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Volume 15, issue 23
Atmos. Chem. Phys., 15, 13569–13584, 2015
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 13569–13584, 2015
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 09 Dec 2015

Research article | 09 Dec 2015

Reactive uptake of ammonia to secondary organic aerosols: kinetics of organonitrogen formation

Y. Liu et al.

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Aiken, A. C., Peter F. DeCarlo, and Jimenez, J. L.: Elemental analysis of organic species with electron ionization high-resolution mass spectrometry, Anal. Chem., 79, 8350–8358, https://doi.org/10.1021/ac071150w, 2007.
Alexander, D. T. L., Crozier, P. A., and Anderson, J. R.: Brown carbon spheres in East Asian outflow and their optical properties, Science, 321, 833–836, https://doi.org/10.1126/science.1155296, 2008.
Andrade-Eiroa, A., Leroy, V., Dagaut, P., and Bedjanian, Y.: Determination of polycyclic aromatic hydrocarbons in kerosene and bio-kerosene soot, Chemosphere, 78, 1342–1349, https://doi.org/10.1016/j.chemosphere.2010.01.005, 2010.
Andreae, M. O. and Gelencsér, A.: Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols, Atmos. Chem. Phys., 6, 3131–3148, https://doi.org/10.5194/acp-6-3131-2006, 2006.
Arey, J., Aschmann, S. M., Kwok, E. S. C., and Atkinson, R.: Alkyl nitrate, hydroxyalkyl nitrate, and hydroxycarbonyl formation from the nox–air photooxidations of C5-C8 n-alkanes, J. Phys. Chem. A., 105, 1020–1027, https://doi.org/10.1021/jp003292z, 2001.
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This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed efficiently via the uptake of ammonia by newly formed secondary organic aerosol using a smog chamber equipped with a HR-ToF-AMS. Based on the measured kinetics, this study suggests that light absorption by NOC in atmospheric particles may be important in regions where the BC contribution is minimal and NOC from ammonia should be considered with respect to overall deposition of nitrogen to ecosystems.
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed...
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