Articles | Volume 23, issue 18
https://doi.org/10.5194/acp-23-10439-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-10439-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Air pollution reductions caused by the COVID-19 lockdown open up a way to preserve the Himalayan glaciers
Centre for climate change
research, Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, India
Bernd Heinold
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
T. P. Sabin
Centre for climate change
research, Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, India
Anne Kubin
Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany
Katty Huang
Urban Climate, Risk & Health, UCL, London, UK
Alexandru Rap
School of Earth and Environment, University of Leeds, Leeds, UK
Rolf Müller
Institute of Energy and Climate Research (IEK-7), Forschungszentrum Jülich, Jülich, Germany
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Shubhajyoti Roy, Satheesh P. R. Chandran, Suvarna Fadnavis, Vijay Sagar, Michaela I. Hegglin, and Rolf Müller
EGUsphere, https://doi.org/10.5194/egusphere-2025-1098, https://doi.org/10.5194/egusphere-2025-1098, 2025
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We show stratospheric ozone intrusions associated with sudden stratospheric warming events enhance ozone in the lower troposphere over the South Asia. The ozone enhancement increases ozone radiative forcing by 0.04±0.03 W.m-2 over South Asia. This increase in ozone radiative forcing potentially exacerbates regional climate warming.
Hazel Vernier, Demilson Quintão, Bruno Biazon, Eduardo Landulfo, Giovanni Souza, V. Amanda Santos, J. S. Fabio Lopes, C. P. Alex Mendes, A. S. José da Matta, K. Pinheiro Damaris, Benoit Grosslin, P. M. P. Maria Jorge, Maria de Fátima Andrade, Neeraj Rastogi, Akhil Raj, Hongyu Liu, Mahesh Kovilakam, Suvarna Fadnavis, Frank G. Wienhold, Mathieu Colombier, D. Chris Boone, Gwenael Berthet, Nicolas Dumelie, Lilian Joly, and Jean-Paul Vernier
EGUsphere, https://doi.org/10.5194/egusphere-2025-924, https://doi.org/10.5194/egusphere-2025-924, 2025
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The eruption of Hunga Tonga-Hunga Ha'apai injected large amounts of water vapor and sea salt into the stratosphere, altering traditional views of volcanic aerosols. Using balloon-borne samplers, we collected aerosol samples and found high levels of sea salt and calcium, suggesting sulfate depletion due to gypsum formation. These findings highlight the need to consider sea salt in climate models to better predict volcanic impacts on the atmosphere and climate.
Prashant Chavan, Suvarna Fadnavis, Anton Laakso, Jean-Paul Vernier, Simone Tilmes, and Rolf Müller
EGUsphere, https://doi.org/10.5194/egusphere-2024-3825, https://doi.org/10.5194/egusphere-2024-3825, 2025
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Our simulations with volcanoes, when compared without volcanoes, show that volcanic aerosol precursors enter the tropical stratosphere, propagating upward and enhancing sulphate aerosol and heating. This stratospheric heating caused by the volcanoes reduces the amplitude of the QBO and disrupts its phases. Since QBO also modulates tropical convection and weather, we suggest including volcanic emissions and the QBO in the weather prediction model for a better forecast.
Yasin Elshorbany, Jerald R. Ziemke, Sarah Strode, Hervé Petetin, Kazuyuki Miyazaki, Isabelle De Smedt, Kenneth Pickering, Rodrigo J. Seguel, Helen Worden, Tamara Emmerichs, Domenico Taraborrelli, Maria Cazorla, Suvarna Fadnavis, Rebecca R. Buchholz, Benjamin Gaubert, Néstor Y. Rojas, Thiago Nogueira, Thérèse Salameh, and Min Huang
Atmos. Chem. Phys., 24, 12225–12257, https://doi.org/10.5194/acp-24-12225-2024, https://doi.org/10.5194/acp-24-12225-2024, 2024
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We investigated tropospheric ozone spatial variability and trends from 2005 to 2019 and related those to ozone precursors on global and regional scales. We also investigate the spatiotemporal characteristics of the ozone formation regime in relation to ozone chemical sources and sinks. Our analysis is based on remote sensing products of the tropospheric column of ozone and its precursors, nitrogen dioxide, formaldehyde, and total column CO, as well as ozonesonde data and model simulations.
Jan Clemens, Bärbel Vogel, Lars Hoffmann, Sabine Griessbach, Nicole Thomas, Suvarna Fadnavis, Rolf Müller, Thomas Peter, and Felix Ploeger
Atmos. Chem. Phys., 24, 763–787, https://doi.org/10.5194/acp-24-763-2024, https://doi.org/10.5194/acp-24-763-2024, 2024
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The source regions of the Asian tropopause aerosol layer (ATAL) are debated. We use balloon-borne measurements of the layer above Nainital (India) in August 2016 and atmospheric transport models to find ATAL source regions. Most air originated from the Tibetan plateau. However, the measured ATAL was stronger when more air originated from the Indo-Gangetic Plain and weaker when more air originated from the Pacific. Hence, the results indicate important anthropogenic contributions to the ATAL.
