuscript has not been submitted
A. Stohl, Z. Klimont, S. Eckhardt, K. Kupiainen, V. P. Shevchenko, V. M. Kopeikin, and A. N. Novigatsky
Atmos. Chem. Phys., 13, 8833–8855, https://doi.org/10.5194/acp-13-8833-2013, https://doi.org/10.5194/acp-13-8833-2013, 2013
S. Eckhardt, O. Hermansen, H. Grythe, M. Fiebig, K. Stebel, M. Cassiani, A. Baecklund, and A. Stohl
Atmos. Chem. Phys., 13, 8401–8409, https://doi.org/10.5194/acp-13-8401-2013, https://doi.org/10.5194/acp-13-8401-2013, 2013
R. Kallenborn, K. Breivik, S. Eckhardt, C. R. Lunder, S. Manø, M. Schlabach, and A. Stohl
Atmos. Chem. Phys., 13, 6983–6992, https://doi.org/10.5194/acp-13-6983-2013, https://doi.org/10.5194/acp-13-6983-2013, 2013
M. Laborde, M. Crippa, T. Tritscher, Z. Jurányi, P. F. Decarlo, B. Temime-Roussel, N. Marchand, S. Eckhardt, A. Stohl, U. Baltensperger, A. S. H. Prévôt, E. Weingartner, and M. Gysel
Atmos. Chem. Phys., 13, 5831–5856, https://doi.org/10.5194/acp-13-5831-2013, https://doi.org/10.5194/acp-13-5831-2013, 2013
T. J. Garrett and C. Zhao
Atmos. Meas. Tech., 6, 1227–1243, https://doi.org/10.5194/amt-6-1227-2013, https://doi.org/10.5194/amt-6-1227-2013, 2013
F. Waquet, C. Cornet, J.-L. Deuzé, O. Dubovik, F. Ducos, P. Goloub, M. Herman, T. Lapyonok, L. C. Labonnote, J. Riedi, D. Tanré, F. Thieuleux, and C. Vanbauce
Atmos. Meas. Tech., 6, 991–1016, https://doi.org/10.5194/amt-6-991-2013, https://doi.org/10.5194/amt-6-991-2013, 2013
B. van Diedenhoven, B. Cairns, A. M. Fridlind, A. S. Ackerman, and T. J. Garrett
Atmos. Chem. Phys., 13, 3185–3203, https://doi.org/10.5194/acp-13-3185-2013, https://doi.org/10.5194/acp-13-3185-2013, 2013
A. Kylling, R. Buras, S. Eckhardt, C. Emde, B. Mayer, and A. Stohl
Atmos. Meas. Tech., 6, 649–660, https://doi.org/10.5194/amt-6-649-2013, https://doi.org/10.5194/amt-6-649-2013, 2013
F. Freutel, J. Schneider, F. Drewnick, S.-L. von der Weiden-Reinmüller, M. Crippa, A. S. H. Prévôt, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, R. Sarda-Estève, J. F. Burkhart, S. Eckhardt, A. Stohl, V. Gros, A. Colomb, V. Michoud, J. F. Doussin, A. Borbon, M. Haeffelin, Y. Morille, M. Beekmann, and S. Borrmann
Atmos. Chem. Phys., 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, https://doi.org/10.5194/acp-13-933-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
A survey of radiative and physical properties of North Atlantic mesoscale cloud morphologies from multiple identification methodologies
Extensive coverage of ultrathin tropical tropopause layer cirrus clouds revealed by balloon-borne lidar observations
The effects of warm-air intrusions in the high Arctic on cirrus clouds
The characteristics of cloud macro-parameters caused by the seeder–feeder process inside clouds measured by millimeter-wave cloud radar in Xi'an, China
Shallow- and deep-convection characteristics in the greater Houston, Texas, area using cell tracking methodology
Observations of the macrophysical properties of cumulus cloud fields over the tropical western Pacific and their connection to meteorological variables
A Lagrangian perspective on the lifecycle and cloud radiative effect of deep convective clouds over Africa
Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic
Technical note: Retrieval of the supercooled liquid fraction in mixed-phase clouds from Himawari-8 observations
Technical note: Bimodal parameterizations of in situ ice cloud particle size distributions
Inter-relations of precipitation, aerosols, and clouds over Andalusia, southern Spain, revealed by the Andalusian Global ObseRvatory of the Atmosphere (AGORA)
On the relationship between mesoscale cellular convection and meteorological forcing: comparing the Southern Ocean against the North Pacific
Aerosol-related effects on the occurrence of heterogeneous ice formation over Lauder, New Zealand ∕ Aotearoa
Low-level Arctic clouds: a blind zone in our knowledge of the radiation budget
Climatologically invariant scale invariance seen in distributions of cloud horizontal sizes
Variability and properties of liquid-dominated clouds over the ice-free and sea-ice-covered Arctic Ocean
The correlation between Arctic sea ice, cloud phase and radiation using A-train satellites
Asymmetries in cloud microphysical properties ascribed to sea ice leads via water vapour transport in the central Arctic
Quantifying the dependence of drop spectrum width on cloud drop number concentration for cloud remote sensing
The evolution of deep convective systems and their associated cirrus outflows
Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean
Characterisation of low-base and mid-base clouds and their thermodynamic phase over the Southern and Arctic Ocean
Rapid saturation of cloud water adjustments to shipping emissions
Sensitivities of cloud radiative effects to large-scale meteorology and aerosols from global observations
Distinct secondary ice production processes observed in radar Doppler spectra: insights from a case study
Investigating the development of clouds within marine cold-air outbreaks
Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations
Examining cloud vertical structure and radiative effects from satellite retrievals and evaluation of CMIP6 scenarios
Influence of cloud microphysics schemes on weather model predictions of heavy precipitation
Convective organization and 3D structure of tropical cloud systems deduced from synergistic A-Train observations and machine learning
Seasonal controls on isolated convective storm drafts, precipitation intensity, and life cycle as observed during GoAmazon2014/5
Uncertainty in aerosol–cloud radiative forcing is driven by clean conditions
Surface-based observations of cold-air outbreak clouds during the COMBLE field campaign
Boundary layer moisture variability at the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic observatory during marine conditions
Profile-based estimated inversion strength
Characteristics of supersaturation in midlatitude cirrus clouds and their adjacent cloud-free air
Establishment of an analytical model for remote sensing of typical stratocumulus cloud profiles under various precipitation and entrainment conditions
Satellite remote sensing of regional and seasonal Arctic cooling showing a multi-decadal trend towards brighter and more liquid clouds
Microphysical processes of super typhoon Lekima (2019) and their impacts on polarimetric radar remote sensing of precipitation
The impacts of dust aerosol and convective available potential energy on precipitation vertical structure in southeastern China as seen from multisource observations
Heavy snowfall event over the Swiss Alps: did wind shear impact secondary ice production?
On the global relationship between polarimetric radio occultation differential phase shift and ice water content
Observations of microphysical properties and radiative effects of a contrail cirrus outbreak over the North Atlantic
Natural marine cloud brightening in the Southern Ocean
Distinct regional meteorological influences on low-cloud albedo susceptibility over global marine stratocumulus regions
Diurnal cycles of cloud cover and its vertical distribution over the Tibetan Plateau revealed by satellite observations, reanalysis datasets, and CMIP6 outputs
Satellite observations of seasonality and long-term trends in cirrus cloud properties over Europe: investigation of possible aviation impacts
Ice crystal characterization in cirrus clouds III: retrieval of ice crystal shape and roughness from observations of halo displays
Technical note: Identification of two ice-nucleating regimes for dust-related cirrus clouds based on the relationship between number concentrations of ice-nucleating particles and ice crystals
Highly supercooled riming and unusual triple-frequency radar signatures over McMurdo Station, Antarctica
Ryan Eastman, Isabel L. McCoy, Hauke Schulz, and Robert Wood
Atmos. Chem. Phys., 24, 6613–6634, https://doi.org/10.5194/acp-24-6613-2024, https://doi.org/10.5194/acp-24-6613-2024, 2024
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for 1 year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is, in part, a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds' radiative effect. Future studies must account for differing properties and processes among cloud types.
