Articles | Volume 13, issue 17
https://doi.org/10.5194/acp-13-8833-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-8833-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| Highlight paper
| 
05 Sep 2013
Research article | Highlight paper |
| 05 Sep 2013
Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions
NILU – Norwegian Institute for Air Research, Kjeller, Norway
Z. Klimont
International Institute for Applied Systems Analysis (IIASA), Laxenburg, Austria
S. Eckhardt
NILU – Norwegian Institute for Air Research, Kjeller, Norway
K. Kupiainen
International Institute for Applied Systems Analysis (IIASA), Laxenburg, Austria
Finnish Environment Institute (SYKE), Helsinki, Finland
V. P. Shevchenko
P.P. Shirshov Institute of Oceanology, Russian Academy of Sciences, Moscow, Russia
V. M. Kopeikin
A.M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Moscow, Russia
A. N. Novigatsky
P.P. Shirshov Institute of Oceanology, Russian Academy of Sciences, Moscow, Russia
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Stephen M. Platt, Sabine Eckhardt, Benedicte Ferré, Rebecca E. Fisher, Ove Hermansen, Pär Jansson, David Lowry, Euan G. Nisbet, Ignacio Pisso, Norbert Schmidbauer, Anna Silyakova, Andreas Stohl, Tove M. Svendby, Sunil Vadakkepuliyambatta, Jürgen Mienert, and Cathrine Lund Myhre
Atmos. Chem. Phys., 18, 17207–17224, https://doi.org/10.5194/acp-18-17207-2018, https://doi.org/10.5194/acp-18-17207-2018, 2018
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Anna Solvejg Dinger, Kerstin Stebel, Massimo Cassiani, Hamidreza Ardeshiri, Cirilo Bernardo, Arve Kylling, Soon-Young Park, Ignacio Pisso, Norbert Schmidbauer, Jan Wasseng, and Andreas Stohl
Atmos. Meas. Tech., 11, 6169–6188, https://doi.org/10.5194/amt-11-6169-2018, https://doi.org/10.5194/amt-11-6169-2018, 2018
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Christine D. Groot Zwaaftink, Stephan Henne, Rona L. Thompson, Edward J. Dlugokencky, Toshinobu Machida, Jean-Daniel Paris, Motoki Sasakawa, Arjo Segers, Colm Sweeney, and Andreas Stohl
Geosci. Model Dev., 11, 4469–4487, https://doi.org/10.5194/gmd-11-4469-2018, https://doi.org/10.5194/gmd-11-4469-2018, 2018
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Nikolaos Evangeliou, Rona L. Thompson, Sabine Eckhardt, and Andreas Stohl
Atmos. Chem. Phys., 18, 15307–15327, https://doi.org/10.5194/acp-18-15307-2018, https://doi.org/10.5194/acp-18-15307-2018, 2018
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We present BC inversions at high northern latitudes in 2013–2015. The emissions were high close to the gas flaring regions in Russia and in western Canada. The posterior emissions of BC at latitudes > 50° N were estimated as 560 ± 171 kt yr-1, smaller than in bottom-up inventories. Posterior concentrations over the Arctic compared with independent observations from flight and ship campaigns showed small biases. Seasonal maxima were estimated in summer months due to biomass burning, mainly in Europe.
Lauren M. Zamora, Ralph A. Kahn, Klaus B. Huebert, Andreas Stohl, and Sabine Eckhardt
Atmos. Chem. Phys., 18, 14949–14964, https://doi.org/10.5194/acp-18-14949-2018, https://doi.org/10.5194/acp-18-14949-2018, 2018
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We use satellite data and model output to estimate how airborne particles (aerosols) affect cloud ice particles and droplets over the Arctic Ocean. Aerosols from sources like smoke and pollution can change cloud cover, precipitation frequency, and the portion of liquid- vs. ice-containing clouds, which in turn can impact the surface energy budget. By improving our understanding these aerosol–cloud interactions, this work can help climate predictions for the rapidly changing Arctic.
Nikolaos Evangeliou, Vladimir P. Shevchenko, Karl Espen Yttri, Sabine Eckhardt, Espen Sollum, Oleg S. Pokrovsky, Vasily O. Kobelev, Vladimir B. Korobov, Andrey A. Lobanov, Dina P. Starodymova, Sergey N. Vorobiev, Rona L. Thompson, and Andreas Stohl
Atmos. Chem. Phys., 18, 963–977, https://doi.org/10.5194/acp-18-963-2018, https://doi.org/10.5194/acp-18-963-2018, 2018
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We present EC measurements from an uncertain region in terms of emissions (Russia). Its origin is quantified with a Lagrangian model that uses a recently developed feature that allows backward estimation of the specific source locations that contribute to the deposited mass. In NW European Russia transportation and domestic combustion from Finland was important. A systematic underestimation was found in W Siberia at places where gas flaring was important, implying miscalculation or sources.
Bastien Sauvage, Alain Fontaine, Sabine Eckhardt, Antoine Auby, Damien Boulanger, Hervé Petetin, Ronan Paugam, Gilles Athier, Jean-Marc Cousin, Sabine Darras, Philippe Nédélec, Andreas Stohl, Solène Turquety, Jean-Pierre Cammas, and Valérie Thouret
Atmos. Chem. Phys., 17, 15271–15292, https://doi.org/10.5194/acp-17-15271-2017, https://doi.org/10.5194/acp-17-15271-2017, 2017
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We provide the scientific community with a SOFT-IO tool based on the coupling of Lagrangian modeling with emission inventories and aircraft CO measurements, which is able to calculate the contribution of the sources and geographical origins of CO measurements, with good performances. Calculated CO added-value products will help scientists in interpreting large IAGOS CO data set. SOFT-IO could further be applied to other CO data sets or used to help validate emission inventories.
Sabine Eckhardt, Massimo Cassiani, Nikolaos Evangeliou, Espen Sollum, Ignacio Pisso, and Andreas Stohl
Geosci. Model Dev., 10, 4605–4618, https://doi.org/10.5194/gmd-10-4605-2017, https://doi.org/10.5194/gmd-10-4605-2017, 2017
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We extend the backward modelling technique in the existing model FLEXPART to substances deposited at the Earth’s surface by wet scavenging and dry deposition. This means that for existing measurements of a substance in snow, ice cores or rain samples the source regions can be determined. This will help the interpretation of the measurement as well as gaining information of emission strength at the source of the deposited substance.
Ondřej Tichý, Václav Šmídl, Radek Hofman, Kateřina Šindelářová, Miroslav Hýža, and Andreas Stohl
Atmos. Chem. Phys., 17, 12677–12696, https://doi.org/10.5194/acp-17-12677-2017, https://doi.org/10.5194/acp-17-12677-2017, 2017
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In the fall of 2011, iodine-131 (131I) was detected at several radionuclide monitoring stations in central Europe. We estimate the source location and emission variation using only the available 131I measurements. Subsequently, we use the IAEA report about the source term for validation of our results. We find that our algorithm could successfully locate the actual release site. The findings are also in agreement with the values reported by the IAEA.
Franz Conen, Sabine Eckhardt, Hans Gundersen, Andreas Stohl, and Karl Espen Yttri
Atmos. Chem. Phys., 17, 11065–11073, https://doi.org/10.5194/acp-17-11065-2017, https://doi.org/10.5194/acp-17-11065-2017, 2017
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Observation of ice nuclei active at −8 °C show that rainfall drives their abundance throughout all seasons and that they are equally distributed amongst coarse and fine fraction of PM10. Concurrent measurements of fungal spore markers suggest that some fraction of INP-8 may consist of fungal spores during the warm part of the year. Snow cover suppresses the aerosolisation of ice nuclei. Changes in snow cover and rainfall may affect atmospheric concentrations of ice nuclei in future.
Christine D. Groot Zwaaftink, Ólafur Arnalds, Pavla Dagsson-Waldhauserova, Sabine Eckhardt, Joseph M. Prospero, and Andreas Stohl
Atmos. Chem. Phys., 17, 10865–10878, https://doi.org/10.5194/acp-17-10865-2017, https://doi.org/10.5194/acp-17-10865-2017, 2017
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How much dust do Icelandic sources emit and where is this dust deposited? We modelled dust emission and transport from Icelandic sources over 27 years with FLEXPART. Results show that Icelandic dust sources can have emission rates similar to parts of the Sahara and considerable amounts of dust are deposited in the ocean and on glaciers.
Nikolaos Evangeliou, Thomas Hamburger, Anne Cozic, Yves Balkanski, and Andreas Stohl
Atmos. Chem. Phys., 17, 8805–8824, https://doi.org/10.5194/acp-17-8805-2017, https://doi.org/10.5194/acp-17-8805-2017, 2017
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This is the first paper that attempts to assess the source term of the Chernobyl accident using not only activity concentrations but also deposition measurements. This is done by using the FLEXPART model combined with a Bayesian inversion algorithm. Our results show that the altitude of the injection during the first days of the accident might have reached up to 3 km, in contrast to what has been already reported (2.2 km maximum), in order the model to better match observations.
Lauren M. Zamora, Ralph A. Kahn, Sabine Eckhardt, Allison McComiskey, Patricia Sawamura, Richard Moore, and Andreas Stohl
Atmos. Chem. Phys., 17, 7311–7332, https://doi.org/10.5194/acp-17-7311-2017, https://doi.org/10.5194/acp-17-7311-2017, 2017
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Clouds have a major but uncertain effect on Arctic surface temperatures. Here, we used remote sensing observations to better understand aerosol effects on one type of Arctic cloud. By modifying a variety of cloud properties, aerosols in this type of cloud indirectly reduced the net warming effect of these clouds on the surface by ~ 10 % of the clean-background cloud effect, not including changes in cloud fraction. This work will improve our ability to predict future Arctic surface temperatures.
Henrik Grythe, Nina I. Kristiansen, Christine D. Groot Zwaaftink, Sabine Eckhardt, Johan Ström, Peter Tunved, Radovan Krejci, and Andreas Stohl
Geosci. Model Dev., 10, 1447–1466, https://doi.org/10.5194/gmd-10-1447-2017, https://doi.org/10.5194/gmd-10-1447-2017, 2017
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A new and more physically based treatment of how removal by precipitation is calculated by FLEXPART is introduced to take into account more aspects of aerosol diversity. Also new is the definition of clouds and cloud properties. Results from simulations show good agreement with observed atmospheric concentrations for distinctly different aerosols. Atmospheric lifetimes were found to vary from a few hours (large aerosol particles) up to a month (small non-soluble particles)
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This work includes a study on the effects of dust deposition on the mass balance of Brúarjökull, an outlet glacier of Vatnajökull, Iceland's largest ice cap. A model was used to simulate dust deposition on the glacier, and these periods of dust were compared to albedo measurements at two weather stations on Brúarjökull to evaluate the dust impact. We determine the influence of dust events on the snow albedo and the surface energy balance.
Rona L. Thompson, Motoki Sasakawa, Toshinobu Machida, Tuula Aalto, Doug Worthy, Jost V. Lavric, Cathrine Lund Myhre, and Andreas Stohl
Atmos. Chem. Phys., 17, 3553–3572, https://doi.org/10.5194/acp-17-3553-2017, https://doi.org/10.5194/acp-17-3553-2017, 2017
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Methane (CH4) fluxes were estimated for the high northern latitudes for 2005–2013 based on observations of atmospheric CH4 mixing ratios. Methane fluxes were found to be higher than prior estimates in northern Eurasia and Canada, especially in the Western Siberian Lowlands and the Canadian province Alberta. Significant inter-annual variations in the fluxes were found as well as a small positive trend. In Canada, the trend may be related to an increase in soil temperature over the study period.
Ondřej Tichý, Václav Šmídl, Radek Hofman, and Andreas Stohl
Geosci. Model Dev., 9, 4297–4311, https://doi.org/10.5194/gmd-9-4297-2016, https://doi.org/10.5194/gmd-9-4297-2016, 2016
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Estimation of pollutant releases into the atmosphere is an important problem in the environmental sciences. We formulate a probabilistic model, where a full Bayesian estimation allows estimation of all tuning parameters from the measurements. The proposed algorithm is tested and compared with the state-of-the-art method on data from the European Tracer Experiment (ETEX), where advantages of the new method are demonstrated.