Suvarna Fadnavis, Prashant Chavan, Akash Joshi, Sunil M. Sonbawne, Asutosh Acharya, Panuganti C. S. Devara, Alexandru Rap, Felix Ploeger, and Rolf Müller
Atmos. Chem. Phys., 22, 7179–7191, https://doi.org/10.5194/acp-22-7179-2022, https://doi.org/10.5194/acp-22-7179-2022, 2022
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We show that large amounts of anthropogenic aerosols are transported from South Asia to the northern Indian Ocean. These aerosols are then lifted into the UTLS by the ascending branch of the Hadley circulation. They are further transported to the Southern Hemisphere and downward via westerly ducts over the tropical Atlantic and Pacific. These aerosols increase tropospheric heating, resulting in an increase in water vapor, which is then transported to the UTLS.
Prashant Chavan, Suvarna Fadnavis, Tanusri Chakroborty, Christopher E. Sioris, Sabine Griessbach, and Rolf Müller
Atmos. Chem. Phys., 21, 14371–14384, https://doi.org/10.5194/acp-21-14371-2021, https://doi.org/10.5194/acp-21-14371-2021, 2021
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Biomass burning (BB) over Asia is a strong source of carbonaceous aerosols during spring. Here, we show an outflow of Asian BB carbonaceous aerosols into the UTLS. These aerosols enhance atmospheric heating and produce circulation changes that lead to the enhancement of water vapor in the UTLS over the tropics. In the stratosphere, water vapor is further transported to the South Pole by the Brewer–Dobson circulation. Enhancement of water vapor in the UTLS has implications for climate change.
Teresa Jorge, Simone Brunamonti, Yann Poltera, Frank G. Wienhold, Bei P. Luo, Peter Oelsner, Sreeharsha Hanumanthu, Bhupendra B. Singh, Susanne Körner, Ruud Dirksen, Manish Naja, Suvarna Fadnavis, and Thomas Peter
Atmos. Meas. Tech., 14, 239–268, https://doi.org/10.5194/amt-14-239-2021, https://doi.org/10.5194/amt-14-239-2021, 2021
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Balloon-borne frost point hygrometers are crucial for the monitoring of water vapour in the upper troposphere and lower stratosphere. We found that when traversing a mixed-phase cloud with big supercooled droplets, the intake tube of the instrument collects on its inner surface a high percentage of these droplets. The newly formed ice layer will sublimate at higher levels and contaminate the measurement. The balloon is also a source of contamination, but only at higher levels during the ascent.
Sreeharsha Hanumanthu, Bärbel Vogel, Rolf Müller, Simone Brunamonti, Suvarna Fadnavis, Dan Li, Peter Ölsner, Manish Naja, Bhupendra Bahadur Singh, Kunchala Ravi Kumar, Sunil Sonbawne, Hannu Jauhiainen, Holger Vömel, Beiping Luo, Teresa Jorge, Frank G. Wienhold, Ruud Dirkson, and Thomas Peter
Atmos. Chem. Phys., 20, 14273–14302, https://doi.org/10.5194/acp-20-14273-2020, https://doi.org/10.5194/acp-20-14273-2020, 2020
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During boreal summer, anthropogenic sources yield the Asian Tropopause Aerosol Layer (ATAL), found in Asia between about 13 and 18 km altitude. Balloon-borne measurements of the ATAL conducted in northern India in 2016 show the strong variability of the ATAL. To explain its observed variability, model simulations are performed to deduce the origin of air masses on the Earth's surface, which is important to develop recommendations for regulations of anthropogenic surface emissions of the ATAL.
Suvarna Fadnavis, Yasin Elshorbany, Jerald Ziemke, Brice Barret, Alexandru Rap, P. R. Satheesh Chandran, Richard J. Pope, Vijay Sagar, Domenico Taraborrelli, Eric Le Flochmoen, Juan Cuesta, Catherine Wespes, Folkert Boersma, Isolde Glissenaar, Isabelle De Smedt, Michel Van Roozendael, Hervé Petetin, and Isidora Anglou
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Satellites and model simulations show enhancement in tropospheric ozone, which is highly impacted by human-produced nitrous oxides compared to volatile organic compounds. The increased amount of ozone enhances ozone radiative forcing. The ozone enhancement and associated radiative forcing are the highest over South and East Asia. The emissions of nitrous oxides show a higher influence on shifting ozone photochemical regimes than volatile organic compounds.
Anisbel Leon-Marcos, Moritz Zeising, Manuela van Pinxteren, Sebastian Zeppenfeld, Astrid Bracher, Elena Barbaro, Anja Engel, Matteo Feltracco, Ina Tegen, and Bernd Heinold
Geosci. Model Dev., 18, 4183–4213, https://doi.org/10.5194/gmd-18-4183-2025, https://doi.org/10.5194/gmd-18-4183-2025, 2025
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This study represents the primary marine organic aerosol (PMOA) emissions, focusing on their sea–atmosphere transfer. Using the FESOM2.1–REcoM3 model, concentrations of key organic biomolecules were estimated and integrated into the ECHAM6.3–HAM2.3 aerosol–climate model. Results highlight the influence of marine biological activity and surface winds on PMOA emissions, with reasonably good agreement with observations improving aerosol representation in the southern oceans.
