Articles | Volume 13, issue 14
https://doi.org/10.5194/acp-13-6687-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-6687-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
15 Jul 2013
Research article |
| 15 Jul 2013
Performance of the Line-By-Line Radiative Transfer Model (LBLRTM) for temperature, water vapor, and trace gas retrievals: recent updates evaluated with IASI case studies
M. J. Alvarado
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
V. H. Payne
Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California, USA
E. J. Mlawer
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
G. Uymin
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
M. W. Shephard
Environment Canada, Toronto, Ontario, Canada
K. E. Cady-Pereira
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
J. S. Delamere
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
now at: Tech-X, Boulder, Colorado, USA
J.-L. Moncet
Atmospheric and Environmental Research, Lexington, Massachusetts, USA
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Nicole A. June, Anna L. Hodshire, Elizabeth B. Wiggins, Edward L. Winstead, Claire E. Robinson, K. Lee Thornhill, Kevin J. Sanchez, Richard H. Moore, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Matthew M. Coggon, Jonathan M. Dean-Day, T. Paul Bui, Jeff Peischl, Robert J. Yokelson, Matthew J. Alvarado, Sonia M. Kreidenweis, Shantanu H. Jathar, and Jeffrey R. Pierce
Atmos. Chem. Phys., 22, 12803–12825, https://doi.org/10.5194/acp-22-12803-2022, https://doi.org/10.5194/acp-22-12803-2022, 2022
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The evolution of organic aerosol composition and size is uncertain due to variability within and between smoke plumes. We examine the impact of plume concentration on smoke evolution from smoke plumes sampled by the NASA DC-8 during FIREX-AQ. We find that observed organic aerosol and size distribution changes are correlated to plume aerosol mass concentrations. Additionally, coagulation explains the majority of the observed growth.
Helen M. Worden, Gene L. Francis, Susan S. Kulawik, Kevin W. Bowman, Karen Cady-Pereira, Dejian Fu, Jennifer D. Hegarty, Valentin Kantchev, Ming Luo, Vivienne H. Payne, John R. Worden, Róisín Commane, and Kathryn McKain
Atmos. Meas. Tech., 15, 5383–5398, https://doi.org/10.5194/amt-15-5383-2022, https://doi.org/10.5194/amt-15-5383-2022, 2022
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Vivienne H. Payne, Susan S. Kulawik, Emily V. Fischer, Jared F. Brewer, L. Gregory Huey, Kazuyuki Miyazaki, John R. Worden, Kevin W. Bowman, Eric J. Hintsa, Fred Moore, James W. Elkins, and Julieta Juncosa Calahorrano
Atmos. Meas. Tech., 15, 3497–3511, https://doi.org/10.5194/amt-15-3497-2022, https://doi.org/10.5194/amt-15-3497-2022, 2022
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Michael Sitwell, Mark W. Shephard, Yves Rochon, Karen Cady-Pereira, and Enrico Dammers
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Observations of ammonia made using the satellite-borne CrIS instrument were used to improve the ammonia emissions used in the GEM-MACH model. These observations were used to refine estimates of the monthly mean ammonia emissions over North America for May to August 2016. The updated ammonia emissions reduced biases of GEM-MACH surface ammonia fields with surface observations and showed some improvements in the forecasting of species involved in inorganic particulate matter formation.
Vijay Natraj, Ming Luo, Jean-Francois Blavier, Vivienne H. Payne, Derek J. Posselt, Stanley P. Sander, Zhao-Cheng Zeng, Jessica L. Neu, Denis Tremblay, Longtao Wu, Jacola A. Roman, Yen-Hung Wu, and Leonard I. Dorsky
Atmos. Meas. Tech., 15, 1251–1267, https://doi.org/10.5194/amt-15-1251-2022, https://doi.org/10.5194/amt-15-1251-2022, 2022
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Shelley van der Graaf, Enrico Dammers, Arjo Segers, Richard Kranenburg, Martijn Schaap, Mark W. Shephard, and Jan Willem Erisman
Atmos. Chem. Phys., 22, 951–972, https://doi.org/10.5194/acp-22-951-2022, https://doi.org/10.5194/acp-22-951-2022, 2022
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Jennifer D. Hegarty, Karen E. Cady-Pereira, Vivienne H. Payne, Susan S. Kulawik, John R. Worden, Valentin Kantchev, Helen M. Worden, Kathryn McKain, Jasna V. Pittman, Róisín Commane, Bruce C. Daube Jr., and Eric A. Kort
Atmos. Meas. Tech., 15, 205–223, https://doi.org/10.5194/amt-15-205-2022, https://doi.org/10.5194/amt-15-205-2022, 2022
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Anna L. Hodshire, Emily Ramnarine, Ali Akherati, Matthew L. Alvarado, Delphine K. Farmer, Shantanu H. Jathar, Sonia M. Kreidenweis, Chantelle R. Lonsdale, Timothy B. Onasch, Stephen R. Springston, Jian Wang, Yang Wang, Lawrence I. Kleinman, Arthur J. Sedlacek III, and Jeffrey R. Pierce
Atmos. Chem. Phys., 21, 6839–6855, https://doi.org/10.5194/acp-21-6839-2021, https://doi.org/10.5194/acp-21-6839-2021, 2021
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Nikolaos Evangeliou, Yves Balkanski, Sabine Eckhardt, Anne Cozic, Martin Van Damme, Pierre-François Coheur, Lieven Clarisse, Mark W. Shephard, Karen E. Cady-Pereira, and Didier Hauglustaine
Atmos. Chem. Phys., 21, 4431–4451, https://doi.org/10.5194/acp-21-4431-2021, https://doi.org/10.5194/acp-21-4431-2021, 2021
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Ammonia, a substance that has played a key role in sustaining life, has been increasing in the atmosphere, affecting climate and humans. Understanding the reasons for this increase is important for the beneficial use of ammonia. The evolution of satellite products gives us the opportunity to calculate ammonia emissions easier. We calculated global ammonia emissions over the last 10 years, incorporated them into a chemistry model and recorded notable improvement in reproducing observations.
Susan S. Kulawik, John R. Worden, Vivienne H. Payne, Dejian Fu, Steven C. Wofsy, Kathryn McKain, Colm Sweeney, Bruce C. Daube Jr., Alan Lipton, Igor Polonsky, Yuguang He, Karen E. Cady-Pereira, Edward J. Dlugokencky, Daniel J. Jacob, and Yi Yin
Atmos. Meas. Tech., 14, 335–354, https://doi.org/10.5194/amt-14-335-2021, https://doi.org/10.5194/amt-14-335-2021, 2021
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This paper shows comparisons of a new single-footprint methane product from the AIRS satellite to aircraft-based observations. We show that this AIRS methane product provides useful information to study seasonal and global methane trends of this important greenhouse gas.
Chantelle R. Lonsdale, Matthew J. Alvarado, Anna L. Hodshire, Emily Ramnarine, and Jeffrey R. Pierce
Geosci. Model Dev., 13, 4579–4593, https://doi.org/10.5194/gmd-13-4579-2020, https://doi.org/10.5194/gmd-13-4579-2020, 2020
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The System for Atmospheric Modelling (SAM) has been coupled with the detailed gas/aerosol chemistry model, the Aerosol Simulation Program (ASP), to capture cross-plume concentration gradients as fire plumes evolve downwind. SAM-ASP v1.0 will lead to the development of parameterizations of near-source biomass burning chemistry that can be used to more accurately simulate biomass burning chemical and physical transformations of trace gases and aerosols within coarser chemical transport models.
Kazuyuki Miyazaki, Kevin Bowman, Takashi Sekiya, Henk Eskes, Folkert Boersma, Helen Worden, Nathaniel Livesey, Vivienne H. Payne, Kengo Sudo, Yugo Kanaya, Masayuki Takigawa, and Koji Ogochi
Earth Syst. Sci. Data, 12, 2223–2259, https://doi.org/10.5194/essd-12-2223-2020, https://doi.org/10.5194/essd-12-2223-2020, 2020
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This study presents the results from the Tropospheric Chemistry Reanalysis version 2 (TCR-2) for 2005–2018 obtained from the assimilation of multiple satellite measurements of ozone, CO, NO2, HNO3, and SO2 from the OMI, SCIAMACHY, GOME-2, TES, MLS, and MOPITT instruments. The evaluation results demonstrate the capability of the reanalysis products to improve understanding of the processes controlling variations in atmospheric composition, including long-term changes in air quality and emissions.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
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Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Robert L. Herman, John Worden, David Noone, Dean Henze, Kevin Bowman, Karen Cady-Pereira, Vivienne H. Payne, Susan S. Kulawik, and Dejian Fu
Atmos. Meas. Tech., 13, 1825–1834, https://doi.org/10.5194/amt-13-1825-2020, https://doi.org/10.5194/amt-13-1825-2020, 2020
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This study is the first assessment and validation of AIRS HDO / H2O retrieved by optimal estimation. Initial comparisons with in situ measurements from NASA ORACLES are promising: the small bias and consistent rms of AIRS suggest that AIRS has well-characterized HDO / H2O. This analysis opens the possibility of a new 17-year long-term data record of global tropospheric HDO / H2O measured from space.
