Articles | Volume 15, issue 23
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Reactive uptake of ammonia to secondary organic aerosols: kinetics of organonitrogen formation
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
State Key Joint Laboratory of Environmental Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China
J. Liggio
CORRESPONDING AUTHOR
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
R. Staebler
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
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80 citations as recorded by crossref.
- Experimental study on synchrotron radiation photoionization of secondary organic aerosol derived from styrene ozonolysis M. Huang et al. 10.1002/jccs.202200557
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- Influence of Ammonium Sulfate Seed Particle on Optics and Compositions of Toluene Derived Organic Aerosol in Photochemistry T. Lu et al. 10.3390/atmos11090961
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- Abundant nitrogenous secondary organic aerosol formation accelerated by cloud processing Z. Liu et al. 10.1016/j.isci.2023.108317
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- Effect of Humidity on the Reactive Uptake of Ammonia and Dimethylamine by Nitrogen-Containing Secondary Organic Aerosol N. Smith et al. 10.3390/atmos12111502
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
- Heterogeneous reaction of toluene/NO2/O3 on α-Fe2O3 nanoparticles: the impacts of O3, light illumination, and relative humidity on the formation of N-containing organic compounds (NOC) X. He et al. 10.1039/D2EN00426G
- Atmospheric aerosol chemistry and source apportionment of PM10 using stable carbon isotopes and PMF modelling during fireworks over Hyderabad, southern India P. Attri et al. 10.1016/j.heliyon.2024.e26746
- Nanocluster aerosol formation via ozone chemistry on worn clothing: Influence of environmental parameters S. Yang & D. Licina 10.1016/j.buildenv.2024.111474
- Exploring the formation potential and optical properties of secondary organic aerosol from the photooxidation of selected short aliphatic ethers J. Zhu et al. 10.1016/j.jes.2020.03.050
- A novel reaction between ammonia and Criegee intermediates can form amines and suppress oligomers from isoprene X. Li et al. 10.1016/j.scitotenv.2024.177389
- Knudsen cell studies of the uptake of gaseous ammonia and amines onto C3–C7 solid dicarboxylic acids M. Fairhurst et al. 10.1039/C7CP05252A
- Joint impact of atmospheric SO2and NH3on the formation of nanoparticles from photo-oxidation of a typical biomass burning compound X. Jiang et al. 10.1039/D0EN00520G
- Development of an inorganic and organic aerosol model (CHIMERE 2017<i>β</i> v1.0): seasonal and spatial evaluation over Europe F. Couvidat et al. 10.5194/gmd-11-165-2018
- Synergetic effects of NH<sub>3</sub> and NO<sub><i>x</i></sub> on the production and optical absorption of secondary organic aerosol formation from toluene photooxidation S. Liu et al. 10.5194/acp-21-17759-2021
- Continuous Measurement and Molecular Compositions of Atmospheric Water‐Soluble Brown Carbon in the Nearshore Marine Boundary Layer of Northern China: Secondary Formation and Influencing Factors H. Li et al. 10.1029/2023JD038565
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- A new method for the determination of imidazole-like brown carbons using gas chromatography-mass spectrometry P. Chen et al. 10.1016/j.apr.2023.101701
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- Dark Iron-Catalyzed Reactions in Acidic and Viscous Aerosol Systems Efficiently Form Secondary Brown Carbon H. Al-Abadleh et al. 10.1021/acs.est.0c05678
- Secondary organic aerosol formation from the OH-initiated oxidation of guaiacol under different experimental conditions C. Liu et al. 10.1016/j.atmosenv.2019.03.021
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- The effects of humidity and ammonia on the chemical composition of secondary aerosols from toluene/NOx photo-oxidation L. Chen et al. 10.1016/j.scitotenv.2020.138671
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- Characterization of Imidazole Compounds in Aqueous Secondary Organic Aerosol Generated from Evaporation of Droplets Containing Pyruvaldehyde and Inorganic Ammonium X. Lin et al. 10.3390/atmos13060970
- Urgency of controlling agricultural nitrogen sources to alleviate summertime air pollution in the North China Plain R. Wang et al. 10.1016/j.chemosphere.2022.137124
- Airborne flux measurements of ammonia over the southern Great Plains using chemical ionization mass spectrometry S. Schobesberger et al. 10.5194/amt-16-247-2023
- The heterogeneous reactions of toluene/O3/NH3 on hematite nanoparticles: the impact of light illumination on organic ammonium salt formation X. Liu et al. 10.1039/D3EN00625E
- Influence of Inorganic Gases on Formation and Chemical Composition of Monoaromatic Hydrocarbons Secondary Organic Aerosol J. XU & M. HUANG 10.1016/S1872-2040(20)60008-1