Anisbel Leon-Marcos, Manuela van Pinxteren, Sebastian Zeppenfeld, Moritz Zeising, Astrid Bracher, Laurent Oziel, Ina Tegen, and Bernd Heinold
EGUsphere, https://doi.org/10.5194/egusphere-2025-2829, https://doi.org/10.5194/egusphere-2025-2829, 2025
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This study links modelled ocean surface concentrations of key marine organic groups with the aerosol-climate model ECHAM-HAM to quantify species-resolved primary marine organic aerosol emissions from 1990 to 2019. Results show strong seasonality, driven by productivity and summer sea ice loss. Emissions and burdens increased over time with more frequent positive anomalies in the last decade, revealing an overall upward trend with regional differences across the Arctic and aerosol species.
Rolf Müller, Lennart Bengtsson, John Birks, John Burrows, Ruprecht Jaenicke, and Richard S. Stolarski
Hist. Geo Space. Sci. Discuss., https://doi.org/10.5194/hgss-2025-2, https://doi.org/10.5194/hgss-2025-2, 2025
Revised manuscript accepted for HGSS
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This paper reports a few anecdotes from the life of Paul Crutzen, which were contributed by friends and colleagues. Taken together these anecdotes should shed some light on the person Paul Crutzen, which is perhaps less visible, when focusing only on his scientific achievements.
Weiyu Zhang, Paul R. Field, Kwinten Van Weverberg, Piers M. Forster, Cyril J. Morcrette, and Alexandru Rap
EGUsphere, https://doi.org/10.5194/egusphere-2025-2045, https://doi.org/10.5194/egusphere-2025-2045, 2025
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Contrail cirrus is the largest, yet the most uncertain, aviation climate impact term. A newly implemented contrail cirrus scheme in a double-moment cloud microphysics scheme in climate model realistically reproduces the contrail evolution and provides regional forcing estimates within the range reported by other models. The work highlights the importance of initial contrail characteristics and the need for detailed cloud particle representations in climate model contrail simulations.
Oleh Kachula, Bärbel Vogel, Gebhard Günther, and Rolf Müller
EGUsphere, https://doi.org/10.5194/egusphere-2025-1670, https://doi.org/10.5194/egusphere-2025-1670, 2025
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We propose a novel method to define the boundary of the Asian summer monsoon anticyclone (ASMA) and provide the inter-annual and intra-seasonal analyses based on 44 years (1980–2023) and highlight individual years – 2017, 2022 and 2023 during which aircraft campaigns StratoClim, ACCLIP and PHILEAS took place respectively. Our method shows consistent results with previous studies but also provide new information about possible bimodality of the ASMA and inter-annual decrease of the ASMA area.
Shubhajyoti Roy, Satheesh P. R. Chandran, Suvarna Fadnavis, Vijay Sagar, Michaela I. Hegglin, and Rolf Müller
EGUsphere, https://doi.org/10.5194/egusphere-2025-1098, https://doi.org/10.5194/egusphere-2025-1098, 2025
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We show stratospheric ozone intrusions associated with sudden stratospheric warming events enhance ozone in the lower troposphere over the South Asia. The ozone enhancement increases ozone radiative forcing by 0.04±0.03 W.m-2 over South Asia. This increase in ozone radiative forcing potentially exacerbates regional climate warming.
Hazel Vernier, Demilson Quintão, Bruno Biazon, Eduardo Landulfo, Giovanni Souza, V. Amanda Santos, J. S. Fabio Lopes, C. P. Alex Mendes, A. S. José da Matta, K. Pinheiro Damaris, Benoit Grosslin, P. M. P. Maria Jorge, Maria de Fátima Andrade, Neeraj Rastogi, Akhil Raj, Hongyu Liu, Mahesh Kovilakam, Suvarna Fadnavis, Frank G. Wienhold, Mathieu Colombier, D. Chris Boone, Gwenael Berthet, Nicolas Dumelie, Lilian Joly, and Jean-Paul Vernier
EGUsphere, https://doi.org/10.5194/egusphere-2025-924, https://doi.org/10.5194/egusphere-2025-924, 2025
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The eruption of Hunga Tonga-Hunga Ha'apai injected large amounts of water vapor and sea salt into the stratosphere, altering traditional views of volcanic aerosols. Using balloon-borne samplers, we collected aerosol samples and found high levels of sea salt and calcium, suggesting sulfate depletion due to gypsum formation. These findings highlight the need to consider sea salt in climate models to better predict volcanic impacts on the atmosphere and climate.
Prashant Chavan, Suvarna Fadnavis, Anton Laakso, Jean-Paul Vernier, Simone Tilmes, and Rolf Müller
EGUsphere, https://doi.org/10.5194/egusphere-2024-3825, https://doi.org/10.5194/egusphere-2024-3825, 2025
Preprint archived
Short summary
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Our simulations with volcanoes, when compared without volcanoes, show that volcanic aerosol precursors enter the tropical stratosphere, propagating upward and enhancing sulphate aerosol and heating. This stratospheric heating caused by the volcanoes reduces the amplitude of the QBO and disrupts its phases. Since QBO also modulates tropical convection and weather, we suggest including volcanic emissions and the QBO in the weather prediction model for a better forecast.
