Articles | Volume 24, issue 10
https://doi.org/10.5194/acp-24-6219-2024
https://doi.org/10.5194/acp-24-6219-2024
Research article
 | 
28 May 2024
Research article |  | 28 May 2024

The impact of multi-decadal changes in VOC speciation on urban ozone chemistry: a case study in Birmingham, United Kingdom

Jianghao Li, Alastair C. Lewis, Jim R. Hopkins, Stephen J. Andrews, Tim Murrells, Neil Passant, Ben Richmond, Siqi Hou, William J. Bloss, Roy M. Harrison, and Zongbo Shi

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Cited articles

Abernethy, S., O'Connor, F., Jones, C., and Jackson, R.: Methane removal and the proportional reductions in surface temperature and ozone, Philos. T. R. Soc. A, 379, 20210104, https://doi.org/10.1098/rsta.2021.0104, 2021. 
Calvert, J. G., Orlando, J. J., Stockwell, W. R., and Wallington, T. J.: The mechanisms of reactions influencing atmospheric ozone, University of Oxford, ISBN 978-0-19-023302-0, 2015. 
Chen, T., Xue, L., Zheng, P., Zhang, Y., Liu, Y., Sun, J., Han, G., Li, H., Zhang, X., Li, Y., Li, H., Dong, C., Xu, F., Zhang, Q., and Wang, W.: Volatile organic compounds and ozone air pollution in an oil production region in northern China, Atmos. Chem. Phys., 20, 7069–7086, https://doi.org/10.5194/acp-20-7069-2020, 2020. 
Cliff, S. J., Lewis, A. C., Shaw, M. D., Lee, J. D., Flynn, M., Andrews, S. J., Hopkins, J. R., Purvis, R. M., and Yeoman, A. M.: Unreported VOC emissions from road transport including from electric vehicles, Environ. Sci. Technol., 57, 8026–8034, https://doi.org/10.1021/acs.est.3c00845, 2023. 
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Short summary
A summertime ozone event at an urban site in Birmingham is sensitive to volatile organic compounds (VOCs) – particularly those of oxygenated VOCs. The roles of anthropogenic VOC sources in urban ozone chemistry are examined by integrating the 1990–2019 national atmospheric emission inventory into model scenarios. Road transport remains the most powerful means of further reducing ozone in this case study, but the benefits may be offset if solvent emissions of VOCs continue to increase.
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