Articles | Volume 20, issue 7
https://doi.org/10.5194/acp-20-4167-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-4167-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Supercooled liquid water cloud observed, analysed, and modelled at the top of the planetary boundary layer above Dome C, Antarctica
CNRM, Université de Toulouse, Météo-France, CNRS,
Toulouse, France
Massimo Del Guasta
INO-CNR, Sesto Fiorentino, Italy
Eric Bazile
CNRM, Université de Toulouse, Météo-France, CNRS,
Toulouse, France
Niramson Azouz
CNRM, Université de Toulouse, Météo-France, CNRS,
Toulouse, France
Angelo Lupi
ISAC-CNR, Bologna, Italy
Pierre Durand
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS,
Toulouse, France
Jean-Luc Attié
Laboratoire d'Aérologie, Université de Toulouse, CNRS, UPS,
Toulouse, France
Dana Veron
University of Delaware, Newark, USA
Vincent Guidard
CNRM, Université de Toulouse, Météo-France, CNRS,
Toulouse, France
Paolo Grigioni
ENEA, Roma, Italy
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Revised manuscript not accepted
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L. El Amraoui, J.-L. Attié, P. Ricaud, W. A. Lahoz, A. Piacentini, V.-H. Peuch, J. X. Warner, R. Abida, J. Barré, and R. Zbinden
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E. Hache, J.-L. Attié, C. Tourneur, P. Ricaud, L. Coret, W. A. Lahoz, L. El Amraoui, B. Josse, P. Hamer, J. Warner, X. Liu, K. Chance, M. Höpfner, R. Spurr, V. Natraj, S. Kulawik, A. Eldering, and J. Orphal
Atmos. Meas. Tech., 7, 2185–2201, https://doi.org/10.5194/amt-7-2185-2014, https://doi.org/10.5194/amt-7-2185-2014, 2014
F. Carminati, P. Ricaud, J.-P. Pommereau, E. Rivière, S. Khaykin, J.-L. Attié, and J. Warner
Atmos. Chem. Phys., 14, 6195–6211, https://doi.org/10.5194/acp-14-6195-2014, https://doi.org/10.5194/acp-14-6195-2014, 2014
R. M. Zbinden, V. Thouret, P. Ricaud, F. Carminati, J.-P. Cammas, and P. Nédélec
Atmos. Chem. Phys., 13, 12363–12388, https://doi.org/10.5194/acp-13-12363-2013, https://doi.org/10.5194/acp-13-12363-2013, 2013
J.-L. Baray, Y. Courcoux, P. Keckhut, T. Portafaix, P. Tulet, J.-P. Cammas, A. Hauchecorne, S. Godin Beekmann, M. De Mazière, C. Hermans, F. Desmet, K. Sellegri, A. Colomb, M. Ramonet, J. Sciare, C. Vuillemin, C. Hoareau, D. Dionisi, V. Duflot, H. Vérèmes, J. Porteneuve, F. Gabarrot, T. Gaudo, J.-M. Metzger, G. Payen, J. Leclair de Bellevue, C. Barthe, F. Posny, P. Ricaud, A. Abchiche, and R. Delmas
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P. Huszar, H. Teyssèdre, M. Michou, A. Voldoire, D. J. L. Olivié, D. Saint-Martin, D. Cariolle, S. Senesi, D. Salas Y Melia, A. Alias, F. Karcher, P. Ricaud, and T. Halenka
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EGUsphere, https://doi.org/10.5194/egusphere-2024-3744, https://doi.org/10.5194/egusphere-2024-3744, 2024
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The Copernicus Atmosphere Monitoring Service – Regional Production delivers daily forecasts, analyses, and reanalyses of air quality in Europe. The Service relies on a distributed modelling production by eleven leading European modelling teams following stringent requirements with an operational design which has no equivalent in the world. All the products are full, free, open and quality assured and disseminated with a high level of reliability.
Mickaël Bacles, Jonathan Améric, and Vincent Guidard
EGUsphere, https://doi.org/10.5194/egusphere-2024-2941, https://doi.org/10.5194/egusphere-2024-2941, 2024
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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Sulfur dioxide emitted during volcanic eruptions can be hazardous for aviation safety. A recent development aims at improving the forecasts of volcanic sulfur dioxide quantities made by the MOCAGE chemistry transport model. Both TROPOMI and IASI instruments are assimilated in the model. We focus on the eruption event of the La Soufrière Saint-Vincent volcano in April 2021. The combined assimilation of IASI and TROPOMI observations always leads to a better analyses and forecasts.
Francesca Vittorioso, Vincent Guidard, and Nadia Fourrié
Atmos. Meas. Tech., 17, 5279–5299, https://doi.org/10.5194/amt-17-5279-2024, https://doi.org/10.5194/amt-17-5279-2024, 2024
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The future Meteosat Third Generation Infrared Sounder (MTG-IRS) will represent a major innovation for the monitoring of the chemical state of the atmosphere. MTG-IRS will have the advantage of being based on a geostationary platform and acquiring data with a high temporal frequency. This work aims to evaluate its potential impact over Europe within a chemical transport model (MOCAGE). The results indicate that the assimilation of these data always has a positive impact on ozone analysis.
Philippe Ricaud, Pierre Durand, Paolo Grigioni, Massimo Del Guasta, Giuseppe Camporeale, Axel Roy, Jean-Luc Attié, and John Bognar
Atmos. Meas. Tech., 17, 5071–5089, https://doi.org/10.5194/amt-17-5071-2024, https://doi.org/10.5194/amt-17-5071-2024, 2024
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Jonathan J. Day, Gunilla Svensson, Barbara Casati, Taneil Uttal, Siri-Jodha Khalsa, Eric Bazile, Elena Akish, Niramson Azouz, Lara Ferrighi, Helmut Frank, Michael Gallagher, Øystein Godøy, Leslie M. Hartten, Laura X. Huang, Jareth Holt, Massimo Di Stefano, Irene Suomi, Zen Mariani, Sara Morris, Ewan O'Connor, Roberta Pirazzini, Teresa Remes, Rostislav Fadeev, Amy Solomon, Johanna Tjernström, and Mikhail Tolstykh
Geosci. Model Dev., 17, 5511–5543, https://doi.org/10.5194/gmd-17-5511-2024, https://doi.org/10.5194/gmd-17-5511-2024, 2024
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James Brean, David C. S. Beddows, Eija Asmi, Ari Virkkula, Lauriane L. J. Quéléver, Mikko Sipilä, Floortje Van Den Heuvel, Thomas Lachlan-Cope, Anna Jones, Markus Frey, Angelo Lupi, Jiyeon Park, Young Jun Yoon, Ralf Weller, Giselle L. Marincovich, Gabriela C. Mulena, Roy M. Harrison, and Manuel Dall´Osto
EGUsphere, https://doi.org/10.5194/egusphere-2024-987, https://doi.org/10.5194/egusphere-2024-987, 2024
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Geosci. Model Dev., 17, 3385–3408, https://doi.org/10.5194/gmd-17-3385-2024, https://doi.org/10.5194/gmd-17-3385-2024, 2024
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Atmos. Chem. Phys., 24, 613–630, https://doi.org/10.5194/acp-24-613-2024, https://doi.org/10.5194/acp-24-613-2024, 2024
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Florian Dupuy, Pierre Durand, and Thierry Hedde
Nonlin. Processes Geophys., 30, 553–570, https://doi.org/10.5194/npg-30-553-2023, https://doi.org/10.5194/npg-30-553-2023, 2023
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Forecasting near-surface winds over complex terrain requires high-resolution numerical weather prediction models, which drastically increase the duration of simulations and hinder them in running on a routine basis. A faster alternative is statistical downscaling. We explore different ways of calculating near-surface wind speed and direction using artificial intelligence algorithms based on various convolutional neural networks in order to find the best approach for wind downscaling.
Antoine Perrot, Olivier Pannekoucke, and Vincent Guidard
Nonlin. Processes Geophys., 30, 139–166, https://doi.org/10.5194/npg-30-139-2023, https://doi.org/10.5194/npg-30-139-2023, 2023
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This work is a theoretical contribution that provides equations for understanding uncertainty prediction applied in air quality where multiple chemical species can interact. A simplified minimal test bed is introduced that shows the ability of our equations to reproduce the statistics estimated from an ensemble of forecasts. While the latter estimation is the state of the art, solving equations is numerically less costly, depending on the number of chemical species, and motivates this research.
James Brean, David C. S. Beddows, Roy M. Harrison, Congbo Song, Peter Tunved, Johan Ström, Radovan Krejci, Eyal Freud, Andreas Massling, Henrik Skov, Eija Asmi, Angelo Lupi, and Manuel Dall'Osto
Atmos. Chem. Phys., 23, 2183–2198, https://doi.org/10.5194/acp-23-2183-2023, https://doi.org/10.5194/acp-23-2183-2023, 2023
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Our results emphasize how understanding the geographical variation in surface types across the Arctic is key to understanding secondary aerosol sources. We provide a harmonised analysis of new particle formation across the Arctic.
Yetang Wang, Xueying Zhang, Wentao Ning, Matthew A. Lazzara, Minghu Ding, Carleen H. Reijmer, Paul C. J. P. Smeets, Paolo Grigioni, Petra Heil, Elizabeth R. Thomas, David Mikolajczyk, Lee J. Welhouse, Linda M. Keller, Zhaosheng Zhai, Yuqi Sun, and Shugui Hou
Earth Syst. Sci. Data, 15, 411–429, https://doi.org/10.5194/essd-15-411-2023, https://doi.org/10.5194/essd-15-411-2023, 2023
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Here we construct a new database of Antarctic automatic weather station (AWS) meteorological records, which is quality-controlled by restrictive criteria. This dataset compiled all available Antarctic AWS observations, and its resolutions are 3-hourly, daily and monthly, which is very useful for quantifying spatiotemporal variability in weather conditions. Furthermore, this compilation will be used to estimate the performance of the regional climate models or meteorological reanalysis products.