Mark W. Shephard, Enrico Dammers, Karen E. Cady-Pereira, Shailesh K. Kharol, Jesse Thompson, Yonatan Gainariu-Matz, Junhua Zhang, Chris A. McLinden, Andrew Kovachik, Michael Moran, Shabtai Bittman, Christopher E. Sioris, Debora Griffin, Matthew J. Alvarado, Chantelle Lonsdale, Verica Savic-Jovcic, and Qiong Zheng
Atmos. Chem. Phys., 20, 2277–2302, https://doi.org/10.5194/acp-20-2277-2020, https://doi.org/10.5194/acp-20-2277-2020, 2020
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Presented is a description and survey demonstrating the capabilities of the CrIS ammonia product for monitoring, air quality forecast model evaluation, dry deposition estimates, and emission estimates of an agricultural hotspot.
Camille Viatte, Tianze Wang, Martin Van Damme, Enrico Dammers, Frederik Meleux, Lieven Clarisse, Mark W. Shephard, Simon Whitburn, Pierre François Coheur, Karen E. Cady-Pereira, and Cathy Clerbaux
Atmos. Chem. Phys., 20, 577–596, https://doi.org/10.5194/acp-20-577-2020, https://doi.org/10.5194/acp-20-577-2020, 2020
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We study concentrations and spatiotemporal variabilities of atmospheric NH3 from the agricultural sector to gain insights on its effects on the Paris megacity air quality using satellite data from IASI and CrIS.
We evaluate the regional CHIMERE model capacity to reproduce NH3 and particulate matter (PM2.5) concentrations and variabilities in the domain of study.
We quantify the main meteorological parameters driving the optimal conditions involved in the PM2.5 formation from NH3 in Paris.
Enrico Dammers, Chris A. McLinden, Debora Griffin, Mark W. Shephard, Shelley Van Der Graaf, Erik Lutsch, Martijn Schaap, Yonatan Gainairu-Matz, Vitali Fioletov, Martin Van Damme, Simon Whitburn, Lieven Clarisse, Karen Cady-Pereira, Cathy Clerbaux, Pierre Francois Coheur, and Jan Willem Erisman
Atmos. Chem. Phys., 19, 12261–12293, https://doi.org/10.5194/acp-19-12261-2019, https://doi.org/10.5194/acp-19-12261-2019, 2019
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Ammonia is an essential molecule in the environment, but at its current levels it is unsustainable. However, the emissions are highly uncertain. We explore the use of satellites to estimate the ammonia lifetime and emissions around point sources to help improve the budget. The same method applied to different satellite instruments shows consistent results. Comparison to the emission inventories shows that those are underestimating emissions of point sources by on average a factor of 2.5.
Emily Ramnarine, John K. Kodros, Anna L. Hodshire, Chantelle R. Lonsdale, Matthew J. Alvarado, and Jeffrey R. Pierce
Atmos. Chem. Phys., 19, 6561–6577, https://doi.org/10.5194/acp-19-6561-2019, https://doi.org/10.5194/acp-19-6561-2019, 2019
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Biomass burning aerosols have important global radiative effects that depend on particle size. However, model estimates of these effects do not explicitly account for the coagulation of particles in biomass burning plumes. In this work, we present the first use of a sub-grid coagulation scheme in a global aerosol model to account for in-plume coagulation. We find that this in-plume coagulation leads to important changes in the biomass burning aerosol radiative effects.
John R. Worden, Susan S. Kulawik, Dejian Fu, Vivienne H. Payne, Alan E. Lipton, Igor Polonsky, Yuguang He, Karen Cady-Pereira, Jean-Luc Moncet, Robert L. Herman, Fredrick W. Irion, and Kevin W. Bowman
Atmos. Meas. Tech., 12, 2331–2339, https://doi.org/10.5194/amt-12-2331-2019, https://doi.org/10.5194/amt-12-2331-2019, 2019
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In this paper we take the first steps towards generating a multi-decadal record of the deuterium content of water vapor, useful for evaluating the moisture sources and processes affecting water vapor, by estimating the deuterium content from thermal IR radiances from the AIRS instrument. We find the AIRS-based measurements are sensitive to the deuterium content of water vapor in the middle and lower troposphere with a single measurement uncertainty of ~ 3 % and an accuracy of ~ 0.7 %.
Cristen Adams, Chris A. McLinden, Mark W. Shephard, Nolan Dickson, Enrico Dammers, Jack Chen, Paul Makar, Karen E. Cady-Pereira, Naomi Tam, Shailesh K. Kharol, Lok N. Lamsal, and Nickolay A. Krotkov
Atmos. Chem. Phys., 19, 2577–2599, https://doi.org/10.5194/acp-19-2577-2019, https://doi.org/10.5194/acp-19-2577-2019, 2019
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We estimated how much carbon monoxide, ammonia, and nitrogen oxides were emitted in the smoke from the Fort McMurray Horse River wildfire using satellite data and air quality models. The fire emitted amounts of carbon monoxide that were similar to anthropogenic (human-caused) emissions for all of Alberta over a full year. We also estimated large amounts of ammonia and nitrogen oxides emitted from the fire. These results can be used to evaluate the performance of air quality forecasting models.
Kang Sun, Lei Zhu, Karen Cady-Pereira, Christopher Chan Miller, Kelly Chance, Lieven Clarisse, Pierre-François Coheur, Gonzalo González Abad, Guanyu Huang, Xiong Liu, Martin Van Damme, Kai Yang, and Mark Zondlo
Atmos. Meas. Tech., 11, 6679–6701, https://doi.org/10.5194/amt-11-6679-2018, https://doi.org/10.5194/amt-11-6679-2018, 2018
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An agile, physics-based approach is developed to oversample irregular satellite observations to a high-resolution common grid. Instead of assuming each sounding as a point or a polygon as in previous methods, the proposed physical oversampling represents soundings as distributions of sensitivity on the ground. This sensitivity distribution can be determined by the spatial response function of each satellite sensor, parameterized as generalized 2-D super Gaussian functions.
Christopher W. O'Dell, Annmarie Eldering, Paul O. Wennberg, David Crisp, Michael R. Gunson, Brendan Fisher, Christian Frankenberg, Matthäus Kiel, Hannakaisa Lindqvist, Lukas Mandrake, Aronne Merrelli, Vijay Natraj, Robert R. Nelson, Gregory B. Osterman, Vivienne H. Payne, Thomas E. Taylor, Debra Wunch, Brian J. Drouin, Fabiano Oyafuso, Albert Chang, James McDuffie, Michael Smyth, David F. Baker, Sourish Basu, Frédéric Chevallier, Sean M. R. Crowell, Liang Feng, Paul I. Palmer, Mavendra Dubey, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, Coleen M. Roehl, Mahesh K. Sha, Kimberly Strong, Ralf Sussmann, Yao Te, Osamu Uchino, and Voltaire A. Velazco
Atmos. Meas. Tech., 11, 6539–6576, https://doi.org/10.5194/amt-11-6539-2018, https://doi.org/10.5194/amt-11-6539-2018, 2018
Emily V. Fischer, Liye Zhu, Vivienne H. Payne, John R. Worden, Zhe Jiang, Susan S. Kulawik, Steven Brey, Arsineh Hecobian, Daniel Gombos, Karen Cady-Pereira, and Frank Flocke
Atmos. Chem. Phys., 18, 5639–5653, https://doi.org/10.5194/acp-18-5639-2018, https://doi.org/10.5194/acp-18-5639-2018, 2018
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PAN is an atmospheric reservoir for nitrogen oxide radicals, and it plays a lead role in their redistribution in the troposphere. We analyze new Tropospheric Emission Spectrometer (TES) PAN observations over North America during July 2006 to 2009. We identify smoke-impacted TES PAN retrievals by co-location with NOAA Hazard Mapping System (HMS) smoke plumes. Depending on the year, 15–32 % of cases where elevated PAN is identified in TES observations overlap with smoke plumes.
Jingqiu Mao, Annmarie Carlton, Ronald C. Cohen, William H. Brune, Steven S. Brown, Glenn M. Wolfe, Jose L. Jimenez, Havala O. T. Pye, Nga Lee Ng, Lu Xu, V. Faye McNeill, Kostas Tsigaridis, Brian C. McDonald, Carsten Warneke, Alex Guenther, Matthew J. Alvarado, Joost de Gouw, Loretta J. Mickley, Eric M. Leibensperger, Rohit Mathur, Christopher G. Nolte, Robert W. Portmann, Nadine Unger, Mika Tosca, and Larry W. Horowitz
Atmos. Chem. Phys., 18, 2615–2651, https://doi.org/10.5194/acp-18-2615-2018, https://doi.org/10.5194/acp-18-2615-2018, 2018
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This paper is aimed at discussing progress in evaluating, diagnosing, and improving air quality and climate modeling using comparisons to SAS observations as a guide to thinking about improvements to mechanisms and parameterizations in models.
