Articles | Volume 17, issue 12
https://doi.org/10.5194/acp-17-7955-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7955-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
30 Jun 2017
Research article |
| 30 Jun 2017
Aerosol–landscape–cloud interaction: signatures of topography effect on cloud droplet formation
Sami Romakkaniemi
CORRESPONDING AUTHOR
Finnish Meteorological Institute, Kuopio, Finland
Zubair Maalick
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Antti Hellsten
Finnish Meteorological Institute, Helsinki, Finland
Antti Ruuskanen
Finnish Meteorological Institute, Kuopio, Finland
Olli Väisänen
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Irshad Ahmad
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Juha Tonttila
Finnish Meteorological Institute, Kuopio, Finland
Karlsruhe Institute of Technology, Karlsruhe, Germany
Santtu Mikkonen
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Mika Komppula
Finnish Meteorological Institute, Kuopio, Finland
Thomas Kühn
Finnish Meteorological Institute, Kuopio, Finland
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
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Ian Boutle, Wayne Angevine, Jian-Wen Bao, Thierry Bergot, Ritthik Bhattacharya, Andreas Bott, Leo Ducongé, Richard Forbes, Tobias Goecke, Evelyn Grell, Adrian Hill, Adele L. Igel, Innocent Kudzotsa, Christine Lac, Bjorn Maronga, Sami Romakkaniemi, Juerg Schmidli, Johannes Schwenkel, Gert-Jan Steeneveld, and Benoît Vié
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Harri Kokkola, Thomas Kühn, Anton Laakso, Tommi Bergman, Kari E. J. Lehtinen, Tero Mielonen, Antti Arola, Scarlet Stadtler, Hannele Korhonen, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Ina Tegen, Colombe Siegenthaler-Le Drian, Martin G. Schultz, Isabelle Bey, Philip Stier, Nikos Daskalakis, Colette L. Heald, and Sami Romakkaniemi
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Robin G. Stevens, Katharina Loewe, Christopher Dearden, Antonios Dimitrelos, Anna Possner, Gesa K. Eirund, Tomi Raatikainen, Adrian A. Hill, Benjamin J. Shipway, Jonathan Wilkinson, Sami Romakkaniemi, Juha Tonttila, Ari Laaksonen, Hannele Korhonen, Paul Connolly, Ulrike Lohmann, Corinna Hoose, Annica M. L. Ekman, Ken S. Carslaw, and Paul R. Field
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Antti Lipponen, Tero Mielonen, Mikko R. A. Pitkänen, Robert C. Levy, Virginia R. Sawyer, Sami Romakkaniemi, Ville Kolehmainen, and Antti Arola
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Maria Filioglou, Anna Nikandrova, Sami Niemelä, Holger Baars, Tero Mielonen, Ari Leskinen, David Brus, Sami Romakkaniemi, Elina Giannakaki, and Mika Komppula
Atmos. Meas. Tech., 10, 4303–4316, https://doi.org/10.5194/amt-10-4303-2017, https://doi.org/10.5194/amt-10-4303-2017, 2017
Anton Laakso, Hannele Korhonen, Sami Romakkaniemi, and Harri Kokkola
Atmos. Chem. Phys., 17, 6957–6974, https://doi.org/10.5194/acp-17-6957-2017, https://doi.org/10.5194/acp-17-6957-2017, 2017
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Based on simulations, equatorial stratospheric sulfur injections have shown to be an efficient strategy to counteract ongoing global warming. However, equatorial injections would result in relatively larger cooling in low latitudes than in high latitudes. This together with greenhouse-gas-induced warming would lead to cooling in the Equator and warming in the high latitudes. Results of this study show that a more optimal cooling effect is achieved by varying the injection area seasonally.
Antti Arola, Thomas F. Eck, Harri Kokkola, Mikko R. A. Pitkänen, and Sami Romakkaniemi
Atmos. Chem. Phys., 17, 5991–6001, https://doi.org/10.5194/acp-17-5991-2017, https://doi.org/10.5194/acp-17-5991-2017, 2017
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Juha Tonttila, Zubair Maalick, Tomi Raatikainen, Harri Kokkola, Thomas Kühn, and Sami Romakkaniemi
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Olli Väisänen, Antti Ruuskanen, Arttu Ylisirniö, Pasi Miettinen, Harri Portin, Liqing Hao, Ari Leskinen, Mika Komppula, Sami Romakkaniemi, Kari E. J. Lehtinen, and Annele Virtanen
Atmos. Chem. Phys., 16, 10385–10398, https://doi.org/10.5194/acp-16-10385-2016, https://doi.org/10.5194/acp-16-10385-2016, 2016
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In-cloud measurements of aerosol hygroscopicity and cloud droplet activation were conducted in Kuopio, Finland. According to the observations, the less hygroscopic accumulation mode particles were present in the non-activated aerosol, whereas the more hygroscopic particles were scavenged into cloud droplets. The results illustrate the sensitivity of cloud droplet formation to varying chemical composition and highlight the need for proper treatment of anthropogenic aerosols in CCN predictions.
A. Arola, G. L. Schuster, M. R. A. Pitkänen, O. Dubovik, H. Kokkola, A. V. Lindfors, T. Mielonen, T. Raatikainen, S. Romakkaniemi, S. N. Tripathi, and H. Lihavainen
Atmos. Chem. Phys., 15, 12731–12740, https://doi.org/10.5194/acp-15-12731-2015, https://doi.org/10.5194/acp-15-12731-2015, 2015
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There have been relatively few measurement-based estimates for the direct radiative effect of brown carbon so far. This is first time that the direct radiative effect of brown carbon is estimated by exploiting the AERONET-retrieved imaginary indices. We estimated it for four sites in the Indo-Gangetic Plain: Karachi, Lahore,
Kanpur and Gandhi College.
M. Dalirian, H. Keskinen, L. Ahlm, A. Ylisirniö, S. Romakkaniemi, A. Laaksonen, A. Virtanen, and I. Riipinen
Atmos. Chem. Phys., 15, 3815–3829, https://doi.org/10.5194/acp-15-3815-2015, https://doi.org/10.5194/acp-15-3815-2015, 2015
L. Q. Hao, A. Kortelainen, S. Romakkaniemi, H. Portin, A. Jaatinen, A. Leskinen, M. Komppula, P. Miettinen, D. Sueper, A. Pajunoja, J. N. Smith, K. E. J. Lehtinen, D. R. Worsnop, A. Laaksonen, and A. Virtanen
Atmos. Chem. Phys., 14, 13483–13495, https://doi.org/10.5194/acp-14-13483-2014, https://doi.org/10.5194/acp-14-13483-2014, 2014
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Positive matrix factorization (PMF) was applied to the unified high-resolution mass spectra organic species with NO+ and NO2+ ions from the measurement in a mixed region between the boreal forestland and the urban area. The PMF analysis succeeded in separating the mixed spectra into three distinct organic factors and one inorganic factor. The particulate organic nitrate was distinguished by PMF for the first time, with a contribution of one-third of the total nitrate mass.
H. Portin, A. Leskinen, L. Hao, A. Kortelainen, P. Miettinen, A. Jaatinen, A. Laaksonen, K. E. J. Lehtinen, S. Romakkaniemi, and M. Komppula
Atmos. Chem. Phys., 14, 6021–6034, https://doi.org/10.5194/acp-14-6021-2014, https://doi.org/10.5194/acp-14-6021-2014, 2014
S. Romakkaniemi, A. Jaatinen, A. Laaksonen, A. Nenes, and T. Raatikainen
Atmos. Meas. Tech., 7, 1377–1384, https://doi.org/10.5194/amt-7-1377-2014, https://doi.org/10.5194/amt-7-1377-2014, 2014
H. Kokkola, P. Yli-Pirilä, M. Vesterinen, H. Korhonen, H. Keskinen, S. Romakkaniemi, L. Hao, A. Kortelainen, J. Joutsensaari, D. R. Worsnop, A. Virtanen, and K. E. J. Lehtinen
Atmos. Chem. Phys., 14, 1689–1700, https://doi.org/10.5194/acp-14-1689-2014, https://doi.org/10.5194/acp-14-1689-2014, 2014
T. Korhola, H. Kokkola, H. Korhonen, A.-I. Partanen, A. Laaksonen, K. E. J. Lehtinen, and S. Romakkaniemi
Geosci. Model Dev., 7, 161–174, https://doi.org/10.5194/gmd-7-161-2014, https://doi.org/10.5194/gmd-7-161-2014, 2014
A. Lipponen, V. Kolehmainen, S. Romakkaniemi, and H. Kokkola
Geosci. Model Dev., 6, 2087–2098, https://doi.org/10.5194/gmd-6-2087-2013, https://doi.org/10.5194/gmd-6-2087-2013, 2013
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Romanos Foskinis, Ghislain Motos, Maria I. Gini, Olga Zografou, Kunfeng Gao, Stergios Vratolis, Konstantinos Granakis, Ville Vakkari, Kalliopi Violaki, Andreas Aktypis, Christos Kaltsonoudis, Zongbo Shi, Mika Komppula, Spyros N. Pandis, Konstantinos Eleftheriadis, Alexandros Papayannis, and Athanasios Nenes
EGUsphere, https://doi.org/10.5194/egusphere-2024-490, https://doi.org/10.5194/egusphere-2024-490, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Analysis of modeling, in-situ & remote sensing reveal the microphysical state of orographic clouds & their response to aerosol from the boundary layer & free troposphere. We should that this cloud responses to aerosol is robust, as predicted supersaturation and cloud droplet number levels agree with those determined from in-cloud measurements. The ability to determine if clouds are velocity- or aerosol-limited allow for novel model constraints and remote sensing products.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Kalle Nordling, Jukka-Pekka Keskinen, Sami Romakkaniemi, Harri Kokkola, Petri Räisänen, Antti Lipponen, Antti-Ilari Partanen, Jaakko Ahola, Juha Tonttila, Muzaffer Ege Alper, Hannele Korhonen, and Tomi Raatikainen
Atmos. Chem. Phys., 24, 869–890, https://doi.org/10.5194/acp-24-869-2024, https://doi.org/10.5194/acp-24-869-2024, 2024
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Our results show that the global model is stable and it provides meaningful results. This way we can include a physics-based presentation of sub-grid physics (physics which happens on a 100 m scale) in the global model, whose resolution is on a 100 km scale.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
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EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
EGUsphere, https://doi.org/10.5194/egusphere-2023-2768, https://doi.org/10.5194/egusphere-2023-2768, 2023
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The study underscores the influence of semi-volatile organic compounds on the formation of secondary organic aerosol (SOA). Our findings demonstrate their considerable impact on climate, emphasizing the necessity to improve their representation in large-scale climate models. This research provides a nuanced perspective on the challenges in modelling, emphasizing the significance of semi-volatile compounds and their volatility distribution in predicting global climate patterns.
Ville Leinonen, Miska Olin, Sampsa Martikainen, Panu Karjalainen, and Santtu Mikkonen
Atmos. Meas. Tech., 16, 5075–5089, https://doi.org/10.5194/amt-16-5075-2023, https://doi.org/10.5194/amt-16-5075-2023, 2023
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Emission factor calculation was studied to provide models that do not use traditional CO2-based calculation in exhaust plume analysis. Two types of models, one based on the physical dependency of dilution of the exhaust flow rate and speed and two based on the statistical, measured dependency of dilution of the exhaust flow rate, acceleration, speed, altitude change, and/or wind, were developed. These methods could possibly be extended to also calculate non-exhaust emissions in the future.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Athena Augusta Floutsi, Holger Baars, Ronny Engelmann, Dietrich Althausen, Albert Ansmann, Stephanie Bohlmann, Birgit Heese, Julian Hofer, Thomas Kanitz, Moritz Haarig, Kevin Ohneiser, Martin Radenz, Patric Seifert, Annett Skupin, Zhenping Yin, Sabur F. Abdullaev, Mika Komppula, Maria Filioglou, Elina Giannakaki, Iwona S. Stachlewska, Lucja Janicka, Daniele Bortoli, Eleni Marinou, Vassilis Amiridis, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Boris Barja, and Ulla Wandinger
Atmos. Meas. Tech., 16, 2353–2379, https://doi.org/10.5194/amt-16-2353-2023, https://doi.org/10.5194/amt-16-2353-2023, 2023
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DeLiAn is a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio) and the Ångström exponent. The data collection is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarization lidar measurements and currently covers two wavelengths, 355 and 532 nm, for 13 aerosol categories ranging from basic aerosol types to mixtures.
Tuuli Miinalainen, Harri Kokkola, Antti Lipponen, Antti-Pekka Hyvärinen, Vijay Kumar Soni, Kari E. J. Lehtinen, and Thomas Kühn
Atmos. Chem. Phys., 23, 3471–3491, https://doi.org/10.5194/acp-23-3471-2023, https://doi.org/10.5194/acp-23-3471-2023, 2023
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We simulated the effects of aerosol emission mitigation on both global and regional radiative forcing and city-level air quality with a global-scale climate model. We used a machine learning downscaling approach to bias-correct the PM2.5 values obtained from the global model for the Indian megacity New Delhi. Our results indicate that aerosol mitigation could result in both improved air quality and less radiative heating for India.
Ville Leinonen, Harri Kokkola, Taina Yli-Juuti, Tero Mielonen, Thomas Kühn, Tuomo Nieminen, Simo Heikkinen, Tuuli Miinalainen, Tommi Bergman, Ken Carslaw, Stefano Decesari, Markus Fiebig, Tareq Hussein, Niku Kivekäs, Radovan Krejci, Markku Kulmala, Ari Leskinen, Andreas Massling, Nikos Mihalopoulos, Jane P. Mulcahy, Steffen M. Noe, Twan van Noije, Fiona M. O'Connor, Colin O'Dowd, Dirk Olivie, Jakob B. Pernov, Tuukka Petäjä, Øyvind Seland, Michael Schulz, Catherine E. Scott, Henrik Skov, Erik Swietlicki, Thomas Tuch, Alfred Wiedensohler, Annele Virtanen, and Santtu Mikkonen
Atmos. Chem. Phys., 22, 12873–12905, https://doi.org/10.5194/acp-22-12873-2022, https://doi.org/10.5194/acp-22-12873-2022, 2022
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We provide the first extensive comparison of detailed aerosol size distribution trends between in situ observations from Europe and five different earth system models. We investigated aerosol modes (nucleation, Aitken, and accumulation) separately and were able to show the differences between measured and modeled trends and especially their seasonal patterns. The differences in model results are likely due to complex effects of several processes instead of certain specific model features.