Weiyu Zhang, Kwinten Van Weverberg, Cyril J. Morcrette, Wuhu Feng, Kalli Furtado, Paul R. Field, Chih-Chieh Chen, Andrew Gettelman, Piers M. Forster, Daniel R. Marsh, and Alexandru Rap
Atmos. Chem. Phys., 25, 473–489, https://doi.org/10.5194/acp-25-473-2025, https://doi.org/10.5194/acp-25-473-2025, 2025
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Contrail cirrus is the largest, but also most uncertain, contribution of aviation to global warming. We evaluate, for the first time, the impact of the host climate model on contrail cirrus properties. Substantial differences exist between contrail cirrus formation, persistence, and radiative effects in the host climate models. Reliable contrail cirrus simulations require advanced representation of cloud optical properties and microphysics, which should be better constrained by observations.
Kieran M. R. Hunt, Jean-Philippe Baudouin, Andrew G. Turner, A. P. Dimri, Ghulam Jeelani, Pooja, Rajib Chattopadhyay, Forest Cannon, T. Arulalan, M. S. Shekhar, T. P. Sabin, and Eliza Palazzi
Weather Clim. Dynam., 6, 43–112, https://doi.org/10.5194/wcd-6-43-2025, https://doi.org/10.5194/wcd-6-43-2025, 2025
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Western disturbances (WDs) are storms that predominantly affect north India and Pakistan during the winter months, where they play an important role in regional water security, but can also bring a range of natural hazards. In this review, we summarise recent literature across a range of topics: their structure and lifecycle, precipitation and impacts, interactions with large-scale weather patterns, representation in models, how well they are forecast, and their response to changes in climate.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Julian Hofer, Moritz Haarig, Ulla Wandinger, Bernd Heinold, Ina Tegen, Matthias Faust, Holger Baars, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
EGUsphere, https://doi.org/10.5194/egusphere-2024-3159, https://doi.org/10.5194/egusphere-2024-3159, 2024
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This study investigates how hematite (an iron oxide mineral) in the Saharan Desert dust affects how dust particles interact with radiation. Using lidar data from Cabo Verde (2021–2022) and hematite content from atmospheric model simulations, the results show that higher hematite fraction leads to stronger particle backscattering at specific wavelengths. These findings can improve the representaiton of mineral dust in climate models, particularly regarding their radiative effect.
Yiran Zhang-Liu, Rolf Müller, Jens-Uwe Grooß, Sabine Robrecht, Bärbel Vogel, Abdul Mannan Zafar, and Ralph Lehmann
Atmos. Chem. Phys., 24, 12557–12574, https://doi.org/10.5194/acp-24-12557-2024, https://doi.org/10.5194/acp-24-12557-2024, 2024
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HCl null cycles in Antarctica are important for maintaining high values of ozone-destroying chlorine in Antarctic spring. These HCl null cycles are not affected by (1) using the most recent recommendations of chemical kinetics (compared to older recommendations), (2) accounting for dehydration in the Antarctic winter vortex, and (3) considering the observed (but unexplained) depletion of HCl in mid-winter in the Antarctic vortex throughout Antarctic winter.
Yasin Elshorbany, Jerald R. Ziemke, Sarah Strode, Hervé Petetin, Kazuyuki Miyazaki, Isabelle De Smedt, Kenneth Pickering, Rodrigo J. Seguel, Helen Worden, Tamara Emmerichs, Domenico Taraborrelli, Maria Cazorla, Suvarna Fadnavis, Rebecca R. Buchholz, Benjamin Gaubert, Néstor Y. Rojas, Thiago Nogueira, Thérèse Salameh, and Min Huang
Atmos. Chem. Phys., 24, 12225–12257, https://doi.org/10.5194/acp-24-12225-2024, https://doi.org/10.5194/acp-24-12225-2024, 2024
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We investigated tropospheric ozone spatial variability and trends from 2005 to 2019 and related those to ozone precursors on global and regional scales. We also investigate the spatiotemporal characteristics of the ozone formation regime in relation to ozone chemical sources and sinks. Our analysis is based on remote sensing products of the tropospheric column of ozone and its precursors, nitrogen dioxide, formaldehyde, and total column CO, as well as ozonesonde data and model simulations.
Ling Zou, Reinhold Spang, Sabine Griessbach, Lars Hoffmann, Farahnaz Khosrawi, Rolf Müller, and Ines Tritscher
Atmos. Chem. Phys., 24, 11759–11774, https://doi.org/10.5194/acp-24-11759-2024, https://doi.org/10.5194/acp-24-11759-2024, 2024
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This study provided estimates of the occurrence of ice polar stratospheric clouds (PSCs) observed by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) and their connection with temperatures above the frost point (Tice) using a Lagrangian model derived from ERA5. We found that ice PSCs above Tice with temperature fluctuations along the backward trajectory are 33 % in the Arctic and 9 % in the Antarctic. This quantitative assessment enhances our understanding of ice PSCs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Andreas Walbröl, Janosch Michaelis, Sebastian Becker, Henning Dorff, Kerstin Ebell, Irina Gorodetskaya, Bernd Heinold, Benjamin Kirbus, Melanie Lauer, Nina Maherndl, Marion Maturilli, Johanna Mayer, Hanno Müller, Roel A. J. Neggers, Fiona M. Paulus, Johannes Röttenbacher, Janna E. Rückert, Imke Schirmacher, Nils Slättberg, André Ehrlich, Manfred Wendisch, and Susanne Crewell
Atmos. Chem. Phys., 24, 8007–8029, https://doi.org/10.5194/acp-24-8007-2024, https://doi.org/10.5194/acp-24-8007-2024, 2024
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To support the interpretation of the data collected during the HALO-(AC)3 campaign, which took place in the North Atlantic sector of the Arctic from 7 March to 12 April 2022, we analyze how unusual the weather and sea ice conditions were with respect to the long-term climatology. From observations and ERA5 reanalysis, we found record-breaking warm air intrusions and a large variety of marine cold air outbreaks. Sea ice concentration was mostly within the climatological interquartile range.