Silvia Becagli, Elena Barbaro, Simone Bonamano, Laura Caiazzo, Alcide di Sarra, Matteo Feltracco, Paolo Grigioni, Jost Heintzenberg, Luigi Lazzara, Michel Legrand, Alice Madonia, Marco Marcelli, Chiara Melillo, Daniela Meloni, Caterina Nuccio, Giandomenico Pace, Ki-Tae Park, Suzanne Preunkert, Mirko Severi, Marco Vecchiato, Roberta Zangrando, and Rita Traversi
Atmos. Chem. Phys., 22, 9245–9263, https://doi.org/10.5194/acp-22-9245-2022, https://doi.org/10.5194/acp-22-9245-2022, 2022
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Measurements of phytoplanktonic dimethylsulfide and its oxidation products in the Antarctic atmosphere allow us to understand the role of the oceanic (sea ice melting, Chl α and dimethylsulfoniopropionate) and atmospheric (wind direction and speed, humidity, solar radiation and transport processes) factors in the biogenic aerosol formation, concentration and characteristic ratio between components in an Antarctic coastal site facing the polynya of the Ross Sea.
Patrick Le Moigne, Eric Bazile, Anning Cheng, Emanuel Dutra, John M. Edwards, William Maurel, Irina Sandu, Olivier Traullé, Etienne Vignon, Ayrton Zadra, and Weizhong Zheng
The Cryosphere, 16, 2183–2202, https://doi.org/10.5194/tc-16-2183-2022, https://doi.org/10.5194/tc-16-2183-2022, 2022
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This paper describes an intercomparison of snow models, of varying complexity, used for numerical weather prediction or academic research. The results show that the simplest models are, under certain conditions, able to reproduce the surface temperature just as well as the most complex models. Moreover, the diversity of surface parameters of the models has a strong impact on the temporal variability of the components of the simulated surface energy balance.
Christophe Genthon, Dana E. Veron, Etienne Vignon, Jean-Baptiste Madeleine, and Luc Piard
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The surface atmosphere of the high Antarctic Plateau is very cold and clean. Such conditions favor water vapor supersaturation. A 3-year quasi-continuous series of atmospheric moisture in a ~40 m atmospheric layer at Dome C is reported that documents time variability, vertical profiles and occurrences of supersaturation. Supersaturation with respect to ice is frequently observed throughout the column, with relative humidities occasionally reaching values near liquid water saturation.
Christophe Genthon, Dana Veron, Etienne Vignon, Delphine Six, Jean-Louis Dufresne, Jean-Baptiste Madeleine, Emmanuelle Sultan, and François Forget
Earth Syst. Sci. Data, 13, 5731–5746, https://doi.org/10.5194/essd-13-5731-2021, https://doi.org/10.5194/essd-13-5731-2021, 2021
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A 10-year dataset of observation in the atmospheric boundary layer at Dome C on the high Antarctic plateau is presented. This is obtained with sensors at six levels along a tower higher than 40 m. The temperature inversion can reach more than 25 °C along the tower in winter, while full mixing by convection can occur in summer. Different amplitudes of variability for wind and temperature at the different levels reflect different signatures of solar vs. synoptic forcing of the boundary layer.
Congbo Song, Manuel Dall'Osto, Angelo Lupi, Mauro Mazzola, Rita Traversi, Silvia Becagli, Stefania Gilardoni, Stergios Vratolis, Karl Espen Yttri, David C. S. Beddows, Julia Schmale, James Brean, Agung Ghani Kramawijaya, Roy M. Harrison, and Zongbo Shi
Atmos. Chem. Phys., 21, 11317–11335, https://doi.org/10.5194/acp-21-11317-2021, https://doi.org/10.5194/acp-21-11317-2021, 2021
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We present a cluster analysis of relatively long-term (2015–2019) aerosol aerodynamic volume size distributions up to 20 μm in the Arctic for the first time. The study found that anthropogenic and natural aerosols comprised 27 % and 73 % of the occurrence of the coarse-mode aerosols, respectively. Our study shows that about two-thirds of the coarse-mode aerosols are related to two sea-spray-related aerosol clusters, indicating that sea spray aerosol may more complex in the Arctic environment.
Mohammad El Aabaribaoune, Emanuele Emili, and Vincent Guidard
Atmos. Meas. Tech., 14, 2841–2856, https://doi.org/10.5194/amt-14-2841-2021, https://doi.org/10.5194/amt-14-2841-2021, 2021
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This work aims to use correlated IASI errors in the ozone band within a chemical transport model assimilation. The validation of the results against ozone observations from ozonesondes, MLS, and OMI instruments has shown an improvement of the ozone distribution. The computational time was also highly reduced. The surface sea temperature was also improved. The work aims to improve the quality of the ozone prediction, which is important for air quality, climate, and meteorological applications.
Iris-Amata Dion, Cyrille Dallet, Philippe Ricaud, Fabien Carminati, Thibaut Dauhut, and Peter Haynes
Atmos. Chem. Phys., 21, 2191–2210, https://doi.org/10.5194/acp-21-2191-2021, https://doi.org/10.5194/acp-21-2191-2021, 2021
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Ice in the tropopause has a strong radiative effect on climate. The amount of ice injected (∆IWC) up to the tropical tropopause layer has been shown to be the highest over the Maritime Continent (MC), a region that includes Indonesia. ∆IWC is studied over islands and sea of the MC. Space-borne observations of ice, precipitation and lightning are used to estimate ∆IWC and are compared to ∆IWC estimated from the ERA5 reanalyses. It is shown that Java is the area of the greatest ∆IWC over the MC.
Lilian Joly, Olivier Coopmann, Vincent Guidard, Thomas Decarpenterie, Nicolas Dumelié, Julien Cousin, Jérémie Burgalat, Nicolas Chauvin, Grégory Albora, Rabih Maamary, Zineb Miftah El Khair, Diane Tzanos, Joël Barrié, Éric Moulin, Patrick Aressy, and Anne Belleudy
Atmos. Meas. Tech., 13, 3099–3118, https://doi.org/10.5194/amt-13-3099-2020, https://doi.org/10.5194/amt-13-3099-2020, 2020
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This article presents an instrument weighing less than 3 kg for accurate and rapid measurement of greenhouse gases between 0 and 30 km altitude using a meteorological balloon. This article shows the interest of these measurements for the validation of simulations of infrared satellite observations.
Olivier Coopmann, Vincent Guidard, Nadia Fourrié, Béatrice Josse, and Virginie Marécal
Atmos. Meas. Tech., 13, 2659–2680, https://doi.org/10.5194/amt-13-2659-2020, https://doi.org/10.5194/amt-13-2659-2020, 2020
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The objective of this paper is to make a new selection of IASI channels by taking into account inter-channel observation-error correlations. Our selection further reduces the analysis error by 3 % in temperature, 1.8 % in humidity and 0.9 % in ozone compared to Collard’s selection, when using the same number of channels. A selection of 400 IASI channels is proposed at the end of the paper which is able to further reduce analysis errors.
Thomas Lachlan-Cope, David C. S. Beddows, Neil Brough, Anna E. Jones, Roy M. Harrison, Angelo Lupi, Young Jun Yoon, Aki Virkkula, and Manuel Dall'Osto
Atmos. Chem. Phys., 20, 4461–4476, https://doi.org/10.5194/acp-20-4461-2020, https://doi.org/10.5194/acp-20-4461-2020, 2020
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We present a statistical cluster analysis of the physical characteristics of particle size distributions collected at Halley (Antarctica) for the year 2015. Complex interactions between multiple ecosystems, coupled with different atmospheric circulation, result in very different aerosol size distributions populating the Southern Hemisphere.
Samuel Quesada-Ruiz, Jean-Luc Attié, William A. Lahoz, Rachid Abida, Philippe Ricaud, Laaziz El Amraoui, Régina Zbinden, Andrea Piacentini, Mathieu Joly, Henk Eskes, Arjo Segers, Lyana Curier, Johan de Haan, Jukka Kujanpää, Albert Christiaan Plechelmus Oude Nijhuis, Johanna Tamminen, Renske Timmermans, and Pepijn Veefkind
Atmos. Meas. Tech., 13, 131–152, https://doi.org/10.5194/amt-13-131-2020, https://doi.org/10.5194/amt-13-131-2020, 2020
Renske Timmermans, Arjo Segers, Lyana Curier, Rachid Abida, Jean-Luc Attié, Laaziz El Amraoui, Henk Eskes, Johan de Haan, Jukka Kujanpää, William Lahoz, Albert Oude Nijhuis, Samuel Quesada-Ruiz, Philippe Ricaud, Pepijn Veefkind, and Martijn Schaap
Atmos. Chem. Phys., 19, 12811–12833, https://doi.org/10.5194/acp-19-12811-2019, https://doi.org/10.5194/acp-19-12811-2019, 2019
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We present an evaluation of the added value of the Sentinel-4 and Sentinel-5P missions for air quality analyses of NO2. For this, synthetic observations for both missions are generated and combined with a chemistry transport model. While hourly Sentinel-4 NO2 observations over Europe benefit modelled NO2 analyses throughout the entire day, daily Sentinel-5P NO2 observations with global coverage show an impact up to 3–6 h after overpass. This supports the need for a combination of missions.
Manuel Dall'Osto, David C. S. Beddows, Peter Tunved, Roy M. Harrison, Angelo Lupi, Vito Vitale, Silvia Becagli, Rita Traversi, Ki-Tae Park, Young Jun Yoon, Andreas Massling, Henrik Skov, Robert Lange, Johan Strom, and Radovan Krejci
Atmos. Chem. Phys., 19, 7377–7395, https://doi.org/10.5194/acp-19-7377-2019, https://doi.org/10.5194/acp-19-7377-2019, 2019
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We present a cluster analysis of particle size distributions simultaneously collected from three European high Arctic sites centred in the Fram Strait during a 3-year period. Confined for longer time periods by consolidated pack sea ice regions, the Greenland site shows lower ultrafine-mode aerosol concentrations during summer relative to the Svalbard sites. Our study supports international environmental cooperation concerning the Arctic region.