Xiao Lu, Lin Zhang, Xu Yue, Jiachen Zhang, Daniel A. Jaffe, Andreas Stohl, Yuanhong Zhao, and Jingyuan Shao
Atmos. Chem. Phys., 16, 14687–14702, https://doi.org/10.5194/acp-16-14687-2016, https://doi.org/10.5194/acp-16-14687-2016, 2016
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Increasing wildfire activities in the mountainous western US may present a challenge for the region to attain a recently revised ozone air quality standard in summer. We quantify the wildfire influence on the ozone variability, trends, and number of high ozone days over this region in summers 1989–2010 using a Lagrangian dispersion model and statistical regression models.
Massimo Cassiani, Andreas Stohl, Dirk Olivié, Øyvind Seland, Ingo Bethke, Ignacio Pisso, and Trond Iversen
Geosci. Model Dev., 9, 4029–4048, https://doi.org/10.5194/gmd-9-4029-2016, https://doi.org/10.5194/gmd-9-4029-2016, 2016
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FLEXPART is a community model used by many scientists. Here, an alternative FLEXPART model version has been developed, tailored to use with the output data generated by the Norwegian Earth System Model (NorESM1-M). The model provides an advanced tool to analyse and diagnose atmospheric transport properties of the climate model NorESM. To validate the model, several tests were performed that offered the possibility to investigate some aspects of offline global dispersion modelling.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Xuekun Fang, Min Shao, Andreas Stohl, Qiang Zhang, Junyu Zheng, Hai Guo, Chen Wang, Ming Wang, Jiamin Ou, Rona L. Thompson, and Ronald G. Prinn
Atmos. Chem. Phys., 16, 3369–3382, https://doi.org/10.5194/acp-16-3369-2016, https://doi.org/10.5194/acp-16-3369-2016, 2016
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This is the first study reporting top-down estimates of benzene and toluene emissions in southern China using atmospheric measurement data from a rural site in the area, an atmospheric transport model and an inverse modeling method. This study shows in detail the temporal and spatial differences between the inversion estimate and four different bottom-up emission inventories (RCP, REAS, MEIC; Yin et al., 2015). We propose that more observations are urgently needed in future.
A. Stohl, B. Aamaas, M. Amann, L. H. Baker, N. Bellouin, T. K. Berntsen, O. Boucher, R. Cherian, W. Collins, N. Daskalakis, M. Dusinska, S. Eckhardt, J. S. Fuglestvedt, M. Harju, C. Heyes, Ø. Hodnebrog, J. Hao, U. Im, M. Kanakidou, Z. Klimont, K. Kupiainen, K. S. Law, M. T. Lund, R. Maas, C. R. MacIntosh, G. Myhre, S. Myriokefalitakis, D. Olivié, J. Quaas, B. Quennehen, J.-C. Raut, S. T. Rumbold, B. H. Samset, M. Schulz, Ø. Seland, K. P. Shine, R. B. Skeie, S. Wang, K. E. Yttri, and T. Zhu
Atmos. Chem. Phys., 15, 10529–10566, https://doi.org/10.5194/acp-15-10529-2015, https://doi.org/10.5194/acp-15-10529-2015, 2015
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This paper presents a summary of the findings of the ECLIPSE EU project. The project has investigated the climate and air quality impacts of short-lived climate pollutants (especially methane, ozone, aerosols) and has designed a global mitigation strategy that maximizes co-benefits between air quality and climate policy. Transient climate model simulations allowed quantifying the impacts on temperature (e.g., reduction in global warming by 0.22K for the decade 2041-2050) and precipitation.
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
S. Eckhardt, B. Quennehen, D. J. L. Olivié, T. K. Berntsen, R. Cherian, J. H. Christensen, W. Collins, S. Crepinsek, N. Daskalakis, M. Flanner, A. Herber, C. Heyes, Ø. Hodnebrog, L. Huang, M. Kanakidou, Z. Klimont, J. Langner, K. S. Law, M. T. Lund, R. Mahmood, A. Massling, S. Myriokefalitakis, I. E. Nielsen, J. K. Nøjgaard, J. Quaas, P. K. Quinn, J.-C. Raut, S. T. Rumbold, M. Schulz, S. Sharma, R. B. Skeie, H. Skov, T. Uttal, K. von Salzen, and A. Stohl
Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, https://doi.org/10.5194/acp-15-9413-2015, 2015
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The concentrations of sulfate, black carbon and other aerosols in the Arctic are characterized by high values in late winter and spring (so-called Arctic Haze) and low values in summer. Models have long been struggling to capture this seasonality. In this study, we evaluate sulfate and BC concentrations from different updated models and emissions against a comprehensive pan-Arctic measurement data set. We find that the models improved but still struggle to get the maximum concentrations.
L. J. Kramer, D. Helmig, J. F. Burkhart, A. Stohl, S. Oltmans, and R. E. Honrath
Atmos. Chem. Phys., 15, 6827–6849, https://doi.org/10.5194/acp-15-6827-2015, https://doi.org/10.5194/acp-15-6827-2015, 2015
M. Martinez-Camara, B. Béjar Haro, A. Stohl, and M. Vetterli
Geosci. Model Dev., 7, 2303–2311, https://doi.org/10.5194/gmd-7-2303-2014, https://doi.org/10.5194/gmd-7-2303-2014, 2014
T. Trickl, H. Vogelmann, H. Giehl, H.-E. Scheel, M. Sprenger, and A. Stohl
Atmos. Chem. Phys., 14, 9941–9961, https://doi.org/10.5194/acp-14-9941-2014, https://doi.org/10.5194/acp-14-9941-2014, 2014
M. Maione, F. Graziosi, J. Arduini, F. Furlani, U. Giostra, D. R. Blake, P. Bonasoni, X. Fang, S. A. Montzka, S. J. O'Doherty, S. Reimann, A. Stohl, and M. K. Vollmer
Atmos. Chem. Phys., 14, 9755–9770, https://doi.org/10.5194/acp-14-9755-2014, https://doi.org/10.5194/acp-14-9755-2014, 2014
K. E. Yttri, C. Lund Myhre, S. Eckhardt, M. Fiebig, C. Dye, D. Hirdman, J. Ström, Z. Klimont, and A. Stohl
Atmos. Chem. Phys., 14, 6427–6442, https://doi.org/10.5194/acp-14-6427-2014, https://doi.org/10.5194/acp-14-6427-2014, 2014
H. Grythe, J. Ström, R. Krejci, P. Quinn, and A. Stohl
Atmos. Chem. Phys., 14, 1277–1297, https://doi.org/10.5194/acp-14-1277-2014, https://doi.org/10.5194/acp-14-1277-2014, 2014
J. Brioude, D. Arnold, A. Stohl, M. Cassiani, D. Morton, P. Seibert, W. Angevine, S. Evan, A. Dingwell, J. D. Fast, R. C. Easter, I. Pisso, J. Burkhart, and G. Wotawa
Geosci. Model Dev., 6, 1889–1904, https://doi.org/10.5194/gmd-6-1889-2013, https://doi.org/10.5194/gmd-6-1889-2013, 2013
M. Cassiani, A. Stohl, and S. Eckhardt
Atmos. Chem. Phys., 13, 9975–9996, https://doi.org/10.5194/acp-13-9975-2013, https://doi.org/10.5194/acp-13-9975-2013, 2013
S. Eckhardt, O. Hermansen, H. Grythe, M. Fiebig, K. Stebel, M. Cassiani, A. Baecklund, and A. Stohl
Atmos. Chem. Phys., 13, 8401–8409, https://doi.org/10.5194/acp-13-8401-2013, https://doi.org/10.5194/acp-13-8401-2013, 2013
M. Laborde, M. Crippa, T. Tritscher, Z. Jurányi, P. F. Decarlo, B. Temime-Roussel, N. Marchand, S. Eckhardt, A. Stohl, U. Baltensperger, A. S. H. Prévôt, E. Weingartner, and M. Gysel
Atmos. Chem. Phys., 13, 5831–5856, https://doi.org/10.5194/acp-13-5831-2013, https://doi.org/10.5194/acp-13-5831-2013, 2013
F. Freutel, J. Schneider, F. Drewnick, S.-L. von der Weiden-Reinmüller, M. Crippa, A. S. H. Prévôt, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, R. Sarda-Estève, J. F. Burkhart, S. Eckhardt, A. Stohl, V. Gros, A. Colomb, V. Michoud, J. F. Doussin, A. Borbon, M. Haeffelin, Y. Morille, M. Beekmann, and S. Borrmann
Atmos. Chem. Phys., 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, https://doi.org/10.5194/acp-13-933-2013, 2013
Matthew Boyer, Diego Aliaga, Lauriane L. J. Quéléver, Silvia Bucci, Hélène Angot, Lubna Dada, Benjamin Heutte, Lisa Beck, Marina Duetsch, Andreas Stohl, Ivo Beck, Tiia Laurila, Nina Sarnela, Roseline C. Thakur, Branka Miljevic, Markku Kulmala, Tuukka Petäjä, Mikko Sipilä, Julia Schmale, and Tuija Jokinen
Atmos. Chem. Phys., 24, 12595–12621, https://doi.org/10.5194/acp-24-12595-2024, https://doi.org/10.5194/acp-24-12595-2024, 2024
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We analyze the seasonal cycle and sources of gases that are relevant for the formation of aerosol particles in the central Arctic. Since theses gases can form new particles, they can influence Arctic climate. We show that the sources of these gases are associated with changes in the Arctic environment during the year, especially with respect to sea ice. Therefore, the concentration of these gases will likely change in the future as the Arctic continues to warm.
Martin Vojta, Andreas Plach, Saurabh Annadate, Sunyoung Park, Gawon Lee, Pallav Purohit, Florian Lindl, Xin Lan, Jens Mühle, Rona L. Thompson, and Andreas Stohl
Atmos. Chem. Phys., 24, 12465–12493, https://doi.org/10.5194/acp-24-12465-2024, https://doi.org/10.5194/acp-24-12465-2024, 2024
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We constrain the global emissions of the very potent greenhouse gas sulfur hexafluoride (SF6) between 2005 and 2021. We show that SF6 emissions are decreasing in the USA and in the EU, while they are substantially growing in China, leading overall to an increasing global emission trend. The national reports for the USA, EU, and China all underestimated their SF6 emissions. However, stringent mitigation measures can successfully reduce SF6 emissions, as can be seen in the EU emission trend.
Olga B. Popovicheva, Marina A. Chichaeva, Nikolaos Evangeliou, Sabine Eckhardt, Evangelia Diapouli, and Nikolay S. Kasimov
EGUsphere, https://doi.org/10.5194/egusphere-2024-3124, https://doi.org/10.5194/egusphere-2024-3124, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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High-quality measurements of light-absorbing carbon were performed at the polar aerosol station "Island Bely” (Western Siberian Arctic) from 2019 to 2022. The maximum light absorption coefficients were seen in summer due to gas flaring contribution, which is the most significant source in the region. However, the increasing Siberian wildfires had a special share in carbon contribution to this high Arctic station with a persistent smoke layer extending over the whole troposphere in summer.
Lucie Bakels, Daria Tatsii, Anne Tipka, Rona Thompson, Marina Dütsch, Michael Blaschek, Petra Seibert, Katharina Baier, Silvia Bucci, Massimo Cassiani, Sabine Eckhardt, Christine Groot Zwaaftink, Stephan Henne, Pirmin Kaufmann, Vincent Lechner, Christian Maurer, Marie D. Mulder, Ignacio Pisso, Andreas Plach, Rakesh Subramanian, Martin Vojta, and Andreas Stohl
Geosci. Model Dev., 17, 7595–7627, https://doi.org/10.5194/gmd-17-7595-2024, https://doi.org/10.5194/gmd-17-7595-2024, 2024
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Computer models are essential for improving our understanding of how gases and particles move in the atmosphere. We present an update of the atmospheric transport model FLEXPART. FLEXPART 11 is more accurate due to a reduced number of interpolations and a new scheme for wet deposition. It can simulate non-spherical aerosols and includes linear chemical reactions. It is parallelised using OpenMP and includes new user options. A new user manual details how to use FLEXPART 11.