Cynthia H. Whaley, Paul A. Makar, Mark W. Shephard, Leiming Zhang, Junhua Zhang, Qiong Zheng, Ayodeji Akingunola, Gregory R. Wentworth, Jennifer G. Murphy, Shailesh K. Kharol, and Karen E. Cady-Pereira
Atmos. Chem. Phys., 18, 2011–2034, https://doi.org/10.5194/acp-18-2011-2018, https://doi.org/10.5194/acp-18-2011-2018, 2018
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Using a modified air quality forecasting model, we have found that a significant fraction (> 50 %) of ambient ammonia comes from re-emission from plants and soils in the broader Athabasca Oil Sands region and much of Alberta and Saskatchewan. We also found that about 20 % of ambient ammonia in Alberta and Saskatchewan came from forest fires in the summer of 2013. The addition of these two processes improved modelled ammonia, which was a motivating factor in undertaking this research.
Karen E. Cady-Pereira, Vivienne H. Payne, Jessica L. Neu, Kevin W. Bowman, Kazuyuki Miyazaki, Eloise A. Marais, Susan Kulawik, Zitely A. Tzompa-Sosa, and Jennifer D. Hegarty
Atmos. Chem. Phys., 17, 9379–9398, https://doi.org/10.5194/acp-17-9379-2017, https://doi.org/10.5194/acp-17-9379-2017, 2017
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Air quality is a major issue for megacities. Our paper looks at satellite measurements over Mexico City and Lagos of several trace gases gases related to air quality to determine the temporal and spatial variability of these gases, and it relates this variability to local conditions, such as topography, winds and biomass burning events. We find that, while Mexico City is known for severe pollution events, the levels of of pollution in Lagos are much higher and more persistent.
Enrico Dammers, Mark W. Shephard, Mathias Palm, Karen Cady-Pereira, Shannon Capps, Erik Lutsch, Kim Strong, James W. Hannigan, Ivan Ortega, Geoffrey C. Toon, Wolfgang Stremme, Michel Grutter, Nicholas Jones, Dan Smale, Jacob Siemons, Kevin Hrpcek, Denis Tremblay, Martijn Schaap, Justus Notholt, and Jan Willem Erisman
Atmos. Meas. Tech., 10, 2645–2667, https://doi.org/10.5194/amt-10-2645-2017, https://doi.org/10.5194/amt-10-2645-2017, 2017
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Presented here is the validation of the CrIS fast physical retrieval (CFPR) NH3 column and profile measurements using ground-based Fourier transform infrared (FTIR) observations. The overall FTIR and CrIS total columns have a positive correlation of r = 0.77 (N = 218) with very little bias (a slope of 1.02). Furthermore, we find that CrIS and FTIR profile comparison differences are mostly within the range of the estimated retrieval uncertainties, with differences in the range of ~ 20 to 40 %.
Zhe Jiang, Helen Worden, John R. Worden, Daven K. Henze, Dylan B. A. Jones, Avelino F. Arellano, Emily V. Fischer, Liye Zhu, Kazuyuki Miyazaki, K. Folkert Boersma, and Vivienne H. Payne
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-382, https://doi.org/10.5194/acp-2017-382, 2017
Preprint withdrawn
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We investigated the variation of US tropospheric NO2 in the past decade. We demonstrated significant divergence between the time variation in tropospheric NO2 columns from OMI retrievals and surface measurements. Our analysis suggests limited contributions from local effects such as fossil fuel emissions, lightning, or instrument artifacts, and indicates possible important contributions from long-range transport of Asian emissions that are modulated by ENSO.
Vivienne H. Payne, Emily V. Fischer, John R. Worden, Zhe Jiang, Liye Zhu, Thomas P. Kurosu, and Susan S. Kulawik
Atmos. Chem. Phys., 17, 6341–6351, https://doi.org/10.5194/acp-17-6341-2017, https://doi.org/10.5194/acp-17-6341-2017, 2017
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Peroxyacetyl nitrate (PAN) plays a key role in atmospheric chemistry and long-range transport of pollution. In this paper, we present measurements of PAN from the Tropospheric Emission Spectrometer, an instrument on board the NASA Aura satellite since 2004. We focus on measurements of PAN in tropical regions, where data from ground-based and aircraft campaigns are particularly sparse. We observe temporal changes in PAN associated with changes in fires, convection and emissions.
Shailesh K. Kharol, Chris A. McLinden, Christopher E. Sioris, Mark W. Shephard, Vitali Fioletov, Aaron van Donkelaar, Sajeev Philip, and Randall V. Martin
Atmos. Chem. Phys., 17, 5921–5929, https://doi.org/10.5194/acp-17-5921-2017, https://doi.org/10.5194/acp-17-5921-2017, 2017
Min Huang, Gregory R. Carmichael, R. Bradley Pierce, Duseong S. Jo, Rokjin J. Park, Johannes Flemming, Louisa K. Emmons, Kevin W. Bowman, Daven K. Henze, Yanko Davila, Kengo Sudo, Jan Eiof Jonson, Marianne Tronstad Lund, Greet Janssens-Maenhout, Frank J. Dentener, Terry J. Keating, Hilke Oetjen, and Vivienne H. Payne
Atmos. Chem. Phys., 17, 5721–5750, https://doi.org/10.5194/acp-17-5721-2017, https://doi.org/10.5194/acp-17-5721-2017, 2017
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In support of the HTAP phase 2 experiment, we conducted a number of regional-scale Sulfur Transport and dEposition Model base and sensitivity simulations over North America during May–June 2010. The STEM chemical boundary conditions were downscaled from three (GEOS-Chem, RAQMS, and ECMWF C-IFS) global chemical transport models' simulations. Analyses were performed on large spatial–temporal scales relative to HTAP1 and also on subcontinental and event scales including the use of satellite data.
Susan S. Kulawik, Chris O'Dell, Vivienne H. Payne, Le Kuai, Helen M. Worden, Sebastien C. Biraud, Colm Sweeney, Britton Stephens, Laura T. Iraci, Emma L. Yates, and Tomoaki Tanaka
Atmos. Chem. Phys., 17, 5407–5438, https://doi.org/10.5194/acp-17-5407-2017, https://doi.org/10.5194/acp-17-5407-2017, 2017
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We introduce new vertically resolved GOSAT products that better separate locally and remotely influenced CO2. Current GOSAT column results for CO2 (XCO2) are sensitive to fluxes on continental scales, whereas flux estimates from surface and tower measurements are affected by sampling bias and model transport uncertainty. These new GOSAT measurements of boundary layer CO2 are validated against aircraft and surface observations of CO2 and are compared to vertically resolved MOPITT CO.
Chantelle R. Lonsdale, Jennifer D. Hegarty, Karen E. Cady-Pereira, Matthew J. Alvarado, Daven K. Henze, Matthew D. Turner, Shannon L. Capps, John B. Nowak, J. Andy Neuman, Ann M. Middlebrook, Roya Bahreini, Jennifer G. Murphy, Milos Z. Markovic, Trevor C. VandenBoer, Lynn M. Russell, and Amy Jo Scarino
Atmos. Chem. Phys., 17, 2721–2739, https://doi.org/10.5194/acp-17-2721-2017, https://doi.org/10.5194/acp-17-2721-2017, 2017
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This study takes advantage of the high-resolution observations of NH3(g) made by the TES satellite instrument over Bakersfield during the CalNex campaign, along with campaign measurements, to compare CMAQ model results in the San Joaquin Valley, California. Additionally we evaluate the CMAQ bi-directional ammonia flux results using the CARB emissions inventory against these satellite and campaign measurements, not previously explored in combination.
Annmarie Eldering, Chris W. O'Dell, Paul O. Wennberg, David Crisp, Michael R. Gunson, Camille Viatte, Charles Avis, Amy Braverman, Rebecca Castano, Albert Chang, Lars Chapsky, Cecilia Cheng, Brian Connor, Lan Dang, Gary Doran, Brendan Fisher, Christian Frankenberg, Dejian Fu, Robert Granat, Jonathan Hobbs, Richard A. M. Lee, Lukas Mandrake, James McDuffie, Charles E. Miller, Vicky Myers, Vijay Natraj, Denis O'Brien, Gregory B. Osterman, Fabiano Oyafuso, Vivienne H. Payne, Harold R. Pollock, Igor Polonsky, Coleen M. Roehl, Robert Rosenberg, Florian Schwandner, Mike Smyth, Vivian Tang, Thomas E. Taylor, Cathy To, Debra Wunch, and Jan Yoshimizu
Atmos. Meas. Tech., 10, 549–563, https://doi.org/10.5194/amt-10-549-2017, https://doi.org/10.5194/amt-10-549-2017, 2017
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This paper describes the measurements of atmospheric carbon dioxide collected in the first 18 months of the satellite mission known as the Orbiting Carbon Observatory-2 (OCO-2). The paper shows maps of the carbon dioxide data, data density, and other data fields that illustrate the data quality. This mission has collected a more precise, more dense dataset of carbon dioxide then we have ever had previously.