Silvia M. Calderón, Juha Tonttila, Angela Buchholz, Jorma Joutsensaari, Mika Komppula, Ari Leskinen, Liqing Hao, Dmitri Moisseev, Iida Pullinen, Petri Tiitta, Jian Xu, Annele Virtanen, Harri Kokkola, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 12417–12441, https://doi.org/10.5194/acp-22-12417-2022, https://doi.org/10.5194/acp-22-12417-2022, 2022
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The spatial and temporal restrictions of observations and oversimplified aerosol representation in large eddy simulations (LES) limit our understanding of aerosol–stratocumulus interactions. In this closure study of in situ and remote sensing observations and outputs from UCLALES–SALSA, we have assessed the role of convective overturning and aerosol effects in two cloud events observed at the Puijo SMEAR IV station, Finland, a diurnal-high aerosol case and a nocturnal-low aerosol case.
Sini Isokääntä, Paul Kim, Santtu Mikkonen, Thomas Kühn, Harri Kokkola, Taina Yli-Juuti, Liine Heikkinen, Krista Luoma, Tuukka Petäjä, Zak Kipling, Daniel Partridge, and Annele Virtanen
Atmos. Chem. Phys., 22, 11823–11843, https://doi.org/10.5194/acp-22-11823-2022, https://doi.org/10.5194/acp-22-11823-2022, 2022
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This research employs air mass history analysis and observations to study how clouds and precipitation affect atmospheric aerosols during transport to a boreal forest site. The mass concentrations of studied chemical species showed exponential decrease as a function of accumulated rain along the air mass route. Our analysis revealed in-cloud sulfate formation, while no major changes in organic mass were seen. Most of the in-cloud-formed sulfate could be assigned to particle sizes above 200 nm.
Marje Prank, Juha Tonttila, Jaakko Ahola, Harri Kokkola, Thomas Kühn, Sami Romakkaniemi, and Tomi Raatikainen
Atmos. Chem. Phys., 22, 10971–10992, https://doi.org/10.5194/acp-22-10971-2022, https://doi.org/10.5194/acp-22-10971-2022, 2022
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Aerosols and clouds persist as the dominant sources of uncertainty in climate projections. In this modelling study, we investigate the role of marine aerosols in influencing the lifetime of low-level clouds. Our high resolution simulations show that sea spray can both extend and shorten the lifetime of the cloud layer depending on the model setup. The impact of the primary marine organics is relatively limited while secondary aerosol from monoterpenes can have larger impact.
Ajit Ahlawat, Kay Weinhold, Jesus Marval, Paolo Tronville, Ari Leskinen, Mika Komppula, Holger Gerwig, Lars Gerling, Stephan Weber, Rikke Bramming Jørgensen, Thomas Nørregaard Jensen, Marouane Merizak, Ulrich Vogt, Carla Ribalta, Mar Viana, Andre Schmitz, Maria Chiesa, Giacomo Gerosa, Lothar Keck, Markus Pesch, Gerhard Steiner, Thomas Krinke, Torsten Tritscher, Wolfram Birmili, and Alfred Wiedensohler
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-155, https://doi.org/10.5194/amt-2022-155, 2022
Revised manuscript not accepted
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Measurements of ultrafine particles must be done with quality-assured instruments. The performance of portable instruments such as NanoScan SMPS, and GRIMM Mini WRAS spectrometer measuring the particle number size distribution in the range from 10 to 200 nm were investigated. The influence of different aerosol types and maintenance activities on these instruments were explored. The results show that these portable instruments are suitable for mobile UFP measurements for source identification.
Petri Tiitta, Ari Leskinen, Ville A. Kaikkonen, Eero O. Molkoselkä, Anssi J. Mäkynen, Jorma Joutsensaari, Silvia Calderon, Sami Romakkaniemi, and Mika Komppula
Atmos. Meas. Tech., 15, 2993–3009, https://doi.org/10.5194/amt-15-2993-2022, https://doi.org/10.5194/amt-15-2993-2022, 2022
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The novel holographic imaging instrument (ICEMET) was adapted to measure the microphysical properties of liquid clouds, and these values were compared with parallel measurements of a cloud droplet spectrometer (FM-120) and particle measurements using a twin-inlet system. When the intercomparison was carried out during isoaxial sampling, our results showed good agreement in terms of variability between the instruments. This agreement was confirmed using Mutual and Pearson correlation analyses.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Jaakko Ahola, Tomi Raatikainen, Muzaffer Ege Alper, Jukka-Pekka Keskinen, Harri Kokkola, Antti Kukkurainen, Antti Lipponen, Jia Liu, Kalle Nordling, Antti-Ilari Partanen, Sami Romakkaniemi, Petri Räisänen, Juha Tonttila, and Hannele Korhonen
Atmos. Chem. Phys., 22, 4523–4537, https://doi.org/10.5194/acp-22-4523-2022, https://doi.org/10.5194/acp-22-4523-2022, 2022
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Clouds are important for the climate, and cloud droplets have a significant role in cloud properties. Cloud droplets form when air rises and cools and water vapour condenses on small particles that can be natural or of anthropogenic origin. Currently, the updraft velocity, meaning how fast the air rises, is poorly represented in global climate models. In our study, we show three methods that will improve the depiction of updraft velocity and which properties are vital to updrafts.
Xiaoxia Shang, Holger Baars, Iwona S. Stachlewska, Ina Mattis, and Mika Komppula
Atmos. Chem. Phys., 22, 3931–3944, https://doi.org/10.5194/acp-22-3931-2022, https://doi.org/10.5194/acp-22-3931-2022, 2022
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This study reports pollen observations at four lidar stations (Hohenpeißenberg, Germany; Kuopio, Finland; Leipzig, Germany; and Warsaw, Poland) during the intensive observation campaign organized in May 2020. A novel simple method for the characterization of the pure pollen is proposed, based on lidar measurements. It was applied to evaluate the pollen depolarization ratio and for the aerosol classifications.
Tomi Raatikainen, Marje Prank, Jaakko Ahola, Harri Kokkola, Juha Tonttila, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 3763–3778, https://doi.org/10.5194/acp-22-3763-2022, https://doi.org/10.5194/acp-22-3763-2022, 2022
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Mineral dust or similar ice-nucleating particles (INPs) are needed to initiate cloud droplet freezing at temperatures common in shallow clouds. In this work we examine how INPs that are released from the sea surface impact marine clouds. Our high-resolution simulations show that turbulent updraughts carry these particles effectively up to the clouds, where they initiate cloud droplet freezing. Sea surface INP emissions become more important with decreasing background dust INP concentrations.
Jessica Slater, Hugh Coe, Gordon McFiggans, Juha Tonttila, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 2937–2953, https://doi.org/10.5194/acp-22-2937-2022, https://doi.org/10.5194/acp-22-2937-2022, 2022
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This paper shows the specific impact of black carbon (BC) on the aerosol–planetary boundary layer (PBL) feedback and its influence on a Beijing haze episode. Overall, this paper shows that strong temperature inversions prevent BC heating within the PBL from significantly increasing PBL height, while BC above the PBL suppresses PBL development significantly through the day. From this we suggest a method by which both locally and regionally emitted BC may impact urban pollution episodes.
Kimmo Korhonen, Thomas Bjerring Kristensen, John Falk, Vilhelm B. Malmborg, Axel Eriksson, Louise Gren, Maja Novakovic, Sam Shamun, Panu Karjalainen, Lassi Markkula, Joakim Pagels, Birgitta Svenningsson, Martin Tunér, Mika Komppula, Ari Laaksonen, and Annele Virtanen
Atmos. Chem. Phys., 22, 1615–1631, https://doi.org/10.5194/acp-22-1615-2022, https://doi.org/10.5194/acp-22-1615-2022, 2022
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We investigated the ice-nucleating abilities of particulate emissions from a modern diesel engine using the portable ice-nuclei counter SPIN, a continuous-flow diffusion chamber instrument. Three different fuels were studied without blending, including fossil diesel and two renewable fuels, testing different emission aftertreatment systems and photochemical aging. We found that the diesel emissions were inefficient ice nuclei, and aging had no or little effect on their ice-nucleating abilities.
Jutta Kesti, John Backman, Ewan J. O'Connor, Anne Hirsikko, Eija Asmi, Minna Aurela, Ulla Makkonen, Maria Filioglou, Mika Komppula, Hannele Korhonen, and Heikki Lihavainen
Atmos. Chem. Phys., 22, 481–503, https://doi.org/10.5194/acp-22-481-2022, https://doi.org/10.5194/acp-22-481-2022, 2022
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In this study we combined aerosol particle measurements at the surface with a scanning Doppler lidar providing vertical profiles of the atmosphere to study the effect of different boundary layer conditions on aerosol particle properties in the understudied Arabian Peninsula region. The instrumentation used in this study enabled us to identify periods when pollution from remote sources was mixed down to the surface and initiated new particle formation in the growing boundary layer.
Ian Boutle, Wayne Angevine, Jian-Wen Bao, Thierry Bergot, Ritthik Bhattacharya, Andreas Bott, Leo Ducongé, Richard Forbes, Tobias Goecke, Evelyn Grell, Adrian Hill, Adele L. Igel, Innocent Kudzotsa, Christine Lac, Bjorn Maronga, Sami Romakkaniemi, Juerg Schmidli, Johannes Schwenkel, Gert-Jan Steeneveld, and Benoît Vié
Atmos. Chem. Phys., 22, 319–333, https://doi.org/10.5194/acp-22-319-2022, https://doi.org/10.5194/acp-22-319-2022, 2022
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Fog forecasting is one of the biggest problems for numerical weather prediction. By comparing many models used for fog forecasting with others used for fog research, we hoped to help guide forecast improvements. We show some key processes that, if improved, will help improve fog forecasting, such as how water is deposited on the ground. We also showed that research models were not themselves a suitable baseline for comparison, and we discuss what future observations are required to improve them.
Xiaoxia Shang, Tero Mielonen, Antti Lipponen, Elina Giannakaki, Ari Leskinen, Virginie Buchard, Anton S. Darmenov, Antti Kukkurainen, Antti Arola, Ewan O'Connor, Anne Hirsikko, and Mika Komppula
Atmos. Meas. Tech., 14, 6159–6179, https://doi.org/10.5194/amt-14-6159-2021, https://doi.org/10.5194/amt-14-6159-2021, 2021
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The long-range-transported smoke particles from a Canadian wildfire event were observed with a multi-wavelength Raman polarization lidar and a ceilometer over Kuopio, Finland, in June 2019. The optical properties and the mass concentration estimations were reported for such aged smoke aerosols over northern Europe.
Antti Hellsten, Klaus Ketelsen, Matthias Sühring, Mikko Auvinen, Björn Maronga, Christoph Knigge, Fotios Barmpas, Georgios Tsegas, Nicolas Moussiopoulos, and Siegfried Raasch
Geosci. Model Dev., 14, 3185–3214, https://doi.org/10.5194/gmd-14-3185-2021, https://doi.org/10.5194/gmd-14-3185-2021, 2021
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Large-eddy simulation (LES) of the urban atmospheric boundary layer involves a large separation of turbulent scales, leading to prohibitive computational costs. An online LES–LES nesting scheme is implemented into the PALM model system 6.0 to overcome this problem. Test results show that the accuracy within the high-resolution nest domains approach the non-nested high-resolution reference results. The nesting can reduce the CPU by time up to 80 % compared to the fine-resolution reference runs.
Stephanie Bohlmann, Xiaoxia Shang, Ville Vakkari, Elina Giannakaki, Ari Leskinen, Kari E. J. Lehtinen, Sanna Pätsi, and Mika Komppula
Atmos. Chem. Phys., 21, 7083–7097, https://doi.org/10.5194/acp-21-7083-2021, https://doi.org/10.5194/acp-21-7083-2021, 2021
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Measurements of the multi-wavelength Raman polarization lidar PollyXT and a Halo Photonics StreamLine Doppler lidar have been combined with measurements of pollen type and concentration using a traditional pollen trap at the rural forest site in Vehmasmäki, Finland. Depolarization ratios were measured at three wavelengths. High depolarization ratios were detected during an event with high birch and spruce pollen concentrations and a wavelength dependence of the depolarization ratio was observed.
Ville Vakkari, Holger Baars, Stephanie Bohlmann, Johannes Bühl, Mika Komppula, Rodanthi-Elisavet Mamouri, and Ewan James O'Connor
Atmos. Chem. Phys., 21, 5807–5820, https://doi.org/10.5194/acp-21-5807-2021, https://doi.org/10.5194/acp-21-5807-2021, 2021
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The depolarization ratio is a valuable parameter for aerosol categorization from remote sensing measurements. Here, we introduce particle depolarization ratio measurements at the 1565 nm wavelength, which is substantially longer than previously utilized wavelengths and enhances our capabilities to study the wavelength dependency of the particle depolarization ratio.
Maria Mylonaki, Elina Giannakaki, Alexandros Papayannis, Christina-Anna Papanikolaou, Mika Komppula, Doina Nicolae, Nikolaos Papagiannopoulos, Aldo Amodeo, Holger Baars, and Ourania Soupiona
Atmos. Chem. Phys., 21, 2211–2227, https://doi.org/10.5194/acp-21-2211-2021, https://doi.org/10.5194/acp-21-2211-2021, 2021
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We introduce an automated aerosol type classification method, SCAN. The output of SCAN is compared with two aerosol classification methods: (1) the Mahalanobis distance automatic aerosol type classification and (2) a neural network aerosol typing algorithm. A total of 97 free tropospheric aerosol layers from four EARLINET stations in the period 2014–2018 were classified.
Antti Ruuskanen, Sami Romakkaniemi, Harri Kokkola, Antti Arola, Santtu Mikkonen, Harri Portin, Annele Virtanen, Kari E. J. Lehtinen, Mika Komppula, and Ari Leskinen
Atmos. Chem. Phys., 21, 1683–1695, https://doi.org/10.5194/acp-21-1683-2021, https://doi.org/10.5194/acp-21-1683-2021, 2021
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The study focuses mainly on cloud-scavenging efficiency of absorbing particulate matter (mainly black carbon) but additionally covers cloud-scavenging efficiency of scattering particles and statistics of cloud condensation nuclei. The main findings give insight into how black carbon is distributed in different particle sizes and the sensitivity to cloud scavenged. The main findings are useful for large-scale modelling for evaluating cloud scavenging.