Willem E. van Caspel, Zbigniew Klimont, Chris Heyes, and Hilde Fagerli
Atmos. Chem. Phys., 24, 11545–11563, https://doi.org/10.5194/acp-24-11545-2024, https://doi.org/10.5194/acp-24-11545-2024, 2024
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Methane in the atmosphere contributes to the production of ozone gas – an air pollutant and greenhouse gas. Our results highlight that simultaneous reductions in methane emissions help avoid offsetting the air pollution benefits already achieved by the already-approved precursor emission reductions by 2050 in the European Monitoring and Evaluation Programme region, while also playing an important role in bringing air pollution further down towards World Health Organization guideline limits.
Katharina Baier, Lucie Bakels, and Andreas Stohl
EGUsphere, https://doi.org/10.5194/egusphere-2024-2801, https://doi.org/10.5194/egusphere-2024-2801, 2024
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As extremely dry and warm conditions over the Amazon basin can cause huge damages, we study the role of atmospheric transport into the western Amazon for such events. We show that the physical processes depend on the climate variability El Niño Southern Oscillation (ENSO). While warm and dry air from the Atlantic Ocean is transported to the western Amazon for extreme events during the warm ENSO phase, we expect continental regions to have a stronger impact for the other extreme events we found.
Nikolaos Evangeliou, Ondrej Tichy, Marit Svendby Otervik, Sabine Eckhardt, Yves Balkanski, and Didier Hauglustaine
Aerosol Research Discuss., https://doi.org/10.5194/ar-2024-22, https://doi.org/10.5194/ar-2024-22, 2024
Revised manuscript under review for AR
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The COVID-19 lockdown measures in 2020 reduced emissions of various substances improving air quality. However, PM2.5 stayed unchanged due to NH3 and related chemical transformations. Higher humidity favoured more SO42- production so as accumulated NH3 did. Excess NH3 neutralised HNO3 towards NO3-. In high NH3 conditions such as those in 2020, a small reduction of NOx levels drives faster oxidation toward NO3- and slower deposition of total inorganic NO3- causing high secondary PM2.5.
Michel Legrand, Mstislav Vorobyev, Daria Bokuchava, Stanislav Kutuzov, Andreas Plach, Andreas Stohl, Alexandra Khairedinova, Vladimir Mikhalenko, Maria Vinogradova, Sabine Eckhardt, and Susanne Preunkert
EGUsphere, https://doi.org/10.5194/egusphere-2024-1381, https://doi.org/10.5194/egusphere-2024-1381, 2024
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A record of ammonium covering the years 1750 to 2008 was extracted from a 182-meter-long ice core drilled in 2009 at Mt. Elbrus in the Caucasus, Russia. Changes in ammonia emissions in southeastern Europe during the pre-industrial and industrial periods were investigated. The level of ammonium in 1750 indicates a significant contribution of natural sources to the ammonia budget, contrasting with present-day conditions, where agricultural emissions outweigh those from biogenic sources in Europe.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter G. Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1617, https://doi.org/10.5194/egusphere-2024-1617, 2024
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Aerosol particles are an important part of the Earth system, but their concentrations are spatially and temporally heterogeneous, as well as variable in size and composition. Here we present a new compilation of PM2.5 and PM10 aerosol observations, focusing on the spatial variability across different observational stations, including composition, and demonstrate a method for comparing the datasets to model output.
Karl Espen Yttri, Are Bäcklund, Franz Conen, Sabine Eckhardt, Nikolaos Evangeliou, Markus Fiebig, Anne Kasper-Giebl, Avram Gold, Hans Gundersen, Cathrine Lund Myhre, Stephen Matthew Platt, David Simpson, Jason D. Surratt, Sönke Szidat, Martin Rauber, Kjetil Tørseth, Martin Album Ytre-Eide, Zhenfa Zhang, and Wenche Aas
Atmos. Chem. Phys., 24, 2731–2758, https://doi.org/10.5194/acp-24-2731-2024, https://doi.org/10.5194/acp-24-2731-2024, 2024
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We discuss carbonaceous aerosol (CA) observed at the high Arctic Zeppelin Observatory (2017 to 2020). We find that organic aerosol is a significant fraction of the Arctic aerosol, though less than sea salt aerosol and mineral dust, as well as non-sea-salt sulfate, originating mainly from anthropogenic sources in winter and from natural sources in summer, emphasizing the importance of wildfires for biogenic secondary organic aerosol and primary biological aerosol particles observed in the Arctic.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
Preprint withdrawn
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Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
Ondřej Tichý, Sabine Eckhardt, Yves Balkanski, Didier Hauglustaine, and Nikolaos Evangeliou
Atmos. Chem. Phys., 23, 15235–15252, https://doi.org/10.5194/acp-23-15235-2023, https://doi.org/10.5194/acp-23-15235-2023, 2023
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We show declining trends in NH3 emissions over Europe for 2013–2020 using advanced dispersion and inverse modelling and satellite measurements from CrIS. Emissions decreased by −26% since 2013, showing that the abatement strategies adopted by the European Union have been very efficient. Ammonia emissions are low in winter and peak in summer due to temperature-dependent soil volatilization. The largest decreases were observed in central and western Europe in countries with high emissions.
Jenny Oh, Chubashini Shunthirasingham, Ying Duan Lei, Faqiang Zhan, Yuening Li, Abigaëlle Dalpé Castilloux, Amina Ben Chaaben, Zhe Lu, Kelsey Lee, Frank A. P. C. Gobas, Sabine Eckhardt, Nick Alexandrou, Hayley Hung, and Frank Wania
Atmos. Chem. Phys., 23, 10191–10205, https://doi.org/10.5194/acp-23-10191-2023, https://doi.org/10.5194/acp-23-10191-2023, 2023
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An emerging brominated flame retardant (BFR) called TBECH (1,2-dibromo-4-(1,2-dibromoethyl)cyclohexane) has never been produced or imported for use in Canada yet is found to be one of the most abundant gaseous BFRs in the Canadian atmosphere. The recorded spatial and temporal variability of TBECH suggest that the release from imported consumer products containing TBECH is the most likely explanation for its environmental occurrence in Canada.
Monica Crippa, Diego Guizzardi, Tim Butler, Terry Keating, Rosa Wu, Jacek Kaminski, Jeroen Kuenen, Junichi Kurokawa, Satoru Chatani, Tazuko Morikawa, George Pouliot, Jacinthe Racine, Michael D. Moran, Zbigniew Klimont, Patrick M. Manseau, Rabab Mashayekhi, Barron H. Henderson, Steven J. Smith, Harrison Suchyta, Marilena Muntean, Efisio Solazzo, Manjola Banja, Edwin Schaaf, Federico Pagani, Jung-Hun Woo, Jinseok Kim, Fabio Monforti-Ferrario, Enrico Pisoni, Junhua Zhang, David Niemi, Mourad Sassi, Tabish Ansari, and Kristen Foley
Earth Syst. Sci. Data, 15, 2667–2694, https://doi.org/10.5194/essd-15-2667-2023, https://doi.org/10.5194/essd-15-2667-2023, 2023
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This study responds to the global and regional atmospheric modelling community's need for a mosaic of air pollutant emissions with global coverage, long time series, spatially distributed data at a high time resolution, and a high sectoral resolution in order to enhance the understanding of transboundary air pollution. The mosaic approach to integrating official regional emission inventories with a global inventory based on a consistent methodology ensures policy-relevant results.
Marianne Tronstad Lund, Gunnar Myhre, Ragnhild Bieltvedt Skeie, Bjørn Hallvard Samset, and Zbigniew Klimont
Atmos. Chem. Phys., 23, 6647–6662, https://doi.org/10.5194/acp-23-6647-2023, https://doi.org/10.5194/acp-23-6647-2023, 2023
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Here we show that differences, in magnitude and trend, between recent global anthropogenic emission inventories have a notable influence on simulated regional abundances of anthropogenic aerosol over the 1990–2019 period. This, in turn, affects estimates of radiative forcing. Our findings form a basis for comparing existing and upcoming studies on anthropogenic aerosols using different emission inventories.
Anja Eichler, Michel Legrand, Theo M. Jenk, Susanne Preunkert, Camilla Andersson, Sabine Eckhardt, Magnuz Engardt, Andreas Plach, and Margit Schwikowski
The Cryosphere, 17, 2119–2137, https://doi.org/10.5194/tc-17-2119-2023, https://doi.org/10.5194/tc-17-2119-2023, 2023
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We investigate how a 250-year history of the emission of air pollutants (major inorganic aerosol constituents, black carbon, and trace species) is preserved in ice cores from four sites in the European Alps. The observed uniform timing in species-dependent longer-term concentration changes reveals that the different ice-core records provide a consistent, spatially representative signal of the pollution history from western European countries.
Rüdiger Brecht, Lucie Bakels, Alex Bihlo, and Andreas Stohl
Geosci. Model Dev., 16, 2181–2192, https://doi.org/10.5194/gmd-16-2181-2023, https://doi.org/10.5194/gmd-16-2181-2023, 2023
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We use neural-network-based single-image super-resolution to improve the upscaling of meteorological wind fields to be used for particle dispersion models. This deep-learning-based methodology improves the standard linear interpolation typically used in particle dispersion models. The improvement of wind fields leads to substantial improvement in the computed trajectories of the particles.
Matthew Boyer, Diego Aliaga, Jakob Boyd Pernov, Hélène Angot, Lauriane L. J. Quéléver, Lubna Dada, Benjamin Heutte, Manuel Dall'Osto, David C. S. Beddows, Zoé Brasseur, Ivo Beck, Silvia Bucci, Marina Duetsch, Andreas Stohl, Tiia Laurila, Eija Asmi, Andreas Massling, Daniel Charles Thomas, Jakob Klenø Nøjgaard, Tak Chan, Sangeeta Sharma, Peter Tunved, Radovan Krejci, Hans Christen Hansson, Federico Bianchi, Katrianne Lehtipalo, Alfred Wiedensohler, Kay Weinhold, Markku Kulmala, Tuukka Petäjä, Mikko Sipilä, Julia Schmale, and Tuija Jokinen
Atmos. Chem. Phys., 23, 389–415, https://doi.org/10.5194/acp-23-389-2023, https://doi.org/10.5194/acp-23-389-2023, 2023
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The Arctic is a unique environment that is warming faster than other locations on Earth. We evaluate measurements of aerosol particles, which can influence climate, over the central Arctic Ocean for a full year and compare the data to land-based measurement stations across the Arctic. Our measurements show that the central Arctic has similarities to but also distinct differences from the stations further south. We note that this may change as the Arctic warms and sea ice continues to decline.
