Articles | Volume 24, issue 14
https://doi.org/10.5194/acp-24-8139-2024
https://doi.org/10.5194/acp-24-8139-2024
Research article
 | 
19 Jul 2024
Research article |  | 19 Jul 2024

NOx emissions in France in 2019–2021 as estimated by the high-spatial-resolution assimilation of TROPOMI NO2 observations

Robin Plauchu, Audrey Fortems-Cheiney, Grégoire Broquet, Isabelle Pison, Antoine Berchet, Elise Potier, Gaëlle Dufour, Adriana Coman, Dilek Savas, Guillaume Siour, and Henk Eskes

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Subject: Gases | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Cited articles

Almaraz, M., Bai, E., Wang, C., Trousdell, J., Conley, S., Faloona, I., and Houlton, B. Z.: Agriculture is a major source of NOx pollution in California, Science Advances, 4, eaao3477, https://doi.org/10.1126/sciadv.aao3477, 2018. a
Barré, J., Petetin, H., Colette, A., Guevara, M., Peuch, V.-H., Rouil, L., Engelen, R., Inness, A., Flemming, J., Pérez García-Pando, C., Bowdalo, D., Meleux, F., Geels, C., Christensen, J. H., Gauss, M., Benedictow, A., Tsyro, S., Friese, E., Struzewska, J., Kaminski, J. W., Douros, J., Timmermans, R., Robertson, L., Adani, M., Jorba, O., Joly, M., and Kouznetsov, R.: Estimating lockdown-induced European NO2 changes using satellite and surface observations and air quality models, Atmos. Chem. Phys., 21, 7373–7394, https://doi.org/10.5194/acp-21-7373-2021, 2021. a, b, c, d
Bauwens, M., Compernolle, S., Stavrakou, T., Müller, J.-F., Van Gent, J., Eskes, H., Levelt, P. F., Van Der A, R., Veefkind, J., Vlietinck, J., Yu, H., and Zehner, C.: Impact of coronavirus outbreak on NO2 pollution assessed using TROPOMI and OMI observations, Geophys. Res. Lett., 47, e2020GL087978, https://doi.org/10.1029/2020GL087978, 2020. a
Berchet, A., Sollum, E., Thompson, R. L., Pison, I., Thanwerdas, J., Broquet, G., Chevallier, F., Aalto, T., Berchet, A., Bergamaschi, P., Brunner, D., Engelen, R., Fortems-Cheiney, A., Gerbig, C., Groot Zwaaftink, C. D., Haussaire, J.-M., Henne, S., Houweling, S., Karstens, U., Kutsch, W. L., Luijkx, I. T., Monteil, G., Palmer, P. I., van Peet, J. C. A., Peters, W., Peylin, P., Potier, E., Rödenbeck, C., Saunois, M., Scholze, M., Tsuruta, A., and Zhao, Y.: The Community Inversion Framework v1.0: a unified system for atmospheric inversion studies, Geosci. Model Dev., 14, 5331–5354, https://doi.org/10.5194/gmd-14-5331-2021, 2021. a, b
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This study uses the Community Inversion Framework and CHIMERE model to assess the potential of TROPOMI-S5P PAL NO2 tropospheric column data to estimate NOx emissions in France (2019–2021). Results show a 3 % decrease in average emissions compared to the 2016 CAMS-REG/INS, lower than the 14 % decrease from CITEPA. The study highlights challenges in capturing emission anomalies due to limited data coverage and error levels but shows promise for local inventory improvements.
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