Christopher E. Sioris, Chris A. McLinden, Mark W. Shephard, Vitali E. Fioletov, and Ihab Abboud
Atmos. Chem. Phys., 17, 1931–1943, https://doi.org/10.5194/acp-17-1931-2017, https://doi.org/10.5194/acp-17-1931-2017, 2017
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The contribution of the oil sands region to the local aerosol optical depth (AOD) is sought. Satellite data are used since they provide spatial coverage over many years. Satellites measure AOD with high correlation and small biases relative to coincident AERONET AODs. Trends are determined using annual mean AODs, and an increasing trend is found near the Shell mines. Spatially variable and high surface albedo is challenging for some sensors. Measuring polarization appears to be an asset.
Brian Connor, Hartmut Bösch, James McDuffie, Tommy Taylor, Dejian Fu, Christian Frankenberg, Chris O'Dell, Vivienne H. Payne, Michael Gunson, Randy Pollock, Jonathan Hobbs, Fabiano Oyafuso, and Yibo Jiang
Atmos. Meas. Tech., 9, 5227–5238, https://doi.org/10.5194/amt-9-5227-2016, https://doi.org/10.5194/amt-9-5227-2016, 2016
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We present an analysis of uncertainties in global measurements of the column-averaged dry-air mole fraction of CO2 (XCO2) by the satellite OCO-2. The analysis is based on our best estimates for uncertainties in the OCO-2 operational algorithm and its inputs. From these results we estimate the "variable error", which differs between soundings, to infer the error in the difference of XCO2 between any two soundings. Variable errors are usually < 1 ppm over ocean and ~ 0.5–2 ppm over land.
Hilke Oetjen, Vivienne H. Payne, Jessica L. Neu, Susan S. Kulawik, David P. Edwards, Annmarie Eldering, Helen M. Worden, and John R. Worden
Atmos. Chem. Phys., 16, 10229–10239, https://doi.org/10.5194/acp-16-10229-2016, https://doi.org/10.5194/acp-16-10229-2016, 2016
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We developed and tested a strategy for combining TES and IASI free-tropospheric ozone data. A time series of the merged ozone data is presented for regional monthly means over the western US, Europe, and eastern Asia. We show that free-tropospheric ozone over Europe and the western US has remained relatively constant over the past decade but that, contrary to expectations, ozone over Asia in recent years does not continue the rapid rate of increase observed from 2004–2010.
Matthew J. Alvarado, Chantelle R. Lonsdale, Helen L. Macintyre, Huisheng Bian, Mian Chin, David A. Ridley, Colette L. Heald, Kenneth L. Thornhill, Bruce E. Anderson, Michael J. Cubison, Jose L. Jimenez, Yutaka Kondo, Lokesh K. Sahu, Jack E. Dibb, and Chien Wang
Atmos. Chem. Phys., 16, 9435–9455, https://doi.org/10.5194/acp-16-9435-2016, https://doi.org/10.5194/acp-16-9435-2016, 2016
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Understanding the scattering and absorption of light by aerosols is necessary for understanding air quality and climate change. We used data from the 2008 ARCTAS campaign to evaluate aerosol optical property models using a closure methodology that separates errors in these models from other errors in aerosol emissions, chemistry, or transport. We find that the models on average perform reasonably well, and make suggestions for how remaining biases could be reduced.
Hélène Brogniez, Stephen English, Jean-François Mahfouf, Andreas Behrendt, Wesley Berg, Sid Boukabara, Stefan Alexander Buehler, Philippe Chambon, Antonia Gambacorta, Alan Geer, William Ingram, E. Robert Kursinski, Marco Matricardi, Tatyana A. Odintsova, Vivienne H. Payne, Peter W. Thorne, Mikhail Yu. Tretyakov, and Junhong Wang
Atmos. Meas. Tech., 9, 2207–2221, https://doi.org/10.5194/amt-9-2207-2016, https://doi.org/10.5194/amt-9-2207-2016, 2016
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Because a systematic difference between measurements of water vapor performed by space-borne observing instruments in the microwave spectral domain and their numerical modeling was recently highlighted, this work discusses and gives an overview of the various errors and uncertainties associated with each element in the comparison process. Indeed, the knowledge of absolute errors in any observation of the climate system is key, more specifically because we need to detect small changes.
Andrew M. Dzambo, David D. Turner, and Eli J. Mlawer
Atmos. Meas. Tech., 9, 1613–1626, https://doi.org/10.5194/amt-9-1613-2016, https://doi.org/10.5194/amt-9-1613-2016, 2016
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Radiosondes are used to characterize the humidity in the middle and upper troposphere, but suffer from a solar radiation induced dry bias. This work investigates the accuracy of two published correction algorithms using comparisons with other instruments.
M. W. Shephard, C. A. McLinden, K. E. Cady-Pereira, M. Luo, S. G. Moussa, A. Leithead, J. Liggio, R. M. Staebler, A. Akingunola, P. Makar, P. Lehr, J. Zhang, D. K. Henze, D. B. Millet, J. O. Bash, L. Zhu, K. C. Wells, S. L. Capps, S. Chaliyakunnel, M. Gordon, K. Hayden, J. R. Brook, M. Wolde, and S.-M. Li
Atmos. Meas. Tech., 8, 5189–5211, https://doi.org/10.5194/amt-8-5189-2015, https://doi.org/10.5194/amt-8-5189-2015, 2015
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This study provides direct validations of Tropospheric Emission Spectrometer (TES) satellite retrieved profiles against coincident aircraft profiles of carbon monoxide, ammonia, methanol, and formic acid, all of which are of interest for air quality. The comparisons are performed over the Canadian oil sands region during an intensive field campaign in support of the Joint Canada-Alberta Implementation Plan for the Oil Sands Monitoring (JOSM). Initial model evaluations are also provided.
L. Zhu, D. Henze, J. Bash, G.-R. Jeong, K. Cady-Pereira, M. Shephard, M. Luo, F. Paulot, and S. Capps
Atmos. Chem. Phys., 15, 12823–12843, https://doi.org/10.5194/acp-15-12823-2015, https://doi.org/10.5194/acp-15-12823-2015, 2015
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We implement new diurnal variation scheme for ammonia livestock emissions and bidirectional exchange scheme and its adjoint in the GEOS-Chem global chemical transport model. Updated diurnal variability improves modeled-to-hourly in situ measurements comparison. The ammonium soil pool in the bidirectional exchange model largely extends the ammonia lifetime in the atmosphere. Large model biases remain as livestock emissions are still underestimated.
J. R. Worden, A. J. Turner, A. Bloom, S. S. Kulawik, J. Liu, M. Lee, R. Weidner, K. Bowman, C. Frankenberg, R. Parker, and V. H. Payne
Atmos. Meas. Tech., 8, 3433–3445, https://doi.org/10.5194/amt-8-3433-2015, https://doi.org/10.5194/amt-8-3433-2015, 2015
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Here we demonstrate the potential for estimating lower tropospheric CH4 concentrations through the combination of free-tropospheric methane measurements from the Aura Tropospheric Emission Spectrometer (TES) and XCH4 (dry-mole air fraction of methane) from the Greenhouse Gases Observing Satellite - Thermal And Near-infrared for carbon Observation (GOSAT TANSO).
A. J. Turner, D. J. Jacob, K. J. Wecht, J. D. Maasakkers, E. Lundgren, A. E. Andrews, S. C. Biraud, H. Boesch, K. W. Bowman, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, A. Kuze, J. Notholt, H. Ohyama, R. Parker, V. H. Payne, R. Sussmann, C. Sweeney, V. A. Velazco, T. Warneke, P. O. Wennberg, and D. Wunch
Atmos. Chem. Phys., 15, 7049–7069, https://doi.org/10.5194/acp-15-7049-2015, https://doi.org/10.5194/acp-15-7049-2015, 2015
M. J. Alvarado, C. R. Lonsdale, R. J. Yokelson, S. K. Akagi, H. Coe, J. S. Craven, E. V. Fischer, G. R. McMeeking, J. H. Seinfeld, T. Soni, J. W. Taylor, D. R. Weise, and C. E. Wold
Atmos. Chem. Phys., 15, 6667–6688, https://doi.org/10.5194/acp-15-6667-2015, https://doi.org/10.5194/acp-15-6667-2015, 2015
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Being able to understand and simulate the chemical evolution of biomass burning smoke plumes under a wide variety of conditions is a critical part of forecasting the impact of these fires on air quality, atmospheric composition, and climate. Here we use an improved model of this chemistry to simulate the evolution of ozone and secondary organic aerosol within a young biomass burning smoke plume from the Williams prescribed burn in chaparral, which was sampled over California in November 2009.
M. W. Shephard and K. E. Cady-Pereira
Atmos. Meas. Tech., 8, 1323–1336, https://doi.org/10.5194/amt-8-1323-2015, https://doi.org/10.5194/amt-8-1323-2015, 2015
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Presented is a robust retrieval algorithm that demonstrates the capabilities of utilizing Cross-track Infrared Sounder (CrIS) satellite observations to globally retrieval ammonia (NH3) concentrations. Initial NH3 retrieval results show that CrIS is (i) sensitive to NH3 in the boundary layer, with peak vertical sensitivity typically around 850–750hPa (~2km), (ii) has a minimum detection limit of ~1ppbv (peak profile value typically at the surface), and (iii) typically has up to ~1 DOFS.
