Articles | Volume 21, issue 6
https://doi.org/10.5194/acp-21-4453-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-4453-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report: Ice nucleating abilities of biomass burning, African dust, and sea spray aerosol particles over the Yucatán Peninsula
Fernanda Córdoba
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
Posgrado en Ciencias Químicas, Universidad Nacional Autónoma de México, Mexico City, Mexico
Carolina Ramírez-Romero
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
Posgrado en Ciencias de la Tierra, Universidad Nacional Autónoma de México, Mexico City, Mexico
Diego Cabrera
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
Graciela B. Raga
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
Javier Miranda
Instituto de Física, Universidad Nacional Autónoma de México, Mexico City, Mexico
Harry Alvarez-Ospina
Facultad de Ciencias, Universidad Nacional Autónoma de México, Mexico City, Mexico
Daniel Rosas
Facultad de Química, Universidad Autónoma de Yucatán, Mérida, Mexico
Bernardo Figueroa
Laboratorio de Ingeniería y Procesos Costeros, Instituto de Ingeniería, Universidad Nacional Autónoma de México, Sisal, Yucatán, Mexico
Jong Sung Kim
Department of Community Health and Epidemiology, Dalhousie University, Halifax, NS, Canada
Jacqueline Yakobi-Hancock
Department of Community Health and Epidemiology, Dalhousie University, Halifax, NS, Canada
Talib Amador
Facultad de Química, Universidad Autónoma de Yucatán, Mérida, Mexico
Wilfrido Gutierrez
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
deceased
Manuel García
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
Allan K. Bertram
Department of Chemistry, University of British Columbia, Vancouver, BC, Canada
Darrel Baumgardner
Droplet Measurement Technologies, LLC, Colorado, USA
Luis A. Ladino
CORRESPONDING AUTHOR
Centro de Ciencias de la Atmósfera, Universidad Nacional Autónoma de México, Mexico City, Mexico
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Young-Chul Song, Ariana G. Bé, Scot T. Martin, Franz M. Geiger, Allan K. Bertram, Regan J. Thomson, and Mijung Song
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Luisa Ickes, Grace C. E. Porter, Robert Wagner, Michael P. Adams, Sascha Bierbauer, Allan K. Bertram, Merete Bilde, Sigurd Christiansen, Annica M. L. Ekman, Elena Gorokhova, Kristina Höhler, Alexei A. Kiselev, Caroline Leck, Ottmar Möhler, Benjamin J. Murray, Thea Schiebel, Romy Ullrich, and Matthew E. Salter
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W. Richard Leaitch, John K. Kodros, Megan D. Willis, Sarah Hanna, Hannes Schulz, Elisabeth Andrews, Heiko Bozem, Julia Burkart, Peter Hoor, Felicia Kolonjari, John A. Ogren, Sangeeta Sharma, Meng Si, Knut von Salzen, Allan K. Bertram, Andreas Herber, Jonathan P. D. Abbatt, and Jeffrey R. Pierce
Atmos. Chem. Phys., 20, 10545–10563, https://doi.org/10.5194/acp-20-10545-2020, https://doi.org/10.5194/acp-20-10545-2020, 2020
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Black carbon is a factor in the warming of the Arctic atmosphere due to its ability to absorb light, but the uncertainty is high and few observations have been made in the high Arctic above 80° N. We combine airborne and ground-based observations in the springtime Arctic, at and above 80° N, with simulations from a global model to show that light absorption by black carbon may be much larger than modelled. However, the uncertainty remains high.
Cited articles
Ardon-Dryer, K. and Levin, Z.: Ground-based measurements of immersion freezing in the eastern Mediterranean, Atmos. Chem. Phys., 14, 5217–5231, https://doi.org/10.5194/acp-14-5217-2014, 2014. a, b, c, d
Atkinson, J. D., Murray, B. J., Woodhouse, M. T., Whale, T. F., Baustian,
K. J., Carslaw, K. S., Dobbie, S., O'Sullivan, D., and Malkin, T. L.: The
importance of feldspar for ice nucleation by mineral dust in mixed-phase clouds, Nature, 498, 355–358, https://doi.org/10.1038/nature12278, 2013. a
Augustin-Bauditz, S., Wex, H., Kanter, S., Ebert, M., Niedermeier, D., Stolz,
F., Prager, A., and Stratmann, F.: The immersion mode ice nucleation behavior
of mineral dusts: A comparison of different pure and surface modified dusts,
Geophys. Res. Lett., 41, 7375–7382, https://doi.org/10.1002/2014GL061317, 2014. a
Barnes, I., Hjorth, J., and Mihalopoulos, N.: Dimethyl sulfide and dimethyl
sulfoxide and their oxidation in the atmosphere, Chem. Rev., 106, 940–975,
https://doi.org/10.1021/cr020529+, 2006. a
Beall, C. M., Lucero, D., Hill, T. C., DeMott, P. J., Stokes, M. D., and Prather, K. A.: Best practices for precipitation sample storage for offline studies of ice nucleation in marine and coastal environments, Atmos. Meas. Tech., 13, 6473–6486, https://doi.org/10.5194/amt-13-6473-2020, 2020. a