Thomas Lesigne, François Ravetta, Aurélien Podglajen, Vincent Mariage, and Jacques Pelon
Atmos. Chem. Phys., 24, 5935–5952, https://doi.org/10.5194/acp-24-5935-2024, https://doi.org/10.5194/acp-24-5935-2024, 2024
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Upper tropical clouds have a strong impact on Earth's climate but are challenging to observe. We report the first long-duration observations of tropical clouds from lidars flying on board stratospheric balloons. Comparisons with spaceborne observations reveal the enhanced sensitivity of balloon-borne lidar to optically thin cirrus. These clouds, which have a significant coverage and lie in the uppermost troposphere, are linked with the dehydration of air masses on their way to the stratosphere.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
Atmos. Chem. Phys., 24, 5971–5987, https://doi.org/10.5194/acp-24-5971-2024, https://doi.org/10.5194/acp-24-5971-2024, 2024
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For decades the earth's temperature has been rising. The Arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm-air intrusions, air masses are transported into the Arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Huige Di and Yun Yuan
Atmos. Chem. Phys., 24, 5783–5801, https://doi.org/10.5194/acp-24-5783-2024, https://doi.org/10.5194/acp-24-5783-2024, 2024
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We observed the seeder–feeder process among double-layer clouds using a cloud radar and microwave radiometer. By defining the parameters of the seeding depth and seeding time of the upper cloud affecting the lower cloud, we find that the cloud particle terminal velocity is significantly enhanced during the seeder–feeder period, and the lower the height and thinner the thickness of the height difference between double-layer clouds, the lower the height and thicker the thickness of seeding depth.
Kristofer S. Tuftedal, Bernat Puigdomènech Treserras, Mariko Oue, and Pavlos Kollias
Atmos. Chem. Phys., 24, 5637–5657, https://doi.org/10.5194/acp-24-5637-2024, https://doi.org/10.5194/acp-24-5637-2024, 2024
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This study analyzed coastal convective cells from June through September 2018–2021. The cells were classified and their lifecycles were analyzed to better understand their characteristics. Features such as convective-core growth, for example, are shown. The study found differences in the initiation location of shallow convection and in the aerosol loading in deep convective environments. This work provides a foundation for future analyses of convection or other tracked events elsewhere.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
William K. Jones, Martin Stengel, and Philip Stier
Atmos. Chem. Phys., 24, 5165–5180, https://doi.org/10.5194/acp-24-5165-2024, https://doi.org/10.5194/acp-24-5165-2024, 2024
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Storm clouds cover large areas of the tropics. These clouds both reflect incoming sunlight and trap heat from the atmosphere below, regulating the temperature of the tropics. Over land, storm clouds occur in the late afternoon and evening and so exist both during the daytime and at night. Changes in this timing could upset the balance of the respective cooling and heating effects of these clouds. We find that isolated storms have a larger effect on this balance than their small size suggests.
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
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The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Ziming Wang, Husi Letu, Huazhe Shang, and Luca Bugliaro
EGUsphere, https://doi.org/10.5194/egusphere-2023-2667, https://doi.org/10.5194/egusphere-2023-2667, 2024
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Supercooled liquid fraction (SLF) in mixed-phase clouds is retrieved for the first time using passive geostationary satellite observations based on differences in liquid droplet and ice particle radiative properties. The retrieved results are well comparable to global distributions observed by active instruments, and the feasibility of the retrieval method to analyze the observed trends of SLF has been validated.
Irene Bartolomé García, Odran Sourdeval, Reinhold Spang, and Martina Krämer
Atmos. Chem. Phys., 24, 1699–1716, https://doi.org/10.5194/acp-24-1699-2024, https://doi.org/10.5194/acp-24-1699-2024, 2024
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How many ice crystals of each size are in a cloud is a key parameter for the retrieval of cloud properties. The distribution of ice crystals is obtained from in situ measurements and used to create parameterizations that can be used when analyzing the remote-sensing data. Current parameterizations are based on data sets that do not include reliable measurements of small crystals, but in our study we use a data set that includes very small ice crystals to improve these parameterizations.
Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, Lucas Alados-Arboledas, Agustín Millares, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 24, 1571–1585, https://doi.org/10.5194/acp-24-1571-2024, https://doi.org/10.5194/acp-24-1571-2024, 2024
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The south-central interior of Andalusia experiences complex precipitation patterns as a result of the semi-arid Mediterranean climate and the influence of Saharan dust. This study monitored the inter-relations between aerosols, clouds, meteorological variables, and precipitation systems using ground-based remote sensing and in situ instruments.
Francisco Lang, Steven T. Siems, Yi Huang, Tahereh Alinejadtabrizi, and Luis Ackermann
Atmos. Chem. Phys., 24, 1451–1466, https://doi.org/10.5194/acp-24-1451-2024, https://doi.org/10.5194/acp-24-1451-2024, 2024
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Marine low-level clouds play a crucial role in the Earth's energy balance, trapping heat from the surface and reflecting sunlight back into space. These clouds are distinguishable by their large-scale spatial structures, primarily characterized as hexagonal patterns with either filled (closed) or empty (open) cells. Utilizing satellite observations, these two cloud type patterns have been categorized over the Southern Ocean and North Pacific Ocean through a pattern recognition program.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
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An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Hannes Jascha Griesche, Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 24, 597–612, https://doi.org/10.5194/acp-24-597-2024, https://doi.org/10.5194/acp-24-597-2024, 2024
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The Arctic is strongly affected by climate change and the role of clouds therein is not yet completely understood. Measurements from the Arctic expedition PS106 were used to simulate radiative fluxes with and without clouds at very low altitudes (below 165 m), and their radiative effect was calculated to be 54 Wm-2. The low heights of these clouds make them hard to observe. This study shows the importance of accurate measurements and simulations of clouds and gives suggestions for improvements.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Viewed from space, a defining feature of Earth's atmosphere is the wide spectrum of cloud sizes. A recent study predicted the distribution of cloud sizes, and this paper compares the prediction to observations. Although there is nuance in viewing perspective, we find robust agreement with theory across different climatological conditions, including land–ocean contrasts, time of year, or latitude, suggesting a minor role for Coriolis forces, aerosol loading, or surface temperature.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Grégory V. Cesana, Olivia Pierpaoli, Matteo Ottaviani, Linh Vu, and Zhonghai Jin
EGUsphere, https://doi.org/10.5194/egusphere-2023-2940, https://doi.org/10.5194/egusphere-2023-2940, 2023
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Better characterizing the relationship between sea ice and clouds is key to understanding Arctic climate, because clouds and sea ice affect surface radiation and modulate Arctic surface warming. Our results indicate that Arctic liquid clouds robustly increase in response to sea-ice decrease. This increase has a cooling effect on the surface, because more solar radiation is reflected back to space, and it should contribute to dampening future Arctic surface warming.
Pablo Saavedra Garfias, Heike Kalesse-Los, Luisa von Albedyll, Hannes Griesche, and Gunnar Spreen
Atmos. Chem. Phys., 23, 14521–14546, https://doi.org/10.5194/acp-23-14521-2023, https://doi.org/10.5194/acp-23-14521-2023, 2023
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An important Arctic climate process is the release of heat fluxes from sea ice openings to the atmosphere that influence the clouds. The characterization of this process is the objective of this study. Using synergistic observations from the MOSAiC expedition, we found that single-layer cloud properties show significant differences when clouds are coupled or decoupled to the water vapour transport which is used as physical link between the upwind sea ice openings and the cloud under observation.
Matthew D. Lebsock and Mikael Witte
Atmos. Chem. Phys., 23, 14293–14305, https://doi.org/10.5194/acp-23-14293-2023, https://doi.org/10.5194/acp-23-14293-2023, 2023
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This paper evaluates measurements of cloud drop size distributions made from airplanes. We find that as the number of cloud drops increases the distribution of the cloud drop sizes narrows. The data are used to develop a simple equation that relates the drop number to the width of the drop sizes. We then use this equation to demonstrate that existing approaches to observe the drop number from satellites contain errors that can be corrected by including the new relationship.
George Horner and Edward Gryspeerdt
Atmos. Chem. Phys., 23, 14239–14253, https://doi.org/10.5194/acp-23-14239-2023, https://doi.org/10.5194/acp-23-14239-2023, 2023
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Tropical deep convective clouds, and the thin cirrus (ice) clouds that flow out from them, are important for modulating the energy budget of the tropical atmosphere. This work uses a new method to track the evolution of the properties of these clouds across their entire lifetimes. We find these clouds cool the atmosphere in the first 6 h before switching to a warming regime after the deep convective core has dissipated, which is sustained beyond 120 h from the initial convective event.