Imane Farouk, Nadia Fourrié, and Vincent Guidard
Atmos. Meas. Tech., 12, 3001–3017, https://doi.org/10.5194/amt-12-3001-2019, https://doi.org/10.5194/amt-12-3001-2019, 2019
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A selection for homogeneous scenes for the assimilation of IASI radiances is proposed by using information on the collocated imager pixels inside each infrared observation. A revised method for the selection, which represents a compromise between two methods to select homogeneous scenes using homogeneity criteria already proposed in the literature, has a positive impact on the observation minus the simulation statistics. It has been tested in a numerical weather prediction model for clear sky.
Iris-Amata Dion, Philippe Ricaud, Peter Haynes, Fabien Carminati, and Thibaut Dauhut
Atmos. Chem. Phys., 19, 6459–6479, https://doi.org/10.5194/acp-19-6459-2019, https://doi.org/10.5194/acp-19-6459-2019, 2019
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Water vapour and ice cirrus clouds near the tropical tropopause layer (TTL) have a strong radiative impact on climate. Based on space-borne observations, we have developed a model linking ice in the upper troposphere from the Microwave Limb Sounder (MLS) to precipitation in the troposphere from the Tropical Rainfall Measurement Mission (TRMM). Our study quantifies the amount of ice injected into the TTL by deep convection over tropical lands and oceans by investigating the diurnal cycle of ice.
Federica Pacifico, Claire Delon, Corinne Jambert, Pierre Durand, Eleanor Morris, Mat J. Evans, Fabienne Lohou, Solène Derrien, Venance H. E. Donnou, Arnaud V. Houeto, Irene Reinares Martínez, and Pierre-Etienne Brilouet
Atmos. Chem. Phys., 19, 2299–2325, https://doi.org/10.5194/acp-19-2299-2019, https://doi.org/10.5194/acp-19-2299-2019, 2019
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Biogenic fluxes from soil at a local and regional scale are crucial to study air pollution and climate. Here we present field measurements of soil fluxes of nitric oxide (NO) and ammonia (NH3) observed over four different land cover types, i.e. bare soil, grassland, maize field, and forest, at an inland rural site in Benin, West Africa, during the DACCIWA field campaign in
June and July 2016.
Amelie Driemel, John Augustine, Klaus Behrens, Sergio Colle, Christopher Cox, Emilio Cuevas-Agulló, Fred M. Denn, Thierry Duprat, Masato Fukuda, Hannes Grobe, Martial Haeffelin, Gary Hodges, Nicole Hyett, Osamu Ijima, Ain Kallis, Wouter Knap, Vasilii Kustov, Charles N. Long, David Longenecker, Angelo Lupi, Marion Maturilli, Mohamed Mimouni, Lucky Ntsangwane, Hiroyuki Ogihara, Xabier Olano, Marc Olefs, Masao Omori, Lance Passamani, Enio Bueno Pereira, Holger Schmithüsen, Stefanie Schumacher, Rainer Sieger, Jonathan Tamlyn, Roland Vogt, Laurent Vuilleumier, Xiangao Xia, Atsumu Ohmura, and Gert König-Langlo
Earth Syst. Sci. Data, 10, 1491–1501, https://doi.org/10.5194/essd-10-1491-2018, https://doi.org/10.5194/essd-10-1491-2018, 2018
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The Baseline Surface Radiation Network (BSRN) collects and centrally archives high-quality ground-based radiation measurements in 1 min resolution. More than 10 300 months, i.e., > 850 years, of high-radiation data in 1 min resolution from the years 1992 to 2017 are available. The network currently comprises 59 stations collectively representing all seven continents as well as island-based stations in the Pacific, Atlantic, Indian and Arctic oceans.
Nizar Jaidan, Laaziz El Amraoui, Jean-Luc Attié, Philippe Ricaud, and François Dulac
Atmos. Chem. Phys., 18, 9351–9373, https://doi.org/10.5194/acp-18-9351-2018, https://doi.org/10.5194/acp-18-9351-2018, 2018
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The Mediterranean Basin, surrounded by three continents with diverse pollution sources, is particularly sensitive to climate change due to its location and diversity of ecosystems. In this work, we investigate the future change of surface ozone from 2000 to 2100 over this region using a set of atmospheric model outputs and ground-based observations. We also highlight how the future climate change and the increase of methane concentrations can offset the benefit of the pollution reduction policy.
Evelyn Freney, Karine Sellegri, Mounir Chrit, Kouji Adachi, Joel Brito, Antoine Waked, Agnès Borbon, Aurélie Colomb, Régis Dupuy, Jean-Marc Pichon, Laetitia Bouvier, Claire Delon, Corinne Jambert, Pierre Durand, Thierry Bourianne, Cécile Gaimoz, Sylvain Triquet, Anaïs Féron, Matthias Beekmann, François Dulac, and Karine Sartelet
Atmos. Chem. Phys., 18, 7041–7056, https://doi.org/10.5194/acp-18-7041-2018, https://doi.org/10.5194/acp-18-7041-2018, 2018
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The focus of these experiments, within the ChArMEx project, were to better understand the chemical properties of ambient aerosols over the Mediterranean region. A series of airborne measurements were performed aboard the French research aircraft, the ATR42, during the summer period. Aerosol and gas-phase chemical mass spectrometry allowed us to understand the sources and formation of organic aerosols. Numerical models were incorporated into this study to help interpret our observations.
Vanessa Brocchi, Gisèle Krysztofiak, Valéry Catoire, Jonathan Guth, Virginie Marécal, Régina Zbinden, Laaziz El Amraoui, François Dulac, and Philippe Ricaud
Atmos. Chem. Phys., 18, 6887–6906, https://doi.org/10.5194/acp-18-6887-2018, https://doi.org/10.5194/acp-18-6887-2018, 2018
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The Mediterranean Basin still suffers from a limited amount of in situ measurements for a good characterization of its environmental state. This study shows that intercontinental transport of very high CO concentrations can affect the upper Mediterranean Basin troposphere. By using modeling, 5- to 12-day eastward transport of biomass burning starting from North America and Siberia impacts the mid-troposphere of the Mediterranean Basin.
Yannick Kangah, Philippe Ricaud, Jean-Luc Attié, Naoko Saitoh, Jérôme Vidot, Pascal Brunel, and Samuel Quesada-Ruiz
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2018-21, https://doi.org/10.5194/amt-2018-21, 2018
Revised manuscript not accepted
Jean-Baptiste Renard, François Dulac, Pierre Durand, Quentin Bourgeois, Cyrielle Denjean, Damien Vignelles, Benoit Couté, Matthieu Jeannot, Nicolas Verdier, and Marc Mallet
Atmos. Chem. Phys., 18, 3677–3699, https://doi.org/10.5194/acp-18-3677-2018, https://doi.org/10.5194/acp-18-3677-2018, 2018
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A campaign was performed in the summer of 2013 above the Mediterranean basin, including in situ counting balloon-borne aerosol measurements (LOAC), for the detection of mineral dust. Three modes in the dust particle volume size distributions were detected, at roughly 0.2, 4, and 30 mm. Particles larger than 40 mm were often observed. They were lifted several days before and their persistence after transport over long distances is in conflict with dust sedimentation calculations.
Javier Andrey-Andrés, Nadia Fourrié, Vincent Guidard, Raymond Armante, Pascal Brunel, Cyril Crevoisier, and Bernard Tournier
Atmos. Meas. Tech., 11, 803–818, https://doi.org/10.5194/amt-11-803-2018, https://doi.org/10.5194/amt-11-803-2018, 2018
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A new generation of the Infrared Atmospheric Sounding Interferometer (IASI) sounders, whose highly accurate measurements are commonly used in environment applications, has already been designed: IASI New Generation (IASI-NG). A database of IASI and IASI-NG simulated observations was built to set a common framework for future impact studies. This first study showed the IASI-NG benefit with an improvement of the temperature retrievals throughout the atmosphere and a lower benefit for the humidity.
Piet Termonia, Claude Fischer, Eric Bazile, François Bouyssel, Radmila Brožková, Pierre Bénard, Bogdan Bochenek, Daan Degrauwe, Mariá Derková, Ryad El Khatib, Rafiq Hamdi, Ján Mašek, Patricia Pottier, Neva Pristov, Yann Seity, Petra Smolíková, Oldřich Španiel, Martina Tudor, Yong Wang, Christoph Wittmann, and Alain Joly
Geosci. Model Dev., 11, 257–281, https://doi.org/10.5194/gmd-11-257-2018, https://doi.org/10.5194/gmd-11-257-2018, 2018
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This paper describes the ALADIN System that has been developed by the international ALADIN consortium of 16 European and northern African partners since its creation in 1990. The paper also describes how its model configurations are used by the consortium partners for their operational weather forecasting applications and for weather and climate research.
Xuemeng Chen, Aki Virkkula, Veli-Matti Kerminen, Hanna E. Manninen, Maurizio Busetto, Christian Lanconelli, Angelo Lupi, Vito Vitale, Massimo Del Guasta, Paolo Grigioni, Riikka Väänänen, Ella-Maria Duplissy, Tuukka Petäjä, and Markku Kulmala
Atmos. Chem. Phys., 17, 13783–13800, https://doi.org/10.5194/acp-17-13783-2017, https://doi.org/10.5194/acp-17-13783-2017, 2017
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An air ion spectrometer was deployed for characterizing air ions for the first time at the Concordia station at Dome C on the Antarctic Plateau. We observed different ion processes: new particle formation (NPF), wind-induced ion production, and ion formation related to cloud and/or fog formation. Insights into these phenomena are presented. Additionally, the analysis on the growth of NPF events showed a size dependency of growth rates (GRs), i.e. GRs increase with particle sizes.
Uri Dayan, Philippe Ricaud, Régina Zbinden, and François Dulac
Atmos. Chem. Phys., 17, 13233–13263, https://doi.org/10.5194/acp-17-13233-2017, https://doi.org/10.5194/acp-17-13233-2017, 2017
Elisabeth Schlosser, Anna Dittmann, Barbara Stenni, Jordan G. Powers, Kevin W. Manning, Valérie Masson-Delmotte, Mauro Valt, Anselmo Cagnati, Paolo Grigioni, and Claudio Scarchilli
The Cryosphere, 11, 2345–2361, https://doi.org/10.5194/tc-11-2345-2017, https://doi.org/10.5194/tc-11-2345-2017, 2017
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To derive paleotemperatures from ice cores we must know all processes involved in ice formation. At the Antarctic base Dome C, a unique precipitation data set plus stable water isotope data enabled us to study atmospheric processes influencing isotope ratios of precipitation in detail. Meteorological data from both automatic weather station and an atmospheric model were used to investigate how different atmospheric flow patterns determine the precipitation parameters used in paleoclimatology.