Bigg, E.: Ice nucleus concentrations in remote areas, J. Atmos. Sci., 30,
1153–1157, https://doi.org/10.1175/1520-0469(1973)030<1153:INCIRA>2.0.CO;2, 1973. a
Boose, Y., Sierau, B., García, M. I., Rodríguez, S., Alastuey, A., Linke, C., Schnaiter, M., Kupiszewski, P., Kanji, Z. A., and Lohmann, U.: Ice nucleating particles in the Saharan Air Layer, Atmos. Chem. Phys., 16, 9067–9087, https://doi.org/10.5194/acp-16-9067-2016, 2016. a, b, c
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster,
P., Kerminen, V., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S.,
Sherwood, S., Stevens, B., and Zhang, X.: Clouds and Aerosols in Climate
Change 2013: The Physical Science Basis, Contribution of Working Group I to
IPCC AR5, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 1535 pp., 2013. a, b
Cavazos, T.: Downscaling large-scale circulation to local winter rainfall in
north–eastern Mexico, Int. J. Climatol., 17, 1069–1082,
https://doi.org/10.1002/(SICI)1097-0088(199708)17:10<1069::AID-JOC183>3.0.CO;2-I, 1997. a
Creamean, J. M., Kirpes, R. M., Pratt, K. A., Spada, N. J., Maahn, M., de Boer, G., Schnell, R. C., and China, S.: Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location, Atmos. Chem. Phys., 18, 18023–18042, https://doi.org/10.5194/acp-18-18023-2018, 2018. a
DeMott, P. J., Sassen, K., Poellot, M. R., Baumgardner, D., Rogers, D. C.,
Brooks, S. D., Prenni, A. J., and Kreidenweis, S. M.: African dust aerosols
as atmospheric ice nuclei, Geophys. Res. Lett., 30, 1732,
https://doi.org/10.1029/2003GL017410, 2003. a, b
DeMott, P. J., Prenni, A. J., Liu, X., Kreidenweis, S. M., Petters, M. D.,
Twohy, C. H., Richardson, M., Eidhammer, T., and Rogers, D.: Predicting
global atmospheric ice nuclei distributions and their impacts on
climate, P. Natl. Acad. Sci. USA, 107, 11217–11222, https://doi.org/10.1073/pnas.0910818107, 2010. a, b
DeMott, P. J., Hill, T. C., McCluskey, C. S., Prather, K. A., Collins, D. B., Sullivan, R. C., Ruppel, M. J., Mason, R, H., Irish, V. E., Lee, T., Hwang, C. Y., Rhee, T. S., Snider, J. R., McMeeking, G. R., Dhaniyala, S., Lewis, E. R., Wentzell, J. J., Abbatt, J., Lee, C., Sultana, C., Ault, A. P., Axson, J. L., Diaz Martinez, M., Venero, I., Santos-Figueroa, G., Stokes, M. D., Deane, G. B., Mayol-Bracero, O. L., Grassian, V. H., Bertram, T. H., Bertram, A. K., Moffett, B. F., and Franc, G. D.:
Sea spray aerosol as a unique source of ice nucleating particles,
P. Natl. Acad. Sci. USA, 113, 5797–5803, https://doi.org/10.1073/pnas.1514034112, 2016. a, b, c, d, e
DeMott, P. J., Hill, T. C., McCluskey, C. S., Prather, K. A., Collins, D. B., Sullivan, R. C., Ruppel, M. J., Mason, R, H., Irish, V. E., Lee, T., Hwang, C. Y., Rhee, T. S., Snider, J. R., McMeeking, G. R., Dhaniyala, S., Lewis, E. R., Wentzell, J. J., Abbatt, J., Lee, C., Sultana, C., Ault, A. P., Axson, J. L., Diaz Martinez, M., Venero, I., Santos-Figueroa, G., Stokes, M. D., Deane, G. B., Mayol-Bracero, O. L., Grassian, V. H., Bertram, T. H., Bertram, A. K. Moffett, B. F., and Franc, G. D.: Comparative measurements of ambient atmospheric concentrations of ice nucleating particles using multiple immersion freezing methods and a continuous flow diffusion chamber, Atmos. Chem. Phys., 17, 11227–11245, https://doi.org/10.5194/acp-17-11227-2017, 2017. a
DiMego, G. J., Bosart, L. F., and Endersen, G. W.: An examination of the
frequency and mean conditions surrounding frontal incursions into the Gulf of
Mexico and Caribbean Sea, Mon. Weather Rev., 104, 709–718,
https://doi.org/10.1175/1520-0493(1976)104<0709:AEOTFA>2.0.CO;2, 1976. a
Espinosa, A., Miranda, J., and Pineda, J.: Uncertainty evaluation in correlated quantities: application to elemental analysis of atmospheric aerosols, Rev. Mex. Fis., E56, 134–140, 2010. a
Espinosa, A., Reyes-Herrera, J., Miranda, J., Mercado, F., Veytia, M., Cuautle, M., and Cruz, J.: Development of an X-ray fluorescence spectrometer for environmental science applications, Instrum. Sci. Technol., 40, 603–617,
https://doi.org/10.1080/10739149.2012.693560, 2012. a
García de Fuentes, A. and Morales, J.: Dinámica regional de
Yucatán 1980–2000, Invest. Geográficas, 157–172, available at: http://www.scielo.org.mx/scielo.php?script=sci_arttext&pid=S0188-46112000000200010&lng=es&nrm=iso (last access: 18 January 2020), 2000. a
Gong, X., Wex, H., Müller, T., Wiedensohler, A., Höhler, K., Kandler, K., Ma, N., Dietel, B., Schiebel, T., Möhler, O., and Stratmann, F.: Characterization of aerosol properties at Cyprus, focusing on cloud condensation nuclei and ice-nucleating particles, Atmos. Chem. Phys., 19, 10883–10900, https://doi.org/10.5194/acp-19-10883-2019, 2019. a