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
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For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Barbara Dietel, Odran Sourdeval, and Corinna Hoose
EGUsphere, https://doi.org/10.5194/egusphere-2023-2281, https://doi.org/10.5194/egusphere-2023-2281, 2023
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The uncertainty of cloud phase over the Southern Ocean and the Arctic Ocean leads to large uncertainties in the radiation budget of weather and climate models. This study investigates the phase of low-base and mid-base clouds using satellite-based remote sensing data. A comprehensive analysis of the correlation of cloud phase with various parameters such as temperature, aerosols, sea ice, vertical and horizontal cloud extent, and cloud radiative effect is presented.
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
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Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
Hendrik Andersen, Jan Cermak, Alyson Douglas, Timothy A. Myers, Peer Nowack, Philip Stier, Casey J. Wall, and Sarah Wilson Kemsley
Atmos. Chem. Phys., 23, 10775–10794, https://doi.org/10.5194/acp-23-10775-2023, https://doi.org/10.5194/acp-23-10775-2023, 2023
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This study uses an observation-based cloud-controlling factor framework to study near-global sensitivities of cloud radiative effects to a large number of meteorological and aerosol controls. We present near-global sensitivity patterns to selected thermodynamic, dynamic, and aerosol factors and discuss the physical mechanisms underlying the derived sensitivities. Our study hopes to guide future analyses aimed at constraining cloud feedbacks and aerosol–cloud interactions.
Anne-Claire Billault-Roux, Paraskevi Georgakaki, Josué Gehring, Louis Jaffeux, Alfons Schwarzenboeck, Pierre Coutris, Athanasios Nenes, and Alexis Berne
Atmos. Chem. Phys., 23, 10207–10234, https://doi.org/10.5194/acp-23-10207-2023, https://doi.org/10.5194/acp-23-10207-2023, 2023
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Secondary ice production plays a key role in clouds and precipitation. In this study, we analyze radar measurements from a snowfall event in the Jura Mountains. Complex signatures are observed, which reveal that ice crystals were formed through various processes. An analysis of multi-sensor data suggests that distinct ice multiplication processes were taking place. Both the methods used and the insights gained through this case study contribute to a better understanding of snowfall microphysics.
Rebecca J. Murray-Watson, Edward Gryspeerdt, and Tom Goren
Atmos. Chem. Phys., 23, 9365–9383, https://doi.org/10.5194/acp-23-9365-2023, https://doi.org/10.5194/acp-23-9365-2023, 2023
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Clouds formed in Arctic marine cold air outbreaks undergo a distinct evolution, but the factors controlling their transition from high-coverage to broken cloud fields are poorly understood. We use satellite and reanalysis data to study how these clouds develop in time and the different influences on their evolution. The aerosol concentration is correlated with cloud break-up; more aerosol is linked to prolonged coverage and a stronger cooling effect, with implications for a more polluted Arctic.
Michael S. Diamond
Atmos. Chem. Phys., 23, 8259–8269, https://doi.org/10.5194/acp-23-8259-2023, https://doi.org/10.5194/acp-23-8259-2023, 2023
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Fuel sulfur regulations were implemented for ships in 2020 to improve air quality but may also accelerate global warming. We use spatial statistics and satellite retrievals to detect changes in the size of cloud droplets and find evidence for a resulting decrease in cloud brightness within a major shipping corridor after the sulfur limits went into effect. Our results confirm both that the regulations are being followed and that they are having a warming influence via their effect on clouds.
Hao Luo, Johannes Quaas, and Yong Han
Atmos. Chem. Phys., 23, 8169–8186, https://doi.org/10.5194/acp-23-8169-2023, https://doi.org/10.5194/acp-23-8169-2023, 2023
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Clouds exhibit a wide range of vertical structures with varying microphysical and radiative properties. We show a global survey of spatial distribution, vertical extent and radiative effect of various classified cloud vertical structures using joint satellite observations from the new CCCM datasets during 2007–2010. Moreover, the long-term trends in CVSs are investigated based on different CMIP6 future scenarios to capture the cloud variations with different, increasing anthropogenic forcings.
Gregor Köcher, Tobias Zinner, and Christoph Knote
Atmos. Chem. Phys., 23, 6255–6269, https://doi.org/10.5194/acp-23-6255-2023, https://doi.org/10.5194/acp-23-6255-2023, 2023
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Polarimetric radar observations of 30 d of convective precipitation events are used to statistically analyze 5 state-of-the-art microphysics schemes of varying complexity. The frequency and area of simulated heavy-precipitation events are in some cases significantly different from those observed, depending on the microphysics scheme. Analysis of simulated particle size distributions and reflectivities shows that some schemes have problems reproducing the correct particle size distributions.
Claudia J. Stubenrauch, Giulio Mandorli, and Elisabeth Lemaitre
Atmos. Chem. Phys., 23, 5867–5884, https://doi.org/10.5194/acp-23-5867-2023, https://doi.org/10.5194/acp-23-5867-2023, 2023
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Organized convection leads to large convective cloud systems and intense rain and may change with a warming climate. Their complete 3D description, attained by machine learning techniques in combination with various satellite observations, together with a cloud system concept, link convection to anvil properties, while convective organization can be identified by the horizontal structure of intense rain.
Scott E. Giangrande, Thiago S. Biscaro, and John M. Peters
Atmos. Chem. Phys., 23, 5297–5316, https://doi.org/10.5194/acp-23-5297-2023, https://doi.org/10.5194/acp-23-5297-2023, 2023
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Our study tracks thunderstorms observed during the wet and dry seasons of the Amazon Basin using weather radar. We couple this precipitation tracking with opportunistic overpasses of a wind profiler and other ground observations to add unique insights into the upwards and downwards air motions within these clouds at various stages in the storm life cycle. The results of a simple updraft model are provided to give physical explanations for observed seasonal differences.
Edward Gryspeerdt, Adam C. Povey, Roy G. Grainger, Otto Hasekamp, N. Christina Hsu, Jane P. Mulcahy, Andrew M. Sayer, and Armin Sorooshian
Atmos. Chem. Phys., 23, 4115–4122, https://doi.org/10.5194/acp-23-4115-2023, https://doi.org/10.5194/acp-23-4115-2023, 2023
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The impact of aerosols on clouds is one of the largest uncertainties in the human forcing of the climate. Aerosol can increase the concentrations of droplets in clouds, but observational and model studies produce widely varying estimates of this effect. We show that these estimates can be reconciled if only polluted clouds are studied, but this is insufficient to constrain the climate impact of aerosol. The uncertainty in aerosol impact on clouds is currently driven by cases with little aerosol.
Zackary Mages, Pavlos Kollias, Zeen Zhu, and Edward P. Luke
Atmos. Chem. Phys., 23, 3561–3574, https://doi.org/10.5194/acp-23-3561-2023, https://doi.org/10.5194/acp-23-3561-2023, 2023
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Cold-air outbreaks (when cold air is advected over warm water and creates low-level convection) are a dominant cloud regime in the Arctic, and we capitalized on ground-based observations, which did not previously exist, from the COMBLE field campaign to study them. We characterized the extent and strength of the convection and turbulence and found evidence of secondary ice production. This information is useful for model intercomparison studies that will represent cold-air outbreak processes.
Maria P. Cadeddu, Virendra P. Ghate, David D. Turner, and Thomas E. Surleta
Atmos. Chem. Phys., 23, 3453–3470, https://doi.org/10.5194/acp-23-3453-2023, https://doi.org/10.5194/acp-23-3453-2023, 2023
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We analyze the variability in marine boundary layer moisture at the Eastern North Atlantic site on a monthly and daily temporal scale and examine its fundamental role in the control of boundary layer cloudiness and precipitation. The study also highlights the complex interaction between large-scale and local processes controlling the boundary layer moisture and the importance of the mesoscale spatial distribution of vapor to support convection and precipitation.
Zhenquan Wang, Jian Yuan, Robert Wood, Yifan Chen, and Tiancheng Tong
Atmos. Chem. Phys., 23, 3247–3266, https://doi.org/10.5194/acp-23-3247-2023, https://doi.org/10.5194/acp-23-3247-2023, 2023
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This study develops a novel profile-based algorithm based on the ERA5 to estimate the inversion strength in the planetary boundary layer better than the previous inversion index, which is a key low-cloud-controlling factor. This improved measure is more effective at representing the meteorological influence on low-cloud variations. It can better constrain the meteorological influence on low clouds to better isolate cloud responses to aerosols or to estimate low cloud feedbacks in climate models.
Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 23, 3103–3117, https://doi.org/10.5194/acp-23-3103-2023, https://doi.org/10.5194/acp-23-3103-2023, 2023
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Cirrus clouds affect Earth's atmosphere, deeming our study important. Here we use water vapor measurements by lidar and study the relative humidity (RHi) within and around midlatitude cirrus clouds. We find high supersaturations in the cloud-free air and within the clouds, especially near the cloud top. We study two cloud types with different formation processes. Finally, we conclude that the shape of the distribution of RHi can be used as an indicator of different cloud evolutionary stages.
Huazhe Shang, Souichiro Hioki, Guillaume Penide, Céline Cornet, Husi Letu, and Jérôme Riedi
Atmos. Chem. Phys., 23, 2729–2746, https://doi.org/10.5194/acp-23-2729-2023, https://doi.org/10.5194/acp-23-2729-2023, 2023
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We find that cloud profiles can be divided into four prominent patterns, and the frequency of these four patterns is related to intensities of cloud-top entrainment and precipitation. Based on these analyses, we further propose a cloud profile parameterization scheme allowing us to represent these patterns. Our results shed light on how to facilitate the representation of cloud profiles and how to link them to cloud entrainment or precipitating status in future remote-sensing applications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Yabin Gou, Haonan Chen, Hong Zhu, and Lulin Xue
Atmos. Chem. Phys., 23, 2439–2463, https://doi.org/10.5194/acp-23-2439-2023, https://doi.org/10.5194/acp-23-2439-2023, 2023
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This article investigates the complex precipitation microphysics associated with super typhoon Lekima using a host of in situ and remote sensing observations, including rain gauge and disdrometer data, as well as polarimetric radar observations. The impacts of precipitation microphysics on multi-source data consistency and radar precipitation estimation are quantified. It is concluded that the dynamical precipitation microphysical processes must be considered in radar precipitation estimation.
Hongxia Zhu, Rui Li, Shuping Yang, Chun Zhao, Zhe Jiang, and Chen Huang
Atmos. Chem. Phys., 23, 2421–2437, https://doi.org/10.5194/acp-23-2421-2023, https://doi.org/10.5194/acp-23-2421-2023, 2023
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The impacts of atmospheric dust aerosols and cloud dynamic conditions on precipitation vertical development in southeastern China were studied using multiple satellite observations. It was found that the precipitating drops under dusty conditions grow faster in the middle layer but slower in the upper and lower layers compared with their pristine counterparts. Quantitative estimation of the sensitivity of the precipitation top temperature to the dust aerosol optical depth is also provided.
Zane Dedekind, Jacopo Grazioli, Philip H. Austin, and Ulrike Lohmann
Atmos. Chem. Phys., 23, 2345–2364, https://doi.org/10.5194/acp-23-2345-2023, https://doi.org/10.5194/acp-23-2345-2023, 2023
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Simulations allowing ice particles to collide with one another producing more ice particles represented surface observations of ice particles accurately. An increase in ice particles formed through collisions was related to sharp changes in the wind direction and speed with height. Changes in wind speed and direction can therefore cause more enhanced collisions between ice particles and alter how fast and how much precipitation forms. Simulations were conducted with the atmospheric model COSMO.
Ramon Padullés, Estel Cardellach, and F. Joseph Turk
Atmos. Chem. Phys., 23, 2199–2214, https://doi.org/10.5194/acp-23-2199-2023, https://doi.org/10.5194/acp-23-2199-2023, 2023
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The results of comparing the polarimetric radio occultation observables and the ice water content retrieved from the CloudSat radar in a global and statistical way show a strong correlation between the geographical patterns of both quantities for a wide range of heights. This implies that horizontally oriented hydrometeors are systematically present through the whole globe and through all vertical levels, which could provide insights on the physical processes leading to precipitation.
Ziming Wang, Luca Bugliaro, Tina Jurkat-Witschas, Romy Heller, Ulrike Burkhardt, Helmut Ziereis, Georgios Dekoutsidis, Martin Wirth, Silke Groß, Simon Kirschler, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 23, 1941–1961, https://doi.org/10.5194/acp-23-1941-2023, https://doi.org/10.5194/acp-23-1941-2023, 2023
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Differences in the microphysical properties of contrail cirrus and natural cirrus in a contrail outbreak situation during the ML-CIRRUS campaign over the North Atlantic flight corridor can be observed from in situ measurements. The cirrus radiative effect in the area of the outbreak, derived from satellite observation-based radiative transfer modeling, is warming in the early morning and cooling during the day.
Gerald G. Mace, Sally Benson, Ruhi Humphries, Peter M. Gombert, and Elizabeth Sterner
Atmos. Chem. Phys., 23, 1677–1685, https://doi.org/10.5194/acp-23-1677-2023, https://doi.org/10.5194/acp-23-1677-2023, 2023
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The number of cloud droplets per unit volume is a significantly important property of clouds that controls their reflective properties. Computer models of the Earth's atmosphere and climate have low skill at predicting the reflective properties of Southern Ocean clouds. Here we investigate the properties of those clouds using satellite data and find that the cloud droplet number and cloud albedo in the Southern Ocean are related to the oceanic phytoplankton abundance near Antarctica.
Jianhao Zhang and Graham Feingold
Atmos. Chem. Phys., 23, 1073–1090, https://doi.org/10.5194/acp-23-1073-2023, https://doi.org/10.5194/acp-23-1073-2023, 2023
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Using observations from space, we show maps of potential brightness changes in marine warm clouds in response to increases in cloud droplet concentrations. The environmental and aerosol conditions in which these clouds reside covary differently in each ocean basin, leading to distinct evolutions of cloud brightness changes. This work stresses the central importance of the covariability between meteorology and aerosol for scaling up the radiative response of cloud brightness changes.
Yuxin Zhao, Jiming Li, Lijie Zhang, Cong Deng, Yarong Li, Bida Jian, and Jianping Huang
Atmos. Chem. Phys., 23, 743–769, https://doi.org/10.5194/acp-23-743-2023, https://doi.org/10.5194/acp-23-743-2023, 2023
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Diurnal variations of clouds play an important role in the radiative budget and precipitation. Based on satellite observations, reanalysis, and CMIP6 outputs, the diurnal variations in total cloud cover and cloud vertical distribution over the Tibetan Plateau are explored. The diurnal cycle of cirrus is a key focus and found to have different characteristics from those found in the tropics. The relationship between the diurnal cycle of cirrus and meteorological factors is also discussed.
Qiang Li and Silke Groß
Atmos. Chem. Phys., 22, 15963–15980, https://doi.org/10.5194/acp-22-15963-2022, https://doi.org/10.5194/acp-22-15963-2022, 2022
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The IPCC report identified that cirrus clouds have a significant impact on the radiation balance comparable to the CO2 effects, which, however, is still hard to parameterize. The current study investigates the possible impact of aviation on cirrus properties based on the analysis of 10-year lidar measurements of CALIPSO. The results reveal that there is a significant positive trend in cirrus depolarization ratio in the last 10 years before COVID-19, which is strongly correlated with aviation.
Linda Forster and Bernhard Mayer
Atmos. Chem. Phys., 22, 15179–15205, https://doi.org/10.5194/acp-22-15179-2022, https://doi.org/10.5194/acp-22-15179-2022, 2022
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We present a novel retrieval using ground-based imaging observations of halo displays together with radiative transfer simulations to help improve our understanding of ice crystal properties representative of cirrus clouds. Analysis of 4400 calibrated HaloCam images featuring a 22° halo revealed aggregates of hexagonal columns of 20 µm effective radius with a mixture of about 37 % smooth and 63% severely roughened surfaces as the best match in general.
Yun He, Zhenping Yin, Fuchao Liu, and Fan Yi
Atmos. Chem. Phys., 22, 13067–13085, https://doi.org/10.5194/acp-22-13067-2022, https://doi.org/10.5194/acp-22-13067-2022, 2022
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A method is proposed to identify the sole presence of heterogeneous nucleation and competition between heterogeneous and homogeneous nucleation for dust-related cirrus clouds by characterizing the relationship between dust ice-nucleating particle concentration calculated from CALIOP using the POLIPHON method and in-cloud ice crystal number concentration from the DARDAR-Nice dataset. Two typical cirrus cases are shown as a demonstration, and the proposed method can be extended to a global scale.