Jayanarayanan Kuttippurath, Gopalakrishna Pillai Gopikrishnan, Rolf Müller, Sophie Godin-Beekmann, and Jerome Brioude
Atmos. Chem. Phys., 24, 6743–6756, https://doi.org/10.5194/acp-24-6743-2024, https://doi.org/10.5194/acp-24-6743-2024, 2024
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The current understanding and observational evidence do not provide any support for the possibility of an ozone hole occurring outside Antarctica today with respect to the present-day stratospheric halogen levels.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
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Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Felix Ploeger, Thomas Birner, Edward Charlesworth, Paul Konopka, and Rolf Müller
Atmos. Chem. Phys., 24, 2033–2043, https://doi.org/10.5194/acp-24-2033-2024, https://doi.org/10.5194/acp-24-2033-2024, 2024
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We present a novel mechanism of how regional anomalies in water vapour concentrations in the upper troposphere and lower stratosphere impact regional atmospheric circulation systems. These impacts include a displaced upper-level Asian monsoon circulation and strengthened prevailing westerlies in the Pacific region. Current climate models have biases in simulating these regional water vapour anomalies and circulation impacts, but the biases can be avoided by improving the model transport.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Matthias Faust, Holger Baars, Bernd Heinold, Julian Hofer, Ina Tegen, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
Geosci. Model Dev., 17, 1271–1295, https://doi.org/10.5194/gmd-17-1271-2024, https://doi.org/10.5194/gmd-17-1271-2024, 2024
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Mineral dust aerosol particles vary greatly in their composition depending on source region, which leads to different physicochemical properties. Most atmosphere–aerosol models consider mineral dust aerosols to be compositionally homogeneous, which ultimately increases model uncertainty. Here, we present an approach to explicitly consider the heterogeneity of the mineralogical composition for simulations of the Saharan atmospheric dust cycle with regard to dust transport towards the Atlantic.
Reinhold Spang, Rolf Müller, and Alexandru Rap
Atmos. Chem. Phys., 24, 1213–1230, https://doi.org/10.5194/acp-24-1213-2024, https://doi.org/10.5194/acp-24-1213-2024, 2024
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Cirrus clouds play an important role in the radiation budget of the Earth. Despite recent progress in their observation, the radiative impact of ultra-thin cirrus clouds (UTC) in the tropopause region and in the lowermost stratosphere remains poorly constrained. Sensitivity model simulations with different ice parameters provide an uncertainty range for the radiative effect of UTCs. There is a need for better observed UTCs to enable the simulation of their potentially large effect on climate.
Jan Clemens, Bärbel Vogel, Lars Hoffmann, Sabine Griessbach, Nicole Thomas, Suvarna Fadnavis, Rolf Müller, Thomas Peter, and Felix Ploeger
Atmos. Chem. Phys., 24, 763–787, https://doi.org/10.5194/acp-24-763-2024, https://doi.org/10.5194/acp-24-763-2024, 2024
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The source regions of the Asian tropopause aerosol layer (ATAL) are debated. We use balloon-borne measurements of the layer above Nainital (India) in August 2016 and atmospheric transport models to find ATAL source regions. Most air originated from the Tibetan plateau. However, the measured ATAL was stronger when more air originated from the Indo-Gangetic Plain and weaker when more air originated from the Pacific. Hence, the results indicate important anthropogenic contributions to the ATAL.
Bärbel Vogel, C. Michael Volk, Johannes Wintel, Valentin Lauther, Jan Clemens, Jens-Uwe Grooß, Gebhard Günther, Lars Hoffmann, Johannes C. Laube, Rolf Müller, Felix Ploeger, and Fred Stroh
Atmos. Chem. Phys., 24, 317–343, https://doi.org/10.5194/acp-24-317-2024, https://doi.org/10.5194/acp-24-317-2024, 2024
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Over the Indian subcontinent, polluted air is rapidly uplifted to higher altitudes during the Asian monsoon season. We present an assessment of vertical transport in this region using different wind data provided by the European Centre for Medium-Range Weather Forecasts (ECMWF), as well as high-resolution aircraft measurements. In general, our findings confirm that the newest ECMWF reanalysis product, ERA5, yields a better representation of transport compared to the predecessor, ERA-Interim.
Rolf Müller, Ulrich Pöschl, Thomas Koop, Thomas Peter, and Ken Carslaw
Atmos. Chem. Phys., 23, 15445–15453, https://doi.org/10.5194/acp-23-15445-2023, https://doi.org/10.5194/acp-23-15445-2023, 2023
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Paul J. Crutzen was a pioneer in atmospheric sciences and a kind-hearted, humorous person with empathy for the private lives of his colleagues and students. He made fundamental scientific contributions to a wide range of scientific topics in all parts of the atmosphere. Paul was among the founders of the journal Atmospheric Chemistry and Physics. His work will continue to be a guide for generations of scientists and environmental policymakers to come.