Gong, X., Wex, H., van Pinxteren, M., Triesch, N., Fomba, K. W., Lubitz, J., Stolle, C., Robinson, T.-B., Müller, T., Herrmann, H., and Stratmann, F.: Characterization of aerosol particles at Cabo Verde close to sea level and at the cloud level – Part 2: Ice-nucleating particles in air, cloud and seawater, Atmos. Chem. Phys., 20, 1451–1468, https://doi.org/10.5194/acp-20-1451-2020, 2020a. a, b, c, d
Gong, X., Wex, H., Voigtländer, J., Fomba, K. W., Weinhold, K., van Pinxteren, M., Henning, S., Müller, T., Herrmann, H., and Stratmann, F.: Characterization of aerosol particles at Cabo Verde close to sea level and at the cloud level – Part 1: Particle number size distribution, cloud condensation nuclei and their origins, Atmos. Chem. Phys., 20, 1431–1449, https://doi.org/10.5194/acp-20-1431-2020, 2020b. a
Griffin, D. W., Garrison, V. H., Herman, J. R., and Shinn, E. A.: African
desert dust in the Caribbean atmosphere: microbiology and public health,
Aerobiologia, 17, 203–213, https://doi.org/10.1023/A:1011868218901, 2001. a
Guyon, P., Frank, G. P., Welling, M., Chand, D., Artaxo, P., Rizzo, L., Nishioka, G., Kolle, O., Fritsch, H., Silva Dias, M. A. F., Gatti, L. V., Cordova, A. M., and Andreae, M. O.: Airborne measurements of trace gas and aerosol particle emissions from biomass burning in Amazonia, Atmos. Chem. Phys., 5, 2989–3002, https://doi.org/10.5194/acp-5-2989-2005, 2005. a
Harrison, A. D., Lever, K., Sanchez-Marroquin, A., Holden, M. A., Whale, T. F., Tarn, M. D., McQuaid, J. B., and Murray, B. J.: The ice-nucleating ability of quartz immersed in water and its atmospheric importance compared to K-feldspar, Atmos. Chem. Phys., 19, 11343–11361, https://doi.org/10.5194/acp-19-11343-2019, 2019. a
Herrera-Silveira, J. A., Cirerol, N. A., Ghinaglia, L. T., Comín, F. A.,
and Madden, C.: Coastal eutrophication in the yucatán
peninsula, Environ. Anal. Gulf Mex., 512–516, 2004a. a
Herrera-Silveira, J. A., Comin, F. A., Aranda-Cirerol, N., Troccoli, L., and
Capurro, L.: Coastal water quality assessment in the Yucatan Peninsula:
management implications, Ocean Coast. Manage., 47, 625–639,
https://doi.org/10.1016/j.ocecoaman.2004.12.005, 2004b. a
Iannone, R., Chernoff, D. I., Pringle, A., Martin, S. T., and Bertram, A. K.: The ice nucleation ability of one of the most abundant types of fungal spores found in the atmosphere, Atmos. Chem. Phys., 11, 1191–1201, https://doi.org/10.5194/acp-11-1191-2011, 2011. a, b, c, d
INEGI: Principales resultados por localidad, Instituto Nacional de Estadistica y Geografia, Censo Poblacion y Vivienda, available at:
http://www.beta.inegi.org.mx/app/geo2/ahl/ (last access: 18 January 2019), 2010. a
INEGI: Principales resultados de la Encuesta Intercensal 2015 Yucatan, Instituto Nacional de Estadistica y Geografia, available at:
http://www.internet.contenidos.inegi.org.mx/contenidos/Productos/prod_serv/contenidos/espanol/bvinegi/productos/nueva_estruc/702825078966.pdf (last access: 18 January 2019), 2015. a
INEGI: Anuario estadistico y geogrifico de Yucatan 2017, Instituto Nacional de Estadistica y Geografia, available at: http://www.inegi.org.mx (last access: 18 January 2019), 2017. a
INEGI: Informacion por Entididad Federativa, Instituto Nacional de Estadistica y Geografia, available at:
http://www.cuentame.inegi.org.mx/monografias/informacion/yuc/territorio/clima.aspx?tema=me&e=31 (last access: 1 November 2019), 2019. a
Irish, V. E., Elizondo, P., Chen, J., Chou, C., Charette, J., Lizotte, M., Ladino, L. A., Wilson, T. W., Gosselin, M., Murray, B. J., Polishchuk, E., Abbatt, J. P. D., Miller, L. A., and Bertram, A. K.: Ice-nucleating particles in Canadian Arctic sea-surface microlayer and bulk seawater, Atmos. Chem. Phys., 17, 10583–10595, https://doi.org/10.5194/acp-17-10583-2017, 2017. a
Irish, V. E., Hanna, S. J., Willis, M. D., China, S., Thomas, J. L., Wentzell, J. J. B., Cirisan, A., Si, M., Leaitch, W. R., Murphy, J. G., Abbatt, J. P. D., Laskin, A., Girard, E., and Bertram, A. K.: Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014, Atmos. Chem. Phys., 19, 1027–1039, https://doi.org/10.5194/acp-19-1027-2019, 2019. a, b, c
Jahn, L. G., Polen, M. J., Jahl, L. G., Brubaker, T. A., Somers, J., and
Sullivan, R. C.: Biomass combustion produces ice-active minerals in
biomass-burning aerosol and bottom ash, P. Natl. Acad. Sci. USA, 117,
21928–21937, https://doi.org/10.1073/pnas.1922128117, 2020. a
Jones, J., Darvell, L., Bridgeman, T., Pourkashanian, M., and Williams, A.: An investigation of the thermal and catalytic behaviour of potassium in biomass combustion, P. Combust. Inst., 31, 1955–1963,
https://doi.org/10.1016/j.proci.2006.07.093, 2007. a