Frederic Tridon, Israel Silber, Alessandro Battaglia, Stefan Kneifel, Ann Fridlind, Petros Kalogeras, and Ranvir Dhillon
Atmos. Chem. Phys., 22, 12467–12491, https://doi.org/10.5194/acp-22-12467-2022, https://doi.org/10.5194/acp-22-12467-2022, 2022
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The role of ice precipitation in the Earth water budget is not well known because ice particles are complex, and their formation involves intricate processes. Riming of ice crystals by supercooled water droplets is an efficient process, but little is known about its importance at high latitudes. In this work, by exploiting the deployment of an unprecedented number of remote sensing systems in Antarctica, we find that riming occurs at much lower temperatures compared with the mid-latitudes.
Cited articles
Ackerman, A. S., Kirkpatrick, M. P., Stevens, D. E., and Toon, O. B.: The impact of humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432, 1014–1017, https://doi.org/10.1038/nature03137.1, 2004.
Albrecht, B. A.: Aerosols, Cloud Microphysics, and Fractional Cloudiness, Science, 245, 1227–1230, 1989.
Amann, M., Bertok, I., Borken-Kleefeld, J., Cofala, J., Heyes, C., Höglund-Isaksson, L., Klimont, Z., Nguyen, B., Posch, M., Rafaj, P., Sandler, R., Schöpp, W., Wagner, F., and Winiwarter, W.: Cost-effective control of air quality and greenhouse gases in Europe: Modeling and policy applications, Environ. Modell. Softw., 26, 1489–1501, https://doi.org/10.1016/j.envsoft.2011.07.012, 2011.
Ancellet, G., Pelon, J., Blanchard, Y., Quennehen, B., Bazureau, A., Law, K. S., and Schwarzenboeck, A.: Transport of aerosol to the Arctic: analysis of CALIOP and French aircraft data during the spring 2008 POLARCAT campaign, Atmos. Chem. Phys., 14, 8235–8254, https://doi.org/10.5194/acp-14-8235-2014, 2014.
Andersen, H. and Cermak, J.: How thermodynamic environments control stratocumulus microphysics and interactions with aerosols, Environ. Res. Lett., 10, 24004, https://doi.org/10.1088/1748-9326/10/2/024004, 2015.
Andreae, M. O. and Rosenfeld, D.: Aerosol-cloud-precipitation interactions, Part 1. The nature and sources of cloud-active aerosols, Earth-Sci. Rev., 89, 13–41, https://doi.org/10.1016/j.earscirev.2008.03.001, 2008.
Avey, L., Garrett, T. J., and Stohl, A.: Evaluation of the aerosol indirect effect using satellite, tracer transport model, and aircraft data from the International Consortium for Atmospheric Research on Transport and Transformation, J. Geophys. Res.-Atmos., 112, 1–10, https://doi.org/10.1029/2006JD007581, 2007.
Belchansky, G. I., Douglas, D. C., and Platonov, N. G.: Duration of the Arctic sea ice melt season: Regional and interannual variability, 1979-2001, J. Climate, 17, 67–80, https://doi.org/10.1175/1520-0442(2004)017<0067:DOTASI>2.0.CO;2, 2004.
Berg, L. K., Berkowitz, C. M., Barnard, J. C., Senum, G., and Springston, S. R.: Observations of the first aerosol indirect effect in shallow cumuli, Geophys. Res. Lett., 38, L03809, https://doi.org/10.1029/2010GL046047, 2011.
Berrisford, P., Dee, D., Fielding, K., Fuentes, M., Kallberg, P., Kobayashi, S., and Uppala, S.: The ERA-Interim Archive, ECMWF, Reading, UK, 1, available at: http://old.ecmwf.int/publications/library/do/references/list/782009 (last access: 11 November 2015), 2009.
Bilde, M. and Svenningsson, B.: CCN activation of slightly soluble organics: The importance of small amounts of inorganic salt and particle phase, Tellus B, 56, 128–134, https://doi.org/10.1111/j.1600-0889.2004.00090.x, 2004.
Boisvert, L. N. and Stroeve, J. C.: The Arctic is becoming warmer and wetter as revealed by the Atmospheric Infrared Sounder, Geophys. Res. Lett., 42, 4439–4446, https://doi.org/10.1002/2015GL063775, 2015.
Brenguier, J. and Wood, R.: Observational strategies from the micro to meso scale, in: Clouds in the Perturbed Climate System: Their Relationship to Energy Balance, Atmospheric Dynamics, and Precipitation, edited by: Heintzenberg, J. and Charlson, R. J., 487–510, available at: ftp://ftp-projects.zmaw.de/aerocom/meetings/frankfurt_2007/brenguier.pdf (last access: 11 November 2015), MIT Press, MASS, Cambridge, 2009.
Bréon, F.-M. and Colzy, S.: Cloud detection from the spaceborne POLDER instrument and validation against surface synoptic observations, J. Appl. Meteorol., 38, 777–785, https://doi.org/10.1175/1520-0450(1999)038<0777:CDFTSP>2.0.CO;2, 1999.
Bréon, F.-M., Tanré, D., and Generoso, S.: Aerosol effect on cloud droplet size monitored from satellite, Science (New York, N. Y.), 295, 834–8, https://doi.org/10.1126/science.1066434, 2002.
Buriez, J. C., Vanbauce, C., Parol, F., Goloub, P., Herman, M., Bonnel, B., Fouquart, Y., Couvert, P., and Seze, G.: Cloud detection and derivation of cloud properties from POLDER, Int. J. Remote Sens., 18, 2785–2813, https://doi.org/10.1080/014311697217332, 1997.
Chang, F. L. and Coakley, J. A.: Relationships between marine stratus cloud optical depth and temperature: Inferences from AVHRR observations, J. Climate, 20, 2022–2036, https://doi.org/10.1175/JCLI4115.1, 2007.
Chen, Y.-C., Christensen, M. W., Stephens, G. L., and Seinfeld, J. H.: Satellite-based estimate of global aerosol–cloud radiative forcing by marine warm clouds, Nat. Geosci., advance on, 7, 643–646, https://doi.org/10.1038/ngeo2214, 2014.
Coakley, J. A. and Walsh, C. D.: Limits to the aerosol indirect radiative effect derived from observations of ship tracks, J. Atmos. Sci., 59, 668–680, https://doi.org/10.1175/1520-0469(2002)059<0668:LTTAIR>2.0.CO;2, 2002.
Costantino, L. and Bréon, F. M.: Aerosol indirect effect on warm clouds over South-East Atlantic, from co-located MODIS and CALIPSO observations, Atmos. Chem. Phys., 13, 69–88, https://doi.org/10.5194/acp-13-69-2013, 2013.
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi, S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P., Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C., Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B., Hersbach, H., Hólm, E. V., Isaksen, L., Kållberg, P., Köhler, M., Matricardi, M., Mcnally, A. P., Monge-Sanz, B. M., Morcrette, J. J., Park, B. K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J. N., and Vitart, F.: The ERA-Interim reanalysis: Configuration and performance of the data assimilation system, Q. J. Roy. Meteorol. Soc., 137, 553–597, https://doi.org/10.1002/qj.828, 2011.
Desmons, M., Ferlay, N., Parol, F., Mcharek, L., and Vanbauce, C.: Improved information about the vertical location and extent of monolayer clouds from POLDER3 measurements in the oxygen A-band, Atmos. Meas. Tech., 6, 2221–2238, https://doi.org/10.5194/amt-6-2221-2013, 2013.
Dusek, U., Frank, G. P., Hildebrandt, L., Curtius, J., Schneider, J., Walter, S., Chand, D., Drewnick, F., Hings, S., Jung, D., Borrmann, S., and Andreae, M. O.: Size matters more than chemistry for cloud-nucleating ability of aerosol particles, Science (New York, N. Y.), 312, 1375–1378, https://doi.org/10.1126/science.1125261, 2006.