M. J. Alvarado, V. H. Payne, K. E. Cady-Pereira, J. D. Hegarty, S. S. Kulawik, K. J. Wecht, J. R. Worden, J. V. Pittman, and S. C. Wofsy
Atmos. Meas. Tech., 8, 965–985, https://doi.org/10.5194/amt-8-965-2015, https://doi.org/10.5194/amt-8-965-2015, 2015
H. Oetjen, V. H. Payne, S. S. Kulawik, A. Eldering, J. Worden, D. P. Edwards, G. L. Francis, H. M. Worden, C. Clerbaux, J. Hadji-Lazaro, and D. Hurtmans
Atmos. Meas. Tech., 7, 4223–4236, https://doi.org/10.5194/amt-7-4223-2014, https://doi.org/10.5194/amt-7-4223-2014, 2014
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We apply the TES ozone retrieval algorithm to IASI radiances and characterise the uncertainties and information content of the retrieved ozone profiles. We find that our biases with respect to sondes and our degrees of freedom for signal for ozone are comparable to previously published results from other IASI ozone algorithms. We find that predicted and empirical errors are consistent. In general, the precision of the IASI ozone profiles is better than 20%.
V. H. Payne, M. J. Alvarado, K. E. Cady-Pereira, J. R. Worden, S. S. Kulawik, and E. V. Fischer
Atmos. Meas. Tech., 7, 3737–3749, https://doi.org/10.5194/amt-7-3737-2014, https://doi.org/10.5194/amt-7-3737-2014, 2014
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Peroxyacetyl nitrate (PAN) plays an important role in the distribution of lower-atmospheric ozone. PAN can be transported far from the original pollution source, leading to ozone formation and degraded air quality in remote areas. Satellite observations from the Tropospheric Emission Spectrometer (TES) are sensitive to PAN at lower altitude than previous global data sets. We describe characteristics of the data and show elevated PAN associated with boreal fires and outflow of Asian pollution.
K. E. Cady-Pereira, S. Chaliyakunnel, M. W. Shephard, D. B. Millet, M. Luo, and K. C. Wells
Atmos. Meas. Tech., 7, 2297–2311, https://doi.org/10.5194/amt-7-2297-2014, https://doi.org/10.5194/amt-7-2297-2014, 2014
C. L. Heald, D. A. Ridley, J. H. Kroll, S. R. H. Barrett, K. E. Cady-Pereira, M. J. Alvarado, and C. D. Holmes
Atmos. Chem. Phys., 14, 5513–5527, https://doi.org/10.5194/acp-14-5513-2014, https://doi.org/10.5194/acp-14-5513-2014, 2014
K. C. Wells, D. B. Millet, K. E. Cady-Pereira, M. W. Shephard, D. K. Henze, N. Bousserez, E. C. Apel, J. de Gouw, C. Warneke, and H. B. Singh
Atmos. Chem. Phys., 14, 2555–2570, https://doi.org/10.5194/acp-14-2555-2014, https://doi.org/10.5194/acp-14-2555-2014, 2014
J. Worden, K. Wecht, C. Frankenberg, M. Alvarado, K. Bowman, E. Kort, S. Kulawik, M. Lee, V. Payne, and H. Worden
Atmos. Chem. Phys., 13, 3679–3692, https://doi.org/10.5194/acp-13-3679-2013, https://doi.org/10.5194/acp-13-3679-2013, 2013
Related subject area
Subject: Radiation | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Understanding the trends in reflected solar radiation: a latitude- and month-based perspective
Evaluating the representation of Arctic cirrus solar radiative effects in the Integrated Forecasting System with airborne measurements
Uncertainty in simulated brightness temperature due to sensitivity to atmospheric gas spectroscopic parameters from the centimeter- to submillimeter-wave range
Direct observational evidence from space of the effect of CO2 increase on longwave spectral radiances: the unique role of high-spectral-resolution measurements
LIME: Lunar Irradiance Model of ESA, a new tool for absolute radiometric calibration using the Moon
Influence of cloud retrieval errors due to three-dimensional radiative effects on calculations of broadband shortwave cloud radiative effect
Estimation of 1 km downwelling shortwave radiation over the Tibetan Plateau under all-sky conditions
Record-breaking statistics detect islands of cooling in a sea of warming
Radiative closure and cloud effects on the radiation budget based on satellite and shipborne observations during the Arctic summer research cruise, PS106
Impacts of active satellite sensors' low-level cloud detection limitations on cloud radiative forcing in the Arctic
Longwave radiative effect of the cloud–aerosol transition zone based on CERES observations
Ice and mixed-phase cloud statistics on the Antarctic Plateau
Photovoltaic power potential in West Africa using long-term satellite data
A semi-empirical potential energy surface and line list for H216O extending into the near-ultraviolet
Global distribution and 14-year changes in erythemal irradiance, UV atmospheric transmission, and total column ozone for2005–2018 estimated from OMI and EPIC observations
Biomass-burning-induced surface darkening and its impact on regional meteorology in eastern China
Air pollution slows down surface warming over the Tibetan Plateau
Estimation of hourly land surface heat fluxes over the Tibetan Plateau by the combined use of geostationary and polar-orbiting satellites
Estimations of global shortwave direct aerosol radiative effects above opaque water clouds using a combination of A-Train satellite sensors
Uncertainty of atmospheric microwave absorption model: impact on ground-based radiometer simulations and retrievals
Simulated and observed horizontal inhomogeneities of optical thickness of Arctic stratus
Net radiative effects of dust in the tropical North Atlantic based on integrated satellite observations and in situ measurements
Comparison of global observations and trends of total precipitable water derived from microwave radiometers and COSMIC radio occultation from 2006 to 2013
Characterizing energy budget variability at a Sahelian site: a test of NWP model behaviour
Scale dependence of cirrus horizontal heterogeneity effects on TOA measurements – Part I: MODIS brightness temperatures in the thermal infrared
Aerosol scattering effects on water vapor retrievals over the Los Angeles Basin
Directional, horizontal inhomogeneities of cloud optical thickness fields retrieved from ground-based and airbornespectral imaging
Airborne observations of far-infrared upwelling radiance in the Arctic
Retrieval of aerosol optical depth from surface solar radiation measurements using machine learning algorithms, non-linear regression and a radiative transfer-based look-up table
Microwave signatures of ice hydrometeors from ground-based observations above Summit, Greenland
Shortwave direct radiative effects of above-cloud aerosols over global oceans derived from 8 years of CALIOP and MODIS observations
Retrieving high-resolution surface solar radiation with cloud parameters derived by combining MODIS and MTSAT data
Instantaneous longwave radiative impact of ozone: an application on IASI/MetOp observations
A method to retrieve super-thin cloud optical depth over ocean background with polarized sunlight
Airborne observations and simulations of three-dimensional radiative interactions between Arctic boundary layer clouds and ice floes
Deriving polarization properties of desert-reflected solar spectra with PARASOL data
Using IASI to simulate the total spectrum of outgoing long-wave radiances
Investigation of the "elevated heat pump" hypothesis of the Asian monsoon using satellite observations
Improved retrieval of direct and diffuse downwelling surface shortwave flux in cloudless atmosphere using dynamic estimates of aerosol content and type: application to the LSA-SAF project
Surface-sensible and latent heat fluxes over the Tibetan Plateau from ground measurements, reanalysis, and satellite data
Influence of local surface albedo variability and ice crystal shape on passive remote sensing of thin cirrus
Combining MODIS, AVHRR and in situ data for evapotranspiration estimation over heterogeneous landscape of the Tibetan Plateau
Modeling polarized solar radiation from the ocean–atmosphere system for CLARREO inter-calibration applications
HIRS channel 12 brightness temperature dataset and its correlations with major climate indices
Multi-satellite aerosol observations in the vicinity of clouds
CLARA-SAL: a global 28 yr timeseries of Earth's black-sky surface albedo
Quantitative comparison of the variability in observed and simulated shortwave reflectance
Regional radiative impact of volcanic aerosol from the 2009 eruption of Mt. Redoubt
Airborne hyperspectral observations of surface and cloud directional reflectivity using a commercial digital camera
Direct and semi-direct radiative forcing of smoke aerosols over clouds
Ruixue Li, Bida Jian, Jiming Li, Deyu Wen, Lijie Zhang, Yang Wang, and Yuan Wang
Atmos. Chem. Phys., 24, 9777–9803, https://doi.org/10.5194/acp-24-9777-2024, https://doi.org/10.5194/acp-24-9777-2024, 2024
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Hemispheric or interannual averages of reflected solar radiation (RSR) can mask signals from seasonally active or region-specific mechanisms. We examine RSR characteristics from latitude and month perspectives, revealing decreased trends observed by CERES in both hemispheres driven by clear-sky atmospheric and cloud components at 30–50° N and cloud components at 0–50° S. AVHRR achieves symmetry criteria within uncertainty and is suitable for the long-term analysis of hemispheric RSR symmetry.