Jacopo Grazioli, Christophe Genthon, Brice Boudevillain, Claudio Duran-Alarcon, Massimo Del Guasta, Jean-Baptiste Madeleine, and Alexis Berne
The Cryosphere, 11, 1797–1811, https://doi.org/10.5194/tc-11-1797-2017, https://doi.org/10.5194/tc-11-1797-2017, 2017
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We present medium and long-term measurements of precipitation in a coastal region of Antarctica. These measurements are among the first of their kind on the Antarctic continent and combine remote sensing with in situ observations. The benefits of this synergy are demonstrated and the lessons learned from this measurements, which are still ongoing, are very important for the creation of similar observatories elsewhere on the continent.
Philippe Ricaud, Eric Bazile, Massimo del Guasta, Christian Lanconelli, Paolo Grigioni, and Achraf Mahjoub
Atmos. Chem. Phys., 17, 5221–5237, https://doi.org/10.5194/acp-17-5221-2017, https://doi.org/10.5194/acp-17-5221-2017, 2017
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The novelty of the paper is to combine a large set of measurements and meteorological models to study the genesis of thick cloud and diamond dust/ice fog (ice crystals) episodes above Dome C, Antarctica. The originality of the work is to attribute the presence of thick cloud and diamond dust/ice fog to advection and microphysical processes with oceanic and continental origin of air masses, respectively. Thick cloud episodes are reproduced by the models but not diamond dust/ice fog episode.
Gianluca Di Natale, Luca Palchetti, Giovanni Bianchini, and Massimo Del Guasta
Atmos. Meas. Tech., 10, 825–837, https://doi.org/10.5194/amt-10-825-2017, https://doi.org/10.5194/amt-10-825-2017, 2017
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We evaluate the simultaneous remote sensing of atmospheric vertical profiles of water vapour and temperature along with some micro-physical parameters, such as ice-particle effective diameter and ice water content of cirrus clouds, using far infrared spectral measurements of the downwelling longwave radiation. The developed methodology allows to retrieve the atmospheric state with good accuracy and high repetition rate, about 12 min, opening the capability to identify fast atmospheric events.
Rachid Abida, Jean-Luc Attié, Laaziz El Amraoui, Philippe Ricaud, William Lahoz, Henk Eskes, Arjo Segers, Lyana Curier, Johan de Haan, Jukka Kujanpää, Albert Oude Nijhuis, Johanna Tamminen, Renske Timmermans, and Pepijn Veefkind
Atmos. Chem. Phys., 17, 1081–1103, https://doi.org/10.5194/acp-17-1081-2017, https://doi.org/10.5194/acp-17-1081-2017, 2017
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A detailed Observing System Simulation Experiment is performed to quantify the impact of future satellite instrument S-5P carbon monoxide (CO) on tropospheric analyses and forecasts. We focus on Europe for the period of northern summer 2003, when there was a severe heat wave episode. S-5P is able to capture the CO from forest fires that occurred in Portugal. Furthermore, our results provide evidence of S-5P CO benefits for monitoring processes contributing to atmospheric pollution.
François Gheusi, Pierre Durand, Nicolas Verdier, François Dulac, Jean-Luc Attié, Philippe Commun, Brice Barret, Claude Basdevant, Antoine Clenet, Solène Derrien, Alexis Doerenbecher, Laaziz El Amraoui, Alain Fontaine, Emeric Hache, Corinne Jambert, Elodie Jaumouillé, Yves Meyerfeld, Laurent Roblou, and Flore Tocquer
Atmos. Meas. Tech., 9, 5811–5832, https://doi.org/10.5194/amt-9-5811-2016, https://doi.org/10.5194/amt-9-5811-2016, 2016
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Boundary-layer pressurised balloons allow for horizontal multi-day flights in the lower atmosphere, carrying light scientific payloads. Ozonesondes, usually used for balloon soundings have too short a lifetime for such flights. An adaptation is proposed, whereby conventional sondes are operated with short measurement phases alternating with longer periods of dormancy. The sondes were operated over the western Mediterranean, offering an original perspective on tropospheric ozone.
Barbara Stenni, Claudio Scarchilli, Valerie Masson-Delmotte, Elisabeth Schlosser, Virginia Ciardini, Giuliano Dreossi, Paolo Grigioni, Mattia Bonazza, Anselmo Cagnati, Daniele Karlicek, Camille Risi, Roberto Udisti, and Mauro Valt
The Cryosphere, 10, 2415–2428, https://doi.org/10.5194/tc-10-2415-2016, https://doi.org/10.5194/tc-10-2415-2016, 2016
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Here, we focus on the Concordia Station, central East Antarctic plateau, providing a multi-year record (2008–2010) of daily precipitation types identified from crystal morphologies, precipitation amounts and isotopic composition. Relationships between local meteorological data and precipitation oxygen isotope composition are investigated. Our dataset is available for in-depth model evaluation at the synoptic scale.
Luca Ferrero, David Cappelletti, Maurizio Busetto, Mauro Mazzola, Angelo Lupi, Christian Lanconelli, Silvia Becagli, Rita Traversi, Laura Caiazzo, Fabio Giardi, Beatrice Moroni, Stefano Crocchianti, Martin Fierz, Griša Močnik, Giorgia Sangiorgi, Maria G. Perrone, Marion Maturilli, Vito Vitale, Roberto Udisti, and Ezio Bolzacchini
Atmos. Chem. Phys., 16, 12601–12629, https://doi.org/10.5194/acp-16-12601-2016, https://doi.org/10.5194/acp-16-12601-2016, 2016
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This study reports results from systematic vertical aerosol profiles measured in the Arctic using a tethered balloon platform. The collected data allowed for finding common rules of aerosol behavior along height and seasons. Transport events, secondary aerosol formation and ship impact are examples of the issues investigated along height. The importance of these issues is related to their climatic implications in reference to the aerosol direct and indirect effects in the Arctic atmosphere.
Swagata Payra, Philippe Ricaud, Rachid Abida, Laaziz El Amraoui, Jean-Luc Attié, Emmanuel Rivière, Fabien Carminati, and Thomas von Clarmann
Atmos. Meas. Tech., 9, 4355–4373, https://doi.org/10.5194/amt-9-4355-2016, https://doi.org/10.5194/amt-9-4355-2016, 2016
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The study deals with the budget of water vapour (H2O) at the tropical tropopause. The MOCAGE-VALENTINA assimilation tool has been used to assimilate Microwave Limb Sounder H2O space-borne measurements within the 316–5 hPa range from August 2011 to March 2013. Diagnostics are developed to assess the quality of the analyses depending on several parameters. Sensitivity studies show the improvement on the analyses when assimilating measurements of better quality, mainly over the convective areas.
Fleur Couvreux, Eric Bazile, Guylaine Canut, Yann Seity, Marie Lothon, Fabienne Lohou, Françoise Guichard, and Erik Nilsson
Atmos. Chem. Phys., 16, 8983–9002, https://doi.org/10.5194/acp-16-8983-2016, https://doi.org/10.5194/acp-16-8983-2016, 2016
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This study evaluates the ability of operational models to predict the boundary-layer turbulent processes and mesoscale variability observed during the Boundary Layer Late-Afternoon and Sunset Turbulence field campaign. The models succeed in reproducing the variability from one day to another in terms of cloud cover, temperature and boundary-layer depth. However, they exhibit some systematic biases. The high-resolution model reproduces the vertical structures better.
Hélène Angot, Olivier Magand, Detlev Helmig, Philippe Ricaud, Boris Quennehen, Hubert Gallée, Massimo Del Guasta, Francesca Sprovieri, Nicola Pirrone, Joël Savarino, and Aurélien Dommergue
Atmos. Chem. Phys., 16, 8249–8264, https://doi.org/10.5194/acp-16-8249-2016, https://doi.org/10.5194/acp-16-8249-2016, 2016
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While the Arctic has been extensively monitored, there is still much to be learned from the Antarctic continent regarding the processes that govern the budget of atmospheric mercury species. We report here the first year-round measurements of gaseous elemental mercury (Hg(0)) in the atmosphere and in snowpack interstitial air on the East Antarctic ice sheet. The striking reactivity observed on the Antarctic plateau most likely influences the cycle of atmospheric mercury on a continental scale.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
C. Darbieu, F. Lohou, M. Lothon, J. Vilà-Guerau de Arellano, F. Couvreux, P. Durand, D. Pino, E. G. Patton, E. Nilsson, E. Blay-Carreras, and B. Gioli
Atmos. Chem. Phys., 15, 10071–10086, https://doi.org/10.5194/acp-15-10071-2015, https://doi.org/10.5194/acp-15-10071-2015, 2015
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A case study of the BLLAST experiment is considered to explore the decay of turbulence that occurs in the convective boundary layer over land during the afternoon. Based on observations and on a large-eddy simulation, the analysis reveals two phases in the afternoon: a first quasi-stationary phase when the turbulent kinetic energy slowly decays without significant change in the turbulence structure and a second phase of more rapid decay with a change in spectral turbulence characteristics.
F. Besson, E. Bazile, C. Soci, J.-M. Soubeyroux, G. Ouzeau, and M. Perrin
Adv. Sci. Res., 12, 137–140, https://doi.org/10.5194/asr-12-137-2015, https://doi.org/10.5194/asr-12-137-2015, 2015
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Due to the evolution of the observation network, hourly 2m temperature analysis performed by reanalysis systems shows temporal inhomogeneities. In this study, the diurnal temperature cycle has been reconstructed for stations which only record extreme temperatures to produce new “pseudo” hourly temperature observations. Then they are provided to analysis systems; the results have shown that it enables reducing the bias in temperature analysis.