Michael Weger and Bernd Heinold
Atmos. Chem. Phys., 23, 13769–13790, https://doi.org/10.5194/acp-23-13769-2023, https://doi.org/10.5194/acp-23-13769-2023, 2023
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This study investigates the effects of complex terrain on air pollution trapping using a numerical model which simulates the dispersion of emissions under real meteorological conditions. The additionally simulated aerosol age allows us to distinguish areas that accumulate aerosol over time from areas that are more influenced by fresh emissions. The Dresden Basin, a widened section of the Elbe Valley in eastern Germany, is selected as the target area in a case study to demonstrate the concept.
Fabian Senf, Bernd Heinold, Anne Kubin, Jason Müller, Roland Schrödner, and Ina Tegen
Atmos. Chem. Phys., 23, 8939–8958, https://doi.org/10.5194/acp-23-8939-2023, https://doi.org/10.5194/acp-23-8939-2023, 2023
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Wildfire smoke is a significant source of airborne atmospheric particles that can absorb sunlight. Extreme fires in particular, such as those during the 2019–2020 Australian wildfire season (Black Summer fires), can considerably affect our climate system. In the present study, we investigate the various effects of Australian smoke using a global climate model to clarify how the Earth's atmosphere, including its circulation systems, adjusted to the extraordinary amount of Australian smoke.
Bernd Heinold, Holger Baars, Boris Barja, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Nick Schutgens, Fabian Senf, Roland Schrödner, Diego Villanueva, and Ina Tegen
Atmos. Chem. Phys., 22, 9969–9985, https://doi.org/10.5194/acp-22-9969-2022, https://doi.org/10.5194/acp-22-9969-2022, 2022
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The extreme 2019–2020 Australian wildfires produced massive smoke plumes lofted into the lower stratosphere by pyrocumulonimbus convection. Most climate models do not adequately simulate the injection height of such intense fires. By combining aerosol-climate modeling with prescribed pyroconvective smoke injection and lidar observations, this study shows the importance of the representation of the most extreme wildfire events for estimating the atmospheric energy budget.
Liubov Poshyvailo-Strube, Rolf Müller, Stephan Fueglistaler, Michaela I. Hegglin, Johannes C. Laube, C. Michael Volk, and Felix Ploeger
Atmos. Chem. Phys., 22, 9895–9914, https://doi.org/10.5194/acp-22-9895-2022, https://doi.org/10.5194/acp-22-9895-2022, 2022
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Brewer–Dobson circulation (BDC) controls the composition of the stratosphere, which in turn affects radiation and climate. As the BDC cannot be measured directly, it is necessary to infer its strength and trends indirectly. In this study, we test in the
model worlddifferent methods for estimating the mean age of air trends based on a combination of stratospheric water vapour and methane data. We also provide simple practical advice of a more reliable estimation of the mean age of air trends.
Suvarna Fadnavis, Prashant Chavan, Akash Joshi, Sunil M. Sonbawne, Asutosh Acharya, Panuganti C. S. Devara, Alexandru Rap, Felix Ploeger, and Rolf Müller
Atmos. Chem. Phys., 22, 7179–7191, https://doi.org/10.5194/acp-22-7179-2022, https://doi.org/10.5194/acp-22-7179-2022, 2022
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We show that large amounts of anthropogenic aerosols are transported from South Asia to the northern Indian Ocean. These aerosols are then lifted into the UTLS by the ascending branch of the Hadley circulation. They are further transported to the Southern Hemisphere and downward via westerly ducts over the tropical Atlantic and Pacific. These aerosols increase tropospheric heating, resulting in an increase in water vapor, which is then transported to the UTLS.
Michael Weger, Holger Baars, Henriette Gebauer, Maik Merkel, Alfred Wiedensohler, and Bernd Heinold
Geosci. Model Dev., 15, 3315–3345, https://doi.org/10.5194/gmd-15-3315-2022, https://doi.org/10.5194/gmd-15-3315-2022, 2022
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Numerical models are an important tool to assess the air quality in cities,
as they can provide near-continouos data in time and space. In this paper,
air pollution for an entire city is simulated at a high spatial resolution of 40 m.
At this spatial scale, the effects of buildings on the atmosphere,
like channeling or blocking of the air flow, are directly represented by diffuse obstacles in the used model CAIRDIO. For model validation, measurements from air-monitoring sites are used.
Valentin Lauther, Bärbel Vogel, Johannes Wintel, Andrea Rau, Peter Hoor, Vera Bense, Rolf Müller, and C. Michael Volk
Atmos. Chem. Phys., 22, 2049–2077, https://doi.org/10.5194/acp-22-2049-2022, https://doi.org/10.5194/acp-22-2049-2022, 2022
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We show airborne in situ measurements of the very short-lived ozone-depleting substances CH2Cl2 and CHCl3, revealing particularly high concentrations of both species in the lower stratosphere. Back-trajectory calculations and 3D model simulations show that the air masses with high concentrations originated in the Asian boundary layer and were transported via the Asian summer monsoon. We also identify a fast transport pathway into the stratosphere via the North American monsoon and by hurricanes.