Juha Tonttila, Ali Afzalifar, Harri Kokkola, Tomi Raatikainen, Hannele Korhonen, and Sami Romakkaniemi
Atmos. Chem. Phys., 21, 1035–1048, https://doi.org/10.5194/acp-21-1035-2021, https://doi.org/10.5194/acp-21-1035-2021, 2021
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The focus of this study is on rain enhancement by deliberate injection of small particles into clouds (
cloud seeding). The particles, usually released from an aircraft, are expected to enhance cloud droplet growth, but its practical feasibility is somewhat uncertain. To improve upon this, we simulate the seeding effects with a numerical model. The model reproduces the main features seen in field observations, with a strong sensitivity to the total mass of the injected particle material.
Xiaoxia Shang, Elina Giannakaki, Stephanie Bohlmann, Maria Filioglou, Annika Saarto, Antti Ruuskanen, Ari Leskinen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 15323–15339, https://doi.org/10.5194/acp-20-15323-2020, https://doi.org/10.5194/acp-20-15323-2020, 2020
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Measurements of the multi-wavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at a rural forest site in Kuopio, Finland. The depolarization ratio was enhanced when there were pollen grains in the atmosphere, illustrating the potential of lidar to track pollen grains in the atmosphere. The depolarization ratio of pure pollen particles was assessed for birch and pine pollen using a novel algorithm.
Eemeli Holopainen, Harri Kokkola, Anton Laakso, and Thomas Kühn
Geosci. Model Dev., 13, 6215–6235, https://doi.org/10.5194/gmd-13-6215-2020, https://doi.org/10.5194/gmd-13-6215-2020, 2020
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This paper introduces an in-cloud wet deposition scheme for liquid and ice phase clouds for global aerosol–climate models. With the default setup, our wet deposition scheme behaves spuriously and better representation can be achieved with this scheme when black carbon is mixed with soluble compounds at emission time. This work is done as many of the global models fail to reproduce the transport of black carbon to the Arctic, which may be due to the poor representation of wet removal in models.
Mona Kurppa, Pontus Roldin, Jani Strömberg, Anna Balling, Sasu Karttunen, Heino Kuuluvainen, Jarkko V. Niemi, Liisa Pirjola, Topi Rönkkö, Hilkka Timonen, Antti Hellsten, and Leena Järvi
Geosci. Model Dev., 13, 5663–5685, https://doi.org/10.5194/gmd-13-5663-2020, https://doi.org/10.5194/gmd-13-5663-2020, 2020
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High-resolution modelling is needed to solve the aerosol concentrations in a complex urban area. Here, the performance of an aerosol module within the PALM model to simulate the detailed horizontal and vertical distribution of aerosol particles is studied. Further, sensitivity to the meteorological and aerosol boundary conditions is assessed using both model and observation data. The horizontal distribution is sensitive to the wind speed and stability, and the vertical to the wind direction.
Santtu Mikkonen, Zoltán Németh, Veronika Varga, Tamás Weidinger, Ville Leinonen, Taina Yli-Juuti, and Imre Salma
Atmos. Chem. Phys., 20, 12247–12263, https://doi.org/10.5194/acp-20-12247-2020, https://doi.org/10.5194/acp-20-12247-2020, 2020
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We determined decennial statistical time trends and diurnal statistical patterns of atmospheric particle number concentrations in various relevant size fractions in the city centre of Budapest in an interval of 2008–2018. The mean overall decrease rate of particles in different size fractions was approximately −5 % scaled for the 10-year measurement interval. The decline can be interpreted as a consequence of the decreased anthropogenic emissions in the city.
Jessica Slater, Juha Tonttila, Gordon McFiggans, Paul Connolly, Sami Romakkaniemi, Thomas Kühn, and Hugh Coe
Atmos. Chem. Phys., 20, 11893–11906, https://doi.org/10.5194/acp-20-11893-2020, https://doi.org/10.5194/acp-20-11893-2020, 2020
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The feedback effect between aerosol particles, radiation and meteorology reduces turbulent motion and results in increased surface aerosol concentrations during Beijing haze. Observational analysis and regional modelling studies have examined the feedback effect but these studies are limited. In this work, we set up a high-resolution model for the Beijing environment to examine the sensitivity of the aerosol feedback effect to initial meteorological conditions and aerosol loading.
Jaakko Ahola, Hannele Korhonen, Juha Tonttila, Sami Romakkaniemi, Harri Kokkola, and Tomi Raatikainen
Atmos. Chem. Phys., 20, 11639–11654, https://doi.org/10.5194/acp-20-11639-2020, https://doi.org/10.5194/acp-20-11639-2020, 2020
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In this study, we present an improved cloud model that reproduces the behaviour of mixed-phase clouds containing liquid droplets and ice crystals in more detail than before. This model is a convenient computational tool that enables the study of phenomena that cannot fit into a laboratory. These clouds have a significant role in climate, but they are not yet properly understood. Here, we show the advantages of the new model in a case study focusing on Arctic mixed-phase clouds.
Konstantinos-Matthaios Doulgeris, Mika Komppula, Sami Romakkaniemi, Antti-Pekka Hyvärinen, Veli-Matti Kerminen, and David Brus
Atmos. Meas. Tech., 13, 5129–5147, https://doi.org/10.5194/amt-13-5129-2020, https://doi.org/10.5194/amt-13-5129-2020, 2020
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We intercompared three cloud spectrometers ground setups in conditions with frequently occurring supercooled clouds. The measurements were conducted during the Pallas Cloud Experiment (PaCE) in 2013, in the Finnish sub-Arctic region at Sammaltunturi station. The main meteorological parameters influencing the spectrometers' performance was the wind direction. Final recommendations and our view on the main limitations of each spectrometer ground setup are presented.
Innocent Kudzotsa, Harri Kokkola, Juha Tonttila, Tomi Raatikainen, and Sami Romakkaniemi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-851, https://doi.org/10.5194/acp-2020-851, 2020
Publication in ACP not foreseen
Maria Filioglou, Elina Giannakaki, John Backman, Jutta Kesti, Anne Hirsikko, Ronny Engelmann, Ewan O'Connor, Jari T. T. Leskinen, Xiaoxia Shang, Hannele Korhonen, Heikki Lihavainen, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 20, 8909–8922, https://doi.org/10.5194/acp-20-8909-2020, https://doi.org/10.5194/acp-20-8909-2020, 2020
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Dust optical properties are region-dependent. Saharan, Asian, and Arabian dusts do not pose similar optical properties in terms of lidar ratios; thus, a universal lidar ratio for dust particles will lead to biases. The present study analyses observations over the United Arab Emirates, quantifying the optical and geometrical extents of the aerosol layers in the area, providing at the same time the Arabian dust properties along with chemical analysis of dust samples collected in the region.
Sini Isokääntä, Eetu Kari, Angela Buchholz, Liqing Hao, Siegfried Schobesberger, Annele Virtanen, and Santtu Mikkonen
Atmos. Meas. Tech., 13, 2995–3022, https://doi.org/10.5194/amt-13-2995-2020, https://doi.org/10.5194/amt-13-2995-2020, 2020
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Online mass spectrometry produces large amounts of data. These data can be interpreted with statistical methods, enabling scientists to more easily understand the underlying processes. We compared these techniques on car exhaust measurements. We show differences and similarities between the methods and give recommendations on applicability of the methods on certain types of data. We show that applying multiple methods leads to more robust results, thus increasing reliability of the findings.
Thomas Kühn, Kaarle Kupiainen, Tuuli Miinalainen, Harri Kokkola, Ville-Veikko Paunu, Anton Laakso, Juha Tonttila, Rita Van Dingenen, Kati Kulovesi, Niko Karvosenoja, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 20, 5527–5546, https://doi.org/10.5194/acp-20-5527-2020, https://doi.org/10.5194/acp-20-5527-2020, 2020
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We investigate the effects of black carbon (BC) mitigation on Arctic climate and human health, accounting for the concurrent reduction of other aerosol species. While BC is attributed a net warming effect on climate, most other aerosol species cool the planet. We find that the direct radiative effect of mitigating BC induces cooling, while aerosol–cloud effects offset this cooling and introduce large uncertainties. Furthermore, the reduced aerosol emissions reduce human mortality considerably.
Kimmo Korhonen, Thomas Bjerring Kristensen, John Falk, Robert Lindgren, Christina Andersen, Ricardo Luis Carvalho, Vilhelm Malmborg, Axel Eriksson, Christoffer Boman, Joakim Pagels, Birgitta Svenningsson, Mika Komppula, Kari E. J. Lehtinen, and Annele Virtanen
Atmos. Chem. Phys., 20, 4951–4968, https://doi.org/10.5194/acp-20-4951-2020, https://doi.org/10.5194/acp-20-4951-2020, 2020
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Ice-nucleating abilities of particulate emissions from solid-fuel-burning cookstoves were studied using a portable ice nuclei counter in an extensive laboratory experiment campaign. We found that even small changes in combustion conditions may affect the ice-nucleating ability of the emissions significantly. Also six different physico-chemical properties of the emissions were studied, but no clear correlation to their ice-nucleating ability was found.
Kalliopi Artemis Voudouri, Elina Giannakaki, Mika Komppula, and Dimitris Balis
Atmos. Chem. Phys., 20, 4427–4444, https://doi.org/10.5194/acp-20-4427-2020, https://doi.org/10.5194/acp-20-4427-2020, 2020
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In this paper we present the variability in cirrus cloud properties using a PollyXT Raman lidar over high and tropical latitudes. The kind of information presented here can be rather useful in the cirrus parameterisations required as input to radiative transfer models and can be a complementary tool for satellite products that cannot provide cloud vertical structure.
Björn Maronga, Sabine Banzhaf, Cornelia Burmeister, Thomas Esch, Renate Forkel, Dominik Fröhlich, Vladimir Fuka, Katrin Frieda Gehrke, Jan Geletič, Sebastian Giersch, Tobias Gronemeier, Günter Groß, Wieke Heldens, Antti Hellsten, Fabian Hoffmann, Atsushi Inagaki, Eckhard Kadasch, Farah Kanani-Sühring, Klaus Ketelsen, Basit Ali Khan, Christoph Knigge, Helge Knoop, Pavel Krč, Mona Kurppa, Halim Maamari, Andreas Matzarakis, Matthias Mauder, Matthias Pallasch, Dirk Pavlik, Jens Pfafferott, Jaroslav Resler, Sascha Rissmann, Emmanuele Russo, Mohamed Salim, Michael Schrempf, Johannes Schwenkel, Gunther Seckmeyer, Sebastian Schubert, Matthias Sühring, Robert von Tils, Lukas Vollmer, Simon Ward, Björn Witha, Hauke Wurps, Julian Zeidler, and Siegfried Raasch
Geosci. Model Dev., 13, 1335–1372, https://doi.org/10.5194/gmd-13-1335-2020, https://doi.org/10.5194/gmd-13-1335-2020, 2020
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In this paper, we describe the PALM model system 6.0. PALM is a Fortran-based turbulence-resolving code and has been applied for studying a variety of atmospheric and oceanic boundary layers for about 20 years. The model is optimized for use on massively parallel computer architectures. During the last years, PALM has been significantly improved and now offers a variety of new components that are especially designed to simulate the urban atmosphere at building-resolving resolution.
Elina Giannakaki, Panos Kokkalis, Eleni Marinou, Nikolaos S. Bartsotas, Vassilis Amiridis, Albert Ansmann, and Mika Komppula
Atmos. Meas. Tech., 13, 893–905, https://doi.org/10.5194/amt-13-893-2020, https://doi.org/10.5194/amt-13-893-2020, 2020
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A new method, called ElEx, is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. Comparisons with both Raman lidar profiles during nightime and sun photometer daytime aerosol optical depth observations demonstrate the potential of the ElEx methodology.
Ville Leinonen, Petri Tiitta, Olli Sippula, Hendryk Czech, Ari Leskinen, Juha Karvanen, Sini Isokääntä, and Santtu Mikkonen
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-13, https://doi.org/10.5194/gmd-2020-13, 2020
Revised manuscript not accepted
Stephanie Bohlmann, Xiaoxia Shang, Elina Giannakaki, Maria Filioglou, Annika Saarto, Sami Romakkaniemi, and Mika Komppula
Atmos. Chem. Phys., 19, 14559–14569, https://doi.org/10.5194/acp-19-14559-2019, https://doi.org/10.5194/acp-19-14559-2019, 2019
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Measurements of the multiwavelength Raman polarization lidar PollyXT have been combined with measurements of pollen type and concentration using a traditional pollen sampler at the rural forest site in Vehmasmäki, Finland. High particle depolarization ratios were observed during an intense pollination event of birch pollen occasionally mixed with spruce pollen. Our observations illustrate the potential of the particle depolarization ratio to track pollen grains in the atmosphere.
Anina Gilgen, Stiig Wilkenskjeld, Jed O. Kaplan, Thomas Kühn, and Ulrike Lohmann
Clim. Past, 15, 1885–1911, https://doi.org/10.5194/cp-15-1885-2019, https://doi.org/10.5194/cp-15-1885-2019, 2019
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Using the global aerosol–climate model ECHAM-HAM-SALSA, the effect of humans on European climate in the Roman Empire was quantified. Both land use and novel estimates of anthropogenic aerosol emissions were considered. We conducted simulations with fixed sea-surface temperatures to gain a first impression about the anthropogenic impact. While land use effects induced a regional warming for one of the reconstructions, aerosol emissions led to a cooling associated with aerosol–cloud interactions.
Santtu Mikkonen, Mikko R. A. Pitkänen, Tuomo Nieminen, Antti Lipponen, Sini Isokääntä, Antti Arola, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 19, 12531–12543, https://doi.org/10.5194/acp-19-12531-2019, https://doi.org/10.5194/acp-19-12531-2019, 2019
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Atmospheric measurement data never come without measurement error. Too often, these errors are neglected when researchers make inferences from their data. We applied multiple line-fitting methods to simulated data mimicking two central variables in aerosol research. Our results show that an ordinary least squares fit, typically used to describe relationships, underestimates the slope of the fit and that methods taking the measurement uncertainty into account performed significantly better.
Sieglinde Callewaert, Sophie Vandenbussche, Nicolas Kumps, Arve Kylling, Xiaoxia Shang, Mika Komppula, Philippe Goloub, and Martine De Mazière
Atmos. Meas. Tech., 12, 3673–3698, https://doi.org/10.5194/amt-12-3673-2019, https://doi.org/10.5194/amt-12-3673-2019, 2019
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This article presents the updated MAPIR algorithm, which uses infrared satellite data to obtain the global 3-D distribution of mineral aerosols. A description of the method together with its technical improvements is given. Additionally, a 10-year data set was generated and used to evaluate this new algorithm against AERONET, CALIOP, CATS and two ground-based lidar stations. We have shown that the new MAPIR algorithm provides reliable aerosol optical depth and dust layer mean altitude profiles.