Johannes Röttenbacher, André Ehrlich, Hanno Müller, Florian Ewald, Anna E. Luebke, Benjamin Kirbus, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 8085–8104, https://doi.org/10.5194/acp-24-8085-2024, https://doi.org/10.5194/acp-24-8085-2024, 2024
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Weather prediction models simplify the physical processes related to light scattering by clouds consisting of complex ice crystals. Whether these simplifications are the cause for uncertainties in their prediction can be evaluated by comparing them with measurement data. Here we do this for Arctic ice clouds over sea ice using airborne measurements from two case studies. The model performs well for thick ice clouds but not so well for thin ones. This work can be used to improve the model.
Donatello Gallucci, Domenico Cimini, Emma Turner, Stuart Fox, Philip W. Rosenkranz, Mikhail Y. Tretyakov, Vinia Mattioli, Salvatore Larosa, and Filomena Romano
Atmos. Chem. Phys., 24, 7283–7308, https://doi.org/10.5194/acp-24-7283-2024, https://doi.org/10.5194/acp-24-7283-2024, 2024
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Nowadays, atmospheric radiative transfer models are widely used to simulate satellite and ground-based observations. A meaningful comparison between observations and simulations requires an estimate of the uncertainty associated with both. This work quantifies the uncertainty in atmospheric radiative transfer models in the microwave range, providing the uncertainty associated with simulations of new-generation satellite microwave sensors.
João Teixeira, R. Chris Wilson, and Heidar Th. Thrastarson
Atmos. Chem. Phys., 24, 6375–6383, https://doi.org/10.5194/acp-24-6375-2024, https://doi.org/10.5194/acp-24-6375-2024, 2024
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This paper presents direct evidence from space (solely based on observations) that CO2 increase leads to the theoretically expected effects on longwave spectral radiances. This is achieved by using a methodology that allows us to isolate the CO2 effects from the temperature and water vapor effects. By searching for ensembles of temperature and water vapor profiles that are similar to each other but have different values of CO2, it is possible to estimate the direct effects of CO2 on the spectra.
Carlos Toledano, Sarah Taylor, África Barreto, Stefan Adriaensen, Alberto Berjón, Agnieszka Bialek, Ramiro González, Emma Woolliams, and Marc Bouvet
Atmos. Chem. Phys., 24, 3649–3671, https://doi.org/10.5194/acp-24-3649-2024, https://doi.org/10.5194/acp-24-3649-2024, 2024
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The calibration of Earth observation sensors is key to ensuring the continuity of long-term and global climate records. Satellite sensors, calibrated prior to launch, are susceptible to degradation in space. The Moon provides a stable calibration reference; however, its illumination depends on the Sun–Earth–Moon geometry and must be modelled. A new lunar irradiance model is presented, built upon observations over 5 years at a high-altitude observatory and a rigorous calibration and validation.
Adeleke S. Ademakinwa, Zahid H. Tushar, Jianyu Zheng, Chenxi Wang, Sanjay Purushotham, Jianwu Wang, Kerry G. Meyer, Tamas Várnai, and Zhibo Zhang
Atmos. Chem. Phys., 24, 3093–3114, https://doi.org/10.5194/acp-24-3093-2024, https://doi.org/10.5194/acp-24-3093-2024, 2024
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Clouds play a critical role in our climate system. At present and in the near future, satellite-based remote sensing is the only means to obtain regional and global observations of cloud properties. The current satellite remote sensing algorithms are mostly based on the so-called 1D radiative transfer. This deviation from the 3D world reality can lead to large errors. In this study we investigate how this error affects our estimation of cloud radiative effects.
Peizhen Li, Lei Zhong, Yaoming Ma, Yunfei Fu, Meilin Cheng, Xian Wang, Yuting Qi, and Zixin Wang
Atmos. Chem. Phys., 23, 9265–9285, https://doi.org/10.5194/acp-23-9265-2023, https://doi.org/10.5194/acp-23-9265-2023, 2023
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In this paper, all-sky downwelling shortwave radiation (DSR) over the entire Tibetan Plateau (TP) at a spatial resolution of 1 km was estimated using an improved parameterization scheme. The influence of topography and different radiative attenuations were comprehensively taken into account. The derived DSR showed good agreement with in situ measurements. The accuracy was better than six other DSR products. The derived DSR also provided more reasonable and detailed spatial patterns.
Elisa T. Sena, Ilan Koren, Orit Altaratz, and Alexander B. Kostinski
Atmos. Chem. Phys., 22, 16111–16122, https://doi.org/10.5194/acp-22-16111-2022, https://doi.org/10.5194/acp-22-16111-2022, 2022
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We used record-breaking statistics together with spatial information to create record-breaking SST maps. The maps reveal warming patterns in the overwhelming majority of the ocean and coherent islands of cooling, where low records occur more frequently than high ones. Some of these cooling spots are well known; however, a surprising elliptical area in the Southern Ocean is observed as well. Similar analyses can be performed on other key climatological variables to explore their trend patterns.
Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Hannes J. Griesche, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 22, 9313–9348, https://doi.org/10.5194/acp-22-9313-2022, https://doi.org/10.5194/acp-22-9313-2022, 2022
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This article describes an intercomparison of radiative fluxes and cloud properties from satellite, shipborne observations, and 1D radiative transfer simulations. The analysis focuses on research for PS106 expedition aboard the German research vessel, Polarstern. The results are presented in detailed case studies, time series for the PS106 cruise and extended to the central Arctic region. The findings illustrate the main periods of agreement and discrepancies of both points of view.
Yinghui Liu
Atmos. Chem. Phys., 22, 8151–8173, https://doi.org/10.5194/acp-22-8151-2022, https://doi.org/10.5194/acp-22-8151-2022, 2022
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Cloud detection from state-of-art satellite radar and lidar misses low-level clouds. Using in situ observations, this study confirms this cloud detection limitation over the Arctic Ocean. Impacts of this detection limitation from combined satellite radar and lidar on the monthly mean radiation flux estimations at the surface and at the top of the atmosphere in the Arctic are limited but larger from only satellite radar or satellite lidar in monthly mean and instantaneous values.
Babak Jahani, Hendrik Andersen, Josep Calbó, Josep-Abel González, and Jan Cermak
Atmos. Chem. Phys., 22, 1483–1494, https://doi.org/10.5194/acp-22-1483-2022, https://doi.org/10.5194/acp-22-1483-2022, 2022
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The change in the state of sky from cloudy to cloudless (or vice versa) comprises an additional phase called
transition zonewith characteristics laying between those of aerosols and clouds. This study presents an approach for the quantification of the broadband longwave radiative effects of the cloud–aerosol transition zone at the top of the atmosphere during daytime over the ocean based on satellite observations and radiative transfer simulations.
William Cossich, Tiziano Maestri, Davide Magurno, Michele Martinazzo, Gianluca Di Natale, Luca Palchetti, Giovanni Bianchini, and Massimo Del Guasta
Atmos. Chem. Phys., 21, 13811–13833, https://doi.org/10.5194/acp-21-13811-2021, https://doi.org/10.5194/acp-21-13811-2021, 2021
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The presence of clouds over Concordia, in the Antarctic Plateau, is investigated. Results are obtained by applying a machine learning algorithm to measurements of the infrared radiation emitted by the atmosphere toward the surface. The clear-sky, ice cloud, and mixed-phase cloud occurrence at different timescales is studied. A comparison with satellite measurements highlights the ability of the algorithm to identify multiple cloud conditions and study their variability at different timescales.
Ina Neher, Susanne Crewell, Stefanie Meilinger, Uwe Pfeifroth, and Jörg Trentmann
Atmos. Chem. Phys., 20, 12871–12888, https://doi.org/10.5194/acp-20-12871-2020, https://doi.org/10.5194/acp-20-12871-2020, 2020
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Photovoltaic power is one current option to meet the rising energy demand with low environmental impact. Global horizontal irradiance (GHI) is the fuel for photovoltaic power installations and needs to be evaluated to plan and dimension power plants. In this study, 35 years of satellite-based GHI data are analyzed over West Africa to determine their impact on photovoltaic power generation. The major challenges for the development of a solar-based power system in West Africa are then outlined.
Eamon K. Conway, Iouli E. Gordon, Jonathan Tennyson, Oleg L. Polyansky, Sergei N. Yurchenko, and Kelly Chance
Atmos. Chem. Phys., 20, 10015–10027, https://doi.org/10.5194/acp-20-10015-2020, https://doi.org/10.5194/acp-20-10015-2020, 2020
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Water vapour has a complex spectrum and absorbs from the microwave to the near-UV where it dissociates. There is limited knowledge of the absorption features in the near-UV, and there is a large disagreement for the available models and experiments. We created a new ab initio model that is in good agreement with observation at 363 nm. At lower wavelengths, our calculations suggest that the latest experiments overestimate absorption. This has implications for trace gas retrievals in the near-UV.