Kaaden, N., Massling, A., Schladitz, A., Müller, T., Kandler, K., Schütz, L., Weinzierl, B., Petzold, A., Tesche, M., Leinert, S., Deutscher, C., Ebert, M., Weinbruch. S., and Wiedensohler. A.:
State of mixing, shape factor, number size distribution, and hygroscopic
growth of the Saharan anthropogenic and mineral dust aerosol at Tinfou,
Morocco, Tellus B, 61, 51–63, https://doi.org/10.1111/j.1600-0889.2008.00388.x, 2009. a
Kishcha, P., da Silva, A. M., Starobinets, B., Long, C. N., Kalashnikova, O., and Alpert, P.: Meridional distribution of aerosol optical thickness over the tropical Atlantic Ocean, Atmos. Chem. Phys. Discuss., 14, 23309–23339, https://doi.org/10.5194/acpd-14-23309-2014, 2014. a, b, c
Knopf, D., Alpert, P., Wang, B., and Aller, J.: Stimulation of ice nucleation
by marine diatoms, Nat. Geosci., 4, 88–90, https://doi.org/10.1038/NGEO1037, 2011. a, b
Kohn, M., Lohmann, U., Welti, A., and Kanji, Z. A.: Immersion mode ice
nucleation measurements with the new Portable Immersion Mode Cooling chAmber
(PIMCA), J. Geophys. Res., 121, 4713–4733, https://doi.org/10.1002/2016JD024761, 2016. a, b, c
Koop, T., Luo, B., Tsias, A., and Peter, T.: Water activity as the determinant for homogeneous ice nucleation in aqueous solutions, Nature, 406, 611–614, https://doi.org/10.1029/2000JD900413, 2000. a
Lacher, L., Adams, M., Barry, K., Bertozzi, B., Bras, Y., Boffo, C., Castarede, D., Cziczo, D. J., DeMott, P. J., Goodell, M., Höhler, K., Hill, T. C. J., Jentzsch, C., Ladino, L. A., Levin, E. J. T., Mertes, S., Möhler, O., Murray, B. J., Nadolny, J., Pfeuffer, T., Picard, D., Ramirez Romero, M. C., Ribeiro, M., Richter, S., Schrod, J., Sellegri, K., Stratmann, F., Thomson, E., Wex, H., Wolf, M., and Freney, E.: The Puy de Dôme Ice Nucleation Intercomparison (PICNIC): Comparison between online and offline freezing techniques in ambient air, in preparation, 2021. a, b
Ladino, L. A., Raga, G. B., Alvarez-Ospina, H., Andino-Enríquez, M. A., Rosas, I., Martínez, L., Salinas, E., Miranda, J., Ramírez-Díaz, Z., Figueroa, B., Chou, C., Bertram, A. K., Quintana, E. T., Maldonado, L. A., García-Reynoso, A., Si, M., and Irish, V. E.: Ice-nucleating particles in a coastal tropical site, Atmos. Chem. Phys., 19, 6147–6165, https://doi.org/10.5194/acp-19-6147-2019, 2019. a, b, c, d, e
Ladino, L. A., Juarez-Perez, J., Ramirez-Diaz, Z., Miller, L. A., Herrera, J., Raga, G. B., Simpson, K. G., Cruz, G., Pereira, D. L., and Córdoba, F.: The UNAM-Droplet Freezing Assay: An Evaluation of the Ice Nucleating Capacity of the Sea-Surface Microlayer and Surface Mixed Layer in Tropical and Subpolar Waters (edited by Dr. Michel Grutter), Atmósfera,
https://doi.org/10.20937/ATM.52938, in press, 2020. a
Lee, C., Sultana, C. M., Collins, D. B., Santander, M. V., Axson, J. L., Malfatti, F., Cornwell, G. C., Grandquist, J. R., Deane, G. B., Stokes, M. D., Azam, F., Grassian, V. H., and Prather, K. A.: Advancing model systems for fundamental laboratory studies of
sea spray aerosol using the microbial loop, J. Phys. Chem. A, 119,
8860–8870, https://doi.org/10.1021/acs.jpca.5b03488, 2015. a
Levin, E., McMeeking, G., DeMott, P., McCluskey, C., Carrico, C., Nakao, S., Jayarathne, T., Stone, E., Stockwell, C., Yokelson, R., and Kreidenweis, S.:
Ice-nucleating particle emissions from biomass combustion and the potential
importance of soot aerosol, J. Geophys. Res., 121, 5888–5903,
https://doi.org/10.1002/2016JD024879, 2016. a, b
Li, J., Pósfai, M., Hobbs, P. V., and Buseck, P. R.: Individual aerosol
particles from biomass burning in southern Africa: 2, Compositions and aging
of inorganic particles, J. Geophys. Res.-Atmos., 108, 8484,
https://doi.org/10.1029/2002JD002310, 2003. a
Linke, C., Möhler, O., Veres, A., Mohácsi, Á., Bozóki, Z., Szabó, G., and Schnaiter, M.: Optical properties and mineralogical composition of different Saharan mineral dust samples: a laboratory study, Atmos. Chem. Phys., 6, 3315–3323, https://doi.org/10.5194/acp-6-3315-2006, 2006. a
Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715–737, https://doi.org/10.5194/acp-5-715-2005, 2005. a
Lohmann, U., Lüönd, F., and Mahrt, F.: An introduction to clouds: From the microscale to climate, Cambridge University Press, Cambridge, UK, 2016. a
Lüönd, F., Stetzer, O., Welti, A., and Lohmann, U.: Experimental study on the ice nucleation ability of size-selected kaolinite particles in the immersion mode, J. Geophys. Res., 115, D14201, https://doi.org/10.1029/2009JD012959, 2010. a
Marcolli, C., Gedamke, S., Peter, T., and Zobrist, B.: Efficiency of immersion mode ice nucleation on surrogates of mineral dust, Atmos. Chem. Phys., 7, 5081–5091, https://doi.org/10.5194/acp-7-5081-2007, 2007. a