Martin Vojta, Andreas Plach, Rona L. Thompson, and Andreas Stohl
Geosci. Model Dev., 15, 8295–8323, https://doi.org/10.5194/gmd-15-8295-2022, https://doi.org/10.5194/gmd-15-8295-2022, 2022
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In light of recent global warming, we aim to improve methods for modeling greenhouse gas emissions in order to support the successful implementation of the Paris Agreement. In this study, we investigate certain aspects of a Bayesian inversion method that uses computer simulations and atmospheric observations to improve estimates of greenhouse gas emissions. We explore method limitations, discuss problems, and suggest improvements.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Hanna K. Lappalainen, Tuukka Petäjä, Timo Vihma, Jouni Räisänen, Alexander Baklanov, Sergey Chalov, Igor Esau, Ekaterina Ezhova, Matti Leppäranta, Dmitry Pozdnyakov, Jukka Pumpanen, Meinrat O. Andreae, Mikhail Arshinov, Eija Asmi, Jianhui Bai, Igor Bashmachnikov, Boris Belan, Federico Bianchi, Boris Biskaborn, Michael Boy, Jaana Bäck, Bin Cheng, Natalia Chubarova, Jonathan Duplissy, Egor Dyukarev, Konstantinos Eleftheriadis, Martin Forsius, Martin Heimann, Sirkku Juhola, Vladimir Konovalov, Igor Konovalov, Pavel Konstantinov, Kajar Köster, Elena Lapshina, Anna Lintunen, Alexander Mahura, Risto Makkonen, Svetlana Malkhazova, Ivan Mammarella, Stefano Mammola, Stephany Buenrostro Mazon, Outi Meinander, Eugene Mikhailov, Victoria Miles, Stanislav Myslenkov, Dmitry Orlov, Jean-Daniel Paris, Roberta Pirazzini, Olga Popovicheva, Jouni Pulliainen, Kimmo Rautiainen, Torsten Sachs, Vladimir Shevchenko, Andrey Skorokhod, Andreas Stohl, Elli Suhonen, Erik S. Thomson, Marina Tsidilina, Veli-Pekka Tynkkynen, Petteri Uotila, Aki Virkkula, Nadezhda Voropay, Tobias Wolf, Sayaka Yasunaka, Jiahua Zhang, Yubao Qiu, Aijun Ding, Huadong Guo, Valery Bondur, Nikolay Kasimov, Sergej Zilitinkevich, Veli-Matti Kerminen, and Markku Kulmala
Atmos. Chem. Phys., 22, 4413–4469, https://doi.org/10.5194/acp-22-4413-2022, https://doi.org/10.5194/acp-22-4413-2022, 2022
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We summarize results during the last 5 years in the northern Eurasian region, especially from Russia, and introduce recent observations of the air quality in the urban environments in China. Although the scientific knowledge in these regions has increased, there are still gaps in our understanding of large-scale climate–Earth surface interactions and feedbacks. This arises from limitations in research infrastructures and integrative data analyses, hindering a comprehensive system analysis.
Christine D. Groot Zwaaftink, Wenche Aas, Sabine Eckhardt, Nikolaos Evangeliou, Paul Hamer, Mona Johnsrud, Arve Kylling, Stephen M. Platt, Kerstin Stebel, Hilde Uggerud, and Karl Espen Yttri
Atmos. Chem. Phys., 22, 3789–3810, https://doi.org/10.5194/acp-22-3789-2022, https://doi.org/10.5194/acp-22-3789-2022, 2022
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We investigate causes of a poor-air-quality episode in northern Europe in October 2020 during which EU health limits for air quality were vastly exceeded. Such episodes may trigger measures to improve air quality. Analysis based on satellite observations, transport simulations, and surface observations revealed two sources of pollution. Emissions of mineral dust in Central Asia and biomass burning in Ukraine arrived almost simultaneously in Norway, and transport continued into the Arctic.
Stephen M. Platt, Øystein Hov, Torunn Berg, Knut Breivik, Sabine Eckhardt, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Markus Fiebig, Rebecca Fisher, Georg Hansen, Hans-Christen Hansson, Jost Heintzenberg, Ove Hermansen, Dominic Heslin-Rees, Kim Holmén, Stephen Hudson, Roland Kallenborn, Radovan Krejci, Terje Krognes, Steinar Larssen, David Lowry, Cathrine Lund Myhre, Chris Lunder, Euan Nisbet, Pernilla B. Nizzetto, Ki-Tae Park, Christina A. Pedersen, Katrine Aspmo Pfaffhuber, Thomas Röckmann, Norbert Schmidbauer, Sverre Solberg, Andreas Stohl, Johan Ström, Tove Svendby, Peter Tunved, Kjersti Tørnkvist, Carina van der Veen, Stergios Vratolis, Young Jun Yoon, Karl Espen Yttri, Paul Zieger, Wenche Aas, and Kjetil Tørseth
Atmos. Chem. Phys., 22, 3321–3369, https://doi.org/10.5194/acp-22-3321-2022, https://doi.org/10.5194/acp-22-3321-2022, 2022
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Here we detail the history of the Zeppelin Observatory, a unique global background site and one of only a few in the high Arctic. We present long-term time series of up to 30 years of atmospheric components and atmospheric transport phenomena. Many of these time series are important to our understanding of Arctic and global atmospheric composition change. Finally, we discuss the future of the Zeppelin Observatory and emerging areas of future research on the Arctic atmosphere.
Jessica L. McCarty, Juha Aalto, Ville-Veikko Paunu, Steve R. Arnold, Sabine Eckhardt, Zbigniew Klimont, Justin J. Fain, Nikolaos Evangeliou, Ari Venäläinen, Nadezhda M. Tchebakova, Elena I. Parfenova, Kaarle Kupiainen, Amber J. Soja, Lin Huang, and Simon Wilson
Biogeosciences, 18, 5053–5083, https://doi.org/10.5194/bg-18-5053-2021, https://doi.org/10.5194/bg-18-5053-2021, 2021
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Fires, including extreme fire seasons, and fire emissions are more common in the Arctic. A review and synthesis of current scientific literature find climate change and human activity in the north are fuelling an emerging Arctic fire regime, causing more black carbon and methane emissions within the Arctic. Uncertainties persist in characterizing future fire landscapes, and thus emissions, as well as policy-relevant challenges in understanding, monitoring, and managing Arctic fire regimes.
Ulas Im, Kostas Tsigaridis, Gregory Faluvegi, Peter L. Langen, Joshua P. French, Rashed Mahmood, Manu A. Thomas, Knut von Salzen, Daniel C. Thomas, Cynthia H. Whaley, Zbigniew Klimont, Henrik Skov, and Jørgen Brandt
Atmos. Chem. Phys., 21, 10413–10438, https://doi.org/10.5194/acp-21-10413-2021, https://doi.org/10.5194/acp-21-10413-2021, 2021
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Future (2015–2050) simulations of the aerosol burdens and their radiative forcing and climate impacts over the Arctic under various emission projections show that although the Arctic aerosol burdens are projected to decrease significantly by 10 to 60 %, regardless of the magnitude of aerosol reductions, surface air temperatures will continue to increase by 1.9–2.6 ℃, while sea-ice extent will continue to decrease, implying reductions of greenhouse gases are necessary to mitigate climate change.
Karl Espen Yttri, Francesco Canonaco, Sabine Eckhardt, Nikolaos Evangeliou, Markus Fiebig, Hans Gundersen, Anne-Gunn Hjellbrekke, Cathrine Lund Myhre, Stephen Matthew Platt, André S. H. Prévôt, David Simpson, Sverre Solberg, Jason Surratt, Kjetil Tørseth, Hilde Uggerud, Marit Vadset, Xin Wan, and Wenche Aas
Atmos. Chem. Phys., 21, 7149–7170, https://doi.org/10.5194/acp-21-7149-2021, https://doi.org/10.5194/acp-21-7149-2021, 2021
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Carbonaceous aerosol sources and trends were studied at the Birkenes Observatory. A large decrease in elemental carbon (EC; 2001–2018) and a smaller decline in levoglucosan (2008–2018) suggest that organic carbon (OC)/EC from traffic/industry is decreasing, whereas the abatement of OC/EC from biomass burning has been less successful. Positive matrix factorization apportioned 72 % of EC to fossil fuel sources and 53 % (PM2.5) and 78 % (PM10–2.5) of OC to biogenic sources.
Nikolaos Evangeliou, Yves Balkanski, Sabine Eckhardt, Anne Cozic, Martin Van Damme, Pierre-François Coheur, Lieven Clarisse, Mark W. Shephard, Karen E. Cady-Pereira, and Didier Hauglustaine
Atmos. Chem. Phys., 21, 4431–4451, https://doi.org/10.5194/acp-21-4431-2021, https://doi.org/10.5194/acp-21-4431-2021, 2021
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Ammonia, a substance that has played a key role in sustaining life, has been increasing in the atmosphere, affecting climate and humans. Understanding the reasons for this increase is important for the beneficial use of ammonia. The evolution of satellite products gives us the opportunity to calculate ammonia emissions easier. We calculated global ammonia emissions over the last 10 years, incorporated them into a chemistry model and recorded notable improvement in reproducing observations.
Nikolaos Evangeliou, Stephen M. Platt, Sabine Eckhardt, Cathrine Lund Myhre, Paolo Laj, Lucas Alados-Arboledas, John Backman, Benjamin T. Brem, Markus Fiebig, Harald Flentje, Angela Marinoni, Marco Pandolfi, Jesus Yus-Dìez, Natalia Prats, Jean P. Putaud, Karine Sellegri, Mar Sorribas, Konstantinos Eleftheriadis, Stergios Vratolis, Alfred Wiedensohler, and Andreas Stohl
Atmos. Chem. Phys., 21, 2675–2692, https://doi.org/10.5194/acp-21-2675-2021, https://doi.org/10.5194/acp-21-2675-2021, 2021
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Following the transmission of SARS-CoV-2 to Europe, social distancing rules were introduced to prevent further spread. We investigate the impacts of the European lockdowns on black carbon (BC) emissions by means of in situ observations and inverse modelling. BC emissions declined by 23 kt in Europe during the lockdowns as compared with previous years and by 11 % as compared to the period prior to lockdowns. Residential combustion prevailed in Eastern Europe, as confirmed by remote sensing data.
Ondřej Tichý, Lukáš Ulrych, Václav Šmídl, Nikolaos Evangeliou, and Andreas Stohl
Geosci. Model Dev., 13, 5917–5934, https://doi.org/10.5194/gmd-13-5917-2020, https://doi.org/10.5194/gmd-13-5917-2020, 2020
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We study the estimation of the temporal profile of an atmospheric release using formalization as a linear inverse problem. The problem is typically ill-posed, so all state-of-the-art methods need some form of regularization using additional information. We provide a sensitivity study on the prior source term and regularization parameters for the shape of the source term with a demonstration on the ETEX experimental release and the Cs-134 and Cs-137 dataset from the Chernobyl accident.
Marianne T. Lund, Borgar Aamaas, Camilla W. Stjern, Zbigniew Klimont, Terje K. Berntsen, and Bjørn H. Samset
Earth Syst. Dynam., 11, 977–993, https://doi.org/10.5194/esd-11-977-2020, https://doi.org/10.5194/esd-11-977-2020, 2020
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Achieving the Paris Agreement temperature goals requires both near-zero levels of long-lived greenhouse gases and deep cuts in emissions of short-lived climate forcers (SLCFs). Here we quantify the near- and long-term global temperature impacts of emissions of individual SLCFs and CO2 from 7 economic sectors in 13 regions in order to provide the detailed knowledge needed to design efficient mitigation strategies at the sectoral and regional levels.
Arve Kylling, Hamidreza Ardeshiri, Massimo Cassiani, Anna Solvejg Dinger, Soon-Young Park, Ignacio Pisso, Norbert Schmidbauer, Kerstin Stebel, and Andreas Stohl
Atmos. Meas. Tech., 13, 3303–3318, https://doi.org/10.5194/amt-13-3303-2020, https://doi.org/10.5194/amt-13-3303-2020, 2020
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Atmospheric turbulence and its effect on tracer dispersion in particular may be measured by cameras sensitive to the absorption of ultraviolet (UV) sunlight by sulfur dioxide (SO2). Using large eddy simulation and 3D Monte Carlo radiative transfer modelling of a SO2 plume, we demonstrate that UV camera images of SO2 plumes may be used to derive plume statistics of relevance for the study of atmospheric turbulent dispersion.
Yugo Kanaya, Kazuyo Yamaji, Takuma Miyakawa, Fumikazu Taketani, Chunmao Zhu, Yongjoo Choi, Yuichi Komazaki, Kohei Ikeda, Yutaka Kondo, and Zbigniew Klimont
Atmos. Chem. Phys., 20, 6339–6356, https://doi.org/10.5194/acp-20-6339-2020, https://doi.org/10.5194/acp-20-6339-2020, 2020
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Fundamental disagreements among bottom-up emission inventories exist about the sign of the black carbon emissions trend from China over the past decade. Our decadal observations on Fukue Island clearly indicate its rapid reduction, after correcting for interannual meteorological variability, which supports inventories reflecting governmental clean air actions after 2010. The reduction pace surpasses those of SSP1 scenarios for 2015–2030, suggesting highly successful emission control policies.