Konstantina Nakoudi, Elina Giannakaki, Aggeliki Dandou, Maria Tombrou, and Mika Komppula
Atmos. Meas. Tech., 12, 2595–2610, https://doi.org/10.5194/amt-12-2595-2019, https://doi.org/10.5194/amt-12-2595-2019, 2019
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We characterized the height of the boundary layer (BLH) over New Delhi for almost a year using ground and satellite lidar measurements as well as model simulations. In the presence of multiple aerosol layers, the employed algorithm was very efficient. Due to prevailing meteorological conditions, the seasonal BLH cycle was slightly weaker than the one expected from the climatology. The aim was to assess the feasibility of the employed algorithm and compare the results to independent sources.
Mona Kurppa, Antti Hellsten, Pontus Roldin, Harri Kokkola, Juha Tonttila, Mikko Auvinen, Christoph Kent, Prashant Kumar, Björn Maronga, and Leena Järvi
Geosci. Model Dev., 12, 1403–1422, https://doi.org/10.5194/gmd-12-1403-2019, https://doi.org/10.5194/gmd-12-1403-2019, 2019
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This paper describes the implementation of a sectional aerosol module, SALSA, into the PALM model system 6.0. The first evaluation study shows excellent agreements with measurements. Furthermore, we show that ignoring the dry deposition of aerosol particles can overestimate aerosol number concentrations by 20 %, whereas condensation and dissolutional growth increase the total aerosol mass by over 10 % in this specific urban environment.
Liqing Hao, Olga Garmash, Mikael Ehn, Pasi Miettinen, Paola Massoli, Santtu Mikkonen, Tuija Jokinen, Pontus Roldin, Pasi Aalto, Taina Yli-Juuti, Jorma Joutsensaari, Tuukka Petäjä, Markku Kulmala, Kari E. J. Lehtinen, Douglas R. Worsnop, and Annele Virtanen
Atmos. Chem. Phys., 18, 17705–17716, https://doi.org/10.5194/acp-18-17705-2018, https://doi.org/10.5194/acp-18-17705-2018, 2018
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An aerosol mass spectrometer was used to characterize aerosol chemical composition during new particle formation periods. The time profiles of mass concentrations and chemical composition of observed aerosol particles are subjected to joint effects of boundary layer dilution, atmospheric chemistry and aerosol mixing in different boundary layers. During the nighttime, the increase in organic aerosol mass correlated well with the increase in condensed highly oxygenated organic molecules' mass.
Harri Kokkola, Thomas Kühn, Anton Laakso, Tommi Bergman, Kari E. J. Lehtinen, Tero Mielonen, Antti Arola, Scarlet Stadtler, Hannele Korhonen, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Ina Tegen, Colombe Siegenthaler-Le Drian, Martin G. Schultz, Isabelle Bey, Philip Stier, Nikos Daskalakis, Colette L. Heald, and Sami Romakkaniemi
Geosci. Model Dev., 11, 3833–3863, https://doi.org/10.5194/gmd-11-3833-2018, https://doi.org/10.5194/gmd-11-3833-2018, 2018
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In this paper we present a global aerosol–chemistry–climate model with the focus on its representation for atmospheric aerosol particles. In the model, aerosols are simulated using the aerosol module SALSA2.0, which in this paper is compared to satellite, ground, and aircraft-based observations of the properties of atmospheric aerosol. Based on this study, the model simulated aerosol properties compare well with the observations.
Scarlet Stadtler, Thomas Kühn, Sabine Schröder, Domenico Taraborrelli, Martin G. Schultz, and Harri Kokkola
Geosci. Model Dev., 11, 3235–3260, https://doi.org/10.5194/gmd-11-3235-2018, https://doi.org/10.5194/gmd-11-3235-2018, 2018
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Atmospheric aerosols interact with our climate system and have adverse health effects. Nevertheless, these particles are a source of uncertainty in climate projections and the formation process of secondary aerosols formed by organic gas-phase precursors is particularly not fully understood. In order to gain a deeper understanding of secondary organic aerosol formation, this model system explicitly represents gas-phase and aerosol formation processes. Finally, this allows for process discussion.
Robin G. Stevens, Katharina Loewe, Christopher Dearden, Antonios Dimitrelos, Anna Possner, Gesa K. Eirund, Tomi Raatikainen, Adrian A. Hill, Benjamin J. Shipway, Jonathan Wilkinson, Sami Romakkaniemi, Juha Tonttila, Ari Laaksonen, Hannele Korhonen, Paul Connolly, Ulrike Lohmann, Corinna Hoose, Annica M. L. Ekman, Ken S. Carslaw, and Paul R. Field
Atmos. Chem. Phys., 18, 11041–11071, https://doi.org/10.5194/acp-18-11041-2018, https://doi.org/10.5194/acp-18-11041-2018, 2018
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We perform a model intercomparison of summertime high Arctic clouds. Observed concentrations of aerosol particles necessary for cloud formation fell to extremely low values, coincident with a transition from cloudy to nearly cloud-free conditions. Previous analyses have suggested that at these low concentrations, the radiative properties of the clouds are determined primarily by these particle concentrations. The model results strongly support this hypothesis.
Lauri Laakso, Santtu Mikkonen, Achim Drebs, Anu Karjalainen, Pentti Pirinen, and Pekka Alenius
Ocean Sci., 14, 617–632, https://doi.org/10.5194/os-14-617-2018, https://doi.org/10.5194/os-14-617-2018, 2018
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Meteorological observations at Utö Atmospheric and Marine Research Station, the Baltic Sea, started in 1881 and seawater temperature and salinity observations in 1900. Based on the dataset of more than 100 years of observations, we see an increase in atmospheric temperature after the 1980s, in line with reduced sea ice cover. We also found an increase in seawater temperatures, modulated by changes in salinities. The results indicate that the climate at Utö may have shifted into a new phase.
Jorma Joutsensaari, Matthew Ozon, Tuomo Nieminen, Santtu Mikkonen, Timo Lähivaara, Stefano Decesari, M. Cristina Facchini, Ari Laaksonen, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 18, 9597–9615, https://doi.org/10.5194/acp-18-9597-2018, https://doi.org/10.5194/acp-18-9597-2018, 2018
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New particle formation (NPF) in the atmosphere is globally an important source of aerosol particles. NPF events are typically identified and analyzed manually by researchers from particle size distribution data day by day, which is time consuming and might be inconsistent. We have developed an automatic analysis method based on deep learning for NPF event identification. The developed method can be easily utilized to analyze any long-term datasets more accurately and consistently.
Ian Boutle, Jeremy Price, Innocent Kudzotsa, Harri Kokkola, and Sami Romakkaniemi
Atmos. Chem. Phys., 18, 7827–7840, https://doi.org/10.5194/acp-18-7827-2018, https://doi.org/10.5194/acp-18-7827-2018, 2018
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Aerosol processes are a key mechanism in the development of fog. Poor representation of aerosol–fog interaction can result in large biases in fog forecasts, such as surface temperatures which are too high and fog which is too deep and long lived. A relatively simple representation of aerosol–fog interaction can actually lead to significant improvements in forecasting. Aerosol–fog interaction can have a large effect on the climate system but is poorly represented in climate models.
Martin G. Schultz, Scarlet Stadtler, Sabine Schröder, Domenico Taraborrelli, Bruno Franco, Jonathan Krefting, Alexandra Henrot, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Colombe Siegenthaler-Le Drian, Sebastian Wahl, Harri Kokkola, Thomas Kühn, Sebastian Rast, Hauke Schmidt, Philip Stier, Doug Kinnison, Geoffrey S. Tyndall, John J. Orlando, and Catherine Wespes
Geosci. Model Dev., 11, 1695–1723, https://doi.org/10.5194/gmd-11-1695-2018, https://doi.org/10.5194/gmd-11-1695-2018, 2018
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The chemistry–climate model ECHAM-HAMMOZ contains a detailed representation of tropospheric and stratospheric reactive chemistry and state-of-the-art parameterizations of aerosols. It thus allows for detailed investigations of chemical processes in the climate system. Evaluation of the model with various observational data yields good results, but the model has a tendency to produce too much OH in the tropics. This highlights the important interplay between atmospheric chemistry and dynamics.
Antti Lipponen, Tero Mielonen, Mikko R. A. Pitkänen, Robert C. Levy, Virginia R. Sawyer, Sami Romakkaniemi, Ville Kolehmainen, and Antti Arola
Atmos. Meas. Tech., 11, 1529–1547, https://doi.org/10.5194/amt-11-1529-2018, https://doi.org/10.5194/amt-11-1529-2018, 2018
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Atmospheric aerosols are small solid or liquid particles suspended in the atmosphere and they have a significant effect on the climate. Satellite data are used to get global estimates of atmospheric aerosols. In this work, a statistics-based Bayesian aerosol retrieval algorithm was developed to improve the accuracy and quantify the uncertainties related to the aerosol estimates. The algorithm is tested with NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) satellite data.
Mikko Auvinen, Leena Järvi, Antti Hellsten, Üllar Rannik, and Timo Vesala
Geosci. Model Dev., 10, 4187–4205, https://doi.org/10.5194/gmd-10-4187-2017, https://doi.org/10.5194/gmd-10-4187-2017, 2017
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Correct spatial interpretation of a micrometeorological measurement requires the determination of its effective source area, or footprint. In urban areas the use of analytical models becomes highly questionable. This work introduces a computational methodology that enables the generation of footprints for complex urban sites. The methodology is based on conducting high-resolution flow and particle analysis on a model that features a detailed topographic description of a real city environment.
Elham Baranizadeh, Tuomo Nieminen, Taina Yli-Juuti, Markku Kulmala, Tuukka Petäjä, Ari Leskinen, Mika Komppula, Ari Laaksonen, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 17, 13361–13371, https://doi.org/10.5194/acp-17-13361-2017, https://doi.org/10.5194/acp-17-13361-2017, 2017
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Extrapolation of the particle formation rates from one measured larger size (e.g., 7 nm) to smaller sizes (e.g., 3 nm) based on simplified growth-scavenging dynamics works fairly well to estimate mean daily formation rates, but it fails to predict the time evolution of the particle population. This points to the challenges in predicting atmospheric nucleation rates for locations where the particle growth and loss rates are size- and time-dependent.
Maria Filioglou, Anna Nikandrova, Sami Niemelä, Holger Baars, Tero Mielonen, Ari Leskinen, David Brus, Sami Romakkaniemi, Elina Giannakaki, and Mika Komppula
Atmos. Meas. Tech., 10, 4303–4316, https://doi.org/10.5194/amt-10-4303-2017, https://doi.org/10.5194/amt-10-4303-2017, 2017
Anton Laakso, Hannele Korhonen, Sami Romakkaniemi, and Harri Kokkola
Atmos. Chem. Phys., 17, 6957–6974, https://doi.org/10.5194/acp-17-6957-2017, https://doi.org/10.5194/acp-17-6957-2017, 2017
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Based on simulations, equatorial stratospheric sulfur injections have shown to be an efficient strategy to counteract ongoing global warming. However, equatorial injections would result in relatively larger cooling in low latitudes than in high latitudes. This together with greenhouse-gas-induced warming would lead to cooling in the Equator and warming in the high latitudes. Results of this study show that a more optimal cooling effect is achieved by varying the injection area seasonally.
S. Wittke, K. Karila, E. Puttonen, A. Hellsten, M. Auvinen, and M. Karjalainen
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-1-W1, 425–431, https://doi.org/10.5194/isprs-archives-XLII-1-W1-425-2017, https://doi.org/10.5194/isprs-archives-XLII-1-W1-425-2017, 2017
Antti Arola, Thomas F. Eck, Harri Kokkola, Mikko R. A. Pitkänen, and Sami Romakkaniemi
Atmos. Chem. Phys., 17, 5991–6001, https://doi.org/10.5194/acp-17-5991-2017, https://doi.org/10.5194/acp-17-5991-2017, 2017
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One of the issues that hinder the measurement-based assessment of aerosol–cloud interactions by remote sensing methods is that typically aerosols and clouds cannot be measured simultaneously by passive remote sensing methods. AERONET includes the SDA product that provides the fine-mode AOD also in mixed cloud–aerosol observations. These measurements have not yet been fully exploited in studies of aerosol–cloud interactions. We applied SDA for this kind of analysis.
Juha Tonttila, Zubair Maalick, Tomi Raatikainen, Harri Kokkola, Thomas Kühn, and Sami Romakkaniemi
Geosci. Model Dev., 10, 169–188, https://doi.org/10.5194/gmd-10-169-2017, https://doi.org/10.5194/gmd-10-169-2017, 2017
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Novel techniques for modelling the aerosol–cloud interactions are implemented in a cloud-resolving model. The new methods improve the representation of the poorly constrained effects of cloud processing, precipitation and the wet removal of particles on the aerosol population and the associated feedbacks. The detailed representation of these processes yields more realistic simulation of the evolution of boundary layer clouds and fogs, as compared to results obtained using more simple methods.
Petri Tiitta, Ari Leskinen, Liqing Hao, Pasi Yli-Pirilä, Miika Kortelainen, Julija Grigonyte, Jarkko Tissari, Heikki Lamberg, Anni Hartikainen, Kari Kuuspalo, Aki-Matti Kortelainen, Annele Virtanen, Kari E. J. Lehtinen, Mika Komppula, Simone Pieber, André S. H. Prévôt, Timothy B. Onasch, Douglas R. Worsnop, Hendryk Czech, Ralf Zimmermann, Jorma Jokiniemi, and Olli Sippula
Atmos. Chem. Phys., 16, 13251–13269, https://doi.org/10.5194/acp-16-13251-2016, https://doi.org/10.5194/acp-16-13251-2016, 2016
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Real-time measurements of OA aging and SOA formation from logwood combustion were conducted under dark and UV oxidation. Substantial SOA formation was observed in all experiments, leading to twice the initial OA mass emphasizing the importance of the burning conditions for the aging processes. The results prove that emissions are subject to intensive chemical processing in the atmosphere; e.g. the most of the POA was found to become oxidized after the ozone addition, forming aged POA.
