Articles | Volume 15, issue 23
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Reactive uptake of ammonia to secondary organic aerosols: kinetics of organonitrogen formation
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
State Key Joint Laboratory of Environmental Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China
J. Liggio
CORRESPONDING AUTHOR
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
R. Staebler
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
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52 citations as recorded by crossref.
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- Knudsen cell studies of the uptake of gaseous ammonia and amines onto C3–C7 solid dicarboxylic acids M. Fairhurst et al. 10.1039/C7CP05252A
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- Smog chamber study of the effects of NOx and NH3 on the formation of secondary organic aerosols and optical properties from photo-oxidation of toluene X. Qi et al. 10.1016/j.scitotenv.2020.138632
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- Aqueous Reaction of Dicarbonyls with Ammonia as a Potential Source of Organic Nitrogen in Airborne Nanoparticles C. Stangl & M. Johnston 10.1021/acs.jpca.7b02464
- Chemical analysis of particulate products of aged 1,3,5-trimethylbenzene secondary organic aerosol in the presence of ammonia M. Huang et al. 10.1016/j.apr.2017.08.003
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2 citations as recorded by crossref.
- Sources and Impacts of Atmospheric NH3: Current Understanding and Frontiers for Modeling, Measurements, and Remote Sensing in North America L. Zhu et al. 10.1007/s40726-015-0010-4
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Latest update: 07 Jun 2023
Short summary
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed efficiently via the uptake of ammonia by newly formed secondary organic aerosol using a smog chamber equipped with a HR-ToF-AMS. Based on the measured kinetics, this study suggests that light absorption by NOC in atmospheric particles may be important in regions where the BC contribution is minimal and NOC from ammonia should be considered with respect to overall deposition of nitrogen to ecosystems.
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed...
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