Jay Herman, Alexander Cede, Liang Huang, Jerald Ziemke, Omar Torres, Nickolay Krotkov, Matthew Kowalewski, and Karin Blank
Atmos. Chem. Phys., 20, 8351–8380, https://doi.org/10.5194/acp-20-8351-2020, https://doi.org/10.5194/acp-20-8351-2020, 2020
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The amount of erythemal irradiance reaching the Earth's surface has been calculated from ozone, aerosol, and reflectivity data obtained from OMI and DSCOVR/EPIC satellite instruments showing areas with high levels of solar UV radiation. Changes in erythemal irradiance, cloud transmission, aerosol transmission, and ozone absorption have been estimated for 14 years 2005–2018 in units of percent per year for 191 locations, mostly large cities, and from EPIC for the entire illuminated Earth.
Rong Tang, Xin Huang, Derong Zhou, and Aijun Ding
Atmos. Chem. Phys., 20, 6177–6191, https://doi.org/10.5194/acp-20-6177-2020, https://doi.org/10.5194/acp-20-6177-2020, 2020
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Biomass-burning-induced large areas of dark char (i.e.
surface darkening) could influence the radiative energy balance. During the harvest season in eastern China, satellite retrieval shows that surface albedo was significantly decreased. Observational evidence of meteorological perturbations from the surface darkening is identified, which is further examined by model simulation. This work highlights the importance of burning-induced albedo change in weather forecast and regional climate.
Aolin Jia, Shunlin Liang, Dongdong Wang, Bo Jiang, and Xiaotong Zhang
Atmos. Chem. Phys., 20, 881–899, https://doi.org/10.5194/acp-20-881-2020, https://doi.org/10.5194/acp-20-881-2020, 2020
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The Tibetan Plateau (TP) plays a vital role in regional and global climate change due to its location and orography. After generating a long-term surface radiation (SR) dataset, we characterized the SR spatiotemporal variation along with temperature. Evidence from multiple data sources indicated that the TP dimming was primarily driven by increased aerosols from human activities, and the cooling effect of aerosol loading offsets TP surface warming, revealing the human impact on regional warming.
Lei Zhong, Yaoming Ma, Zeyong Hu, Yunfei Fu, Yuanyuan Hu, Xian Wang, Meilin Cheng, and Nan Ge
Atmos. Chem. Phys., 19, 5529–5541, https://doi.org/10.5194/acp-19-5529-2019, https://doi.org/10.5194/acp-19-5529-2019, 2019
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Fine-temporal-resolution turbulent heat fluxes at the plateau scale have significant importance for studying diurnal variation characteristics of atmospheric boundary and weather systems in the Tibetan Plateau (TP) and its surroundings. Time series of land surface heat fluxes with high temporal resolution over the entire TP were derived. The derived surface heat fluxes proved to be in good agreement with in situ measurements and were superior to GLDAS flux products.
Meloë S. Kacenelenbogen, Mark A. Vaughan, Jens Redemann, Stuart A. Young, Zhaoyan Liu, Yongxiang Hu, Ali H. Omar, Samuel LeBlanc, Yohei Shinozuka, John Livingston, Qin Zhang, and Kathleen A. Powell
Atmos. Chem. Phys., 19, 4933–4962, https://doi.org/10.5194/acp-19-4933-2019, https://doi.org/10.5194/acp-19-4933-2019, 2019
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Significant efforts are required to estimate the direct radiative effects of aerosols above clouds (DAREcloudy). We have used a combination of passive and active A-Train satellite sensors and derive mainly positive global and regional DAREcloudy values (e.g., global seasonal values between 0.13 and 0.26 W m-2). Despite differences in methods and sensors, the DAREcloudy values in this study are generally higher than previously reported. We discuss the primary reasons for these higher estimates.
Domenico Cimini, Philip W. Rosenkranz, Mikhail Y. Tretyakov, Maksim A. Koshelev, and Filomena Romano
Atmos. Chem. Phys., 18, 15231–15259, https://doi.org/10.5194/acp-18-15231-2018, https://doi.org/10.5194/acp-18-15231-2018, 2018
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The paper presents a general approach to quantify the uncertainty related to atmospheric absorption models. These models describe how the atmosphere interacts with radiation, and they have general implications for atmospheric sciences.
The presented approach contributes to a better understanding of the total uncertainty affecting atmospheric radiative properties, thus reducing the chances of systematic errors when observations are exploited for weather forecast or climate trend derivations.
Michael Schäfer, Katharina Loewe, André Ehrlich, Corinna Hoose, and Manfred Wendisch
Atmos. Chem. Phys., 18, 13115–13133, https://doi.org/10.5194/acp-18-13115-2018, https://doi.org/10.5194/acp-18-13115-2018, 2018
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Airborne observed horizontal fields of cloud optical thickness are compared with semi-idealized large eddy simulations of Arctic stratus. The comparison focuses on horizontal cloud inhomogeneities and directional features of the small-scale cloud structures. Using inhomogeneity parameters and autocorrelation analysis it is investigated, if the observed small-scale cloud inhomogeneities can be represented by the model. Forcings for cloud inhomogeneities are investigated in a sensitivity study.
Qianqian Song, Zhibo Zhang, Hongbin Yu, Seiji Kato, Ping Yang, Peter Colarco, Lorraine A. Remer, and Claire L. Ryder
Atmos. Chem. Phys., 18, 11303–11322, https://doi.org/10.5194/acp-18-11303-2018, https://doi.org/10.5194/acp-18-11303-2018, 2018
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Mineral dust is the most abundant atmospheric aerosol component in terms of dry mass. In this study, we integrate recent aircraft measurements of dust microphysical and optical properties with satellite retrievals of aerosol and radiative fluxes to quantify the dust direct radiative effects on the shortwave and longwave radiation at both the top of the atmosphere and the surface in the tropical North Atlantic during summer months.
Shu-Peng Ho, Liang Peng, Carl Mears, and Richard A. Anthes
Atmos. Chem. Phys., 18, 259–274, https://doi.org/10.5194/acp-18-259-2018, https://doi.org/10.5194/acp-18-259-2018, 2018
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In this study, we compare 7 years of atmospheric total precipitable water (TPW) derived from multiple microwave radiometers to collocated TPW estimates derived from COSMIC radio occultation under various atmospheric conditions over the oceans. Results show that these two TPW trends from independent observations are larger than previous estimates and are a strong indication of the positive water vapor–temperature feedback on a warming planet.
Anna Mackie, Paul I. Palmer, and Helen Brindley
Atmos. Chem. Phys., 17, 15095–15119, https://doi.org/10.5194/acp-17-15095-2017, https://doi.org/10.5194/acp-17-15095-2017, 2017
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We compare the balance of solar and thermal radiation at the surface and the top of the atmosphere from a forecasting model to observations at a site in Niamey, Niger, in the Sahel. To interpret the energy budgets we examine other factors, such as cloud properties, water vapour and aerosols, which we use to understand the differences between the observation and model. We find that some differences are linked to lack of ice in clouds, underestimated aerosol loading and surface temperatures.
Thomas Fauchez, Steven Platnick, Kerry Meyer, Céline Cornet, Frédéric Szczap, and Tamás Várnai
Atmos. Chem. Phys., 17, 8489–8508, https://doi.org/10.5194/acp-17-8489-2017, https://doi.org/10.5194/acp-17-8489-2017, 2017
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This study presents impact of cirrus cloud horizontal heterogeneity on simulated thermal infrared brightness temperatures at the top of the atmosphere for spatial resolutions ranging from 50 m to 10 km. The cirrus is generated by the 3DCLOUD code and the radiative transfer by the 3DMCPOL code. Brightness temperatures are mostly impacted by the horizontal transport effect and plane-parallel bias at high and coarse spatial resolutions, respectively, with a minimum around 100 m–250 m.
Zhao-Cheng Zeng, Qiong Zhang, Vijay Natraj, Jack S. Margolis, Run-Lie Shia, Sally Newman, Dejian Fu, Thomas J. Pongetti, Kam W. Wong, Stanley P. Sander, Paul O. Wennberg, and Yuk L. Yung
Atmos. Chem. Phys., 17, 2495–2508, https://doi.org/10.5194/acp-17-2495-2017, https://doi.org/10.5194/acp-17-2495-2017, 2017
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We propose a novel approach to describing the scattering effects of atmospheric aerosols using H2O retrievals in the near infrared. We found that the aerosol scattering effect is the primary contributor to the variations in the wavelength dependence of the H2O SCD retrievals and the scattering effects can be derived using H2O retrievals from multiple bands. This proposed method could potentially contribute towards reducing biases in greenhouse gas retrievals from space.
Michael Schäfer, Eike Bierwirth, André Ehrlich, Evelyn Jäkel, Frank Werner, and Manfred Wendisch
Atmos. Chem. Phys., 17, 2359–2372, https://doi.org/10.5194/acp-17-2359-2017, https://doi.org/10.5194/acp-17-2359-2017, 2017
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Cloud optical thickness fields, retrieved from solar spectral radiance measurements, are used to investigate the directional structure of horizontal cloud inhomogeneities with scalar one-dimensional inhomogeneity parameters, two-dimensional auto-correlation functions, and two-dimensional Fourier analysis. The investigations reveal that it is not sufficient to quantify horizontal cloud inhomogeneities by one-dimensional inhomogeneity parameters; two-dimensional parameters are necessary.
