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Volume 16, issue 22
Atmos. Chem. Phys., 16, 14585–14598, 2016
https://doi.org/10.5194/acp-16-14585-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: The CERN CLOUD experiment (ACP/AMT inter-journal SI)

Atmos. Chem. Phys., 16, 14585–14598, 2016
https://doi.org/10.5194/acp-16-14585-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 23 Nov 2016

Research article | 23 Nov 2016

A Monte Carlo approach for determining cluster evaporation rates from concentration measurements

Oona Kupiainen-Määttä

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Adamov, A., Junninen, H., Duplissy, J., Sipilä, M., Kulmala, M., and CLOUD collaboration: Cluster measurements at CLOUD using a high resolution ion mobility spectrometer-mass spectrometer combination, AIP Conf. Proc., 1527, 350–353, https://doi.org/10.1063/1.4803275, 2013.
Benson, D. R., Yu, J. H., Markovich, A., and Lee, S.-H.: Ternary homogeneous nucleation of H2SO4, NH3, and H2O under conditions relevant to the lower troposphere, Atmos. Chem. Phys., 11, 4755–4766, https://doi.org/10.5194/acp-11-4755-2011, 2011.
Berndt, T., Stratmann, F., Sipilä, M., Vanhanen, J., Petäjä, T., Mikkilä, J., Grüner, A., Spindler, G., Lee Mauldin III, R., Curtius, J., Kulmala, M., and Heintzenberg, J.: Laboratory study on new particle formation from the reaction OH + SO2: influence of experimental conditions, H2O vapour, NH3 and the amine tert-butylamine on the overall process, Atmos. Chem. Phys., 10, 7101–7116, https://doi.org/10.5194/acp-10-7101-2010, 2010.
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The article introduces a new method for determining the evaporation rates of small molecular clusters based on cluster concentration measurements. Evaporation rates cannot be measured directly or computed very accurately from any classical or quantum theory, so the presented method will give new understanding about molecular clusters. In addition, it can give some information about what happens to clusters during the measurement process.
The article introduces a new method for determining the evaporation rates of small molecular...
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