H. P. Pietersen, J. Vilà-Guerau de Arellano, P. Augustin, A. van de Boer, O. de Coster, H. Delbarre, P. Durand, M. Fourmentin, B. Gioli, O. Hartogensis, F. Lohou, M. Lothon, H. G. Ouwersloot, D. Pino, and J. Reuder
Atmos. Chem. Phys., 15, 4241–4257, https://doi.org/10.5194/acp-15-4241-2015, https://doi.org/10.5194/acp-15-4241-2015, 2015
C. Crevoisier, C. Clerbaux, V. Guidard, T. Phulpin, R. Armante, B. Barret, C. Camy-Peyret, J.-P. Chaboureau, P.-F. Coheur, L. Crépeau, G. Dufour, L. Labonnote, L. Lavanant, J. Hadji-Lazaro, H. Herbin, N. Jacquinet-Husson, S. Payan, E. Péquignot, C. Pierangelo, P. Sellitto, and C. Stubenrauch
Atmos. Meas. Tech., 7, 4367–4385, https://doi.org/10.5194/amt-7-4367-2014, https://doi.org/10.5194/amt-7-4367-2014, 2014
A. T. J. de Laat, I. Aben, M. Deeter, P. Nédélec, H. Eskes, J.-L. Attié, P. Ricaud, R. Abida, L. El Amraoui, and J. Landgraf
Atmos. Meas. Tech., 7, 3783–3799, https://doi.org/10.5194/amt-7-3783-2014, https://doi.org/10.5194/amt-7-3783-2014, 2014
P. Ricaud, B. Sič, L. El Amraoui, J.-L. Attié, R. Zbinden, P. Huszar, S. Szopa, J. Parmentier, N. Jaidan, M. Michou, R. Abida, F. Carminati, D. Hauglustaine, T. August, J. Warner, R. Imasu, N. Saitoh, and V.-H. Peuch
Atmos. Chem. Phys., 14, 11427–11446, https://doi.org/10.5194/acp-14-11427-2014, https://doi.org/10.5194/acp-14-11427-2014, 2014
M. Lothon, F. Lohou, D. Pino, F. Couvreux, E. R. Pardyjak, J. Reuder, J. Vilà-Guerau de Arellano, P Durand, O. Hartogensis, D. Legain, P. Augustin, B. Gioli, D. H. Lenschow, I. Faloona, C. Yagüe, D. C. Alexander, W. M. Angevine, E Bargain, J. Barrié, E. Bazile, Y. Bezombes, E. Blay-Carreras, A. van de Boer, J. L. Boichard, A. Bourdon, A. Butet, B. Campistron, O. de Coster, J. Cuxart, A. Dabas, C. Darbieu, K. Deboudt, H. Delbarre, S. Derrien, P. Flament, M. Fourmentin, A. Garai, F. Gibert, A. Graf, J. Groebner, F. Guichard, M. A. Jiménez, M. Jonassen, A. van den Kroonenberg, V. Magliulo, S. Martin, D. Martinez, L. Mastrorillo, A. F. Moene, F. Molinos, E. Moulin, H. P. Pietersen, B. Piguet, E. Pique, C. Román-Cascón, C. Rufin-Soler, F. Saïd, M. Sastre-Marugán, Y. Seity, G. J. Steeneveld, P. Toscano, O. Traullé, D. Tzanos, S. Wacker, N. Wildmann, and A. Zaldei
Atmos. Chem. Phys., 14, 10931–10960, https://doi.org/10.5194/acp-14-10931-2014, https://doi.org/10.5194/acp-14-10931-2014, 2014
L. El Amraoui, J.-L. Attié, P. Ricaud, W. A. Lahoz, A. Piacentini, V.-H. Peuch, J. X. Warner, R. Abida, J. Barré, and R. Zbinden
Atmos. Meas. Tech., 7, 3035–3057, https://doi.org/10.5194/amt-7-3035-2014, https://doi.org/10.5194/amt-7-3035-2014, 2014
W. M. Angevine, E. Bazile, D. Legain, and D. Pino
Atmos. Chem. Phys., 14, 8165–8172, https://doi.org/10.5194/acp-14-8165-2014, https://doi.org/10.5194/acp-14-8165-2014, 2014
E. Hache, J.-L. Attié, C. Tourneur, P. Ricaud, L. Coret, W. A. Lahoz, L. El Amraoui, B. Josse, P. Hamer, J. Warner, X. Liu, K. Chance, M. Höpfner, R. Spurr, V. Natraj, S. Kulawik, A. Eldering, and J. Orphal
Atmos. Meas. Tech., 7, 2185–2201, https://doi.org/10.5194/amt-7-2185-2014, https://doi.org/10.5194/amt-7-2185-2014, 2014
F. Carminati, P. Ricaud, J.-P. Pommereau, E. Rivière, S. Khaykin, J.-L. Attié, and J. Warner
Atmos. Chem. Phys., 14, 6195–6211, https://doi.org/10.5194/acp-14-6195-2014, https://doi.org/10.5194/acp-14-6195-2014, 2014
R. M. Zbinden, V. Thouret, P. Ricaud, F. Carminati, J.-P. Cammas, and P. Nédélec
Atmos. Chem. Phys., 13, 12363–12388, https://doi.org/10.5194/acp-13-12363-2013, https://doi.org/10.5194/acp-13-12363-2013, 2013
J.-L. Baray, Y. Courcoux, P. Keckhut, T. Portafaix, P. Tulet, J.-P. Cammas, A. Hauchecorne, S. Godin Beekmann, M. De Mazière, C. Hermans, F. Desmet, K. Sellegri, A. Colomb, M. Ramonet, J. Sciare, C. Vuillemin, C. Hoareau, D. Dionisi, V. Duflot, H. Vérèmes, J. Porteneuve, F. Gabarrot, T. Gaudo, J.-M. Metzger, G. Payen, J. Leclair de Bellevue, C. Barthe, F. Posny, P. Ricaud, A. Abchiche, and R. Delmas
Atmos. Meas. Tech., 6, 2865–2877, https://doi.org/10.5194/amt-6-2865-2013, https://doi.org/10.5194/amt-6-2865-2013, 2013
P. Huszar, H. Teyssèdre, M. Michou, A. Voldoire, D. J. L. Olivié, D. Saint-Martin, D. Cariolle, S. Senesi, D. Salas Y Melia, A. Alias, F. Karcher, P. Ricaud, and T. Halenka
Atmos. Chem. Phys., 13, 10027–10048, https://doi.org/10.5194/acp-13-10027-2013, https://doi.org/10.5194/acp-13-10027-2013, 2013
E. Järvinen, A. Virkkula, T. Nieminen, P. P. Aalto, E. Asmi, C. Lanconelli, M. Busetto, A. Lupi, R. Schioppo, V. Vitale, M. Mazzola, T. Petäjä, V.-M. Kerminen, and M. Kulmala
Atmos. Chem. Phys., 13, 7473–7487, https://doi.org/10.5194/acp-13-7473-2013, https://doi.org/10.5194/acp-13-7473-2013, 2013
J. Gazeaux, C. Clerbaux, M. George, J. Hadji-Lazaro, J. Kuttippurath, P.-F. Coheur, D. Hurtmans, T. Deshler, M. Kovilakam, P. Campbell, V. Guidard, F. Rabier, and J.-N. Thépaut
Atmos. Meas. Tech., 6, 613–620, https://doi.org/10.5194/amt-6-613-2013, https://doi.org/10.5194/amt-6-613-2013, 2013
R. Baghi, P. Durand, C. Jambert, C. Jarnot, C. Delon, D. Serça, N. Striebig, M. Ferlicoq, and P. Keravec
Atmos. Meas. Tech., 5, 3119–3132, https://doi.org/10.5194/amt-5-3119-2012, https://doi.org/10.5194/amt-5-3119-2012, 2012
Related subject area
Subject: Clouds and Precipitation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Microphysical view of the development and ice production of mid-latitude stratiform clouds with embedded convection during an extratropical cyclone
Clouds and precipitation in the initial phase of marine cold-air outbreaks as observed by airborne remote sensing
Estimating the snow density using collocated Parsivel and Micro-Rain Radar measurements: a preliminary study from ICE-POP 2017/2018
Technical note: On the ice microphysics of isolated thunderstorms and non-thunderstorms in southern China – a radar polarimetric perspective
Distinctive aerosol–cloud–precipitation interactions in marine boundary layer clouds from the ACE-ENA and SOCRATES aircraft field campaigns
Theoretical Framework for Measuring Cloud Effective Supersaturation Fluctuations with an Advanced Optical System
Drivers of droplet formation in east Mediterranean orographic clouds
Observability of moisture transport divergence in Arctic atmospheric rivers by dropsondes
Elucidating the boundary layer turbulence dissipation rate using high-resolution measurements from a radar wind profiler network over the Tibetan Plateau
Environmental controls on isolated convection during the Amazonian wet season
Isotopic composition of convective rainfall in the inland tropics of Brazil
Measurement report: Cloud and environmental properties associated with aggregated shallow marine cumulus and cumulus congestus
How does riming influence the observed spatial variability of ice water in mixed-phase clouds?