Leyang Feng, Steven J. Smith, Caleb Braun, Monica Crippa, Matthew J. Gidden, Rachel Hoesly, Zbigniew Klimont, Margreet van Marle, Maarten van den Berg, and Guido R. van der Werf
Geosci. Model Dev., 13, 461–482, https://doi.org/10.5194/gmd-13-461-2020, https://doi.org/10.5194/gmd-13-461-2020, 2020
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We describe the methods used for generating gridded emission datasets produced for use by the modeling community, particularly for the Coupled Model Intercomparison Project Phase 6 (CMIP6). The development of three sets of gridded data (historical open burning, historical anthropogenic, and future scenarios) was coordinated to produce consistent data over 1750–2100. We discuss the methodologies used to produce these data along with limitations and potential for future work.
Ignacio Pisso, Espen Sollum, Henrik Grythe, Nina I. Kristiansen, Massimo Cassiani, Sabine Eckhardt, Delia Arnold, Don Morton, Rona L. Thompson, Christine D. Groot Zwaaftink, Nikolaos Evangeliou, Harald Sodemann, Leopold Haimberger, Stephan Henne, Dominik Brunner, John F. Burkhart, Anne Fouilloux, Jerome Brioude, Anne Philipp, Petra Seibert, and Andreas Stohl
Geosci. Model Dev., 12, 4955–4997, https://doi.org/10.5194/gmd-12-4955-2019, https://doi.org/10.5194/gmd-12-4955-2019, 2019
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We present the latest release of the Lagrangian transport model FLEXPART, which simulates the transport, diffusion, dry and wet deposition, radioactive decay, and 1st-order chemical reactions of atmospheric tracers. The model has been recently updated both technically and in the representation of physicochemical processes. We describe the changes, document the most recent input and output files, provide working examples, and introduce testing capabilities.
Jens Mühle, Cathy M. Trudinger, Luke M. Western, Matthew Rigby, Martin K. Vollmer, Sunyoung Park, Alistair J. Manning, Daniel Say, Anita Ganesan, L. Paul Steele, Diane J. Ivy, Tim Arnold, Shanlan Li, Andreas Stohl, Christina M. Harth, Peter K. Salameh, Archie McCulloch, Simon O'Doherty, Mi-Kyung Park, Chun Ok Jo, Dickon Young, Kieran M. Stanley, Paul B. Krummel, Blagoj Mitrevski, Ove Hermansen, Chris Lunder, Nikolaos Evangeliou, Bo Yao, Jooil Kim, Benjamin Hmiel, Christo Buizert, Vasilii V. Petrenko, Jgor Arduini, Michela Maione, David M. Etheridge, Eleni Michalopoulou, Mike Czerniak, Jeffrey P. Severinghaus, Stefan Reimann, Peter G. Simmonds, Paul J. Fraser, Ronald G. Prinn, and Ray F. Weiss
Atmos. Chem. Phys., 19, 10335–10359, https://doi.org/10.5194/acp-19-10335-2019, https://doi.org/10.5194/acp-19-10335-2019, 2019
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We discuss atmospheric concentrations and emissions of the strong greenhouse gas perfluorocyclobutane. A large fraction of recent emissions stem from China, India, and Russia, probably as a by-product from the production of fluoropolymers and fluorochemicals. Most historic emissions likely stem from developed countries. Total emissions are higher than what is being reported. Clearly, more measurements and better reporting are needed to understand emissions of this and other greenhouse gases.
Karl Espen Yttri, David Simpson, Robert Bergström, Gyula Kiss, Sönke Szidat, Darius Ceburnis, Sabine Eckhardt, Christoph Hueglin, Jacob Klenø Nøjgaard, Cinzia Perrino, Ignazio Pisso, Andre Stephan Henry Prevot, Jean-Philippe Putaud, Gerald Spindler, Milan Vana, Yan-Lin Zhang, and Wenche Aas
Atmos. Chem. Phys., 19, 4211–4233, https://doi.org/10.5194/acp-19-4211-2019, https://doi.org/10.5194/acp-19-4211-2019, 2019
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Carbonaceous aerosols from natural sources were abundant regardless of season. Residential wood burning (RWB) emissions were occasionally equally as large as or larger than of fossil-fuel sources, depending on season and region. RWB emissions are poorly constrained; thus emissions inventories need improvement. Harmonizing emission factors between countries is likely the most important step to improve model calculations for biomass burning emissions and European PM2.5 concentrations in general.
Nikolaos Evangeliou, Arve Kylling, Sabine Eckhardt, Viktor Myroniuk, Kerstin Stebel, Ronan Paugam, Sergiy Zibtsev, and Andreas Stohl
Atmos. Chem. Phys., 19, 1393–1411, https://doi.org/10.5194/acp-19-1393-2019, https://doi.org/10.5194/acp-19-1393-2019, 2019
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We simulated the peatland fires that burned in Greenland in summer 2017. Using satellite data, we estimated that the total burned area was 2345 ha, the fuel amount consumed 117 kt C and the emissions of BC, OC and BrC 23.5, 731 and 141 t, respectively. About 30 % of the emissions were deposited on snow or ice surfaces. This caused a maximum albedo change of 0.007 and a surface radiative forcing of 0.03–0.04 W m−2, with local maxima of up to 0.63–0.77 W m−2. Overall, the fires had a small impact.
Stephen M. Platt, Sabine Eckhardt, Benedicte Ferré, Rebecca E. Fisher, Ove Hermansen, Pär Jansson, David Lowry, Euan G. Nisbet, Ignacio Pisso, Norbert Schmidbauer, Anna Silyakova, Andreas Stohl, Tove M. Svendby, Sunil Vadakkepuliyambatta, Jürgen Mienert, and Cathrine Lund Myhre
Atmos. Chem. Phys., 18, 17207–17224, https://doi.org/10.5194/acp-18-17207-2018, https://doi.org/10.5194/acp-18-17207-2018, 2018
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We measured atmospheric mixing ratios of methane over the Arctic Ocean around Svalbard and compared observed variations to inventories for anthropogenic, wetland, and biomass burning methane emissions and an atmospheric transport model. With knowledge of where variations were expected due to the aforementioned land-based emissions, we were able to identify and quantify a methane source from the ocean north of Svalbard, likely from sub-sea hydrocarbon seeps and/or gas hydrate decomposition.
Anna Solvejg Dinger, Kerstin Stebel, Massimo Cassiani, Hamidreza Ardeshiri, Cirilo Bernardo, Arve Kylling, Soon-Young Park, Ignacio Pisso, Norbert Schmidbauer, Jan Wasseng, and Andreas Stohl
Atmos. Meas. Tech., 11, 6169–6188, https://doi.org/10.5194/amt-11-6169-2018, https://doi.org/10.5194/amt-11-6169-2018, 2018
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This study presents an artificial release experiment aimed to improve the understanding of turbulence in the atmospheric boundary layer. A new set of image processing methods was developed to analyse the turbulent dispersion of sulfur dioxide (SO2) puffs. For this a tomographic setup of six SO2 cameras was used to image artificially released SO2 gas.
Christine D. Groot Zwaaftink, Stephan Henne, Rona L. Thompson, Edward J. Dlugokencky, Toshinobu Machida, Jean-Daniel Paris, Motoki Sasakawa, Arjo Segers, Colm Sweeney, and Andreas Stohl
Geosci. Model Dev., 11, 4469–4487, https://doi.org/10.5194/gmd-11-4469-2018, https://doi.org/10.5194/gmd-11-4469-2018, 2018
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A Lagrangian particle dispersion model is used to simulate global fields of methane, constrained by observations through nudging. We show that this rather simple and computationally inexpensive method can give results similar to or as good as a computationally expensive Eulerian chemistry transport model with a data assimilation scheme. The three-dimensional methane fields are of interest to applications such as inverse modelling and satellite retrievals.
Nikolaos Evangeliou, Rona L. Thompson, Sabine Eckhardt, and Andreas Stohl
Atmos. Chem. Phys., 18, 15307–15327, https://doi.org/10.5194/acp-18-15307-2018, https://doi.org/10.5194/acp-18-15307-2018, 2018
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We present BC inversions at high northern latitudes in 2013–2015. The emissions were high close to the gas flaring regions in Russia and in western Canada. The posterior emissions of BC at latitudes > 50° N were estimated as 560 ± 171 kt yr-1, smaller than in bottom-up inventories. Posterior concentrations over the Arctic compared with independent observations from flight and ship campaigns showed small biases. Seasonal maxima were estimated in summer months due to biomass burning, mainly in Europe.
Lauren M. Zamora, Ralph A. Kahn, Klaus B. Huebert, Andreas Stohl, and Sabine Eckhardt
Atmos. Chem. Phys., 18, 14949–14964, https://doi.org/10.5194/acp-18-14949-2018, https://doi.org/10.5194/acp-18-14949-2018, 2018
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We use satellite data and model output to estimate how airborne particles (aerosols) affect cloud ice particles and droplets over the Arctic Ocean. Aerosols from sources like smoke and pollution can change cloud cover, precipitation frequency, and the portion of liquid- vs. ice-containing clouds, which in turn can impact the surface energy budget. By improving our understanding these aerosol–cloud interactions, this work can help climate predictions for the rapidly changing Arctic.
Chandra Venkataraman, Michael Brauer, Kushal Tibrewal, Pankaj Sadavarte, Qiao Ma, Aaron Cohen, Sreelekha Chaliyakunnel, Joseph Frostad, Zbigniew Klimont, Randall V. Martin, Dylan B. Millet, Sajeev Philip, Katherine Walker, and Shuxiao Wang
Atmos. Chem. Phys., 18, 8017–8039, https://doi.org/10.5194/acp-18-8017-2018, https://doi.org/10.5194/acp-18-8017-2018, 2018
Meng Li, Zbigniew Klimont, Qiang Zhang, Randall V. Martin, Bo Zheng, Chris Heyes, Janusz Cofala, Yuxuan Zhang, and Kebin He
Atmos. Chem. Phys., 18, 3433–3456, https://doi.org/10.5194/acp-18-3433-2018, https://doi.org/10.5194/acp-18-3433-2018, 2018
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In this paper, we conducted a comprehensive evaluation of two widely used anthropogenic emission inventories over China, ECLIPSE and MIX, to explore the potential sources of uncertainties and find clues to improving emission inventories. We found that SO2 emission estimates are consistent between the two inventories (with 1 % differences), while NOx emissions in ECLIPSE's estimates are 16 % lower than those in MIX. Discrepancies at the sector and provincial levels are much higher.
Rachel M. Hoesly, Steven J. Smith, Leyang Feng, Zbigniew Klimont, Greet Janssens-Maenhout, Tyler Pitkanen, Jonathan J. Seibert, Linh Vu, Robert J. Andres, Ryan M. Bolt, Tami C. Bond, Laura Dawidowski, Nazar Kholod, June-ichi Kurokawa, Meng Li, Liang Liu, Zifeng Lu, Maria Cecilia P. Moura, Patrick R. O'Rourke, and Qiang Zhang
Geosci. Model Dev., 11, 369–408, https://doi.org/10.5194/gmd-11-369-2018, https://doi.org/10.5194/gmd-11-369-2018, 2018
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Historical emission trends are key inputs to Earth systems and atmospheric chemistry models. We present a new data set of historical (1750–2014) anthropogenic gases (CO, CH4, NH3, NOx, SO2, NMVOCs, BC, OC, and CO2) developed with the Community Emissions Data System (CEDS). This improves on existing inventories as it uses consistent methods and data across emissions species, has annual resolution for a longer and more recent time series, and is designed to be transparent and reproducible.