Mason, R. H., Chou, C., McCluskey, C. S., Levin, E. J. T., Schiller, C. L., Hill, T. C. J., Huffman, J. A., DeMott, P. J., and Bertram, A. K.: The micro-orifice uniform deposit impactor–droplet freezing technique (MOUDI-DFT) for measuring concentrations of ice nucleating particles as a function of size: improvements and initial validation, Atmos. Meas. Tech., 8, 2449–2462, https://doi.org/10.5194/amt-8-2449-2015, 2015a. a, b, c, d, e, f, g, h
Mason, R. H., Si, M., Li, J., Chou, C., Dickie, R., Toom-Sauntry, D., Pöhlker, C., Yakobi-Hancock, J. D., Ladino, L. A., Jones, K., Leaitch, W. R., Schiller, C. L., Abbatt, J. P. D., Huffman, J. A., and Bertram, A. K.: Ice nucleating particles at a coastal marine boundary layer site: correlations with aerosol type and meteorological conditions, Atmos. Chem. Phys., 15, 12547–12566, https://doi.org/10.5194/acp-15-12547-2015, 2015b. a, b
Mason, R. H., Si, M., Chou, C., Irish, V. E., Dickie, R., Elizondo, P., Wong, R., Brintnell, M., Elsasser, M., Lassar, W. M., Pierce, K. M., Leaitch, W. R., MacDonald, A. M., Platt, A., Toom-Sauntry, D., Sarda-Estève, R., Schiller, C. L., Suski, K. J., Hill, T. C. J., Abbatt, J. P. D., Huffman, J. A., DeMott, P. J., and Bertram, A. K.: Size-resolved measurements of ice-nucleating particles at six locations in North America and one in Europe, Atmos. Chem. Phys., 16, 1637–1651, https://doi.org/10.5194/acp-16-1637-2016, 2016. a, b, c, d
McCluskey, C. S., DeMott, P. J., Prenni, A. J., Levin, E. J., McMeeking, G. R., Sullivan, A. P., Hill, T. C., Nakao, S., Carrico, C. M., and Kreidenweis, S. M.: Characteristics of atmospheric ice nucleating particles associated with biomass burning in the US: Prescribed burns and wildfires, J. Geophys. Res., 119, 10458–10470, https://doi.org/10.1002/2014JD021980, 2014. a, b, c, d
McCluskey, C. S., Hill, T., Humphries, R., Rauker, A., Moreau, S., Strutton, P., Chambers, S., Williams, A., McRobert, I., Ward, J., Keywood, M. D., Harnwell, J., Ponsonby, W., Loh, Z. M., Krummel, P. B., Protat, A., Kreidenweis, S. M., and DeMott, P. J.: Observations of ice nucleating particles over Southern Ocean waters, Geophys. Res. Lett., 45, 11989–11997, https://doi.org/10.1029/2018GL079981, 2018. a, b
Mülmenstädt, J., Sourdeval, O., Delanoë, J., and Quaas, J.:
Frequency of occurrence of rain from liquid-, mixed-, and ice-phase clouds
derived from A-Train satellite retrievals, Geophys. Res. Lett., 42,
6502–6509, https://doi.org/10.1002/2015GL064604, 2015. a
Murray, B. J., Broadley, S. L., Wilson, T. W., Atkinson, J. D., and Wills, R. H.: Heterogeneous freezing of water droplets containing kaolinite particles, Atmos. Chem. Phys., 11, 4191–4207, https://doi.org/10.5194/acp-11-4191-2011, 2011. a
Murray, B. J., O'Sullivan, D., Atkinson, J., and Webb, M.: Ice nucleation by
particles immersed in supercooled cloud droplets, Chem. Soc. Rev., 41,
6519–6554, https://doi.org/10.1039/C2CS35200A, 2012. a, b
Nagare, B., Marcolli, C., Welti, A., Stetzer, O., and Lohmann, U.: Comparing contact and immersion freezing from continuous flow diffusion chambers, Atmos. Chem. Phys., 16, 8899–8914, https://doi.org/10.5194/acp-16-8899-2016, 2016. a, b, c
O'Dowd, C. D., Facchini, M. C., Cavalli, F., Ceburnis, D., Mircea, M.,
Decesari, S., Fuzzi, S., Yoon, Y. J., and Putaud, J.-P.: Biogenically driven
organic contribution to marine aerosol, Nature, 431, 676–680,
https://doi.org/10.1038/nature02959, 2004. a, b
Ovadnevaite, J., Ceburnis, D., Leinert, S., Dall'Osto, M., Canagaratna, M.,
O'Doherty, S., Berresheim, H., and O'Dowd, C. D.: Submicron NE Atlantic marine aerosol chemical composition and abundance: Seasonal trends and air mass categorization, J. Geophys. Res.-Atmos., 119, 11850–11863, https://doi.org/10.1002/2013JD021330, 2014. a
Parungo, F., Nagamoto, C., Rosinski, J., and Haagenson, P.: A study of marine
aerosols over the Pacific Ocean, J. Atmos. Chem., 4, 199–226,
https://doi.org/10.1007/BF00052001, 1986. a
Peppler, R. A., Bahrmann, C., Barnard, J. C., Campbell, J., Cheng, M.-D., Ferrare, R., Halthore, R., HeiIman, L., Hlavka, D., Laulainen, N. S., Lin, C.-J., Ogren., J. A., Poellot., M. R., Remer, L. A., Sassen, K., Spinhirne, J. D., Splitt, M. E., and Turner, D. D.:
ARM Southern Great Plains site observations of the smoke pall associated with
the 1998 Central American fires, B. Am. Meteorol. Soc., 81, 2563–2592,
https://doi.org/10.1175/1520-0477(2000)081<2563:ASGPSO>2.3.CO;2, 2000. a
Petters, M., Parsons, M., Prenni, A., DeMott, P., Kreidenweis, S., Carrico, C., Sullivan, A., McMeeking, G., Levin, E., Wold. C., Collett Jr., J. L., and Moosmüller, H.: Ice nuclei
emissions from biomass burning, J. Geophys. Res.-Atmos., 114, D07209,
https://doi.org/10.1029/2008JD011532, 2009. a
Pósfai, M., Simonics, R., Li, J., Hobbs, P. V., and Buseck, P. R.:
Individual aerosol particles from biomass burning in southern Africa: 1.