Dina Khordakova, Christian Rolf, Jens-Uwe Grooß, Rolf Müller, Paul Konopka, Andreas Wieser, Martina Krämer, and Martin Riese
Atmos. Chem. Phys., 22, 1059–1079, https://doi.org/10.5194/acp-22-1059-2022, https://doi.org/10.5194/acp-22-1059-2022, 2022
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Extreme storms transport humidity from the troposphere to the stratosphere. Here it has a strong impact on the climate. With ongoing global warming, we expect more storms and, hence, an enhancement of this effect. A case study was performed in order to measure the impact of the direct injection of water vapor into the lower stratosphere. The measurements displayed a significant transport of water vapor into the lower stratosphere, and this was supported by satellite and reanalysis data.
Prashant Chavan, Suvarna Fadnavis, Tanusri Chakroborty, Christopher E. Sioris, Sabine Griessbach, and Rolf Müller
Atmos. Chem. Phys., 21, 14371–14384, https://doi.org/10.5194/acp-21-14371-2021, https://doi.org/10.5194/acp-21-14371-2021, 2021
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Biomass burning (BB) over Asia is a strong source of carbonaceous aerosols during spring. Here, we show an outflow of Asian BB carbonaceous aerosols into the UTLS. These aerosols enhance atmospheric heating and produce circulation changes that lead to the enhancement of water vapor in the UTLS over the tropics. In the stratosphere, water vapor is further transported to the South Pole by the Brewer–Dobson circulation. Enhancement of water vapor in the UTLS has implications for climate change.
Jayanarayanan Kuttippurath, Wuhu Feng, Rolf Müller, Pankaj Kumar, Sarath Raj, Gopalakrishna Pillai Gopikrishnan, and Raina Roy
Atmos. Chem. Phys., 21, 14019–14037, https://doi.org/10.5194/acp-21-14019-2021, https://doi.org/10.5194/acp-21-14019-2021, 2021
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The Arctic winter/spring 2020 was one of the coldest with a strong and long-lasting vortex, high chlorine activation, severe denitrification, and unprecedented ozone loss. The loss was even equal to the levels of some of the warm Antarctic winters. Total column ozone values below 220 DU for several weeks and ozone loss saturation were observed during the period. These results show an unusual meteorology and warrant dedicated studies on the impact of climate change on ozone loss.
Tobias Peter Bauer, Peter Holtermann, Bernd Heinold, Hagen Radtke, Oswald Knoth, and Knut Klingbeil
Geosci. Model Dev., 14, 4843–4863, https://doi.org/10.5194/gmd-14-4843-2021, https://doi.org/10.5194/gmd-14-4843-2021, 2021
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We present the coupled atmosphere–ocean model system ICONGETM. The added value and potential of using the latest coupling technologies are discussed in detail. An exchange grid handles the different coastlines from the unstructured atmosphere and the structured ocean grids. Due to a high level of automated processing, ICONGETM requires only minimal user input. The application to a coastal upwelling scenario demonstrates significantly improved model results compared to uncoupled simulations.
James Keeble, Birgit Hassler, Antara Banerjee, Ramiro Checa-Garcia, Gabriel Chiodo, Sean Davis, Veronika Eyring, Paul T. Griffiths, Olaf Morgenstern, Peer Nowack, Guang Zeng, Jiankai Zhang, Greg Bodeker, Susannah Burrows, Philip Cameron-Smith, David Cugnet, Christopher Danek, Makoto Deushi, Larry W. Horowitz, Anne Kubin, Lijuan Li, Gerrit Lohmann, Martine Michou, Michael J. Mills, Pierre Nabat, Dirk Olivié, Sungsu Park, Øyvind Seland, Jens Stoll, Karl-Hermann Wieners, and Tongwen Wu
Atmos. Chem. Phys., 21, 5015–5061, https://doi.org/10.5194/acp-21-5015-2021, https://doi.org/10.5194/acp-21-5015-2021, 2021
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Stratospheric ozone and water vapour are key components of the Earth system; changes to both have important impacts on global and regional climate. We evaluate changes to these species from 1850 to 2100 in the new generation of CMIP6 models. There is good agreement between the multi-model mean and observations, although there is substantial variation between the individual models. The future evolution of both ozone and water vapour is strongly dependent on the assumed future emissions scenario.
Michael Weger, Oswald Knoth, and Bernd Heinold
Geosci. Model Dev., 14, 1469–1492, https://doi.org/10.5194/gmd-14-1469-2021, https://doi.org/10.5194/gmd-14-1469-2021, 2021
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A new numerical air-quality transport model for cities is presented, in which buildings are described diffusively. The used diffusive-obstacles approach helps to reduce the computational costs for high-resolution simulations as the grid spacing can be more coarse than in traditional approaches. The research which led to this model development was primarily motivated by the need for a computationally feasible downscaling tool for urban wind and pollution fields from meteorological model output.