Nikolaos Evangeliou, Vladimir P. Shevchenko, Karl Espen Yttri, Sabine Eckhardt, Espen Sollum, Oleg S. Pokrovsky, Vasily O. Kobelev, Vladimir B. Korobov, Andrey A. Lobanov, Dina P. Starodymova, Sergey N. Vorobiev, Rona L. Thompson, and Andreas Stohl
Atmos. Chem. Phys., 18, 963–977, https://doi.org/10.5194/acp-18-963-2018, https://doi.org/10.5194/acp-18-963-2018, 2018
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We present EC measurements from an uncertain region in terms of emissions (Russia). Its origin is quantified with a Lagrangian model that uses a recently developed feature that allows backward estimation of the specific source locations that contribute to the deposited mass. In NW European Russia transportation and domestic combustion from Finland was important. A systematic underestimation was found in W Siberia at places where gas flaring was important, implying miscalculation or sources.
Bastien Sauvage, Alain Fontaine, Sabine Eckhardt, Antoine Auby, Damien Boulanger, Hervé Petetin, Ronan Paugam, Gilles Athier, Jean-Marc Cousin, Sabine Darras, Philippe Nédélec, Andreas Stohl, Solène Turquety, Jean-Pierre Cammas, and Valérie Thouret
Atmos. Chem. Phys., 17, 15271–15292, https://doi.org/10.5194/acp-17-15271-2017, https://doi.org/10.5194/acp-17-15271-2017, 2017
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We provide the scientific community with a SOFT-IO tool based on the coupling of Lagrangian modeling with emission inventories and aircraft CO measurements, which is able to calculate the contribution of the sources and geographical origins of CO measurements, with good performances. Calculated CO added-value products will help scientists in interpreting large IAGOS CO data set. SOFT-IO could further be applied to other CO data sets or used to help validate emission inventories.
Sabine Eckhardt, Massimo Cassiani, Nikolaos Evangeliou, Espen Sollum, Ignacio Pisso, and Andreas Stohl
Geosci. Model Dev., 10, 4605–4618, https://doi.org/10.5194/gmd-10-4605-2017, https://doi.org/10.5194/gmd-10-4605-2017, 2017
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We extend the backward modelling technique in the existing model FLEXPART to substances deposited at the Earth’s surface by wet scavenging and dry deposition. This means that for existing measurements of a substance in snow, ice cores or rain samples the source regions can be determined. This will help the interpretation of the measurement as well as gaining information of emission strength at the source of the deposited substance.
Ondřej Tichý, Václav Šmídl, Radek Hofman, Kateřina Šindelářová, Miroslav Hýža, and Andreas Stohl
Atmos. Chem. Phys., 17, 12677–12696, https://doi.org/10.5194/acp-17-12677-2017, https://doi.org/10.5194/acp-17-12677-2017, 2017
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In the fall of 2011, iodine-131 (131I) was detected at several radionuclide monitoring stations in central Europe. We estimate the source location and emission variation using only the available 131I measurements. Subsequently, we use the IAEA report about the source term for validation of our results. We find that our algorithm could successfully locate the actual release site. The findings are also in agreement with the values reported by the IAEA.
Franz Conen, Sabine Eckhardt, Hans Gundersen, Andreas Stohl, and Karl Espen Yttri
Atmos. Chem. Phys., 17, 11065–11073, https://doi.org/10.5194/acp-17-11065-2017, https://doi.org/10.5194/acp-17-11065-2017, 2017
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Observation of ice nuclei active at −8 °C show that rainfall drives their abundance throughout all seasons and that they are equally distributed amongst coarse and fine fraction of PM10. Concurrent measurements of fungal spore markers suggest that some fraction of INP-8 may consist of fungal spores during the warm part of the year. Snow cover suppresses the aerosolisation of ice nuclei. Changes in snow cover and rainfall may affect atmospheric concentrations of ice nuclei in future.
Christine D. Groot Zwaaftink, Ólafur Arnalds, Pavla Dagsson-Waldhauserova, Sabine Eckhardt, Joseph M. Prospero, and Andreas Stohl
Atmos. Chem. Phys., 17, 10865–10878, https://doi.org/10.5194/acp-17-10865-2017, https://doi.org/10.5194/acp-17-10865-2017, 2017
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How much dust do Icelandic sources emit and where is this dust deposited? We modelled dust emission and transport from Icelandic sources over 27 years with FLEXPART. Results show that Icelandic dust sources can have emission rates similar to parts of the Sahara and considerable amounts of dust are deposited in the ocean and on glaciers.
Augustin Colette, Camilla Andersson, Astrid Manders, Kathleen Mar, Mihaela Mircea, Maria-Teresa Pay, Valentin Raffort, Svetlana Tsyro, Cornelius Cuvelier, Mario Adani, Bertrand Bessagnet, Robert Bergström, Gino Briganti, Tim Butler, Andrea Cappelletti, Florian Couvidat, Massimo D'Isidoro, Thierno Doumbia, Hilde Fagerli, Claire Granier, Chris Heyes, Zig Klimont, Narendra Ojha, Noelia Otero, Martijn Schaap, Katarina Sindelarova, Annemiek I. Stegehuis, Yelva Roustan, Robert Vautard, Erik van Meijgaard, Marta Garcia Vivanco, and Peter Wind
Geosci. Model Dev., 10, 3255–3276, https://doi.org/10.5194/gmd-10-3255-2017, https://doi.org/10.5194/gmd-10-3255-2017, 2017
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The EURODELTA-Trends numerical experiment has been designed to assess the capability of chemistry-transport models to capture the evolution of surface air quality over the 1990–2010 period in Europe. It also includes sensitivity experiments in order to analyse the relative contribution of (i) emission changes, (ii) meteorological variability, and (iii) boundary conditions to air quality trends. The article is a detailed presentation of the experiment design and participating models.
Nikolaos Evangeliou, Thomas Hamburger, Anne Cozic, Yves Balkanski, and Andreas Stohl
Atmos. Chem. Phys., 17, 8805–8824, https://doi.org/10.5194/acp-17-8805-2017, https://doi.org/10.5194/acp-17-8805-2017, 2017
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This is the first paper that attempts to assess the source term of the Chernobyl accident using not only activity concentrations but also deposition measurements. This is done by using the FLEXPART model combined with a Bayesian inversion algorithm. Our results show that the altitude of the injection during the first days of the accident might have reached up to 3 km, in contrast to what has been already reported (2.2 km maximum), in order the model to better match observations.
Zbigniew Klimont, Kaarle Kupiainen, Chris Heyes, Pallav Purohit, Janusz Cofala, Peter Rafaj, Jens Borken-Kleefeld, and Wolfgang Schöpp
Atmos. Chem. Phys., 17, 8681–8723, https://doi.org/10.5194/acp-17-8681-2017, https://doi.org/10.5194/acp-17-8681-2017, 2017
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This paper presents a comprehensive assessment of global anthropogenic emissions of particulate matter for 1990–2010. Global emissions have not changed much in this period, showing a strong decoupling from the increase in energy consumption (and carbon dioxide emissions). Regional trends were different – increase in East Asia and Africa and decline in Europe and North America. In 2010, 60 % of emissions originated in Asia and more than half from cooking and heating stoves.
Lauren M. Zamora, Ralph A. Kahn, Sabine Eckhardt, Allison McComiskey, Patricia Sawamura, Richard Moore, and Andreas Stohl
Atmos. Chem. Phys., 17, 7311–7332, https://doi.org/10.5194/acp-17-7311-2017, https://doi.org/10.5194/acp-17-7311-2017, 2017
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Clouds have a major but uncertain effect on Arctic surface temperatures. Here, we used remote sensing observations to better understand aerosol effects on one type of Arctic cloud. By modifying a variety of cloud properties, aerosols in this type of cloud indirectly reduced the net warming effect of these clouds on the surface by ~ 10 % of the clean-background cloud effect, not including changes in cloud fraction. This work will improve our ability to predict future Arctic surface temperatures.
Eri Saikawa, Hankyul Kim, Min Zhong, Alexander Avramov, Yu Zhao, Greet Janssens-Maenhout, Jun-ichi Kurokawa, Zbigniew Klimont, Fabian Wagner, Vaishali Naik, Larry W. Horowitz, and Qiang Zhang
Atmos. Chem. Phys., 17, 6393–6421, https://doi.org/10.5194/acp-17-6393-2017, https://doi.org/10.5194/acp-17-6393-2017, 2017
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We analyze differences in existing air pollutant emission estimates to better understand the magnitude of emissions as well as the source regions and sectors of air pollution in China. We find large disagreements among the inventories, and we show that these differences have a significant impact on regional air quality simulations. Better understanding of air pollutant emissions at more disaggregated levels is essential for air pollution mitigation in China.
Henrik Grythe, Nina I. Kristiansen, Christine D. Groot Zwaaftink, Sabine Eckhardt, Johan Ström, Peter Tunved, Radovan Krejci, and Andreas Stohl
Geosci. Model Dev., 10, 1447–1466, https://doi.org/10.5194/gmd-10-1447-2017, https://doi.org/10.5194/gmd-10-1447-2017, 2017
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A new and more physically based treatment of how removal by precipitation is calculated by FLEXPART is introduced to take into account more aspects of aerosol diversity. Also new is the definition of clouds and cloud properties. Results from simulations show good agreement with observed atmospheric concentrations for distinctly different aerosols. Atmospheric lifetimes were found to vary from a few hours (large aerosol particles) up to a month (small non-soluble particles)
Monika Wittmann, Christine Dorothea Groot Zwaaftink, Louise Steffensen Schmidt, Sverrir Guðmundsson, Finnur Pálsson, Olafur Arnalds, Helgi Björnsson, Throstur Thorsteinsson, and Andreas Stohl
The Cryosphere, 11, 741–754, https://doi.org/10.5194/tc-11-741-2017, https://doi.org/10.5194/tc-11-741-2017, 2017
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This work includes a study on the effects of dust deposition on the mass balance of Brúarjökull, an outlet glacier of Vatnajökull, Iceland's largest ice cap. A model was used to simulate dust deposition on the glacier, and these periods of dust were compared to albedo measurements at two weather stations on Brúarjökull to evaluate the dust impact. We determine the influence of dust events on the snow albedo and the surface energy balance.
Rona L. Thompson, Motoki Sasakawa, Toshinobu Machida, Tuula Aalto, Doug Worthy, Jost V. Lavric, Cathrine Lund Myhre, and Andreas Stohl
Atmos. Chem. Phys., 17, 3553–3572, https://doi.org/10.5194/acp-17-3553-2017, https://doi.org/10.5194/acp-17-3553-2017, 2017
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Methane (CH4) fluxes were estimated for the high northern latitudes for 2005–2013 based on observations of atmospheric CH4 mixing ratios. Methane fluxes were found to be higher than prior estimates in northern Eurasia and Canada, especially in the Western Siberian Lowlands and the Canadian province Alberta. Significant inter-annual variations in the fluxes were found as well as a small positive trend. In Canada, the trend may be related to an increase in soil temperature over the study period.
Gunnar Myhre, Wenche Aas, Ribu Cherian, William Collins, Greg Faluvegi, Mark Flanner, Piers Forster, Øivind Hodnebrog, Zbigniew Klimont, Marianne T. Lund, Johannes Mülmenstädt, Cathrine Lund Myhre, Dirk Olivié, Michael Prather, Johannes Quaas, Bjørn H. Samset, Jordan L. Schnell, Michael Schulz, Drew Shindell, Ragnhild B. Skeie, Toshihiko Takemura, and Svetlana Tsyro
Atmos. Chem. Phys., 17, 2709–2720, https://doi.org/10.5194/acp-17-2709-2017, https://doi.org/10.5194/acp-17-2709-2017, 2017
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Over the past decades, the geographical distribution of emissions of substances that alter the atmospheric energy balance has changed due to economic growth and pollution regulations. Here, we show the resulting changes to aerosol and ozone abundances and their radiative forcing using recently updated emission data for the period 1990–2015, as simulated by seven global atmospheric composition models. The global mean radiative forcing is more strongly positive than reported in IPCC AR5.