Compositions and size distributions of carbonaceous particles, J. Geophys.
Res., 108, 8483, https://doi.org/10.1029/2002jd002291, 2003. a
Prather, K. A., Bertram, T. H., Grassian, V. H., Deane, G. B., Stokes, M. D., DeMott, P. J., Aluwihare, L. I., Palenik, B. P., Azam, F., Seinfeld, J. H., Moffet, R. C., Molina, M. J., Cappa, C. D., Geiger, F. M., Roberts, G. C., Russell, L. M., Ault, A. P., Baltrusaitis, J., Collins, D.B., Corrigan, C. E., Cuadra-Rodriguez, L. A., Ebben, C. J., Forestieri, S. D., Guasco, T. L., Hersey, S.P., Kim, M. J., Lambert, W.F., Modini, R. L., Mui, W., Pedler, B. E., Ruppel, M. J., Ryder, O. S., Schoepp, N. G., Sullivan, R. C., and Zhao, D.: Bringing the ocean into the laboratory to probe the chemical
complexity of sea spray aerosol, P. Natl. Acad. Sci. USA, 110, 7550–7555,
https://doi.org/10.1073/pnas.1300262110, 2013. a, b, c
Prenni, A. J., Petters, M. D., Kreidenweis, S. M., Heald, C. L., Martin, S. T., Artaxo, P., Garland, R. M., Wollny, A. G., and Pöschl, U.: Relative roles of biogenic emissions and Saharan dust as ice nuclei in the Amazon basin, Nat. Geosci., 2, 402–405, https://doi.org/10.1038/ngeo517, 2009. a
Prenni, A. J., DeMott, P. J., Sullivan, A. P., Sullivan, R. C., Kreidenweis,
S. M., and Rogers, D. C.: Biomass burning as a potential source for
atmospheric ice nuclei: Western wildfires and prescribed burns, Geophys. Res.
Lett., 39, L11805, https://doi.org/10.1029/2012GL051915, 2012. a, b
Price, H., Baustian, K., McQuaid, J., Blyth, A., Bower, K., Choularton, T., Cotton, R., Cui, Z., Field, P., Gallagher, M., Hawker, R., Merrington, A., Miltenberger, A., Neely III, R. R., Parker, S. T., Rosenberg, P. D., Taylor, J. W., Trembath, J., Vergara-Temprado, J., Whale, T. F., Wilson, T. W., Young, G., and Murray, B. J.: Atmospheric
Ice-Nucleating Particles in the Dusty Tropical Atlantic, J. Geophys. Res.,
123, 2175–2193, https://doi.org/10.1002/2017JD027560, 2018. a, b, c
Prospero, J. M. and Lamb, P. J.: African droughts and dust transport to the
Caribbean: Climate change implications, Science, 302, 1024–1027,
https://doi.org/10.1126/science.1089915, 2003. a
Prospero, J. M. and Mayol-Bracero, O. L.: Understanding the transport and
impact of African dust on the Caribbean basin, B. Am. Meteorol. Soc., 94,
1329–1337, https://doi.org/10.1175/BAMS-D-12-00142.1, 2013. a
Pruppacher, H. and Klett, J.: Microphysics of Clouds and Precipitation,
D. Reidel Publishing Company, Dordrecht, the Netherlands, 954 pp., 1997. a
Querol, X., Tobías, A., Pérez, N., Karanasiou, A., Amato, F., Stafoggia, M., García-Pando, C. P., Ginoux, P., Forastiere, F., Gumy, S., Mudu, P., and Alastuey, A.: Monitoring the impact of desert dust outbreaks for air quality
for health studies, Environ. Int., 130, 104867,
https://doi.org/10.1016/j.envint.2019.05.061, 2019. a, b
Quinn, P. K., Collins, D. B., Grassian, V. H., Prather, K. A., and Bates,
T. S.: Chemistry and related properties of freshly emitted sea spray aerosol,
Chem. Rev., 115, 4383–4399, https://doi.org/10.1021/cr500713g, 2015. a
Raga, G. B., Ladino, L. A., Baumgardner, D., Ramirez-Romero, C., Cordoba, F., Alvarez-Ospina, H., Rosas, D., Amador, T., Miranda, J., Rosas, I., Jaramillo, A., Yakobi-Hancock, J., Kim, J., Martínez, L., Salinas, E., and Figueroa, B.: African Dust and Biomass Burning over Yucatan, B. Am. Meteorol. Soc., in review, 2021. a, b, c
Ramírez-Romero, C., Jaramillo, A., Córdoba, M. F., Raga, G. B., Miranda, J., Alvarez-Ospina, H., Rosas, D., Amador, T., Kim, J. S., Yakobi-Hancock, J., Baumgardner, D., and Ladino, L. A.: African dust particles over the western Caribbean – Part I: Impact on air quality over the Yucatán Peninsula, Atmos. Chem. Phys., 21, 239–253, https://doi.org/10.5194/acp-21-239-2021, 2021. a, b, c, d, e
Reicher, N., Budke, C., Eickhoff, L., Raveh-Rubin, S., Kaplan-Ashiri, I., Koop, T., and Rudich, Y.: Size-dependent ice nucleation by airborne particles during dust events in the eastern Mediterranean, Atmos. Chem. Phys., 19, 11143–11158, https://doi.org/10.5194/acp-19-11143-2019, 2019. a, b, c
Reid, J. S., Koppmann, R., Eck, T. F., and Eleuterio, D. P.: A review of biomass burning emissions part II: intensive physical properties of biomass burning particles, Atmos. Chem. Phys., 5, 799–825, https://doi.org/10.5194/acp-5-799-2005, 2005. a