Aki Pajunoja, Weiwei Hu, Yu J. Leong, Nathan F. Taylor, Pasi Miettinen, Brett B. Palm, Santtu Mikkonen, Don R. Collins, Jose L. Jimenez, and Annele Virtanen
Atmos. Chem. Phys., 16, 11163–11176, https://doi.org/10.5194/acp-16-11163-2016, https://doi.org/10.5194/acp-16-11163-2016, 2016
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The phase state of ambient particles was inferred from bounce measurements conducted at a rural site in central Alabama during the SOAS campaign. The organic-dominated ambient particles are mostly in the liquid phase at summertime conditions but they turn semisolid when dried in the measurement setup. Bounce humidograms reveal that the hygroscopicity and oxidation of the particles decreases the liquefying RH. The effect of oxidation is emphasized by oxidation flow reactor measurements.
Elham Baranizadeh, Benjamin N. Murphy, Jan Julin, Saeed Falahat, Carly L. Reddington, Antti Arola, Lars Ahlm, Santtu Mikkonen, Christos Fountoukis, David Patoulias, Andreas Minikin, Thomas Hamburger, Ari Laaksonen, Spyros N. Pandis, Hanna Vehkamäki, Kari E. J. Lehtinen, and Ilona Riipinen
Geosci. Model Dev., 9, 2741–2754, https://doi.org/10.5194/gmd-9-2741-2016, https://doi.org/10.5194/gmd-9-2741-2016, 2016
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The molecular mechanisms through which new ultrafine (< 100 nm) aerosol particles are formed in the atmosphere have puzzled the scientific community for decades. In the past few years, however, significant progress has been made in unraveling these processes through laboratory studies and computational efforts. In this work we have implemented these new developments to an air quality model and study the implications of anthropogenically driven particle formation for European air quality.
Olli Väisänen, Antti Ruuskanen, Arttu Ylisirniö, Pasi Miettinen, Harri Portin, Liqing Hao, Ari Leskinen, Mika Komppula, Sami Romakkaniemi, Kari E. J. Lehtinen, and Annele Virtanen
Atmos. Chem. Phys., 16, 10385–10398, https://doi.org/10.5194/acp-16-10385-2016, https://doi.org/10.5194/acp-16-10385-2016, 2016
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In-cloud measurements of aerosol hygroscopicity and cloud droplet activation were conducted in Kuopio, Finland. According to the observations, the less hygroscopic accumulation mode particles were present in the non-activated aerosol, whereas the more hygroscopic particles were scavenged into cloud droplets. The results illustrate the sensitivity of cloud droplet formation to varying chemical composition and highlight the need for proper treatment of anthropogenic aerosols in CCN predictions.
Tero Mielonen, Anca Hienola, Thomas Kühn, Joonas Merikanto, Antti Lipponen, Tommi Bergman, Hannele Korhonen, Pekka Kolmonen, Larisa Sogacheva, Darren Ghent, Antti Arola, Gerrit de Leeuw, and Harri Kokkola
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-625, https://doi.org/10.5194/acp-2016-625, 2016
Revised manuscript not accepted
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We studied the temperature dependence of AOD and its radiative effects over the southeastern US. We used spaceborne observations of AOD, LST and tropospheric NO2 with simulations of ECHAM-HAMMOZ. The level of AOD in this region is governed by anthropogenic emissions but the temperature dependency is most likely caused by BVOC emissions. According to the observations and simulations, the regional clear-sky DRE for biogenic aerosols is −0.43 ± 0.88 W/m2/K and −0.86 ± 0.06 W/m2/K, respectively.
Jani Huttunen, Harri Kokkola, Tero Mielonen, Mika Esa Juhani Mononen, Antti Lipponen, Juha Reunanen, Anders Vilhelm Lindfors, Santtu Mikkonen, Kari Erkki Juhani Lehtinen, Natalia Kouremeti, Alkiviadis Bais, Harri Niska, and Antti Arola
Atmos. Chem. Phys., 16, 8181–8191, https://doi.org/10.5194/acp-16-8181-2016, https://doi.org/10.5194/acp-16-8181-2016, 2016
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For a good estimate of the current forcing by anthropogenic aerosols, knowledge in past is needed. One option to lengthen time series is to retrieve aerosol optical depth from solar radiation measurements. We have evaluated several methods for this task. Most of the methods produce aerosol optical depth estimates with a good accuracy. However, machine learning methods seem to be the most applicable not to produce any systematic biases, since they do not need constrain the aerosol properties.
Elina Giannakaki, Pieter G. van Zyl, Detlef Müller, Dimitris Balis, and Mika Komppula
Atmos. Chem. Phys., 16, 8109–8123, https://doi.org/10.5194/acp-16-8109-2016, https://doi.org/10.5194/acp-16-8109-2016, 2016
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Optical and microphysical properties of different aerosol types over South Africa measured with a multi-wavelength polarization Raman lidar are presented. Aerosol characterization of elevated layers was performed. This study could assist in bridging existing gaps relating to aerosol properties over South Africa.
Ronny Engelmann, Thomas Kanitz, Holger Baars, Birgit Heese, Dietrich Althausen, Annett Skupin, Ulla Wandinger, Mika Komppula, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Ina Mattis, Holger Linné, and Albert Ansmann
Atmos. Meas. Tech., 9, 1767–1784, https://doi.org/10.5194/amt-9-1767-2016, https://doi.org/10.5194/amt-9-1767-2016, 2016
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The atmospheric science community demands for autonomous and quality-assured vertically resolved measurements of aerosol and cloud properties. For this purpose, a portable lidar called Polly
was developed at TROPOS in 2003. This lidar type was continuously improved with gained experience from EARLINET, worldwide field campaigns, and institute collaborations within the last 10 years. We present recent changes to the setup of our portable multiwavelength Raman and polarization lidar PollyXT.
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
A. Arola, G. L. Schuster, M. R. A. Pitkänen, O. Dubovik, H. Kokkola, A. V. Lindfors, T. Mielonen, T. Raatikainen, S. Romakkaniemi, S. N. Tripathi, and H. Lihavainen
Atmos. Chem. Phys., 15, 12731–12740, https://doi.org/10.5194/acp-15-12731-2015, https://doi.org/10.5194/acp-15-12731-2015, 2015
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There have been relatively few measurement-based estimates for the direct radiative effect of brown carbon so far. This is first time that the direct radiative effect of brown carbon is estimated by exploiting the AERONET-retrieved imaginary indices. We estimated it for four sites in the Indo-Gangetic Plain: Karachi, Lahore,
Kanpur and Gandhi College.
J. Joutsensaari, P. Yli-Pirilä, H. Korhonen, A. Arola, J. D. Blande, J. Heijari, M. Kivimäenpää, S. Mikkonen, L. Hao, P. Miettinen, P. Lyytikäinen-Saarenmaa, C. L. Faiola, A. Laaksonen, and J. K. Holopainen
Atmos. Chem. Phys., 15, 12139–12157, https://doi.org/10.5194/acp-15-12139-2015, https://doi.org/10.5194/acp-15-12139-2015, 2015
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Global warming will induce large-scale insect outbreaks in boreal forests. Our results from field and laboratory experiments, satellite observations and global-scale modelling suggest that more frequent insect outbreaks, in addition to temperature-dependent increases in VOC emissions, could result in substantial increases in biogenic SOA formation and therefore affect both aerosol direct and indirect forcing of climate at regional scales. This should be considered in future climate predictions.
P. Zieger, P. P. Aalto, V. Aaltonen, M. Äijälä, J. Backman, J. Hong, M. Komppula, R. Krejci, M. Laborde, J. Lampilahti, G. de Leeuw, A. Pfüller, B. Rosati, M. Tesche, P. Tunved, R. Väänänen, and T. Petäjä
Atmos. Chem. Phys., 15, 7247–7267, https://doi.org/10.5194/acp-15-7247-2015, https://doi.org/10.5194/acp-15-7247-2015, 2015
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The effect of water uptake (hygroscopicity) on aerosol light scattering properties is generally lower for boreal aerosol due to the dominance of organic substances. A columnar optical closure study using ground-based and airborne measurements of aerosol optical, chemical and microphysical properties was conducted and the implications and limitations are discussed.
A. Leskinen, P. Yli-Pirilä, K. Kuuspalo, O. Sippula, P. Jalava, M.-R. Hirvonen, J. Jokiniemi, A. Virtanen, M. Komppula, and K. E. J. Lehtinen
Atmos. Meas. Tech., 8, 2267–2278, https://doi.org/10.5194/amt-8-2267-2015, https://doi.org/10.5194/amt-8-2267-2015, 2015
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A 29 m3 Teflon chamber was characterized and tested with oxidation experiments of toluene. Secondary organic aerosol yields of 12-42 % were obtained. These yields are comparable to those obtained in other laboratories.
J. Tonttila, E. J. O'Connor, A. Hellsten, A. Hirsikko, C. O'Dowd, H. Järvinen, and P. Räisänen
Atmos. Chem. Phys., 15, 5873–5885, https://doi.org/10.5194/acp-15-5873-2015, https://doi.org/10.5194/acp-15-5873-2015, 2015
E. Giannakaki, A. Pfüller, K. Korhonen, T. Mielonen, L. Laakso, V. Vakkari, H. Baars, R. Engelmann, J. P. Beukes, P. G. Van Zyl, M. Josipovic, P. Tiitta, K. Chiloane, S. Piketh, H. Lihavainen, K. E. J. Lehtinen, and M. Komppula
Atmos. Chem. Phys., 15, 5429–5442, https://doi.org/10.5194/acp-15-5429-2015, https://doi.org/10.5194/acp-15-5429-2015, 2015
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In this study we summarize 1 year of Raman lidar observations over South Africa. The analyses of lidar measurements presented here could assist in bridging existing gaps in the knowledge of vertical distribution of aerosols above South Africa, since limited long-term data of this type are available for this region. For the first time, we have been able to cover the full seasonal cycle on geometrical characteristics and optical properties of free tropospheric aerosol layers in the region.
M. Dalirian, H. Keskinen, L. Ahlm, A. Ylisirniö, S. Romakkaniemi, A. Laaksonen, A. Virtanen, and I. Riipinen
Atmos. Chem. Phys., 15, 3815–3829, https://doi.org/10.5194/acp-15-3815-2015, https://doi.org/10.5194/acp-15-3815-2015, 2015
J. Tonttila, H. Järvinen, and P. Räisänen
Atmos. Chem. Phys., 15, 703–714, https://doi.org/10.5194/acp-15-703-2015, https://doi.org/10.5194/acp-15-703-2015, 2015
E. M. Dunne, S. Mikkonen, H. Kokkola, and H. Korhonen
Atmos. Chem. Phys., 14, 13631–13642, https://doi.org/10.5194/acp-14-13631-2014, https://doi.org/10.5194/acp-14-13631-2014, 2014
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Marine clouds have a strong effect on the Earth's radiative balance. One proposed climate feedback is that, in a warming climate, marine aerosol emissions will change due to changing wind speeds. We have examined the processes that affect aerosol emissions and removal over 15 years, and high-temporal-resolution output over 2 months. We conclude that wind trends are unlikely to cause a strong feedback in marine regions, but changes in removal processes or transport from continental regions may.
L. Q. Hao, A. Kortelainen, S. Romakkaniemi, H. Portin, A. Jaatinen, A. Leskinen, M. Komppula, P. Miettinen, D. Sueper, A. Pajunoja, J. N. Smith, K. E. J. Lehtinen, D. R. Worsnop, A. Laaksonen, and A. Virtanen
Atmos. Chem. Phys., 14, 13483–13495, https://doi.org/10.5194/acp-14-13483-2014, https://doi.org/10.5194/acp-14-13483-2014, 2014
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Positive matrix factorization (PMF) was applied to the unified high-resolution mass spectra organic species with NO+ and NO2+ ions from the measurement in a mixed region between the boreal forestland and the urban area. The PMF analysis succeeded in separating the mixed spectra into three distinct organic factors and one inorganic factor. The particulate organic nitrate was distinguished by PMF for the first time, with a contribution of one-third of the total nitrate mass.