Ondřej Tichý, Václav Šmídl, Radek Hofman, and Andreas Stohl
Geosci. Model Dev., 9, 4297–4311, https://doi.org/10.5194/gmd-9-4297-2016, https://doi.org/10.5194/gmd-9-4297-2016, 2016
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Estimation of pollutant releases into the atmosphere is an important problem in the environmental sciences. We formulate a probabilistic model, where a full Bayesian estimation allows estimation of all tuning parameters from the measurements. The proposed algorithm is tested and compared with the state-of-the-art method on data from the European Tracer Experiment (ETEX), where advantages of the new method are demonstrated.
Xiao Lu, Lin Zhang, Xu Yue, Jiachen Zhang, Daniel A. Jaffe, Andreas Stohl, Yuanhong Zhao, and Jingyuan Shao
Atmos. Chem. Phys., 16, 14687–14702, https://doi.org/10.5194/acp-16-14687-2016, https://doi.org/10.5194/acp-16-14687-2016, 2016
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Increasing wildfire activities in the mountainous western US may present a challenge for the region to attain a recently revised ozone air quality standard in summer. We quantify the wildfire influence on the ozone variability, trends, and number of high ozone days over this region in summers 1989–2010 using a Lagrangian dispersion model and statistical regression models.
Massimo Cassiani, Andreas Stohl, Dirk Olivié, Øyvind Seland, Ingo Bethke, Ignacio Pisso, and Trond Iversen
Geosci. Model Dev., 9, 4029–4048, https://doi.org/10.5194/gmd-9-4029-2016, https://doi.org/10.5194/gmd-9-4029-2016, 2016
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FLEXPART is a community model used by many scientists. Here, an alternative FLEXPART model version has been developed, tailored to use with the output data generated by the Norwegian Earth System Model (NorESM1-M). The model provides an advanced tool to analyse and diagnose atmospheric transport properties of the climate model NorESM. To validate the model, several tests were performed that offered the possibility to investigate some aspects of offline global dispersion modelling.
B. Quennehen, J.-C. Raut, K. S. Law, N. Daskalakis, G. Ancellet, C. Clerbaux, S.-W. Kim, M. T. Lund, G. Myhre, D. J. L. Olivié, S. Safieddine, R. B. Skeie, J. L. Thomas, S. Tsyro, A. Bazureau, N. Bellouin, M. Hu, M. Kanakidou, Z. Klimont, K. Kupiainen, S. Myriokefalitakis, J. Quaas, S. T. Rumbold, M. Schulz, R. Cherian, A. Shimizu, J. Wang, S.-C. Yoon, and T. Zhu
Atmos. Chem. Phys., 16, 10765–10792, https://doi.org/10.5194/acp-16-10765-2016, https://doi.org/10.5194/acp-16-10765-2016, 2016
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This paper evaluates the ability of six global models and one regional model in reproducing short-lived pollutants (defined here as ozone and its precursors, aerosols and black carbon) concentrations over Asia using satellite, ground-based and airborne observations.
Key findings are that models homogeneously reproduce the trace gas observations although nitrous oxides are underestimated, whereas the aerosol distributions are heterogeneously reproduced, implicating important uncertainties.
N. Evangeliou, Y. Balkanski, W. M. Hao, A. Petkov, R. P. Silverstein, R. Corley, B. L. Nordgren, S. P. Urbanski, S. Eckhardt, A. Stohl, P. Tunved, S. Crepinsek, A. Jefferson, S. Sharma, J. K. Nøjgaard, and H. Skov
Atmos. Chem. Phys., 16, 7587–7604, https://doi.org/10.5194/acp-16-7587-2016, https://doi.org/10.5194/acp-16-7587-2016, 2016
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In this study, we focused on how vegetation fires that occurred in northern Eurasia during the period 2002–2013 influenced the budget of BC in the Arctic. An average area of 250 000 km2 yr−1 was burned in northern Eurasia and the global emissions of BC ranged between 8.0 and 9.5 Tg yr−1, while 102 ± 29 kt yr−1 BC from biomass burning was deposited on the Arctic. About 46 % of the Arctic BC from vegetation fires originated from Siberia, 6 % from Kazakhstan, 5 % from Europe, and about 1 % from Mon
Pauli Paasonen, Kaarle Kupiainen, Zbigniew Klimont, Antoon Visschedijk, Hugo A. C. Denier van der Gon, and Markus Amann
Atmos. Chem. Phys., 16, 6823–6840, https://doi.org/10.5194/acp-16-6823-2016, https://doi.org/10.5194/acp-16-6823-2016, 2016
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In this paper we show the first results of size-segregated anthropogenic particle number emissions from the GAINS emission scenario model. The shares of different sources and their predicted changes from 2010 to 2030 are described, showing clear difference in sources dominating the particle number and mass emissions. We also point out the main uncertainties in number emissions. The GAINS particle number emissions can be applied in improving the evaluation of aerosol climate and health effects.
Wolfgang Knorr, Frank Dentener, Stijn Hantson, Leiwen Jiang, Zbigniew Klimont, and Almut Arneth
Atmos. Chem. Phys., 16, 5685–5703, https://doi.org/10.5194/acp-16-5685-2016, https://doi.org/10.5194/acp-16-5685-2016, 2016
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Wildfires are generally expected to increase in frequency and severity due to climate change. For Europe this could mean increased air pollution levels during the summer. Until 2050, predicted changes are moderate, but under a scenario of strong climate change, these may increase considerably during the later part of the current century. In Portugal and several parts of the Mediterranean, emissions may become relevant for meeting WHO concentration targets.
Quentin Coopman, Timothy J. Garrett, Jérôme Riedi, Sabine Eckhardt, and Andreas Stohl
Atmos. Chem. Phys., 16, 4661–4674, https://doi.org/10.5194/acp-16-4661-2016, https://doi.org/10.5194/acp-16-4661-2016, 2016
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We analyze interactions of Arctic clouds with pollution plumes that have been transported long distances from midlatitudes. Constraining for meteorological state, we find that pollution decreases cloud-droplet effective radius and increases cloud optical depth. The impact is highest when the atmosphere is particularly humid and/or stable suggesting that aerosol–cloud interactions depend on the Arctic's climate.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
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Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Xuekun Fang, Min Shao, Andreas Stohl, Qiang Zhang, Junyu Zheng, Hai Guo, Chen Wang, Ming Wang, Jiamin Ou, Rona L. Thompson, and Ronald G. Prinn
Atmos. Chem. Phys., 16, 3369–3382, https://doi.org/10.5194/acp-16-3369-2016, https://doi.org/10.5194/acp-16-3369-2016, 2016
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This is the first study reporting top-down estimates of benzene and toluene emissions in southern China using atmospheric measurement data from a rural site in the area, an atmospheric transport model and an inverse modeling method. This study shows in detail the temporal and spatial differences between the inversion estimate and four different bottom-up emission inventories (RCP, REAS, MEIC; Yin et al., 2015). We propose that more observations are urgently needed in future.
G. Janssens-Maenhout, M. Crippa, D. Guizzardi, F. Dentener, M. Muntean, G. Pouliot, T. Keating, Q. Zhang, J. Kurokawa, R. Wankmüller, H. Denier van der Gon, J. J. P. Kuenen, Z. Klimont, G. Frost, S. Darras, B. Koffi, and M. Li
Atmos. Chem. Phys., 15, 11411–11432, https://doi.org/10.5194/acp-15-11411-2015, https://doi.org/10.5194/acp-15-11411-2015, 2015
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This paper provides monthly emission grid maps at 0.1deg x 0.1deg resolution with global coverage for air pollutants and aerosols anthropogenic emissions in 2008 and 2010.
Countries are consistently inter-compared with sector-specific implied emission factors, per capita emissions and emissions per unit of GDP.
The emission grid maps compose the reference emissions data set for the community modelling hemispheric transport of air pollution (HTAP).
A. Stohl, B. Aamaas, M. Amann, L. H. Baker, N. Bellouin, T. K. Berntsen, O. Boucher, R. Cherian, W. Collins, N. Daskalakis, M. Dusinska, S. Eckhardt, J. S. Fuglestvedt, M. Harju, C. Heyes, Ø. Hodnebrog, J. Hao, U. Im, M. Kanakidou, Z. Klimont, K. Kupiainen, K. S. Law, M. T. Lund, R. Maas, C. R. MacIntosh, G. Myhre, S. Myriokefalitakis, D. Olivié, J. Quaas, B. Quennehen, J.-C. Raut, S. T. Rumbold, B. H. Samset, M. Schulz, Ø. Seland, K. P. Shine, R. B. Skeie, S. Wang, K. E. Yttri, and T. Zhu
Atmos. Chem. Phys., 15, 10529–10566, https://doi.org/10.5194/acp-15-10529-2015, https://doi.org/10.5194/acp-15-10529-2015, 2015
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This paper presents a summary of the findings of the ECLIPSE EU project. The project has investigated the climate and air quality impacts of short-lived climate pollutants (especially methane, ozone, aerosols) and has designed a global mitigation strategy that maximizes co-benefits between air quality and climate policy. Transient climate model simulations allowed quantifying the impacts on temperature (e.g., reduction in global warming by 0.22K for the decade 2041-2050) and precipitation.
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
S. Eckhardt, B. Quennehen, D. J. L. Olivié, T. K. Berntsen, R. Cherian, J. H. Christensen, W. Collins, S. Crepinsek, N. Daskalakis, M. Flanner, A. Herber, C. Heyes, Ø. Hodnebrog, L. Huang, M. Kanakidou, Z. Klimont, J. Langner, K. S. Law, M. T. Lund, R. Mahmood, A. Massling, S. Myriokefalitakis, I. E. Nielsen, J. K. Nøjgaard, J. Quaas, P. K. Quinn, J.-C. Raut, S. T. Rumbold, M. Schulz, S. Sharma, R. B. Skeie, H. Skov, T. Uttal, K. von Salzen, and A. Stohl
Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, https://doi.org/10.5194/acp-15-9413-2015, 2015
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The concentrations of sulfate, black carbon and other aerosols in the Arctic are characterized by high values in late winter and spring (so-called Arctic Haze) and low values in summer. Models have long been struggling to capture this seasonality. In this study, we evaluate sulfate and BC concentrations from different updated models and emissions against a comprehensive pan-Arctic measurement data set. We find that the models improved but still struggle to get the maximum concentrations.
L. J. Kramer, D. Helmig, J. F. Burkhart, A. Stohl, S. Oltmans, and R. E. Honrath
Atmos. Chem. Phys., 15, 6827–6849, https://doi.org/10.5194/acp-15-6827-2015, https://doi.org/10.5194/acp-15-6827-2015, 2015
J.-P. Pietikäinen, K. Kupiainen, Z. Klimont, R. Makkonen, H. Korhonen, R. Karinkanta, A.-P. Hyvärinen, N. Karvosenoja, A. Laaksonen, H. Lihavainen, and V.-M. Kerminen
Atmos. Chem. Phys., 15, 5501–5519, https://doi.org/10.5194/acp-15-5501-2015, https://doi.org/10.5194/acp-15-5501-2015, 2015
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The global aerosol--climate model ECHAM-HAMMOZ is used to study the aerosol burden and forcing changes in the coming decades. We show that aerosol burdens overall can have a decreasing trend leading to reductions in the direct aerosol effect being globally 0.06--0.4W/m2 by 2030, whereas the aerosol indirect radiative effect could decline 0.25--0.82W/m2. We also show that the targeted emission reduction measures can be a much better choice for the climate than overall high reductions globally.
H. S. Gadhavi, K. Renuka, V. Ravi Kiran, A. Jayaraman, A. Stohl, Z. Klimont, and G. Beig
Atmos. Chem. Phys., 15, 1447–1461, https://doi.org/10.5194/acp-15-1447-2015, https://doi.org/10.5194/acp-15-1447-2015, 2015
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Emission inventories are a key component of simulating past, present and future climate. In this article we have evaluated three black carbon emission inventories for emissions of India using observations made from a strategic location. Annual average simulated black carbon concentration is found to be 35% to 60% lower than observed concentration because of underestimation of emissions of southern India in the inventories.