Ríos, B. and Raga, G. B.: Spatio-temporal distribution of burned areas by ecoregions in Mexico and Central America, Int. J. Remote Sens., 39, 949–970, https://doi.org/10.1080/01431161.2017.1392641, 2018. a, b, c, d
Rodriguez-Gomez, C., Ramirez-Romero, C., Cordoba, F., Raga, G. B., Salinas, E., Martinez, L., Rosas, I., Quintana, E. T., Maldonado, L. A., Rosas, D.,
Amador, T., Alvarez, H., and Ladino, L. A.: Characterization of culturable
airborne microorganisms in the Yucatan Peninsula, Atmos. Environ., 223,
117183, https://doi.org/10.1016/j.atmosenv.2019.117183, 2020. a
Rosinski, J., Haagenson, P., Nagamoto, C., and Parungo, F.: Nature of
ice-forming nuclei in marine air masses, J. Aerosol Sci., 18, 291–309,
https://doi.org/10.1016/0021-8502(87)90024-3, 1987. a
Rosinski, J., Haagenson, P., Nagamoto, C., Quintana, B., Parungo, F., and Hoyt, S.: Ice-forming nuclei in air masses over the Gulf of Mexico, J. Aerosol Sci., 19, 539–551, https://doi.org/10.1016/0021-8502(88)90206-6, 1988. a, b
Saarikoski, S., Sillanpää, M., Sofiev, M., Timonen, H., Saarnio, K.,
Teinilä, K., Karppinen, A., Kukkonen, J., and Hillamo, R.: Chemical
composition of aerosols during a major biomass burning episode over northern
Europe in spring 2006: Experimental and modelling assessments, Atmos.
Environ., 41, 3577–3589, https://doi.org/10.1016/j.atmosenv.2006.12.053, 2007. a
Saide, P., Spak, S., Pierce, R., Otkin, J., Schaack, T., Heidinger, A.,
Da Silva, A., Kacenelenbogen, M., Redemann, J., and Carmichael, G.: Central
American biomass burning smoke can increase tornado severity in the US,
Geophys. Res. Lett., 42, 956–965, https://doi.org/10.1002/2014GL062826, 2015. a
Schnell, R. and Vali, G.: Freezing nuclei in marine waters, Tellus A, 27,
321–323, https://doi.org/10.1111/j.2153-3490.1975.tb01682.x, 1975. a
Si, M., Irish, V. E., Mason, R. H., Vergara-Temprado, J., Hanna, S. J., Ladino, L. A., Yakobi-Hancock, J. D., Schiller, C. L., Wentzell, J. J. B., Abbatt, J. P. D., Carslaw, K. S., Murray, B. J., and Bertram, A. K.: Ice-nucleating ability of aerosol particles and possible sources at three coastal marine sites, Atmos. Chem. Phys., 18, 15669–15685, https://doi.org/10.5194/acp-18-15669-2018, 2018. a, b, c, d
Taylor, D. A.: Dust in the wind, Environ. Health Persp., 110, 80–87,
https://doi.org/10.1289/ehp.110-a80, 2002. a
Trujano-Jiménez, F., Ríos, B., Jaramillo, A., Ladino, L. A., and Raga, G. B.: The impact of biomass burning emissions on protected natural areas in central and southern Mexico, Environ. Sci. Pollut. R.,
https://doi.org/10.1007/s11356-020-12095-y, in press, 2021. a, b
Umo, N. S., Murray, B. J., Baeza-Romero, M. T., Jones, J. M., Lea-Langton, A. R., Malkin, T. L., O'Sullivan, D., Neve, L., Plane, J. M. C., and Williams, A.: Ice nucleation by combustion ash particles at conditions relevant to mixed-phase clouds, Atmos. Chem. Phys., 15, 5195–5210, https://doi.org/10.5194/acp-15-5195-2015, 2015. a, b
Vali, G.: Quantitative evaluation of experimental results an the heterogeneous freezing nucleation of supercooled liquids, J. Atmos. Sci., 28, 402–409, https://doi.org/10.1175/1520-0469(1971)028<0402:QEOERA>2.0.CO;2, 1971. a
Welti, A., Lüönd, F., Kanji, Z. A., Stetzer, O., and Lohmann, U.: Time dependence of immersion freezing: an experimental study on size selected kaolinite particles, Atmos. Chem. Phys., 12, 9893–9907, https://doi.org/10.5194/acp-12-9893-2012, 2012. a, b, c
Welti, A., Müller, K., Fleming, Z. L., and Stratmann, F.: Concentration and variability of ice nuclei in the subtropical maritime boundary layer, Atmos. Chem. Phys., 18, 5307–5320, https://doi.org/10.5194/acp-18-5307-2018, 2018. a
Welti, A., Bigg, E. K., DeMott, P. J., Gong, X., Hartmann, M., Harvey, M., Henning, S., Herenz, P., Hill, T. C. J., Hornblow, B., Leck, C., Löffler, M., McCluskey, C. S., Rauker, A. M., Schmale, J., Tatzelt, C., van Pinxteren, M., and Stratmann, F.: Ship-based measurements of ice nuclei concentrations over the Arctic, Atlantic, Pacific and Southern oceans, Atmos. Chem. Phys., 20, 15191–15206, https://doi.org/10.5194/acp-20-15191-2020, 2020. a, b, c