J.-P. Pietikäinen, S. Mikkonen, A. Hamed, A. I. Hienola, W. Birmili, M. Kulmala, and A. Laaksonen
Atmos. Chem. Phys., 14, 11711–11729, https://doi.org/10.5194/acp-14-11711-2014, https://doi.org/10.5194/acp-14-11711-2014, 2014
S. V. Henriksson, J.-P. Pietikäinen, A.-P. Hyvärinen, P. Räisänen, K. Kupiainen, J. Tonttila, R. Hooda, H. Lihavainen, D. O'Donnell, L. Backman, Z. Klimont, and A. Laaksonen
Atmos. Chem. Phys., 14, 10177–10192, https://doi.org/10.5194/acp-14-10177-2014, https://doi.org/10.5194/acp-14-10177-2014, 2014
J. Huttunen, A. Arola, G. Myhre, A. V. Lindfors, T. Mielonen, S. Mikkonen, J. S. Schafer, S. N. Tripathi, M. Wild, M. Komppula, and K. E. J. Lehtinen
Atmos. Chem. Phys., 14, 6103–6110, https://doi.org/10.5194/acp-14-6103-2014, https://doi.org/10.5194/acp-14-6103-2014, 2014
H. Portin, A. Leskinen, L. Hao, A. Kortelainen, P. Miettinen, A. Jaatinen, A. Laaksonen, K. E. J. Lehtinen, S. Romakkaniemi, and M. Komppula
Atmos. Chem. Phys., 14, 6021–6034, https://doi.org/10.5194/acp-14-6021-2014, https://doi.org/10.5194/acp-14-6021-2014, 2014
S. Romakkaniemi, A. Jaatinen, A. Laaksonen, A. Nenes, and T. Raatikainen
Atmos. Meas. Tech., 7, 1377–1384, https://doi.org/10.5194/amt-7-1377-2014, https://doi.org/10.5194/amt-7-1377-2014, 2014
A. Hirsikko, E. J. O'Connor, M. Komppula, K. Korhonen, A. Pfüller, E. Giannakaki, C. R. Wood, M. Bauer-Pfundstein, A. Poikonen, T. Karppinen, H. Lonka, M. Kurri, J. Heinonen, D. Moisseev, E. Asmi, V. Aaltonen, A. Nordbo, E. Rodriguez, H. Lihavainen, A. Laaksonen, K. E. J. Lehtinen, T. Laurila, T. Petäjä, M. Kulmala, and Y. Viisanen
Atmos. Meas. Tech., 7, 1351–1375, https://doi.org/10.5194/amt-7-1351-2014, https://doi.org/10.5194/amt-7-1351-2014, 2014
K. Korhonen, E. Giannakaki, T. Mielonen, A. Pfüller, L. Laakso, V. Vakkari, H. Baars, R. Engelmann, J. P. Beukes, P. G. Van Zyl, A. Ramandh, L. Ntsangwane, M. Josipovic, P. Tiitta, G. Fourie, I. Ngwana, K. Chiloane, and M. Komppula
Atmos. Chem. Phys., 14, 4263–4278, https://doi.org/10.5194/acp-14-4263-2014, https://doi.org/10.5194/acp-14-4263-2014, 2014
H. Kokkola, P. Yli-Pirilä, M. Vesterinen, H. Korhonen, H. Keskinen, S. Romakkaniemi, L. Hao, A. Kortelainen, J. Joutsensaari, D. R. Worsnop, A. Virtanen, and K. E. J. Lehtinen
Atmos. Chem. Phys., 14, 1689–1700, https://doi.org/10.5194/acp-14-1689-2014, https://doi.org/10.5194/acp-14-1689-2014, 2014
T. Korhola, H. Kokkola, H. Korhonen, A.-I. Partanen, A. Laaksonen, K. E. J. Lehtinen, and S. Romakkaniemi
Geosci. Model Dev., 7, 161–174, https://doi.org/10.5194/gmd-7-161-2014, https://doi.org/10.5194/gmd-7-161-2014, 2014
A. Lipponen, V. Kolehmainen, S. Romakkaniemi, and H. Kokkola
Geosci. Model Dev., 6, 2087–2098, https://doi.org/10.5194/gmd-6-2087-2013, https://doi.org/10.5194/gmd-6-2087-2013, 2013
J. Tonttila, P. Räisänen, and H. Järvinen
Atmos. Chem. Phys., 13, 7551–7565, https://doi.org/10.5194/acp-13-7551-2013, https://doi.org/10.5194/acp-13-7551-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The radiative impact of biomass burning aerosols on dust emissions over Namibia and the long-range transport of smoke observed during the Aerosols, Radiation and Clouds in southern Africa (AEROCLO-sA) campaign
Extending the wind profile beyond the surface layer by combining physical and machine learning approaches
Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories
Measurement report: Hygroscopicity of size-selected aerosol particles in the heavily polluted urban atmosphere of Delhi: impacts of chloride aerosol
An observation-constrained estimation of brown carbon aerosol direct radiative effects
The Puy de Dôme ICe Nucleation Intercomparison Campaign (PICNIC): comparison between online and offline methods in ambient air
Optical properties and simple forcing efficiency of the organic aerosols and black carbon emitted by residential wood burning in rural central Europe
Particle phase state and aerosol liquid water greatly impact secondary aerosol formation: insights into phase transition and its role in haze events
Measurement report: Nocturnal subsidence behind the cold front enhances surface particulate matter in plains regions: observations from the mobile multi-lidar system
Increase in precipitation scavenging contributes to long-term reductions of light-absorbing aerosol in the Arctic
Sea spray emissions from the Baltic Sea: comparison of aerosol eddy covariance fluxes and chamber-simulated sea spray emissions
Attribution of aerosol particle number size distributions to major sources using a 11-year-long urban dataset
Higher absorption enhancement of black carbon in summer shown by 2-year measurements at the high-altitude mountain site of Pic du Midi Observatory in the French Pyrenees
Variations of the atmospheric polycyclic aromatic hydrocarbon concentrations, sources, and health risk and the direct medical costs of lung cancer around the Bohai Sea against a background of pollution prevention and control in China
Introducing the novel concept of cumulative concentration roses for studying the transport of ultrafine particles from an airport to adjacent residential areas
Significant spatial gradients in new particle formation frequency in Greece during summer
Impact of desert dust on new particle formation events and the cloud condensation nuclei budget in dust-influenced areas
Active thermokarst regions contain rich sources of ice-nucleating particles
Examining the vertical heterogeneity of aerosols over the Southern Great Plains
Drivers controlling black carbon temporal variability in the lower troposphere of the European Arctic
Efficient droplet activation of ambient black carbon particles in sub-urban environment
Opinion: The strength of long-term comprehensive observations to meet multiple grand challenges in different environments and in the atmosphere
Contribution of fluorescent primary biological aerosol particles to low-level Arctic cloud residuals
Measurement report: Size-resolved mass concentration of equivalent black carbon-containing particles larger than 700 nm and their role in radiation
Aerosol absorption using in situ filter-based photometers and ground-based sun photometry in the Po Valley urban atmosphere
Aerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds
Aircraft ice-nucleating particle and aerosol composition measurements in the western North American Arctic
Mechanisms controlling giant sea salt aerosol size distributions along a tropical orographic coastline
New particle formation leads to enhanced cloud condensation nuclei concentrations on the Antarctic Peninsula
Mixing state and effective density of aerosol particles during the Beijing 2022 Olympic Winter Games
Tropospheric sulfate from Cumbre Vieja volcano at Las Palmas, transported towards Cabo Verde – lidar measurements of aerosol extinction, backscatter and depolarization at 355, 532 and 1064 nm
Measurement report: Shipborne observations of black carbon aerosols in the western Arctic Ocean during summer and autumn 2016–2020: boreal fire impacts
Quantified effect of seawater biogeochemistry on the temperature dependence of sea spray aerosol fluxes
Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause
3D assimilation and radiative impact assessment of aerosol black carbon over the Indian region using aircraft, balloon, ground-based, and multi-satellite observations
Measurement Report: A comparison of ice-nucleating particle and cloud condensation nuclei sources and properties during autumn at contrasting marine and terrestrial locations
Evaluation of aerosol- and gas-phase tracers for identification of transported biomass burning emissions in an industrially influenced location in Texas, USA
Physicochemical characterization and source apportionment of Arctic ice-nucleating particles observed in Ny-Ålesund in autumn 2019
Cyclones enhance the transport of sea spray aerosols to the high atmosphere in the Southern Ocean
Impact of 2020 COVID-19 lockdowns on particulate air pollution across Europe
New particle formation in the tropical free troposphere during CAMP2Ex: statistics and impact of emission sources, convective activity, and synoptic conditions
Explaining apparent particle shrinkage related to new particle formation events in western Saudi Arabia does not require evaporation
Investigation of the effects of the Greek extreme wildfires of August 2021 on air quality and spectral solar irradiance
Characterization of dust-related new particle formation events based on long-term measurement in the North China Plain
Airborne investigation of black carbon interaction with low-level, persistent, mixed-phase clouds in the Arctic summer
The variation in the particle number size distribution during the rainfall: wet scavenging and air mass changing
Opinion: New directions in atmospheric research offered by research infrastructures combined with open and data-intensive science
Characterization of size-segregated particles' turbulent flux and deposition velocity by eddy correlation method at an Arctic site
Vertical distribution of black carbon and its mixing state in the urban boundary layer in summer
Insights into the size-resolved dust emission from field measurements in the Moroccan Sahara
Cyrille Flamant, Jean-Pierre Chaboureau, Marco Gaetani, Kerstin Schepanski, and Paola Formenti
Atmos. Chem. Phys., 24, 4265–4288, https://doi.org/10.5194/acp-24-4265-2024, https://doi.org/10.5194/acp-24-4265-2024, 2024
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In the austral dry season, the atmospheric composition over southern Africa is dominated by biomass burning aerosols and terrigenous aerosols (so-called mineral dust). This study suggests that the radiative effect of biomass burning aerosols needs to be taken into account to properly forecast dust emissions in Namibia.
Boming Liu, Xin Ma, Jianping Guo, Renqiang Wen, Hui Li, Shikuan Jin, Yingying Ma, Xiaoran Guo, and Wei Gong
Atmos. Chem. Phys., 24, 4047–4063, https://doi.org/10.5194/acp-24-4047-2024, https://doi.org/10.5194/acp-24-4047-2024, 2024
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Accurate wind profile estimation, especially for the lowest few hundred meters of the atmosphere, is of great significance for the weather, climate, and renewable energy sector. We propose a novel method that combines the power-law method with the random forest algorithm to extend wind profiles beyond the surface layer. Compared with the traditional algorithm, this method has better stability and spatial applicability and can be used to obtain the wind profiles on different land cover types.
Gabriela R. Unfer, Luiz A. T. Machado, Paulo Artaxo, Marco A. Franco, Leslie A. Kremper, Mira L. Pöhlker, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 3869–3882, https://doi.org/10.5194/acp-24-3869-2024, https://doi.org/10.5194/acp-24-3869-2024, 2024
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Amazonian aerosols and their interactions with precipitation were studied by understanding them in a 3D space based on three parameters that characterize the concentration and size distribution of aerosols. The results showed characteristic arrangements regarding seasonal and diurnal cycles, as well as when interacting with precipitation. The use of this 3D space appears to be a promising tool for aerosol population analysis and for model validation and parameterization.
Anil Kumar Mandariya, Ajit Ahlawat, Mohammed Haneef, Nisar Ali Baig, Kanan Patel, Joshua Apte, Lea Hildebrandt Ruiz, Alfred Wiedensohler, and Gazala Habib
Atmos. Chem. Phys., 24, 3627–3647, https://doi.org/10.5194/acp-24-3627-2024, https://doi.org/10.5194/acp-24-3627-2024, 2024
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The current study explores the temporal variation of size-selected particle hygroscopicity in Delhi for the first time. Here, we report that the high volume fraction contribution of ammonium chloride to aerosol governs the high aerosol hygroscopicity and associated liquid water content based on the experimental data. The episodically high ammonium chloride present in Delhi's atmosphere could lead to haze and fog formation under high relative humidity in the region.
Yueyue Cheng, Chao Liu, Jiandong Wang, Jiaping Wang, Zhouyang Zhang, Li Chen, Dafeng Ge, Caijun Zhu, Jinbo Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 3065–3078, https://doi.org/10.5194/acp-24-3065-2024, https://doi.org/10.5194/acp-24-3065-2024, 2024
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Brown carbon (BrC), a light-absorbing aerosol, plays a pivotal role in influencing global climate. However, assessing BrC radiative effects remains challenging because the required observational data are hardly accessible. Here we develop a new BrC radiative effect estimation method combining conventional observations and numerical models. Our findings reveal that BrC absorbs up to a third of the sunlight at 370 nm that black carbon does, highlighting its importance in aerosol radiative effects.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
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Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Andrea Cuesta-Mosquera, Kristina Glojek, Griša Močnik, Luka Drinovec, Asta Gregorič, Martin Rigler, Matej Ogrin, Baseerat Romshoo, Kay Weinhold, Maik Merkel, Dominik van Pinxteren, Hartmut Herrmann, Alfred Wiedensohler, Mira Pöhlker, and Thomas Müller
Atmos. Chem. Phys., 24, 2583–2605, https://doi.org/10.5194/acp-24-2583-2024, https://doi.org/10.5194/acp-24-2583-2024, 2024
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This study evaluated the air pollution and climate impacts of residential-wood-burning particle emissions from a rural European site. The authors investigate the optical and physical properties that connect the aerosol emissions with climate by evaluating atmospheric radiative impacts via simple-forcing calculations. The study contributes to reducing the lack of information on the understanding of the optical properties of air pollution from anthropogenic sources.
Xiangxinyue Meng, Zhijun Wu, Jingchuan Chen, Yanting Qiu, Taomou Zong, Mijung Song, Jiyi Lee, and Min Hu
Atmos. Chem. Phys., 24, 2399–2414, https://doi.org/10.5194/acp-24-2399-2024, https://doi.org/10.5194/acp-24-2399-2024, 2024
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Our study revealed that particles predominantly exist in a semi-solid or solid state during clean winter days with RH below 30 %. However, a non-liquid to a liquid phase transition occurred when the aerosol liquid water (ALW) mass fraction surpassed 15 % (dry mass) at transition RH thresholds ranging from 40 % to 60 %. We also provide insights into the increasingly important roles of particle phase state variation and ALW in secondary particulate growth during haze formation in Beijing, China.
Yiming Wang, Haolin Wang, Yujie Qin, Xinqi Xu, Guowen He, Nanxi Liu, Shengjie Miao, Xiao Lu, Haichao Wang, and Shaojia Fan
Atmos. Chem. Phys., 24, 2267–2285, https://doi.org/10.5194/acp-24-2267-2024, https://doi.org/10.5194/acp-24-2267-2024, 2024
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We conducted a vertical measurement of winter PM2.5 using a mobile multi-lidar system in four cities. Combined with the surface PM2.5 data, the ERA5 reanalysis data, and GEOS-Chem simulations during Dec 2018–Feb 2019, we found that transport nocturnal PM2.5 enhancement by subsidence (T-NPES) events widely occurred with high frequencies in plains regions in eastern China but happened less often in basin regions like Xi’an and Chengdu. We propose a conceptual model of the T-NPES events.
Dominic Heslin-Rees, Peter Tunved, Johan Ström, Roxana Cremer, Paul Zieger, Ilona Riipinen, Annica M. L. Ekman, Konstantinos Eleftheriadis, and Radovan Krejci
Atmos. Chem. Phys., 24, 2059–2075, https://doi.org/10.5194/acp-24-2059-2024, https://doi.org/10.5194/acp-24-2059-2024, 2024
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Light-absorbing atmospheric particles (e.g. black carbon – BC) exert a warming effect on the Arctic climate. We show that the amount of particle light absorption decreased from 2002 to 2023. We conclude that in addition to reductions in emissions of BC, wet removal plays a role in the long-term reduction of BC in the Arctic, given the increase in surface precipitation experienced by air masses arriving at the site. The potential impact of biomass burning events is shown to have increased.
Julika Zinke, Ernst Douglas Nilsson, Piotr Markuszewski, Paul Zieger, Eva Monica Mårtensson, Anna Rutgersson, Erik Nilsson, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 1895–1918, https://doi.org/10.5194/acp-24-1895-2024, https://doi.org/10.5194/acp-24-1895-2024, 2024
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We conducted two research campaigns in the Baltic Sea, during which we combined laboratory sea spray simulation experiments with flux measurements on a nearby island. To combine these two methods, we scaled the laboratory measurements to the flux measurements using three different approaches. As a result, we derived a parameterization that is dependent on wind speed and wave state for particles with diameters 0.015–10 μm. This parameterization is applicable to low-salinity waters.
Máté Vörösmarty, Philip K. Hopke, and Imre Salma
EGUsphere, https://doi.org/10.5194/egusphere-2024-316, https://doi.org/10.5194/egusphere-2024-316, 2024
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The World Health Organization identified the ultrafine particles, which make up most of the particle number concentrations, as a potential risk factor for humans. The sources of particle numbers are very different from those of the particulate matter mass. We performed source apportionment of size segregated particle number concentrations over the diameter range of 6–1000 nm in Budapest for 11 full years. Six source types were identified, characterised, and quantified.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
Atmos. Chem. Phys., 24, 1801–1824, https://doi.org/10.5194/acp-24-1801-2024, https://doi.org/10.5194/acp-24-1801-2024, 2024
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At a French high-altitude site, where many complex interactions between black carbon (BC), radiation, clouds and snow impact climate, 2 years of refractive BC (rBC) and aerosol optical and microphysical measurements have been made. We observed strong seasonal rBC properties variations, with an enhanced absorption in summer compared to winter. The combination of rBC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the rBC light absorption seasonality.