Sabine Robrecht, Bärbel Vogel, Simone Tilmes, and Rolf Müller
Atmos. Chem. Phys., 21, 2427–2455, https://doi.org/10.5194/acp-21-2427-2021, https://doi.org/10.5194/acp-21-2427-2021, 2021
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Column ozone protects life on Earth from radiation damage. Stratospheric chlorine compounds cause immense ozone loss in polar winter. Whether similar loss processes can occur in the lower stratosphere above North America today or in future is a matter of debate. We show that these ozone loss processes are very unlikely today or in future independently of whether sulfate geoengineering is applied and that less than 0.1 % of column ozone would be destroyed by this process in any future scenario.
Teresa Jorge, Simone Brunamonti, Yann Poltera, Frank G. Wienhold, Bei P. Luo, Peter Oelsner, Sreeharsha Hanumanthu, Bhupendra B. Singh, Susanne Körner, Ruud Dirksen, Manish Naja, Suvarna Fadnavis, and Thomas Peter
Atmos. Meas. Tech., 14, 239–268, https://doi.org/10.5194/amt-14-239-2021, https://doi.org/10.5194/amt-14-239-2021, 2021
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Balloon-borne frost point hygrometers are crucial for the monitoring of water vapour in the upper troposphere and lower stratosphere. We found that when traversing a mixed-phase cloud with big supercooled droplets, the intake tube of the instrument collects on its inner surface a high percentage of these droplets. The newly formed ice layer will sublimate at higher levels and contaminate the measurement. The balloon is also a source of contamination, but only at higher levels during the ascent.
Sreeharsha Hanumanthu, Bärbel Vogel, Rolf Müller, Simone Brunamonti, Suvarna Fadnavis, Dan Li, Peter Ölsner, Manish Naja, Bhupendra Bahadur Singh, Kunchala Ravi Kumar, Sunil Sonbawne, Hannu Jauhiainen, Holger Vömel, Beiping Luo, Teresa Jorge, Frank G. Wienhold, Ruud Dirkson, and Thomas Peter
Atmos. Chem. Phys., 20, 14273–14302, https://doi.org/10.5194/acp-20-14273-2020, https://doi.org/10.5194/acp-20-14273-2020, 2020
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During boreal summer, anthropogenic sources yield the Asian Tropopause Aerosol Layer (ATAL), found in Asia between about 13 and 18 km altitude. Balloon-borne measurements of the ATAL conducted in northern India in 2016 show the strong variability of the ATAL. To explain its observed variability, model simulations are performed to deduce the origin of air masses on the Earth's surface, which is important to develop recommendations for regulations of anthropogenic surface emissions of the ATAL.
Joram J. D. Hooghiem, Maria Elena Popa, Thomas Röckmann, Jens-Uwe Grooß, Ines Tritscher, Rolf Müller, Rigel Kivi, and Huilin Chen
Atmos. Chem. Phys., 20, 13985–14003, https://doi.org/10.5194/acp-20-13985-2020, https://doi.org/10.5194/acp-20-13985-2020, 2020
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Wildfires release a large quantity of pollutants that can reach the stratosphere through pyro-convection events. In September 2017, a stratospheric plume was accidentally sampled during balloon soundings in northern Finland. The source of the plume was identified to be wildfire smoke based on in situ measurements of carbon monoxide (CO) and stable isotope analysis of CO. Furthermore, the age of the plume was estimated using backwards transport modelling to be ~24 d, with its origin in Canada.
Matthew J. Rowlinson, Alexandru Rap, Douglas S. Hamilton, Richard J. Pope, Stijn Hantson, Steve R. Arnold, Jed O. Kaplan, Almut Arneth, Martyn P. Chipperfield, Piers M. Forster, and Lars Nieradzik
Atmos. Chem. Phys., 20, 10937–10951, https://doi.org/10.5194/acp-20-10937-2020, https://doi.org/10.5194/acp-20-10937-2020, 2020
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Tropospheric ozone is an important greenhouse gas which contributes to anthropogenic climate change; however, the effect of human emissions is uncertain because pre-industrial ozone concentrations are not well understood. We use revised inventories of pre-industrial natural emissions to estimate the human contribution to changes in tropospheric ozone. We find that tropospheric ozone radiative forcing is up to 34 % lower when using improved pre-industrial biomass burning and vegetation emissions.
Christof G. Beer, Johannes Hendricks, Mattia Righi, Bernd Heinold, Ina Tegen, Silke Groß, Daniel Sauer, Adrian Walser, and Bernadett Weinzierl
Geosci. Model Dev., 13, 4287–4303, https://doi.org/10.5194/gmd-13-4287-2020, https://doi.org/10.5194/gmd-13-4287-2020, 2020
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Mineral dust aerosol plays an important role in the climate system. Previously, dust emissions have often been represented in global models by prescribed monthly-mean emission fields representative of a specific year. We now apply an online calculation of wind-driven dust emissions. This results in an improved agreement with observations, due to a better representation of the highly variable dust emissions. Increasing the model resolution led to an additional performance gain.
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Short summary
The influence of the COVID-19 lockdown on the Himalayas caused increases in snow cover and a decrease in runoff, ultimately leading to an enhanced snow water equivalent. Our findings highlight that, out of the two processes causing a retreat of Himalayan glaciers – (1) slow response to global climate change and (2) fast response to local air pollution – a policy action on the latter is more likely to be within the reach of possible policy action to help billions of people in southern Asia.
The influence of the COVID-19 lockdown on the Himalayas caused increases in snow cover and a...
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