- Hygroscopicity of nitrogen-containing organic carbon compounds: o-aminophenol and p-aminophenol K. Malek et al. 10.1039/D2EM00163B
- The properties and behavior of α-pinene secondary organic aerosol particles exposed to ammonia under dry conditions D. Bell et al. 10.1039/C6CP08839B
- Enhanced organic aerosol formation induced by inorganic aerosol formed in laboratory photochemical experiments A. Ali et al. 10.1016/j.jaerosci.2024.106481
- High secondary formation of nitrogen-containing organics (NOCs) and its possible link to oxidized organics and ammonium G. Zhang et al. 10.5194/acp-20-1469-2020
- Black carbon in the Lower Fraser Valley, British Columbia: Impact of 2017 wildfires on local air quality and aerosol optical properties R. Healy et al. 10.1016/j.atmosenv.2019.116976
- Photochemical Oxidation of Water-Soluble Organic Carbon (WSOC) on Mineral Dust and Enhanced Organic Ammonium Formation T. Wang et al. 10.1021/acs.est.0c04616
- Atmospheric evolution of emissions from a boreal forest fire: the formation of highly functionalized oxygen-, nitrogen-, and sulfur-containing organic compounds J. Ditto et al. 10.5194/acp-21-255-2021
- Anthropogenic–Biogenic Interactions at Night: Enhanced Formation of Secondary Aerosols and Particulate Nitrogen- and Sulfur-Containing Organics from β-Pinene Oxidation L. Xu et al. 10.1021/acs.est.0c07879
- Synergetic formation of secondary inorganic and organic aerosol: effect of SO<sub>2</sub> and NH<sub>3</sub> on particle formation and growth B. Chu et al. 10.5194/acp-16-14219-2016
- Reactivity of aminophenols in forming nitrogen-containing brown carbon from iron-catalyzed reactions H. Al-Abadleh et al. 10.1038/s42004-022-00732-1
- Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain Y. Liu et al. 10.1038/s41467-022-34733-4
- Molecular Characterization of Water‐Soluble Brown Carbon Chromophores in Beijing, China C. Yan et al. 10.1029/2019JD032018
- Oil sands operations as a large source of secondary organic aerosols J. Liggio et al. 10.1038/nature17646
- Long-path measurements of pollutants and micrometeorology over Highway 401 in Toronto Y. You et al. 10.5194/acp-17-14119-2017
- Heterogeneous interactions between SO<sub>2</sub> and organic peroxides in submicron aerosol S. Wang et al. 10.5194/acp-21-6647-2021
- A comparative study on the formation of nitrogen-containing organic compounds in cloud droplets and aerosol particles G. Zhang et al. 10.1016/j.jes.2024.01.026
- Enhancing effect of NO2 on the formation of light-absorbing secondary organic aerosols from toluene photooxidation S. Liu et al. 10.1016/j.scitotenv.2021.148714
- The impact of ammonium on the distillation of organic carbon in PM2.5 Z. Feng et al. 10.1016/j.scitotenv.2021.150012
- NH3 Weakens the Enhancing Effect of SO2 on Biogenic Secondary Organic Aerosol Formation L. Du et al. 10.1021/acs.estlett.2c00959
- Review of brown carbon aerosols: Recent progress and perspectives J. Yan et al. 10.1016/j.scitotenv.2018.04.083
- Chemical and optical characterization of aqueous secondary organic aerosol generated by reaction of pyruvaldehyde with sodium sulfite M. Zhu et al. 10.1016/j.apr.2024.102124
- Ammonia combustion and emissions in practical applications: a review M. Alnajideen et al. 10.1007/s43979-024-00088-6
- SO<sub>2</sub> and NH<sub>3</sub> emissions enhance organosulfur compounds and fine particle formation from the photooxidation of a typical aromatic hydrocarbon Z. Yang et al. 10.5194/acp-21-7963-2021
- Evidence for the Formation of Imidazole from Carbonyls and Reduced Nitrogen Species at the Individual Particle Level in the Ambient Atmosphere X. Lian et al. 10.1021/acs.estlett.0c00722
- Review of the influencing factors of secondary organic aerosol formation and aging mechanism based on photochemical smog chamber simulation methods Y. Zhang et al. 10.1016/j.jes.2022.10.033
- Evolution of nucleophilic high molecular-weight organic compounds in ambient aerosols: a case study C. He et al. 10.5194/acp-24-1627-2024
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2 citations as recorded by crossref.
- Sources and Impacts of Atmospheric NH3: Current Understanding and Frontiers for Modeling, Measurements, and Remote Sensing in North America L. Zhu et al. 10.1007/s40726-015-0010-4
- Influence of NH3 on secondary organic aerosols from the ozonolysis and photooxidation of α-pinene in a flow reactor Z. Babar et al. 10.1016/j.atmosenv.2017.05.034
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Latest update: 21 Nov 2024
Short summary
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed efficiently via the uptake of ammonia by newly formed secondary organic aerosol using a smog chamber equipped with a HR-ToF-AMS. Based on the measured kinetics, this study suggests that light absorption by NOC in atmospheric particles may be important in regions where the BC contribution is minimal and NOC from ammonia should be considered with respect to overall deposition of nitrogen to ecosystems.
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed...
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