Wenwen Ma, Rong Sun, Xiaoping Wang, Zheng Zong, Shizhen Zhao, Zeyu Sun, Chongguo Tian, Jianhui Tang, Song Cui, Jun Li, and Gan Zhang
Atmos. Chem. Phys., 24, 1509–1523, https://doi.org/10.5194/acp-24-1509-2024, https://doi.org/10.5194/acp-24-1509-2024, 2024
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This is the first report of long-term atmospheric PAH monitoring around the Bohai Sea. The results showed that the concentrations of PAHs in the atmosphere around the Bohai Sea decreased from June 2014 to May 2019, especially the concentrations of highly toxic PAHs. This indicates that the contributions from PAH sources changed to a certain extent in different areas, and it also led to reductions in the related health risk and medical costs following pollution prevention and control.
Julius Seidler, Markus N. Friedrich, Christoph K. Thomas, and Anke C. Nölscher
Atmos. Chem. Phys., 24, 137–153, https://doi.org/10.5194/acp-24-137-2024, https://doi.org/10.5194/acp-24-137-2024, 2024
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Here, we study the transport of ultrafine particles (UFPs) from an airport to two new adjacent measuring sites for 1 year. The number of UFPs in the air and the diurnal variation are typical urban. Winds from the airport show increased number concentrations. Additionally, considering wind frequencies, we estimate that, from all UFPs measured at the two sites, 10 %–14 % originate from the airport and/or other UFP sources from between the airport and site.
Andreas Aktypis, Christos Kaltsonoudis, David Patoulias, Panayiotis Kalkavouras, Angeliki Matrali, Christina N. Vasilakopoulou, Evangelia Kostenidou, Kalliopi Florou, Nikos Kalivitis, Aikaterini Bougiatioti, Konstantinos Eleftheriadis, Stergios Vratolis, Maria I. Gini, Athanasios Kouras, Constantini Samara, Mihalis Lazaridis, Sofia-Eirini Chatoutsidou, Nikolaos Mihalopoulos, and Spyros N. Pandis
Atmos. Chem. Phys., 24, 65–84, https://doi.org/10.5194/acp-24-65-2024, https://doi.org/10.5194/acp-24-65-2024, 2024
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Extensive continuous particle number size distribution measurements took place during two summers (2020 and 2021) at 11 sites in Greece for the investigation of the frequency and the spatial extent of new particle formation. The frequency during summer varied from close to zero in southwestern Greece to more than 60 % in the northern, central, and eastern regions. The spatial variability can be explained by the proximity of the sites to coal-fired power plants and agricultural areas.
Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Fernando Rejano, Andrea Casans, Gloria Titos, Francisco José Olmo, Lubna Dada, Simo Hakala, Tareq Hussein, Katrianne Lehtipalo, Pauli Paasonen, Antti Hyvärinen, Noemí Pérez, Xavier Querol, Sergio Rodríguez, Nikos Kalivitis, Yenny González, Mansour A. Alghamdi, Veli-Matti Kerminen, Andrés Alastuey, Tuukka Petäjä, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 23, 15795–15814, https://doi.org/10.5194/acp-23-15795-2023, https://doi.org/10.5194/acp-23-15795-2023, 2023
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Here we present the first study of the effect of mineral dust on the inhibition/promotion of new particle formation (NPF) events in different dust-influenced areas. Unexpectedly, we show that the occurrence of NPF events is highly frequent during mineral dust outbreaks, occurring even during extreme dust outbreaks. We also show that the occurrence of NPF events during mineral dust outbreaks significantly affects the potential cloud condensation nuclei budget.
Kevin R. Barry, Thomas C. J. Hill, Marina Nieto-Caballero, Thomas A. Douglas, Sonia M. Kreidenweis, Paul J. DeMott, and Jessie M. Creamean
Atmos. Chem. Phys., 23, 15783–15793, https://doi.org/10.5194/acp-23-15783-2023, https://doi.org/10.5194/acp-23-15783-2023, 2023
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Ice-nucleating particles (INPs) are important for the climate due to their influence on cloud properties. To understand potential land-based sources of them in the Arctic, we carried out a survey near the northernmost point of Alaska, a landscape connected to the permafrost (thermokarst). Permafrost contained high concentrations of INPs, with the largest values near the coast. The thermokarst lakes were found to emit INPs, and the water contained elevated concentrations.
Yang Wang, Chanakya Bagya Ramesh, Scott E. Giangrande, Jerome Fast, Xianda Gong, Jiaoshi Zhang, Ahmet Tolga Odabasi, Marcus Vinicius Batista Oliveira, Alyssa Matthews, Fan Mei, John E. Shilling, Jason Tomlinson, Die Wang, and Jian Wang
Atmos. Chem. Phys., 23, 15671–15691, https://doi.org/10.5194/acp-23-15671-2023, https://doi.org/10.5194/acp-23-15671-2023, 2023
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We report the vertical profiles of aerosol properties over the Southern Great Plains (SGP), a region influenced by shallow convective clouds, land–atmosphere interactions, boundary layer turbulence, and the aerosol life cycle. We examined the processes that drive the aerosol population and distribution in the lower troposphere over the SGP. This study helps improve our understanding of aerosol–cloud interactions and the model representation of aerosol processes.
Stefania Gilardoni, Dominic Heslin-Rees, Mauro Mazzola, Vito Vitale, Michael Sprenger, and Radovan Krejci
Atmos. Chem. Phys., 23, 15589–15607, https://doi.org/10.5194/acp-23-15589-2023, https://doi.org/10.5194/acp-23-15589-2023, 2023
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Models still fail in reproducing black carbon (BC) temporal variability in the Arctic. Analysis of equivalent BC concentrations in the European Arctic shows that BC seasonal variability is modulated by the efficiency of removal by precipitation during transport towards high latitudes. Short-term variability is controlled by synoptic-scale circulation patterns. The advection of warm air from lower latitudes is an effective pollution transport pathway during summer.
Ping Tian, Dantong Liu, Kang Hu, Yangzhou Wu, Mengyu Huang, Hui He, Jiujiang Sheng, Chenjie Yu, Dawei Hu, and Deping Ding
EGUsphere, https://doi.org/10.5194/egusphere-2023-2744, https://doi.org/10.5194/egusphere-2023-2744, 2023
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The results here thus provide direct evidence of efficient droplet activation of BC, and the CCN activation fraction of BC was higher than all-particle suggested the higher CCN activity of BC though its hygroscopicity is lower. Our research reveals that the evolution of BC's hygroscopicity and its CCN activation properties through atmospheric aging can be effectively characterized by the photochemical age.
Markku Kulmala, Anna Lintunen, Hanna Lappalainen, Annele Virtanen, Chao Yan, Ekaterina Ezhova, Tuomo Nieminen, Ilona Riipinen, Risto Makkonen, Johanna Tamminen, Anu-Maija Sundström, Antti Arola, Armin Hansel, Kari Lehtinen, Timo Vesala, Tuukka Petäjä, Jaana Bäck, Tom Kokkonen, and Veli-Matti Kerminen
Atmos. Chem. Phys., 23, 14949–14971, https://doi.org/10.5194/acp-23-14949-2023, https://doi.org/10.5194/acp-23-14949-2023, 2023
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To be able to meet global grand challenges, we need comprehensive open data with proper metadata. In this opinion paper, we describe the SMEAR (Station for Measuring Earth surface – Atmosphere Relations) concept and include several examples (cases), such as new particle formation and growth, feedback loops and the effect of COVID-19, and what has been learned from these investigations. The future needs and the potential of comprehensive observations of the environment are summarized.
Gabriel Pereira Freitas, Ben Kopec, Kouji Adachi, Radovan Krejci, Dominic Heslin-Rees, Karl Espen Yttri, Alun Hubbard, Jeffrey M. Welker, and Paul Zieger
EGUsphere, https://doi.org/10.5194/egusphere-2023-2600, https://doi.org/10.5194/egusphere-2023-2600, 2023
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Bioaerosols can participate in ice formation within clouds. In the Arctic, where global warming manifests most, they may become increasingly more important as their sources are prevailing for a longer period of the year. We have directly measured bioaerosols within clouds for a full year at an Arctic mountain site using a novel combination of cloud particle sampling and single-particle techniques. We show that bioaerosols act as cloud seeds and may influence the presence of ice within clouds.
Weilun Zhao, Ying Li, Gang Zhao, Song Guo, Nan Ma, Shuya Hu, and Chunsheng Zhao
Atmos. Chem. Phys., 23, 14889–14902, https://doi.org/10.5194/acp-23-14889-2023, https://doi.org/10.5194/acp-23-14889-2023, 2023
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Studies have concentrated on particles containing black carbon (BC) smaller than 700 nm because of technical limitations. In this study, BC-containing particles larger than 700 nm (BC>700) were measured, highlighting their importance to total BC mass and absorption. The contribution of BC>700 to the BC direct radiative effect was estimated, highlighting the necessity to consider the whole size range of BC-containing particles in the model estimation of BC radiative effects.
Alessandro Bigi, Giorgio Veratti, Elisabeth Andrews, Martine Collaud Coen, Lorenzo Guerrieri, Vera Bernardoni, Dario Massabò, Luca Ferrero, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 23, 14841–14869, https://doi.org/10.5194/acp-23-14841-2023, https://doi.org/10.5194/acp-23-14841-2023, 2023
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Atmospheric particles include compounds that play a key role in the greenhouse effect and air toxicity. Concurrent observations of these compounds by multiple instruments are presented, following deployment within an urban environment in the Po Valley, one of Europe's pollution hotspots. The study compares these data, highlighting the impact of ground emissions, mainly vehicular traffic and biomass burning, on the absorption of sun radiation and, ultimately, on climate change and air quality.
Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li, Wenche Aas, Chris Lunder, Radovan Krejci, Julie Thérèse Pasquier, Jan Henneberger, Robert Oscar David, Christoph Ritter, Claudia Mohr, Paul Zieger, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13941–13956, https://doi.org/10.5194/acp-23-13941-2023, https://doi.org/10.5194/acp-23-13941-2023, 2023
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Low-altitude clouds play a key role in regulating the climate of the Arctic, a region that suffers from climate change more than any other on the planet. We gathered meteorological and aerosol physical and chemical data over a year and utilized them for a parameterization that help us unravel the factors driving and limiting the efficiency of cloud droplet formation. We then linked this information to the sources of aerosol found during each season and to processes of cloud glaciation.
Alberto Sanchez-Marroquin, Sarah L. Barr, Ian T. Burke, James B. McQuaid, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 13819–13834, https://doi.org/10.5194/acp-23-13819-2023, https://doi.org/10.5194/acp-23-13819-2023, 2023
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The sources and concentrations of ice-nucleating particles (INPs) in the Arctic are still poorly understood. Here we report aircraft-based INP concentrations and aerosol composition in the western North American Arctic. The concentrations of INPs and all aerosol particles were low. The aerosol samples contained mostly sea salt and dust particles. Dust particles were more relevant for the INP concentrations than sea salt. However, dust alone cannot account for all of the measured INPs.
Katherine L. Ackerman, Alison D. Nugent, and Chung Taing
Atmos. Chem. Phys., 23, 13735–13753, https://doi.org/10.5194/acp-23-13735-2023, https://doi.org/10.5194/acp-23-13735-2023, 2023
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Sea salt aerosol is an important marine aerosol that may be produced in greater quantities in coastal regions than over the open ocean. This study observed these particles along the windward coastline of O'ahu, Hawai'i, to understand how wind and waves influence their production and dispersal. Overall, wave heights were the strongest variable correlated with changes in aerosol concentrations, while wind speeds played an important role in their horizontal dispersal and vertical mixing.
Jiyeon Park, Hyojin Kang, Yeontae Gim, Eunho Jang, Ki-Tae Park, Sangjong Park, Chang Hoon Jung, Darius Ceburnis, Colin O'Dowd, and Young Jun Yoon
Atmos. Chem. Phys., 23, 13625–13646, https://doi.org/10.5194/acp-23-13625-2023, https://doi.org/10.5194/acp-23-13625-2023, 2023
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We measured the number size distribution of 2.5–300 nm particles and cloud condensation nuclei (CCN) number concentrations at King Sejong Station on the Antarctic Peninsula continuously from 1 January to 31 December 2018. During the pristine and clean periods, 97 new particle formation (NPF) events were detected. For 83 of these, CCN concentrations increased by 2 %–268 % (median 44 %) following 1 to 36 h (median 8 h) after NPF events.
Aodong Du, Jiaxing Sun, Hang Liu, Weiqi Xu, Wei Zhou, Yuting Zhang, Lei Li, Xubing Du, Yan Li, Xiaole Pan, Zifa Wang, and Yele Sun
Atmos. Chem. Phys., 23, 13597–13611, https://doi.org/10.5194/acp-23-13597-2023, https://doi.org/10.5194/acp-23-13597-2023, 2023
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We characterized the impacts of emission controls on particle mixing state and density during the Beijing Olympic Winter Games using a SPAMS in tandem with a DMA and an AAC. OC and sulfate-containing particles increased, while those from primary emissions decreased. The effective particle densities increased and varied largely for different particles, highlighting the impacts of aging and formation processes on the changes of particle density and mixing state.
Henriette Gebauer, Athena Augusta Floutsi, Moritz Haarig, Martin Radenz, Ronny Engelmann, Dietrich Althausen, Annett Skupin, Albert Ansmann, Cordula Zenk, and Holger Baars
EGUsphere, https://doi.org/10.5194/egusphere-2023-2305, https://doi.org/10.5194/egusphere-2023-2305, 2023
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Sulfate aerosol from the volcanic eruption at Las Palmas in 2021 was observed over Cabo Verde. The impact of the eruption was observable even 1500 km away from the emission source and led to an extraordinary strong pollution in the lowermost atmosphere above Cabo Verde. We characterized the aerosol burden based on lidar and sun photometer observations. We compared the volcanic case to the typical background conditions (reference case) to quantify the volcanic pollution.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
EGUsphere, https://doi.org/10.5194/egusphere-2023-2315, https://doi.org/10.5194/egusphere-2023-2315, 2023
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Black carbon aerosols (BC) play important roles in Arctic climate change, yet they are not well understood because of limited observational facts. We observed BC mass concentrations (mBC) in the Western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high BC events in the Arctic Ocean.
