Articles | Volume 15, issue 23
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-13569-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Reactive uptake of ammonia to secondary organic aerosols: kinetics of organonitrogen formation
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
State Key Joint Laboratory of Environmental Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China
J. Liggio
CORRESPONDING AUTHOR
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
R. Staebler
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
Atmospheric Science and Technology Directorate, Science and Technology Branch, Environment Canada, Toronto, M3H 5T4, Canada
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- Molecular Characterization of Water‐Soluble Brown Carbon Chromophores in Beijing, China C. Yan et al. 10.1029/2019JD032018
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- Long-path measurements of pollutants and micrometeorology over Highway 401 in Toronto Y. You et al. 10.5194/acp-17-14119-2017
- Heterogeneous interactions between SO<sub>2</sub> and organic peroxides in submicron aerosol S. Wang et al. 10.5194/acp-21-6647-2021
- A comparative study on the formation of nitrogen-containing organic compounds in cloud droplets and aerosol particles G. Zhang et al. 10.1016/j.jes.2024.01.026
- Enhancing effect of NO2 on the formation of light-absorbing secondary organic aerosols from toluene photooxidation S. Liu et al. 10.1016/j.scitotenv.2021.148714
- The impact of ammonium on the distillation of organic carbon in PM2.5 Z. Feng et al. 10.1016/j.scitotenv.2021.150012
- NH3 Weakens the Enhancing Effect of SO2 on Biogenic Secondary Organic Aerosol Formation L. Du et al. 10.1021/acs.estlett.2c00959
- Review of brown carbon aerosols: Recent progress and perspectives J. Yan et al. 10.1016/j.scitotenv.2018.04.083
- Chemical and optical characterization of aqueous secondary organic aerosol generated by reaction of pyruvaldehyde with sodium sulfite M. Zhu et al. 10.1016/j.apr.2024.102124
- Ammonia combustion and emissions in practical applications: a review M. Alnajideen et al. 10.1007/s43979-024-00088-6
- SO<sub>2</sub> and NH<sub>3</sub> emissions enhance organosulfur compounds and fine particle formation from the photooxidation of a typical aromatic hydrocarbon Z. Yang et al. 10.5194/acp-21-7963-2021
- Evidence for the Formation of Imidazole from Carbonyls and Reduced Nitrogen Species at the Individual Particle Level in the Ambient Atmosphere X. Lian et al. 10.1021/acs.estlett.0c00722
- Review of the influencing factors of secondary organic aerosol formation and aging mechanism based on photochemical smog chamber simulation methods Y. Zhang et al. 10.1016/j.jes.2022.10.033
- Evolution of nucleophilic high molecular-weight organic compounds in ambient aerosols: a case study C. He et al. 10.5194/acp-24-1627-2024
- Comprehensive study about the heterogeneous conversion of NH3on nanoscale TiO2particles: insight into the mechanism and atmospheric implications Q. Ma et al. 10.1039/D2EN00966H
- Influence of Ammonia and Relative Humidity on the Formation and Composition of Secondary Brown Carbon from Oxidation of 1-Methylnaphthalene and Longifolene Y. Cui et al. 10.1021/acsearthspacechem.0c00353
- Effect of NOx and RH on the secondary organic aerosol formation from toluene photooxidation S. Liu et al. 10.1016/j.jes.2021.06.017
2 citations as recorded by crossref.
- Sources and Impacts of Atmospheric NH3: Current Understanding and Frontiers for Modeling, Measurements, and Remote Sensing in North America L. Zhu et al. 10.1007/s40726-015-0010-4
- Influence of NH3 on secondary organic aerosols from the ozonolysis and photooxidation of α-pinene in a flow reactor Z. Babar et al. 10.1016/j.atmosenv.2017.05.034
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Latest update: 13 Nov 2024
Short summary
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed efficiently via the uptake of ammonia by newly formed secondary organic aerosol using a smog chamber equipped with a HR-ToF-AMS. Based on the measured kinetics, this study suggests that light absorption by NOC in atmospheric particles may be important in regions where the BC contribution is minimal and NOC from ammonia should be considered with respect to overall deposition of nitrogen to ecosystems.
This work for the first time demonstrated that organonitrogen compounds (NOC) can be formed...
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