Eckhardt, S., Quennehen, B., Olivié, D. J. L., Berntsen, T. K., Cherian, R., Christensen, J. H., Collins, W., Crepinsek, S., Daskalakis, N., Flanner, M., Herber, A., Heyes, C., Hodnebrog, Ø., Huang, L., Kanakidou, M., Klimont, Z., Langner, J., Law, K. S., Lund, M. T., Mahmood, R., Massling, A., Myriokefalitakis, S., Nielsen, I. E., Nøjgaard, J. K., Quaas, J., Quinn, P. K., Raut, J.-C., Rumbold, S. T., Schulz, M., Sharma, S., Skeie, R. B., Skov, H., Uttal, T., von Salzen, K., and Stohl, A.: Current model capabilities for simulating black carbon and sulfate concentrations in the Arctic atmosphere: a multi-model evaluation using a comprehensive measurement data set, Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, 2015.
Ervens, B., Cubison, M., Andrews, E., Feingold, G., Ogren, J. A., Jimenez, J. L., DeCarlo, P., and Nenes, A.: Prediction of cloud condensation nucleus number concentration using measurements of aerosol size distributions and composition and light scattering enhancement due to humidity, J. Geophys. Res.-Atmos., 112, 1–15, https://doi.org/10.1029/2006JD007426, 2007.
Feingold, G.: Modeling of the first indirect effect: Analysis of measurement requirements, Geophys. Res. Lett., 30, 30, 1997, https://doi.org/10.1029/2003GL017967, 2003a.
Feingold, G.: First measurements of the Twomey indirect effect using ground-based remote sensors, Geophys. Res. Lett., 30, 19–22, https://doi.org/10.1029/2002GL016633, 2003b.
Feingold, G., Remer, L. A., Ramaprasad, J., and Kaufman, Y. J.: Analysis of smoke impact on clouds in Brazilian biomass burning regions: An extension of Twomey's approach, J. Geophys. Res., 106, 22907–22922, 2001.
Fougnie, B., Bracco, G., Lafrance, B., Ruffel, C., Hagolle, O., and Tinel, C.: PARASOL in-flight calibration and performance, Appl. Optics, 46, 5435–5451, https://doi.org/10.1364/AO.46.005435, 2007.
Garrett, T. J. and Zhao, C.: Increased Arctic cloud longwave emissivity associated with pollution from mid-latitudes, Nature 440, 787–789, https://doi.org/10.1038/nature04636, 2006.
Garrett, T. J., Radke, L. F., and Hobbs, P. V.: Aerosol Effects on Cloud Emissivity and Surface Longwave Heating in the Arctic, J. Atmos. Sci., 59, 769–778, https://doi.org/10.1175/1520-0469(2002)059<0769:AEOCEA>2.0.CO;2, 2002.
Garrett, T. J., Zhao, C., Dong, X., Mace, G. G., and Hobbs, P. V.: Effects of varying aerosol regimes on low-level Arctic stratus, Geophys. Res. Lett., 31, L17105, https://doi.org/10.1029/2004GL019928, 2004.
Garrett, T. J., Maestras, M. M., Krueger, S. K., and Shmidt, C. T.: Acceleration by aerosol of a radiative-thermodynamic cloud feedback influencing Arctic surface warming, Geophys. Res. Lett., 36, L19804, https://doi.org/10.1029/2009GL040195, 2009.
Garrett, T. J., Zhao, C., and Novelli, P. C.: Assessing the relative contributions of transport efficiency and scavenging to seasonal variability in Arctic aerosol, Tellus B, 62, 190–196, https://doi.org/10.1111/j.1600-0889.2010.00453.x, 2010.
Garrett, T. J., Brattström, S., Sharma, S., Worthy, D. E. J., and Novelli, P.: The role of scavenging in the seasonal transport of black carbon and sulfate to the Arctic, Geophys. Res. Lett., 38, L16805, https://doi.org/10.1029/2011GL048221, 2011.
Hirdman, D., Sodemann, H., Eckhardt, S., Burkhart, J. F., Jefferson, A., Mefford, T., Quinn, P. K., Sharma, S., Ström, J., and Stohl, A.: Source identification of short-lived air pollutants in the Arctic using statistical analysis of measurement data and particle dispersion model output, Atmos. Chem. Phys., 10, 669–693, https://doi.org/10.5194/acp-10-669-2010, 2010.
Huber, P. J.: The 1972 Wald memorial lectures: robust regression: asymptotics, conjectures, and Monte Carlo, The Annals of Statistics, 1, 799–821, 1973.
Huber, P. J.: Robust Statistics, John Wiley and Sons, Inc., New York, 1981.
Ji, R., Jin, M., and Varpe, Ø.: Sea ice phenology and timing of primary production pulses in the Arctic Ocean, Glob. Change Biol., 19, 734–741, https://doi.org/10.1111/gcb.12074, 2013.
Kaufman, Y. J., Koren, I., Remer, L. A., Rosenfeld, D., and Rudich, Y.: The effect of smoke, dust, and pollution aerosol on shallow cloud development over the Atlantic Ocean, P. Natl. Acad. Sci. USA, 102, 11207–11212, https://doi.org/10.1073/pnas.0505191102, 2005.
Kawamoto, K., Hayasaka, T., Uno, I., and Ohara, T.: A correlative study on the relationship between modeled anthropogenic aerosol concentration and satellite-observed cloud properties over east Asia, J. Geophys. Res.-Atmos., 111, 1–7, https://doi.org/10.1029/2005JD006919, 2006.
Kim, B. G., Miller, M. A., Schwartz, S. E., Liu, Y., and Min, Q.: The role of adiabaticity in the aerosol first indirect effect, J. Geophys. Res.-Atmos., 113, 1–13, https://doi.org/10.1029/2007JD008961, 2008.
King, M. D. and Platnick, S.: Collection 005 change summary for the MODIS cloud optical property (06 _ OD) algorithm high impact change overview: change details:, Terra, 1, 1–23, 2006.
Klein, S. A. and Hartmann, D. L.: The seasonal cycle of low stratiform clouds, J. Climate, 6, 1587–1606, 1993.
Klimont, Z., Smith, S. J., and Cofala, J.: The last decade of global anthropogenic sulfur dioxide: 2000–2011 emissions, Environ. Res. Lett., 8, 014003, https://doi.org/10.1088/1748-9326/8/1/014003, 2013.
Klimont, Z., Hoglund, L., Heyes, C., Rafaj, P., Schoepp, W., Cofala, J., Borken-Kleefeld, J., Purohit, P., Kupiainen, K., Winiwarter, W., Amann, M., Zhao, B., Wang, S. X., Bertok, I., and Sander, R.: Global scenarios of air pollutants and methane: 1990–2050, in preparation, 2016.
Lance, S., Shupe, M. D., Feingold, G., Brock, C. A., Cozic, J., Holloway, J. S., Moore, R. H., Nenes, A., Schwarz, J. P., Spackman, J. R., Froyd, K. D., Murphy, D. M., Brioude, J., Cooper, O. R., Stohl, A., and Burkhart, J. F.: Cloud condensation nuclei as a modulator of ice processes in Arctic mixed-phase clouds, Atmos. Chem. Phys., 11, 8003–8015, https://doi.org/10.5194/acp-11-8003-2011, 2011.
Law, K. S. and Stohl, A.: Arctic air pollution: origins and impacts, Science (New York, N. Y.), 315, 1537–40, https://doi.org/10.1126/science.1137695, 2007.
Law, K. S., Stohl, A., Quinn, P. K., Brock, C., Burkhart, J., Paris, J. D., Ancellet, G., Singh, H. B., Roiger, A., Schlager, H., Dibb, J., Jacob, D. J., Arnold, S. R., Pelon, J., and Thomas, J. L.: Arctic air pollution: new insights from POLARCAT-IPY, B. Am. Meteorol. Soc., 95, 1873–1895, https://doi.org/10.1175/BAMS-D-13-00017.1, 2014.
Lihavainen, H., Kerminen, V. M., and Remer, L. A.: Aerosol-cloud interaction determined by both in situ and satellite data over a northern high-latitude site, Atmos. Chem. Phys., 10, 10987–10995, https://doi.org/10.5194/acp-10-10987-2010, 2009.
Lindholt, L. and Glomsrød, S.: The Arctic: No big bonanza for the global petroleum industry, Energ. Econ., 34, 1465–1474, https://doi.org/10.1016/j.eneco.2012.06.020, 2012.
Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715–737, https://doi.org/10.5194/acp-5-715-2005, 2005.