Lifecycle of updrafts and mass flux in isolated deep convection over the Amazon rainforest: insights from cell tracking
Thermodynamic and cloud evolution in a cold-air outbreak during HALO-(AC)3: quasi-Lagrangian observations compared to the ERA5 and CARRA reanalyses
Powering aircraft with 100 % sustainable aviation fuel reduces ice crystals in contrails
Supercooled liquid water clouds observed over Dome C, Antarctica: temperature sensitivity and cloud radiative forcing
Role of thermodynamic and turbulence processes on the fog life cycle during SOFOG3D experiment
Characterizing the near-global cloud vertical structures over land using high-resolution radiosonde measurements
Investigating the role of typhoon-induced gravity waves and stratospheric hydration in the formation of tropopause cirrus clouds observed during the 2017 Asian monsoon
Differences in microphysical properties of cirrus at high and mid-latitudes
Sub-cloud rain evaporation in the North Atlantic winter trade winds derived by pairing isotopic data with a bin-resolved microphysical model
Overview and statistical analysis of boundary layer clouds and precipitation over the western North Atlantic Ocean
A set of methods to evaluate the below-cloud evaporation effect on local precipitation isotopic composition: a case study for Xi'an, China
Earth-system-model evaluation of cloud and precipitation occurrence for supercooled and warm clouds over the Southern Ocean's Macquarie Island
Pollution slightly enhances atmospheric cooling by low-level clouds in tropical West Africa
Investigating an indirect aviation effect on mid-latitude cirrus clouds – linking lidar-derived optical properties to in situ measurements
Investigating the vertical extent and short-wave radiative effects of the ice phase in Arctic summertime low-level clouds
Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer
Aircraft observations of gravity wave activity and turbulence in the tropical tropopause layer: prevalence, influence on cirrus clouds, and comparison with global storm-resolving models
Influence of air mass origin on microphysical properties of low-level clouds in a subarctic environment
Sensitivity of convectively driven tropical tropopause cirrus properties to ice habits in high-resolution simulations
Upper-tropospheric slightly ice-subsaturated regions: frequency of occurrence and statistical evidence for the appearance of contrail cirrus
Examination of aerosol indirect effects during cirrus cloud evolution
In situ microphysics observations of intense pyroconvection from a large wildfire
Conditions favorable for secondary ice production in Arctic mixed-phase clouds
Interaction between cloud–radiation, atmospheric dynamics and thermodynamics based on observational data from GoAmazon 2014/15 and a cloud-resolving model
Snowfall in Northern Finland derives mostly from ice clouds
Observation of secondary ice production in clouds at low temperatures
In situ and satellite-based estimates of cloud properties and aerosol–cloud interactions over the southeast Atlantic Ocean
Ice fog observed at cirrus temperatures at Dome C, Antarctic Plateau
Life cycle of stratocumulus clouds over 1 year at the coast of the Atacama Desert
Experimental study on the evolution of droplet size distribution during the fog life cycle
Significant continental source of ice-nucleating particles at the tip of Chile's southernmost Patagonia region
Retrieving ice-nucleating particle concentration and ice multiplication factors using active remote sensing validated by in situ observations
Temporal and vertical distributions of the occurrence of cirrus clouds over a coastal station in the Indian monsoon region
Continental thunderstorm ground enhancement observed at an exceptionally low altitude
Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions
In situ observation of riming in mixed-phase clouds using the PHIPS probe
Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice-nucleating particles and instrument inter-comparison in the Hyytiälä boreal forest
Yuanmou Du, Dantong Liu, Delong Zhao, Mengyu Huang, Ping Tian, Dian Wen, Wei Xiao, Wei Zhou, Hui He, Baiwan Pan, Dongfei Zuo, Xiange Liu, Yingying Jing, Rong Zhang, Jiujiang Sheng, Fei Wang, Yu Huang, Yunbo Chen, and Deping Ding
Atmos. Chem. Phys., 24, 13429–13444, https://doi.org/10.5194/acp-24-13429-2024, https://doi.org/10.5194/acp-24-13429-2024, 2024
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By conducting in situ measurements, we investigated ice production processes in stratiform clouds with embedded convection over the North China Plain. The results show that the ice number concentration is strongly related to the distance to the cloud top, and the level with a larger distance to the cloud top has more graupel falling from upper levels, which promotes collision and coalescence between graupel and droplets and enhances secondary ice production.
Imke Schirmacher, Sabrina Schnitt, Marcus Klingebiel, Nina Maherndl, Benjamin Kirbus, André Ehrlich, Mario Mech, and Susanne Crewell
Atmos. Chem. Phys., 24, 12823–12842, https://doi.org/10.5194/acp-24-12823-2024, https://doi.org/10.5194/acp-24-12823-2024, 2024
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During Arctic marine cold-air outbreaks, cold air flows from sea ice over open water. Roll circulations evolve, forming cloud streets. We investigate the initial circulation and cloud development using high-resolution airborne measurements. We compute the distance an air mass traveled over water (fetch) from back trajectories. Cloud streets form at 15 km fetch, cloud cover strongly increases at around 20 km, and precipitation forms at around 30 km.
Wei-Yu Chang, Yung-Chuan Yang, Chen-Yu Hung, Kwonil Kim, Gyuwon Lee, and Ali Tokay
Atmos. Chem. Phys., 24, 11955–11979, https://doi.org/10.5194/acp-24-11955-2024, https://doi.org/10.5194/acp-24-11955-2024, 2024
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Snow density is derived by collocated Micro-Rain Radar (MRR) and Parsivel (ICE-POP 2017/2018). We apply the particle size distribution from Parsivel to a T-matrix backscattering simulation and compare with ZHH from MRR. Bulk density and bulk water fractions are derived from comparing simulated and calculated ZHH. Retrieved bulk density is validated by comparing snowfall rate measurements from Pluvio and the Precipitation Imaging Package. Snowfall rate consistency confirms the algorithm.
Chuanhong Zhao, Yijun Zhang, Dong Zheng, Haoran Li, Sai Du, Xueyan Peng, Xiantong Liu, Pengguo Zhao, Jiafeng Zheng, and Juan Shi
Atmos. Chem. Phys., 24, 11637–11651, https://doi.org/10.5194/acp-24-11637-2024, https://doi.org/10.5194/acp-24-11637-2024, 2024
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Understanding lightning activity is important for meteorology and atmospheric chemistry. However, the occurrence of lightning activity in clouds is uncertain. In this study, we quantified the difference between isolated thunderstorms and non-thunderstorms. We showed that lightning activity was more likely to occur with more graupel volume and/or riming. A deeper ZDR column was associated with lightning occurrence. This information can aid in a deeper understanding of lighting physics.
Xiaojian Zheng, Xiquan Dong, Baike Xi, Timothy Logan, and Yuan Wang
Atmos. Chem. Phys., 24, 10323–10347, https://doi.org/10.5194/acp-24-10323-2024, https://doi.org/10.5194/acp-24-10323-2024, 2024
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The marine boundary layer aerosol–cloud interactions (ACIs) are examined using in situ measurements from two aircraft campaigns over the eastern North Atlantic (ACE-ENA) and Southern Ocean (SOCRATES). The SOCRATES clouds have more and smaller cloud droplets. The ACE-ENA clouds exhibit stronger drizzle formation and growth. Results found distinctive aerosol–cloud interactions for two campaigns. The drizzle processes significantly alter sub-cloud aerosol budgets and impact the ACI assessments.
Ye Kuang, Jiangchuan Tao, Hanbin Xu, Li Liu, Pengfei Liu, Wanyun Xu, Weiqi Xu, Yele Sun, and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-2698, https://doi.org/10.5194/egusphere-2024-2698, 2024
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This study presents a novel optical framework to measure supersaturation, a fundamental parameter in cloud physics, by observing the scattering properties of particles that have or have not grown into cloud droplets. The technique offers high-resolution measurements, capturing essential fluctuations in supersaturation necessary for understanding cloud physics.
Romanos Foskinis, Ghislain Motos, Maria I. Gini, Olga Zografou, Kunfeng Gao, Stergios Vratolis, Konstantinos Granakis, Ville Vakkari, Kalliopi Violaki, Andreas Aktypis, Christos Kaltsonoudis, Zongbo Shi, Mika Komppula, Spyros N. Pandis, Konstantinos Eleftheriadis, Alexandros Papayannis, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9827–9842, https://doi.org/10.5194/acp-24-9827-2024, https://doi.org/10.5194/acp-24-9827-2024, 2024
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Analysis of modeling, in situ, and remote sensing measurements reveals the microphysical state of orographic clouds and their response to aerosol from the boundary layer and free troposphere. We show that cloud response to aerosol is robust, as predicted supersaturation and cloud droplet number levels agree with those determined from in-cloud measurements. The ability to determine if clouds are velocity- or aerosol-limited allows for novel model constraints and remote sensing products.
Henning Dorff, Heike Konow, Vera Schemann, and Felix Ament
Atmos. Chem. Phys., 24, 8771–8795, https://doi.org/10.5194/acp-24-8771-2024, https://doi.org/10.5194/acp-24-8771-2024, 2024
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Using synthetic dropsondes, we assess how discrete spatial sampling and temporal evolution during flight affect the accuracy of real sonde-based moisture transport divergence in Arctic atmospheric rivers (ARs). Non-instantaneous sampling during temporal AR evolution deteriorates the divergence values more than spatial undersampling. Moisture advection is the dominating factor but most sensitive to the sampling method. We suggest a minimum of seven sondes to resolve the AR divergence components.
Deli Meng, Jianping Guo, Xiaoran Guo, Yinjun Wang, Ning Li, Yuping Sun, Zhen Zhang, Na Tang, Haoran Li, Fan Zhang, Bing Tong, Hui Xu, and Tianmeng Chen
Atmos. Chem. Phys., 24, 8703–8720, https://doi.org/10.5194/acp-24-8703-2024, https://doi.org/10.5194/acp-24-8703-2024, 2024
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The turbulence in the planetary boundary layer (PBL) over the Tibetan Plateau (TP) remains unclear. Here we elucidate the vertical profile of and temporal variation in the turbulence dissipation rate in the PBL over the TP based on a radar wind profiler (RWP) network. To the best of our knowledge, this is the first time that the turbulence profile over the whole TP has been revealed. Furthermore, the possible mechanisms of clouds acting on the PBL turbulence structure are investigated.
Leandro Alex Moreira Viscardi, Giuseppe Torri, David K. Adams, and Henrique de Melo Jorge Barbosa
Atmos. Chem. Phys., 24, 8529–8548, https://doi.org/10.5194/acp-24-8529-2024, https://doi.org/10.5194/acp-24-8529-2024, 2024
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We evaluate the environmental conditions that control how clouds grow from fair weather cumulus into severe thunderstorms during the Amazonian wet season. Days with rain clouds begin with more moisture in the air and have strong convergence in the afternoon, while precipitation intensity increases with large-scale vertical velocity, moisture, and low-level wind. These results contribute to understanding how clouds form over the rainforest.