Quentin Libois, Liviu Ivanescu, Jean-Pierre Blanchet, Hannes Schulz, Heiko Bozem, W. Richard Leaitch, Julia Burkart, Jonathan P. D. Abbatt, Andreas B. Herber, Amir A. Aliabadi, and Éric Girard
Atmos. Chem. Phys., 16, 15689–15707, https://doi.org/10.5194/acp-16-15689-2016, https://doi.org/10.5194/acp-16-15689-2016, 2016
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The first airborne measurements performed with the FIRR are presented. Vertical profiles of upwelling spectral radiance in the far-infrared are measured in the Arctic atmosphere for the first time. They show the impact of the temperature inversion on the radiative budget of the atmosphere, especially in the far-infrared. The presence of ice clouds also significantly alters the far-infrared budget, highlighting the critical interplay between water vapour and clouds in this very dry region.
Jani Huttunen, Harri Kokkola, Tero Mielonen, Mika Esa Juhani Mononen, Antti Lipponen, Juha Reunanen, Anders Vilhelm Lindfors, Santtu Mikkonen, Kari Erkki Juhani Lehtinen, Natalia Kouremeti, Alkiviadis Bais, Harri Niska, and Antti Arola
Atmos. Chem. Phys., 16, 8181–8191, https://doi.org/10.5194/acp-16-8181-2016, https://doi.org/10.5194/acp-16-8181-2016, 2016
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For a good estimate of the current forcing by anthropogenic aerosols, knowledge in past is needed. One option to lengthen time series is to retrieve aerosol optical depth from solar radiation measurements. We have evaluated several methods for this task. Most of the methods produce aerosol optical depth estimates with a good accuracy. However, machine learning methods seem to be the most applicable not to produce any systematic biases, since they do not need constrain the aerosol properties.
Claire Pettersen, Ralf Bennartz, Mark S. Kulie, Aronne J. Merrelli, Matthew D. Shupe, and David D. Turner
Atmos. Chem. Phys., 16, 4743–4756, https://doi.org/10.5194/acp-16-4743-2016, https://doi.org/10.5194/acp-16-4743-2016, 2016
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We examined four summers of data from a ground-based atmospheric science instrument suite at Summit Station, Greenland, to isolate the signature of the ice precipitation. By using a combination of instruments with different specialities, we identified a passive microwave signature of the ice precipitation. This ice signature compares well to models using synthetic data characteristic of the site.
Zhibo Zhang, Kerry Meyer, Hongbin Yu, Steven Platnick, Peter Colarco, Zhaoyan Liu, and Lazaros Oreopoulos
Atmos. Chem. Phys., 16, 2877–2900, https://doi.org/10.5194/acp-16-2877-2016, https://doi.org/10.5194/acp-16-2877-2016, 2016
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The frequency of occurrence and shortwave direct radiative effects (DRE) of above-cloud aerosols (ACAs) over global oceans are investigated using 8 years of collocated CALIOP and MODIS observations. We estimated that ACAs have a global ocean annual mean diurnally averaged cloudy-sky DRE of 0.015 W m−2 (range of −0.03 to 0.06 W m−2) at TOA. The DREs at surface and within atmosphere are −0.15 W m−2 (range of −0.09 to −0.21 W m−2), and 0.17 W m−2 (range of 0.11 to 0.24 W m−2), respectively.
Wenjun Tang, Jun Qin, Kun Yang, Shaomin Liu, Ning Lu, and Xiaolei Niu
Atmos. Chem. Phys., 16, 2543–2557, https://doi.org/10.5194/acp-16-2543-2016, https://doi.org/10.5194/acp-16-2543-2016, 2016
Short summary
Short summary
In this paper, we develop a new method to quickly retrieve high-resolution surface solar radiation (SSR) over China by combining MODIS and MTSAT data. The RMSEs of the retrieved SSR at hourly, daily, and monthly scales are about 98.5, 34.2, and 22.1 W m−2. The accuracy is comparable to or even higher than other two satellite radiation products. Finally, we derive an 8-year high-resolution SSR data set (hourly, 5 km) from 2007 to 2014, which would contribute to studies of land surface processes.
S. Doniki, D. Hurtmans, L. Clarisse, C. Clerbaux, H. M. Worden, K. W. Bowman, and P.-F. Coheur
Atmos. Chem. Phys., 15, 12971–12987, https://doi.org/10.5194/acp-15-12971-2015, https://doi.org/10.5194/acp-15-12971-2015, 2015
W. Sun, R. R. Baize, G. Videen, Y. Hu, and Q. Fu
Atmos. Chem. Phys., 15, 11909–11918, https://doi.org/10.5194/acp-15-11909-2015, https://doi.org/10.5194/acp-15-11909-2015, 2015
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Short summary
A method is reported for retrieving super-thin cloud optical depth with polarized light. It is found that near-backscatter p-polarized light is sensitive to clouds, but not to ocean conditions. Near-backscatter p-polarized intensity linearly relates to super-thin cloud optical depth. Based on these findings, super-thin cloud optical depth can be retrieved with little effect from surface reflection.
M. Schäfer, E. Bierwirth, A. Ehrlich, E. Jäkel, and M. Wendisch
Atmos. Chem. Phys., 15, 8147–8163, https://doi.org/10.5194/acp-15-8147-2015, https://doi.org/10.5194/acp-15-8147-2015, 2015
W. Sun, R. R. Baize, C. Lukashin, and Y. Hu
Atmos. Chem. Phys., 15, 7725–7734, https://doi.org/10.5194/acp-15-7725-2015, https://doi.org/10.5194/acp-15-7725-2015, 2015
E. C. Turner, H.-T. Lee, and S. F. B. Tett
Atmos. Chem. Phys., 15, 6561–6575, https://doi.org/10.5194/acp-15-6561-2015, https://doi.org/10.5194/acp-15-6561-2015, 2015
M. M. Wonsick, R. T. Pinker, and Y. Ma
Atmos. Chem. Phys., 14, 8749–8761, https://doi.org/10.5194/acp-14-8749-2014, https://doi.org/10.5194/acp-14-8749-2014, 2014
X. Ceamanos, D. Carrer, and J.-L. Roujean
Atmos. Chem. Phys., 14, 8209–8232, https://doi.org/10.5194/acp-14-8209-2014, https://doi.org/10.5194/acp-14-8209-2014, 2014
Q. Shi and S. Liang
Atmos. Chem. Phys., 14, 5659–5677, https://doi.org/10.5194/acp-14-5659-2014, https://doi.org/10.5194/acp-14-5659-2014, 2014
C. Fricke, A. Ehrlich, E. Jäkel, B. Bohn, M. Wirth, and M. Wendisch
Atmos. Chem. Phys., 14, 1943–1958, https://doi.org/10.5194/acp-14-1943-2014, https://doi.org/10.5194/acp-14-1943-2014, 2014
Y. Ma, Z. Zhu, L. Zhong, B. Wang, C. Han, Z. Wang, Y. Wang, L. Lu, P. M. Amatya, W. Ma, and Z. Hu
Atmos. Chem. Phys., 14, 1507–1515, https://doi.org/10.5194/acp-14-1507-2014, https://doi.org/10.5194/acp-14-1507-2014, 2014
W. Sun and C. Lukashin
Atmos. Chem. Phys., 13, 10303–10324, https://doi.org/10.5194/acp-13-10303-2013, https://doi.org/10.5194/acp-13-10303-2013, 2013
L. Shi, C. J. Schreck III, and V. O. John
Atmos. Chem. Phys., 13, 6907–6920, https://doi.org/10.5194/acp-13-6907-2013, https://doi.org/10.5194/acp-13-6907-2013, 2013
T. Várnai, A. Marshak, and W. Yang
Atmos. Chem. Phys., 13, 3899–3908, https://doi.org/10.5194/acp-13-3899-2013, https://doi.org/10.5194/acp-13-3899-2013, 2013
A. Riihelä, T. Manninen, V. Laine, K. Andersson, and F. Kaspar
Atmos. Chem. Phys., 13, 3743–3762, https://doi.org/10.5194/acp-13-3743-2013, https://doi.org/10.5194/acp-13-3743-2013, 2013
Y. L. Roberts, P. Pilewskie, B. C. Kindel, D. R. Feldman, and W. D. Collins
Atmos. Chem. Phys., 13, 3133–3147, https://doi.org/10.5194/acp-13-3133-2013, https://doi.org/10.5194/acp-13-3133-2013, 2013
C. L. Young, I. N. Sokolik, and J. Dufek
Atmos. Chem. Phys., 12, 3699–3715, https://doi.org/10.5194/acp-12-3699-2012, https://doi.org/10.5194/acp-12-3699-2012, 2012
A. Ehrlich, E. Bierwirth, M. Wendisch, A. Herber, and J.-F. Gayet
Atmos. Chem. Phys., 12, 3493–3510, https://doi.org/10.5194/acp-12-3493-2012, https://doi.org/10.5194/acp-12-3493-2012, 2012
E. M. Wilcox
Atmos. Chem. Phys., 12, 139–149, https://doi.org/10.5194/acp-12-139-2012, https://doi.org/10.5194/acp-12-139-2012, 2012
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