Longley, I. D., Inglis, D. W. F., Gallagher, M. W., Williams, P. I., Allan, J. D., and Coe, H.: Using NOx and CO monitoring data to indicate fine aerosol number concentrations and emission factors in three UK conurbations, Atmos. Environ., 39, 5157–5169, https://doi.org/10.1016/j.atmosenv.2005.05.017, 2005.
Lubin, D. and Vogelmann, A. M.: A climatologically significant aerosol longwave indirect effect in the Arctic, Nature, 439, 453–456, https://doi.org/10.1038/nature04449, 2006.
Lubin, D. and Vogelmann, A. M.: Expected magnitude of the aerosol shortwave indirect effect in springtime Arctic liquid water clouds, Geophys. Res. Lett., 34, L11801, https://doi.org/10.1029/2006GL028750, 2007.
Markus, T., Stroeve, J. C., and Miller, J.: Recent changes in Arctic sea ice melt onset, freezeup, and melt season length, J. Geophys. Res.-Oceans, 114, 1–14, https://doi.org/10.1029/2009JC005436, 2009.
Matsui, T., Masunaga, H., Kreidenweis, S. M., Pielke, R. A., Tao, W. K., Chin, M., and Kaufman, Y. J.: Satellite-based assessment of marine low cloud variability associated with aerosol, atmospheric stability, and the diurnal cycle, J. Geophys. Res.-Atmos., 111, 1–16, https://doi.org/10.1029/2005JD006097, 2006.
Mauger, G. S. and Norris, J. R.: Meteorological bias in satellite estimates of aerosol-cloud relationships, Geophys. Res. Lett., 34, 1–5, https://doi.org/10.1029/2007GL029952, 2007.
Mauritsen, T., Sedlar, J., Tjernström, M., Leck, C., Martin, M., Shupe, M., Sjogren, S., Sierau, B., Persson, P. O. G., Brooks, I. M., and Swietlicki, E.: An Arctic CCN-limited cloud-aerosol regime, Atmos. Chem. Phys., 11, 165–173, https://doi.org/10.5194/acp-11-165-2011, 2011.
Miller, A. W. and Ruiz, G. M.: Arctic shipping and marine invaders, Nature Clim. Change, 4, 413–416, https://doi.org/10.1038/nclimate2244, 2014.
Myhre, G., Stordal, F., Johnsrud, M., Kaufman, Y. J., Rosenfeld, D., Storelvmo, T., Kristjansson, J. E., Berntsen, T. K., Myhre, A., and Isaksen, I. S. A.: Aerosol-cloud interaction inferred from MODIS satellite data and global aerosol models, Atmos. Chem. Phys., 7, 3081–3101, https://doi.org/10.5194/acp-7-3081-2007, 2007.
Nakajima, T., Higurashi, A., Kawamoto, K., and Penner, J. E.: A possible correlation between satellite-derived cloud and aerosol microphysical parameters, Geophys. Res. Lett., 28, 1171–1174, https://doi.org/10.1029/2000GL012186, 2001.
Nygärd, T., Valkonen, T., and Vihma, T.: Characteristics of arctic low-tropospheric humidity inversions based on radio soundings, Atmos. Chem. Phys., 14, 1959–1971, https://doi.org/10.5194/acp-14-1959-2014, 2014.
Overland, J. E. and Wang, M.: When will the summer Arctic be nearly sea ice free?, Geophys. Res. Lett., 40, 2097–2101, https://doi.org/10.1002/grl.50316, 2013.
Painemal, D., Kato, S., and Minnis, P.: Boundary layer regulation in the southeast Atlantic cloud microphysics during the biomass burning season as seen by the A-train satellite constellation, J. Geophys. Res.-Atmos., 119, 11288–11302, https://doi.org/10.1002/2014JD022182, 2014.
Paris, J.-D., Stohl, A., Nédélec, P., Arshinov, M. Yu., Panchenko, M. V., Shmargunov, V. P., Law, K. S., Belan, B. D., and Ciais, P.: Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements, Atmos. Chem. Phys., 9, 9315–9327, https://doi.org/10.5194/acp-9-9315-2009, 2009.
Pincus, R. and Baker, M. B.: Effect of precipitation on the albedo susceptibility of clouds in the marine boundary layer, Nature, 372, 250–252, https://doi.org/10.1038/372250a0, 1994.
Pizzolato, L., Howell, S. E. L., Derksen, C., Dawson, J., and Copland, L.: Changing sea ice conditions and marine transportation activity in Canadian Arctic waters between 1990 and 2012, Climatic Change, 123, 161–173, https://doi.org/10.1007/s10584-013-1038-3, 2014.
Platnick, S., King, M. D., Ackerman, S. A., Menzel, W. P., Baum, B. A., Riédi, J. C., and Frey, R. A.: The MODIS cloud products: Algorithms and examples from terra, IEEE T. Geosci. Remote, 41, 459–472, https://doi.org/10.1109/TGRS.2002.808301, 2003.
Qiu, S., Dong, X., Xi, B., and Li, J. F.: Characterizing Arctic mixed-phase cloud structure and its relationship with humidity and temperature inversion using ARM NSA observations, J. Geophys. Res., 120, 7737–7746, https://doi.org/10.1002/2014JD023022, 2015.
Quinn, P. K., Shaw, G., Andrews, E., Dutton, E. G., Ruoho-Airola, T., and Gong, S. L.: Arctic haze: Current trends and knowledge gaps, Tellus B, 59, 99–114, https://doi.org/10.1111/j.1600-0889.2006.00238.x, 2007.
Richter-Menge, J. and Jeffries, M.: State of the climate in 2010: The Arctic, B. Am. Meteorol. Soc., 92, S143–S160, 2011.
Riedi, J., Marchant, B., Platnick, S., Baum, B. A., Thieuleux, F., Oudard, C., Parol, F., Nicolas, J.-M., and Dubuisson, P.: Cloud thermodynamic phase inferred from merged POLDER and MODIS data, Atmos. Chem. Phys., 10, 11851–11865, https://doi.org/10.5194/acp-10-11851-2010, 2010.
Schwartz, S. E., Harshvardhan, and Benkovitz, C. M.: Influence of anthropogenic aerosol on cloud optical depth and albedo shown by satellite measurements and chemical transport modeling, P. Natl. Acad. Sci. USA, 99, 1784–1789, https://doi.org/10.1073/pnas.261712099, 2002.
Sekiguchi, M.: A study of the direct and indirect effects of aerosols using global satellite data sets of aerosol and cloud parameters, J. Geophys. Res., 108, 1–15, https://doi.org/10.1029/2002JD003359, 2003.
Serreze, M. C. and Francis, J. A.: The Arctic on the fast track of change, Weather, 61, 65–69, https://doi.org/10.1256/wea.197.05, 2006.
Serreze, M. C., Barrett, A. P., Stroeve, J. C., Kindig, D. N., and Holland, M. M.: The emergence of surface-based Arctic amplification, The Cryosphere, 3, 11–19, https://doi.org/10.5194/tc-3-11-2009, 2009.
Shaw, G. E.: The arctic haze phenomenon, B. Am. Meteorol. Soc., 76, 2403–2413, https://doi.org/10.1175/1520-0477(1995)076<2403:TAHP>2.0.CO;2, 1995.
Shindell, D. T., Chin, M., Dentener, F., Doherty, R. M., Faluvegi, G., Fiore, A. M., Hess, P., Koch, D. M., MacKenzie, I. A., Sanderson, M. G., Schultz, M. G., Schulz, M., Stevenson, D. S., Teich, H., Textor, C., Wild, O., Bergmann, D. J., Bey, I., Bian, H., Cuvelier, C., Duncan, B. N., Folberth, G., Horowitz, L. W., Jonson, J., Kaminski, J. W., Marmer, E., Park, R., Pringle, K. J., Schroeder, S., Szopa, S., Takemura, T., Zeng, G., Keating, T. J., and Zuber, A.: A multi-model assessment of pollution transport to the Arctic, Atmos. Chem. Phys., 8, 5353–5372, https://doi.org/10.5194/acp-8-5353-2008, 2008.
Sirois, A. and Barrie, L. A.: Arctic lower tropospheric aerosol trends and composition at Alert, Canada: 1980–1995, J. Geophys. Res., 104, 11599, https://doi.org/10.1029/1999JD900077, 1999.