Vinicius dos Santos, Didier Gastmans, Ana María Durán-Quesada, Ricardo Sánchez-Murillo, Kazimierz Rozanski, Oliver Kracht, and Demilson de Assis Quintão
Atmos. Chem. Phys., 24, 6663–6680, https://doi.org/10.5194/acp-24-6663-2024, https://doi.org/10.5194/acp-24-6663-2024, 2024
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We present novel findings on convective rainfall, summer rain in the late afternoon, by coupling water stable isotopes, micro rain radar, and satellite data. We found the tallest clouds in the afternoon and much smaller clouds at night, resulting in differences in day–night ratios in water stable isotopes. We sampled rain and meteorological variables every 5–10 min, allowing us to evaluate the development of convective rainfall, contributing to knowledge of rainfall related to extreme events.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
Atmos. Chem. Phys., 24, 6123–6152, https://doi.org/10.5194/acp-24-6123-2024, https://doi.org/10.5194/acp-24-6123-2024, 2024
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Marine clouds are found to clump together in regions or lines, readily discernible from satellite images of the ocean. While clustering is also a feature of deep storm clouds, we focus on smaller cloud systems associated with fair weather and brief localized showers. Two aircraft sampled the region around these shallow systems: one incorporated measurements taken within, adjacent to, and below the clouds, while the other provided a survey from above using remote sensing techniques.
Nina Maherndl, Manuel Moser, Imke Schirmacher, Aaron Bansemer, Johannes Lucke, Christiane Voigt, and Maximilian Maahn
EGUsphere, https://doi.org/10.5194/egusphere-2024-1214, https://doi.org/10.5194/egusphere-2024-1214, 2024
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It is not clear, why ice crystals in clouds occur in clusters. Here, airborne measurements of clouds in mid- and high-latitudes are used to study the spatial variability of ice. Further, we investigate the influence of riming, which occurs when liquid droplets freeze onto ice crystals. We find that riming enhances the occurrence of ice clusters. In the Arctic, riming leads to ice clustering at spatial scales of 3–5 km. This is due to updrafts, not necessary higher amounts of liquid water.
Siddhant Gupta, Dié Wang, Scott E. Giangrande, Thiago S. Biscaro, and Michael P. Jensen
Atmos. Chem. Phys., 24, 4487–4510, https://doi.org/10.5194/acp-24-4487-2024, https://doi.org/10.5194/acp-24-4487-2024, 2024
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We examine the lifecycle of isolated deep convective clouds (DCCs) in the Amazon rainforest. Weather radar echoes from the DCCs are tracked to evaluate their lifecycle. The DCC size and intensity increase, reach a peak, and then decrease over the DCC lifetime. Vertical profiles of air motion and mass transport from different seasons are examined to understand the transport of energy and momentum within DCC cores and to address the deficiencies in simulating DCCs using weather and climate models.
Benjamin Kirbus, Imke Schirmacher, Marcus Klingebiel, Michael Schäfer, André Ehrlich, Nils Slättberg, Johannes Lucke, Manuel Moser, Hanno Müller, and Manfred Wendisch
Atmos. Chem. Phys., 24, 3883–3904, https://doi.org/10.5194/acp-24-3883-2024, https://doi.org/10.5194/acp-24-3883-2024, 2024
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A research aircraft is used to track the changes in air temperature, moisture, and cloud properties for air that moves from cold Arctic sea ice onto warmer oceanic waters. The measurements are compared to two reanalysis models named ERA5 and CARRA. The biggest differences are found for air temperature over the sea ice and moisture over the ocean. CARRA data are more accurate than ERA5 because they better simulate the sea ice, the transition from sea ice to open ocean, and the forming clouds.
Raphael Satoru Märkl, Christiane Voigt, Daniel Sauer, Rebecca Katharina Dischl, Stefan Kaufmann, Theresa Harlaß, Valerian Hahn, Anke Roiger, Cornelius Weiß-Rehm, Ulrike Burkhardt, Ulrich Schumann, Andreas Marsing, Monika Scheibe, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Reetu Sallinen, Tobias Schripp, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 3813–3837, https://doi.org/10.5194/acp-24-3813-2024, https://doi.org/10.5194/acp-24-3813-2024, 2024
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In situ measurements of contrails from a large passenger aircraft burning 100 % sustainable aviation fuel (SAF) show a 56 % reduction in contrail ice crystal numbers compared to conventional Jet A-1. Results from a climate model initialized with the observations suggest a significant decrease in radiative forcing from contrails. Our study confirms that future increased use of low aromatic SAF can reduce the climate impact from aviation.
Philippe Ricaud, Massimo Del Guasta, Angelo Lupi, Romain Roehrig, Eric Bazile, Pierre Durand, Jean-Luc Attié, Alessia Nicosia, and Paolo Grigioni
Atmos. Chem. Phys., 24, 613–630, https://doi.org/10.5194/acp-24-613-2024, https://doi.org/10.5194/acp-24-613-2024, 2024
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Clouds affect the Earth's climate in ways that depend on the type of cloud (solid/liquid water). From observations at Concordia (Antarctica), we show that in supercooled liquid water (liquid water for temperatures below 0°C) clouds (SLWCs), temperature and SLWC radiative forcing increase with liquid water (up to 70 W m−2). We extrapolated that the maximum SLWC radiative forcing can reach 40 W m−2 over the Antarctic Peninsula, highlighting the importance of SLWCs for global climate prediction.
Cheikh Dione, Martial Haeffelin, Frédéric Burnet, Christine Lac, Guylaine Canut, Julien Delanoë, Jean-Charles Dupont, Susana Jorquera, Pauline Martinet, Jean-François Ribaud, and Felipe Toledo
Atmos. Chem. Phys., 23, 15711–15731, https://doi.org/10.5194/acp-23-15711-2023, https://doi.org/10.5194/acp-23-15711-2023, 2023
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This paper documents the role of thermodynamics and turbulence in the fog life cycle over southwestern France. It is based on a unique dataset collected during the SOFOG3D field campaign in autumn and winter 2019–2020. The paper gives a threshold for turbulence driving the different phases of the fog life cycle and the role of advection in the night-time dissipation of fog. The results can be operationalised to nowcast fog and improve short-range forecasts in numerical weather prediction models.
Hui Xu, Jianping Guo, Bing Tong, Jinqiang Zhang, Tianmeng Chen, Xiaoran Guo, Jian Zhang, and Wenqing Chen
Atmos. Chem. Phys., 23, 15011–15038, https://doi.org/10.5194/acp-23-15011-2023, https://doi.org/10.5194/acp-23-15011-2023, 2023
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The radiative effect of cloud remains one of the largest uncertain factors in climate change, largely due to the lack of cloud vertical structure (CVS) observations. The study presents the first near-global CVS climatology using high-vertical-resolution soundings. Single-layer cloud mainly occurs over arid regions. As the number of cloud layers increases, clouds tend to have lower bases and thinner layer thicknesses. The occurrence frequency of cloud exhibits a pronounced seasonal diurnal cycle.
Amit Kumar Pandit, Jean-Paul Vernier, Thomas Duncan Fairlie, Kristopher M. Bedka, Melody A. Avery, Harish Gadhavi, Madineni Venkat Ratnam, Sanjeev Dwivedi, Kasimahanthi Amar Jyothi, Frank G. Wienhold, Holger Vömel, Hongyu Liu, Bo Zhang, Buduru Suneel Kumar, Tra Dinh, and Achuthan Jayaraman
EGUsphere, https://doi.org/10.5194/egusphere-2023-2236, https://doi.org/10.5194/egusphere-2023-2236, 2023
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This study investigates the formation mechanism of a tropopause cirrus cloud layer observed at extremely cold temperatures over Hyderabad in India during the 2017 Asian summer monsoon using balloon-borne sensors. Ice crystals smaller than 50 microns were found in this optically thin cirrus cloud layer. Combined analysis of back-trajectories, satellite, and model data revealed that the formation of this layer was influenced by gravity waves and stratospheric hydration induced by typhoon Hato.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
Atmos. Chem. Phys., 23, 13167–13189, https://doi.org/10.5194/acp-23-13167-2023, https://doi.org/10.5194/acp-23-13167-2023, 2023
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In this study, we show the differences in the microphysical properties between high-latitude (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region on cloud formation. We show that HL cirrus are characterized by a lower concentration of larger ice crystals when compared to ML cirrus.
Mampi Sarkar, Adriana Bailey, Peter Blossey, Simon P. de Szoeke, David Noone, Estefanía Quiñones Meléndez, Mason D. Leandro, and Patrick Y. Chuang
Atmos. Chem. Phys., 23, 12671–12690, https://doi.org/10.5194/acp-23-12671-2023, https://doi.org/10.5194/acp-23-12671-2023, 2023
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We study rain evaporation characteristics below shallow cumulus clouds over the North Atlantic Ocean by pairing isotope observations with a microphysical model. The modeled fraction of rain mass that evaporates below the cloud strongly depends on the raindrop size and distribution width. Moreover, the higher the rain mass fraction evaporated, the greater the change in deuterium excess. In this way, rain evaporation could be studied independently using only isotope and microphysical observations.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Meng Xing, Weiguo Liu, Jing Hu, and Zheng Wang
Atmos. Chem. Phys., 23, 9123–9136, https://doi.org/10.5194/acp-23-9123-2023, https://doi.org/10.5194/acp-23-9123-2023, 2023
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The below-cloud evaporation effect (BCE) on precipitation largely impacts the final isotopic composition. However, determining the BCE effect remains poorly constrained. Our work used a ΔdΔδ diagram to differentiate the below-cloud processes. Moreover, by comparing two different computing methods, we considered that both methods are suitable for evaluation the BCE, except for snowfall events. Overall, our work compiled a set of effective methods to evaluate the BCE effect.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
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Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
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The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Rachel Atlas and Christopher S. Bretherton
Atmos. Chem. Phys., 23, 4009–4030, https://doi.org/10.5194/acp-23-4009-2023, https://doi.org/10.5194/acp-23-4009-2023, 2023
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The tropical tropopause layer exists between the troposphere and the stratosphere in the tropics. Very thin cirrus clouds cool Earth's surface by scrubbing water vapor (a greenhouse gas) out of air parcels as they ascend through the tropical tropopause layer on their way to the stratosphere. We show observational evidence from aircraft that small-scale (< 100 km) gravity waves and turbulence increase the amount of ice in these clouds and may allow them to remove more water vapor from the air.