Karine Sellegri, Theresa Barthelmeß, Jonathan Trueblood, Antonia Cristi, Evelyn Freney, Clémence Rose, Neill Barr, Mike Harvey, Karl Safi, Stacy Deppeler, Karen Thompson, Wayne Dillon, Anja Engel, and Cliff Law
Atmos. Chem. Phys., 23, 12949–12964, https://doi.org/10.5194/acp-23-12949-2023, https://doi.org/10.5194/acp-23-12949-2023, 2023
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The amount of sea spray emitted to the atmosphere depends on the ocean temperature, but this dependency is not well understood, especially when ocean biology is involved. In this study, we show that sea spray emissions are increased by up to a factor of 4 at low seawater temperatures compared to moderate temperatures, and we quantify the temperature dependence as a function of the ocean biogeochemistry.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
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The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Nair Krishnan Kala, Narayana Sarma Anand, Mohanan R. Manoj, Srinivasan Prasanth, Harshavardhana S. Pathak, Thara Prabhakaran, Pramod D. Safai, Krishnaswamy K. Moorthy, and Sreedharan K. Satheesh
Atmos. Chem. Phys., 23, 12801–12819, https://doi.org/10.5194/acp-23-12801-2023, https://doi.org/10.5194/acp-23-12801-2023, 2023
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We present a 3D data set of aerosol black carbon over the Indian mainland by assimilating data from surface, aircraft, and balloon measurements, along with multi-satellite observations. Radiative transfer computations using height-resolved aerosol absorption show higher warming in the free troposphere and will have large implications for atmospheric stability. This data set will help reduce the uncertainty in aerosol radiative effects in climate model simulations over the Indian region.
Elise K. Wilbourn, Larissa Lacher, Carlos Guerrero, Hemanth S. K. Vepuri, Kristina Höhler, Jens Nadolny, Ottmar Möhler, and Naruki Hiranuma
EGUsphere, https://doi.org/10.5194/egusphere-2023-1456, https://doi.org/10.5194/egusphere-2023-1456, 2023
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Ambient ice and cloud particles were measured at terrestrial and temperate marine sites. Ice particles were more abundant in the former site while the fraction of ice particles relative to total ambient particles was higher in the latter site. We found continental and biogenic materials as a major source of ice particles in the terrestrial site. A positive correlation was found for ice and cloud particle concentrations in the marine site, implying they originate from the same source.
Sujan Shrestha, Shan Zhou, Manisha Mehra, Meghan Guagenti, Subin Yoon, Sergio L. Alvarez, Fangzhou Guo, Chun-Ying Chao, James H. Flynn III, Yuxuan Wang, Robert J. Griffin, Sascha Usenko, and Rebecca J. Sheesley
Atmos. Chem. Phys., 23, 10845–10867, https://doi.org/10.5194/acp-23-10845-2023, https://doi.org/10.5194/acp-23-10845-2023, 2023
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We evaluated different methods for assessing the influence of long-range transport of biomass burning (BB) plumes at a coastal site in Texas, USA. We show that the aerosol composition and optical properties exhibited good agreement, while CO and acetonitrile trends were less specific for assessing BB source influence. Our results demonstrate that the network of aerosol optical measurements can be useful for identifying the influence of aged BB plumes in anthropogenically influenced areas.
Guangyu Li, Elise K. Wilbourn, Zezhen Cheng, Jörg Wieder, Allison Fagerson, Jan Henneberger, Ghislain Motos, Rita Traversi, Sarah D. Brooks, Mauro Mazzola, Swarup China, Athanasios Nenes, Ulrike Lohmann, Naruki Hiranuma, and Zamin A. Kanji
Atmos. Chem. Phys., 23, 10489–10516, https://doi.org/10.5194/acp-23-10489-2023, https://doi.org/10.5194/acp-23-10489-2023, 2023
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In this work, we present results from an Arctic field campaign (NASCENT) in Ny-Ålesund, Svalbard, on the abundance, variability, physicochemical properties, and potential sources of ice-nucleating particles (INPs) relevant for mixed-phase cloud formation. This work improves the data coverage of Arctic INPs and aerosol properties, allowing for the validation of models predicting cloud microphysical and radiative properties of mixed-phase clouds in the rapidly warming Arctic.
Jun Shi, Jinpei Yan, Shanshan Wang, Shuhui Zhao, Miming Zhang, Suqing Xu, Qi Lin, Hang Yang, and Siying Dai
Atmos. Chem. Phys., 23, 10349–10359, https://doi.org/10.5194/acp-23-10349-2023, https://doi.org/10.5194/acp-23-10349-2023, 2023
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An underway aerosol-monitoring system was used to determine the Na+ concentration during different cyclone periods in the Southern Ocean in order to assess the potential effects of cyclones on sea spray aerosol (SSA) emissions. It was estimated that more than 23 % of SSAs were transported upwards during cyclone periods. Vertically transported SSAs can be regarded as an important source of CCN and hence have an effect on climate in the middle and high latitudes of the Southern Hemisphere.
Jean-Philippe Putaud, Enrico Pisoni, Alexander Mangold, Christoph Hueglin, Jean Sciare, Michael Pikridas, Chrysanthos Savvides, Jakub Ondracek, Saliou Mbengue, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Laurent Poulain, Dominik van Pinxteren, Hartmut Herrmann, Andreas Massling, Claus Nordstroem, Andrés Alastuey, Cristina Reche, Noemí Pérez, Sonia Castillo, Mar Sorribas, Jose Antonio Adame, Tuukka Petaja, Katrianne Lehtipalo, Jarkko Niemi, Véronique Riffault, Joel F. de Brito, Augustin Colette, Olivier Favez, Jean-Eudes Petit, Valérie Gros, Maria I. Gini, Stergios Vratolis, Konstantinos Eleftheriadis, Evangelia Diapouli, Hugo Denier van der Gon, Karl Espen Yttri, and Wenche Aas
Atmos. Chem. Phys., 23, 10145–10161, https://doi.org/10.5194/acp-23-10145-2023, https://doi.org/10.5194/acp-23-10145-2023, 2023
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Many European people are still exposed to levels of air pollution that can affect their health. COVID-19 lockdowns in 2020 were used to assess the impact of the reduction in human mobility on air pollution across Europe by comparing measurement data with values that would be expected if no lockdown had occurred. We show that lockdown measures did not lead to consistent decreases in the concentrations of fine particulate matter suspended in the air, and we investigate why.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Simo Hakala, Ville Vakkari, Heikki Lihavainen, Antti-Pekka Hyvärinen, Kimmo Neitola, Jenni Kontkanen, Veli-Matti Kerminen, Markku Kulmala, Tuukka Petäjä, Tareq Hussein, Mamdouh I. Khoder, Mansour A. Alghamdi, and Pauli Paasonen
Atmos. Chem. Phys., 23, 9287–9321, https://doi.org/10.5194/acp-23-9287-2023, https://doi.org/10.5194/acp-23-9287-2023, 2023
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Things are not always as they first seem in ambient aerosol measurements. Observations of decreasing particle sizes are often interpreted as resulting from particle evaporation. We show that such observations can counterintuitively be explained by particles that are constantly growing in size. This requires one to account for the previous movements of the observed air. Our explanation implies a larger number of larger particles, meaning more significant effects of aerosols on climate and health.
Akriti Masoom, Ilias Fountoulakis, Stelios Kazadzis, Ioannis-Panagiotis Raptis, Anna Kampouri, Basil E. Psiloglou, Dimitra Kouklaki, Kyriakoula Papachristopoulou, Eleni Marinou, Stavros Solomos, Anna Gialitaki, Dimitra Founda, Vasileios Salamalikis, Dimitris Kaskaoutis, Natalia Kouremeti, Nikolaos Mihalopoulos, Vassilis Amiridis, Andreas Kazantzidis, Alexandros Papayannis, Christos S. Zerefos, and Kostas Eleftheratos
Atmos. Chem. Phys., 23, 8487–8514, https://doi.org/10.5194/acp-23-8487-2023, https://doi.org/10.5194/acp-23-8487-2023, 2023
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We analyse the spatial and temporal aerosol spectral optical properties during the extreme wildfires of August 2021 in Greece and assess their effects on air quality and solar radiation quantities related to health, agriculture, and energy. Different aerosol conditions are identified (pure smoke, pure dust, dust–smoke together); the largest impact on solar radiation quantities is found for cases with mixed dust–smoke aerosols. Such situations are expected to occur more frequently in the future.
Xiaojing Shen, Junying Sun, Huizheng Che, Yangmei Zhang, Chunhong Zhou, Ke Gui, Wanyun Xu, Quan Liu, Junting Zhong, Can Xia, Xinyao Hu, Sinan Zhang, Jialing Wang, Shuo Liu, Jiayuan Lu, Aoyuan Yu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 8241–8257, https://doi.org/10.5194/acp-23-8241-2023, https://doi.org/10.5194/acp-23-8241-2023, 2023
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New particle formation (NPF) events occur when the dust episodes' fade is analysed based on long-term measurement of particle number size distribution. Analysis shows that the observed formation and growth rates are approximately 50 % of and 30 % lower than those of other NPF events. As a consequence of the uptake of precursor gases on mineral dust, the physical and chemical properties of submicron particles, as well as the ability to be cloud condensation nuclei, can be changed.
Marco Zanatta, Stephan Mertes, Olivier Jourdan, Regis Dupuy, Emma Järvinen, Martin Schnaiter, Oliver Eppers, Johannes Schneider, Zsófia Jurányi, and Andreas Herber
Atmos. Chem. Phys., 23, 7955–7973, https://doi.org/10.5194/acp-23-7955-2023, https://doi.org/10.5194/acp-23-7955-2023, 2023
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Black carbon (BC) particles influence the Arctic radiative balance. Vertical measurements of black carbon were conducted during the ACLOUD campaign in the European Arctic to study the interaction of BC with clouds. This study shows that clouds influence the vertical variability of BC properties across the inversion layer and that multiple activation and transformation mechanisms of BC may occur in the presence of low-level, persistent, mixed-phase clouds.
Guangdong Niu, Ximeng Qi, Liangduo Chen, Lian Xue, Shiyi Lai, Xin Huang, Jiaping Wang, Xuguang Chi, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 23, 7521–7534, https://doi.org/10.5194/acp-23-7521-2023, https://doi.org/10.5194/acp-23-7521-2023, 2023
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The reported below-cloud wet-scavenging coefficients (BWSCs) are much higher than theoretical data, but the reason remains unclear. Based on long-term observation, we find that air mass changing during rainfall events causes the overestimation of BWSCs. Thus, the discrepancy in BWSCs between observation and theory is not as large as currently believed. To obtain reasonable BWSCs and parameterizations from field observations, the effect of air mass changes needs to be considered.
Andreas Petzold, Ulrich Bundke, Anca Hienola, Paolo Laj, Cathrine Lund Myhre, Alex Vermeulen, Angeliki Adamaki, Werner Kutsch, Valerie Thouret, Damien Boulanger, Markus Fiebig, Markus Stocker, Zhiming Zhao, and Ari Asmi
EGUsphere, https://doi.org/10.5194/egusphere-2023-1423, https://doi.org/10.5194/egusphere-2023-1423, 2023
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The atmosphere-centred European environmental research infrastructures ACTRIS, IAGOS and ICOS can assume a leading role in atmospheric sciences thanks to their capacities for acquisition and reporting of long-term and high-quality observational data. We elaborate on the novel research opportunities which evolve from the combination of open access to data, data interoperability and tools and technologies offered by data-intensive science through the European Open Science Cloud.
Antonio Donateo, Gianluca Pappaccogli, Daniela Famulari, Mauro Mazzola, Federico Scoto, and Stefano Decesari
Atmos. Chem. Phys., 23, 7425–7445, https://doi.org/10.5194/acp-23-7425-2023, https://doi.org/10.5194/acp-23-7425-2023, 2023
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This work aims to measure the turbulent fluxes and the dry deposition velocity for size-segregated particles (from ultrafine to quasi-coarse range) at an Arctic site (Svalbard). Aiming to characterize the effect of surface properties on dry deposition, continuous observations were performed from the coldest months (on snow surface) to the snow melting period and throughout the summer (snow-free surface). A data fit of the deposition velocity as a function of particle diameters will be provided.
Hang Liu, Xiaole Pan, Shandong Lei, Yuting Zhang, Aodong Du, Weijie Yao, Guiqian Tang, Tao Wang, Jinyuan Xin, Jie Li, Yele Sun, Junji Cao, and Zifa Wang
Atmos. Chem. Phys., 23, 7225–7239, https://doi.org/10.5194/acp-23-7225-2023, https://doi.org/10.5194/acp-23-7225-2023, 2023
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We provide the average vertical profiles of black carbon (BC) concentration, size distribution and coating thickness at different times of the day in an urban area based on 112 vertical profiles. In addition, it is found that BC in the residual layer generally has a thicker coating, higher absorption enhancement and hygroscopicity than on the surface. Such aged BC could enter into the boundary layer and influence the BC properties in the early morning.
Cristina González-Flórez, Martina Klose, Andrés Alastuey, Sylvain Dupont, Jerónimo Escribano, Vicken Etyemezian, Adolfo Gonzalez-Romero, Yue Huang, Konrad Kandler, George Nikolich, Agnesh Panta, Xavier Querol, Cristina Reche, Jesús Yus-Díez, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 7177–7212, https://doi.org/10.5194/acp-23-7177-2023, https://doi.org/10.5194/acp-23-7177-2023, 2023
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Atmospheric mineral dust consists of tiny mineral particles that are emitted by wind erosion from arid regions. Its particle size distribution (PSD) affects its impact on the Earth's system. Nowadays, there is an incomplete understanding of the emitted dust PSD and a lot of debate about its variability. Here, we try to address these issues based on the measurements performed during a wind erosion and dust emission field campaign in the Moroccan Sahara within the framework of FRAGMENT project.
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Short summary
Surface topography affects aerosol–cloud interactions in boundary layer clouds. Local topography effects should be screened out from in situ observations before results can be generalised into a larger scale. Here we present modelling and observational results from a measurement station residing in a 75 m tower on top of a 150 m hill, and analyse how landscape affects the cloud formation, and which factors should be taken into account when aerosol effect on cloud droplet formation is studied.
Surface topography affects aerosol–cloud interactions in boundary layer clouds. Local topography...
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