Sodemann, H., Pommier, M., Arnold, S. R., Monks, S. A., Stebel, K., Burkhart, J. F., Hair, J. W., Diskin, G. S., Clerbaux, C., Coheur, P.-F., Hurtmans, D., Schlager, H., Blechschmidt, A.-M., Kristjánsson, J. E., and Stohl, A.: Episodes of cross-polar transport in the Arctic troposphere during July 2008 as seen from models, satellite, and aircraft observations, Atmos. Chem. Phys., 11, 3631–3651, https://doi.org/10.5194/acp-11-3631-2011, 2011.
Sporre, M. K., Glantz, P., Tunved, P., Swietlicki, E., Kulmala, M., and Lihavainen, H.: A study of the indirect aerosol effect on subarctic marine liquid low-level clouds using MODIS cloud data and ground-based aerosol measurements, Atmos. Res., 116, 56–66, https://doi.org/10.1016/j.atmosres.2011.09.014, 2012.
Stephens, G. L., Vane, D. G., Boain, R. J., Mace, G. G., Sassen, K., Wang, Z., Illingworth, A. J., O'Connor, E. J., Rossow, W. B., Durden, S. L., Miller, S. D., Austin, R. T., Benedetti, A., and Mitrescu, C.: The cloudsat mission and the A-Train: A new dimension of space-based observations of clouds and precipitation, B. Am. Meteorol. Soc., 83, 1771–1790+1742, https://doi.org/10.1175/BAMS-83-12-1771, 2002.
Stohl, A.: Characteristics of atmospheric transport into the Arctic troposphere, J. Geophys. Res., 111, D11306, https://doi.org/10.1029/2005JD006888, 2006.
Stohl, A., Hittenberger, M., and Wotawa, G.: Validation of the lagrangian particle dispersion model FLEXPART against large-scale tracer experiment data, Atmos. Environ., 32, 4245–4264, https://doi.org/10.1016/S1352-2310(98)00184-8, 1998.
Stohl, A., Forster, C., Frank, A., Seibert, P., and Wotawa, G.: Technical note: The Lagrangian particle dispersion model FLEXPART version 6.2, Atmos. Chem. Phys., 5, 2461–2474, https://doi.org/10.5194/acp-5-2461-2005, 2005.
Stohl, A., Berg, T., Burkhart, J. F., Fjǽraa, A. M., Forster, C., Herber, A., Hov, Ø., Lunder, C., McMillan, W. W., Oltmans, S., Shiobara, M., Simpson, D., Solberg, S., Stebel, K., Ström, J., Tørseth, K., Treffeisen, R., Virkkunen, K., and Yttri, K. E.: Arctic smoke – record high air pollution levels in the European Arctic due to agricultural fires in Eastern Europe in spring 2006, Atmos. Chem. Phys., 7, 511–534, https://doi.org/10.5194/acp-7-511-2007, 2007.
Stohl, A., Klimont, Z., Eckhardt, S., Kupiainen, K., Shevchenko, V. P., Kopeikin, V. M., and Novigatsky, A. N.: Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions, Atmos. Chem. Phys., 13, 8833–8855, https://doi.org/10.5194/acp-13-8833-2013, 2013.
Stohl, A., Aamaas, B., Amann, M., Baker, L. H., Bellouin, N., Berntsen, T. K., Boucher, O., Cherian, R., Collins, W., Daskalakis, N., Dusinska, M., Eckhardt, S., Fuglestvedt, J. S., Harju, M., Heyes, C., Hodnebrog, Ø., Hao, J., Im, U., Kanakidou, M., Klimont, Z., Kupiainen, K., Law, K. S., Lund, M. T., Maas, R., MacIntosh, C. R., Myhre, G., Myriokefalitakis, S., Olivié, D., Quaas, J., Quennehen, B., Raut, J.-C., Rumbold, S. T., Samset, B. H., Schulz, M., Seland, Ø., Shine, K. P., Skeie, R. B., Wang, S., Yttri, K. E., and Zhu, T.: Evaluating the climate and air quality impacts of short-lived pollutants, Atmos. Chem. Phys., 15, 10529–10566, https://doi.org/10.5194/acp-15-10529-2015, 2015.
Tietze, K., Riedi, J., Stohl, A., and Garrett, T. J.: Space-based evaluation of interactions between aerosols and low-level Arctic clouds during the Spring and Summer of 2008, Atmos. Chem. Phys., 11, 3359-3373, https://doi.org/10.5194/acp-11-3359-2011, 2011.
Twomey, S.: The influence of Pollution on the shortwave Albedo of Clouds, J. Atmos. Sci., 34, 1149–1152,https://doi.org/10.1175/1520-0469(1977)034<1149:TIOPOT>2.0.CO;2 1977.
Venables, W. N. and Ripley, B. D.: Modern Applied Statistics with S-PLUS, Springer Science and Business Media, New York, NY, 2013.
Wang, F., Guo, J., Wu, Y., Zhang, X., Deng, M., Li, X., Zhang, J., and Zhao, J.: Satellite observed aerosol-induced variability in warm cloud properties under different meteorological conditions over eastern China, Atmos. Environ., 84, 122–132, https://doi.org/10.1016/j.atmosenv.2013.11.018, 2014.
Warneke, C., Bahreini, R., Brioude, J., Brock, C. A., De Gouw, J. A., Fahey, D. W., Froyd, K. D., Holloway, J. S., Middlebrook, A., Miller, L., Montzka, S., Murphy, D. M., Peischl, J., Ryerson, T. B., Schwarz, J. P., Spademan, J. R., and Veres, P.: Biomass burning in Siberia and Kazakhstan as an important source for haze over the Alaskan Arctic in April 2008, Geophys. Res. Lett., 36, 2–7, https://doi.org/10.1029/2008GL036194, 2009.
Weisz, E., Li, J., Menzel, W. P., Heidinger, A. K., Kahn, B. H., and Liu, C. Y.: Comparison of AIRS, MODIS, CloudSat and CALIPSO cloud top height retrievals, Geophys. Res. Lett., 34, 1–5, https://doi.org/10.1029/2007GL030676, 2007.
Wesslén, C., Tjernström, M., Bromwich, D. H., De Boer, G., Ekman, A. M. L., Bai, L. S., and Wang, S. H.: The Arctic summer atmosphere: An evaluation of reanalyses using ASCOS data, Atmos. Chem. Phys., 14, 2605–2624, https://doi.org/10.5194/acp-14-2605-2014, 2014.
Westerling, A. L., Hidalgo, H. G., Cayan, D. R., and Swetnam, T. W.: Warming and earlier spring increase western U. S. forest wildfire activity, Science (New York, N. Y.), 313, 940–943, https://doi.org/10.1126/science.1128834, 2006.
Yoshimori, M., Watanabe, M., Abe-Ouchi, A., Shiogama, H., and Ogura, T.: Relative contribution of feedback processes to Arctic amplification of temperature change in MIROC GCM, Clim. Dynam., 42, 1613–1630, https://doi.org/10.1007/s00382-013-1875-9, 2013.
Zhao, C. and Garrett, T. J.: Effects of Arctic Haze on surface Cloud radiative forcing, Geophys. Res. Lett., 42, 557–564, https://doi.org/10.1002/2014GL062015, 2015.
Zhao, C., Klein, S. A., Xie, S., Liu, X., Boyle, J. S., and Zhang, Y.: Aerosol first indirect effects on non-precipitating low-level liquid cloud properties as simulated by CAM5 at ARM sites, Geophys. Res. Lett., 39, 1–7, https://doi.org/10.1029/2012GL051213, 2012.
Zygmuntowska, M., Mauritsen, T., Quaas, J., and Kaleschke, L.: Arctic clouds and surface radiation-a critical comparison of satellite retrievals and the ERA-interim reanalysis, Atmos. Chem. Phys., 12, 6667–6677, https://doi.org/10.5194/acp-12-6667-2012, 2012.
Short summary
We analyze interactions of Arctic clouds with pollution plumes that have been transported long distances from midlatitudes. Constraining for meteorological state, we find that pollution decreases cloud-droplet effective radius and increases cloud optical depth. The impact is highest when the atmosphere is particularly humid and/or stable suggesting that aerosol–cloud interactions depend on the Arctic's climate.
We analyze interactions of Arctic clouds with pollution plumes that have been transported long...
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