Konstantinos Matthaios Doulgeris, Ville Vakkari, Ewan J. O'Connor, Veli-Matti Kerminen, Heikki Lihavainen, and David Brus
Atmos. Chem. Phys., 23, 2483–2498, https://doi.org/10.5194/acp-23-2483-2023, https://doi.org/10.5194/acp-23-2483-2023, 2023
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We investigated how different long-range-transported air masses can affect the microphysical properties of low-level clouds in a clean subarctic environment. A connection was revealed. Higher values of cloud droplet number concentrations were related to continental air masses, whereas the lowest values of number concentrations were related to marine air masses. These were characterized by larger cloud droplets. Clouds in all regions were sensitive to increases in cloud number concentration.
Fayçal Lamraoui, Martina Krämer, Armin Afchine, Adam B. Sokol, Sergey Khaykin, Apoorva Pandey, and Zhiming Kuang
Atmos. Chem. Phys., 23, 2393–2419, https://doi.org/10.5194/acp-23-2393-2023, https://doi.org/10.5194/acp-23-2393-2023, 2023
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Cirrus in the tropical tropopause layer (TTL) can play a key role in vertical transport. We investigate the role of different cloud regimes and the associated ice habits in regulating the properties of the TTL. We use high-resolution numerical experiments at the scales of large-eddy simulations (LESs) and aircraft measurements. We found that LES-scale parameterizations that predict ice shape are crucial for an accurate representation of TTL cirrus and thus the associated (de)hydration process.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Flor Vanessa Maciel, Minghui Diao, and Ryan Patnaude
Atmos. Chem. Phys., 23, 1103–1129, https://doi.org/10.5194/acp-23-1103-2023, https://doi.org/10.5194/acp-23-1103-2023, 2023
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Aerosol indirect effects on cirrus clouds are investigated during cirrus evolution, using global-scale in situ observations and climate model simulations. As cirrus evolves, the mechanisms to form ice crystals also change with time. Both small and large aerosols are found to affect cirrus properties. Southern Hemisphere cirrus appears to be more sensitive to additional aerosols. The climate model underestimates ice crystal mass, likely due to biases of relative humidity and vertical velocity.
David E. Kingsmill, Jeffrey R. French, and Neil P. Lareau
Atmos. Chem. Phys., 23, 1–21, https://doi.org/10.5194/acp-23-1-2023, https://doi.org/10.5194/acp-23-1-2023, 2023
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This study uses in situ aircraft measurements to characterize the size and shape distributions of 10 µm to 6 mm diameter particles observed during six penetrations of wildfire-induced pyroconvection. Particles sampled in one penetration of a smoke plume are most likely pyrometeors composed of ash. The other penetrations are through pyrocumulus clouds where particle composition is most likely a combination of hydrometeors (ice particles) and pyrometeors (ash).
Julie Thérèse Pasquier, Jan Henneberger, Fabiola Ramelli, Annika Lauber, Robert Oscar David, Jörg Wieder, Tim Carlsen, Rosa Gierens, Marion Maturilli, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 15579–15601, https://doi.org/10.5194/acp-22-15579-2022, https://doi.org/10.5194/acp-22-15579-2022, 2022
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It is important to understand how ice crystals and cloud droplets form in clouds, as their concentrations and sizes determine the exact radiative properties of the clouds. Normally, ice crystals form from aerosols, but we found evidence for the formation of additional ice crystals from the original ones over a large temperature range within Arctic clouds. In particular, additional ice crystals were formed during collisions of several ice crystals or during the freezing of large cloud droplets.
Layrson J. M. Gonçalves, Simone M. S. C. Coelho, Paulo Y. Kubota, and Dayana C. Souza
Atmos. Chem. Phys., 22, 15509–15526, https://doi.org/10.5194/acp-22-15509-2022, https://doi.org/10.5194/acp-22-15509-2022, 2022
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This research aims to study the environmental conditions that are favorable and not favorable to cloud formation, in this case specifically for the Amazon region. The results found in this research will be used to improve the representation of clouds in numerical models that are used in weather and climate prediction. In general, it is expected that with better knowledge regarding the cloud–radiation interaction, it is possible to make a better forecast of weather and climate.
Claudia Mignani, Lukas Zimmermann, Rigel Kivi, Alexis Berne, and Franz Conen
Atmos. Chem. Phys., 22, 13551–13568, https://doi.org/10.5194/acp-22-13551-2022, https://doi.org/10.5194/acp-22-13551-2022, 2022
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We determined over the course of 8 winter months the phase of clouds associated with snowfall in Northern Finland using radiosondes and observations of ice particle habits at ground level. We found that precipitating clouds were extending from near ground to at least 2.7 km altitude and approximately three-quarters of them were likely glaciated. Possible moisture sources and ice formation processes are discussed.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
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The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Étienne Vignon, Lea Raillard, Christophe Genthon, Massimo Del Guasta, Andrew J. Heymsfield, Jean-Baptiste Madeleine, and Alexis Berne
Atmos. Chem. Phys., 22, 12857–12872, https://doi.org/10.5194/acp-22-12857-2022, https://doi.org/10.5194/acp-22-12857-2022, 2022
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The near-surface atmosphere over the Antarctic Plateau is cold and pristine and resembles to a certain extent the high troposphere where cirrus clouds form. In this study, we use innovative humidity measurements at Concordia Station to study the formation of ice fogs at temperatures <−40°C. We provide observational evidence that ice fogs can form through the homogeneous freezing of solution aerosols, a common nucleation pathway for cirrus clouds.
Jan H. Schween, Camilo del Rio, Juan-Luis García, Pablo Osses, Sarah Westbrook, and Ulrich Löhnert
Atmos. Chem. Phys., 22, 12241–12267, https://doi.org/10.5194/acp-22-12241-2022, https://doi.org/10.5194/acp-22-12241-2022, 2022
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Marine stratocumulus clouds of the eastern Pacific play an essential role in the Earth's climate. These clouds form the major source of water to parts of the extreme dry Atacama Desert at the northern coast of Chile. For the first time these clouds are observed over a whole year with three remote sensing instruments. It is shown how these clouds are influenced by the land–sea wind system and the distribution of ocean temperatures.
Marie Mazoyer, Frédéric Burnet, and Cyrielle Denjean
Atmos. Chem. Phys., 22, 11305–11321, https://doi.org/10.5194/acp-22-11305-2022, https://doi.org/10.5194/acp-22-11305-2022, 2022
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The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
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Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Saleem Ali, Sanjay Kumar Mehta, Aravindhavel Ananthavel, and Tondapu Venkata Ramesh Reddy
Atmos. Chem. Phys., 22, 8321–8342, https://doi.org/10.5194/acp-22-8321-2022, https://doi.org/10.5194/acp-22-8321-2022, 2022
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Multiple cirrus clouds frequently occur over regions of deep convection in the tropics. Tropical convection has a strong diurnal pattern, with peaks in the afternoon to early evening, over the continents. Continuous micropulse lidar observations over a coastal station in the Indian monsoon region enable us, for the first time, to demonstrate a robust diurnal pattern of single and multiple cirrus occurrences, with peaks during the late afternoon and early morning hours, respectively.
Ivana Kolmašová, Ondřej Santolík, Jakub Šlegl, Jana Popová, Zbyněk Sokol, Petr Zacharov, Ondřej Ploc, Gerhard Diendorfer, Ronald Langer, Radek Lán, and Igor Strhárský
Atmos. Chem. Phys., 22, 7959–7973, https://doi.org/10.5194/acp-22-7959-2022, https://doi.org/10.5194/acp-22-7959-2022, 2022
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Gamma ray radiation related to thunderstorms was previously observed at the high-altitude mountain observatories or on the western coast of Japan, usually being terminated by lightning discharges. We show unusual observations of gamma rays at an altitude below 1000 m, coinciding with peculiar rapid variations in the vertical electric field, which are linked to inverted intracloud lightning discharges. This indicates that a strong, lower positive-charge region was present inside the thundercloud.
Cuiqi Zhang, Zhijun Wu, Jingchuan Chen, Jie Chen, Lizi Tang, Wenfei Zhu, Xiangyu Pei, Shiyi Chen, Ping Tian, Song Guo, Limin Zeng, Min Hu, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7539–7556, https://doi.org/10.5194/acp-22-7539-2022, https://doi.org/10.5194/acp-22-7539-2022, 2022
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The immersion ice nucleation effectiveness of aerosols from multiple sources in the urban environment remains elusive. In this study, we demonstrate that the immersion ice-nucleating particle (INP) concentration increased dramatically during a dust event in an urban atmosphere. Pollutant aerosols, including inorganic salts formed through secondary transformation (SIA) and black carbon (BC), might not act as effective INPs under mixed-phase cloud conditions.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Chem. Phys., 22, 7087–7103, https://doi.org/10.5194/acp-22-7087-2022, https://doi.org/10.5194/acp-22-7087-2022, 2022
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Riming, i.e., the accretion of small droplets on the surface of ice particles via collision, is one of the major uncertainties in model prediction of mixed-phase clouds. We discuss the occurrence (up to 50% of particles) and aging of rimed ice particles and show correlations of the occurrence and the degree of riming with ambient meteorological parameters using data gathered by the Particle Habit Imaging and Polar Scattering (PHIPS) probe during three airborne in situ field campaigns.
Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 5117–5145, https://doi.org/10.5194/acp-22-5117-2022, https://doi.org/10.5194/acp-22-5117-2022, 2022
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The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
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Short summary
Thin (~ 100 m) supercooled liquid water (SLW, water staying in liquid phase below 0 °C) clouds have been detected, analysed, and modelled over the Dome C (Concordia, Antarctica) station during the austral summer 2018–2019 using observations and meteorological analyses. The SLW clouds were observed at the top of the planetary boundary layer and the SLW content was always strongly underestimated by the model indicating an incorrect simulation of the surface energy budget of the Antarctic Plateau.
Thin (~ 100 m) supercooled liquid water (SLW, water staying in liquid phase below 0 °C)...
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