M. Martinez-Camara, B. Béjar Haro, A. Stohl, and M. Vetterli
Geosci. Model Dev., 7, 2303–2311, https://doi.org/10.5194/gmd-7-2303-2014, https://doi.org/10.5194/gmd-7-2303-2014, 2014
S. V. Henriksson, J.-P. Pietikäinen, A.-P. Hyvärinen, P. Räisänen, K. Kupiainen, J. Tonttila, R. Hooda, H. Lihavainen, D. O'Donnell, L. Backman, Z. Klimont, and A. Laaksonen
Atmos. Chem. Phys., 14, 10177–10192, https://doi.org/10.5194/acp-14-10177-2014, https://doi.org/10.5194/acp-14-10177-2014, 2014
S. Safieddine, A. Boynard, P.-F. Coheur, D. Hurtmans, G. Pfister, B. Quennehen, J. L. Thomas, J.-C. Raut, K. S. Law, Z. Klimont, J. Hadji-Lazaro, M. George, and C. Clerbaux
Atmos. Chem. Phys., 14, 10119–10131, https://doi.org/10.5194/acp-14-10119-2014, https://doi.org/10.5194/acp-14-10119-2014, 2014
T. Trickl, H. Vogelmann, H. Giehl, H.-E. Scheel, M. Sprenger, and A. Stohl
Atmos. Chem. Phys., 14, 9941–9961, https://doi.org/10.5194/acp-14-9941-2014, https://doi.org/10.5194/acp-14-9941-2014, 2014
M. Maione, F. Graziosi, J. Arduini, F. Furlani, U. Giostra, D. R. Blake, P. Bonasoni, X. Fang, S. A. Montzka, S. J. O'Doherty, S. Reimann, A. Stohl, and M. K. Vollmer
Atmos. Chem. Phys., 14, 9755–9770, https://doi.org/10.5194/acp-14-9755-2014, https://doi.org/10.5194/acp-14-9755-2014, 2014
S. Chatani, M. Amann, A. Goel, J. Hao, Z. Klimont, A. Kumar, A. Mishra, S. Sharma, S. X. Wang, Y. X. Wang, and B. Zhao
Atmos. Chem. Phys., 14, 9259–9277, https://doi.org/10.5194/acp-14-9259-2014, https://doi.org/10.5194/acp-14-9259-2014, 2014
W. C. Keene, J. L. Moody, J. N. Galloway, J. M. Prospero, O. R. Cooper, S. Eckhardt, and J. R. Maben
Atmos. Chem. Phys., 14, 8119–8135, https://doi.org/10.5194/acp-14-8119-2014, https://doi.org/10.5194/acp-14-8119-2014, 2014
K. Markakis, M. Valari, A. Colette, O. Sanchez, O. Perrussel, C. Honore, R. Vautard, Z. Klimont, and S. Rao
Atmos. Chem. Phys., 14, 7323–7340, https://doi.org/10.5194/acp-14-7323-2014, https://doi.org/10.5194/acp-14-7323-2014, 2014
S. X. Wang, B. Zhao, S. Y. Cai, Z. Klimont, C. P. Nielsen, T. Morikawa, J. H. Woo, Y. Kim, X. Fu, J. Y. Xu, J. M. Hao, and K. B. He
Atmos. Chem. Phys., 14, 6571–6603, https://doi.org/10.5194/acp-14-6571-2014, https://doi.org/10.5194/acp-14-6571-2014, 2014
K. E. Yttri, C. Lund Myhre, S. Eckhardt, M. Fiebig, C. Dye, D. Hirdman, J. Ström, Z. Klimont, and A. Stohl
Atmos. Chem. Phys., 14, 6427–6442, https://doi.org/10.5194/acp-14-6427-2014, https://doi.org/10.5194/acp-14-6427-2014, 2014
H. Grythe, J. Ström, R. Krejci, P. Quinn, and A. Stohl
Atmos. Chem. Phys., 14, 1277–1297, https://doi.org/10.5194/acp-14-1277-2014, https://doi.org/10.5194/acp-14-1277-2014, 2014
J. L. Moody, W. C. Keene, O. R. Cooper, K. J. Voss, R. Aryal, S. Eckhardt, B. Holben, J. R. Maben, M. A. Izaguirre, and J. N. Galloway
Atmos. Chem. Phys., 14, 691–717, https://doi.org/10.5194/acp-14-691-2014, https://doi.org/10.5194/acp-14-691-2014, 2014
J. Brioude, D. Arnold, A. Stohl, M. Cassiani, D. Morton, P. Seibert, W. Angevine, S. Evan, A. Dingwell, J. D. Fast, R. C. Easter, I. Pisso, J. Burkhart, and G. Wotawa
Geosci. Model Dev., 6, 1889–1904, https://doi.org/10.5194/gmd-6-1889-2013, https://doi.org/10.5194/gmd-6-1889-2013, 2013
M. Cassiani, A. Stohl, and S. Eckhardt
Atmos. Chem. Phys., 13, 9975–9996, https://doi.org/10.5194/acp-13-9975-2013, https://doi.org/10.5194/acp-13-9975-2013, 2013
B. Zhao, S. X. Wang, H. Liu, J. Y. Xu, K. Fu, Z. Klimont, J. M. Hao, K. B. He, J. Cofala, and M. Amann
Atmos. Chem. Phys., 13, 9869–9897, https://doi.org/10.5194/acp-13-9869-2013, https://doi.org/10.5194/acp-13-9869-2013, 2013
S. Eckhardt, O. Hermansen, H. Grythe, M. Fiebig, K. Stebel, M. Cassiani, A. Baecklund, and A. Stohl
Atmos. Chem. Phys., 13, 8401–8409, https://doi.org/10.5194/acp-13-8401-2013, https://doi.org/10.5194/acp-13-8401-2013, 2013
A. Colette, B. Bessagnet, R. Vautard, S. Szopa, S. Rao, S. Schucht, Z. Klimont, L. Menut, G. Clain, F. Meleux, G. Curci, and L. Rouïl
Atmos. Chem. Phys., 13, 7451–7471, https://doi.org/10.5194/acp-13-7451-2013, https://doi.org/10.5194/acp-13-7451-2013, 2013
R. Kallenborn, K. Breivik, S. Eckhardt, C. R. Lunder, S. Manø, M. Schlabach, and A. Stohl
Atmos. Chem. Phys., 13, 6983–6992, https://doi.org/10.5194/acp-13-6983-2013, https://doi.org/10.5194/acp-13-6983-2013, 2013
M. Laborde, M. Crippa, T. Tritscher, Z. Jurányi, P. F. Decarlo, B. Temime-Roussel, N. Marchand, S. Eckhardt, A. Stohl, U. Baltensperger, A. S. H. Prévôt, E. Weingartner, and M. Gysel
Atmos. Chem. Phys., 13, 5831–5856, https://doi.org/10.5194/acp-13-5831-2013, https://doi.org/10.5194/acp-13-5831-2013, 2013
A. Kylling, R. Buras, S. Eckhardt, C. Emde, B. Mayer, and A. Stohl
Atmos. Meas. Tech., 6, 649–660, https://doi.org/10.5194/amt-6-649-2013, https://doi.org/10.5194/amt-6-649-2013, 2013
F. Freutel, J. Schneider, F. Drewnick, S.-L. von der Weiden-Reinmüller, M. Crippa, A. S. H. Prévôt, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, R. Sarda-Estève, J. F. Burkhart, S. Eckhardt, A. Stohl, V. Gros, A. Colomb, V. Michoud, J. F. Doussin, A. Borbon, M. Haeffelin, Y. Morille, M. Beekmann, and S. Borrmann
Atmos. Chem. Phys., 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, https://doi.org/10.5194/acp-13-933-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
Multi-model effective radiative forcing of the 2020 sulfur cap for shipping
Representation of iron aerosol size distributions of anthropogenic emissions is critical in evaluating atmospheric soluble iron input to the ocean
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
Impact of biomass burning aerosols (BBA) on the tropical African climate in an ocean–atmosphere–aerosol coupled climate model
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm
Dust aerosol from the Aralkum Desert influences the radiation budget and atmospheric dynamics of Central Asia
Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Synergistic effects of the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) on dust activities in North China during the following spring
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
Steady-State Mixing State of Black Carbon Aerosols from a Particle-Resolved Model
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Distinctive dust weather intensities in North China resulted from two types of atmospheric circulation anomalies
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Modeling impacts of dust mineralogy on fast climate response
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK climate model
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Solar radiation estimation in West Africa: impact of dust conditions during 2021 dry season
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Biomass Burning Emissions Analysis Based on MODIS AOD and AeroCom Multi-Model Simulations
Global aviation contrail climate effects from 2019 to 2021
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Warming effects of reduced sulfur emissions from shipping
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer campaigns of ACTIVATE 2020: Life cycle, transport, and distribution
Simulated phase state and viscosity of secondary organic aerosols over China
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
A global dust emission dataset for estimating dust radiative forcings in climate models
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
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Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
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In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
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Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
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In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
EGUsphere, https://doi.org/10.5194/egusphere-2024-1924, https://doi.org/10.5194/egusphere-2024-1924, 2024
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Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with characteristic time of less than one day. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1923, https://doi.org/10.5194/egusphere-2024-1923, 2024
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The Mongolian cyclone, compared to the cold high-pressure system, caused more frequent and severe dust weather in North China during the spring seasons of 2015–2023. Different intensities of 500 hPa cyclonic and anticyclonic anomalies, control near-surface meteorological conditions, leading to two dust weather types in North China. The common predictor for the two types of dust weather successfully captured 76.1 % of dust days and provided a dust signal two days in advance.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Ryan Schmedding and Andreas Zuend
EGUsphere, https://doi.org/10.5194/egusphere-2024-1690, https://doi.org/10.5194/egusphere-2024-1690, 2024
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-1538, https://doi.org/10.5194/egusphere-2024-1538, 2024
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosol that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK's Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust we also need to represent ice nucleation by the organic components of soils.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
EGUsphere, https://doi.org/10.5194/egusphere-2024-1604, https://doi.org/10.5194/egusphere-2024-1604, 2024
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Solar energy production in West Africa is set to rise, needing accurate solar radiation estimates, which is affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cut errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
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We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1487, https://doi.org/10.5194/egusphere-2024-1487, 2024
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke-amount observations, aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss-rate assumptions vary enormously among models, causing uncertainties that require systematic in-situ measurements to resolve.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
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The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
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The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
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Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-1428, https://doi.org/10.5194/egusphere-2024-1428, 2024
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Sulfur emissions from shipping has been reduced by about 80 % as a result of the new regulation introduced in 2020. This has reduced aerosol in the atmosphere and its cooling effect through interactions with clouds. As a result, our coupled climate model simulations predict a global warming of 0.04 K averaged over three decades, potentially surpassing the Paris target of 1.5 K or contributing to recent temperature spikes, particularly notable in the Arctic with a mean warming of 0.15 K.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
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Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
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A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Jason L. Tackett, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1127, https://doi.org/10.5194/egusphere-2024-1127, 2024
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We use the GEOS-Chem model to simulate aerosols over the western North Atlantic Ocean (WNAO) during the winter and summer campaigns of ACTIVATE 2020. Model results are evaluated against in situ and remote sensing measurements from two aircraft as well as ground-based and satellite observations. The improved understanding of the aerosol life cycle, composition, transport pathways, and distribution has important implications for characterizing aerosol-cloud-meteorology interactions over the WNAO.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
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Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
EGUsphere, https://doi.org/10.5194/egusphere-2024-1124, https://doi.org/10.5194/egusphere-2024-1124, 2024
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This study derives a desert dust emission dataset for 1841–2000, by employing a combination of observed dust records from sedimentary cores as well as reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to match better against observations than other mechanistic models.
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
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The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
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During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
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Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
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Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
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Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
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