Wex, H., Huang, L., Zhang, W., Hung, H., Traversi, R., Becagli, S., Sheesley, R. J., Moffett, C. E., Barrett, T. E., Bossi, R., Skov, H., Hünerbein, A., Lubitz, J., Löffler, M., Linke, O., Hartmann, M., Herenz, P., and Stratmann, F.: Annual variability of ice-nucleating particle concentrations at different Arctic locations, Atmos. Chem. Phys., 19, 5293–5311, https://doi.org/10.5194/acp-19-5293-2019, 2019. a
Wheeler, M., Mason, R., Steunenberg, K., Wagstaff, M., Chou, C., and Bertram,
A.: Immersion freezing of supermicron mineral dust particles: Freezing
results, testing different schemes for describing ice nucleation, and ice
nucleation active site densities, J. Phys. Chem. A, 119, 4358–4372,
https://doi.org/10.1021/jp507875q, 2015. a, b, c, d, e
Wilbourn, E. K., Thornton, D. C., Ott, C., Graff, J., Quinn, P. K., Bates,
T. S., Betha, R., Russell, L. M., Behrenfeld, M. J., and Brooks, S. D.: Ice
nucleation by marine aerosols over the North Atlantic Ocean in late spring,
J. Geophys. Res., 125, e2019JD030913, https://doi.org/10.1029/2019JD030913, 2020. a
Wilson, T. W., Ladino, L. A., Alpert, P. A., Breckels, M. N., Brooks, I. M., Browse, J., Burrows, S. M., Carslaw, K. S., Huffman, J. A., Judd, C., Kilthau, W. P., Mason, R.H., McFiggans, G., Miller, L. A., Nájera, J. J. Polishchuk, E., Rae, S., Schiller, C. L., Si, M., Vergara Temprado, J., Whale, T. F., Wong, J. P., Wurl, O., Yakobi-Hancock, J. D., Abbatt, J. P., Aller, J. Y., Bertram, A. K., Knopf, D. A., and Murray, B. J.: A marine biogenic source of atmospheric ice-nucleating particles, Nature, 525, 234–238, https://doi.org/10.1038/nature14986, 2015. a
Wu, P.-C., Tsai, J.-C., Li, F.-C., Lung, S.-C., and Su, H.-J.: Increased levels of ambient fungal spores in Taiwan are associated with dust events from China, Atmos. Environ., 38, 4879–4886, https://doi.org/10.1016/j.atmosenv.2004.05.039, 2004. a
Xia, L. and Gao, Y.: Chemical composition and size distributions of coastal
aerosols observed on the US East Coast, Mar. Chem., 119, 77–90,
https://doi.org/10.1016/j.marchem.2010.01.002, 2010. a
Yakobi-Hancock, J. D., Ladino, L. A., and Abbatt, J. P.: Review of Recent
Developments and Shortcomings in the Characterization of Potential
Atmospheric Ice Nuclei: Focus on the Tropics, Rev. Cienc., 17,
15–34, https://doi.org/10.25100/rc.v17i3.476, 2014. a
Yoch, D. C.: Dimethylsulfoniopropionate: its sources, role in the marine food
web, and biological degradation to dimethylsulfide, Appl. Environ.
Microb., 68, 5804–5815, https://doi.org/10.1128/AEM.68.12.5804, 2002. a
Yokelson, R. J., Crounse, J. D., DeCarlo, P. F., Karl, T., Urbanski, S., Atlas, E., Campos, T., Shinozuka, Y., Kapustin, V., Clarke, A. D., Weinheimer, A., Knapp, D. J., Montzka, D. D., Holloway, J., Weibring, P., Flocke, F., Zheng, W., Toohey, D., Wennberg, P. O., Wiedinmyer, C., Mauldin, L., Fried, A., Richter, D., Walega, J., Jimenez, J. L., Adachi, K., Buseck, P. R., Hall, S. R., and Shetter, R.: Emissions from biomass burning in the Yucatan, Atmos. Chem. Phys., 9, 5785–5812, https://doi.org/10.5194/acp-9-5785-2009, 2009.
a, b
Zhang, H., Hu, D., Chen, J., Ye, X., Wang, S. X., Hao, J. M., Wang, L., Zhang, R., and An, Z.: Particle size distribution and polycyclic aromatic
hydrocarbons emissions from agricultural crop residue burning,
Environ. Sci. Technol., 45, 5477–5482, https://doi.org/10.1021/es1037904, 2011. a
Zimmermann, F., Weinbruch, S., Schütz, L., Hofmann, H., Ebert, M., Kandler, K., and Worringen, A.: Ice nucleation properties of the most abundant mineral dust phases, J. Geophys. Res., 113, D23204, https://doi.org/10.1029/2008JD010655, 2008. a
Short summary
Most precipitation from deep clouds over the continents and in the intertropical convergence zone is strongly influenced by the presence of ice crystals whose formation requires the presence of aerosol particles. In the present study, the ability of three different aerosol types (i.e., marine aerosol, biomass burning, and African dust) to facilitate ice particle formation was assessed in the Yucatán Peninsula, Mexico.
Most precipitation from deep clouds over the continents and in the intertropical convergence...
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